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Vibrational coherences in ultrafast pump–probe (PP) and 2D electronic spectroscopy (2DES) provide insights into the excited state dynamics of molecules. Femtosecond coherence spectra and 2D beat maps yield information about displacements of excited state surfaces for key vibrational modes. Half-broadband 2DES uses a PP configuration with a white light continuum probe to extend the detection range and resolve vibrational coherences in the excited state absorption (ESA). However, the interpretation of these spectra is difficult as they are strongly dependent on the spectrum of the pump laser and the relative displacement of the excited states along the vibrational coordinates. We demonstrate the impact of these convoluting factors for a model based upon cresyl violet. A careful consideration of the position of the pump spectrum can be a powerful tool in resolving the ESA coherences to gain insights into excited state displacements. This paper also highlights the need for caution in considering the spectral window of the pulse when interpreting these spectra. [ABSTRACT FROM AUTHOR]

The use of cavities to impact molecular structure and dynamics has become popular. As cavities, in particular plasmonic nanocavities, are lossy and the lifetime of their modes can be very short, their lossy nature must be incorporated into the calculations. The Lindblad master equation is commonly considered an appropriate tool to describe this lossy nature. This approach requires the dynamics of the density operator and is thus substantially more costly than approaches employing the Schrödinger equation for the quantum wave function when several or many nuclear degrees of freedom are involved. In this work, we compare numerically the Lindblad and Schrödinger descriptions discussed in the literature for a molecular example where the cavity is pumped by a laser. The laser and cavity properties are varied over a range of parameters. It is found that the Schrödinger description adequately describes the dynamics of the polaritons and emission signal as long as the laser intensity is moderate and the pump time is not much longer than the lifetime of the cavity mode. Otherwise, it is demonstrated that the Schrödinger description gradually fails. We also show that the failure of the Schrödinger description can often be remedied by renormalizing the wave function at every step of time propagation. The results are discussed and analyzed. [ABSTRACT FROM AUTHOR]

Er3+/Yb3+ co-doped Na2O–CaF2–ZnO–Al2O3–SiO2 glasses with different Zn/Si ratios were prepared using the melt-quenching technique. The thermal stability was investigated by differential scanning calorimetry. Additionally, the absorption spectra were also analyzed to gather more information about their properties. The down-conversion luminescence corresponding to the strongest fluorescence at a wavelength of 547 nm was obtained under the 378 nm excitation, and a 4S3/2 level fluorescence lifetime was studied. By utilizing a laser pump with a wavelength of 980 nm, the process of both up-conversion and down-conversion luminescence was accomplished. In particular, the glasses substantially enhance fluorescence properties when the Zn/Si ratio is about 0.16. The changes in the Zn/Si ratio lead to modifications in the glass network structure, changing the coordination field environment around the fluorescence center and ultimately impacting the luminescence properties of the rare-earth ions. These effects are evidenced through the findings obtained from Fourier transform infrared spectroscopy and fluorescence spectroscopy analysis of the glass material. [ABSTRACT FROM AUTHOR]

Molecular lasers pumped by quantum cascade laser (QCL) open new possibilities for THz generation and its numerous applications, in particular, for high resolution molecular spectroscopy. In this article, a THz water laser pumped by a mid-infrared QCL was demonstrated using the broad tunability of the pump laser. Twenty D 2 O laser lines were measured under a continuous wave pumping regime, in a spectral range expending from 63 to 177 cm − 1 (1.9–5.3 THz), and with an output power ranging from tens to hundreds of μ W. This letter contains a description of the experimental setup used to produce the THz laser radiation and a comparison of the measured output power with a molecular gain factor used to sort out the most favorable laser lines. In addition to the measured laser transitions, a complete list of laser frequencies together with their corresponding molecular gain is given in the supplementary material, for both H 2 O and D 2 O isotopologues excited in their bending and stretching vibrational states. [ABSTRACT FROM AUTHOR]

Forward stimulated Raman scattering and backward stimulated Raman scattering (BSRS) are measured when an intense 532 nm nanosecond pulsed laser is focused into water and heavy water. The investigation reveals a significant observation: the formation of the ice VII structure exclusively occurs in the backward direction when optical breakdown takes place, provided that the input energy falls below 90 mJ for liquid water or 75 mJ for heavy water. This phase transition is attributed to secondary shock compression, which comes from energy transfer and compression between the BSRS in plasmas with the pump laser. The optical breakdown experiment under pre-pressure reveals that the shock compression in the back direction is approximately 2.3 times that of the forward direction. This research is useful for shock compression and dynamics in plasmas. [ABSTRACT FROM AUTHOR]

Over the past six decades, dye laser technology has improved substantially. The usage of solid matrices containing laser dyes is becoming more and more popular as a viable substitute for the traditional liquid dye solutions. In this research, we designed and built a tunable solid dye laser device which consists of three main parts. (i) The active material producing the laser beam, which is a polymer rod [glycidyl methacrylate (GMA) polymer] doped with the laser dyes pyrromethene 597 (PM-597) or Nile blue (Nb-690). (ii) The pumping source is xenon linear flashlamp driven by a homemade power supply. (iii) Two broadband mirrors providing the optical feedback stable optical resonator. The properties of the gain medium and hence the laser emission characteristics were determined, and the results showed the efficiency of the homemade tunable solid dye laser device, that is suitable for a variety of applications. [ABSTRACT FROM AUTHOR]

Quantitative measurements of atmospheric total OH reactivity (k OH ') provide crucial insights into atmospheric photochemistry. However, widespread application of total OH reactivity measurements is challenging due to insufficient equipment and the complexity of existing instrumentation. In this work, we report the development of a portable laser-flash photolysis Faraday rotation spectroscopy (LP-FRS) instrument for real-time and in-situ measurement of k OH '. To achieve efficient overlapping between the pump and probe laser and realize a long effective absorption path length, thus enabling high sensitivity measurement, a specific Herriott-type pump-probe optical multi-pass cell was designed with an overlapping factor of up to 75.4 %. The instrument's optical box dimensions were 130 cm × 40 cm × 35 cm. The obtained efficient absorption path was ~ 28.5 m in a base length of 77.2 cm. The k OH ' detection precisions of the LP-FRS instrument were 2.3 s-1 and 1.0 s-1 with averaging times of 60 s and 300 s, respectively. The k OH ' measurement uncertainty was evaluated to be within 2 s-1. Field measurement was performed, and the difference between the measured k OH ' and the model simulated from the measured reactive species was analysed. The developed portable LP-FRS instrument extends the measurement methods of atmospheric total OH reactivity, and has certain advantages in cost, operation, and transportation, which will play an increasingly important role in future atmospheric chemistry research. [ABSTRACT FROM AUTHOR]

