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We present a quantum network that distributes entangled photons between the University of Illinois Urbana-Champaign and a public library in Urbana. The network allows members of the public to perform measurements on the photons. We describe its design and implementation and outreach based on the network. Over 400 instances of public interaction have been logged with the system since it was launched in November 2023., Comment: 7 Pages, 8 Figures

We experimentally investigate the properties of hyperentangled states displaying simultaneous entanglement in multiple degrees of freedom, and find that Bell tests beyond the standard Clauser, Horne, Shimony, Holt inequality can reveal a higher-dimensional nature in a device-independent way. Specifically, we show that hyperentangled states possess more than just simultaneous entanglement in separate degrees of freedom but also entanglement in a higher dimensional Hilbert space. We also verify the steerability of hyperentangled quantum states by steering different photonic degrees of freedom., Comment: 11 pages, 4 figures, 1 table

We propose two optimal phase-estimation schemes that can be used for quantum-enhanced long-baseline interferometry. By using distributed entanglement, it is possible to eliminate the loss of stellar photons during transmission over the baselines. The first protocol is a sequence of gates using nonlinear optical elements, optimized over all possible measurement schemes to saturate the Cram\'er-Rao bound. The second approach builds on an existing protocol, which encodes the time of arrival of the stellar photon into a quantum memory. Our modified version reduces both the number of ancilla qubits and the number of gate operations by a factor of two., Comment: 14 pages, 9 figures

Deterministic sources of high-fidelity entangled qubit pairs encoded in the dual-rail photonic basis, i.e., presence of a single photon in one of two orthogonal modes, are a key enabling technology of many applications of quantum information processing, including high-rate high-fidelity quantum communications over long distances. The most popular and mature sources of such photonic entanglement, e.g., those that leverage spontaneous parametric down-conversion (SPDC) or spontaneous four-wave mixing (sFWM), generate an entangled (so-called, continuous-variable) quantum state that contains contributions from high-order photon terms that lie outside the span of the dual-rail basis, which is detrimental to most applications. One often uses low pump power to mitigate the effects of those high-order terms. However that reduces the pair generation rate, and the source becomes inherently probabilistic. We investigate a cascaded source that performs a linear-optical entanglement swap between two SPDC sources, to generate a heralded photonic entangled state that has a higher fidelity (to the ideal Bell state) compared to a free-running SPDC source. Further, with the Bell swap providing a heralding trigger, we show how to build a multiplexed source, which despite reasonable switching losses and detector loss and noise, yields a Fidelity versus Success Probability trade-off of a high-efficiency source of high-fidelity dual-rail photonic entanglement. We find however that there is a threshold of $1.5$ dB of loss per switch, beyond which multiplexing hurts the Fidelity versus Success Probability trade-off., Comment: 24 pages, 32 figures, 7 appendices. Comments and reviews are welcome!

In a quantum-noise limited system, weak-value amplification using post-selection normally does not produce more sensitive measurements than standard methods for ideal detectors: the increased weak value is compensated by the reduced power due to the small post-selection probability. Here we experimentally demonstrate recycled weak-value measurements using a pulsed light source and optical switch to enable nearly deterministic weak-value amplification of a mirror tilt. Using photon counting detectors, we demonstrate a signal improvement by a factor of $4.4 \pm 0.2$ and a signal-to-noise ratio improvement of $2.10 \pm 0.06$, compared to a single-pass weak-value experiment, and also compared to a conventional direct measurement of the tilt. The signal-to-noise ratio improvement could reach around 6 for the parameters of this experiment, assuming lower loss elements., Comment: 6 pages, 3 figures

Just as classical information technology rests on a foundation built of interconnected information-processing systems, quantum information technology (QIT) must do the same. A critical component of such systems is the interconnect, a device or process that allows transfer of information between disparate physical media, for example, semiconductor electronics, individual atoms, light pulses in optical fiber, or microwave fields. While interconnects have been well engineered for decades in the realm of classical information technology, quantum interconnects (QuICs) present special challenges, as they must allow the transfer of fragile quantum states between different physical parts or degrees of freedom of the system. The diversity of QIT platforms (superconducting, atomic, solid-state color center, optical, etc.) that will form a quantum internet poses additional challenges. As quantum systems scale to larger size, the quantum interconnect bottleneck is imminent, and is emerging as a grand challenge for QIT. For these reasons, it is the position of the community represented by participants of the NSF workshop on Quantum Interconnects that accelerating QuIC research is crucial for sustained development of a national quantum science and technology program. Given the diversity of QIT platforms, materials used, applications, and infrastructure required, a convergent research program including partnership between academia, industry and national laboratories is required. This document is a summary from a U.S. National Science Foundation supported workshop held on 31 October - 1 November 2019 in Alexandria, VA. Attendees were charged to identify the scientific and community needs, opportunities, and significant challenges for quantum interconnects over the next 2-5 years., Comment: This is an updated version V2, including expanded text and listing of all co-authors. To whom correspondence should be addressed: Marko Lon\v{c}ar: loncar@seas.harvard.edu; Michael G. Raymer: raymer@uoregon.edu

