108 results on '"Levelt, P.F."'
Search Results
2. Meer meten, robuuster rekenen : Eindrapport van het Adviescollege Meten en Berekenen Stikstof
- Author
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Hordijk, L., Erisman, J.W., Eskes, H., Hanekamp, J.C., Krol, M.C., Levelt, P.F., Schaap, M., Vries, W. de, Hordijk, L., Erisman, J.W., Eskes, H., Hanekamp, J.C., Krol, M.C., Levelt, P.F., Schaap, M., and Vries, W. de
- Abstract
Taak van het adviescollege was om te beoordelen of de huidige meet- en rekensystematiek voor stikstofemissie en -depositie voldoende wetenschappelijke onderbouwing biedt voor het stikstofbeleid. In de eerste fase keek het adviescollege naar de algemene inrichting van de meet- en rekensystematiek. In de tweede fase werkte het adviescollege, waar nodig, de eerste bevindingen verder uit en besteedde daarnaast bijzondere aandacht aan NEMA (voor de bepaling van de landbouwemissies) en AERIUS Calculator als toetsingsinstrument bij vergunningverlening.
- Published
- 2020
3. Niet uit de lucht gegrepen : Eerste rapport van het Adviescollege Meten en Berekenen Stikstof
- Author
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Hordijk, L., Erisman, J.W., Eskes, H., Hanekamp, J.C., Krol, M.C., Levelt, P.F., Schaap, M., Vries, W. de, Hordijk, L., Erisman, J.W., Eskes, H., Hanekamp, J.C., Krol, M.C., Levelt, P.F., Schaap, M., and Vries, W. de
- Abstract
Het Adviescollege Meten en Berekenen Stikstof is in december 2019 begonnen aan de eerste fase van zijn opdracht om advies te geven over de wetenschappelijke kwaliteit van de Nederlandse systematiek voor het meten van en rekenen aan stikstofverbindingen ter onderbouwing van het (toekomstig) beleid van de Rijksoverheid en provincies. Het uitgangspunt was de vraag: zijn de data, methoden en modellen die worden ingezet van voldoende wetenschappelijke kwaliteit en daarmee doelgeschikt?
- Published
- 2020
4. Molecules with large-amplitude torsional motion partially oriented in a nematic liquid crystal: Ethane and isotopomers
- Author
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Burnell, E.E., Lange, C.A. de, Barnhoorn, J.B.S., Aben, I., and Levelt, P.F.
- Subjects
Liquid crystals -- Structure ,Ethanes -- Structure ,Ethanes -- Atomic properties ,Solvents -- Chemical properties ,Solvents -- Structure ,Nuclear magnetic resonance -- Analysis ,Chemicals, plastics and rubber industries - Abstract
A consistent set of experimental nuclear magnetic resonance (NMR) dipolar and quadrupolar coupling for ethane and its isotopomers are studied. The calculated deuterium quadrupolar couplings show discrepancies supporting the notion that average electric field gradients are important in liquid-crystal solvent.
- Published
- 2005
5. Variational assimilation of GOME total-column ozone satellite data in a 2D latitude-longitude tracer-transport model
- Author
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Eskes, H.J., Piters, A.J.M., Levelt, P.F., Allaart, M.A.F., and Kelder, H.M.
- Subjects
Ozone -- Measurement ,Weather forecasting -- Research ,Atmosphere -- Models ,Earth sciences ,Science and technology - Abstract
A four-dimensional data-assimilation method is described to derive synoptic ozone fields from total-column ozone satellite measurements. The ozone columns are advected by a 2D tracer-transport model, using ECMWF wind fields at a single pressure level. Special attention is paid to the modeling of the forecast error covariance and quality control. The temporal and spatial dependence of the forecast error is taken into account, resulting in a global error field at any instant in time that provides a local estimate of the accuracy of the assimilated field. The authors discuss the advantages of the 4D-variational (4D- Var) approach over sequential assimilation schemes. One of the attractive features of the 4D-Var technique is its ability to incorporate measurements at later times t > t(sub o) in the analysis at time t(sub o), in a way consistent with the time evolution as described by the model. This significantly improves the offline analyzed ozone fields.
- Published
- 1999
6. Summary of Results from the NOAA Shale Oil and Natural Gas Nexus (SONGNEX) Study
- Author
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de Gouw, J.A. (author), Warneke, C. (author), Trainer, M. (author), Peischl, J. (author), Ryerson, T.B. (author), de Bruin, Joep (author), Levelt, P.F. (author), Veefkind, Joris Pepijn (author), Vlemmix, T. (author), de Gouw, J.A. (author), Warneke, C. (author), Trainer, M. (author), Peischl, J. (author), Ryerson, T.B. (author), de Bruin, Joep (author), Levelt, P.F. (author), Veefkind, Joris Pepijn (author), and Vlemmix, T. (author)
- Abstract
In March and April of 2015, the NOAA WP-3D research aircraft made airborne measurements over several different oil and natural gas production regions in the central and western U.S. ranging from North Dakota to Texas. The study was conducted at a time when the domestic production of natural gas was at an all-time high and the production of crude oil near an all-time high, but also when drilling activity had abruptly decreased due to a drop in the price of oil. In this presentation, we will give a summary of the measurement results obtained in the different production regions. Emission fluxes of greenhouse gases (CH4) and air pollutants (VOCs, NOx, air toxics) were determined through mass balance and from enhancement ratios versus methane. While photochemistry was generally weak during the flights, some trace gases showed evidence for secondary formation. Measurements by mass spectrometry showed the presence of some less commonly observed trace gases including nitrogen heterocyclic compounds. Emissions of pollutants are expressed as a fraction of the produced natural gas and crude oil. Such metrics can be compared with emission factors for fossil fuel combustion by other sources (motor vehicles and power plants) and allow a comparison of emissions from different stages in the lifecycle of fossil fuels. We have also studied NOx emissions from oil and natural gas production through trend analysis of the NO2columns from the Ozone Monitoring Instrument. This analysis shows that the drilling of new wells and the extraction of crude oil and natural gas both lead to NOx emissions. These results are compared with a new fuel-based emission inventory for NOx emissions from oil and natural gas production., A33C-04 presented at 2018 Fall Meeting, AGU, Washington, D.C., 10-14 Dec. Session: A33C Emissions of Atmospheric Pollutants from Oil, Gas, and Coal Operations I, Atmospheric Remote Sensing
- Published
- 2018
7. Cavity-Ring-Down Spectroscopy on Water Vapor in the Range 555–604 nm
- Author
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Naus, H., Ubachs, W., Levelt, P.F., Polyansky, O.L., Zobov, N.F., and Tennyson, J.
- Published
- 2001
- Full Text
- View/download PDF
8. Impact of aerosols on the OMI tropospheric NO2 retrievals over industrialized regions: How accurate is the aerosol correction of cloud-free scenes via a simple cloud model? (discussion paper)
- Author
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Chimot, J.J., Vlemmix, T., Veefkind, J.P., De Haan, J.F., and Levelt, P.F.
- Subjects
OA-Fund TU Delft - Abstract
The Ozone Monitoring Instrument (OMI) instrument has provided daily global measurements of tropospheric NO2 for more than a decade. Numerous studies have drawn attention to the complexities related to measurements of tropospheric NO2 in the presence of aerosols. Fine particles affect the OMI spectral measurements and the length of the average light path followed by the photons. However, they are not explicitly taken into account in the current OMI tropospheric NO2 retrieval chain. Instead, the operational OMI O2-O2 cloud retrieval algorithm is applied both to cloudy scenes and to cloud free scenes with aerosols present. This paper describes in detail the complex interplay between the spectral effects of aerosols, the OMI O2-O2 cloud retrieval algorithm and the impact on the accuracy of the tropospheric NO2 retrievals through the computed Air Mass Factor (AMF) over cloud-free scenes. Collocated OMI NO2 and MODIS Aqua aerosol products are analysed over East China, in industrialized area. In addition, aerosol effects on the tropospheric NO2 AMF and the retrieval of OMI cloud parameters are simulated. Both the observation-based and the simulation-based approach demonstrate that the retrieved cloud fraction linearly increases with increasing Aerosol Optical Thickness (AOT), but the magnitude of this increase depends on the aerosol properties and surface albedo. This increase is induced by the additional scattering effects of aerosols which enhance the scene brightness. The decreasing effective cloud pressure with increasing AOT represents primarily the absorbing effects of aerosols. The study cases show that the actual aerosol correction based on the implemented OMI cloud model results in biases between ?20 and ?40 % for the DOMINO tropospheric NO2 product in cases of high aerosol pollution (AOT ? 0.6) and elevated particles. On the contrary, when aerosols are relatively close to the surface or mixed with NO2, aerosol correction based on the cloud model results in overestimation of the DOMINO tropospheric NO2 product, between 10 and 20 %. These numbers are in line with comparison studies between ground-based and OMI tropospheric NO2 measurements under conditions with high aerosol pollution and elevated particles. This highlights the need to implement an improved aerosol correction in the computation of tropospheric NO2 AMFs.
- Published
- 2015
9. OMI tropospheric NO2 profiles from cloud slicing: Constraints on surface emissions, convective transport and lightning NOx (discussion paper)
- Author
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Belmonte Rivas, M., Veefkind, J.P., Eskes, H., and Levelt, P.F.