To date, supercontinuum light in the visible and near‐infrared ranges is readily realizable by the optical Kerr effect through self‐phase modulation of ultrashort laser pulses in transparent media. However, it is still a challenge to extend the supercontinuum spectrum down to the deep‐ultraviolet (DUV) range, which is particularly needed for exploring ultrafast dynamics in chemistry, materials, and biology. Here, an approach of non‐resonant coherent Raman scattering is developed to generate ultra‐broadband visible‐DUV supercontinuum in ambient air with a spectral range spanning over 250 nm and a wavelength down to 220 nm. A rovibrational coherence is established in air molecules by filamentation of a near‐infrared femtosecond 800 nm pulse and two femtosecond Raman laser pulses at 267 and 400 nm are introduced into the coherent media to induce non‐resonant coherent Stokes and anti‐Stokes Raman scatterings, which serve as the spectral bridges to link the neighboring Raman pump laser spectra, resulting in ultra‐broadband supercontinuum light. The mechanism is further verified by examining the broadening of picosecond N2+ laser lines with narrow bandwidths (10–30 cm−1), which forms a supercontinuum spectrum spanning over 150 nm. The work provides a viable route for the establishment of coherent DUV supercontinuum in the gas media at designed wavelength ranges. [ABSTRACT FROM AUTHOR]

We design and simulate a near-zero flat dispersion As2S3 photonic crystal fiber (PCF) with a circular shape to generate a broad and smooth supercontinuum (SC). A near-zero flattened dispersion in the all-normal dispersion PCF is maintained in the 4–6.2 μ m wavelength range. A 6 μ m hyperbolic pulse is injected into this fiber, producing a flat spectrum from 2.45 to 8.4 μ m at a peak power of 5 kW. The generated SC in anomalous dispersion PCF can cover multi-octaves by a pump laser with a 6500 nm wavelength, 10 kW of peak power, and a 90 fs duration in 10 cm of the proposed fiber structure. These results are achieved by optimizing the fiber structure through the core size. In general, the proposed structures could be used for broadband smooth low-cost SC generation. [ABSTRACT FROM AUTHOR]

Bright yellow upconversion emission spectra at 595 nm were investigated in Nd3+ ions doped gadolinium orthovanadate (GdVO 4) single crystals. 556-fold enhancement of the intensity of upconversion emission at 595 nm was investigated at the sample temperature of 400 °C, which followed the exponential increase with temperature. The lg-lg relationships of the detected upconversion emission spectra and the input pumping laser were discussed, which dropped to 2.28 at high temperature from 5.98 at low temperature and implied fewer photons are required at higher temperatures. Thermal phonon-assisted excitation and electron-phonon coupling activities played important roles in the one photon upconversion emission excited by the laser centered at 1064 nm, and over 3700-fold enhancement of the emission peaks at 756 nm was observed. The finding in this work provides thermal stability analysis in Nd3+ ions doped laser materials and expands rare earth ions upconversion mechanisms. [ABSTRACT FROM AUTHOR]

Herein, the lasing threshold and gain characteristics of ultraviolet‐C optically pumped edge‐emitting lasers with thick single‐quantum‐well (SQW) active regions are investigated by the variable‐stripe length method. Positive net modal gain is observed in lasers with AlGaN‐based SQWs with thicknesses up to 12 nm. The lasers show a reduction of the threshold power density with increasing SQW thickness, with the lowest threshold of 1.3 MW cm−2 achieved for a 9 nm SQW laser. The high gain and low threshold in lasers with thick quantum wells are attributed to lasing from excited states, where the polarization fields are screened by the carriers in the fundamental state and the barriers, thus recovering larger electron and hole wavefunctions overlap. These findings are supported by k · p simulations, and for a 9 nm SQW, the calculation predicts a contribution of the fundamental transition to the gain of 75% for non‐resonant optical excitation and below 1% for resonant optical or electrical excitation. [ABSTRACT FROM AUTHOR]

The effect of wet etching on the characteristics of ultraviolet‐B (UV‐B) lasers fabricated on AlGaN templates grown as crystals or wet‐etched AlN nanopillars is compared in detail. Specifically, a tetramethylammonium hydroxide (TMAH) solution is used to form templates with AlN nanopillars of different diameters, followed by determining the dependence of the dislocation density in AlGaN crystals grown on the templates, the threshold power density (Pth) of an optically pumped UV‐B laser, and the threshold current density (Jth) of a UV‐B laser diode (LD) on the extent of etching. It is observed that the pillar diameter decreases almost linearly as the etching time with the TMAH solution increases. The dislocation density of AlGaN crystals grown on AlGaN templates is almost independent of the etching time. Meanwhile, Pth of the optically pumped UV‐B laser is almost halved upon etching with TMAH. Finally, the Jth of the UV‐B LD tends to decrease by 10%–20% upon etching. The optical gain is estimated by optical excitation; wet etching of AlN nanopillars with TMAH solution results in a larger optical gain at the same excitation intensity, indicating that nonradiative recombination centers, such as point defects, are reduced. [ABSTRACT FROM AUTHOR]

We demonstrate an all-fiber oscillator with high optical-to-optical efficiency using laser diodes working at 915nm as the pump sources to reduce the demand for thermal management. When the output power of the bidirectional pumped oscillator is 1.16kW, the optical-to-optical efficiency is as high as 75.4%. In this working state, the output characteristics of the oscillator are observed. The Raman suppression ratio is 41.23dB and the beam quality factor Mx2 = 1.14, My2 = 1.29. Analyzing the time trajectory of the highest power output, there are no significant characteristic peaks in the time domain signal and the frequency domain signal, which indicates that the oscillator has good stability.Improving the output characteristics of the 915nm pumping lasers has a positive significance for the application of non-strict ambient temperature control. [ABSTRACT FROM AUTHOR]

