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185 results on '"Liao, Qiaogan"'

11. Efficient Ternary Organic Solar Cells with Suppressed Nonradiative Recombination and Fine‐Tuned Morphology via IT‐4F as Guest Acceptor.

Author

Zhang, Yang, Huang, Tianhuan, Weng, Nan, Chen, Yiwen, Wang, Dongjie, Zhang, Zheling, Liao, Qiaogan, and Zhang, Jian

Subjects
ENERGY levels (Quantum mechanics), ENERGY dissipation, OPEN-circuit voltage, SOLAR cells, MORPHOLOGY
Abstract

The large open circuit voltage (VOC) loss is currently one of the main obstacles to achieving efficient organic solar cells (OSCs). In this study, the ternary OSCs comprising PM6:BTP‐eC9:IT‐4F demonstrate a superior efficiency of 18.2 %. Notably, the utilization of the medium bandgap acceptor IT‐4F as the third component results in an exceptionally low nonradiative recombination energy loss of 0.28 V. The desirable energy level cascade is formed among PM6, BTP‐eC9, and IT‐4F due to the low‐lying HOMO and LUMO energy levels of IT‐4F. More importantly, the VOC of PM6:BTP‐eC9:IT‐4F OSCs can reach as high as 0.86 V, which is higher than both binary OSCs without sacrificing JSC and FF. Besides, this strategy proved that IT‐4F can not only broaden the absorption range but also work as a morphology modifier in PM6:BTP‐eC9:IT‐4F OSCs, and there also exists efficient energy transfer between BTP‐eC9 and IT‐4F. This result provides a promising way to suppress the nonradiative recombination energy loss and realize higher VOC than the two binary OSCs in ternary OSCs to obtain high power conversion efficiencies. [ABSTRACT FROM AUTHOR]

Published
2024
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12. Simultaneous realization of bulk and interface regulation based on 2,4-diamino-6,7-diisopropylpteridine phosphate for efficient and stable inverted perovskite solar cells

Author

He, Zhen, primary, Xiong, Jian, additional, Zhang, Yongsong, additional, Liu, Fu, additional, Liu, Naihe, additional, Dai, Junqian, additional, Liang, Yongchao, additional, Zhang, Zheling, additional, Wang, Dongjie, additional, Huang, Yu, additional, Liao, Qiaogan, additional, Wang, Jiang, additional, and Zhang, Jian, additional

Published
2024
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13. Multi-functional thermal management for efficient and stable inverted perovskite solar cells

Author

Zhang, yong song, primary, He, Zhen, additional, Xiong, Jian, additional, Zhan, Shiping, additional, Liu, Fu, additional, Su, Meng, additional, Wang, Dongjie, additional, Huang, Yu, additional, Liao, Qiaogan, additional, Lu, Jiang-rong, additional, Zhang, Zheling, additional, Yuan, Changlai, additional, Wang, Jiang, additional, Dai, Qilin, additional, and Zhang, Jian, additional

Published
2024
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15. Target Therapy for Buried Interface Enables Stable Perovskite Solar Cells with 25.05% Efficiency

Author

Ji, Xiaofei, primary, Bi, Leyu, additional, Fu, Qiang, additional, Li, Bolin, additional, Wang, Junwei, additional, Jeong, Sang Young, additional, Feng, Kui, additional, Ma, Suxiang, additional, Liao, Qiaogan, additional, Lin, Francis R., additional, Woo, Han Young, additional, Lu, Linfeng, additional, Jen, Alex K.‐Y., additional, and Guo, Xugang, additional

Published
2023
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17. Dopant‐Free Polymeric Hole Transport Materials with a DA'D–A Backbone for Efficient and Stable Inverted Perovskite Solar Cells.

