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Cooling of atomic motion is a crucial tool for many branches of atomic physics, ranging from fundamental physics explorations to quantum information and sensing. For trapped ions, electromagnetically-induced-transparency (EIT) cooling has received attention for the relative speed, low laser power requirements, and broad cooling bandwidth of the technique. However, in applications where the ion used for cooling has hyperfine structure to enable long coherence times, it is difficult to find a closed three-level system in which to perform standard EIT cooling. Here, we demonstrate successful EIT cooling on 25Mg+ by the addition of an extra laser frequency; this method can be applied to any ion with non-zero nuclear spin. Furthermore, we demonstrate simultaneous EIT cooling of all axial modes in mixed-species crystals 9Be+ - 25Mg+ and 9Be+ - 25Mg+ - 9Be+ through the 25Mg+ ion., Comment: 10 pages, 6 figures, 2 tables

We show experimentally that a broad class of interactions involving quantum harmonic oscillators can be made stronger (amplified) using a unitary squeezing protocol. While our demonstration uses the motional and spin states of a single trapped $^{25}$Mg$^{+}$ ion, the scheme applies generally to Hamiltonians involving just a single harmonic oscillator as well as Hamiltonians coupling the oscillator to another quantum degree of freedom such as a qubit, covering a large range of systems of interest in quantum information and metrology applications. Importantly, the protocol does not require knowledge of the parameters of the Hamiltonian to be amplified, nor does it require a well-defined phase relationship between the squeezing interaction and the rest of the system dynamics, making it potentially useful in instances where certain aspects of a signal or interaction may be unknown or uncontrolled.

Transport, separation, and merging of trapped ion crystals are essential operations for most large-scale quantum computing architectures. In this work, we develop a theoretical framework that describes the dynamics of ions in time-varying potentials with a motional squeeze operator, followed by a motional displacement operator. Using this framework, we develop a new, general protocol for trapped ion transport, separation, and merging. We show that motional squeezing can prepare an ion wave packet to enable transfer from the ground state of one trapping potential to another. The framework and protocol are applicable if the potential is harmonic over the extent of the ion wave packets at all times. As illustrations, we discuss two specific operations: changing the strength of the confining potential for a single ion, and separating same-species ions with their mutual Coulomb force. Both of these operations are, ideally, free of residual motional excitation.

Universal control of multiple qubits -- the ability to entangle qubits and to perform arbitrary individual qubit operations -- is a fundamental resource for quantum computation, simulation, and networking. Here, we implement a new laser-free scheme for universal control of trapped ion qubits based on microwave magnetic fields and radiofrequency magnetic field gradients. We demonstrate high-fidelity entanglement and individual control by creating symmetric and antisymmetric two-qubit maximally entangled states with fidelities in the intervals [0.9983, 1] and [0.9964, 0.9988], respectively, at 68% confidence, corrected for state initialization error. This technique is robust against multiple sources of decoherence, usable with essentially any trapped ion species, and has the potential to perform simultaneous entangling operations on many pairs of ions without increasing control signal power or complexity.

Strong and precisely-controlled interactions between quantum objects are essential for quantum information processing, simulation, and sensing, and for the formation of exotic quantum matter. A well-established paradigm for coupling otherwise weakly-interacting quantum objects is to use auxiliary bosonic quantum excitations to mediate the interactions. Important examples include photon-mediated interactions between atoms, superconducting qubits, and color centers in diamond, and phonon-mediated interactions between trapped ions and between optical and microwave photons. Boson-mediated interactions can in principle be amplified through parametric driving of the boson channel; the drive need not couple directly to the interacting quantum objects. This technique has been proposed for a variety of quantum platforms, but has not to date been realized in the laboratory. Here we experimentally demonstrate the amplification of a boson-mediated interaction between two trapped-ion qubits by parametric modulation of the trapping potential. The amplification provides up to a 3.25-fold increase in the interaction strength, validated by measuring the speedup of two-qubit entangling gates. This amplification technique can be used in any quantum platform where parametric modulation of the boson channel is possible, enabling exploration of new parameter regimes and enhanced quantum information processing., Comment: 12 pages, 4 figures, one parametric drive tone

We report high-fidelity state readout of a trapped ion qubit using a trap-integrated photon detector. We determine the hyperfine qubit state of a single $^9$Be$^+$ ion held in a surface-electrode rf ion trap by counting state-dependent ion fluorescence photons with a superconducting nanowire single-photon detector (SNSPD) fabricated into the trap structure. The average readout fidelity is 0.9991(1), with a mean readout duration of 46 $\mu$s, and is limited by the polarization impurity of the readout laser beam and by off-resonant optical pumping. Because there are no intervening optical elements between the ion and the detector, we can use the ion fluorescence as a self-calibrated photon source to determine the detector quantum efficiency and its dependence on photon incidence angle and polarization., Comment: 15 pages, 11 figures, including supplemental material