The synthesis of multiple narrow optical spectral lines, precisely and independently tuned across the near- to mid-infrared region, is a pivotal research area that enables selective and real-time detection of trace gas species within complex gas mixtures. However, existing methods for developing such light sources suffer from limited flexibility and very low pulse energy, particularly in the mid-infrared domain. Here, we introduce a concept that is based on the combination of an appropriate design of near-infrared fiber laser pump and cascaded configuration of gas-filled anti-resonant hollow-core fiber technology. This concept enables the synthesis of multiple independently tunable spectral lines, with >1 μJ high pulse energies and a few nanoseconds pulse width in the near- and mid-infrared regions. The number and wavelengths of the generated spectral lines can be dynamically reconfigured. A proof-of-concept laser beam synthesized of two narrow spectral lines at 3.99 µm and 4.25 µm wavelengths is demonstrated and combined with photoacoustic modality for real-time SO2 and CO2 detection. The proposed concept also constitutes a promising way for infrared multispectral microscopic imaging. Here, the authors develop a concept for the synthesis of multiple narrow and intense optical spectral lines over a broad infrared region. This concept constitutes a promising way for multi-gas detection and multispectral microscopic imaging. [ABSTRACT FROM AUTHOR]

Generation of short wavelengths is obtained using the gas cells having different lengths. A Ti:sapphire laser system at 1 kHz or 10 Hz repetition rate is used to produce high harmonic generation (HHG). The gas cell producing optimum harmonic spectrum is determined using the 1 kHz laser system. The optimum harmonic signal is obtained under the phase-matched condition. The total harmonic yield is increased by adjusting argon gas pressure in the different gas cell lengths (length of the interaction mediums). Harmonics up to the 27th order are obtained. The 1D model is used for the calculation of harmonic yield at different interaction lengths. The high-power laser system at the 10 Hz repetition rate is used to generate high-order harmonics. The harmonic orders are extended to the 35th harmonic in argon gas. A harmonic spectrum in H2 gas is generated using different pump laser power. The power dependence of the harmonic signal from H2 gas is obtained. The variation of the harmonic spectrum for the different cell parameters is explained as a constructive or destructive buildup of generated harmonics while they propagate through the gas cell. [ABSTRACT FROM AUTHOR]

This research proposes a new technique for measuring the energy characteristics (losses of energy in the spark gap, related to light radiation, ionization, excitation, and heating of the working gas during the development of plasma; discharge power) of two-electrode gas dischargers in the subnanosecond range. The work examines the voltage waveforms across the discharge gas gap and the discharge current waveform obtained by the reflectometry method in the subnanosecond range. To do this, the traditional technique for measuring such characteristics was modified. This allows us to restore the back edge of the voltage pulse across the discharge gap at the breakdown delay and the breakdown stages, which is usually lost in the subnanosecond range when measuring such waveforms. For modification, calculated data on the ionization frequency were used. This allows us to replace the plasma of the discharge gap with a constant resistor in those sections of the voltage waveform where the characteristic ionization time is more than an order of magnitude longer than the duration of the voltage pulse applied to the gap. The waveforms of the voltage across the discharge gap and the discharge current obtained in this way allowed us to calculate the power dynamics and total energy introduced into the gas discharge plasma. These parameters are important both for calculating the efficiency of gas switches and for other applications of gas discharge plasma, in particular laser pumping. [ABSTRACT FROM AUTHOR]

The potential energy curves and transition dipole moments of seven Λ-S states and six Ω states of LuH+ cation are calculated by using the multireference configuration interaction method plus Davidson correction with the pseudopotential electron basis set, and the spectroscopic parameters of the bound states are obtained. The spin–orbit coupling effect is considered in the calculations. The Franck–Condon factors (FCFs) and the Einstein spontaneous emission coefficients are obtained. The results indicate that the A2Δ3/2(ν′ = 0) ↔ X2Σ+1/2(ν″ = 0) and B2Π1/2(ν′ = 0) ↔ X2Σ+1/2 (ν″ = 0) transitions provide highly diagonally distributed FCFs. Spontaneous radiative lifetimes of A2Δ3/2 (ν′ = 0) and B2Π1/2 (ν′ = 0) excited states are both obtained. The cooling schemes of LuH+ cation are obtained using the ab initio method. For the B2Π1/2 ↔ X2Σ+1/2 transition, the influence of the intermediate state on the construction of quasi-closed cyclic transitions can be neglected. A main pump laser and two repumping lasers are required to construct the A2Δ3/2 ↔ X2Σ+1/2 and B2Π1/2 ↔ X2Σ+1/2 quasi-cycling transitions for laser cooling of LuH+ molecular cation. The results in this work provide reliable theoretical guidance for further experiments of laser cooling of LuH+ cation. [ABSTRACT FROM AUTHOR]

We present a high performance top emitting room temperature monolithic terahertz (THz) quantum cascade laser based on difference frequency generation (DFG) and a buried modulated distributed feedback grating. Using a semi-insulating InP:Fe substrate combined with an index-coupled grating could minimize the internal losses for the THz mode. The laser consists of two separate transversely superimposed gratings. The first grating provides selective feedback for the mid-infrared pump modes and is realized in an index-coupled DFG grating designed for single-mode operation for two distinct MIR wavelengths. The second metallic grating for THz extraction is carefully aligned to the spatial distribution of the MIR modes. The resulting device lases pulses up to 150 °C in the single mode. The maximum THz output power at RT is 100 μW measured at 3.37 THz. A THz wavelength tuning of around 0.065 nm/K was achieved through thermal tuning of the MIR pump lasers. [ABSTRACT FROM AUTHOR]

The laser plasmas produced from the interaction of the high-power laser with the target surface are suitable sources for soft X-ray laser, which has many applications in industry and medicine. In order to create the maximum efficiency of the output soft X-ray laser, the parameters of the pump laser should be optimize. In a double-pulse pump laser, the intensity and width of the pre-pulse, the intensity and width of the main pulse and the delay time between the two pulses are effective parameters in the output X-ray production. In this research, by using a machine learning based on the multiple regression equation, the dependence of the gain coefficient on the pump pulse parameters are investigated and a statistical model for predicting the gain coefficient of soft x-ray laser based on the feature of the pump pulse is presented without the need to numerical solution of the complex hydrodynamic equations. [ABSTRACT FROM AUTHOR]