Fiber-based quantum communication networks are currently limited without quantum repeaters. Satellite-based quantum links have been proposed to extend the network domain. We have developed a quantum communication system, suitable for realistic satellite-to-ground communication. With this system, we have executed an entanglement-based quantum key distribution (QKD) protocol developed by Bennett, Brassard, and Mermin in 1992 (BBM92), achieving quantum bit error rates (QBER) below 2$\%$ in all bases. More importantly, we demonstrate low QBER execution of a higher dimensional hyperentanglement-based QKD protocol, using photons simultaneously entangled in polarization and time-bin, leading to significantly higher secure key rates, at the cost of increased technical complexity and system size. We show that our protocol is suitable for a space-to-ground link, after incorporating Doppler shift compensation, and verify its security using a rigorous finite-key analysis. Additionally, We discuss system engineering considerations relevant to those and other quantum communication protocols, and their dependence on what photonic degrees of freedom are utilized., Comment: 30 pages, 11 figures, and 4 tables

To build a global quantum communication network, low-transmission, fiber-based communication channels can be supplemented by using a free-space channel between a satellite and a ground station on Earth. We have constructed a system that generates hyperentangled photonic "ququarts" and measures them to execute multiple quantum communication protocols of interest. We have successfully executed and characterized superdense teleportation, a modified remote-state preparation protocol that transfers more quantum information than standard teleportation, for the same classical information cost, and moreover, is in principle deterministic. Our measurements show an average fidelity of $0.94\pm0.02$, with a phase resolution of $\sim7^{\circ}$, allowing reliable transmission of $>10^5$ distinguishable quantum states. Additionally, we have demonstrated the ability to compensate for the Doppler shift, which would otherwise prevent sending time-bin encoded states from a rapidly moving satellite, thus allowing the low-error execution of phase-sensitive protocols during an orbital pass. Finally, we show that the estimated number of received coincidence counts in a realistic implementation is sufficient to enable faithful reconstruction of the received state in a single pass., Comment: 34 pages, 14 figures, 3 tables

The human eye contains millions of rod photoreceptor cells, and each one is a single-photon detector. Whether people can actually see a single photon, which requires the rod signal to propagate through the rest of the noisy visual system and be perceived in the brain, has been the subject of research for nearly 100 years. Early experiments hinted that people could see just a few photons, but classical light sources are poor tools for answering these questions. Single-photon sources have opened up a new area of vision research, providing the best evidence yet that humans can indeed see single photons, and could even be used to test quantum effects through the visual system. We discuss our program to study the lower limits of human vision with a heralded single-photon source based on spontaneous parametric downconversion, and present two proposed experiments to explore quantum effects through the visual system: testing the perception of superposition states, and using a human observer as a detector in a Bell test., Comment: 7 pages, 6 figures

On-demand generation of indistinguishable single- and multi-photon states is a key technology for scaling up optical quantum information and communication applications. Nonlinear parametric photon-pair sources and heralded single-photon sources (HSPSs) had been the most standard resource of quantum information applications for decades. However, the intrinsic uncertainty of the produced number of photon pairs in such sources is a critical drawback that prevents on-demand photon-pair and heralded single-photon generation. Here we demonstrate large-scale time multiplexing of indistinguishable heralded single photons, employing a low-loss HSPS and adjustable delay line. We observed 66.7% presence probability of single-photon states collected into a single-mode optical fiber by multiplexing 40 periodic time bins of heralded single photons. To our knowledge, this is the highest fiber-coupled single-photon probability achieved to date. A high indistinguishability (~90%) of our time-multiplexed photons has also been confirmed. We also experimentally investigate trade-off relations of single-photon probability and unwanted multi-photon contribution by using different pump powers for a HSPS. Our results demonstrate that low-loss, large-scale multiplexing can realize highly efficient single-photon generation as well as highly scalable multi-photon generation from inefficient HSPSs. We predict that our large-scale time multiplexing will pave the way toward generation of > 30 coincident photons with unprecedented efficiencies, enabling a new frontier in optical quantum information processing.