Two vertical-external-cavity surface-emitting laser (VECSEL) systems producing ultraviolet (UV) radiation at 235 nm and 313 nm are demonstrated. The systems are suitable for quantum information processing applications with trapped beryllium ions. Each system consists of a compact, single-frequency, continuous-wave VECSEL producing high-power near-infrared light, tunable over tens of nanometers. One system generates 2.4 W at 940 nm, using a gain mirror based on GaInAs/GaAs quantum wells, which is converted to 54 mW of 235 nm light for photoionization of neutral beryllium atoms. The other system uses a novel gain mirror based on GaInNAs/GaAs quantum-wells, enabling wavelength extension with manageable strain in the GaAs lattice. This system generates 1.6 W at 1252 nm, which is converted to 41 mW of 313 nm light that is used to laser cool trapped $^{9}$Be$^{+}$ ions and to implement quantum state preparation and detection. The 313 nm system is also suitable for implementing high-fidelity quantum gates, and more broadly, our results extend the capabilities of VECSEL systems for applications in atomic, molecular, and optical physics., Comment: 8 pages, 7 figures

Scaling quantum information processors is a challenging task, requiring manipulation of a large number of qubits with high fidelity and a high degree of connectivity. For trapped ions, this could be realized in a two-dimensional array of interconnected traps in which ions are separated, transported and recombined to carry out quantum operations on small subsets of ions. Here, we use a junction connecting orthogonal linear segments in a two-dimensional (2D) trap array to reorder a two-ion crystal. The secular motion of the ions experiences low energy gain and the internal qubit levels maintain coherence during the reordering process, therefore demonstrating a promising method for providing all-to-all connectivity in a large-scale, two- or three-dimensional trapped-ion quantum information processor.

The dominant error sources for state-of-the-art laser-free trapped-ion entangling gates are decoherence of the qubit state and the ion motion. The effect of these decoherence mechanisms can be suppressed with additional control fields, or with techniques that have the disadvantage of reducing gate speed. Here, we propose using a near-motional-frequency magnetic field gradient to implement a laser-free gate that is simultaneously resilient to both types of decoherence, does not require additional control fields, and has a relatively small cost in gate speed.

A mixed-species geometric phase gate has been proposed for implementing quantum logic spectroscopy on trapped ions that combines probe and information transfer from the spectroscopy to the logic ion in a single pulse. We experimentally realize this method, show how it can be applied as a technique for identifying transitions in currently intractable atoms or molecules, demonstrate its reduced temperature sensitivity, and observe quantum-enhanced frequency sensitivity when it is applied to multi-ion chains. Potential applications include improved readout of trapped-ion clocks and simplified error syndrome measurements for quantum error correction., Comment: Changes: Title; description of the basic method; more detail on data analysis and systematic effects

We present a new method of spin-motion coupling for trapped ions using microwaves and a magnetic field gradient oscillating close to the ions' motional frequency. We demonstrate and characterize this coupling experimentally using a single ion in a surface-electrode trap that incorporates current-carrying electrodes to generate the microwave field and the oscillating magnetic field gradient. Using this method, we perform resolved-sideband cooling of a single motional mode to its ground state., Comment: 9 pages, 4 figures

Detection of the weakest forces in nature and the search for new physics are aided by increasingly sensitive measurements of the motion of mechanical oscillators. However, the attainable knowledge of an oscillator's motion is limited by quantum fluctuations that exist even if the oscillator is in its lowest possible energy state. Here we demonstrate a widely applicable technique for amplifying coherent displacements of a mechanical oscillator with initial magnitudes well below these zero-point fluctuations. When applying two orthogonal "squeezing" interactions before and after a small displacement, the displacement is amplified, ideally with no added quantum noise. We implement this protocol with a trapped-ion mechanical oscillator and measure an increase of up to 17.5(3) decibels in sensitivity to small displacements., Comment: 23 pages, 6 figures

We present a general theory for laser-free entangling gates with trapped-ion hyperfine qubits, using either static or oscillating magnetic-field gradients combined with a pair of uniform microwave fields symmetrically detuned about the qubit frequency. By transforming into a `bichromatic' interaction picture, we show that either ${\hat{\sigma}_{\phi}\otimes\hat{\sigma}_{\phi}}$ or ${\hat{\sigma}_{z}\otimes\hat{\sigma}_{z}}$ geometric phase gates can be performed. The gate basis is determined by selecting the microwave detuning. The driving parameters can be tuned to provide intrinsic dynamical decoupling from qubit frequency fluctuations. The ${\hat{\sigma}_{z}\otimes\hat{\sigma}_{z}}$ gates can be implemented in a novel manner which eases experimental constraints. We present numerical simulations of gate fidelities assuming realistic parameters.

