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Real-time probing of electrons can uncover intricate relaxation mechanisms and many-body interactions hidden in strongly correlated materials. While experimenters have used ultrafast optical pump-probe methods in bulk materials, laser heating and insensitivity below the surface prevent their application to encapsulated low-dimensional electron systems at millikelvin temperatures, home to numerous intriguing electronic phases. Here, we introduce time, momentum, and energy resolved pump-probe tunneling spectroscopy (Tr-MERTS). The method allows the injection of electrons at particular energies and observation of their subsequent decay in energy-momentum space. Using Tr-MERTS, we visualize electronic decay processes in Landau levels with lifetimes up to tens of microseconds. Although most observed features agree with simple energy-relaxation, we discover an unexpected splitting in the nonequilibrium energy spectrum in the vicinity of a ferromagnetic state. An exact diagonalization study of the system suggests that the splitting arises from a maximally spin-polarized higher energy state, distinct from a conventional equilibrium skyrmion. Furthermore, we observe time-dependent relaxation of the splitting, which we attribute to single-flipped spins forming topological spin textures. These results establish Tr-MERTS as a powerful tool for studying the dynamics and properties of a two-dimensional electronic system beyond equilibrium.

The interplay of strong Coulomb interactions and of topology is currently under intense scrutiny in various condensed matter and atomic systems. One example of this interplay is the phase competition of fractional quantum Hall states and the Wigner solid in the two-dimensional electron gas. Here we report a Wigner solid at ν = 1.79 and its melting due to fractional correlations occurring at ν = 9/5. This Wigner solid, that we call the reentrant integer quantum Hall Wigner solid, develops in a range of Landau level filling factors that is related by particle-hole symmetry to the so called reentrant Wigner solid. We thus find that the Wigner solid in the GaAs/AlGaAs system straddles the partial filling factor 1/5 not only at the lowest filling factors, but also near ν = 9/5. Our results highlight the particle-hole symmetry as a fundamental symmetry of the extended family of Wigner solids and paint a complex picture of the competition of the Wigner solid with fractional quantum Hall states.

Strongly correlated quantum particles in lattice potentials are the building blocks for a wide variety of quantum insulators-for instance, Mott phases and density waves breaking lattice symmetry

What are the ground states of an interacting, low-density electron system? In the absence of disorder, it has long been expected that as the electron density is lowered, the exchange energy gained by aligning the electron spins should exceed the enhancement in the kinetic (Fermi) energy, leading to a (Bloch) ferromagnetic transition. At even lower densities, another transition to a (Wigner) solid, an ordered array of electrons, should occur. Experimental access to these regimes, however, has been limited because of the absence of a material platform that supports an electron system with very high quality (low disorder) and low density simultaneously. Here we explore the ground states of interacting electrons in an exceptionally clean, two-dimensional electron system confined to a modulation-doped AlAs quantum well. The large electron effective mass in this system allows us to reach very large values of the interaction parameter [Formula: see text] , defined as the ratio of the Coulomb to Fermi energies. As we lower the electron density via gate bias, we find a sequence of phases, qualitatively consistent with the above scenario: a paramagnetic phase at large densities, a spontaneous transition to a ferromagnetic state when [Formula: see text] surpasses 35, and then a phase with strongly nonlinear current-voltage characteristics, suggestive of a pinned Wigner solid, when [Formula: see text] exceeds [Formula: see text]. However, our sample makes a transition to an insulating state at [Formula: see text] , preceding the onset of the spontaneous ferromagnetism, implying that besides interaction, the role of disorder must also be taken into account in understanding the different phases of a realistic dilute electron system.

In 1929, Felix Bloch suggested that the paramagnetic Fermi sea of electrons should make a spontaneous transition to a fully magnetized state at very low densities, because the exchange energy gained by aligning the spins exceeds the enhancement in the kinetic energy1. However, experimental realizations of this effect have been hard to implement. Here, we report the observation of an abrupt, interaction-driven transition to full magnetization, highly reminiscent of Bloch ferromagnetism. Our platform utilizes the two-dimensional Fermi sea of composite fermions near half-filling of the lowest Landau level. We measure the Fermi wavevector—which directly provides the spin polarization—and observe a sudden transition from a partially spin-polarized to a fully spin-polarized ground state as we lower the density of the composite fermions. Our theoretical calculations that take Landau level mixing into account provide a semi-quantitative account of this phenomenon. Composite fermions can be tuned to very low effective density in a clean two-dimensional electron gas, which allows the formation of a Bloch ferromagnet.

