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Over the past decade classical optical systems with gain or loss, modelled by non-Hermitian parity-time symmetric Hamiltonians, have been deeply investigated. Yet, their applicability to the quantum domain with number-resolved photonic states is fundamentally voided by quantum-limited amplifier noise. Here, we show that second-quantised Hermitian Hamiltonians on the Fock space give rise to non-Hermitian effective Hamiltonians that generate the dynamics of corresponding creation and annihilation operators. Using this equivalence between $\mathcal{PT}$-symmetry and symplectic Bogoliubov transformations, we create a quantum optical scheme comprising squeezing, phase-shifters, and beam-splitters for simulating arbitrary non-unitary processes by way of singular value decomposition. In contrast to the post-selection scheme for non-Hermitian quantum simulation, the success probability in this approach is independent of the system size or simulation time, and can be efficiently Trotterised similar to a unitary transformation., Comment: 7 pages, 1 figure

The heralded generation of entangled states underpins many photonic quantum technologies. As quantum error correction thresholds are determined by underlying physical noise mechanisms, a detailed and faithful characterization of resource states is required. Non-computational leakage, e.g. more than one photon occupying a dual-rail encoded qubit, is an error not captured by standard forms of state tomography, which postselect on photons remaining in the computational subspace. Here we use the continuous-variable (CV) formalism and first quantized state representation to develop a simulation framework that reconstructs photonic quantum states in the presence of partial distinguishability and resulting non-computational leakage errors. Using these tools, we analyze a variety of Bell state generation circuits and find that the five photon discrete Fourier transform (DFT) Bell state generation scheme [Phys Rev. Lett. 126 23054 (2021)] is most robust to such errors for near-ideal photons. Through characterization of a photonic entangling gate, we demonstrate how leakage errors prevent a modular characterization of concatenated gates using current tomographical procedures. Our work is a necessary step in revealing the true noise models that must be addressed in fault-tolerant photonic quantum computing architectures., Comment: 24 pages, 16 figures

Multi-photon interference is at the heart of photonic quantum technologies. Arrays of integrated cavities can support bright sources of single-photons with high purity and small footprint, but the inevitable spectral distinguishability between photons generated from non-identical cavities is an obstacle to scaling. In principle, this problem can be alleviated by measuring photons with high timing resolution, which erases spectral information through the time-energy uncertainty relation. Here, we experimentally demonstrate that detection can be implemented with a temporal resolution sufficient to interfere photons detuned on the scales necessary for cavity-based integrated photon sources. By increasing the effective timing resolution of the system from 200ps to 20ps, we observe a 20% increase in the visibility of quantum interference between independent photons from integrated micro-ring resonator sources that are detuned by 6.8GHz. We go on to show how time-resolved detection of non-ideal photons can be used to improve the fidelity of an entangling operation and to mitigate the reduction of computational complexity in boson sampling experiments. These results pave the way for photonic quantum information processing with many photon sources without the need for active alignment., Comment: 8 pages, 5 figures, 9 page supplementary material

Parity-time ($PT$) symmetric Hamiltonians are generally non-Hermitian and give rise to exotic behaviour in quantum systems at exceptional points, where eigenvectors coalesce. The recent realisation of $PT$-symmetric Hamiltonians in quantum systems has ignited efforts to simulate and investigate many-particle quantum systems across exceptional points. Here we use a programmable integrated photonic chip to simulate a model comprised of twin pairs of $PT$-symmetric Hamiltonians, with each the time reverse of its twin. We simulate quantum dynamics across exceptional points including two- and three-particle interference, and a particle-trembling behaviour that arises due to interference between subsystems undergoing time-reversed evolutions. These results show how programmable quantum simulators can be used to investigate foundational questions in quantum mechanics., Comment: 15 pages, 7 figures

Encoding high-dimensional quantum information into single photons can provide a variety of benefits for quantum technologies, such as improved noise resilience. However, the efficient generation of on-demand, high-dimensional entanglement was thought to be out of reach for current and near-future photonic quantum technologies. We present a protocol for the near-deterministic generation of $N$-photon, $d$-dimensional photonic Greenberger-Horne-Zeilinger (GHZ) states using an array of $d$ non-interacting single-photon emitters. We analyse the impact on performance of common sources of error for quantum emitters, such as photon spectral distinguishability and temporal mismatch, and find they are readily correctable with time-resolved detection to yield high fidelity GHZ states of multiple qudits. When applied to a quantum key distribution scenario, our protocol exhibits improved loss tolerance and key rates when increasing the dimensionality beyond binary encodings., Comment: 15 pages, 6 figures