Studying a single atomic ion confined in a time-dependent periodic anharmonic potential, we find large amplitude trajectories stable for millions of oscillation periods in the presence of stochastic laser cooling. The competition between energy gain from the time-dependent drive and damping leads to the stabilization of such stochastic limit cycles. Instead of converging to the global minimum of the averaged potential, the steady-state phase-space distribution develops multiple peaks in the regions of phase space where the frequency of the motion is close to a multiple of the periodic drive. Such distinct nonequilibrium behaviour can be observed in realistic radio-frequency traps with laser-cooled ions, suggesting that Paul traps offer a well-controlled test-bed for studying transport and dynamics of microscopically driven systems., Comment: 6 pages, 2 figures

We study the stochastic dynamics of a particle in a periodically driven potential. For atomic ions trapped in radio-frequency Paul traps, noise heating and laser cooling typically act slowly in comparison with the unperturbed motion. These stochastic processes can be accounted for in terms of a probability distribution defined over the action variables, which would otherwise be conserved within the regular regions of the Hamiltonian phase space. We present a semiclassical theory of low-saturation laser cooling applicable from the limit of low-amplitude motion to large-amplitude motion, accounting fully for the time-dependent and anharmonic trap. We employ our approach to a detailed study of the stochastic dynamics of a single ion, drawing general conclusions regarding the nonequilibrium dynamics of laser-cooled trapped ions. We predict a regime of anharmonic motion in which laser cooling becomes diffusive (i.e., it is equally likely to cool the ion as it is to heat it), and can also turn into effective heating. This implies that a high-energy ion could be easily lost from the trap despite being laser cooled; however, we find that this loss can be counteracted using a laser detuning much larger than Doppler detuning., Comment: 23 pages, 7 figures

We present a comprehensive phase-space treatment of the motion of charged particles in electrodynamic traps. Focusing on five-wire surface-electrode Paul traps, we study the details of integrable and chaotic motion of a single ion. We introduce appropriate phase-space measures and give a universal characterization of the trap effectiveness as a function of the parameters. We rigorously derive the commonly used (time-independent) pseudopotential approximation, quantify its regime of validity and analyze the mechanism of its breakdown within the time-dependent potential. The phase space approach that we develop gives a general framework for describing ion dynamics in a broad variety of surface Paul traps. To probe this framework experimentally, we propose and analyze, using numerical simulations, an experiment that can be realized with an existing four-wire trap. We predict a robust experimental signature of the existence of trapping pockets within a mixed regular and chaotic phase-space structure. Intricately rich escape dynamics suggest that surface traps give access to exploring microscopic Hamiltonian transport phenomena in phase space., Comment: 22 pages, 14 figures

Effective spin-spin interactions between N+1 qubits enable the determination of the eigenvalue of an arbitrary Pauli product of dimension N with a constant, small number of multi-qubit gates that is independent of N and encodes the eigenvalue in the measurement basis states of an extra ancilla qubit. Such interactions are available whenever qubits can be coupled to a shared harmonic oscillator, a situation that can be realized in several physical qubit implementations. For example, suitable interactions have already been realized for up to 14 qubits in ion traps. It should be possible to implement stabilizer codes for quantum error correction with a constant number of multi-qubit gates, in contrast to typical constructions using a number of two-qubit gates that increases as a function of N. The special case of finding the parity of N qubits only requires a small number of operations that is independent of N. This compares favorably to algorithms for computing the parity on conventional machines, which implies a genuine quantum advantage., Comment: 10 pages, no figures

Electric-field noise from the surfaces of ion-trap electrodes couples to the ion's charge causing heating of the ion's motional modes. This heating limits the fidelity of quantum gates implemented in quantum information processing experiments. The exact mechanism that gives rise to electric-field noise from surfaces is not well-understood and remains an active area of research. In this work, we detail experiments intended to measure ion motional heating rates with exchangeable surfaces positioned in close proximity to the ion, as a sensor to electric-field noise. We have prepared samples with various surface conditions, characterized in situ with scanned probe microscopy and electron spectroscopy, ranging in degrees of cleanliness and structural order. The heating-rate data, however, show no significant differences between the disparate surfaces that were probed. These results suggest that the driving mechanism for electric-field noise from surfaces is due to more than just thermal excitations alone., Comment: 5 pages, 4 figures