- Subjects
OA-Fund TU Delft - Abstract
We derive a global climatology of tropospheric NO2 profiles from OMI cloudy observations for the year 2006 using the cloud slicing method on six pressure levels centered about 280, 380, 500, 620, 720 and 820 hPa. A comparison between OMI and the TM4 model tropospheric NO2 profiles reveals striking overall similarities, which confer great confidence to the cloud-slicing approach, along with localized discrepancies that seem to probe into particular model processes. Anomalies detected at the lowest levels can be traced to deficiencies in the model surface emission inventory, at mid tropospheric levels to convective transport and horizontal advective diffusion, and at the upper tropospheric levels to model lightning NOx production and the placement of deeply transported NO2 plumes such as from the Asian summer monsoon. The vertical information contained in the OMI cloud-sliced NO2 profiles provides a global observational constraint that can be used to evaluate chemistry transport models (CTMs) and guide the development of key parameterization schemes.
- Published
- 2015
10. NOx emission estimates during the 2014 Youth Olympic Games in Nanjing (discussion paper)
- Author
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Ding, J., Van der A, R.J., Mijling, B., Levelt, P.F., and Hao, N.
- Subjects
OA-Fund TU Delft - Abstract
The Nanjing Government has taken temporary environmental regulations to guarantee good air quality during the Youth Olympic Games (YOG) in 2014. We study the effect of those regulations by applying the emission estimate algorithm DECSO (Daily Emission estimates Constrained by Satellite Observations) to measurements of the Ozone Monitoring Instrument (OMI). We improved DECSO by updating the chemical transport model CHIMERE from v2006 to v2013 and by adding an Observation minus Forecast (OmF) criterion to filter outlying satellite retrievals due to high aerosol concentrations. The comparison of model results with both ground and satellite observations indicates that CHIMERE v2013 is better performing than CHIMERE v2006. After filtering the satellite observations with high aerosol loads that were leading to large OmF values, unrealistic jumps in the emission estimates are removed. Despite the cloudy conditions during the YOG we could still see a decrease of tropospheric NO2 column concentrations of about 32% in the OMI observations as compared to the average NO2 concentrations from 2005 to 2012. The results of the improved DECSO algorithm for NOx emissions show a reduction of at least 25% during the YOG period. This indicates that air quality regulations taken by the local government were successful. The algorithm is also able to detect an emission reduction of 10% during the Chinese Spring Festival. This study demonstrates the capacity of the DECSO algorithm to capture the change of NOx emissions on a monthly scale. We also show that the observed concentrations and the derived emissions show different patterns that provide complimentary information. For example, the Nanjing smog episode in December 2013 led to a strong increase in NO2 concentrations without an increase in NOx emissions. Furthermore, DECSO gives us important information of the non-trivial seasonal relation between NOx emissions and NO2 concentrations on a local scale.
- Published
- 2014
11. Past changes in the vertical distribution of ozone: Part 1: Measurement techniques, uncertainties and availability
- Author
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Hassler, B., Petropavlovskikh, I., Staehelin, J., August, T., Bhartia, P.K., Clerbaux, C., Degenstein, D., De Mazière, M., Dinelli, B.M., Dudhia, A., Dufour, G., Frith, S.M., Froidevaux, L., Godin-Beekmann, S., Granville, J., Harris, N.R.P., Hoppel, K., Hubert, D., Kasai, Y., Kurylo, M.J., Kyrölä, E., Levelt, P.F., McElroy, C.T., McPeters, R.D., Munro, R., Nakajima, H., Parrish, A., Raspollini, P., Remsberg, E.E., Rosenlof, K.H., Rozanov, A., Sano, T., Sasano, Y., Shiotani, M., Smit, H.G.J., Stiller, G., Tamminen, J., Tarasick, D.W., Urban, J., Van Der A, R.J., Veefkind, J.P., Vigouroux, C., Von Clarmann, T., Von Savigny, C., Walker, K.A., Weber, M., Wild, J., and Zawodny, J.M.
- Subjects
Earth sciences ,ddc:550 - Abstract
Peak stratospheric chlorofluorocarbon (CFC) and other ozone depleting substance (ODS) concentrations were reached in the mid- to late 1990s. Detection and attribution of the expected recovery of the stratospheric ozone layer in an atmosphere with reduced ODSs as well as efforts to understand the evolution of stratospheric ozone in the presence of increasing greenhouse gases are key current research topics. These require a critical examination of the ozone changes with an accurate knowledge of the spatial (geographical and vertical) and temporal ozone response. For such an examination, it is vital that the quality of the measurements used be as high as possible and measurement uncertainties well quantified. In preparation for the 2014 United Nations Environment Programme (UNEP)/World Meteorological Organization (WMO) Scientific Assessment of Ozone Depletion, the SPARC/IO3C/IGACO-O3/NDACC (SI2N) Initiative was designed to study and document changes in the global ozone profile distribution. This requires assessing long-term ozone profile data sets in regards to measurement stability and uncertainty characteristics. The ultimate goal is to establish suitability for estimating long-term ozone trends to contribute to ozone recovery studies. Some of the data sets have been improved as part of this initiative with updated versions now available. This summary presents an overview of stratospheric ozone profile measurement data sets (ground and satellite based) available for ozone recovery studies. Here we document measurement techniques, spatial and temporal coverage, vertical resolution, native units and measurement uncertainties. In addition, the latest data versions are briefly described (including data version updates as well as detailing multiple retrievals when available for a given satellite instrument). Archive location information for each data set is also given., Atmospheric Measurement Techniques, 7 (5), ISSN:1867-1381, ISSN:1867-8548
- Published
- 2014
- Full Text
- View/download PDF
12. MAX-DOAS tropospheric nitrogen dioxide column measurements compared with the Lotos-Euros air quality model
- Author
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Vlemmix, T., Eskes, H.J., Piters, A.J.M., Schaap, M., Sauter, F.J., Kelder, H., Levelt, P.F., Vlemmix, T., Eskes, H.J., Piters, A.J.M., Schaap, M., Sauter, F.J., Kelder, H., and Levelt, P.F.
- Abstract
A 14-month data set of MAX-DOAS (Multi-Axis Differential Optical Absorption Spectroscopy) tropospheric NO2 column observations in De Bilt, the Netherlands, has been compared with the regional air quality model Lotos-Euros. The model was run on a 7×7 km2 grid, the same resolution as the emission inventory used. A study was performed to assess the effect of clouds on the retrieval accuracy of the MAX-DOAS observations. Good agreement was found between modeled and measured tropospheric NO2 columns, with an average difference of less than 1% of the average tropospheric column (14.5 · 1015 molec cm−2). The comparisons show little cloud cover dependence after cloud corrections for which ceilometer data were used. Hourly differences between observations and model show a Gaussian behavior with a standard deviation (σ) of 5.5 · 1015 molec cm−2. For daily averages of tropospheric NO2 columns, a correlation of 0.72 was found for all observations, and 0.79 for cloud free conditions. The measured and modeled tropospheric NO2 columns have an almost identical distribution over the wind direction. A significant difference between model and measurements was found for the average weekly cycle, which shows a much stronger decrease during the weekend for the observations; for the diurnal cycle, the observed range is about twice as large as the modeled range. The results of the comparison demonstrate that averaged over a long time period, the tropospheric NO2 column observations are representative for a large spatial area despite the fact that they were obtained in an urban region. This makes the MAX-DOAS technique especially suitable for validation of satellite observations and air quality models in urban regions.