Accurate models of real quantum systems are important for investigating their behaviour, yet are difficult to distill empirically. Here, we report an algorithm -- the Quantum Model Learning Agent (QMLA) -- to reverse engineer Hamiltonian descriptions of a target system. We test the performance of QMLA on a number of simulated experiments, demonstrating several mechanisms for the design of candidate Hamiltonian models and simultaneously entertaining numerous hypotheses about the nature of the physical interactions governing the system under study. QMLA is shown to identify the true model in the majority of instances, when provided with limited a priori information, and control of the experimental setup. Our protocol can explore Ising, Heisenberg and Hubbard families of models in parallel, reliably identifying the family which best describes the system dynamics. We demonstrate QMLA operating on large model spaces by incorporating a genetic algorithm to formulate new hypothetical models. The selection of models whose features propagate to the next generation is based upon an objective function inspired by the Elo rating scheme, typically used to rate competitors in games such as chess and football. In all instances, our protocol finds models that exhibit $F_1$-score $\geq 0.88$ when compared with the true model, and it precisely identifies the true model in 72% of cases, whilst exploring a space of over $250,000$ potential models. By testing which interactions actually occur in the target system, QMLA is a viable tool for both the exploration of fundamental physics and the characterisation and calibration of quantum devices., Comment: 29 pages, 7 figures

Identifying the boundary beyond which quantum machines provide a computational advantage over their classical counterparts is a crucial step in charting their usefulness. Gaussian Boson Sampling (GBS), in which photons are measured from a highly entangled Gaussian state, is a leading approach in pursuing quantum advantage. State-of-the-art quantum photonics experiments that, once programmed, run in minutes, would require 600 million years to simulate using the best pre-existing classical algorithms. Here, we present substantially faster classical GBS simulation methods, including speed and accuracy improvements to the calculation of loop hafnians, the matrix function at the heart of GBS. We test these on a $\sim \! 100,000$ core supercomputer to emulate a range of different GBS experiments with up to 100 modes and up to 92 photons. This reduces the run-time of classically simulating state-of-the-art GBS experiments to several months -- a nine orders of magnitude improvement over previous estimates. Finally, we introduce a distribution that is efficient to sample from classically and that passes a variety of GBS validation methods, providing an important adversary for future experiments to test against., Comment: 18 pages, 16 figures

Photons are natural carriers of high-dimensional quantum information, and, in principle, can benefit from higher quantum information capacity and noise-resilience. However, schemes to generate the resources required for high-dimensional quantum computing have so far been lacking in linear optics. Here, we show how to generate GHZ states in arbitrary dimensions and numbers of photons using linear optical circuits described by Fourier transform matrices. Combining our results with recent schemes for qudit Bell measurements, we show that universal linear optical quantum computing can be performed in arbitrary dimensions.

Integrated photonics is at the heart of many classical technologies, from optical communications to biosensors, LIDAR, and data center fiber interconnects. There is strong evidence that these integrated technologies will play a key role in quantum systems as they grow from few-qubit prototypes to tens of thousands of qubits. The underlying laser and optical quantum technologies, with the required functionality and performance, can only be realized through the integration of these components onto quantum photonic integrated circuits (QPICs) with accompanying electronics. In the last decade, remarkable advances in quantum photonic integration and a dramatic reduction in optical losses have enabled benchtop experiments to be scaled down to prototype chips with improvements in efficiency, robustness, and key performance metrics. The reduction in size, weight, power, and improvement in stability that will be enabled by QPICs will play a key role in increasing the degree of complexity and scale in quantum demonstrations. In the next decade, with sustained research, development, and investment in the quantum photonic ecosystem (i.e. PIC-based platforms, devices and circuits, fabrication and integration processes, packaging, and testing and benchmarking), we will witness the transition from single- and few-function prototypes to the large-scale integration of multi-functional and reconfigurable QPICs that will define how information is processed, stored, transmitted, and utilized for quantum computing, communications, metrology, and sensing. This roadmap highlights the current progress in the field of integrated quantum photonics, future challenges, and advances in science and technology needed to meet these challenges., Comment: Submitted to the Journal of Physics: Photonics

