Search

We propose a scheme to realize quantum controlled-Z (CZ) gates through single gradient metasurface. Using its unique parallel beam-splitting feature, i.e., a series of connected beam splitters with the same splitting ratio, one metasurface can support a CZ gate, several independent CZ gates, or a cascaded CZ gates. Taking advantage of the input polarization determined output path-locking feature, both polarization-encoded and path-encoded CZ gates can be demonstrated on the same metasurface, which further improves the integration level of quantum devices. Our research paves the way for integrating quantum logical function through the metasurface.

Gradient metasurface, formed by a set of subwavelength unit cells with different phase modulation, is widely used in polarized beam splitting (BS) in the classical and quantum optics. Specifically, its phase gradient allows the path and polarization of multiple output lights to be locked by corresponding inputs.Using this unique path-polarization locked property, we demonstrate that the single metasurface can function as sequentially linked beamsplitters, enabling the parallelization of a series of BS processes. Such a parallel BS metasurface provides a multi-beam interference capability for both classical and quantum light manipulation. Taking this advantage, we first prepare path and polarization hybrid entangled states of two, three, and multi photons from unentangled photon sources. Then, the ability of parallel BS-facilitated entanglement is applied to demonstrate entanglement fusion among entangled photon pairs, which can greatly enlarge the entanglement dimension. The principle of parallel BS through the metasurface opens up a versatile way to manipulate the quantum state at the micro/nano scale, which will have potential applications in on-chip quantum optics and quantum information processing.

We study the resonant enhancement of linear and nonlinear chiroptical effects in asymmetric silicon metasurfaces supporting multipolar Mie resonances and quasi-bound states in the continuum (quasi-BICs). We demonstrate theoretically and observe in experiment the pronounced linear circular dichroism at the quasi-BIC resonances. We further find that both local field enhancement and third-harmonic signal are large for Mie resonances and some quasi-BIC modes. We explain the selectivity of the nonlinear enhancement by employing the concept of critical coupling being more favorable for the modes with moderately large radiative quality factors ($Q$ factors). We demonstrate experimentally strong nonlinear chiroptical response associated with high efficiency of the third-harmonic generation and large nonlinear circular dichroism varying from $+0.918\pm0.049$ to $-0.771\pm0.004$ for the samples with different asymmetries. We believe our results suggest a general strategy for engineering nonlinear chiroptical response in dielectric resonant metasurfaces., Comment: 23 pages, 5 figures

Nanophotonic platforms such as metasurfaces, achieving arbitrary phase profiles within ultrathin thickness, emerge as miniaturized, ultracompact and kaleidoscopic optical vortex generators. However, it is often required to segment or interleave independent subarray metasurfaces to multiplex optical vortices in a single nano device, which in turn affects the compactness and channel capacity of the device. Here, inspired by phyllotaxis patterns in pine cones and sunflowers, we theoretically prove and experimentally report that multiple optical vortices can be produced in a single compact phyllotaxis nanosieve, both in free space and on a chip, where one metaatom may contribute to many vortices simultaneously. The time resolved dynamics of on chip interference wavefronts between multiple plasmonic vortices was revealed by ultrafast time-resolved photoemission electron microscopy. Our nature inspired optical vortex generator would facilitate various vortex related optical applications, including structured wavefront shaping, free space and plasmonic vortices, and high capacity information metaphotonics.

Compact and robust cold atom sources are increasingly important for quantum research, especially for transferring cutting-edge quantum science into practical applications. In this letter, we report on a novel scheme that utilizes a metasurface optical chip to replace the conventional bulky optical elements used to produce a cold atomic ensemble with a single incident laser beam, which is split by the metasurface into multiple beams of the desired polarization states. Atom numbers $~10^7$ and temperatures (about 35 ${\mu}$K) of relevance to quantum sensing are achieved in a compact and robust fashion. Our work highlights the substantial progress towards fully integrated cold atom quantum devices by exploiting metasurface optical chips, which may have great potential in quantum sensing, quantum computing and other areas.

Phase, polarization, amplitude and frequency represent the basic dimensions of light, playing crucial roles for both fundamental light-mater interactions and all major optical applications. Metasurface emerges as a compact platform to manipulate these knobs, but previous metasurfaces have limited flexibility to simultaneous control them. Here, we introduce a multi-freedom metasurface that can simultaneously and independently modulate phase, polarization and amplitude in an analytical form, and further realize frequency multiplexing by a k-space engineering technique. The multi-freedom metasurface seamlessly combine geometric Pancharatnam-Berry phase and detour phase, both of which are frequency-independent. As a result, it allows complex-amplitude vectorial hologram at various frequencies based on the same design strategy, without sophisticated nanostructure searching of massive size parameters. Based on this principle, we experimentally demonstrate full-color complex-amplitude vectorial meta-holograms in the visible with a metal-insulator metal architecture, unlocking the long-sought full potential of advanced light field manipulation through ultrathin metasurfaces.

Optical metasurfaces open new avenues for precise wavefront control of light for integrated quantum technology. Here, we demonstrate a hybrid integrated quantum photonic system that is capable to entangle and disentangle two-photon spin states at a dielectric metasurface. By interfering single-photon pairs at a nanostructured dielectric metasurface, a path-entangled two-photon NOON state with circular polarization is generated that exhibits a quantum HOM interference visibility of 86 $\pm$ 4%. Furthermore, we demonstrate nonclassicality and phase sensitivity in a metasurface-based interferometer with a fringe visibility of 86.8 $\pm$ 1.1 % in the coincidence counts. This high visibility proves the metasurface-induced path entanglement inside the interferometer. Our findings provide a promising way to hybrid-integrated quantum technology with high-dimensional functionalities in various applications like imaging, sensing, and computing.

Nonlinear nanostructured surfaces provide a paradigm shift in nonlinear optics with new ways to control and manipulate frequency conversion processes at the nanoscale, also offering novel opportunities for applications in photonics, chemistry, material science, and biosensing. Here, we develop a general approach to employ sharp resonances in metasurfaces originated from the physics of bound states in the continuum for both engineering and enhancing the nonlinear response. We study experimentally the third-harmonic generation from metasurfaces composed of symmetry-broken silicon meta-atoms and reveal that the harmonic generation intensity depends critically on the asymmetry parameter. We employ the concept of the critical coupling of light to the metasurface resonances to uncover the effect of radiative and nonradiative losses on the nonlinear conversion efficiency., Comment: 7 pages, 4 figures

The abrupt phase change of light at metasurfaces provides high flexibility in wave manipulation without the need of accumulation of propagating phase through dispersive materials. In the linear optical regime, one important application field of metasurfaces is imaging by planar metalenses, which enables device miniaturization and aberration correction compared to conventional optical microlens systems. With the incorporation of nonlinear responses into passive metasurfaces, optical functionalities of metalenses are anticipated to be further enriched, leading to completely new applications areas. Here, we demonstrate imaging with nonlinear metalenses that combine the function of an ultrathin planar lens with simultaneous frequency conversion. With such nonlinear metalenses, we experimentally demonstrate imaging of objects with near infrared light while the image appears in the second harmonic signal of visible frequency range. Furthermore, the functionality of these nonlinear metalenses can be modified by switching the handedness of the circularly polarized fundamental wave, leading to either real or virtual nonlinear image formation. Nonlinear metalenses do not only enable infrared light imaging through a visible detector but also have the ability to modulate nonlinear optical responses through an ultrathin metasurface device while the fundamental wave remains unaffected, which offers the capability of nonlinear information processing with novel optoelectronic devices.