- Published
- 2015
13. MAX-DOAS observations of aerosols, formaldehyde and nitrogen dioxide in the Beijing area: Comparison of two profile retrieval approaches
- Author
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Vlemmix, T. (author), Hendrick, F. (author), Pinardi, G. (author), De Smedt, I. (author), Fayt, C. (author), Hermans, C. (author), Piters, A. (author), Wang, P. (author), Levelt, P.F. (author), Van Roozendael, M. (author), Vlemmix, T. (author), Hendrick, F. (author), Pinardi, G. (author), De Smedt, I. (author), Fayt, C. (author), Hermans, C. (author), Piters, A. (author), Wang, P. (author), Levelt, P.F. (author), and Van Roozendael, M. (author)
- Abstract
A 4-year data set of MAX-DOAS observations in the Beijing area (2008–2012) is analysed with a focus on NO2, HCHO and aerosols. Two very different retrieval methods are applied. Method A describes the tropospheric profile with 13 layers and makes use of the optimal estimation method. Method B uses 2–4 parameters to describe the tropospheric profile and an inversion based on a least-squares fit. For each constituent (NO2, HCHO and aerosols) the retrieval outcomes are compared in terms of tropospheric column densities, surface concentrations and "characteristic profile heights" (i.e. the height below which 75% of the vertically integrated tropospheric column density resides). We find best agreement between the two methods for tropospheric NO2 column densities, with a standard deviation of relative differences below 10%, a correlation of 0.99 and a linear regression with a slope of 1.03. For tropospheric HCHO column densities we find a similar slope, but also a systematic bias of almost 10% which is likely related to differences in profile height. Aerosol optical depths (AODs) retrieved with method B are 20% high compared to method A. They are more in agreement with AERONET measurements, which are on average only 5% lower, however with considerable relative differences (standard deviation ~ 25%). With respect to near-surface volume mixing ratios and aerosol extinction we find considerably larger relative differences: 10 ± 30, ?23 ± 28 and ?8 ± 33% for aerosols, HCHO and NO2 respectively. The frequency distributions of these near-surface concentrations show however a quite good agreement, and this indicates that near-surface concentrations derived from MAX-DOAS are certainly useful in a climatological sense. A major difference between the two methods is the dynamic range of retrieved characteristic profile heights which is larger for method B than for method A. This effect is most pronounced for HCHO, where retrieved profile shapes with method A are very close to the a p, Geoscience & Remote Sensing, Civil Engineering and Geosciences
- Published
- 2015
- Full Text
- View/download PDF
14. Impact of aerosols on the OMI tropospheric NO2 retrievals over industrialized regions: How accurate is the aerosol correction of cloud-free scenes via a simple cloud model? (discussion paper)
- Author
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Chimot, J.J. (author), Vlemmix, T. (author), Veefkind, J.P. (author), De Haan, J.F. (author), Levelt, P.F. (author), Chimot, J.J. (author), Vlemmix, T. (author), Veefkind, J.P. (author), De Haan, J.F. (author), and Levelt, P.F. (author)
- Abstract
The Ozone Monitoring Instrument (OMI) instrument has provided daily global measurements of tropospheric NO2 for more than a decade. Numerous studies have drawn attention to the complexities related to measurements of tropospheric NO2 in the presence of aerosols. Fine particles affect the OMI spectral measurements and the length of the average light path followed by the photons. However, they are not explicitly taken into account in the current OMI tropospheric NO2 retrieval chain. Instead, the operational OMI O2-O2 cloud retrieval algorithm is applied both to cloudy scenes and to cloud free scenes with aerosols present. This paper describes in detail the complex interplay between the spectral effects of aerosols, the OMI O2-O2 cloud retrieval algorithm and the impact on the accuracy of the tropospheric NO2 retrievals through the computed Air Mass Factor (AMF) over cloud-free scenes. Collocated OMI NO2 and MODIS Aqua aerosol products are analysed over East China, in industrialized area. In addition, aerosol effects on the tropospheric NO2 AMF and the retrieval of OMI cloud parameters are simulated. Both the observation-based and the simulation-based approach demonstrate that the retrieved cloud fraction linearly increases with increasing Aerosol Optical Thickness (AOT), but the magnitude of this increase depends on the aerosol properties and surface albedo. This increase is induced by the additional scattering effects of aerosols which enhance the scene brightness. The decreasing effective cloud pressure with increasing AOT represents primarily the absorbing effects of aerosols. The study cases show that the actual aerosol correction based on the implemented OMI cloud model results in biases between ?20 and ?40 % for the DOMINO tropospheric NO2 product in cases of high aerosol pollution (AOT ? 0.6) and elevated particles. On the contrary, when aerosols are relatively close to the surface or mixed with NO2, aerosol correction based on the cloud model results in overes, Geoscience & Remote Sensing, Civil Engineering and Geosciences
- Published
- 2015
15. NOx emission estimates during the 2014 Youth Olympic Games in Nanjing
- Author
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Ding, J. (author), Van der A, R.J. (author), Mijling, B. (author), Levelt, P.F. (author), Hao, N. (author), Ding, J. (author), Van der A, R.J. (author), Mijling, B. (author), Levelt, P.F. (author), and Hao, N. (author)
- Abstract
The Nanjing Government applied temporary environmental regulations to guarantee good air quality during the Youth Olympic Games (YOG) in 2014. We study the effect of those regulations by applying the emission estimate algorithm DECSO (Daily Emission estimates Constrained by Satellite Observations) to measurements of the Ozone Monitoring Instrument (OMI). We improved DECSO by updating the chemical transport model CHIMERE from v2006 to v2013 and by adding an Observation minus Forecast (OmF) criterion to filter outlying satellite retrievals due to high aerosol concentrations. The comparison of model results with both ground and satellite observations indicates that CHIMERE v2013 is better performing than CHIMERE v2006. After filtering the satellite observations with high aerosol loads that were leading to large OmF values, unrealistic jumps in the emission estimates are removed. Despite the cloudy conditions during the YOG we could still see a decrease of tropospheric NO2 column concentrations of about 32 % in the OMI observations when compared to the average NO2 columns from 2005 to 2012. The results of the improved DECSO algorithm for NOx emissions show a reduction of at least 25 % during the YOG period and afterwards. This indicates that air quality regulations taken by the local government have an effect in reducing NOx emissions. The algorithm is also able to detect an emission reduction of 10 % during the Chinese Spring Festival. This study demonstrates the capacity of the DECSO algorithm to capture the change of NOx emissions on a monthly scale. We also show that the observed NO2 columns and the derived emissions show different patterns that provide complimentary information. For example, the Nanjing smog episode in December 2013 led to a strong increase in NO2 concentrations without an increase in NOx emissions. Furthermore, DECSO gives us important information on the non-trivial seasonal relation between NOx emissions and NO2 concentrations on a local scale., Geoscience & Remote Sensing, Civil Engineering and Geosciences
- Published
- 2015
16. OMI tropospheric NO2 profiles from cloud slicing: Constraints on surface emissions, convective transport and lightning NOx (discussion paper)
- Author
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Belmonte Rivas, M. (author), Veefkind, J.P. (author), Eskes, H. (author), Levelt, P.F. (author), Belmonte Rivas, M. (author), Veefkind, J.P. (author), Eskes, H. (author), and Levelt, P.F. (author)
- Abstract
We derive a global climatology of tropospheric NO2 profiles from OMI cloudy observations for the year 2006 using the cloud slicing method on six pressure levels centered about 280, 380, 500, 620, 720 and 820 hPa. A comparison between OMI and the TM4 model tropospheric NO2 profiles reveals striking overall similarities, which confer great confidence to the cloud-slicing approach, along with localized discrepancies that seem to probe into particular model processes. Anomalies detected at the lowest levels can be traced to deficiencies in the model surface emission inventory, at mid tropospheric levels to convective transport and horizontal advective diffusion, and at the upper tropospheric levels to model lightning NOx production and the placement of deeply transported NO2 plumes such as from the Asian summer monsoon. The vertical information contained in the OMI cloud-sliced NO2 profiles provides a global observational constraint that can be used to evaluate chemistry transport models (CTMs) and guide the development of key parameterization schemes., Geoscience & Remote Sensing, Civil Engineering and Geosciences
- Published
- 2015
17. TROPOMI on the ESA Sentinel-5 Precursor: A GMES mission for global observations of the atmospheric composition for climate, air quality and ozone layer applications
- Author
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Veefkind, J.P., Aben, I., McMullan, K., Förster, H., Vries, J. de, Otter, G., Claas, J., Eskes, H.J., Haan, J.F. de, Kleipool, Q., Weele, M. van, Hasekamp, O., Hoogeveen, R., Landgraf, J., Snel, R., Tol, P., Ingmann, P., Voors, R., Kruizinga, B., Vink, R., Visser, H., and Levelt, P.F.
- Subjects
Earth observation ,OM - Opto-Mechatronics ,TS - Technical Sciences ,Industrial Innovation ,Atmospheric composition ,Ozone layer ,Climate ,Satellite remote sensing ,Air quality ,Mechatronics, Mechanics & Materials ,Aviation - Abstract
The ESA (European Space Agency) Sentinel-5 Precursor (S-5 P) is a low Earth orbit polar satellite to provide information and services on air quality, climate and the ozone layer in the timeframe 2015-2022. The S-5 P mission is part of the Global Monitoring of the Environment and Security (GMES) Space Component Programme. The payload of the mission is the TROPOspheric Monitoring Instrument (TROPOMI) that will measure key atmospheric constituents including ozone, NO2, SO2, CO, CH4, CH2O and aerosol properties. TROPOMI has heritage to both the Ozone Monitoring Instrument (OMI) as well as to the SCanning Imaging Absorption spectroMeter for Atmospheric CartograpHY (SCIAMACHY). The S-5 P will extend the data records of these missions as well as be a preparatory mission for the Sentinel-5 mission planned for 2020 onward. The mission is pre-operational and is the link between the current scientific and the operational Sentinel-4/-5 missions. This contribution describes the science and mission objectives, the mission and the instrument, and the data products. While building on a solid foundation of the heritage instruments, the S-5P/TROPOMI mission is an exciting step forward with a strong focus on the troposphere. This is achieved by a combination of a high spatial resolution and improved signal-to-noise, as well as dedicated data product development. It is anticipated that the S-5 P mission will make a large contribution to the monitoring of the global atmospheric composition, as well as to the scientific knowledge of relevant atmospheric processes. © 2012 Elsevier Inc.
- Published
- 2012
18. Retrieval of tropospheric NO₂ using the MAX-DOAS method combined with relative intensity measurements for aerosol correction
- Author
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Vlemmix, T., Piters, A.J.M., Stammes, P., Wang, P., Levelt, P.F., and Fluids and Flows
- Abstract
Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) is a technique to measure trace gas amounts in the lower troposphere from ground-based scattered sunlight observations. MAX-DOAS observations are especially suitable for validation of tropospheric trace gas observations from satellite, since they have a representative range of several kilometers, both in the horizontal and in the vertical dimension. A two-step retrieval scheme is presented here, to derive aerosol corrected tropospheric NO2 columns from MAX-DOAS observations. In a first step, boundary layer aerosols, characterized in terms of aerosol optical thickness (AOT), are estimated from relative intensity observations, which are defined as the ratio of the sky radiance at elevation a and the sky radiance in the zenith. Relative intensity measurements have the advantage of a strong dependence on boundary layer AOT and almost no dependence on boundary layer height. In a second step, tropospheric NO2 columns are derived from differential slant columns, based on AOT-dependent air mass factors. This two-step retrieval scheme was applied to cloud free periods in a twelve month data set of observations in De Bilt, The Netherlands. In a comparison with AERONET (Cabauw site) a mean difference in AOT (AERONET minus MAX-DOAS) of -0.01±0.08 was found, and a correlation of 0.85. Tropospheric-NO2 columns were compared with OMI-satellite tropospheric NO2. For ground-based observations restricted to uncertainties below 10%, no significant difference was found, and a correlation of 0.88.