Linear-optical circuits are elementary building blocks for classical and quantum information processing with light. In particular, due to its monolithic structure, integrated photonics offers great phase-stability and can rely on the large scale manufacturability provided by the semiconductor industry. New devices, based on such optical circuits, hold the promise of faster and energy-efficient computations in machine learning applications and even implementing quantum algorithms intractable for classical computers. However, this technological revolution requires accurate and scalable certification protocols for devices that can be comprised of thousands of optical modes. Here, we present a novel technique to reconstruct the transfer matrix of linear optical networks that is based on the recent advances in low-rank matrix recovery and convex optimisation problems known as PhaseLift algorithms. Conveniently, our characterisation protocol can be performed with a coherent classical light source and photodiodes. We prove that this method is robust to noise and scales efficiently with the number of modes. We experimentally tested the proposed characterisation protocol on a programmable integrated interferometer designed for quantum information processing. We compared the transfer matrix reconstruction obtained with our method against the one provided by a more demanding reconstruction scheme based on two-photon quantum interference. For 5-dimensional random unitaries, the average circuit fidelity between the matrices obtained from the two reconstructions is 0.993., Comment: main document: 11 pages with 4 figures, appendix section: 15 pages

General purpose quantum computers can, in principle, entangle a number of noisy physical qubits to realise composite qubits protected against errors. Architectures for measurement-based quantum computing intrinsically support error-protected qubits and are the most viable approach for constructing an all-photonic quantum computer. Here we propose and demonstrate an integrated silicon photonic architecture that both entangles multiple photons, and encodes multiple physical qubits on individual photons, to produce error-protected qubits. We realise reconfigurable graph states to compare several schemes with and without error-correction encodings and implement a range of quantum information processing tasks. We observe a success rate increase from 62.5% to 95.8% when running a phase estimation algorithm without and with error protection, respectively. Finally, we realise hypergraph states, which are a generalised class of resource states that offer protection against correlated errors. Our results show how quantum error-correction encodings can be implemented with resource-efficient photonic architectures to improve the performance of quantum algorithms.

While integrated photonics is a robust platform for quantum information processing, architectures for photonic quantum computing place stringent demands on high quality information carriers. Sources of single photons that are highly indistinguishable and pure, that are either near-deterministic or heralded with high efficiency, and that are suitable for mass-manufacture, have been elusive. Here, we demonstrate on-chip photon sources that simultaneously meet each of these requirements. Our photon sources are fabricated in silicon using mature processes, and exploit a novel dual-mode pump-delayed excitation scheme to engineer the emission of spectrally pure photon pairs through intermodal spontaneous four-wave mixing in low-loss spiralled multi-mode waveguides. We simultaneously measure a spectral purity of $0.9904 \pm 0.0006$, a mutual indistinguishably of $0.987 \pm 0.002$, and $>90\%$ intrinsic heralding efficiency. We measure on-chip quantum interference with a visibility of $0.96 \pm 0.02$ between heralded photons from different sources. These results represent a decisive step for scaling quantum information processing in integrated photonics.

Generations of technologies with fundamentally new information processing capabilities will emerge if microscopic physical systems can be controlled to encode, transmit, and process quantum information, at scale and with high fidelity. In the decade after its 2008 inception, the technology of integrated quantum photonics enabled the generation, processing, and detection of quantum states of light, at a steadily increasing scale and level of complexity. Using both established and advanced fabrication techniques, the field progressed from the demonstrations of fixed circuits comprising few components and operating on two photons, to programmable circuitry approaching 1000 components with integrated generation of multi-photon states. A continuation in this trend over the next decade would usher in a versatile platform for future quantum technologies. This Review summarises the advances in integrated photonic quantum technologies (materials, devices, and functionality), and its demonstrated on-chip applications including secure quantum communications, simulations of quantum physical and chemical systems, Boson sampling, and linear-optic quantum information processing., Comment: 6 figures

An isolated system of interacting quantum particles is described by a Hamiltonian operator. Hamiltonian models underpin the study and analysis of physical and chemical processes throughout science and industry, so it is crucial they are faithful to the system they represent. However, formulating and testing Hamiltonian models of quantum systems from experimental data is difficult because it is impossible to directly observe which interactions the quantum system is subject to. Here, we propose and demonstrate an approach to retrieving a Hamiltonian model from experiments, using unsupervised machine learning. We test our methods experimentally on an electron spin in a nitrogen-vacancy interacting with its spin bath environment, and numerically, finding success rates up to 86%. By building agents capable of learning science, which recover meaningful representations, we can gain further insight on the physics of quantum systems., Comment: 27 pages, 8 figures