In this work, experimental studies on the effect of dephasing on modulation transfer are reported. Here Potassium D1 transition, i.e., 39K 4S1/2(F) → 4P1/2(F/), is used as the medium. The 4 S→4P connection is modified by introducing two independent lasers. The separation between ground hyperfine states 4S1/2(F = 2,1) is almost half of Doppler width (~ 815 MHz). Hence, the two-level connections satisfied by respective lasers are overlapping in nature. In such cases, the existing optical pumping for particular F = 1, 2→ F/ channel influences each other. Further, the D1 transition itself is an open transition, i.e., it does not have any cyclic decay route. Hence, decay from each of the F/=2,1 states can also influence the population in the other F/state. Our pump-probe spectroscopy results clearly show the presence of Four Wave Mixing due to degenerate two-level and Vee (V) coupling, Electromagnetically Induced Transparency (EIT) signals due to single Lambda (Λ) and Double Λ connections. We have studied these signals as a function of dephasing, which is mainly contributed by transit time broadening for two different regimes of pump laser intensities: (i) below and (ii) above saturation intensity level of 4S1/2(F) → 4P1/2(F/) transition. The pump laser is current modulated, and phase-sensitive detection is performed on the probe transmission to study modulation transfer under different values of coherent dephasing. For this purpose, the beam size of the pump laser is varied systematically. This study provides a scope to explore the modulation transfer as a function of transit time broadening, and it may find applications in photonics technology where potassium vapor is used as a medium. [ABSTRACT FROM AUTHOR]

Widely separated optical parametric oscillation (OPO) in an integrated Kerr microresonator offers a compact, highly coherent, and low‐power laser source, accessing previously inaccessible frequencies. Yet, extending the sideband of OPO from telecom to beyond 2 µm is still challenged by competing nonlinear effects and reduced Q factors at these extended wavelengths. In this work, efficient signal‐idler separations reaching 99 THz (1250–2130 nm) are demonstrated with a modest 8.1 mW threshold power, leveraging the heightened nonlinearity of GeSbS chalcogenide glass in the integrated microresonators. By pioneering energy dissipation control via pulley couplers, competing nonlinear phenomena are effectively suppressed, enabling the first demonstration of a widely separated OPO (wOPO) in the anomalous dispersion regime. Moreover, the wOPO features a robust existence region across a variety of device geometries, resilient to microresonator width alterations of up to 300 nm. These findings underscore the potential of integrated microresonators to adeptly bridge the telecom band to the MIR spectrum, achieving this transition with minimal power and controlled nonlinearities, a promising avenue for contemporary integrated photonics platforms utilizing heterogeneously integrated pump lasers. [ABSTRACT FROM AUTHOR]

Lanthanide-ion-doped red upconversion (UC) fluorescent materials with excellent signal-to-noise ratio, stability, and red-green luminous intensity ratio have proven of tremendous research importance for biomedical, three-dimensional (3D) displays, sensors, and other sectors. In this study, xYb, 1Er: Sr 5 (PO 4) 3 F (S-FAP) (x=0–5 at%) transparent ceramics with outstanding optical quality were fabricated by hot pressing the co-precipitation powder with high sintering activity. The energy dispersive X-ray (EDX) results showed that the trivalent lanthanide ions were evenly doped into the S-FAP ceramic lattice. Increased Yb3+ doping considerably restricted the growth of ceramic grain size, which should be attributable to a decrease in sintering activity under high Yb doping conditions. The co-doping of Yb3+ successfully resulted in a significant improvement in up/down conversion efficiency via effective energy transfer mechanisms and the optimization of the electron population at the energy level of red-green emission. Furthermore, single-band red upconversion luminescence with the greatest red-green upconversion luminescence integral intensity ratio of 125.74 was discovered under 980 nm laser pumping at room temperature. The energy transition process involved in the phenomenon of the up-conversion luminescence intensity shift of red-green emission has been thoroughly examined. Finally, the noncontact optical thermometric ability based on fluorescence intensity ratio (FIR) technology showed that the maximum absolute sensitivity (Sa) of the 5Yb1Er sample in the temperature range of 320–556 K is 1.1×10−3 K−1, implying the possible use of Yb/Er-doped S-FAP transparent ceramics in the field of optical thermometers. [ABSTRACT FROM AUTHOR]

Optical frequency combs in the 2 μm wavelength region are important for applications ranging from sensing of gases such as CO2 and CO to optical communications, LIDAR, and gravitational wave detection. The development of low-loss waveguides and high-Q microresonators with anomalous dispersion and the availability of tunable narrow linewidth lasers around 1.55 μm have enabled the realization of small footprint soliton combs and low-threshold Kerr combs in this wavelength region; demonstrations of microresonator frequency combs in the 2 μm wavelength region have been limited. Here, we harness an intracavity pumping scheme to demonstrate a low-threshold (< 100 mW) microresonator Kerr comb at 2 μm. We exploit Brillouin lasing in a silica microsphere (∼310 μm diameter) to create an intracavity pump, which then generates a ∼140 nm wide Kerr comb in the backscattered Stokes direction. We demonstrate the tolerance of the comb generation scheme to microsphere dimensions and the input pump wavelength by achieving Kerr comb generation in microspheres of diameters ranging from 295 to 318 μm and also at different input pump wavelengths for a particular microsphere diameter. Intracavity pumping opens up opportunities for the development of soliton combs and Kerr combs in the mid-IR wavelength region for applications such as dual-comb spectroscopy, LIDAR, and optical communications. [ABSTRACT FROM AUTHOR]

Diode-pumped multi-mode graded-index (GRIN) fiber Raman lasers provide prominent brightness enhancement both in linear and half-open cavities with random distributed feedback via natural Rayleigh backscattering. Femtosecond laser-inscribed random refractive index structures allow for the sufficient reduction in the Raman threshold by means of Rayleigh backscattering signal enhancement by +50 + 66 dB relative to the intrinsic fiber level. At the same time, they offer an opportunity to generate Stokes beams with a shape close to fundamental transverse mode (LP01), as well as to select higher-order modes such as LP11 with a near-1D longitudinal random structure shifted off the fiber axis. Further development of the inscription technology includes the fabrication of 3D ring-shaped random structures using a spatial light modulator (SLM) in a 100/140 μm GRIN multi-mode fiber. This allows for the generation of a multi-mode diode-pumped GRIN fiber random Raman laser at 976 nm with a ring-shaped output beam at a relatively low pumping threshold (~160 W), demonstrated for the first time to our knowledge. [ABSTRACT FROM AUTHOR]