- Published
- 2010
19. MAX-DOAS observations of aerosols, formaldehyde and nitrogen dioxide in the Beijing area: Comparison of two profile retrieval approaches
- Author
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Vlemmix, T. (author), Hendrick, F. (author), Pinardi, G. (author), De Smedt, I. (author), Fayt, C. (author), Hermans, C. (author), Piters, A. (author), Wang, P. (author), Levelt, P.F. (author), Van Roozendael, M. (author), Vlemmix, T. (author), Hendrick, F. (author), Pinardi, G. (author), De Smedt, I. (author), Fayt, C. (author), Hermans, C. (author), Piters, A. (author), Wang, P. (author), Levelt, P.F. (author), and Van Roozendael, M. (author)
- Abstract
A four year data set of MAX-DOAS observations in the Beijing area (2008–2012) is analysed with a focus on NO2, HCHO, and aerosols. Two very different retrieval methods are applied. Method A describes the tropospheric profile with 13 layers and makes use of the optimal estimation method. Method B uses 2–4 parameters to describe the tropospheric profile and an inversion based on a least-squares fit. For each constituent (NO2, HCHO and aerosols) the retrieval outcomes are compared in terms of tropospheric columns, surface concentrations, and "characteristic profile heights" (i.e. the height below which 75% of the vertically integrated tropospheric column resides). We find best agreement between the two methods for tropospheric NO2 columns, with a standard deviation of relative differences below 10%, a correlation of 0.99 and a linear regression with a slope of 1.03. For tropospheric HCHO columns we find a similar slope, but also a systematic bias of almost 10% which is likely related to differences in profile height. Aerosol optical depths (AODs) retrieved with method B are 20% high compared to method A. They are more in agreement with AERONET measurements, which are on average only 5% lower, however with considerable relative differences (standard deviation ~25%). With respect to near surface volume mixing ratios and aerosol extinction we find considerably larger relative differences: 10 ± 30%, ?23 ± 28% and ?8 ± 33% for aerosols, HCHO and NO2 respectively. The frequency distributions of these near-surface concentrations show however a quite good agreement, and this indicates that near-surface concentrations derived from MAX-DOAS are certainly useful in a climatological sense. A major difference between the two methods is the dynamic range of retrieved characteristic profile heights which is larger for method B than for method A. This effect is most pronounced for HCHO, where retrieved profile shapes with method A are very close to the a priori, and moderate for NO2 a, Geoscience & Remote Sensing, Civil Engineering and Geosciences
- Published
- 2014
- Full Text
- View/download PDF
20. Ozone Profile Retrieval Algorithm (OPERA) for nadir-looking satellite instruments in the UV-VIS
- Author
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Van Peet, J.C.A. (author), Van der A, R.J. (author), Tuinder, O.N.E. (author), Wolfram, E. (author), Salvador, J. (author), Levelt, P.F. (author), Kelder, H.M. (author), Van Peet, J.C.A. (author), Van der A, R.J. (author), Tuinder, O.N.E. (author), Wolfram, E. (author), Salvador, J. (author), Levelt, P.F. (author), and Kelder, H.M. (author)
- Abstract
For the retrieval of the vertical distribution of ozone in the atmosphere the Ozone ProfilE Retrieval Algorithm (OPERA) has been further developed. The new version (1.26) of OPERA is capable of retrieving ozone profiles from UV–VIS observations of most nadir-looking satellite instruments like GOME, SCIAMACHY, OMI and GOME-2. The setup of OPERA is described and results are presented for GOME and GOME-2 observations. The retrieved ozone profiles are globally compared to ozone sondes for the years 1997 and 2008. Relative differences between GOME/GOME-2 and ozone sondes are within the limits as specified by the user requirements from the Climate Change Initiative (CCI) programme of ESA (20%in the troposphere, 15% in the stratosphere). To demonstrate the performance of the algorithm under extreme circumstances, the 2009 Antarctic ozone hole season was investigated in more detail using GOME-2 ozone profiles and lidar data, which showed an unusual persistence of the vortex over the Río Gallegos observing station (51 S, 69.3 W). By applying OPERA to multiple instruments, a time series of ozone profiles from 1996 to 2013 from a single robust algorithm can be created, Geoscience and Remote Sensing, Civil Engineering and Geosciences
- Published
- 2014
- Full Text
- View/download PDF
21. Evaluation of broadband surface solar irradiance derived from the Ozone Monitoring Instrument
- Author
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Wang, P. (author), Sneep, M. (author), Veefkind, J.P. (author), Stammes, P. (author), Levelt, P.F. (author), Wang, P. (author), Sneep, M. (author), Veefkind, J.P. (author), Stammes, P. (author), and Levelt, P.F. (author)
- Abstract
Surface solar irradiance (SSI) data are important for planning and estimating the production of solar power plants. Long-term high quality surface solar radiation data are needed for monitoring climate change. This paper presents a new surface solar irradiance dataset, the broadband (0.2–4 ?m) surface solar irradiance product derived from the Ozone Monitoring Instrument (OMI). The OMI SSI algorithm is based on the Heliosat method and uses the OMI O2–O2 cloud product as main input. The OMI SSI data are validated against the globally distributed Baseline Surface Radiation Network (BSRN) measurements at 19 stations for the year 2008. Furthermore, the monthly mean OMI SSI data are compared to independent surface solar irradiance products from International Satellite Cloud Climatology Project Flux Data (ISCCP-FD) and Clouds and the Earth's Radiant Energy System (CERES) data for the year 2005. The mean difference between OMI SSI and BSRN global (direct + diffuse) irradiances is ? 1.2 W m? 2 (? 0.2%), the root mean square error is 100.1 W m? 2 (18.1%), and the mean absolute error is 67.8 W m? 2 (12.2%). The differences between OMI SSI and BSRN global irradiances are smaller over continental and coastal sites and larger over deserts and islands. OMI SSI has a good agreement with the CERES shortwave (SW) model B surface downward flux (SDF) product. The correlation coefficient and index of agreement between monthly mean 1-degree gridded OMI SSI and CERES SW SDF are > 0.99. OMI SSI is lower than CERES SW SDF which is partly due to the solar zenith angle. On average, OMI SSI is 13.5 W m? 2 (2.5%) lower than the ISCCP-FD SW surface downward flux and the correlation coefficient and index of agreement are > 0.98 for every month., Geoscience & Remote Sensing, Civil Engineering and Geosciences
- Published
- 2014
- Full Text
- View/download PDF
22. NOx emission estimates during the 2014 Youth Olympic Games in Nanjing (discussion paper)
- Author
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Ding, J. (author), Van der A, R.J. (author), Mijling, B. (author), Levelt, P.F. (author), Hao, N. (author), Ding, J. (author), Van der A, R.J. (author), Mijling, B. (author), Levelt, P.F. (author), and Hao, N. (author)
- Abstract
The Nanjing Government has taken temporary environmental regulations to guarantee good air quality during the Youth Olympic Games (YOG) in 2014. We study the effect of those regulations by applying the emission estimate algorithm DECSO (Daily Emission estimates Constrained by Satellite Observations) to measurements of the Ozone Monitoring Instrument (OMI). We improved DECSO by updating the chemical transport model CHIMERE from v2006 to v2013 and by adding an Observation minus Forecast (OmF) criterion to filter outlying satellite retrievals due to high aerosol concentrations. The comparison of model results with both ground and satellite observations indicates that CHIMERE v2013 is better performing than CHIMERE v2006. After filtering the satellite observations with high aerosol loads that were leading to large OmF values, unrealistic jumps in the emission estimates are removed. Despite the cloudy conditions during the YOG we could still see a decrease of tropospheric NO2 column concentrations of about 32% in the OMI observations as compared to the average NO2 concentrations from 2005 to 2012. The results of the improved DECSO algorithm for NOx emissions show a reduction of at least 25% during the YOG period. This indicates that air quality regulations taken by the local government were successful. The algorithm is also able to detect an emission reduction of 10% during the Chinese Spring Festival. This study demonstrates the capacity of the DECSO algorithm to capture the change of NOx emissions on a monthly scale. We also show that the observed concentrations and the derived emissions show different patterns that provide complimentary information. For example, the Nanjing smog episode in December 2013 led to a strong increase in NO2 concentrations without an increase in NOx emissions. Furthermore, DECSO gives us important information of the non-trivial seasonal relation between NOx emissions and NO2 concentrations on a local scale., Geoscience & Remote Sensing, Civil Engineering and Geosciences
- Published
- 2014
- Full Text
- View/download PDF
23. ESA CAMELOT study : Challenges in future operational missions for GMES atmospheric monitoring, sentinel 4 and 5
- Author
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Levelt, P.F., Veefkind, J.P., and Fluids and Flows
- Abstract
No abstract.
- Published
- 2009
24. MAX-DOAS aerosol corrected tropospheric vertical columns of nitrogen dioxide
- Author
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Vlemmix, T., Piters, A.J.M., Stammes, P., Wang, P., Levelt, P.F., Apituley, A., Russchenberg, H.W.J., Monna, W.A.A., and Fluids and Flows
- Abstract
Nitrogen Dioxide (NO2) is an important component of air pollution. It is observed on a global scale by satellite instruments such as GOME, SCIAMACHY and OMI. Worldwide there are only few observation sites where nitrogen dioxide tropospheric columns are monitored on an operational basis. For satellite validation it is essential to perform these ground based measurements with good global and seasonal coverage preferably in a network of similar and intercalibrated instruments. Since November 2007 multiaxis differential optical absorption spectroscopy (MAXDOAS) observations of NO2 are performed on an operational basis at the Royal Netherlands Meteorological Institute (KNMI). For this a Mini MAX-DOAS instrument is used. This relatively low cost instrument could be a candidate for a global network as mentioned above. We will explain the tropospheric column retrieval algorithm which includes a correction for aerosols. The Doubling Adding radiative transfer model is used to create look up tables for the Air Mass Factors as a function of radiation intensity which depends on aerosol optical thickness (AOT) and boundary layer height. In addition we will show results from several studies based on the observations. First: a comparison of retrieved AOT and direct sun observations of AOT from the CESAR site in Cabauw, The Netherlands. Second: an analysis of the retrieved tropospheric vertical columns of NO2 in this highly polluted region. Third: comparison with SCIAMACHY and OMI tropospheric NO2 columns. Finally: first results from the CINDI inter-comparison campaign for NO2 measuring instruments. This campaign has taken place in Cabauw, in June and July 2009. Many different groups have participate in this campaign which had resulted in a variety of simultaneous in-situ and remote sensing observations of NO2, other trace gases and aerosols.