Implementing large instances of quantum algorithms requires the processing of many quantum information carriers in a hardware platform that supports the integration of different components. While established semiconductor fabrication processes can integrate many photonic components, the generation and algorithmic processing of many photons has been a bottleneck in integrated photonics. Here we report the on-chip generation and processing of quantum states of light with up to eight photons in quantum sampling algorithms. Switching between different optical pumping regimes, we implement the Scattershot, Gaussian and standard boson sampling protocols in the same silicon chip, which integrates linear and nonlinear photonic circuitry. We use these results to benchmark a quantum algorithm for calculating molecular vibronic spectra. Our techniques can be readily scaled for the on-chip implementation of specialised quantum algorithms with tens of photons, pointing the way to efficiency advantages over conventional computers.

Nitrogen-vacancy (NV) centres in diamond are appealing nano-scale quantum sensors for temperature, strain, electric fields and, most notably, for magnetic fields. However, the cryogenic temperatures required for low-noise single-shot readout that have enabled the most sensitive NV-magnetometry reported to date, are impractical for key applications, e.g. biological sensing. Overcoming the noisy readout at room-temperature has until now demanded repeated collection of fluorescent photons, which increases the time-cost of the procedure thus reducing its sensitivity. Here we show how machine learning can process the noisy readout of a single NV centre at room-temperature, requiring on average only one photon per algorithm step, to sense magnetic field strength with a precision comparable to those reported for cryogenic experiments. Analysing large data sets from NV centres in bulk diamond, we report absolute sensitivities of $60$ nT s$^{1/2}$ including initialisation, readout, and computational overheads. We show that dephasing times can be simultaneously estimated, and that time-dependent fields can be dynamically tracked at room temperature. Our results dramatically increase the practicality of early-term single spin sensors., Comment: including supplementary informations

The ability to control multidimensional quantum systems is key for the investigation of fundamental science and for the development of advanced quantum technologies. Here we demonstrate a multidimensional integrated quantum photonic platform able to robustly generate, control and analyze high-dimensional entanglement. We realize a programmable bipartite entangled system with dimension up to $15 \times 15$ on a large-scale silicon-photonics quantum circuit. The device integrates more than 550 photonic components on a single chip, including 16 identical photon-pair sources. We verify the high precision, generality and controllability of our multidimensional technology, and further exploit these abilities to demonstrate key quantum applications experimentally unexplored before, such as quantum randomness expansion and self-testing on multidimensional states. Our work provides a prominent experimental platform for the development of multidimensional quantum technologies., Comment: Science, (2018)

We experimentally demonstrate that tomographic measurements can be performed for states of qubits before they are prepared. A variant of the quantum teleportation protocol is used as a channel between two instants in time, allowing measurements for polarisation states of photons to be implemented 88 ns before they are created. Measurement data taken at the early time and later unscrambled according to the results of the protocol's Bell measurements, produces density matrices with an average fidelity of $0.90 \pm 0.01$ against the ideal states of photons created at the later time. Process tomography of the time-reverse quantum channel finds an average process fidelity of $0.84 \pm 0.02$. While our proof-of-principle implementation necessitates some post-selection, the general protocol is deterministic and requires no post-selection to sift desired states and reject a larger ensemble., Comment: Comments welcome

It is predicted that quantum computers will dramatically outperform their conventional counterparts. However, large-scale universal quantum computers are yet to be built. Boson sampling is a rudimentary quantum algorithm tailored to the platform of photons in linear optics, which has sparked interest as a rapid way to demonstrate this quantum supremacy. Photon statistics are governed by intractable matrix functions known as permanents, which suggests that sampling from the distribution obtained by injecting photons into a linear-optical network could be solved more quickly by a photonic experiment than by a classical computer. The contrast between the apparently awesome challenge faced by any classical sampling algorithm and the apparently near-term experimental resources required for a large boson sampling experiment has raised expectations that quantum supremacy by boson sampling is on the horizon. Here we present classical boson sampling algorithms and theoretical analyses of prospects for scaling boson sampling experiments, showing that near-term quantum supremacy via boson sampling is unlikely. While the largest boson sampling experiments reported so far are with 5 photons, our classical algorithm, based on Metropolised independence sampling (MIS), allowed the boson sampling problem to be solved for 30 photons with standard computing hardware. We argue that the impact of experimental photon losses means that demonstrating quantum supremacy by boson sampling would require a step change in technology., Comment: 25 pages, 9 figures. Comments welcome

