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2. Impact of Severe Plastic Deformation on Kinetics and Thermodynamics of Hydrogen Storage in Magnesium and Its Alloys

Author

Edalati, Kaveh, Akiba, Etsuo, Botta, Walter J., Estrin, Yuri, Floriano, Ricardo, Fruchart, Daniel, Grosdidier, Thierry, Horita, Zenji, Huot, Jacques, Li, Hai-Wen, Lin, Huai-Jun, Revesz, Adam, and Zehetbauer, Michael J.

Subjects
Condensed Matter - Materials Science, Physics - Chemical Physics
Abstract

Magnesium and its alloys are the most investigated materials for solid-state hydrogen storage in the form of metal hydrides, but there are still unresolved problems with the kinetics and thermodynamics of hydrogenation and dehydrogenation of this group of materials. Severe plastic deformation (SPD) methods, such as equal-channel angular pressing (ECAP), high-pressure torsion (HPT), intensive rolling and fast forging, have been widely used to enhance the activation, air resistance, and hydrogenation/dehydrogenation kinetics of Mg-based hydrogen storage materials by introducing ultrafine/nanoscale grains and crystal lattice defects. These severely deformed materials, particularly in the presence of alloying additives or second-phase nanoparticles, can show not only fast hydrogen absorption/desorption kinetics but also good cycling stability. It was shown that some materials that are apparently inert to hydrogen can absorb hydrogen after SPD processing. Moreover, the SPD methods were effectively used for hydrogen binding-energy engineering and synthesizing new magnesium alloys with low thermodynamic stability for reversible low/room-temperature hydrogen storage, such as nanoglasses, high-entropy alloys, and metastable phases including the high-pressure {\gamma}-MgH2 polymorph. This article reviews recent advances in the development of Mg-based hydrogen storage materials by SPD processing and discusses their potential in future applications.

Published
2023
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3. High-Entropy Hydrides for Fast and Reversible Hydrogen Storage at Room Temperature: Binding-Energy Engineering via First-Principles Calculations and Experiments

Author

Mohammadi, Abbas, Ikeda, Yuji, Edalati, Parisa, Mito, Masaki, Grabowski, Blazej, Li, Hai-Wen, and Edalati, Kaveh

Subjects
Condensed Matter - Materials Science
Abstract

Despite high interest in compact and safe storage of hydrogen in the solid-state hydride form, the design of alloys that can reversibly and quickly store hydrogen at room temperature under pressures close to atmospheric pressure is a long-lasting challenge. In this study, first-principles calculations are combined with experiments to develop high-entropy alloys (HEAs) for room-temperature hydrogen storage. TixZr2-xCrMnFeNi (x = 0.4-1.6) alloys with the Laves phase structure and low hydrogen binding energies of -0.1 to -0.15 eV are designed and synthesized. The HEAs reversibly store hydrogen in the form of Laves phase hydrides at room temperature, while (de)hydrogenation pressure systematically reduces with increasing the zirconium fraction in good agreement with the binding energy calculations. The kinetics of hydrogenation are fast, the hydrogenation occurs without any activation or catalytic treatment, the hydrogen storage performance remains stable for at least 1000 cycles, and the storage capacity is higher than that for commercial LaNi5. The current findings demonstrate that a combination of theoretical calculations and experiments is a promising pathway to design new high-entropy hydrides with high performance for hydrogen storage.