Author

Li, Bolin, Yang, Jie, Liao, Qiaogan, Ji, Xiaofei, Wang, Yimei, Yang, Jin, Liu, Bin, Liang, Qiming, Wang, Zhaojin, Li, Henan, Wang, Kai, Sun, Huiliang, Niu, Li, and Guo, Xugang

Subjects
SOLAR cells, FRONTIER orbitals, SPINE, PEROVSKITE
Abstract

Dopant‐free hole transport layers (HTLs) play a crucial role in achieving high‐efficiency and stable perovskite solar cells (PSCs). However, only a limited number of these HTLs have demonstrated power conversion efficiencies (PCEs) surpassing 21%. Herein, the design and synthesis of two polymeric HTLs with a novel DA'D–A backbone are presented. The incorporation of two A units (benzothiazole and imide functionalized aromatics) in the polymer imparts a rigid backbone, high mobility, appropriate film morphology, excellent thermal stability, and a deeper highest occupied molecular orbital energy level, crucial for achieving a more suitable energy‐level alignment between HTL and perovskite layer. Notably, the champion PSC based on our HTLs exhibits a remarkable PCE of 22.02% with minimal hysteresis and excellent thermal stability, surpassing the performance of devices based on the benchmark polymeric HTL PTAA under identical conditions. These findings underscore the immense potential of our DA'D‐A backbone strategy in developing high‐performance dopant‐free polymer HTLs for enhancing the PCE of PSCs. [ABSTRACT FROM AUTHOR]

Published
2024
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21. 18.73% efficiency organic solar cells with a medium bandgap acceptor as a third component.

Author

Zhang, Zheling, Zhang, Yang, Deng, Zhenqi, Huang, Tianhuan, Wang, Dongjie, Zhang, Xiaoling, Liao, Qiaogan, and Zhang, Jian

Abstract

To improve the photovoltaic performance of organic solar cells (OSCs), it is important to optimize all relevant parameters. However, it is challenging work to select suitable semiconductors for constructing a desirable active blend film with realizable device performance. In this study, we used an effective methodology to enhance the photovoltaic performance of OSCs by adding a third component (IT-M) with a medium bandgap. The addition of IT-M improved the blend film morphology, which helped to enhance light absorption and exciton dissociation as well as suppress charge recombination. The compatibility between IT-M and BTP-eC9 was found to be satisfactory, resulting in optimized phase separation and cascaded energy level alignment between the two acceptors. This in turn facilitated balanced charge transport. Additionally, a small amount of IT-M was found to be sufficient to achieve desirable blend film phase separation and molecular stacking, which is advantageous in forming interconnected and continuous network structures. As a result, the optimized OSCs achieved an impressive power conversion efficiency of 18.73% and all-around improved photovoltaic performance parameters. This study demonstrates an effective approach to improve the device performance of OSCs by introducing a suitable second acceptor. [ABSTRACT FROM AUTHOR]

Published
2023
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23. Terminal Cyano-Functionalized Fused Bithiophene Imide Dimer-Based n-Type Small Molecular Semiconductors: Synthesis, Structure–Property Correlations, and Thermoelectric Performances

Author

Wang, Dong, primary, Li, Jianfeng, additional, Yang, Kun, additional, Wang, Yimei, additional, Jeong, Sang Young, additional, Chen, Zhicai, additional, Liao, Qiaogan, additional, Li, Bangbang, additional, Woo, Han Young, additional, Deng, Xianyu, additional, and Guo, Xugang, additional

Published
2023
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24. Thermally Crosslinked Hole Conductor Enables Stable Inverted Perovskite Solar Cells with 23.9% Efficiency

Author

Zhang, Cuiping, primary, Liao, Qiaogan, additional, Chen, Jinyu, additional, Li, Bolin, additional, Xu, Chaoying, additional, Wei, Kun, additional, Du, Guozheng, additional, Wang, Yang, additional, Liu, Dachang, additional, Deng, Jidong, additional, Luo, Zhide, additional, Pang, Shuping, additional, Yang, Ye, additional, Li, Jingrui, additional, Yang, Li, additional, Guo, Xugang, additional, and Zhang, Jinbao, additional

Published
2023
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29. Intramolecular Noncovalent Interaction‐Enabled Dopant‐Free Hole‐Transporting Materials for High‐Performance Inverted Perovskite Solar Cells

Author

Yang, Kun, primary, Liao, Qiaogan, additional, Huang, Jun, additional, Zhang, Zilong, additional, Su, Mengyao, additional, Chen, Zhicai, additional, Wu, Ziang, additional, Wang, Dong, additional, Lai, Ziwei, additional, Woo, Han Young, additional, Cao, Yan, additional, Gao, Peng, additional, and Guo, Xugang, additional

Published
2021
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30. Isomeric Dithienothiophene‐Based Hole Transport Materials: Role of Sulphur Atoms Positions on Photovoltaic Performance of Inverted Perovskite Solar Cells.