Efficiently characterising quantum systems, verifying operations of quantum devices and validating underpinning physical models, are central challenges for the development of quantum technologies and for our continued understanding of foundational physics. Machine-learning enhanced by quantum simulators has been proposed as a route to improve the computational cost of performing these studies. Here we interface two different quantum systems through a classical channel - a silicon-photonics quantum simulator and an electron spin in a diamond nitrogen-vacancy centre - and use the former to learn the latter's Hamiltonian via Bayesian inference. We learn the salient Hamiltonian parameter with an uncertainty of approximately $10^{-5}$. Furthermore, an observed saturation in the learning algorithm suggests deficiencies in the underlying Hamiltonian model, which we exploit to further improve the model itself. We go on to implement an interactive version of the protocol and experimentally show its ability to characterise the operation of the quantum photonic device. This work demonstrates powerful new quantum-enhanced techniques for investigating foundational physical models and characterising quantum technologies.

Random unitary matrices find a number of applications in quantum information science, and are central to the recently defined boson sampling algorithm for photons in linear optics. We describe an operationally simple method to directly implement Haar random unitary matrices in optical circuits, with no requirement for prior or explicit matrix calculations. Our physically-motivated and compact representation directly maps independent probability density functions for parameters in Haar random unitary matrices, to optical circuit components. We go on to extend the results to the case of random unitaries for qubits.

Linear optics underpins tests of fundamental quantum mechanics and computer science, as well as quantum technologies. Here we experimentally demonstrate the longstanding goal of a single reprogrammable optical circuit that is sufficient to implement all possible linear optical protocols up to the size of that circuit. Our six-mode universal system consists of a cascade of 15 Mach-Zehnder interferometers with 30 thermo-optic phase shifters integrated into a single photonic chip that is electrically and optically interfaced for arbitrary setting of all phase shifters, input of up to six photons and their measurement with a 12 single-photon detector system. We programmed this system to implement heralded quantum logic and entangling gates, boson sampling with verification tests, and six-dimensional complex Hadamards. We implemented 100 Haar random unitaries with average fidelity 0.999 $\pm$ 0.001. Our system is capable of switching between these and any other linear optical protocol in seconds. These results point the way to applications across fundamental science and quantum technologies., Comment: Comments welcome

The foundational ideas of quantum mechanics continue to give rise to counterintuitive theories and physical effects that are in conflict with a classical description of Nature. Experiments with light at the single photon level have historically been at the forefront of tests of fundamental quantum theory and new developments in photonics engineering continue to enable new experiments. Here we review recent photonic experiments to test two foundational themes in quantum mechanics: wave-particle duality, central to recent complementarity and delayed-choice experiments; and Bell nonlocality where recent theoretical and technological advances have allowed all controversial loopholes to be separately addressed in different photonics experiments., Comment: 10 pages, 5 figures, published as a Nature Physics Insight review article

The first quantum technologies to solve computational problems that are beyond the capabilities of classical computers are likely to be devices that exploit characteristics inherent to a particular physical system, to tackle a bespoke problem suited to those characteristics. Evidence implies that the detection of ensembles of photons, which have propagated through a linear optical circuit, is equivalent to sampling from a probability distribution that is intractable to classical simulation. However, it is probable that the complexity of this type of sampling problem means that its solution is classically unverifiable within a feasible number of trials, and the task of establishing correct operation becomes one of gathering sufficiently convincing circumstantial evidence. Here, we develop scalable methods to experimentally establish correct operation for this class of sampling algorithm, which we implement with two different types of optical circuits for 3, 4, and 5 photons, on Hilbert spaces of up to 50,000 dimensions. With only a small number of trials, we establish a confidence >99% that we are not sampling from a uniform distribution or a classical distribution, and we demonstrate a unitary specific witness that functions robustly for small amounts of data. Like the algorithmic operations they endorse, our methods exploit the characteristics native to the quantum system in question. Here we observe and make an application of a "bosonic clouding" phenomenon, interesting in its own right, where photons are found in local groups of modes superposed across two locations. Our broad approach is likely to be practical for all architectures for quantum technologies where formal verification methods for quantum algorithms are either intractable or unknown., Comment: Comments welcome

