1. Strain control of a bandwidth-driven spin reorientation in Ca$_{3}$Ru$_{2}$O$_{7}$
- Author
-
Dashwood, C. D., Walker, A. H., Kwasigroch, M. P., Veiga, L. S. I., Faure, Q., Vale, J. G., Porter, D. G., Manuel, P., Khalyavin, D. D., Orlandi, F., Colin, C. V., Fabelo, O., Krüger, F., Perry, R. S., Johnson, R. D., Green, A. G., and McMorrow, D. F.
- Subjects
Condensed Matter - Strongly Correlated Electrons - Abstract
The layered-ruthenate family of materials possess an intricate interplay of structural, electronic and magnetic degrees of freedom that yields a plethora of delicately balanced ground states. This is exemplified by Ca$_{3}$Ru$_{2}$O$_{7}$, which hosts a coupled transition in which the lattice parameters jump, the Fermi surface partially gaps and the spins undergo a $90^{\circ}$ in-plane reorientation. Here, we show how the transition is driven by a lattice strain that tunes the electronic bandwidth. We apply uniaxial stress to single crystals of Ca$_{3}$Ru$_{2}$O$_{7}$, using neutron and resonant x-ray scattering to simultaneously probe the structural and magnetic responses. These measurements demonstrate that the transition can be driven by externally induced strain, stimulating the development of a theoretical model in which an internal strain is generated self-consistently to lower the electronic energy. We understand the strain to act by modifying tilts and rotations of the RuO$_{6}$ octahedra, which directly influences the nearest-neighbour hopping. Our results offer a blueprint for uncovering the driving force behind coupled phase transitions, as well as a route to controlling them., Comment: 12 pages, 6 figures (+ 12 pages, 6 figures of supplemental material)
- Published
- 2022
- Full Text
- View/download PDF