Measurement of the ground-state spin polarization of quantum systems offers great potential for the discovery and characterization of correlated electronic states. However, spin polarization measurements have mainly involved optical1–3 and NMR4,5 techniques that perturb the delicate ground states and, for quantum Hall systems, have provided conflicting results1,4,6. Here we present spin-resolved pulsed tunnelling (SRPT) that precisely determines the phase diagram of the ground-state spin polarization as a function of magnetic field and Landau level (LL) filling factor (ν) with negligible perturbation to the system. Our phase diagram shows a variety of polarized, unpolarized and topological spin states in the lowest (N = 0) LL, which can largely be described by a weakly interacting composite fermion (CF) model7. However, the phase diagram shows unexpected behaviour in the N = 1 LL. We observe fully polarized ν = 5/2 and 8/3 states but a partially depolarized ν = 7/3 state. This behaviour deviates from the conventional theoretical picture7,8 of weakly interacting fractional quasiparticles, but instead suggests unusual electronic correlations and the possibility of new non-Abelian phases9–11. The results establish SRPT as a powerful technique for investigating correlated electron phenomena. The spin polarization of a quantum Hall system is determined by a spin-resolved tunnelling method. This technique shows a substantial regime where the weakly interacting composite fermion picture is not valid.

The Hubbard model constitutes one of the most celebrated theoretical frameworks of condensed-matter physics. It describes strongly correlated phases of interacting quantum particles confined in a lattice potential. For bosons, in the last two decades the Hubbard Hamiltonian has been deeply scrutinised in the regime of short-range on-site interactions. On the other hand, extensions to longer-range off-site couplings between neighbouring lattice sites have remained mostly elusive experimentally. Entering this regime constitutes a well identified research frontier where quantum matter phases can spontaneously break the lattice symmetry. Here we unveil one of such phases, precisely the long-sought-after checkerboard solid. It is accessed by confining semiconductors dipolar excitons in a two-dimensional square lattice. The exciton checkerboard is signalled by a strongly minimised compressibility at half-filling of the lattice sites, in quantitative agreement with theoretical expectations. Our observations thus highlight that dipolar excitons enable controlled implementations of extended Bose-Hubbard Hamiltonians.

A low-disorder, two-dimensional electron system (2DES) subjected to a large perpendicular magnetic field and cooled to very low temperatures provides a rich platform for studies of many-body quantum phases. The magnetic field quenches the electrons' kinetic energy and quantizes the energy into a set of Landau levels, allowing the Coulomb interaction to dominate. In excited Landau levels, the fine interplay between short- and long-range interactions stabilizes bubble phases, Wigner crystals with more than one electron per unit cell. Here, we present the screening properties of bubble phases, probed via a simple capacitance technique where the 2DES is placed between a top and a bottom gate and the electric field penetrating through the 2DES is measured. The bubbles formed at very low temperatures screen the electric field poorly as they are pinned by the residual disorder potential, allowing a large electric field to reach the top gate. As the temperature is increased, the penetrating electric field decreases and, surprisingly, exhibits a pronounced minimum at a temperature that appears to coincide with the melting temperature of the bubble phase. We deduce a quantitative phase diagram, as a function of Landau level filling factor (\ensuremath{\nu}) and temperature, for the transition from the bubble to liquid phases for $4\ensuremath{\le}\ensuremath{\nu}\ensuremath{\le}5$.

Domain walls in fractional quantum Hall ferromagnets are gapless helical one-dimensional channels formed at the boundaries of topologically distinct quantum Hall (QH) liquids. Na\"{i}vely, these helical domain walls (hDWs) constitute two counter-propagating chiral states with opposite spins. Coupled to an s-wave superconductor, helical channels are expected to lead to topological superconductivity with high order non-Abelian excitations. Here we investigate transport properties of hDWs in the $\nu=2/3$ fractional QH regime. Experimentally we found that current carried by hDWs is substantially smaller than the prediction of the na\"{i}ve model. Luttinger liquid theory of the system reveals redistribution of currents between quasiparticle charge, spin and neutral modes, and predicts the reduction of the hDW current. Inclusion of spin-non-conserving tunneling processes reconciles theory with experiment. The theory confirms emergence of spin modes required for the formation of fractional topological superconductivity., Comment: 26 pages, 8 figures