We report correlation measurements on two $^9$Be$^+$ ions that violate a chained Bell inequality obeyed by any local-realistic theory. The correlations can be modeled as derived from a mixture of a local-realistic probabilistic distribution and a distribution that violates the inequality. A statistical framework is formulated to quantify the local-realistic fraction allowable in the observed distribution without the fair-sampling or independent-and-identical-distributions assumptions. We exclude models of our experiment whose local-realistic fraction is above 0.327 at the 95 \% confidence level. This bound is significantly lower than 0.586, the minimum fraction derived from a perfect Clauser-Horne-Shimony-Holt inequality experiment. Furthermore, our data provides a device-independent certification of the deterministically created Bell states.

We demonstrate superconducting nanowire single photon detectors with 76 +/- 4 % system detection efficiency at a wavelength of 315 nm and an operating temperature of 3.2 K, with a background count rate below 1 count per second at saturated detection efficiency. We propose integrating these detectors into planar surface electrode radio-frequency Paul traps for use in trapped ion quantum information processing. We operate detectors integrated into test ion trap structures at 3.8 K both with and without typical radio-frequency trapping electric fields. The trapping fields reduce system detection efficiency by 9 %, but do not increase background count rates., Comment: 16 pages, 7 figures

We implement faster-than-adiabatic two-qubit phase gates using smooth state-dependent forces. The forces are designed to leave no final motional excitation, independently of the initial motional state in the harmonic, small-oscillations limit. They are simple, explicit functions of time and the desired logical phase of the gate, and are based on quadratic invariants of motion and Lewis-Riesenfeld phases of the normal modes., Comment: 14 pages, 9 figures

We report high-fidelity laser-beam-induced quantum logic gates on magnetic-field-insensitive qubits comprised of hyperfine states in $^{9}$Be$^+$ ions with a memory coherence time of more than 1 s. We demonstrate single-qubit gates with error per gate of $3.8(1)\times 10^{-5}$. By creating a Bell state with a deterministic two-qubit gate, we deduce a gate error of $8(4)\times10^{-4}$. We characterize the errors in our implementation and discuss methods to further reduce imperfections towards values that are compatible with fault-tolerant processing at realistic overhead., Comment: 12 pages, 7 figures

Entangled states are a crucial resource for quantum-based technologies such as quantum computers and quantum communication systems (1,2). Exploring new methods for entanglement generation is important for diversifying and eventually improving current approaches. Here, we create entanglement in atomic ions by applying laser fields to constrain the evolution to a restricted number of states, in an approach that has become known as "quantum Zeno dynamics" (3-5). With two trapped $^9\rm{Be}^+$ ions, we obtain Bell state fidelities up to $0.990^{+2}_{-5}$, with three ions, a W-state (6) fidelity of $0.910^{+4}_{-7}$ is obtained. Compared to other methods of producing entanglement in trapped ions, this procedure is relatively insensitive to certain imperfections such as fluctuations in laser intensity, laser frequency, and ion-motion frequencies., Comment: 44 pages, 10 figures

Precision control over hybrid physical systems at the quantum level is important for the realization of many quantum-based technologies. In the field of quantum information processing (QIP) and quantum networking, various proposals discuss the possibility of hybrid architectures where specific tasks are delegated to the most suitable subsystem. For example, in quantum networks, it may be advantageous to transfer information from a subsystem that has good memory properties to another subsystem that is more efficient at transporting information between nodes in the network. For trapped-ions, a hybrid system formed of different species introduces extra degrees of freedom that can be exploited to expand and refine the control of the system. Ions of different elements have previously been used in QIP experiments for sympathetic cooling, creation of entanglement through dissipation, and quantum non-demolition (QND) measurement of one species with another. Here, we demonstrate an entangling quantum gate between ions of different elements which can serve as an important building block of QIP, quantum networking, precision spectroscopy, metrology, and quantum simulation. A geometric phase gate between a $^9$Be$^+$ ion and a $^{25}$Mg$^+$ ion is realized through an effective spin-spin interaction generated by state-dependent forces induced with laser beams. Combined with single-qubit gates and same-species entangling gates, this mixed-element entangling gate provides a complete set of gates over such a hybrid system for universal QIP. Using a sequence of such gates, we demonstrate a Controlled-NOT (CNOT) gate and a SWAP gate. We further demonstrate the robustness of these gates against thermal excitation and show improved detection in quantum logic spectroscopy (QLS). We also observe a strong violation of a CHSH-type Bell inequality on entangled states composed of different ion species., Comment: 7 pages, 4 figures