Linear optical circuits of growing complexity are playing an increasing role in emerging photonic quantum technologies. Individual photonic devices are typically described by a unitary matrix containing amplitude and phase information, the characterisation of which is a key task. We present a constructive scheme to retrieve the unitary matrix describing an arbitrary linear optical device using data obtained from one-photon and two-photon ensembles. The scheme is stable on the arbitrarily increasable length scale of the photon packet and independent of photon loss at input and output ports of the device. We find a one-to-one correspondence between ideal data and unitary matrix, and identify the class of non-unitary matrices capable of reproducing the data. The method is extended for coherent state probes, which can simulate two-photon statistics with a reduced visibility. We analyse the performance of reconstruction to simulated noise., Comment: Comments welcome

Emerging models of quantum computation driven by multi-photon quantum interference, while not universal, may offer an exponential advantage over classical computers for certain problems. Implementing these circuits via geometric phase gates could mitigate requirements for error correction to achieve fault tolerance while retaining their relative physical simplicity. We report an experiment in which a geometric phase is embedded in an optical network with no closed-loops, enabling quantum interference between two photons as a function of the phase., Comment: Comments welcome

Quantum computational algorithms exploit quantum mechanics to solve problems exponentially faster than the best classical algorithms. Shor's quantum algorithm for fast number factoring is a key example and the prime motivator in the international effort to realise a quantum computer. However, due to the substantial resource requirement, to date, there have been only four small-scale demonstrations. Here we address this resource demand and demonstrate a scalable version of Shor's algorithm in which the n qubit control register is replaced by a single qubit that is recycled n times: the total number of qubits is one third of that required in the standard protocol. Encoding the work register in higher-dimensional states, we implement a two-photon compiled algorithm to factor N=21. The algorithmic output is distinguishable from noise, in contrast to previous demonstrations. These results point to larger-scale implementations of Shor's algorithm by harnessing scalable resource reductions applicable to all physical architectures., Comment: 7 pages, 3 figures

We report the first demonstration of quantum interference in multimode interference (MMI) devices and a new complete characterization technique that can be applied to any photonic device that removes the need for phase stable measurements. MMI devices provide a compact and robust realization of NxM optical circuits, which will dramatically reduce the complexity and increase the functionality of future generations of quantum photonic circuits.

We demonstrate photonic quantum circuits that operate at the stringent levels that will be required for future quantum information science and technology. These circuits are fabricated from silica-on-silicon waveguides forming directional couplers and interferometers. While our focus is on the operation of quantum circuits, to test this operation required construction of a spectrally tuned photon source to produce near-identical pairs of photons. We show non-classical interference with two photons and a two-photon entangling logic gate that operate with near-unit fidelity. These results are a significant step towards large-scale operation of photonic quantum circuits.

We show how an entangled cluster state encoded in the polarization of single photons can be straightforwardly expanded by deterministically entangling additional qubits encoded in the path degree of freedom of the constituent photons. This can be achieved using a polarization--path controlled-phase gate. We experimentally demonstrate a practical and stable realization of this approach by using a Sagnac interferometer to entangle a path qubit and polarization qubit on a single photon. We demonstrate precise control over phase of the path qubit to change the measurement basis and experimentally demonstrate properties of measurement-based quantum computing using a 2 photon, 3 qubit cluster state.

We describe a quantum key distribution protocol based on pairs of entangled qubits that generates a secure key between two partners in an environment of unknown and slowly varying reference frame. A direction of particle delivery is required, but the phases between the computational basis states need not be known or fixed. The protocol can simplify the operation of existing setups and has immediate applications to emerging scenarios such as earth-to-satellite links and the use of integrated photonic waveguides. We compute the asymptotic secret key rate for a two-qubit source, which coincides with the rate of the six-state protocol for white noise. We give the generalization of the protocol to higher-dimensional systems and detail a scheme for physical implementation in the three dimensional qutrit case., Comment: 4 pages, 2 figures, comments welcome

Discrimination between unknown processes chosen from a finite set is experimentally shown to be possible even in the case of non-orthogonal processes. We demonstrate unambiguous deterministic quantum process discrimination (QPD) of non-orthogonal processes using properties of entanglement, additional known unitaries, or higher dimensional systems. Single qubit measurement and unitary processes and multipartite unitaries (where the unitary acts non-separably across two distant locations) acting on photons are discriminated with a confidence of $\geq97%$ in all cases., Comment: 4 pages, 3 figures, comments welcome. Revised version includes multi-partite QPD