Anomalous nematic states, recently discovered in ultraclean two-dimensional electron gas, emerge from quantum Hall stripe phases upon further cooling. These states are hallmarked by a local minimum (maximum) in the hard (easy) longitudinal resistance and by an incipient plateau in the Hall resistance in nearly half-filled Landau levels. Here, we demonstrate that a modest in-plane magnetic field, applied either along $\left < 110 \right >$ or $\left < 1\bar10 \right >$ crystal axis of GaAs, destroys anomalous nematic states and restores quantum Hall stripe phases aligned along their native $\left < 110 \right >$ direction. These findings confirm that anomalous nematic states are distinct from other ground states and will assist future theories to identify their origin., 5 pages, 4 figures

We create laterally large and low disorder quantum well based quantum dots to study single electron additions to two dimensional electron systems (2DES). Electrons tunnel into these dots across an AlGaAs tunnel barrier from a single $n+$ electrode. Using single-electron capacitance spectroscopy in a dilution refrigerator, we identify capacitance peaks for the addition of the first electron to a dot and record subsequent peaks in the addition spectrum up to occupancies of thousands of electrons. Here, we report two remarkable phenomena that occur in the filling factor range $\nu=2$ to $\nu=5$ while selectively probing electron additions to the edge states of the dot: (1) Coulomb blockade peaks arise from the entrance of two electrons rather than one; (2) at and near filling factor 5/2 and at fixed gate voltage, these double-height peaks appear uniformly with a periodicity of $h/2e$. At other filling factors in the range $\nu=2$ to $\nu=5$, the mean periodicity for the twice-height electron peaks remains $h/2e$, but the twice-height peaks are instead further bunched into pairs of double-height peaks, with pairs spaced $h/e$ apart. The unusual two-electron Coulomb blockade peaks suggest a novel pair tunneling effect that involves electron correlations that arise in the quantum dot, with spectra at $\nu=5/2$ identical to those previously only seen in superconducting dots., Comment: Added discussion to "bunching phenomena" section in supplement

Exciton-polaritons are hybrid light-matter excitations arising from the nonperturbative coupling of a photonic mode and an excitonic resonance. Behaving as interacting photons, they show optical third-order nonlinearities providing effects such as optical parametric oscillation or amplification. It has been suggested that polariton-polariton interactions can be greatly enhanced by inducing aligned electric dipoles in their excitonic part. However, direct evidence of a true particle-particle interaction, such as superfluidity or parametric scattering, is still missing. In this Letter, we demonstrate that dipolar interactions can be used to enhance parametric effects such as self-phase modulation in waveguide polaritons. By quantifying these optical nonlinearities, we provide a reliable experimental measurement of the direct dipolar enhancement of polariton-polariton interactions.

We introduce a design of electrically isolated floating bilayer GaAs quantum wells (QW) in which application of a large gating voltage controllably and highly reproducibly induces charges that remain trapped in the bilayer after removal of the gating voltage. At smaller gate voltages, the bilayer is fully electrically isolated from external electrodes by thick insulating barriers. This design permits full control of the total and differential densities of two coupled 2D electron systems. The floating bilayer design provides a unique approach for studying systems inaccessible by simple transport measurements. It also provides the ability to measure the charge transfer between the layers, even when the in-plane resistivities of the 2D systems diverge. We measure the capacitance and inter-layer tunneling spectra of the QW bilayer with independent control of the top and bottom layer electron densities. Our measurements display strongly enhanced inter-layer tunneling current at the total filling factor of 1, a signature of exciton condensation of a strongly interlayer-correlated bilayer system. With fully tunable densities of individual layers, the floating bilayer QW system provides a versatile platform to access previously unavailable information on the quantum phases in electron bilayer systems.

The effect of spin-orbit interaction was studied in a high-quality $p$-AlGaAs/GaAs/AlGaAs structure with a square quantum well using acoustic methods. The structure grown on a GaAs (100) substrate was symmetrically doped with carbon on both sides of the quantum well. Shubnikov-de Haas-type oscillations of the ac conductance of two-dimensional holes were measured. At a low magnetic field $B, Comment: 6 pages, 7 figures