High‐power broadband near‐infrared (NIR) light sources have received extensive attention in long‐distance night vision lighting, non‐invasive detection and imaging, and quantitative analysis of organic components. However, developing targeted NIR‐emitting phosphors with high external quantum efficiency (EQE) and thermal stability remains a challenge to raise the NIR output power and expand the applications. Herein, Ga1.98−xScxO3:0.02Cr3+ luminescent ceramics are prepared with redshifted emission peaks from 710 to 820 nm depending on the weakened crystal field. The optimized Ga1.18Sc0.8O3:0.02Cr3+ ceramic exhibits a high EQE of 79.6% and excellent thermal stability (I423 K/I298 K = 72%) under 468 nm excitation, which brings a saturation threshold up to 893 mW@3 W mm−2 under 450 nm laser pumping. The high‐power laser‐driven broadband NIR light source demonstrates potential in non‐invasive detection and quantitative analysis of alcohol concentration. This study opens up new avenues for the exploration of high‐power broadband NIR light sources. [ABSTRACT FROM AUTHOR]

2 μm pulsed lasers not only have critical applications in military, medical, and processing fields but are also an important frontier in laser physics. The development of these pulsed lasers has been hindered by the lack of laser crystals with both high thermal conductivity and broad spectral properties. In this work, Tm, Ho:CaGdAlO4 disordered crystal with ultra-broad emission spectra around 2 μm was achieved successfully by modulating the emission intensities of Tm3+ and Ho3+ ions to the same level. The FWHM of the absorption spectra at 793 nm for the <001> and <100> directions are 18.69 and 19.44 nm, respectively, which is beneficial for commercial laser diode pumping. More importantly, the FWHM of the emission spectrum is 264 nm, which is the widest one reported in the previous literature. The results indicate that the Tm, Ho:CaGdAlO4 crystal with its broader spectra has the potential to generate an ultrashort pulse laser. [ABSTRACT FROM AUTHOR]

Coherent optics has profoundly impacted diverse applications ranging from communications, LiDAR to quantum computations. However, developing coherent systems in integrated photonics comes at great expense in hardware integration and energy efficiency. Here we demonstrate a high-coherence parallelization strategy for advanced integrated coherent systems at minimal cost. By using a self-injection locked microcomb to injection lock distributed feedback lasers, we achieve a record high on-chip gain of 60 dB with no degradation in coherence. This strategy enables highly coherent channels with linewidths down to 10 Hz and power over 20 dBm. The overall electrical-to-optical efficiency reaches 19%, comparable to that of advanced semiconductor lasers. This method supports a silicon photonic communication link with an unprecedented data rate beyond 60 Tbit/s and reduces phase-related DSP consumption by 99.99999% compared to traditional III-V laser pump schemes. This work paves the way for realizing scalable, high-performance coherent integrated photonic systems, potentially benefiting numerous applications. Researchers demonstrate the high-coherence parallelization in integrated photonics. Their high-coherence, high-power, multiwavelength light source drives a silicon photonic link with a 60 Tbit/s data rate and significantly reduces digital signal processing consumption. [ABSTRACT FROM AUTHOR]

Mode‐locked ultrashort pulse sources with a repetition rate of up to several tens of gigahertz greatly facilitate versatile photonic applications such as frequency synthesis, metrology, radar, and optical communications. Dissipative Kerr soliton microcombs provide an attractive solution as a broadband, high‐repetition‐rate compact laser system in this context. However, its operation usually requires sophisticated pump laser control to initiate and stabilize the soliton microcombs, particularly in millimeter‐sized ultrahigh‐Q whispering‐gallery resonators. Here, a mechanically actuated soliton microcomb oscillator is realized with a microwave repetition rate of 15 GHz. This enables direct initiation, subsequent long‐term stabilization, and fine tuning of soliton combs without pump laser tunability that is generally required for soliton microcomb operation. The prospects for using this method with a wide range of applications are revealed that will benefit from mechanical soliton actuation such as optical clocks, spectral extension, and dual‐comb spectroscopy. [ABSTRACT FROM AUTHOR]

Widespread commercial adoption of telecom‐band quantum key distribution (QKD) will require fully integrated, room‐temperature transmitters. Implementing highly efficient spontaneous parametric down‐conversion (SPDC) on a platform that offers co‐integration of the pump laser has been an outstanding challenge. Here, using such a platform based on AlGaAs‐on‐insulator waveguides, telecom‐band SPDC (and SHG, second harmonic generation) is reported with exceedingly large efficiencies of 26 GHz generated pairs per mW over a 7 THz bandwidth, which would saturate the usable photon‐flux for a 70‐channel wavelength‐multiplexed QKD system at merely 1.7 mW of pump laser power. [ABSTRACT FROM AUTHOR]

It is shown theoretically that the two-plasmon-decay instability (TPD) in laser–plasma interaction can be excited in the non-eigenmode regime, where the plasma density is larger than the quarter critical density. This appears when the laser amplitude is larger than a certain threshold value, which is found to increase with the plasma density. In this regime, the excited electrostatic modes have a constant frequency around half of the incident light frequency. The theoretical model is validated by particle-in-cell simulations. The simulation results show that the non-eigenmode TPD has a higher threshold amplitude for the pump laser than the non-eigenmode stimulated Raman scattering (SRS) excited in the plasma above the quarter critical density. In inhomogeneous plasma, competition between non-eigenmode TPD and non-eigenmode SRS occurs since the excitation of the former is normally accompanied by the latter. [ABSTRACT FROM AUTHOR]

Polymer fibers are considered ideal transmission media for all-optical networks, but their high intrinsic loss significantly limits their practical use. Quantum dot-doped polymer fiber amplifiers are emerging as a promising solution to this issue and are becoming a significant focus of research in both academia and industry. Based on the properties of CdSe/ZnS quantum dots and PMMA material, this study experimentally explores three fabrication methods for CdSe/ZnS quantum dots-doped PMMA fibers: hollow fiber filling, melt-drawing, and melt extrusion. The advantages and disadvantages of each method and key issues in fiber fabrication are analyzed. Utilizing the CdSe/ZnS quantum dots-doped PMMA fibers that were fabricated, we theoretically analyzed the key factors affecting gain performance, including fiber length, quantum dots doping concentration, and signal light intensity. Under the conditions of 1.5 W power and 445 nm laser pumping, a maximum on-off gain of 16.2 dB was experimentally achieved at 635 nm. Additionally, using a white light LED as the signal source, a broadband on-off gain with a bandwidth exceeding 70 nm and a maximum gain of 12.4 dB was observed in the 580–650 nm range. This research will contribute to the development of quantum dots-doped fiber devices and broadband optical communication technology, providing more efficient solutions for future optical communication networks. [ABSTRACT FROM AUTHOR]