Published
2023
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5. Severe plastic deformation for producing superfunctional ultrafine-grained and heterostructured materials: An interdisciplinary review

Author

Edalati, Kaveh, Ahmed, Anwar Q., Akrami, Saeid, Ameyama, Kei, Aptukov, Valery, Asfandiyarov, Rashid N., Ashida, Maki, Astanin, Vasily, Bachmaier, Andrea, Beloshenko, Victor, Bobruk, Elena V., Bryła, Krzysztof, Cabrera, José María, Carvalho, Amanda P., Chinh, Nguyen Q., Choi, In-Chul, Chulist, Robert, Cubero-Sesin, Jorge M., Davdian, Gregory, Demirtas, Muhammet, Divinski, Sergiy, Durst, Karsten, Dvorak, Jiri, Edalati, Parisa, Emura, Satoshi, Enikeev, Nariman A., Faraji, Ghader, Figueiredo, Roberto B., Floriano, Ricardo, Fouladvind, Marjan, Fruchart, Daniel, Fuji, Masayoshi, Fujiwara, Hiroshi, Gajdics, Marcell, Gheorghe, Diana, Gondek, Łukasz, González-Hernández, Joaquín E., Gornakova, Alena, Grosdidier, Thierry, Gubicza, Jenő, Gunderov, Dmitry, He, Liqing, Higuera, Oscar Fabian, Hirosawa, Shoichi, Hohenwarter, Anton, Horita, Zenji, Horky, Jelena, Huang, Yi, Huot, Jacques, Ikoma, Yoshifumi, Ishihara, Tatsumi, Ivanisenko, Yulia, Jang, Jae-il, Jorge, Alberto M., Jr, Kawabata-Ota, Mie, Kawasaki, Megumi, Khelfa, Tarek, Kobayashi, Junya, Kommel, Lembit, Korneva, Anna, Kral, Petr, Kudriashova, Natalia, Kuramoto, Shigeru, Langdon, Terence G., Lee, Dong-Hyun, Levitas, Valery I., Li, Cong, Li, Hai-Wen, Li, Yongtao, Li, Zheng, Lin, Huai-Jun, Liss, Klaus-Dieter, Liu, Ying, Cardona, Diana Maritza Marulanda, Matsuda, Kenji, Mazilkin, Andrey, Mine, Yoji, Miyamoto, Hiroyuki, Moon, Suk-Chun, Müller, Timo, Muñoz, Jairo Alberto, Murashkin, Maxim Yu., Naeem, Muhammad, Novelli, Marc, Olasz, Dániel, Pippan, Reinhard, Popov, Vladimir V., Popova, Elena N., Purcek, Gencaga, de Rango, Patricia, Renk, Oliver, Retraint, Delphine, Révész, Ádám, Roche, Virginie, Rodriguez-Calvillo, Pablo, Romero-Resendiz, Liliana, Sauvage, Xavier, Sawaguchi, Takahiro, Sena, Hadi, Shahmir, Hamed, Shi, Xiaobin, Sklenicka, Vaclav, Skrotzki, Werner, Skryabina, Nataliya, Staab, Franziska, Straumal, Boris, Sun, Zhidan, Szczerba, Maciej, Takizawa, Yoichi, Tang, Yongpeng, Valiev, Ruslan Z., Vozniak, Alina, Voznyak, Andrei, Wang, Bo, Wang, Jing Tao, Wilde, Gerhard, Zhang, Fan, Zhang, Meng, Zhang, Peng, Zhou, Jianqiang, Zhu, Xinkun, and Zhu, Yuntian T.

Published
2024
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9. Materials for hydrogen-based energy storage: Past, recent progress and future outlook

Author

Yartys, Volodymyr A., Baricco, Marcello, von Colbe, Jose Bellosta, Blanchard, Didier, Bowman Jr., Robert C., Broom, Darren P., Buckley, Craig E., Chang, Fei, Chen, Ping, Cho, Young Whan, Crivello, Jean-Claude, Cuevas, Fermin, David, William I. F., de Jongh, Petra E., Denys, Roman V., Dornheim, Martin, Felderhoff, Michael, Filinchuk, Yaroslav, Froudakis, George E., Grant, David M., Hauback, Bjørn C., Havela, Ladislav, He, Teng, Hirscher, Michael, Humphries, Terry D., Jensen, Torben R., Kim, Sangryun, Kojima, Yoshitsugu, Latroche, Michel, Li, Hai-Wen, Lototskyy, Mykhaylo V., Makepeace, Joshua W., Møller, Kasper T., Naheed, Lubna, Ngene, Peter, Noréus, Dag, Nygård, Magnus Moe, Orimo, Shin-ichi, Paskevicius, Mark, Pasquini, Luca, Ravnsbæk, Dorthe B., Sofianos, M. Veronica, Udovic, Terrence J., Vegge, Tejs, Walker, Gavin S., Webb, Colin J., Weidenthaler, Claudia, and Zlotea, Claudia