We investigate the dynamics of mixed-species ion crystals during transport between spatially distinct locations in a linear Paul trap in the diabatic regime. In a general mixed-species crystal, all degrees of freedom along the direction of transport are excited by an accelerating well, so unlike the case of same-species ions, where only the center-of-mass-mode is excited, several degrees of freedom have to be simultaneously controlled by the transport protocol. We design protocols that lead to low final excitations in the diabatic regime using invariant-based inverse-engineering for two different-species ions and also show how to extend this approach to longer mixed-species ion strings. Fast transport of mixed-species ion strings can significantly reduce the time overhead in certain architectures for scalable quantum information processing with trapped ions., Comment: 6 pages, 4 figures

We describe an ex-situ surface-cleaning procedure that is shown to reduce motional heating from ion-trap electrodes. This precleaning treatment, to be implemented immediately before the final assembly and vacuum processing of ion traps, removes surface contaminants remaining after the electrode-fabrication process. We incorporate a multi-angle ion-bombardment treatment intended to clean the electrode surfaces and interelectrode gaps of microfabricated traps. This procedure helps to minimize redeposition in the gaps between electrodes that can cause electrical shorts. We report heating rates in a stylus-type ion trap prepared in this way that are lower by one order of magnitude compared to a similar untreated stylus-type trap using the same experimental setup., Comment: 4 pages, 3 figures

We show how to create quantum gates of arbitrary speed between trapped ions, using a laser walking wave, with complete insensitivity to drift of the optical phase, and requiring cooling only to the Lamb-Dicke regime. We present pulse sequences that satisfy the requirements and are easy to produce in the laboratory., Comment: 11 pages, 3 figures

Entangled states are a key resource in fundamental quantum physics, quantum cryp-tography, and quantum computation [1].To date, controlled unitary interactions applied to a quantum system, so-called "quantum gates", have been the most widely used method to deterministically create entanglement [2]. These processes require high-fidelity state preparation as well as minimizing the decoherence that inevitably arises from coupling between the system and the environment and imperfect control of the system parameters. Here, on the contrary, we combine unitary processes with engineered dissipation to deterministically produce and stabilize an approximate Bell state of two trapped-ion qubits independent of their initial state. While previous works along this line involved the application of sequences of multiple time-dependent gates [3] or generated entanglement of atomic ensembles dissipatively but relied on a measurement record for steady-state entanglement [4], we implement the process in a continuous time-independent fashion, analogous to optical pumping of atomic states. By continuously driving the system towards steady-state, the entanglement is stabilized even in the presence of experimental noise and decoherence. Our demonstration of an entangled steady state of two qubits represents a step towards dissipative state engineering, dissipative quantum computation, and dissipative phase transitions [5-7]. Following this approach, engineered coupling to the environment may be applied to a broad range of experimental systems to achieve desired quantum dynamics or steady states. Indeed, concurrently with this work, an entangled steady state of two superconducting qubits was demonstrated using dissipation [8]., Comment: 25 pages, 5 figures

We demonstrate a trapped-ion entangling-gate scheme proposed by Bermudez et al. [Phys. Rev. A 85, 040302 (2012)]. Simultaneous excitation of a strong carrier and a single-sideband transition enables deterministic creation of entangled states. The method works for magnetic field-insensitive states, is robust against thermal excitations, includes dynamical decoupling from qubit dephasing errors, and provides simplifications in experimental implementation compared to some other entangling gates with trapped ions. We achieve a Bell state fidelity of 0.974(4) and identify the main sources of error., Comment: 5 pages, 4 figures, 1 table

Microwave near-field quantum control of spin and motional degrees of freedom of 25Mg+ ions can be used to generate two-ion entanglement, as recently demonstrated in Ospelkaus et al. [Nature 476, 181 (2011)]. Here, we describe additional details of the setup and calibration procedures for these experiments. We discuss the design and characteristics of the surface-electrode trap and the microwave system, and compare experimental measurements of the microwave near-fields with numerical simulations. Additionally, we present a method that utilizes oscillating magnetic-field gradients to detect micromotion induced by the ponderomotive radio-frequency potential in linear traps. Finally, we discuss the present limitations of microwave-driven two-ion entangling gates in our system., Comment: 12 pages and 10 figures