In the last decades, nonlinear optical microscopy techniques, such as two-Photon Excited Fluorescence (2PEF), Sum Frequency Generation (SFG), and Hyperspectral Coherent Anti-Stokes Raman Scattering (H-CARS) microscopy, emerged as powerful tools to image biological samples in a label-free, fast, and non-destructive way. Traditionally, these techniques are performed with single point-scanning acquisition schemes featuring a limited field of view and often leading to sample damage when high laser power is used to increase the acquisition speed. Wide-field illumination and camera-based detection schemes offer a solution to these issues, enabling fast imaging over a large field view. However, current laser sources used for nonlinear microscopy operating at several MHz repetition rates are not able to induce nonlinear effects over areas larger than 100 × 100 µm2. Here, we present a powerful 200 kHz repetition rate laser source based on an Ytterbium fiber laser pumping two picosecond optical parametric amplifiers tunable in the 700–900 nm spectral range and rapidly tunable (up to 100 KHz) within a 20 nm sub-range. We exemplify the possibilities of this laser system to perform rapid CARS spectroscopy (2 ms/spectrum) and nonlinear wide-field imaging, up to 3.3 frames/s for 2PEF and SFG and 0.3 hypercubes/s for H-CARS, over a field of view >300 × 300 µm2. [ABSTRACT FROM AUTHOR]

In this work, we demonstrate a Watt-level, high-quality Laguerre–Gaussian (LG) LG0±1 vortex mode directly output from an end-pumped Nd:YVO4 laser by using an axicon-based annular pump beam. A theoretical model for the annular beam end-pumped solid-state laser with an LG vortex mode output was established. Chirality control of the vortex laser was achieved by carefully tilting the output coupler. Watt-level 1064 nm lasers with pure LG0,1/LG0,−1 vortex mode, and the incoherent superposition mode of LG0,1 odd and even petal modes, were achieved successively in our experiments. The intensity profile of the generated pure LG0,1 vortex laser was measured, and it can be well fitted by using the standard expression of the LG0,1 vortex mode. The beam quality of the pure LG0,1 mode is Mx2 = 2.01 and My2 = 2.00 along the x-axis and y-axis, respectively. Our study demonstrates that that axicon-based annular pumping has great potential in developing high-power vortex solid-state lasers with simple and compact structures. [ABSTRACT FROM AUTHOR]

This paper systematically studies the output noise model of the K-Rb-21Ne co-magnetometer and proposes the method for determining the optimal pump laser power density. The amplitude-frequency response and the equivalent model for each frequency band are obtained through the transfer function of the co-magnetometer. Based on the established model and considering the power spectral density characteristics of magnetic noise, the output noise equation is formulated. Consequently, the pump laser power density yielding minimal output noise is determined. Both experimental and simulation results indicate that the pump laser power density yielding minimal output noise is greater than the pump laser power density corresponding to the maximum scale factor. Moreover, when the co-magnetometer operates at the pump laser power density corresponding to the minimal output noise, the output noise can be reduced by approximately 25%, and the Allan variance reaches its optimal value. The optimal Allan variance at 180 °C and 190 °C are 0.01395°/h @100 s and 0.01329°/h @100 s, respectively. Therefore, this pump laser power density is designated as the optimal pump laser power density for the co-magnetometer. Finally, simulations are conducted to investigate the variation patterns of the optimal pump laser power density points and the minimum output noise under different density ratios and gas pressures. The theories and methods proposed in this paper provide significant reference value for selecting the optimal pump laser power density and suppressing magnetic noise in co-magnetometers. [ABSTRACT FROM AUTHOR]

Holmium-doped congruent-composition lithium niobate (LiNbO3:Ho, LN:Ho) crystals were grown by the Czochralski method. The absorption of the LN:1at% Ho3+ crystal was recorded at room temperature. On the basis of the analysis of emission and absorption spectra of the LN:1at% Ho3+ crystal, the possibilities of obtaining, at room temperature, radiation-balanced (RB) lasing in the region of 640–670 nm wavelengths corresponding to the inter-Stark transitions of manifolds 5F5 and 5I8 was theoretically investigated. The RB lasing parameters were calculated and the optimal pump and laser wavelengths were determined: λ O P = 652.1   n m , λ O L = 653.6   n m . The values for the RB lasing efficiency and radiation amplification in the considered wavelength region were obtained: F e f f = 3.23 × 10 − 22 c m 2 ,   F g a i n = 6.08 × 10 − 22   c m 2 . [ABSTRACT FROM AUTHOR]

We study entanglement created between two isolated qubits by interaction with entangled-photon pairs obtained by parametric down-conversion of a laser pump field. The induced entanglement is quantified using the mixed state Concurrence proposed by Wootters et al. [Phys. Rev. Lett. 78, 5022 (1997)]. A universal value of qubit-entanglement, which is independent on the photon-pair wavefunction is identified to leading order in the qubit–field interaction and the pump field amplitude. The qubit entanglement decreases at higher laser pump intensities due to interference between the entangled photon pairs, which creates excitations in the qubit system. Maximal Concurrence is produced by only generating coherences between the ground and the highest excited qubit states. [ABSTRACT FROM AUTHOR]

Temperature is a crucial parameter in the spin-exchange optical pumping (SEOP) process of noble gas ( 3 He), but is hard to measure due to its confinement nature. In this paper, we conduct research upon the temperature and gas flow distribution within a sealed SEOP cell through computational fluid dynamics simulation. The simulation result shows that the external heat exchange of the initial heating of the cell becomes a cooling process in the presence of high pumping laser power absorbed by the alkali metal. The heat from the pumping laser would also cause the gas in the cell to reach a much higher temperature than the oven, with the hottest part appearing on the upper side of the cell. These predicted behaviors from the simulation are later confirmed by our experiment measurement, which strongly indicates that a gas flow and heat flow exist within the cell. These results help us to understand the temperature distribution of 3 He gas in the cell and provide references for the development and improvement of the future SEOP system. [ABSTRACT FROM AUTHOR]

Time-resolved photoionization measurements were performed on o-nitrophenol pumped with UV laser pulses at a central wavelength of 255 nm (4.9 eV) and probed with vacuum ultraviolet (VUV) pulses at 153 nm (8.1 eV). The photoelectron spectrum and time of flight mass spectrum for ions were recorded at each pump–probe delay. The measurements are interpreted with the aid of electronic structure calculations for both the neutral and ionic states. Evidence is found for the formation of a bicyclic intermediate followed by NO dissociation through a process of internal conversion and intersystem crossing. The combination of photoelectron and photoion spectroscopy, together with computational results, provides strong evidence of intersystem crossing that is difficult to establish with only a single technique. [ABSTRACT FROM AUTHOR]