The ability to determine the joint spectral properties of photon pairs produced by the processes of spontaneous parametric downconversion (SPDC) and spontaneous four wave mixing (SFWM) is crucial for guaranteeing the usability of heralded single photons and polarization-entangled pairs for multi-photon protocols. In this paper, we compare six different techniques that yield either a characterization of the joint spectral intensity or of the closely-related purity of heralded single photons. These six techniques include: i) scanning monochromator measurements, ii) a variant of Fourier transform spectroscopy designed to extract the desired information exploiting a resource-optimized technique, iii) dispersive fibre spectroscopy, iv) stimulated-emission-based measurement, v) measurement of the second-order correlation function $g^{(2)}$ for one of the two photons, and vi) two-source Hong-Ou-Mandel interferometry. We discuss the relative performance of these techniques for the specific cases of a SPDC source designed to be factorable and SFWM sources of varying purity, and compare the techniques' relative advantages and disadvantages.

The rod photoreceptors in the retina are known to be sensitive to single photons, but it has long been debated whether these single-photon signals propagate through the rest of the visual system and lead to perception. Recently, single-photon sources developed in the field of quantum optics have enabled direct tests of single-photon vision that were not possible with classical light sources. Using a heralded source based on spontaneous parametric downconversion to generate single photons which were sent to an observer at either an early or late time, Tinsley and Molodtsov et al. (2016) had observers judge when the photon was seen. Based on the above-chance accuracy in both a subset of high-confidence trials and in all post-selected trials, they claimed to show that humans can see single photons. However, we argue that this work suffers from three major issues: self-contradicting results, inappropriate statistical analyses, and a critical lack of statistical power. As a result, we cannot conclude that humans can see single photons based on the data of this study. We present a careful examination of the statistical analyses and the internal consistency of the data, which indicated that none of the key evidence holds., Comment: Referees noted that due to uncertainty in the parameters used to derive our estimate of the maximum accuracy, this analysis is not sufficient to challenge the basic conclusions of Tinsley et al. We agree with this criticism, and consider the Tinsley et al. study to be the best evidence for single-photon vision so far. The analysis techniques here may still be useful in designing future studies

Commercial photon-counting modules based on actively quenched solid-state avalanche photodiode sensors are used in a wide variety of applications. Manufacturers characterize their detectors by specifying a small set of parameters, such as detection efficiency, dead time, dark counts rate, afterpulsing probability and single-photon arrival-time resolution (jitter). However, they usually do not specify the range of conditions over which these parameters are constant or present a sufficient description of the characterization process. In this work, we perform a few novel tests on two commercial detectors and identify an additional set of imperfections that must be specified to sufficiently characterize their behavior. These include rate-dependence of the dead time and jitter, detection delay shift, and "twilighting." We find that these additional non-ideal behaviors can lead to unexpected effects or strong deterioration of the performance of a system using these devices. We explain their origin by an in-depth analysis of the active quenching process. To mitigate the effects of these imperfections, a custom-built detection system is designed using a novel active quenching circuit. Its performance is compared against two commercial detectors in a fast quantum key distribution system with hyper-entangled photons and a random number generator., Comment: 15 pages, 14 figures

In the last two decades, many quantum optics experiments have demonstrated small-scale quantum information processing applications with several photons. Beyond such proof-of-principle demonstrations, efficient preparation of large, but definite, numbers of photons is of great importance for further scaling up and speeding up photonic quantum information processing. Typical single-photon generation techniques based on nonlinear parametric processes face challenges of probabilistic generation. Here we demonstrate efficient synchronization of photons from multiple nonlinear parametric heralded single-photon sources (HSPSs), using quantum memories (QMs). Our low-loss optical memories greatly enhance (~30x) the generation rate of coincidence photons from two independent HSPSs, while maintaining high indistinguishability (95.7%) of the synchronized photons. As an application, we perform the first demonstration of HSPS-based measurement-device-independent quantum key distribution (MDI-QKD). The synchronized HSPSs demonstrated here will pave the way toward efficient quantum communication and larger scale optical quantum computing.