The fractional quantum Hall effect stands as a quintessential manifestation of an interacting two-dimensional electron system. One of the fractional quantum Hall effect's most fundamental characteristics is the energy gap separating the incompressible ground state from its excitations. Yet, despite nearly four decades of investigations, a quantitative agreement between the theoretically calculated and experimentally measured energy gaps is lacking. Here we report a systematic experimental study that incorporates very high-quality two-dimensional electron systems confined to GaAs quantum wells with fixed density and varying well widths. The results demonstrate a clear decrease of the energy gap as the electron layer is made thicker and the short-range component of the Coulomb interaction is weakened. We also provide a quantitative comparison between the measured energy gaps and the available theoretical calculations that takes into account the role of finite layer thickness and Landau level mixing. All the measured energy gaps fall below the calculations, but as the electron layer thickness increases, the results of experiments and calculations come closer. Accounting for the role of disorder in a phenomenological manner, we find better overall agreement between the measured and calculated energy gaps, although some puzzling discrepancies remain.

Memory or transistor devices based on an electron's spin rather than its charge degree of freedom offer certain distinct advantages and comprise a cornerstone of spintronics. Recent years have witnessed the emergence of a new field, valleytronics, which seeks to exploit an electron's valley index rather than its spin. An important component in this quest would be the ability to control the valley index in a convenient fashion. Here we show that the valley polarization can be switched from zero to 1 by a small reduction in density, simply tuned by a gate bias, in a two-dimensional electron system. This phenomenon, which is akin to Bloch spin ferromagnetism, arises fundamentally as a result of electron-electron interaction in an itinerant, dilute electron system. Essentially, the kinetic energy favors an equal distribution of electrons over the available valleys, whereas the interaction between electrons prefers single-valley occupancy below a critical density. The gate-bias-tuned transition we observe is accompanied by a sudden, twofold change in sample resistance, making the phenomenon of interest for potential valleytronic transistor device applications. Our observation constitutes a quintessential demonstration of valleytronics in a very simple experiment.

We report a two-dimensional artificial lattice for dipolar excitons confined in a GaAs double quantum well. Exploring the regime of large fillings per lattice site, we verify that the lattice depth competes with the magnitude of excitons repulsive dipolar interactions to control the degree of localisation in the lattice potential. Moreover, we show that dipolar excitons radiate a narrow-band photoluminescence, with a spectral width of a few hundreds of micro-eV at 340 mK, in both localised and delocalised regimes. This makes our device suitable for explorations of dipolar excitons quasi-condensation in a periodic potential., 5 pages, 4 figures

From measured magnetic field dependences of attenuation and velocity of surface acoustic waves (SAW), we calculated the real part of electron the conductivity in a 75-nm-wide n-GaAs/AlGaAs quantum well in magnetic fields of up to 18 T at frequencies of 30–300 MHz in the temperature range 20–500 mK. We observed slow magneto-oscillations of the conductivity depended on SAW intensity and occurred due to elastic intersubband scattering between the symmetric (S) and antisymmetric (AS) subbands formed by Coulomb repulsion between the electrons. Our theoretical description of the magneto-oscillations allowed estimating the quantum and the intersubband scattering times. The experimentally obtained subband splitting value 0.42 meV was close to the theoretically found 0.57 meV. Additionally, in tilted magnetic fields of 0.5–1.5, T we observed crossings of the Landau levels between the S and AS subbands. According to the developed theory, the crossings at the in-plane field below 1.5 T occur due to different dependences of cyclotron energies in the subbands on the in-plane field. Namely, the cyclotron energy in the S (AS) subband decreases (increases) with the rising of the in-plane field. Work supported by “BASIS,” NSF DMR-1644779 and DMR-1420541, GBMF4420, and State of Florida.]

Two-dimensional electrons confined to GaAs quantum wells are hallmark platforms for probing electron-electron interaction. Many key observations have been made in these systems as sample quality improved over the years. Here, we present a breakthrough in sample quality via source-material purification and innovation in GaAs molecular beam epitaxy vacuum chamber design. Our samples display an ultra-high mobility of $44\times10^6$ cm$^2$/Vs at an electron density of $2.0\times10^{11}$ /cm$^2$. These results imply only 1 residual impurity for every $10^{10}$ Ga/As atoms. The impact of such low impurity concentration is manifold. Robust stripe/bubble phases are observed, and several new fractional quantum Hall states emerge. Furthermore, the activation gap of the $\nu=5/2$ state, which is widely believed to be non-Abelian and of potential use for topological quantum computing, reaches $\Delta\simeq820$ mK. We expect that our results will stimulate further research on interaction-driven physics in a two-dimensional setting and significantly advance the field., Comment: 15 pages, 4 figures in main text. 4 pages, 2 figures in supplement. Nat. Mater. (2021)