- Published
- 2009
25. Operational MAX-DOAS tropospheric column observations of NO_2 used for validation of OMI and SCIAMACHY
- Author
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Vlemmix, T., Piters, A.J.M., Levelt, P.F., Wang, P., Stammes, P., and Fluids and Flows
- Abstract
only.
- Published
- 2009
26. ESA CAMELOT study : Challenges in future operational missions for GMES atmospheric monitoring sentinels 4 and 5 and S5p
- Author
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Levelt, P.F., Veefkind, J.P., Kerridge, B.J., Siddans, R., De Leeuw, G., Remedios, J., Coheur, P.-F., and Fluids and Flows
- Subjects
SDG 13 - Climate Action - Abstract
This is the final report of the CAMELOT (Chemistry of the Atmosphere Mission concEpts and sentineL Observations Techniques) study. The key objective of the CAMELOT study was to contribute to the definition of the air quality and climate protocol monitoring parts of GMES Sentinels 4 and 5 missions. This report presents the conclusions and recommendations of this study, regarding the Sentinel 4 and 5 Level 1B requirements and the mission scenario’s.
- Published
- 2009
27. Improving retrieval of volcanic sulphur dioxide from backscattered UV satellite observations
- Author
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Yang, Kai, Krotkov, N.A., Krueger, A.J., Carn, S.A., Bhartia, P.K., Levelt, P.F., and Fluids and Flows
- Abstract
Existing algorithms that use satellite measurements of solar backscattered ultraviolet (BUV) radiances to retrieve sulfur dioxide (SO2) vertical columns underestimate the large SO2 amounts encountered in fresh volcanic eruption clouds. To eliminate this underestimation we have developed a new technique, named the Iterative Spectral Fitting (ISF) algorithm, for accurate retrieval of SO2 vertical columns in the full range of volcanic emissions. The ISF algorithm is applied to Ozone Monitoring Instrument (OMI) BUV measurements of the Sierra Negra eruption (Galàpagos Islands, Ecuador) in October 2005. The results represent major improvements over the operational OMI SO2 products. Based on the ISF data, we report the largest SO2 vertical column amount (>1000 Dobson Units (DU), where 1 DU = 2.69 × 1016 molecules/cm2) ever observed by a space borne instrument, implying that very high concentrations of SO2 can occur in the lower troposphere during effusive eruptions.
- Published
- 2009
28. Sensing the Troposphere from Space
- Author
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Levelt, P.F., Veefkind, J.P., Dobber, M.R., Boersma, F., Eskes, H.J., Weele, van, M., Aben, I., Clerbaux, C., Camy-Peyret, C., Coheur, P.-F., Bhartia, P.K., Tamminen, J., Apituley, A., Russchenberg, H.W.J., and Fluids and Flows
- Subjects
SDG 13 - Climate Action ,SDG 11 - Sustainable Cities and Communities - Abstract
The growth of human population and the industrialisation in the 19th and 20th century has led to dramatic changes in the Earth System. The chemical composition of the lowest part of the atmosphere, the troposphere, is changing as a result of human activities. The Earth has entered the "Anthropocene" epoch, where the activities of humans play a key role in air quality and climate change. The rapid development of megacities (see Figure 1) and the strong development in the Asian countries are clear examples of rapid changes that affected the atmosphere in the last decades and will continue to do so in the future. For understanding climate change and air quality, global changes in the chemical composition of the troposphere need to be taken into account/addressed. Especially the global inventory of emission sources play a key role in understanding and modelling the troposphere in relation to climate change and air pollution. Also regional and long-range transport of pollution, as well as the rapid development of pollution levels during the day, are important for understanding air quality and climate change and their interaction Atmospheric measurements from space started in the 70th’s with US sensors SBUV[)] and TOMS[2], focussing on the ozone layer residing in the higher layers in the atmosphere. Sensing the lower atmospheric layers from space is a recent development in satellite remote sensing, where SCIAMACHY[[3]] on board ESA’s ENVISAT), OMI[4] on board NASA’s EOS-Aura) and GOME-2[5] (on board METOP-1) instruments play a leading role. Unprecedented measurements from space from OMI reveal tropospheric pollution maps on a daily basis with urban scale resolution. Measurements from Thermal Infrared instruments like MOPITT [6], AIRS[7] , IASI[[8]] and TES[[9]] also provide unique information on the troposphere, providing tropospheric profile information. In this paper an overview will be given of satellite measurements from space of the chemical composition of the troposphere and their role in climate change and air pollution. Also challenges and future developments for tropospheric measurements from space will be discussed, including the Dutch initiative satellite instrument (TROPOMI) for detection of the tropospheric composition.
- Published
- 2009
29. TROPOMI end-to-end performance studies
- Author
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Voors, R., Vries, de, J., Veefkind, J.P., Gloudemans, A., Mika, A., Levelt, P.F., Meynart, R., Shimoda, H., Habib, S., and Fluids and Flows
- Subjects
Ozone Monitoring Instrument ,Geography ,Spectrometer ,Meteorology ,Imaging spectrometer ,Nadir ,Air quality index ,Spectrograph ,SCIAMACHY ,Remote sensing ,Trace gas - Abstract
The TROPOspheric Monitoring Instrument (TROPOMI) is a UV/VIS/NIR/SWIR non-scanning nadir viewing imaging spectrometer that combines a wide swath (110°) with high spatial resolution (8 x 8 km). Its main heritages are from the Ozone Monitoring Instrument (OMI) and from SCIAMACHY. Since its launch in 2004 OMI has been providing, on a daily basis and on a global scale, a wealth of data on ozone, NO 2 and minor trace gases, aeros ols and local pollution, a scanning spectrometer launched in 2004. The TROPOMI UV/VIS/NIR and SWIR heritage is a combination of OMI and SCIAMACHY. In the framework of development programs for a follow-up mission for the successful Ozone Monitoring Instrument, we have developed the so-called TROPOMI Integrated Development Environment. This is a GRID based software simulation tool for OMI follow-up missions. It includes scene generation, an instrument simulator, a level 0-1b processing chain, as well as several level 1b-2 processing chai ns. In addition it contains an error-analyzer, i.e. a tool to feedback the level 2 results to th e input of the scene generator. The paper gives a description of the TROPOMI instrument and focuses on design aspects as well as on the performance, as tested in the end-to-end development environment TIDE. Keywords: TROPOMI, Air Quality, Grid Assist, TIDE, spectrograph
- Published
- 2008
30. Breadboarding activities of the TROPOMI-SWIR module
- Author
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Hoogeveen, R.W.M., Jongma, R.T., Tol, P.J.J., Gloudemans, A., Aben, I., Vries, J.de, Visser, H., Boslooper, E.C., Dobber, M., Levelt, P.F., and TNO Industrie en Techniek
- Subjects
Optical instrument lenses ,Short-wave infrared ,Troposphere ,Optical instrumentation ,Space technology ,Remote sensing ,Aviation ,Carbon monoxide ,Immersed grating ,Methane - Abstract
The TROPOMI instrument concept is part of the TRAQ mission proposal to ESA in response to the Call for Ideas in 2005. TRAQ (TRopospheric composition and Air Quality) has been accepted for a further pre-phase A study for the next Earth Explorer core Mission. A very similar instrument has been proposed for the CAMEO platform to the US National Research Council decadal study, which has also been accepted for further study. TROPOMI is a nadir-viewing grating-based imaging spectrometer using the Dutch OMI and SCIAMACHY heritage. It includes an UV-VIS-NIR module that consists of three UV-VIS channels continuously covering the 270-490 nm range to determine O3, NO2, HCHO, SO 2, aerosols and a NIR-channel covering 710-775 nm for cloud detection and information on the aerosol height distribution using the oxygen A band. TROPOMI also includes a SWIR module covering 2305-2385 nm that mainly focuses on determination of CO and CH4 total columns. All species are measured with sensitivity down to the Earth's surface, thus addressing issues of anthropogenic emissions and their impact on air quality and climate. In the TRAQ mission, unique diurnal time sampling with up to 5 daytime observations over midlatitude regions (Europe, North-America, China) is foreseen by using a non-sun-synchronous, medium-inclination drifting orbit and a 2600 km wide observational swath. Several more general aspects related to the TROPOMI instrument are discussed in a separate paper in this conference. This paper focuses on the development of the SWIR module. A breadboard model (BBM) has been designed and constructed which is as much as possible functionally flight representative. Critical technologies to be demonstrated with the BBM are the SWIR HgCdTe-based 2D focal plane array, the on-board SWIR calibration LED, and in particular, the SRON/TNO developed silicon-based immersed grating that allows a hugely reduced instrument volume. In the presentation the results of a performance analysis of the TROPOMI-S WIR channel will be discussed, as well as results of the detector characterization program on a representative off-the-shelf FPA, and details of the photolithographic production of the immersed grating.