Author

Yang, Jie, Huang, Jiachen, Zhang, Chao, Sun, Huiliang, Li, Bolin, Wang, Yimei, Feng, Kui, Liao, Qiaogan, Bai, Qingqing, Niu, Li, Wang, Hua, and Guo, Xugang

Subjects
SOLAR cells, PEROVSKITE, X-ray photoelectron spectroscopy, SULFUR, ATOMS
Abstract

Hole transport materials (HTMs) are of great significance to improve the efficiency and long‐term stability of perovskite solar cells (PVSCs). Herein, a series of new HTMs based on isomeric dithienothiophene (DTT) are designed and synthesized. Effects of sulphur (S) atoms positions on defect passivation and performance of PVSCs are systematically investigated through theoretical computation, X‐ray diffraction, X‐ray photoelectron spectroscopy, etc. The three molecules display noticeable isomeric effect in energy level, light absorption, and hole mobility. With S atoms varied from bottom‐bottom‐bottom in 3T‐1 to bottom‐bottom‐top in 3T‐2, then to bottom‐top‐bottom in 3T‐3, the grown perovskite crystallite on the corresponding HTMs shows more homeogenous film morphology and less pinhole traps. Meanwhile, nonradiative recombination losses can be suppressed and hole extraction efficiency at HTM/perovskite surface can be improved from 3T‐1 to 3T‐3. As a result, the remarkable improvement of short‐circuit current density nd open‐circuit voltage in inverted perovskite solar cells can be realized with increasing the sulphur atoms contribution to the molecular conjugation. More importantly, 3T‐3‐based dopant‐free HTM achieves a top power conversion efficiency of 19.23% in PVSCs with good device stability under green solvent processing. These results demonstrate the role of S atoms positions in HTMs on photovoltaic performance of PVSCs and the potential of DTT in developing eco‐friendly HTMs toward efficient PVSCs. [ABSTRACT FROM AUTHOR]

Published
2022
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31. A Cost-Effective D-A-D Type Hole-Transport Material Enabling 20% Efficiency Inverted Perovskite Solar Cells

Author

Huang, Jiachen, Yang, Jie, Sun, Huiliang, Feng, Kui, Liao, Qiaogan, Li, Bolin, Yan, He, Guo, Xugang, Huang, Jiachen, Yang, Jie, Sun, Huiliang, Feng, Kui, Liao, Qiaogan, Li, Bolin, Yan, He, and Guo, Xugang

Abstract

High-performance, cost-effective hole-transport materials (HTMs) are greatly desired for the commercialization of perovskite solar cells (PVSCs). Herein, two new HTMs, TPA-FO and TPA-PDO, are devised and synthesized, which have a donor-acceptor-donor (D-A-D) type molecule design featuring carbonyl group-functionalized arenes as the acceptor (A) units. The carbonyl group at the central core of HTMs can not only tune frontier molecular orbital (FMO) energy levels and surface wettability, but also can enable efficient surface passivation effects, resulting in reduced recombination loss. When employed as HTMs in inverted PVSCs without using dopant, TPA-FO with one carbonyl group yields a high power conversion efficiency (PCE) of 20.24%, which is among the highest values reported in the inverted PVSCs with dopant-free HTMs. More importantly, the facile one-step synthetic process enables a low cost of 30 USD g–1 for TPA-FO, much cheaper than the most studied HTMs used for high-efficiency dopant-free PVSCs. These results demonstrate the potential of D-A-D type molecules with carbonyl group-functionalized arene core in developing the low-cost dopant-free HTMs toward highly efficient PVSCs.