We propose and examine the use of biphoton pairs, such as those created in parametric down conversion or four-wave mixing, to enhance the precision and the resolution of measuring optical displacements by position-sensitive detection. We show that the precision of measuring a small optical beam displacement with this method can be significantly enhanced by the correlation between the two photons, given the same optical mode. The improvement is largest if the correlations between the photons are strong, and falls off as the biphoton correlation weakens. More surprisingly, we find that the smallest resolvable parameter of a simple split detector scales as the inverse of the number of biphotons for small biphoton number ("Heisenberg scaling"), because the Fisher information diverges as the parameter to be estimated decreases in value. One usually sees this scaling only for systems with many entangled degrees of freedom. We discuss the transition for the split-detection scheme to the standard quantum limit scaling for imperfect correlations as the biphoton number is increased. An analysis of an $N$-pixel detector is also given to investigate the benefit of using a higher resolution detector. The physical limit of these metrology schemes is determined by the uncertainty in the birth zone of the biphoton in the nonlinear crystal., Comment: 12 pages, 5 figures

We report on the generation of an indistinguishable heralded single-photon state, using highly nondegenerate spontaneous parametric downconversion (SPDC). Spectrally factorable photon pairs can be generated by incorporating a broadband pump pulse and a group-velocity matching (GVM) condition in a periodically-poled potassium titanyl phosphate (PPKTP) crystal. The heralding photon is in the near IR, close to the peak detection efficiency of off-the-shelf Si single-photon detectors; meanwhile, the heralded photon is in the telecom L-band where fiber losses are at a minimum. We observe spectral factorability of the SPDC source and consequently high purity (90%) of the produced heralded single photons by several different techniques. Because this source can also realize a high heralding efficiency (> 90%), it would be suitable for time-multiplexing techniques, enabling a pseudo-deterministic single-photon source, a critical resource for optical quantum information and communication technology.

We present a loophole-free violation of local realism using entangled photon pairs. We ensure that all relevant events in our Bell test are spacelike separated by placing the parties far enough apart and by using fast random number generators and high-speed polarization measurements. A high-quality polarization-entangled source of photons, combined with high-efficiency, low-noise, single-photon detectors, allows us to make measurements without requiring any fair-sampling assumptions. Using a hypothesis test, we compute p-values as small as $5.9\times 10^{-9}$ for our Bell violation while maintaining the spacelike separation of our events. We estimate the degree to which a local realistic system could predict our measurement choices. Accounting for this predictability, our smallest adjusted p-value is $2.3 \times 10^{-7}$. We therefore reject the hypothesis that local realism governs our experiment., Comment: Supplemental material available as an ancillary file

Photons have proven to be excellent carriers of quantum information, and play essential roles in numerous quantum information processing (QIP) applications. In particular, heralded single- photon sources via spontaneous parametric-down conversion (SPDC) have been a key technology for demonstrating small-scale QIP, yet their low generation efficiency is a critical limitation for further scaling up optical QIP technology. In order to efficiently overcome the probabilistic nature of SPDC, here we demonstrate time multiplexing for up to 30 time slots of a periodically pumped heralded single-photon source, using a switchable low-loss optical storage cavity. We observe a maximum single-photon probability of 38.6% in periodic output time windows, corresponding to 6 times enhancement over a non-multiplexed source, but with no increase in the contribution of unwanted multi-photon events. Combining this time-multiplexing technique with a heralded source producing pure single-photon states should enable larger scale optical QIP systems than ever realized.

Quantum nonlocality is arguably among the most counter-intuitive phenomena predicted by quantum theory. In recent years, the development of an abstract theory of nonlocality has brought a much deeper understanding of the subject. In parallel, experimental progress allowed for the demonstration of quantum nonlocality in a wide range of physical systems, and brings us close to a final loophole-free Bell test. Here we combine these theoretical and experimental developments in order to explore the limits of quantum nonlocality. This approach represents a thorough test of quantum theory, and could provide evidence of new physics beyond the quantum model. Using a versatile and high-fidelity source of pairs of polarization entangled photons, we explore the boundary of quantum correlations, present the most nonlocal correlations ever reported, demonstrate the phenomenon of more nonlocality with less entanglement, and show that non-planar (and hence complex) qubit measurements can be necessary to reproduce the strong qubit correlations that we observed. Our results are in remarkable agreement with quantum predictions., Comment: 6 pages, 5 pages of supplementary information, 5 figures. arXiv admin note: text overlap with arXiv:1405.4502

We use photon pairs hyperentangled in polarization and orbital angular momentum to implement a novel entanglement-enhanced quantum state communication technique, known as SuperDense Teleportation, to communicate a specific class of single-photon ququart states between two remote parties, with an average fidelity of 87.0(1)%, almost twice the classical limit of 44%. We compare this technique with quantum teleportation and remote state preparation and show that SuperDense teleportation requires less classical information and fewer experimental resources. We discuss the information content of this constrained set of states and demonstrate that this set has an exponentially larger state space volume than the lower dimensional general states with the same number of state parameters., Comment: 21 pages, 6 figures, 2 tables, and supplemental information