- Published
- 2007
31. SO2 data from the ozone monitoring instrument
- Author
-
Krotkov, N.A., Yang, K., Krueger, A.J., Carn, S.A., Bhartia, P.K., Levelt, P.F., Lacoste, H., Ouwehand, L., and Fluids and Flows
- Abstract
We discuss collection 2 SO2 data from the Dutch-Finnish Ozone Monitoring Instrument (OMI) on board NASA EOS/Aura spacecraft and show examples of detected volcanic and anthropogenic SO2 emissions. Quantification of anthropogenic SO2 emissions requires collection 3 reprocessing available in the fall 2007.
- Published
- 2007
32. TROPOMI: Solar backscatter satellite instrument for air quality and climate
- Author
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Vries, de, J., Laan, E.C., Hoogeveen, R.W.M., Jongma, R.T., Aben, I., Visser, H.J., Boslooper, E., Saari, H., Dobber, M.R., Veefkind, J.P., Kleipool, Q., Levelt, P.F., Meyneart, R., Neeck, S.P., Electromagnetics, and Fluids and Flows
- Subjects
Backscatter ,Meteorology ,Albedo ,Orbital mechanics ,Remote sensing ,air quality ,SCIAMACHY ,law.invention ,Troposphere ,Telescope ,law ,Environmental science ,Satellite ,Spectrograph ,space instuments ,climate - Abstract
TROPOMI is a nadir-viewing grating-based imaging spectrograph in the line of OMI and SCIAMACHY. TROPOMI is part of the ESA Candidate Core Explorer Mission proposal TRAQ and also of the CAMEO satellite proposed for the US NRC decadal study. A TROPOMI-like instrument is part of the ESA/EU Sentinel 4&5 pre-phase A studies. TROPOMI covers the OMI wavelengths of 270-490 nm to measure O3, NO2, HCHO, SO2 and aerosols and adds a NIR channel and a SWIR module. The NIR-channel (710-775 nm) is used for improved cloud detection and aerosol height distribution. The SWIR module (2305 - 2385 nm) measures CO and CH4 and forms a separate module because of its thermal requirements. TROPOMI is a non-scanning instrument with an OMI-like telescope but optimized to have smaller ground pixels (10 × 10 km2) and sufficient signal-to-noise for dark scenes (albedo 2 %). TROPOMI has the same wide swath as OMI (2600 km). In TRAQ's mid-inclination orbit, this allows up to 5 daytime observations over mid-latitude regions (Europe, North-America, China). The paper gives a description of the TROPOMI instrument and focuses on several important aspects of the design, for example the sun calibration and detector selection status. U7 - Export Date: 2 August 2010 U7 - Source: Scopus U7 - Art. No.: 674409
- Published
- 2007
- Full Text
- View/download PDF
33. Aerosol properties from OMI using the multi-wavelength algorithm
- Author
-
Veihelmann, B., Veefkind, J.P., Braak, R., Levelt, P.F., Haan, de, J.F., Lacoste, H., Ouwehand, L., and Fluids and Flows
- Abstract
The multi-wavelength retrieval algorithm is used to retrieve aerosol parameters from spectra reflectance measurements of the Ozone Monitoring Instrument (OMI). This retrieval algorithm uses up to 19 wavelength bands between 331 nm and 500 nm including a band at 477 nm comprising an absorption band of O2-O2. This absorption band has been included in order to increase the amount of height information that can be extracted from the measurement. A principal component analysis shows that OMI measurements have 2 to 4 degrees of freedom of signal, which for cloud free scenes can be attributed to aerosol parameters. In the multi-wavelength algorithm the aerosol optical thickness at a reference wavelength is retrieved for a set of aerosol models and the best fitting aerosol model is determined. The aerosol models are determined by the single-scattering albedo, the layer height, and the size distribution. The algorithm is capable to distinguish between absorbing aerosol types, such as desert dust and biomass burning, and weakly absorbing aerosols like sea-salt and sulfates. We show retrieved aerosol parameters for various scenes and conditions. Furthermore we show how height information from space borne lidar instruments (e.g. CALIPSO) can be used in the OMI retrievals. U7 - Export Date: 2 August 2010 U7 - Source: Scopus
- Published
- 2007
34. Validation of OMI TOMS-V8 total ozone columns using a data assimilation system
- Author
-
Migliorini, S., Brugge, R., O'Neill, A., Dobber, M.R., Levelt, P.F., McPeters, R., Lacoste, H., Ouwehand, L., and Fluids and Flows
- Abstract
In this paper the OMI ozone column measurements obtained with the TOMS-V8 total ozone algorithm are evaluated against OMI ozone columns simulated by means of ozone analyses resulting from assimilation of standard meteorological observations as well as independent ozone retrievals into a numerical weather prediction model. Intercomparison results between measured versus simulated OMI ozone columns at sza
- Published
- 2007
35. TROPOMI: Solar backscatter satellite instrument for air quality and climate
- Author
-
Vries, J.de, Laan, E.C., Hoogeveen, R.W.M., Jongma, R.T., Aben, U., Visser, H., Boslooper, E.C., Saari, H., Dobber, M., Veefkind, P., Kleipool, Q., Levelt, P.F., and TNO Industrie en Techniek
- Subjects
Ultraviolet spectrographs ,NIR channel ,Satellites ,Climate ,Troposphere ,UV-Visible ,Wavelength ,Air quality ,Imaging systems ,Backscattering ,Aviation ,Trace gas - Abstract
TROPOMI is a nadir-viewing grating-based imaging spectrograph in the line of OMI and SCIAMACHY. TROPOMI is part of the ESA Candidate Core Explorer Mission proposal TRAQ and also of the CAMEO satellite proposed for the US NRC decadal study. A TROPOMI-like instrument is part of the ESA/EU Sentinel 4&5 pre-phase A studies. TROPOMI covers the OMI wavelengths of 270-490 nm to measure O3, NO2, HCHO, SO2 and aerosols and adds a NIR channel and a SWIR module. The NIR-channel (710-775 nm) is used for improved cloud detection and aerosol height distribution. The SWIR module (2305 - 2385 nm) measures CO and CH4 and forms a separate module because of its thermal requirements. TROPOMI is a non-scanning instrument with an OMI-like telescope but optimized to have smaller ground pixels (10 × 10 km2) and sufficient signal-to-noise for dark scenes (albedo 2 %). TROPOMI has the same wide swath as OMI (2600 km). In TRAQ's mid-inclination orbit, this allows up to 5 daytime observations over mid-latitude regions (Europe, North-America, China). The paper gives a description of the TROPOMI instrument and focuses on several important aspects of the design, for example the sun calibration and detector selection status.
- Published
- 2007
36. Sulfur dioxide emissions from Peruvian copper smelters detected by the ozone monitoring instrument
- Author
-
Carn, S.A., Krueger, A.J., Krotkov, N.A., Yang, Kai, Levelt, P.F., and Fluids and Flows
- Abstract
We report the first daily observations of sulfur dioxide (SO2) emissions from copper smelters by a satellite-borne sensor - the Ozone Monitoring Instrument (OMI) on NASA's EOS/Aura spacecraft. Emissions from two Peruvian smelters (La Oroya and Ilo) were detected in up to 80% of OMI overpasses between September 2004 and June 2005. SO2 production by each smelter in this period is assessed and compared with contemporaneous emissions from active volcanoes in Ecuador and southern Colombia. Annual SO2 discharge from the Ilo smelter, La Oroya smelter, and volcanoes in 2004–2005 is estimated and amounts to 0.3-0.1 +0.2, 0.07 ± 0.03, and 1.2 ± 0.5 Tg, respectively. This study confirms OMI's potential as an effective tool for evaluation of anthropogenic and natural SO2 emissions. Smelter plumes transport an array of toxic metals in addition to SO2 and continued monitoring to mitigate health and environmental impacts is recommended.
- Published
- 2007
37. Near-real time retrieval of tropospheric NO₂ from OMI
- Author
-
Boersma, K.F., Eskes, H.J., Veefkind, J.P., Brinksma, E.J., A, van der, R.J., Sneep, M., Oord, van den, G.H.J., Levelt, P.F., Stammes, P., Gleason, J.F., Bucsela, E.J., and Fluids and Flows
- Abstract
We present a new algorithm for the near-real time retrieval – within 3 h of the actual satellite measurement – of tropospheric NO2 columns from the Ozone Monitoring Instrument (OMI). The retrieval is based on the combined retrieval-assimilation-modelling approach developed at KNMI for off-line tropospheric NO2 from the GOME and SCIAMACHY satellite instruments. We have adapted the off-line system such that the required a priori information – profile shapes and stratospheric background NO2 – is now immediately available upon arrival (within 80 min of observation) of the OMI NO2 slant columns and cloud data at KNMI. Slant columns for NO2 are retrieved using differential optical absorption spectroscopy (DOAS) in the 405–465 nm range. Cloud fraction and cloud pressure are provided by a new cloud retrieval algorithm that uses the absorption of the O2-O2 collision complex near 477 nm. On-line availability of stratospheric slant columns and NO2 profiles is achieved by running the TM4 chemistry transport model (CTM) forward in time based on forecast ECMWF meteo and assimilated NO2 information from all previously observed orbits. OMI NO2 slant columns, after correction for spurious across-track variability, show a random error for individual pixels of approximately 0.7×10¹5 molec cm¿². Cloud parameters from OMI's O2-O2 algorithm have similar frequency distributions as retrieved from SCIAMACHY's Fast Retrieval Scheme for Cloud Observables (FRESCO) for August 2006. On average, OMI cloud fractions are higher by 0.011, and OMI cloud pressures exceed FRESCO cloud pressures by 60 hPa. A sequence of OMI observations over Europe in October 2005 shows OMI's capability to track changeable NOx air pollution from day to day in cloud-free situations.