Published
2021

35. Two Compatible Polymer Donors Enabling Ternary Organic Solar Cells with a Small Nonradiative Energy Loss and Broad Composition Tolerance

Author

Tang, Yumin, Yu, Jianwei, Sun, Huiliang, Wu, Ziang, Koh, Chang Woo, Wu, Xia, Liu, Bin, Wang, Junwei, Liao, Qiaogan, Li, Yongchun, Guo, Han, Woo, Han Young, Gao, Feng, Guo, Xugang, Tang, Yumin, Yu, Jianwei, Sun, Huiliang, Wu, Ziang, Koh, Chang Woo, Wu, Xia, Liu, Bin, Wang, Junwei, Liao, Qiaogan, Li, Yongchun, Guo, Han, Woo, Han Young, Gao, Feng, and Guo, Xugang

Abstract

High-performance nonfullerene ternary organic solar cells (OSCs) with two polymer donors are less frequently reported because of the limited numbers of efficient polymer donors with good compatibility. Herein, a wide-bandgap polymer P1 with a deep-lying highest occupied molecular orbital (HOMO) level is incorporated as the third component into the benchmark PM6:Y6 binary system to fabricate ternary OSCs. The introduction of P1 not only leads to extended absorption coverage and forms a cascade-like energy level alignment but also shows excellent compatibility with PM6, resulting in a favorable morphology in the ternary blend. More importantly, P1 possesses a deeper HOMO level (-5.6 eV) than most well-known donor polymers, which enables resulting ternary OSCs with an improved open-circuit voltage. As a result, the optimized ternary OSCs with 40 wt% P1 in donors achieve a power conversion efficiency (PCE) of 16.2% with a small nonradiative recombination loss of 0.23 eV, which is among the highest values of ternary OSCs based on two polymer donors. In addition, the ternary OSCs show a broad composition tolerance with a high PCE of over 14% throughout the whole blend ratios. These results provide an effective approach to fabricate efficient ternary OSCs by synergizing two wide-bandgap polymer donors., Funding Agencies|National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21801124]; Shenzhen Science and Technology Innovation Commission [JCYJ20170817105905899, JCYJ20180504165709042]; National Research Foundation of KoreaNational Research Foundation of Korea [NRF-2016M1A2A2940911, 2019R1A6A1A11044070]; Center for Computational Science and Engineering of SUSTech

Published
2020
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36. A Narrow-Bandgap n-Type Polymer with an Acceptor-Acceptor Backbone Enabling Efficient All-Polymer Solar Cells

Author

Sun, Huiliang, Yu, Han, Shi, Yongqiang, Yu, Jianwei, Peng, Zhongxiang, Zhang, Xianhe, Liu, Bin, Wang, Junwei, Singh, Ranbir, Lee, Jaewon, Li, Yongchun, Wei, Zixiang, Liao, Qiaogan, Kan, Zhipeng, Ye, Long, Yan, He, Gao, Feng, Guo, Xugang, Sun, Huiliang, Yu, Han, Shi, Yongqiang, Yu, Jianwei, Peng, Zhongxiang, Zhang, Xianhe, Liu, Bin, Wang, Junwei, Singh, Ranbir, Lee, Jaewon, Li, Yongchun, Wei, Zixiang, Liao, Qiaogan, Kan, Zhipeng, Ye, Long, Yan, He, Gao, Feng, and Guo, Xugang

Abstract

Narrow-bandgap polymer semiconductors are essential for advancing the development of organic solar cells. Here, a new narrow-bandgap polymer acceptor L14, featuring an acceptor-acceptor (A-A) type backbone, is synthesized by copolymerizing a dibrominated fused-ring electron acceptor (FREA) with distannylated bithiophene imide. Combining the advantages of both the FREA and the A-A polymer, L14 not only shows a narrow bandgap and high absorption coefficient, but also low-lying frontier molecular orbital (FMO) levels. Such FMO levels yield improved electron transfer character, but unexpectedly, without sacrificing open-circuit voltage (V-oc), which is attributed to a small nonradiative recombination loss (E-loss,E-nr) of 0.22 eV. Benefiting from the improved photocurrent along with the high fill factor andV(oc), an excellent efficiency of 14.3% is achieved, which is among the highest values for all-polymer solar cells (all-PSCs). The results demonstrate the superiority of narrow-bandgap A-A type polymers for improving all-PSC performance and pave a way toward developing high-performance polymer acceptors for all-PSCs., Funding Agencies|Shenzhen Science and Technology Innovation Commission [JCYJ20170413173814007, JCYJ20170818113905024, JCYJ20170817105905899, JCYJ20180504165709042]; National Natural Science Foundation of China (NSFC)National Natural Science Foundation of China (NSFC) [21801124]; Stiftelsen for Strategisk Forskning through a Future Research Leader program [FFL18-0322]; Peiyang Scholar Program of Tianjin University; Open Fund of the State Key Laboratory of Luminescent Materials and Devices (South China University of Technology) [2020-skllmd-11]; Center for Computational Science and Engineering of SUSTech

