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The quasiprobability distribution of the discrete Wigner function provides a complete description of a quantum state and is, therefore, a useful alternative to the usual density matrix description. Moreover, the experimental quantum state tomography in discrete Wigner phase space can also be implemented. We observe that for a certain class of states, such as harmonic states, the Wigner matrix is far more sparse compared to the density matrix in the computational basis. Additionally, reading only a small part of the Wigner matrix may suffice to infer certain behavior of quantum dynamics. In such cases, selective Wigner phase space tomography (SWPST) can be more efficient than the usual density matrix tomography (DMT). Employing nuclear magnetic resonance methods on a three-qubit nuclear spin register, we experimentally estimate Wigner matrices of various two-qubit quantum states. As a specific example application of SWPST, we study the evolution of spin coherent states under the quantum chaotic kicked top model and extract signatures of quantum-classical correspondence in the Wigner phase space.

In the usual quantum tunneling, a low-energy quantum particle penetrates across a physical barrier of higher potential energy, by traversing a classically forbidden region, and finally escapes into another region. In an analogous scenario, a classical particle inside a closed regular region in the phase space is dynamically bound from escaping to other regions of the phase space. Here, the physical potential barrier is replaced by dynamical barriers which separate different regions of the phase space. However, in the quantum regime, the system can overcome such dynamical barriers and escape through them, giving rise to dynamical tunneling. In chaotic Hamiltonian systems, dynamical tunneling refers to quantum tunneling between states whose classical limit correspond to symmetry-related regular regions separated by a chaotic zone between which any classical transport is prohibited. Here, an experimental realization of dynamical tunneling in spin systems is reported using nuclear magnetic resonance (NMR) architecture. In particular, dynamical tunneling in quantum kicked tops of spin-1 and spin-3/2 systems using two- and three-qubit NMR registers is investigated. By extracting time-dependent expectation values of the angular momentum operator components, size-dependent tunneling behaviour for various initial states is systematically investigated. Further, by monitoring the adverse effects of dephasing noise on the tunneling oscillations, we assert the importance of quantum coherence in enabling dynamical tunneling.

We report an experimental study of phase-synchronization in a pair of interacting nuclear spins subjected to an external drive in nuclear magnetic resonance architecture. A weak transition-selective radio-frequency field applied on one of the spins is observed to cause phase-localization, which is experimentally established by measuring the Husimi distribution function under various drive conditions. To this end, we have developed a general interferometric technique to directly extract values of the Husimi function via the transverse magnetization of the undriven nuclear spin. We further verify the robustness of synchronization to detuning in the system by studying the Arnold tongue behaviour.

The development of efficient algorithms that generate robust quantum controls is crucial for the realization of quantum technologies. The commonly used gradient-based optimization algorithms are limited by their sensitivity to the initial guess, which affects their performance. Here we propose combining the gradient method with the simulated annealing technique to formulate a hybrid algorithm. Our numerical analysis confirms its superior convergence rate. Using the hybrid algorithm, we generate spin-selective $\pi$ pulses and employ them for experimental measurement of local noise-spectra in a three-qubit NMR system. Moreover, here we describe a general method to construct noise-resilient quantum controls by incorporating noisy fields within the optimization routine of the hybrid algorithm. On experimental comparison with similar sequences obtained from standard algorithms, we find remarkable robustness of the hybrid sequences against dephasing errors., Comment: 8 pages, 7 figures

