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In this work, carbon nanotubes (CNT) and β-cyclodextrin (CD) was used to generate magnetic composites (CNT/MnFe2O4and CNT/β- CD/MnFe2O4) to remove the emerging contaminant of tetracycline (TC) antibiotic from various aqueous solutions. Various techniques were used to investigate the structural and surface characteristics of the adsorptive composites. Brunauer–Emmett–Teller (BET) test illustrated that the synthesized magnetic composites have a higher specific active surface than CNT. The effect of water pH, temperature, sorption time, TC content, and type of aqueous solution on the elimination efficiency was explored. Our data followed the isotherm models of Redlich-Peterson and Temkin. The peak of TC adsorption capacity from distilled water using CNT, CNT/MnFe2O4, CNT/β-CD/MnFe2O4was determined 82.66 mg/g, 86.48 mg/g, and 89.53 mg/g, respectively. The TC adsorption capacity using CNT/β-CD/MnFe2O4magnetic composite from urban drinking water and wastewater was determined at 55.02 mg/g and 40.36 mg/g, respectively. The adsorption process revealed that the removal of TC from distilled water using the synthesized adsorbents follows the pseudo-first-order model. In contrast, the removal of TC from municipal drinking water and wastewater follows the pseudo-second-order kinetic model. The TC decontamination process was spontaneous and exothermic and could be performed well at ambient temperature. Overall, the studied adsorbents (CNT and CNT-based magnetic composites) can be used as promising adsorbents in the TC removal processes from aqueous solutions.