We use electromagnetically induced transparency (EIT) laser cooling to cool motional modes of a linear ion chain. As a demonstration, we apply EIT cooling on $^{24}Mg^+$ ions to cool the axial modes of a $^9Be^+$ - $^{24}Mg^+$ ion pair and a $^9Be^+$ - $^{24}Mg^+$ - $^{24}Mg^+$ - $^9Be^+$ ion chain, thereby sympathetically cooling the $^{9}$Be$^{+}$ ions. Compared to previous implementations of conventional Raman sideband cooling, we achieve approximately an order-of-magnitude reduction in the duration required to cool the modes to near the ground state and significant reduction in required laser intensity., Comment: 5 pages, 4 figures

Individual-qubit addressing is a prerequisite for many instances of quantum information processing. We demonstrate this capability on trapped-ion qubits with microwave near-fields delivered by electrode structures integrated into a microfabricated surface-electrode trap. We describe four approaches that may be used in quantum information experiments with hyperfine levels as qubits. We implement individual control on two 25Mg+ ions separated by 4.3 micrometer and find spin-flip crosstalk errors on the order of 10^(-3)., Comment: 5 pages and 4 figures

We investigate the motional dynamics of single and multiple ions during transport between and separation into spatially distinct locations in a multi-zone linear Paul trap. A single 9Be+ ion in a 2 MHz harmonic well located in one zone was laser-cooled to near its ground state of motion and transported 370 micrometers by moving the well to another zone. This was accomplished in 8 microseconds, corresponding to 16 periods of oscillation. Starting from a state with n=0.1 quanta, during transport the ion was excited to a displaced coherent state with n=1.6 quanta but on completion was returned close to its motional ground state with n=0.2. Similar results were achieved for the transport of two ions. We also separated chains of up to 9 ions from one potential well to two distinct potential wells. With two ions this was accomplished in 55 microseconds, with final excitations of about 2 quanta for each ion. Fast coherent transport and separation can significantly reduce the time overhead in certain architectures for scalable quantum information processing with trapped ions., Comment: 5 pages, 5 figures

As experimental platforms for quantum information processing continue to mature, characterization of the quality of unitary gates that can be applied to their quantum bits (qubits) becomes essential. Eventually, the quality must be sufficiently high to support arbitrarily long quantum computations. Randomized benchmarking already provides a platform-independent method for assessing the quality of one-qubit rotations. Here we describe an extension of this method to multi-qubit gates. We provide a platform-independent protocol for evaluating the performance of experimental Clifford unitaries, which form the basis of fault-tolerant quantum computing. We implemented the benchmarking protocol with trapped-ion two-qubit phase gates and one-qubit gates and found an error per random two-qubit Clifford unitary of $0.162 \pm 0.008$, thus setting the first benchmark for such unitaries. By implementing a second set of sequences with an extra two-qubit phase gate at each step, we extracted an error per phase gate of $0.069 \pm 0.017$. We conducted these experiments with movable, sympathetically cooled ions in a multi-zone Paul trap - a system that can in principle be scaled to larger numbers of ions., Comment: Corrected description of parallel single-qubit benchmark experiment. Results unchanged

Anomalous heating of trapped atomic ions is a major obstacle to their use as quantum bits in a scalable quantum computer. The physical origin of this heating is not fully understood, but experimental evidence suggests that it is caused by electric-field noise emanating from the surface of the trap electrodes. In this study, we have investigated the role that adsorbates on the electrodes play by identifying contaminant overlayers, developing an in situ argon-ion beam cleaning procedure, and measuring ion heating rates before and after cleaning the trap electrodes' surfaces. We find a reduction of two orders of magnitude in heating rate after cleaning., Comment: 7 pages, 1 figure

Preparing molecules at rest and in a highly pure quantum state is a long standing dream in chemistry and physics, so far achieved only for a select set of molecules in dedicated experimental setups. Here, a quantum-limited combination of mass spectrometry and Raman spectroscopy is proposed that should be applicable to a wide range of molecular ions. Excitation of electrons in the molecule followed by uncontrolled decay and branching into several lower energy states is avoided. Instead, the molecule is always connected to rotational states within the electronic and vibrational ground-state manifold, while a co-trapped atomic ion provides efficient entropy removal and allows for extraction of information on the molecule. The outlined techniques might enable preparation, manipulation and measurement of a large multitude of molecular ion species with the same instrument, with applications including, but not limited to, precise determination of molecular properties and fundamental tests of physics., Comment: 12 pages, 2 figures, reformatted for resubmission