Subjects
Condensed Matter - Materials Science, Condensed Matter - Other Condensed Matter
Abstract

Magnesium hydride owns the largest share of publications on solid materials for hydrogen storage. The Magnesium group of international experts contributing to IEA Task 32 Hydrogen Based Energy Storage recently published two review papers presenting the activities of the group focused on magnesium hydride based materials and on Mg based compounds for hydrogen and energy storage. This review article not only overviews the latest activities on both fundamental aspects of Mg-based hydrides and their applications, but also presents a historic overview on the topic and outlines projected future developments. Particular attention is paid to the theoretical and experimental studies of Mg-H system at extreme pressures, kinetics and thermodynamics of the systems based on MgH2,nanostructuring, new Mg-based compounds and novel composites, and catalysis in the Mg based H storage systems. Finally, thermal energy storage and upscaled H storage systems accommodating MgH2 are presented.

Published
2020
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35. Liquid Hydrogen Carriers

Author

Li, Hai-Wen, Sasaki, Kazunari, editor, Li, Hai-Wen, editor, Hayashi, Akari, editor, Yamabe, Junichiro, editor, Ogura, Teppei, editor, and Lyth, Stephen M., editor

Published
2016
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46. Impact of severe plastic deformation on kinetics and thermodynamics of hydrogen storage in magnesium and its alloys

Author

Edalati, Kaveh, primary, Akiba, Etsuo, additional, Botta, Walter J., additional, Estrin, Yuri, additional, Floriano, Ricardo, additional, Fruchart, Daniel, additional, Grosdidier, Thierry, additional, Horita, Zenji, additional, Huot, Jacques, additional, Li, Hai-Wen, additional, Lin, Huai-Jun, additional, Révész, Ádám, additional, and Zehetbauer, Michael J., additional

Published
2023
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49. Functional Materials Based on Metal Hydrides

Author

Li, Hai-Wen, Buckley, Craig, Jensen, Torben, and Zhu, Min

Abstract

Our extreme and growing energy consumption, based on fossil fuels, has significantly increased the levels of carbon dioxide in the atmosphere, which may lead to global and irreversible climate changes. We have plenty of renewable energy, e.g., sun and wind, but the fluctuations over time and geography call for a range of new ideas and, possibly, novel technologies. The most difficult challenge appears to be the development of the efficient and reliable storage of renewable energy. Hydrogen has long been considered as a potential means of energy storage; however, storage of hydrogen is also challenging. Therefore, a wide range of hydrogen-containing materials, with energy-related functions, has been discovered over the past few decades. The chemistry of hydrogen is very diverse, and so also are the new hydrides that have been discovered, not only in terms of structure and composition but also in terms of their properties. This has led to a wide range of new possible applications of metal hydrides that permeate beyond solid-state hydrogen storage. A variety of new hydrides, proposed as battery materials, has been discovered. These can exploit properties as fast ion conductors or as conversion-type electrodes with much higher potential energy capacities, compared to materials currently used in commercial batteries. Solar heat storage is also an area of great potential for metal hydrides, in principle offering orders of magnitude better storage performance than phase change materials. Recently, hydrides with optical and superconducting properties have also been investigated. This Special Issue of Inorganics, entitled “Functional Materials Based on Metal Hydrides”, is dedicated to the full range of emerging electronic, photonic, and energy-related, inorganic, hydrogen-containing materials.

Published
2018

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