- Published
- 2007
38. OMI observations of the July 2006 smog episode in Europe
- Author
-
Veefkind, J.P., Levelt, P.F., Eskes, H.J., Braak, R., Veihelmann, B., Gleason, J.F., Haan, de, J.F., Brinksma, E.J., Lacoste, H., Ouwehand, L., and Fluids and Flows
- Abstract
No abstract.
- Published
- 2007
39. Validation results from the joint ESA KNMI NIVR calibration and validation announcement of opportunity for the ozone monitoring instrument
- Author
-
Kroon, M., Brinksma, E.J., Balis, D., Ionov, D.V., Sneep, M., Curier, R.L., Tanskanen, A., Zehner, C., Carpay, J., Levelt, P.F., Lacoste, H., Ouwehand, L., and Fluids and Flows
- Abstract
In this paper we report on the progress achieved within the framework of the joint ESA KNMI NIVR Calibration and Validation Announcement of Opportunity for the Ozone Monitoring Instrument aboard the NASA EOS Aura satellite. This OMI AO effort has rendered a wealth of validation results and scientific insights. Herein this contribution only a selection of the validation results is presented.
- Published
- 2007
40. Extended observations of volcanic SO2 and sulfate aerosol in the stratosphere
- Author
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Carn, S.A., Krotkov, N.A., Yang, Kai, Hoff, R.M., Prata, A.J., Krueger, A.J., Loughlin, S.C., Levelt, P.F., and Fluids and Flows
- Subjects
SDG 13 - Climate Action - Abstract
Sulfate aerosol produced after injection of sulfur dioxide (SO2) into the stratosphere by volcanic eruptions can trigger climate change. We present new satellite data from the Ozone Monitoring Instrument (OMI) and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) missions that reveal the composition, structure and longevity of a stratospheric SO2 cloud and derived sulfate layer following a modest eruption (0.2 Tg total S02) of Soufriere Hills volcano, Montserrat on 20 May 2006. The SO2 cloud alone was tracked for over 3 weeks and a distance of over 20 000 km; unprecedented for an eruption of this size. Derived sulfate aerosol at an altitude of ~20 km had circled the globe by 22 June and remained visible in CALIPSO data until at least 6 July. These synergistic NASA A-Train observations permit a new appreciation of the potential effects of frequent, small-to-moderate volcanic eruptions on stratospheric composition and climate. U7 - Export Date: 2 August 2010 U7 - Source: Scopus
- Published
- 2007
41. Sensitivity analysis of a new SWIR-channel measuring tropospheric CH 4 and CO from space
- Author
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Jongma, R.T., Gloudemans, A.M.S., Hoogeveen, R.W.M., Aben, I., Vries, J. de, Escudero-Sanz, I., Oord, G. van den, Levelt, P.F., and TNO Industrie en Techniek
- Subjects
Signal to noise ratio ,Spectrometers ,Troposphere ,Space technology ,Optical design ,Imaging techniques ,Remote sensing ,Immersed grating ,Short-wave infrared ,Space research ,Optical instrumentation ,Instruments ,Carbon monoxide ,Methane ,Imaging spectrometer - Abstract
In preparation for future atmospheric space missions a consortium of Dutch organizations is performing design studies on a nadir viewing grating-based imaging spectrometer using OMI and SCIAMACHY heritage. The spectrometer measures selected species (O3, NO2, HCHO, H2O, SO 2, aerosols (optical depth, type and absorption index), CO and CH4) with sensitivity down to the Earth's surface, thus addressing science issues on air quality and climate. It includes 3 UV-VIS channels continuously covering the 270-490 nm range, a NIR-channel covering the 710-775 nm range, and a SWIR-channel covering the 2305-2385 nm range. This instrument concept is, named TROPOMI, part of the TRAQ-mission proposal to ESA in response to the Call for Earth Explorer Ideas 2005, and, named TROPI, part of the CAMEO-proposal prepared for the US NRC decadal study-call on Earth science and applications from space. The SWIR-channel is optional in the TROPOMI/TRAQ instrument and included as baseline in the TROPI/CAMEO instrument. This paper focuses on derivation of the instrument requirements of the SWIR-channel by presenting the results of retrieval studies. Synthetic detector spectra are generated by the combination of a forward model and an instrument simulator that includes the properties of state-of-the-art detector technology. The synthetic spectra are input to the CO and CH4 IMLM retrieval algorithm originally developed for SCIAMACHY. The required accuracy of the Level-2 SWIR data products defines the main instrument parameters like spectral resolution and sampling, telescope aperture, detector temperature, and optical bench temperature. The impact of selected calibration and retrieval errors on the Level-2 products has been characterized. The current status of the SWIR-channel optical design with its demanding requirements on ground-pixel size, spectral resolution, and signal-to-noise ratio will be presented.
- Published
- 2006
42. From OMI to TROPOMI: entering the realm of air quality from space
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Vries, J. de, Laan, E.C., Levelt, P.F., Oord, G.H.J. van den, Veefkind, J.P., Dobber, M.R., Aben, I., Jongma, R.T., Escudero-Sanz, I., Court, A.J., and TNO Industrie en Techniek
- Subjects
Ultraviolet visible spectroscopy ,Atmospheric chemistry ,Ozone ,Signal to noise ratio ,Air quality ,Boundary layers ,Aviation ,NASA ,Air masses ,Ozone Monitoring Instrument (OMI) ,Albedo areas ,Separate module - Abstract
The Ozone Monitoring Instrument (OMI) on NASA's AURA satellite is one of the first instruments measuring an extensive set of daily air quality parameters from space. This anwers to a growing interest in obtaining space data for the air we breath next to the higher altitude air masses. OMI combines UV-Visible nadir viewing spectroscopy, small ground pixels and daily global coverage. As SCIAMACHY on ENVISAT, it uses the high sensitivity of UV-Visible spectroscopy to the lowest kilometers of the atmosphere and the boundary layer. It has fairly small ground pixels (13 × 24 km2) to allow for a high fraction of cloudfree observations and to help to observing detailed spatial features. Daily measurements form a prerequisite for air quality data. This paper shows examples of OMI air quality measurements and it explains in what sense these measurements can be improved. This makes use of the results of a study in the Netherlands on air quality user requirements and instrument design for an OMI/SCIAMACHY follow-on instrument. The improvements are implemented in a new instrument, TROPOMI: an O2A channel is added to improve on surface and cloud albedo, cloud fraction and cloud top height and a new separate module is added for the SWIR wavelengths for measuring CO and CH4. The ground pixel is reduced to 10 × 10 km2 and signal-tonoises are improved to allow measurements in low albedo areas. The design makes use of newly developed detectors and new optics to reduce the overall instrument size. Lastly, the paper discusses the problem of data continuity for the coming 10-15 years, i.e. after AURA and ENVISAT end of life.
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- 2006
43. Oog voor klimaat en luchtkwaliteit
- Author
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Levelt, P.F. (author) and Levelt, P.F. (author)
- Abstract
Geoscience and Remote Sensing, Civil Engineering and Geosciences
- Published
- 2012
44. Analysis of satellite-derived Arctic tropospheric BrO columns in conjunction with aircraft measurements during ARCTAS and ARCPAC
- Author
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Choi, S., Wang, Y., Salawitch, R.J., Canty, T., Joiner, J., Zeng, T., Kurosu, T.P., Chance, K., Richter, A., Huey, L.G., Liao, J., Neuman, J.A., Nowak, J.B., Dibb, J.E., Weinheimer, A.J., Diskin, G., Ryerson, T.B., Silva, da, A., Curry, J., Kinnison, D., Tilmes, S., Levelt, P.F., Choi, S., Wang, Y., Salawitch, R.J., Canty, T., Joiner, J., Zeng, T., Kurosu, T.P., Chance, K., Richter, A., Huey, L.G., Liao, J., Neuman, J.A., Nowak, J.B., Dibb, J.E., Weinheimer, A.J., Diskin, G., Ryerson, T.B., Silva, da, A., Curry, J., Kinnison, D., Tilmes, S., and Levelt, P.F.
- Abstract
We derive tropospheric column BrO during the ARCTAS and ARCPAC field campaigns in spring 2008 using retrievals of total column BrO from the satellite UV nadir sensors OMI and GOME-2 using a radiative transfer model and stratospheric column BrO from a photochemical simulation. We conduct a comprehensive comparison of satellite-derived tropospheric BrO column to aircraft in-situ observations of BrO and related species. The aircraft profiles reveal that tropospheric BrO, when present during April 2008, was distributed over a broad range of altitudes rather than being confined to the planetary boundary layer (PBL). Perturbations to the total column resulting from tropospheric BrO are the same magnitude as perturbations due to longitudinal variations in the stratospheric component, so proper accounting of the stratospheric signal is essential for accurate determination of satellite-derived tropospheric BrO. We find reasonably good agreement between satellite-derived tropospheric BrO and columns found using aircraft in-situ BrO profiles, particularly when satellite radiances were obtained over bright surfaces (albedo >0.7), for solar zenith angle
- Published
- 2012
45. Evaluation of stratospheric NO2 retrieved from the Ozone Monitoring Instrument : intercomparison, diurnal cycle and trending
- Author
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Dirksen, R.J., Boersma, K.F., Eskes, H.J., Ionov, D.V., Bucsela, E.J., Levelt, P.F., Kelder, H.M., Dirksen, R.J., Boersma, K.F., Eskes, H.J., Ionov, D.V., Bucsela, E.J., Levelt, P.F., and Kelder, H.M.
