1. Metallic Spin Liquid-like Behavior of LiV$_2$O$_4$
- Author
-
Okabe, H., Hiraishi, M., Koda, A., Kojima, K. M., Takeshita, S., Yamauchi, I., Matsushita, Y., Kuramoto, Y., and Kadono, R.
- Subjects
Condensed Matter - Strongly Correlated Electrons - Abstract
LiV$_2$O$_4$ spinel is known to exhibit heavy fermion-like behavior below a characteristic temperature $T_K\simeq 20$ K, while it preserves a paramagnetic state down to $T\sim10^{-2}$ K due to geometrical frustration. Here, it is shown that the dynamical spin susceptibility $\chi({\bf q},\omega)$ in LiV$_2$O$_4$ exhibits anomalous duality which is modeled as a sum of itinerant ($\chi_{\rm F}$) and local ($\chi_{\rm L}$) components,and that the local spin dynamics inferred from $\chi_{\rm L}({\bf q},\omega)$ is qualitatively different from that expected from time-averaged bulk properties. The anomaly coexists with the marginal Fermi liquid behavior inferred from the $-\ln T$ dependence of the electronic specific heat over a wide temperature range below $T_K$. We argue that such unusual properties of LiV$_2$O$_4$ can be attributed to the putative metallic spin liquid state emerging near the quantum critical point between spin glass and Fermi liquid states., Comment: 5 pages, 3 figures, Supplemental Material
- Published
- 2018
- Full Text
- View/download PDF