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Large-eddy simulation (LES) is an optimal tool to examine aerosol particle concentrations in detail within urban neighbourhoods. The concentrations are a complex result of local emissions, meteorology, aerosol processes and local mixing conditions due to thermal and mechanical effects. Despite this, most studies have focused on simplification of the affecting processes such as examining the impact of local mixing in idealised street canyons or treating aerosols as passive scalars. The aim of this study is to include all these processes into LES using the PALM model system and to examine the importance of radiative heating and aerosol processes in simulating local aerosol particle concentrations and different aerosol metrics within a realistic urban neighbourhood in Helsinki under morning rush hour with calm wind conditions. The model outputs are evaluated against mobile laboratory measurements of air temperature and total particle number concentration (Ntot) as well as drone measurements of lung-deposited surface area (LDSA). The inclusion of radiation interaction in LES has a significant impact on simulated near-surface temperatures in our study domain, increasing them on average from 8.6 to 12.4 ∘ C. The resulting enhanced ventilation reduces the pedestrian-level (4 m) Ntot by 53 %. The reduction in Ntot due to aerosol processes is smaller, only 18 %. Aerosol processes particularly impact the smallest particle range, whereas radiation interaction is more important in the larger particle range. The inclusion of radiation interaction reduces the bias between the modelled and mobile-laboratory-measured air temperatures from - 3.9 to + 0.2 ∘ C and Ntot from + 98 % to - 13 %. With both aerosol and radiation interaction on, the underestimation is 16 %, which might be due to overestimation of the ventilation. The results show how inclusion of radiative interaction is particularly important in simulating PM 2.5 , whereas aerosol processes are more important in simulating LDSA in this calm wind situation. [ABSTRACT FROM AUTHOR]

Numerical models are needed for evaluating aerosol processes in the atmosphere in state-of-the-art chemical transport models, urban-scale dispersion models and climatic models. This article describes a publicly available aerosol dynamics model MAFOR (Multicomponent Aerosol FORmation model; version 2.0); we address the main structure of the model, including the types of operation and the treatments of the aerosol processes. The main advantage of MAFOR v2.0 is the consistent treatment of both the mass- and number-based concentrations of particulate matter. An evaluation of the model is also presented, against a high-resolution observational dataset in a street canyon located in the centre of Helsinki (Finland) during an afternoon traffic rush hour on 13 December 2010. The experimental data included measurements at different locations in the street canyon of ultrafine particles, black carbon, and fine particulate mass PM1. This evaluation has also included an intercomparison with the corresponding predictions of two other prominent aerosol dynamics models, AEROFOR and SALSA. All three models fairly well simulated the decrease of the measured total particle number concentrations with increasing distance from the vehicular emission source. The MAFOR model reproduced the evolution of the observed particle number size distributions more accurately than the other two models. The MAFOR model also predicted the variation of the concentration of PM1 better than the SALSA model. We also analysed the relative importance of various aerosol processes based on the predictions of the three models. As expected, atmospheric dilution dominated over other processes; dry deposition was the second most significant process. Numerical sensitivity tests with the MAFOR model revealed that the uncertainties associated with the properties of the condensing organic vapours affected only the size range of particles smaller than 10 nm in diameter. These uncertainties do not therefore affect significantly the predictions of the whole of the number size distribution and the total number concentration. The MAFOR model version 2 is well documented and versatile to use, providing a range of alternative parametrizations for various aerosol processes. The model includes an efficient numerical integration of particle number and mass concentrations, an operator-splitting of processes, and the use of a fixed sectional method. The model could be used as a module in various atmospheric and climatic models. [ABSTRACT FROM AUTHOR]

The planetary boundary layer (BL) height and stratification are key parameters in determining the exchange of heat, momentum, moisture and trace gases between the surface and the free troposphere. Numerous different methods have been used to quantify the BL height and these methods have been applied to a wide variety of observational data sets obtained from different instruments and to numerical model output. We investigate the BL height at the Hyytiälä SMEAR II station in southern Finland diagnosed from radiosonde observations, a microwave radiometer (MWR) and ERA5 reanalysis. Four different algorithms are used to diagnose the BL height from the radiosondes. The diagnosed BL height is sensitive to the method used and the level of agreement, and the sign of systematic bias, between the 4 different methods depends on the surface-layer stability. For example, for very unstable situations, the median BL height diagnosed from the radiosondes varies from 600 m to 1500 m depending on which method is applied. Good agreement between the BL height in ERA5 and diagnosed from the radiosondes using Richardson number-based methods is found for almost all stability classes, suggesting that ERA5 has adequate vertical resolution near the surface to resolve the BL structure. However, ERA5 overestimates the BL height in very stable conditions highlighting the on-going challenge for numerical models to correctly resolve the stable BL. Furthermore, ERA5 BL height differs most from the radiosondes at 18 UTC suggesting ERA5 does not resolve the evening transition correctly. This study has also shown that BL height estimates from the MWR are reliable in unstable situations but often are inaccurate under stable conditions when, in comparison to ERA5 BL heights, they are much deeper. The errors in the MWR BL height estimates originate from the limitations of the manufacturers algorithm for stable conditions and also the mis-identification of the type of BL. A climatology of the annual and diurnal cycle of BL height and observed surface layer stability was created. The shallowest (353 m) monthly median BL height occurs in February and the deepest (576 m) in June. In winter there is no diurnal cycle in BL height, unstable BLs are rare yet so are very stable BLs. The shallowest BLs occur at night in spring and summer and very stable conditions are most common at night in the warm season. Finally, using ERA5 gridded data we determined that the BL height observed at Hyytiälä is representative of most land areas in southern and central Finland. However, the spatial variability of the BL height is largest during daytime in summer reducing the area over which BL height observations from Hyytiälä would be representative of. [ABSTRACT FROM AUTHOR]

The dispersion of cooking-generated aerosols from an urban street canyon is examined with building-resolving computational fluid dynamics (CFD). Using a comprehensive urban CFD model (PALM) with a sectional aerosol module (SALSA), emissions from deep frying and boiling are considered for near-ground and elevated sources. It is found that, with representative choices of the source flux, the inclusion of aerosol dynamic processes decreases the mean canyon-averaged number concentration by 15-40 % for cooking emissions, whereas the effect is significantly weaker for traffic-generated aerosols. The effects of deposition and coagulation are comparable for boiling, but coagulation dominates for deep frying. Deposition is maximised inside the leeward corner vortices, while coagulation increases away from the source. The characteristic timescales are invoked to explain the spatial structure of deposition and coagulation. In particular, the relative difference between number concentrations for simulations with and without coagulation are strongly correlated with the ageing of particles along fluid trajectories or the mean tracer age. [ABSTRACT FROM AUTHOR]