We analyze how the performance of a quantum-repeater network depends on the protocol employed to distribute entanglement, and we find that the choice of repeater-to-repeater link protocol has a profound impact on communication rate as a function of hardware parameters. We develop numerical simulations of quantum networks using different protocols, where the repeater hardware is modeled in terms of key performance parameters, such as photon generation rate and collection efficiency. These parameters are motivated by recent experimental demonstrations in quantum dots, trapped ions, and nitrogen-vacancy centers in diamond. We find that a quantum-dot repeater with the newest protocol ("MidpointSource") delivers the highest communication rate when there is low probability of establishing entanglement per transmission, and in some cases the rate is orders of magnitude higher than other schemes. Our simulation tools can be used to evaluate communication protocols as part of designing a large-scale quantum network., Comment: 16 pages, 11 figures

We improve the precision of the interferometric weak-value-based beam deflection measurement by introducing a power recycling mirror, creating a resonant cavity. This results in \emph{all} the light exiting to the detector with a large deflection, thus eliminating the inefficiency of the rare postselection. The signal-to-noise ratio of the deflection is itself magnified by the weak value. We discuss ways to realize this proposal, using a transverse beam filter and different cavity designs., Comment: 5 pages, 1 figure

We apply a distance-based Bell-test analysis method [E. Knill et al., Phys. Rev. A. 91, 032105 (2015)] to three experimental data sets where conventional analyses failed or required additional assumptions. The first is produced from a new classical source exploiting a "coincidence-time loophole" for which standard analysis falsely shows a Bell violation. The second is from a source previously shown to violate a Bell inequality; the distance-based analysis agrees with the previous results but with fewer assumptions. The third data set does not show a violation with standard analysis despite the high source quality, but is shown to have a strong violation with the distance-based analysis method., Comment: 7 pages with 6 pages of supplementary information

We present a source of entangled photons that violates a Bell inequality free of the "fair-sampling" assumption, by over 7 standard deviations. This violation is the first experiment with photons to close the detection loophole, and we demonstrate enough "efficiency" overhead to eventually perform a fully loophole-free test of local realism. The entanglement quality is verified by maximally violating additional Bell tests, testing the upper limit of quantum correlations. Finally, we use the source to generate secure private quantum random numbers at rates over 4 orders of magnitude beyond previous experiments., Comment: Main text: 5 pages, 2 figures, 1 table. Supplementary Information: 7 pages, 2 figures

Franson interferometers are increasingly being proposed as a means of securing high-dimensional energy-time entanglement-based quantum key distribution (QKD) systems. Heuristic arguments have been proposed that purport to demonstrate the security of these schemes. We show, however, that such systems are vulnerable to attacks that localize the photons to several temporally separate locations. This demonstrates that a single pair of Franson interferometers is not a practical approach to securing high-dimensional energy-time entanglement based QKD. This observations leads us to investigate the security of modified Franson-based-protocols, where Alice and Bob have two or more Franson interferometers. We show that such setups can improve the sensitivity against attacks that localize the photons to multiple temporal locations. While our results do not constituting a full security proof, they do show that a single pair of Franson interferometers is not secure and that multiple such interferometers could be a promising candidate for experimentally realizable high-dimensional QKD., Comment: 14 pages (single column format)

We consider the use of cyclic weak measurements to improve the sensitivity of weak-value amplification precision measurement schemes. Previous weak-value experiments have used only a small fraction of events, while discarding the rest through the process of "post-selection". We extend this idea by considering recycling of events which are typically unused in a weak measurement. Here we treat a sequence of polarized laser pulses effectively trapped inside an interferometer using a Pockels cell and polarization optics. In principle, all photons can be post-selected, which will improve the measurement sensitivity. We first provide a qualitative argument for the expected improvements from recycling photons, followed by the exact result for the recycling of collimated beam pulses, and numerical calculations for diverging beams. We show that beam degradation effects can be mitigated via profile flipping or Zeno reshaping. The main advantage of such a recycling scheme is an effective power increase, while maintaining an amplified deflection., Comment: 13 pages, 8 figures

We use hyperentangled photons to experimentally implement an entanglement-assisted quantum process tomography technique known as Direct Characterization of Quantum Dynamics. Specifically, hyperentanglement-assisted Bell-state analysis enabled us to characterize a variety of single-qubit quantum processes using far fewer experimental configurations than are required by Standard Quantum Process Tomography (SQPT). Furthermore, we demonstrate how known errors in Bell-state measurement may be compensated for in the data analysis. Using these techniques, we have obtained single-qubit process fidelities as high as 98.2% but with one-third the number experimental configurations required for SQPT. Extensions of these techniques to multi-qubit quantum processes are discussed., Comment: This is part of a joint submission with an implementation with Ions: "Experimental characterization of quantum dynamics through many-body interactions" by Daniel Nigg, Julio T. Barreiro, Philipp Schindler, Masoud Mohseni, Thomas Monz, Michael Chwalla, Markus Hennrich and Rainer Blatt