We have demonstrated transport of Be+ ions through a 2D Paul-trap array that incorporates an X-junction, while maintaining the ions near the motional ground-state of the confining potential well. We expand on the first report of the experiment [1], including a detailed discussion of how the transport potentials were calculated. Two main mechanisms that caused motional excitation during transport are explained, along with the methods used to mitigate such excitation. We reduced the motional excitation below the results in Ref. [1] by a factor of approximately 50. The effect of a mu-metal shield on qubit coherence is also reported. Finally, we examined a method for exchanging energy between multiple motional modes on the few-quanta level, which could be useful for cooling motional modes without directly accessing the modes with lasers. These results establish how trapped ions can be transported in a large-scale quantum processor with high fidelity., Comment: 16 pages

We theoretically and experimentally examine the effects of anharmonic terms in the trapping potential for linear chains of trapped ions. We concentrate on two different effects that become significant at different levels of anharmonicity. The first is a modification of the oscillation frequencies and amplitudes of the ions' normal modes of vibration for multi-ion crystals, resulting from each ion experiencing a different curvature in the potential. In the second effect, which occurs with increased anharmonicity or higher excitation amplitude, amplitude-dependent shifts of the normal-mode frequencies become important. We evaluate normal-mode frequency and amplitude shifts, and comment on the implications for quantum information processing and quantum state engineering. Since the ratio of the anharmonic to harmonic terms typically increases as the ion--electrode distance decreases, anharmonic effects will become more significant as ion trap sizes are reduced. To avoid unwanted problems, anharmonicities should therefore be taken into account at the design stage of trap development., Comment: 26 pages, 7 figures

Control over physical systems at the quantum level is a goal shared by scientists in fields as diverse as metrology, information processing, simulation and chemistry. For trapped atomic ions, the quantized motional and internal degrees of freedom can be coherently manipulated with laser light. Similar control is difficult to achieve with radio frequency or microwave radiation because the essential coupling between internal degrees of freedom and motion requires significant field changes over the extent of the atoms' motion. The field gradients are negligible at these frequencies for freely propagating fields; however, stronger gradients can be generated in the near-field of microwave currents in structures smaller than the free-space wavelength. In the experiments reported here, we coherently manipulate the internal quantum states of the ions on time scales of 20 ns. We also generate entanglement between the internal degrees of freedom of two atoms with a gate operation suitable for general quantum computation. We implement both operations through the magnetic fields from microwave currents in electrodes that are integrated into the micro-fabricated trap structure and create an entangled state with fidelity 76(3) %. This approach, where the quantum control mechanism is integrated into the trapping device in a scalable manner, can potentially benefit quantum information processing, simulation and spectroscopy., Comment: 22 pages, 4 figures, accepted as a letter to Nature

With a 9Be+ trapped-ion hyperfine-states qubit, we demonstrate an error probability per randomized single-qubit gate of 2.0(2) x 10^-5, below the threshold estimate of 10^-4 commonly considered sufficient for fault-tolerant quantum computing. The 9Be+ ion is trapped above a microfabricated surface-electrode ion trap and is manipulated with microwaves applied to a trap electrode. The achievement of low single-qubit-gate errors is an essential step toward the construction of a scalable quantum computer., Comment: 5 pages, 3 figures, 1 table; changed to match published version

The harmonic oscillator is one of the simplest physical systems but also one of the most fundamental. It is ubiquitous in nature, often serving as an approximation for a more complicated system or as a building block in larger models. Realizations of harmonic oscillators in the quantum regime include electromagnetic fields in a cavity [1-3] and the mechanical modes of a trapped atom [4] or macroscopic solid [5]. Quantized interaction between two motional modes of an individual trapped ion has been achieved by coupling through optical fields [6], and entangled motion of two ions in separate locations has been accomplished indirectly through their internal states [7]. However, direct controllable coupling between quantized mechanical oscillators held in separate locations has not been realized previously. Here we implement such coupling through the mutual Coulomb interaction of two ions held in trapping potentials separated by 40 um (similar work is reported in a related paper [8]). By tuning the confining wells into resonance, energy is exchanged between the ions at the quantum level, establishing that direct coherent motional coupling is possible for separately trapped ions. The system demonstrates a building block for quantum information processing and quantum simulation. More broadly, this work is a natural precursor to experiments in hybrid quantum systems, such as coupling a trapped ion to a quantized macroscopic mechanical or electrical oscillator [9-13]., Comment: 5 pages, 4 figures

Integration of fiber optics may play a critical role in the development of quantum information processors based on trapped ions and atoms by enabling scalable collection and delivery of light and coupling trapped ions to optical microcavities. We trap 24Mg+ ions in a surface-electrode Paul trap that includes an integrated optical fiber for detecting 280-nm fluorescence photons. The collection numerical aperture is 0.37 and total collection efficiency is 2.1 %. The ion can be positioned between 80 \mum and 100 \mum from the tip of the fiber by use of an adjustable rf-pseudopotential., Comment: 4 pages, 3 figures.