Published
2020
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38. Achieving highly efficient all-polymer solar cells by green-solvent-processing under ambient atmosphere

Author

Liu, Bin, primary, Sun, Huiliang, additional, Lee, Jin-Woo, additional, Yang, Jie, additional, Wang, Junwei, additional, Li, Yongchun, additional, Li, Bangbang, additional, Xu, Meng, additional, Liao, Qiaogan, additional, Zhang, Wei, additional, Han, Dongxue, additional, Niu, Li, additional, Meng, Hong, additional, Kim, Bumjoon J., additional, and Guo, Xugang, additional

Published
2021
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39. A low-cost and green-solvent-processable hole-transport material enabled by a traditional bidentate ligand for highly efficient inverted perovskite solar cells

Author

Huang, Jiachen, primary, Yang, Jie, additional, Li, Dan, additional, Sun, Huiliang, additional, Su, Mengyao, additional, Ji, Xiaofei, additional, Li, Bolin, additional, Li, Bangbang, additional, Liao, Qiaogan, additional, Han, Dongxue, additional, Yan, He, additional, Niu, Li, additional, Wang, Dong, additional, and Guo, Xugang, additional

Published
2021
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40. A Narrow‐Bandgap n‐Type Polymer with an Acceptor–Acceptor Backbone Enabling Efficient All‐Polymer Solar Cells

Author

Sun, Huiliang, primary, Yu, Han, additional, Shi, Yongqiang, additional, Yu, Jianwei, additional, Peng, Zhongxiang, additional, Zhang, Xianhe, additional, Liu, Bin, additional, Wang, Junwei, additional, Singh, Ranbir, additional, Lee, Jaewon, additional, Li, Yongchun, additional, Wei, Zixiang, additional, Liao, Qiaogan, additional, Kan, Zhipeng, additional, Ye, Long, additional, Yan, He, additional, Gao, Feng, additional, and Guo, Xugang, additional

Published
2020
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41. Two Compatible Polymer Donors Enabling Ternary Organic Solar Cells with a Small Nonradiative Energy Loss and Broad Composition Tolerance

Author

Tang, Yumin, primary, Yu, Jianwei, additional, Sun, Huiliang, additional, Wu, Ziang, additional, Koh, Chang Woo, additional, Wu, Xia, additional, Liu, Bin, additional, Wang, Junwei, additional, Liao, Qiaogan, additional, Li, Yongchun, additional, Guo, Han, additional, Woo, Han Young, additional, Gao, Feng, additional, and Guo, Xugang, additional

Published
2020
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43. Teaching an Old Anchoring Group New Tricks: Enabling Low-Cost, Eco-Friendly Hole-Transporting Materials for Efficient and Stable Perovskite Solar Cells

Author

Wang, Yang, primary, Liao, Qiaogan, additional, Chen, Jianhua, additional, Huang, Wei, additional, Zhuang, Xinming, additional, Tang, Yumin, additional, Li, Bolin, additional, Yao, Xiyu, additional, Feng, Xiyuan, additional, Zhang, Xianhe, additional, Su, Mengyao, additional, He, Zhubing, additional, Marks, Tobin J., additional, Facchetti, Antonio, additional, and Guo, Xugang, additional

Published
2020
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45. Ultranarrow Bandgap Naphthalenediimide‐Dialkylbifuran‐Based Copolymers with High‐Performance Organic Thin‐Film Transistors and All‐Polymer Solar Cells

Author

Shi, Shengbin, primary, Chen, Peng, additional, Wang, Hang, additional, Koh, Chang Woo, additional, Uddin, Mohammad Afsar, additional, Liu, Bin, additional, Liao, Qiaogan, additional, Feng, Kui, additional, Woo, Han Young, additional, Xiao, Guomin, additional, and Guo, Xugang, additional

Published
2020
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48. Intramolecular Noncovalent Interaction‐Enabled Dopant‐Free Hole‐Transporting Materials for High‐Performance Inverted Perovskite Solar Cells.