Quantum teleportation faces increasingly demanding requirements for transmitting large or even entangled systems. However, knowledge of the state to be transmitted eases its reconstruction, resulting in a protocol known as remote state preparation. A number of experimental demonstrations to date have been restricted to single-qubit systems. We report the remote preparation of two-qubit "hybrid" entangled states, including a family of vector-polarization beams. Our single-photon states are encoded in the photon spin and orbital angular momentum. We reconstruct the states by spin-orbit state tomography and transverse polarization tomography. The high fidelities achieved for the vector-polarization states opens the door to optimal coupling of down-converted photons to other physical systems, such as an atom, as required for scalable quantum networks, or plasmons in photonic nanostructures., Comment: Letter: 4 pages, 1 figure. Supplementary material: 1 page

Dense coding is arguably the protocol that launched the field of quantum communication. Today, however, more than a decade after its initial experimental realization, the channel capacity remains fundamentally limited as conceived for photons using linear elements. Bob can only send to Alice three of four potential messages owing to the impossibility of carrying out the deterministic discrimination of all four Bell states with linear optics, reducing the attainable channel capacity from 2 to log_2 3 \approx 1.585 bits. However, entanglement in an extra degree of freedom enables the complete and deterministic discrimination of all Bell states. Using pairs of photons simultaneously entangled in spin and orbital angular momentum, we demonstrate the quantum advantage of the ancillary entanglement. In particular, we describe a dense-coding experiment with the largest reported channel capacity and, to our knowledge, the first to break the conventional linear-optics threshold. Our encoding is suited for quantum communication without alignment and satellite communication., Comment: Letter: 6 pages, 4 figures. Supplementary Information: 4 pages, 1 figure

We discuss a novel method of efficiently producing multi-photon states using repeated spontaneous parametric downconversion. Specifically, by attempting downconversion several times, we can pseudo-deterministically add photons to a mode, producing various several-photon states. We discuss both expected performance and experimental limitations., Comment: 4 pages, 4 figures

Performance of quantum process estimation is naturally limited to fundamental, random, and systematic imperfections in preparations and measurements. These imperfections may lead to considerable errors in the process reconstruction due to the fact that standard data analysis techniques presume ideal devices. Here, by utilizing generic auxiliary quantum or classical correlations, we provide a framework for estimation of quantum dynamics via a single measurement apparatus. By construction, this approach can be applied to quantum tomography schemes with calibrated faulty state generators and analyzers. Specifically, we present a generalization of "Direct Characterization of Quantum Dynamics" [M. Mohseni and D. A. Lidar, Phys. Rev. Lett. 97, 170501 (2006)] with an imperfect Bell-state analyzer. We demonstrate that, for several physically relevant noisy preparations and measurements, only classical correlations and small data processing overhead are sufficient to accomplish the full system identification. Furthermore, we provide the optimal input states for which the error amplification due to inversion on the measurement data is minimal., Comment: 7 pages, 2 figures

It is known that it is impossible to unambiguously distinguish the four Bell states encoded in pairs of photon polarizations using only linear optics. However, hyperentanglement, the simultaneous entanglement in more than one degree of freedom, has been shown to assist the complete Bell analysis of the four Bell states (given a fixed state of the other degrees of freedom). Yet introducing other degrees of freedom also enlarges the total number of Bell-like states. We investigate the limits for unambiguously distinguishing these Bell-like states. In particular, when the additional degree of freedom is qubit-like, we find that the optimal one-shot discrimination schemes are to group the 16 states into 7 distinguishable classes, and that an unambiguous discrimination is possible with two identical copies., Comment: typos corrected, to appear in PRA, 5 pages, 2 figures, 2 tables

Vaidman, in a recent article adopts the method of 'quantum weak measurements in pre- and postselected ensembles' to ascertain whether or not the chained-Zeno counterfactual computation scheme proposed by Hosten et al. is counterfactual; which has been the topic of a debate on the definition of counterfactuality. We disagree with his conclusion, which brings up some interesting aspects of quantum weak measurements and some concerns about the way they are interpreted., Comment: 2 pages