In this work, we discuss and experimentally investigate the whispering gallery modes (WGMs) in a 500 μm radius silicon sphere. We begin by reviewing the basics of WGM resonators, followed by simulations and experimental results obtained with the aforementioned silicon spherical WGM resonator. The recorded WGM signatures in the transmission and scattering spectra excited, in the near-infrared (near-IR) region, agree well with the simulations. Thermo-optic tuning of these WGMs is achieved by introducing a pump laser in the violet-blue region. Red-shifts in wavelength are observed, which increase with the increase in the pump power. A shift of 0.63 nm is observed at a pump power of 6.32 mW. We also study switching by analysing the transient response of the WGM spectra. The measured WGMs exhibit high quality factors ($Q\sim 10^5$Q∼105), which along with the aforesaid tunability, demonstrates the potential of spherical silicon resonator as a platform for photonic applications, e.g. sensing and communication. In summary, this work contributes towards the understanding of the fundamental physics of WGMs and provides insights into silicon WGM resonators. [ABSTRACT FROM AUTHOR]

Erbium-doped glass microsphere laser systems hold significant promise in the applications of bio-medicine and optical fiber sensing. However, their development has been hindered by the relatively high laser pump threshold. In this study, we proposed a unique dual microsphere system where two microspheres are affixed to a single-mode fiber taper and achieved a remarkably low lasing threshold of 19 μW for single-mode laser emission at 1544 nm. This is in sharp contrast with the lasing threshold of 56 μW observed in single microspheres. Our findings represent a significant achievement in the development of low-threshold, compact infrared laser sources for emerging applications in photonics. [ABSTRACT FROM AUTHOR]

9,9‐bis (diphenylphosphorylphenyl) fluorene (FDPO) and dibenzotetrathienoacene (DBTTA), are synthesized as the neutral and anionic ligands, respectively, to prepare the ErIII coordination polymer [Er(DBTTA)3(FDPO)]n. Based on the intramolecular energy transfer, optical gains at 1.5 µm are demonstrated in [Er(DBTTA)3(FDPO)]n‐doped polymer waveguides under excitations of low‐power light‐emitting diodes (LEDs) instead of laser pumping. A ligand‐sensitization scheme between organic ligands and Er3+ ions under an excitation of an ultraviolet (UV) LED is established. Relative gains of 10.5 and 8.5 dB cm−1 are achieved at 1.53 and 1.55 µm, respectively, on a 1‐cm‐long SU‐8 channel waveguide with a cross‐section of 2 × 3 µm2 and a 1.5‐µm‐thick [Er(DBTTA)3(FDPO)]n‐doped polymethylmethacrylate (PMMA) as upper cladding. The ErIII coordination polymer [Er(DBTTA)3(FDPO)]n can be conveniently integrated with various low‐loss inorganic waveguides to compensate for optical losses in the C‐band window. Moreover, by relying on the intramolecular energy transfer and UV LED top‐pumping technology, it is easy to achieve coupling packaging of erbium‐doped waveguide amplifiers (EDWAs) with pump sources in planar photonic integrated chips, effectively reducing the commercial costs. [ABSTRACT FROM AUTHOR]

Dissipative Kerr soliton microcombs in microresonators have enabled fundamental advances in chip-scale precision metrology, communication, spectroscopy, and parallel signal processing. Here we demonstrate polarization-diverse soliton transitions and deterministic switching dynamics of a self-stabilized microcomb in a strongly-coupled dispersion-managed microresonator driven with a single pump laser. The switching dynamics are induced by the differential thermorefractivity between coupled transverse-magnetic and transverse-electric supermodes during the forward-backward pump detunings. The achieved large soliton existence range and deterministic transitions benefit from the switching dynamics, leading to the cross-polarized soliton microcomb formation when driven in the transverse-magnetic supermode of the single resonator. Secondly, we demonstrate two distinct polarization-diverse soliton formation routes – arising from chaotic or periodically-modulated waveforms via pump power selection. Thirdly, to observe the cross-polarized supermode transition dynamics, we develop a parametric temporal magnifier with picosecond resolution, MHz frame rate and sub-ns temporal windows. We construct picosecond temporal transition portraits in 100-ns recording length of the strongly-coupled solitons, mapping the transitions from multiple soliton molecular states to singlet solitons. This study underpins polarization-diverse soliton microcombs for chip-scale ultrashort pulse generation, supporting applications in frequency and precision metrology, communications, spectroscopy and information processing. Thermal Instability hinders reliable generation of dissipative Kerr solitons in Silicon Nitride microresonators. The authors investigate a regime where polarization-diverse soliton transitions and deterministic dynamics of a self-stabilized microcomb in a dispersion managed microresonator driven with a single pump laser. [ABSTRACT FROM AUTHOR]

Microresonator frequency combs (microcombs) hold great potential for precision metrology within a compact form factor, impacting a wide range of applications such as point-of-care diagnostics, environmental monitoring, time-keeping, navigation and astronomy. Through the principle of self-injection locking, electrically-driven chip-based microcombs with minimal complexity are now feasible. However, phase-stabilisation of such self-injection-locked microcombs—a prerequisite for metrological frequency combs—has not yet been attained. Here, we address this critical need by demonstrating full phase-stabilisation of a self-injection-locked microcomb. The microresonator is implemented in a silicon nitride photonic chip, and by controlling a pump laser diode and a microheater with low voltage signals (less than 1.57 V), we achieve independent control of the comb's offset and repetition rate frequencies. Both actuators reach a bandwidth of over 100 kHz, enabling phase-locking of the microcomb to external frequency references. These results establish photonic chip-based, self-injection-locked microcombs as low-complexity yet versatile sources for coherent precision metrology in emerging applications. Phase-stabilized frequency combs are critical for optical precision measurements. They have now been realized in a chip-scale format with CMOS compatible electrical control [ABSTRACT FROM AUTHOR]