In recent years, the performance of different entanglement indicators obtained directly from tomograms has been assessed in continuous-variable and hybrid quantum systems. In this paper, we carry out this task in the case of spin systems. We compute the entanglement indicators from actual experimental data obtained from three liquid-state NMR experiments, and compare them with standard entanglement measures calculated from the corresponding density matrices, both experimentally reconstructed and numerically computed. The gross features of entanglement dynamics and spin squeezing properties are found to be reproduced by these entanglement indicators. However, the extent to which these indicators and spin squeezing track the entanglement during time evolution of the multipartite systems in the NMR experiments is very sensitive to the precise nature and strength of interactions as well as the manner in which the full system is partitioned into subsystems. We also use the IBM quantum computer to implement equivalent circuits that capture the dynamics of the multipartite system in one of the NMR experiments. We compute and compare the entanglement indicators obtained from the tomograms corresponding to the experimental execution and simulation of these equivalent circuits. This exercise shows that these indicators can estimate the degree of entanglement without necessitating detailed state reconstruction procedures, establishing the advantage of the tomographic approach., Comment: 26 pages, 17 figures

We experimentally emulate interaction induced blockade and local spin freezing in two and three qubit Nuclear Magnetic Resonance (NMR) architecture. These phenomena are identical to the Rydberg blockade and Rydberg biased freezing. In Rydberg blockade, the simultaneous excitation of two or more atoms is blocked due to the level shift induced by the strong Van der Waal's interaction. In such a strong interaction regime, one can also observe Rydberg biased freezing, wherein the dynamics is confined to a subspace, with the help of multiple drives with unequal amplitudes. Here we drive NMR qubits with specific transition-selective radio waves, while intermittently characterizing the quantum states via quantum state tomography. This not only allows us to track the population dynamics, but also helps to probe quantum correlations, by means of quantum discord, evolving under blockade and freezing phenomena. While, our work constitutes the first experimental simulations of these phenomena in the NMR platform, it is also the first experimental demonstration of Rydberg biased freezing. Moreover, these studies open up interesting quantum control perspectives in exploiting the above phenomena for entanglement generation as well as subspace manipulations., Comment: 9 pages, 6 figures

Quantum optimal control involves setting up an objective function that evaluates the quality of an operator representing the realized process w.r.t. the target process. Here we propose a stronger objective function which incorporates not only the target operator but also a set of its orthogonal operators. We find significantly superior convergence of optimization routines with the combined influences of all the operators. We refer to this method as the $\textit{push-pull}$ optimization. In particular, we describe adopting the push-pull optimization to a gradient based approach and a variational-principle based approach. We carry out extensive numerical simulations of the push-pull optimization of quantum controls on a pair of Ising coupled qubits. Finally, we demonstrate its experimental application by preparing a long-lived singlet-order in a two-qubit system using NMR techniques.

We investigate the scrambling of information in a hierarchical star-topology system using out-of-time-ordered correlation (OTOC) functions. The system consists of a central qubit directly interacting with a set of satellite qubits, which in turn interact with a second layer of satellite qubits. This particular topology not only allows convenient preparation and filtering of multiple quantum coherences between the central qubit and the first layer but also to engineer scrambling in a controlled manner. Hence, it provides us with an opportunity to experimentally study scrambling of information localized in multi-spin correlations via the construction of relevant OTOCs. Since the measurement of OTOC requires a time evolution, the non-scrambling processes such as decoherence and certain experimental errors create an ambiguity. Therefore, the unambiguous quantification of information scrambling requires suppressing contributions from decoherence to the OTOC dynamics. To this end, we propose and experimentally demonstrate a constant time protocol which is able to filter contribution exclusively from information scrambling., Comment: 10 pages, 7 figures, comments are welcome

Quantum chaotic kicked top model is implemented experimentally in a two qubit system comprising of a pair of spin-1/2 nuclei using Nuclear Magnetic Resonance techniques. The essential nonlinear interaction was realized using indirect spin-spin coupling, while the linear kicks were realized using RF pulses. After a variable number of kicks, quantum state tomography was employed to reconstruct the single-qubit density matrices using which we could extract various measures such as von Neumann entropies, Husimi distributions, and Lyapunov exponents. These measures enabled the study of correspondence with classical phase space as well as to probe distinct features of quantum chaos, such as symmetries and temporal periodicity in the two-qubit kicked top., Comment: 8 pages, 8 figures