We experimentally demonstrate the first quantum system entangled in every degree of freedom (hyperentangled). Using pairs of photons produced in spontaneous parametric downconversion, we verify entanglement by observing a Bell-type inequality violation in each degree of freedom: polarization, spatial mode and time-energy. We also produce and characterize maximally hyperentangled states and novel states simultaneously exhibiting both quantum and classical correlations. Finally, we report the tomography of a 2x2x3x3 system (36-dimensional Hilbert space), which we believe is the first reported photonic entangled system of this size to be so characterized., Comment: 5 pages, 3 figures, 1 table, published version

This is a collection of statements gathered on the occasion of the Quantum Physics of Nature meeting in Vienna., Comment: 3 pages, Quantum Physics of Nature (QUPON) Conference, Vienna, Austria, May 22nd-26th, 2005; v4: more contributions

We experimentally demonstrate the first remote state preparation of arbitrary single-qubit states, encoded in the polarization of photons generated by spontaneous parametric downconversion. Utilizing degenerate and nondegenerate wavelength entangled sources, we remotely prepare arbitrary states at two wavelengths. Further, we derive theoretical bounds on the states that may be remotely prepared for given two-qubit resources., Comment: ~4 pages, 2 figures, comment and references added

Two methods for creating arbitrary two-photon polarization pure states are introduced. Based on these, four schemes for creating two-photon polarization mixed states are proposed and analyzed. The first two schemes can synthesize completely arbitrary two-qubit mixed states, i.e., control all 15 free parameters: Scheme I requires several sets of crystals, while Scheme II requires only a single set, but relies on decohering the pump beam. Additionally, we describe two further schemes which are much easier to implement. Although the total capability of these is still being studied, we show that they can synthesize all two-qubit Werner states, maximally entangled mixed states, Collins-Gisin states, and arbitrary Bell-diagonal states., Comment: 11 pages, 6 figures, accepted by PRA

Geometric phase may enable inherently fault-tolerant quantum computation. However, due to potential decoherence effects, it is important to understand how such phases arise for {\it mixed} input states. We report the first experiment to measure mixed-state geometric phases in optics, using a Mach-Zehnder interferometer, and polarization mixed states that are produced in two different ways: decohering pure states with birefringent elements; and producing a nonmaximally entangled state of two photons and tracing over one of them, a form of remote state preparation., Comment: To appear in Phys. Rev. Lett. 4 pages, 3 figures

We investigate an imbalance between the sensitivity of the common state measures--fidelity, trace distance, concurrence, tangle, von Neumann entropy and linear entropy--when acted on by a depolarizing channel. Further, in this context we explore two classes of two-qubit entangled mixed states. Specifically, we illustrate a sensitivity imbalance between three of these measures for depolarized (i.e., Werner-state like) nonmaximally entangled and maximally entangled mixed states, noting that the size of the imbalance depends on the state's tangle and linear entropy., Comment: 6 pages, 3 figures; corrected typos and expression (17)

Using correlated photons from parametric downconversion, we extend the boundaries of experimentally accessible two-qubit Hilbert space. Specifically, we have created and characterized maximally entangled mixed states (MEMS) that lie above the Werner boundary in the linear entropy-tangle plane. In addition, we demonstrate that such states can be efficiently concentrated, simultaneously increasing both the purity and the degree of entanglement. We investigate a previously unsuspected sensitivity imbalance in common state measures, i.e., the tangle, linear entropy, and fidelity., Comment: 4 pages, 3 figures, 1 table; accepted version

Complete and precise characterization of a quantum dynamical process can be achieved via the method of quantum process tomography. Using a source of correlated photons, we have implemented several methods investigating a wide range of processes, e.g., unitary, decohering, and polarizing. One of these methods, ancilla-assisted process tomography (AAPT), makes use of an additional ``ancilla system,'' and we have theoretically determined the conditions when AAPT is possible. All prior schemes for AAPT make use of entangled states. Our results show that, surprisingly, entanglement is not required for AAPT, and we present process tomography data obtained using an input state that has no entanglement. However, the use of entanglement yields superior results., Comment: To appear in Physical Review Letters

Maximally entangled mixed states are those states that, for a given mixedness, achieve the greatest possible entanglement. For two-qubit systems and for various combinations of entanglement and mixedness measures, the form of the corresponding maximally entangled mixed states is determined primarily analytically. As measures of entanglement, we consider entanglement of formation, relative entropy of entanglement, and negativity; as measures of mixedness, we consider linear and von Neumann entropies. We show that the forms of the maximally entangled mixed states can vary with the combination of (entanglement and mixedness) measures chosen. Moreover, for certain combinations, the forms of the maximally entangled mixed states can change discontinuously at a specific value of the entropy., Comment: 13 pages, 12 figures