The present research includes studying the optical linear and nonlinear characteristics of two organic laser dyes: Nile Blue (NB), Malachite Green (MG) and their mixture at room temperature, a mixture proportions involving organic laser dye concentrations (2×10-5, 4×10-5, 6×10-5, 8×10-5) M in chloroform solvent was analyzed. Every produced sample has had its linear optical characteristics examined. Next, the UV-VIS spectra of various dye concentrations dissolved in absolute chloroform solvent have been examined. Finally, the absorption spectra of every sample have been examined. The results demonstrated that at the same wavelength, absorbance rose along with concentrations. The Z-scan technology was utilized to compute the nonlinear absorption coefficient (β) and nonlinear refractive index (n2) for the produced samples in both open and closed aperture settings. The experiments were carried out using a solid-state laser with a diode pump that runs at 457 nm in wavelength and power of (84 mW). The results showed increasing of the nonlinear refractive index while declining nonlinear absorption coefficient for all organic laser dye samples at higher concentrations. Dyes mixture have large optical characteristics, both linear and nonlinear, in comparison to pure dyes. [ABSTRACT FROM AUTHOR]

We report direct measurement of the laser induced ionization rate of cesium, relevant for a Diode Pumped Alkali Laser (DPAL), via application of an ion chamber diagnostic. Computer simulation predictions of the multi-step ionization mechanism will be compared against measured ionization rates. The results will be shown to accurately predict the low level of ionization to within an order-of-magnitude, as well as relative trends across pump intensities of 8–100 W/cm 2 and cesium densities of 0.3–2.2 × 10 12 cm - 3 . Comparison of fluorescence from 7P energy states with known direct excitation pathways and fluorescence from highly-excited 7D states suggests rapid mixing of high energy states. The application of 300 V on the ion chamber electrodes (sufficient to cause current saturation) has minimal impact on fluorescence. This supports the notion that Rydberg states are populated via a neutral particle process, rather than via electron/ion recombination, as has been previously suggested. [ABSTRACT FROM AUTHOR]

Halide perovskite materials are considered a promising optical gain medium for stimulated emission and have aroused tremendous interest in the field of laser research. The development of low‐threshold optically pumped amplified spontaneous emission (ASE) is critical for the advancement of continuous wave (CW) and electrically pumped micro‐nano lasers. In this work, an efficient ZnS additive is incorporated into the FA0.85MA0.15PbI2.55Br0.45 perovskite films to diminish the ASE threshold and extend the photostability by the dual‐site synergistic passivation. The experimental measurements and first‐principles calculations based on the density functional theory (DFT) are employed to elucidate the doping mechanism. The designed ZnS‐based perovskite films yield a mitigated ASE threshold of 8.5 µJ cm−2 with an elevated optical gain coefficient of 109.06 cm−1, which outperform those of the control films (12.7 µJ cm−2 and 74.10 cm−1). The in‐depth experimental characterizations and theoretical calculations have corroborated that the improvement of ASE performance can be ascribed to the dual‐site synergistic passivation effects of Zn2+ and S2−, which reduces the surface defects of perovskite films, suppresses the nonradiative charge recombination and improves the optical stability. This work provides a resultful strategy to construct the solution‐processed perovskite lasers with low thresholds and superior stability. [ABSTRACT FROM AUTHOR]

Coherent Raman Scattering Imaging offers quick and surface‐sensitive large‐area scans of specimens including fingerprinting of the substances, combined with low detection limits. By using a multi‐photon process, it offers orders of magnitude stronger surface signal in comparison to spontaneous Raman (SR) and fluorescence signals of the substrate are avoided by the detection principle and the near‐infrared laser wavelength. By exciting at a specific wavelength instead of measuring whole spectra the measurement time is remarkably reduced. Here, detecting organic thin films on glass surfaces is investigated. The detection of those thin films is relevant for production processes where the interfacial layer is influenced by the low surface energy of contaminants, especially polysiloxanes. The samples are manufactured by pipetting diluted polydimethylsiloxane (PDMS) in heptane in various concentrations (1%, 0.1%, 0.01%, and 0.001%) on glass substrates. After evaporation of the solvent, thin films of the silicone remain. The resulting average coverage of the thin films equals 100–0.1 μg cm−2. Measurements determine the detectability threshold with SR to 10 μg cm−2, while the acquired spectrum is used to determine characteristic peaks for the pump laser. Afterwards the samples are imaged at those wavenumbers with Coherent Raman Scattering (CRS) Imaging techniques providing a chemically‐specific contrast. [ABSTRACT FROM AUTHOR]

Multimode fibers are attractive for high-power lasers if transverse modes are efficiently controlled. Here, a dielectric thin-film mirror (R~20%) is micro-fabricated on the central area of the end face of a 1 km multimode 100/140 µm graded-index fiber and tested as the output mirror of a Raman laser with highly multimode (M2~34) 940 nm diode pumping. In the cavity with highly reflective input FBG, Raman lasing of the Stokes wave at 976 nm starts at the threshold pump power of ~80 W. Mode-selective properties of mirrors with various diameters were tested experimentally and compared with calculations in COMSOL, with the optimum diameter found to be around 12 µm. The measured Raman laser output beam at 976 nm has a quality factor of M2~2 near the threshold, which confirms a rather good selection of the fundamental transverse mode. The power scaling capabilities, together with a more detailed characterization of the output beam's spatial profile, spectrum, and their stability, are performed. An approximately 35 W output power with an approximately 60% slope efficiency and a narrow spectrum has been demonstrated at the expense of a slight worsening of beam quality to M2~3 without any sign of mirror degradation at the achieved intensity of >30 MW/cm2. Further power scaling of such lasers as well as the application of the proposed technique in high-power fiber lasers are discussed. [ABSTRACT FROM AUTHOR]

Ytterbium laser sources are state-of-the-art systems that are increasingly replacing Ti:Sapphire lasers in most applications requiring high repetition rate pulse trains. However, extending these laser sources to THz Time-Domain Spectroscopy (THz-TDS) poses several challenges not encountered in conventional, lower-power systems. These challenges include pump rejection, thermal lensing in nonlinear media, and pulse durations exceeding 100 fs, which consequently limit the detection bandwidth in TDS applications. In this article, we describe our design of a THz-TDS beamline that seeks to address these issues. We report on the effectiveness of temperature controlling the Gallium Phosphide (GaP) used to generate the THz radiation and its impact on increasing the generation efficiency and aiding pump rejection while avoiding thermal distortions of the residual pump laser beam. We detail our approach to pump rejection, which can be implemented with off-the-shelf products and minimal customization. Finally, we describe our solution based on a commercial optical parametric amplifier to obtain a temporally compressed probe pulse of 55 fs duration. Our study will prove useful to the increasing number of laboratories seeking to move from the high-energy, low-power THz time-domain spectroscopy systems based on Ti:Sapphire lasers, to medium-energy, high-power systems driven by Yb-doped lasers. [ABSTRACT FROM AUTHOR]