We report on the design, fabrication, and preliminary testing of a 150 zone array built in a `surface-electrode' geometry microfabricated on a single substrate. We demonstrate transport of atomic ions between legs of a `Y'-type junction and measure the in-situ heating rates for the ions. The trap design demonstrates use of a basic component design library that can be quickly assembled to form structures optimized for a particular experiment.

The universal quantum computer is a device capable of simulating any physical system and represents a major goal for the field of quantum information science. Algorithms performed on such a device are predicted to offer significant gains for some important computational tasks. In the context of quantum information, "universal" refers to the ability to perform arbitrary unitary transformations in the system's computational space. The combination of arbitrary single-quantum-bit (qubit) gates with an entangling two-qubit gate is a gate set capable of achieving universal control of any number of qubits, provided that these gates can be performed repeatedly and between arbitrary pairs of qubits. Although gate sets have been demonstrated in several technologies, they have as yet been tailored toward specific tasks, forming a small subset of all unitary operators. Here we demonstrate a programmable quantum processor that realises arbitrary unitary transformations on two qubits, which are stored in trapped atomic ions. Using quantum state and process tomography, we characterise the fidelity of our implementation for 160 randomly chosen operations. This universal control is equivalent to simulating any pairwise interaction between spin-1/2 systems. A programmable multi-qubit register could form a core component of a large-scale quantum processor, and the methods used here are suitable for such a device., Comment: 7 pages, 4 figures

We report techniques for the fabrication of multi-zone linear RF Paul traps that exploit the machinability and electrical conductivity of degenerate silicon. The approach was tested by trapping and laser cooling 24Mg+ ions in two trap geometries: a single-zone two-layer trap and a multi-zone surface-electrode trap. From the measured ion motional heating rate we determine an electric field spectral density at the ion's position of approximately 1E-10 (V/m)^2/Hz at a frequency of 1.125 MHz when the ion lies 40 micron above the trap surface. One application of these devices is controlled manipulation of atomic ion qubits, the basis of one form of quantum information processing., Comment: 3 pages; 2 figures; v2: fix heating rate typo

Large-scale quantum information processors must be able to transport and maintain quantum information, and repeatedly perform logical operations. Here we demonstrate a combination of all the fundamental elements required to perform scalable quantum computing using qubits stored in the internal states of trapped atomic ions. We quantify the repeatability of a multi-qubit operation, observing no loss of performance despite qubit transport over macroscopic distances. Key to these results is the use of different pairs of beryllium ion hyperfine states for robust qubit storage, readout and gates, and simultaneous trapping of magnesium re-cooling ions along with the qubit ions., Comment: 9 pages, 4 figures. Accepted to Science, and thus subject to a press embargo

A scalable, multiplexed ion trap for quantum information processing is fabricated and tested. The trap design and fabrication process are optimized for scalability to small trap size and large numbers of interconnected traps, and for integration of control electronics and optics. Multiple traps with similar designs are tested with Cd+, Mg+, and Sr+ ions at room temperature and with Sr+ at 6 K, with respective ion lifetimes of 90 s, 300 +/- 30 s, 56 +/- 6 s, and 4.5 +/- 1.1 hours. The motional heating rate for Mg+ at room temperature and a trap frequency of 1.6 MHz is measured to be 7 +/- 3 quanta per millisecond. For Sr+ at 6 K and 540 kHz the heating rate is measured to be 220 +/- 30 quanta per second., Comment: 18 pages, 12 figures

Hallmarks of quantum mechanics include superposition and entanglement. In the context of large complex systems, these features should lead to situations like Schrodinger's cat, which exists in a superposition of alive and dead states entangled with a radioactive nucleus. Such situations are not observed in nature. This may simply be due to our inability to sufficiently isolate the system of interest from the surrounding environment -- a technical limitation. Another possibility is some as-of-yet undiscovered mechanism that prevents the formation of macroscopic entangled states. Such a limitation might depend on the number of elementary constituents in the system or on the types of degrees of freedom that are entangled. One system ubiquitous to nature where entanglement has not been previously demonstrated is distinct mechanical oscillators. Here we demonstrate deterministic entanglement of separated mechanical oscillators, consisting of the vibrational states of two pairs of atomic ions held in different locations. We also demonstrate entanglement of the internal states of an atomic ion with a distant mechanical oscillator., Comment: 7 pages, 2 figures