Heisenberg in 1929 introduced the "collapse of the wavepacket" into quantum theory. We review here an experiment at Berkeley which demonstrated several aspects of this idea. In this experiment, a pair of daughter photons was produced in an entangled state, in which the sum of their two energies was equal to the sharp energy of their parent photon, in the nonlinear optical process of spontaneous parametric down-conversion. The wavepacket of one daughter photon collapsed upon a measurement-at-a-distance of the other daughter's energy, in such a way that the total energy of the two-photon system was conserved. Heisenberg's energy-time uncertainty principle was also demonstrated to hold in this experiment., Comment: 13 pages, 3 figures. Chiao's Heisenberg Centennial Symposium lecture given in Bamberg, Germany, in Sept. 2001

We report the creation of a wide range of quantum states with controllable degrees of entanglement and entropy using an optical two-qubit source based on spontaneous parametric downconversion. The states are characterised using measures of entanglement and entropy determined from tomographically determined density matrices. The Tangle-Entropy plane is introduced as a graphical representation of these states, and the theoretic upper bound for the maximum amount of entanglement possible for a given entropy is presented. Such a combination of general quantum state creation and accurate characterisation is an essential prerequisite for quantum device development., Comment: 4 pages, 3 figures. Submitted to Physical Review A

Two-qubit states occupy a large and relatively unexplored Hilbert space. Such states can be succinctly characterized by their degree of entanglement and purity. In this letter we investigate entangled mixed states and present a class of states that have the maximum amount of entanglement for a given linear entropy., Comment: 4 pages, 3 figures

We describe in detail the theory underpinning the measurement of density matrices of a pair of quantum two-level systems (``qubits''). Our particular emphasis is on qubits realized by the two polarization degrees of freedom of a pair of entangled photons generated in a down-conversion experiment; however the discussion applies in general, regardless of the actual physical realization. Two techniques are discussed, namely a tomographic reconstruction (in which the density matrix is linearly related to a set of measured quantities) and a maximum likelihood technique which requires numerical optimization (but has the advantage of producing density matrices which are always non-negative definite). In addition a detailed error analysis is presented, allowing errors in quantities derived from the density matrix, such as the entropy or entanglement of formation, to be estimated. Examples based on down-conversion experiments are used to illustrate our results., Comment: 23 pages, 3 figures, submitted to Phys Rev A

We report an experimental confirmation of the power-law relationship between the critical anisotropy parameter and ion number for the linear-to-zigzag phase transition in an ionic crystal. Our experiment uses laser cooled calcium ions confined in a linear radio-frequency trap. Measurements for up to 10 ions are in good agreement with theoretical and numeric predictions. Implications on an upper limit to the size of data registers in ion trap quantum computers are discussed., Comment: Physical Review Letters in press, 4 pages, 4 figures

Using polarization-entangled photons from spontaneous parametric downconversion, we have implemented Ekert's quantum cryptography protocol. The near-perfect correlations of the photons allow the sharing of a secret key between two parties. The presence of an eavesdropper is continually checked by measuring Bell's inequalities. We investigated several possible eavesdropper strategies, including pseudo-quantum non-demolition measurements. In all cases, the eavesdropper's presence was readily apparent. We discuss a procedure to increase her detectability., Comment: 4 pages, 2 encapsulated postscript files, PRL (tentatively) accepted

The phenomenon of quantum interrogation allows one to optically detect the presence of an absorbing object, without the measuring light interacting with it. In an application of the quantum Zeno effect, the object inhibits the otherwise coherent evolution of the light, such that the probability that an interrogating photon is absorbed can in principle be arbitrarily small. We have implemented this technique, demonstrating efficiencies exceeding the 50% theoretical-maximum of the original ``interaction-free'' measurement proposal. We have also predicted and experimentally verified a previously unsuspected dependence on loss; efficiencies of up to 73% were observed and the feasibility of efficiencies up to 85% was demonstrated., Comment: 4 pages, 3 postscript figures. To appear in Phys. Rev. Lett; submitted June 11, 1999

Using a spontaneous-downconversion photon source, we produce true non-maximally entangled states, i.e., without the need for post-selection. The degree and phase of entanglement are readily tunable, and are characterized both by a standard analysis using coincidence minima, and by quantum state tomography of the two-photon state. Using the latter, we experimentally reconstruct the reduced density matrix for the polarization. Finally, we use these states to measure the Hardy fraction, obtaining a result that is $122 \sigma$ from any local-realistic result., Comment: 4 pages, 4 figures. To appear in Phys. Rev. Lett