- Abstract
[1] A 5+ year record of satellite measurements of nitrogen dioxide columns from the Ozone Monitoring Instrument (OMI) is evaluated to establish the quality of the OMI retrievals and to test our understanding of stratospheric NO2. The use of assimilation techniques to retrieve stratospheric vertical columns of NO2 from OMI slant column observations is described in detail. Over remote areas the forecast model state is generally within 0.15 × 1015 molecules/cm2 of the analysis. Dutch OMI NO2 (DOMINO) and Standard Product (SP) stratospheric NO2 columns agree within 0.3 × 1015 molecules/cm2 (13%) with independent, ground-based measurements. This is comparable to the level of consistency (15–20%) among ground-based techniques. On average, DOMINO stratospheric NO2 is higher than SP by 0.2 × 1015 molecules/cm2, but larger differences occur on the synoptic scale. Overlapping OMI orbits poleward of 30° enabled us to extract information on the diurnal variation in stratospheric NO2. We find that in the Arctic, the daytime increase of NO2 has a distinct seasonal dependence that peaks in spring and fall. Daytime increase rates inside the denoxified Arctic polar vortex are low, but we find high rates (>0.4 × 1015 molecules/cm2/h) outside the vortex. A multilinear regression to the DOMINO record shows a distinct quasi-biennial oscillation (QBO) signal in stratospheric NO2 columns over the tropics. The QBO's amplitude is comparable to the annual cycle and stronger over the Southern Hemisphere than over the Northern Hemisphere. We infer near-identical trends from DOMINO observations (+0.4%/decade) as from ground-based instrumentation over Lauder (+0.6%/decade) in the 2004–2010 period.
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- 2011
46. Global satellite analysis of the relation between aerosols and short-lived trace gases
- Author
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Veefkind, J.P., Boersma, K.F., Wang, J., Kurosu, T., Chance, K., Krotkov, N.A., Levelt, P.F., Veefkind, J.P., Boersma, K.F., Wang, J., Kurosu, T., Chance, K., Krotkov, N.A., and Levelt, P.F.
- Abstract
The spatial and temporal correlations between concurrent satellite observations of aerosol optical thickness (AOT) from the Moderate Resolution Imaging Spectroradiometer (MODIS) and tropospheric columns of nitrogen dioxide (NO2), sulfur dioxide (SO2), and formaldehyde (HCHO) from the Ozone Monitoring Instrument (OMI) are used to infer information on the global composition of aerosol particles. When averaging the satellite data over large regions and longer time periods, we find significant correlation between MODIS AOT and OMI trace gas columns for various regions in the world. This shows that these enhanced aerosol and trace gas concentrations originate from common sources, such as fossil fuel combustion, biomass burning, and organic compounds released from the biosphere. This leads us to propose that satellite-inferred AOT to NO2 ratios for regions with comparable photochemical regimes can be used as indicators for the relative regional pollution control of combustion processes. Indeed, satellites observe low AOT to NO2 ratios over the eastern United States and western Europe, and high AOT to NO2 ratios over comparably industrialized regions in eastern Europe and China. Emission databases and OMI SO2 observations over these regions suggest a much stronger sulfur contribution to aerosol formation than over the well-regulated areas of the eastern United States and western Europe. Furthermore, satellite observations show AOT to NO2 ratios are a factor 100 higher over biomass burning regions than over industrialized areas, reflecting the unregulated burning practices with strong primary particle emissions in the tropics compared to the heavily controlled combustion processes in the industrialized Northern Hemisphere. Simulations with a global chemistry transport model (GEOS-Chem) capture most of these variations, although on regional scales significant differences are found. Wintertime aerosol concentrations show strongest correlations with NO2 throughout most of the
- Published
- 2011
47. Accurate satellite-derived estimates of the tropospheric ozone impact on the global radiation budget
- Author
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Joiner, J., Schoeberl, M.R., Vasilkov, A., Oreopoulos, L., Platnick, S., Livesey, N.J., Levelt, P.F., Joiner, J., Schoeberl, M.R., Vasilkov, A., Oreopoulos, L., Platnick, S., Livesey, N.J., and Levelt, P.F.
- Abstract
Estimates of the radiative forcing due to anthropogenically-produced tropospheric O3 are derived primarily from models. Here, we use tropospheric ozone and cloud data from several instruments in the A-train constellation of satellites as well as information from the GEOS-5 Data Assimilation System to accurately estimate the radiative effect of tropospheric O3 for January and July 2005. Since we cannot distinguish between natural and anthropogenic sources with the satellite data, our derived radiative effect reflects the unadjusted (instantaneous) effect of the total tropospheric O3 rather than the anthropogenic component. We improve upon previous estimates of tropospheric ozone mixing ratios from a residual approach using the NASA Earth Observing System (EOS) Aura Ozone Monitoring Instrument (OMI) and Microwave Limb Sounder (MLS) by incorporating cloud pressure information from OMI. We focus specifically on the magnitude and spatial structure of the cloud effect on both the short- and long-wave radiative budget. The estimates presented here can be used to evaluate the various aspects of model-generated radiative forcing. For example, our derived cloud impact is to reduce the radiative effect of tropospheric ozone by ~16%. This is centered within the published range of model-produced cloud effect on unadjusted ozone radiative forcing.
- Published
- 2009
48. Ozone mixing ratios inside tropical deep convective clouds from OMI satellite measurements
- Author
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Ziemke, J.R., Joiner, J., Chandra, S., Bhartia, P.K., Vasilkov, A., Haffner, D.P., Yang, Kai, Schoeberl, M.R., Froidevaux, L., Levelt, P.F., Ziemke, J.R., Joiner, J., Chandra, S., Bhartia, P.K., Vasilkov, A., Haffner, D.P., Yang, Kai, Schoeberl, M.R., Froidevaux, L., and Levelt, P.F.
- Abstract
We have compared spectral ultraviolet overpass irradiances from the Ozone Monitoring Instruments (OMI) against ground-based Brewer measurements at Thessaloniki, Greece from September 2004 to December 2007. It is demonstrated that OMI overestimates UV irradiances by 30%, 17% and 13% for 305 nm, 324 nm, and 380 nm respectively and 20% for erythemally weighted irradiance. The bias between OMI and Brewer increases with increasing aerosol absorption optical thickness. We present methodologies that can be applied for correcting this bias based on experimental results derived from the comparison period and also theoretical approaches using radiative transfer model calculations. All correction approaches minimize the bias and the standard deviation of the ratio OMI versus Brewer ratio. According to the results, the best correction approach suggests that the OMI UV product has to be multiplied by a correction factor CA(¿) of the order of 0.8, 0.88 and 0.9 for 305 nm, 324 nm and 380 nm respectively. Limitations and possibilities for applying such methodologies in a global scale are also discussed.
- Published
- 2009
49. The high-resolution solar reference spectrum between 250 and 550 nm and its application to measurements with the ozone monitoring instrument
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Dobber, M.R., Voors, R., Dirksen, R.J., Kleipool, Q., Levelt, P.F., Dobber, M.R., Voors, R., Dirksen, R.J., Kleipool, Q., and Levelt, P.F.
- Abstract
We have constructed a new high resolution solar reference spectrum in the spectral range between 250 and 550 nm. The primary use of this spectrum is for the calibration of the Dutch¿-¿Finnish Ozone Monitoring Instrument (OMI), but other applications are mentioned. The incentive for deriving a new high resolution solar reference spectrum is that available spectra do not meet our requirements on radiometric accuracy or spectral resolution. In this paper we explain the steps involved in constructing the new spectrum, based on available low and high resolution spectra and discuss the main sources of uncertainty. We compare the result with solar measurements obtained with the OMI as well as with other UV-VIS space-borne spectrometers with a similar spectral resolution. We obtain excellent agreement with the OMI measurements, which indicates that both the newly derived solar reference spectrum and our characterization of the OMI instrument are well understood. We also find good agreement with previously published low resolution spectra. The absolute intensity scale, wavelength calibration and representation of the strength of the Fraunhofer lines have been investigated and optimized to obtain the resulting high resolution solar reference spectrum. © 2008 Springer Science+Business Media B.V. U7 - Export Date: 2 August 2010 U7 - Source: Scopus
- Published
- 2008
50. A future 'Global Atmospheric Composition Mission' (CACM) concept
- Author
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Livesey, N.J., Santee, M., Stek, P., Waters, J., Levelt, P.F., Veefkind, J.P., Kumer, J., Roche, A., Livesey, N.J., Santee, M., Stek, P., Waters, J., Levelt, P.F., Veefkind, J.P., Kumer, J., and Roche, A.
- Abstract
Resolution of important outstanding questions in air quality, climate change and ozone layer stability demands global observations of multiple chemical species with high horizontal and vertical resolution from the boundary layer to the stratopause. We present a mission concept that delivers the needed atmospheric composition observations, along with cloud ice and water vapor data needed for improvements in climate and weather forecasting models. The mission comprises ultraviolet and infrared nadir and microwave limb viewing instruments observing wide swaths each orbit. We review the scientific goals of the mission and the measurement capabilities this concept will deliver. We describe how precessing orbits offer significant improvements in temporal resolution and diurnal coverage compared to sun-synchronous orbits. Such improvements are needed to quantify the impact of critical "fast processes" such as deep convection on the composition and radiative properties of the upper troposphere, a region where water vapor and ozone are strong but poorly understood greenhouse gases. This concept can serve as the "Global Atmospheric Composition Mission" (GACM) recently recommended by the National Academy of Sciences decadal survey as one of 17 priority earth science missions for the coming decade. ©2008 IEEE. U7 - Export Date: 2 August 2010 U7 - Source: Scopus U7 - Art. No.: 4526243
- Published
- 2008
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