Author

Yang, Kun, Liao, Qiaogan, Huang, Jun, Zhang, Zilong, Su, Mengyao, Chen, Zhicai, Wu, Ziang, Wang, Dong, Lai, Ziwei, Woo, Han Young, Cao, Yan, Gao, Peng, and Guo, Xugang

Subjects
*SOLAR cells, *ORGANIC semiconductors, *PEROVSKITE, *HOLE mobility, *THERMAL properties, *SPINE
Abstract

Intramolecular noncovalent interactions (INIs) have served as a powerful strategy for accessing organic semiconductors with enhanced charge transport properties. Herein, we apply the INI strategy for developing dopant‐free hole‐transporting materials (HTMs) by constructing two small‐molecular HTMs featuring an INI‐integrated backbone for high‐performance perovskite solar cells (PVSCs). Upon incorporating noncovalent S⋅⋅⋅O interaction into their simple‐structured backbones, the resulting HTMs, BTORA and BTORCNA, showed self‐planarized backbones, tuned energy levels, enhanced thermal properties, appropriate film morphology, and effective defect passivation. More importantly, the high film crystallinity enables the materials with substantial hole mobilities, thus rendering them as promising dopant‐free HTMs. Consequently, the BTORCNA‐based inverted PVSCs delivered a power conversion efficiency of 21.10 % with encouraging long‐term device stability, outperforming the devices based on BTRA without S⋅⋅⋅O interaction (18.40 %). This work offers a practical approach to designing charge transporting layers with high intrinsic mobilities for high‐performance PVSCs. [ABSTRACT FROM AUTHOR]

Published
2022
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49. A Cost‐Effective D‐A‐D Type Hole‐Transport Material Enabling 20% Efficiency Inverted Perovskite Solar Cells†.

Author

Huang, Jiachen Please check if link to ORCID is correct. --> Please confirm that given names (blue) and surnames/family names (vermilion) have been identified correctly. -->, Yang, Jie, Sun, Huiliang, Feng, Kui, Liao, Qiaogan, Li, Bolin, Yan, He, and Guo, Xugang

Subjects
FRONTIER orbitals, PEROVSKITE, SURFACE passivation, CARBONYL group, SOLAR cells, PASSIVATION, FUNCTIONAL groups
Abstract

Main observation and conclusion: High‐performance, cost‐effective hole‐transport materials (HTMs) are greatly desired for the commercialization of perovskite solar cells (PVSCs). Herein, two new HTMs, TPA‐FO and TPA‐PDO, are devised and synthesized, which have a donor‐acceptor‐donor (D‐A‐D) type molecule design featuring carbonyl group‐functionalized arenes as the acceptor (A) units. The carbonyl group at the central core of HTMs can not only tune frontier molecular orbital (FMO) energy levels and surface wettability, but also can enable efficient surface passivation effects, resulting in reduced recombination loss. When employed as HTMs in inverted PVSCs without using dopant, TPA‐FO with one carbonyl group yields a high power conversion efficiency (PCE) of 20.24%, which is among the highest values reported in the inverted PVSCs with dopant‐free HTMs. More importantly, the facile one‐step synthetic process enables a low cost of 30 USD g–1 for TPA‐FO, much cheaper than the most studied HTMs used for high‐efficiency dopant‐free PVSCs. These results demonstrate the potential of D‐A‐D type molecules with carbonyl group‐functionalized arene core in developing the low‐cost dopant‐free HTMs toward highly efficient PVSCs. [ABSTRACT FROM AUTHOR]

Published
2021
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50. A Narrow‐Bandgap n‐Type Polymer Semiconductor Enabling Efficient All‐Polymer Solar Cells

Author

Shi, Shengbin, primary, Chen, Peng, additional, Chen, Yao, additional, Feng, Kui, additional, Liu, Bin, additional, Chen, Jianhua, additional, Liao, Qiaogan, additional, Tu, Bao, additional, Luo, Jiasi, additional, Su, Mengyao, additional, Guo, Han, additional, Kim, Myung‐Gil, additional, Facchetti, Antonio, additional, and Guo, Xugang, additional

Published
2019
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