A fundamental concept in physics is the Fermi surface, the constant-energy surface in momentum space encompassing all the occupied quantum states at absolute zero temperature. In 1960, Luttinger postulated that the area enclosed by the Fermi surface should remain unaffected even when electron-electron interaction is turned on, so long as the interaction does not cause a phase transition. Understanding what determines the Fermi surface size is a crucial and yet unsolved problem in strongly interacting systems such as high-$T_{c}$ superconductors. Here we present a precise test of the Luttinger theorem for a two-dimensional Fermi liquid system where the exotic quasi-particles themselves emerge from the strong interaction, namely for the Fermi sea of composite fermions (CFs). Via direct, geometric resonance measurements of the CFs' Fermi wavevector down to very low electron densities, we show that the Luttinger theorem is obeyed over a significant range of interaction strengths, in the sense that the Fermi sea area is determined by the density of the \textit{minority carriers} in the lowest Landau level. Our data also address the ongoing debates on whether or not CFs obey particle-hole symmetry, and if they are Dirac particles. We find that particle-hole symmetry is obeyed, but the measured Fermi sea area differs quantitatively from that predicted by the Dirac model for CFs., 6 pages, 4 figures

Hydrostatic pressure is a useful tool that can tune several key parameters in solid state materials. For example, the Land\'e $g$-factor in GaAs two-dimensional electron systems (2DESs) is expected to change from its bulk value $g\simeq-0.44$ to zero and even to positive values under a sufficiently large hydrostatic pressure. Although this presents an intriguing platform to investigate electron-electron interaction in a system with $g=0$, studies are quite limited because the GaAs 2DES density decreases significantly with increasing hydrostatic pressure. Here we show that a simple model, based on pressure-dependent changes in the conduction band alignment, quantitatively explains this commonly observed trend. Furthermore, we demonstrate that the decrease in the 2DES density can be suppressed by more than a factor of 3 through an innovative heterostructure design., Comment: 4 pages, 3 figures

Suppressing electron scattering is essential to achieve high-mobility two-dimensional electron systems (2DESs) that are clean enough to probe exotic interaction-driven phenomena. In heterostructures it is common practice to utilize modulation doping, where the ionized dopants are physically separated from the 2DES channel. The doping-well structure augments modulation doping by providing additional screening for all types of charged impurities in the vicinity of the 2DES, which is necessary to achieve record-breaking samples. Despite its prevalence in the design of ultra-high-mobility 2DESs, the working principles of the doping-well structure have not been reported. Here we elaborate on the mechanics of electron transfer from doping wells to the 2DES, focusing on GaAs/AlGaAs samples grown by molecular beam epitaxy. Based on this understanding we demonstrate how structural parameters in the doping well can be varied to tune the properties of the 2DES., 6 pages, 5 fitures

Microwave-induced resistance oscillations (MIROs) and zero-resistance states (ZRSs) occur in high-mobility two-dimensional electron gas exposed to microwave (MW). We observe that the velocity shift ($\mathrm{\ensuremath{\Delta}}v/v$) oscillates in anticorrelation with MIRO, and $\mathrm{\ensuremath{\Delta}}v/v$ shows peaks at the minimal resistance of MIRO or at ZRS. The SAW velocity features of ZRS remain robust even in the absence of external driving current, which suggests the involvement of intrinsic mechanism in the nonequilibrium phase. In addition, under high-power MW, the phase (${\ensuremath{\varphi}}_{\mathrm{ac}}$) of ZRS stays constant at about 1/4, whereas the phase of the transitions in MIRO is reduced to below 0.10. We argue that the peaks of SAW velocity at ZRS may result from the inhomogeneity of superposed current domain structures. Moreover, a multiphoton process around $\ensuremath{\varepsilon}=1/2$ is observed in the SAW measurements.

A sufficiently large perpendicular magnetic field quenches the kinetic (Fermi) energy of an interacting two-dimensional (2D) system of fermions, making them susceptible to the formation of a Wigner solid (WS) phase in which the charged carriers organize themselves in a periodic array in order to minimize their Coulomb repulsion energy. In low-disorder 2D electron systems confined to modulation-doped GaAs heterostructures, signatures of a magnetic-field-induced WS appear at low temperatures and very small Landau level filling factors ($\nu\simeq1/5$). In dilute GaAs 2D \textit{hole} systems, on the other hand, thanks to the larger hole effective mass and the ensuing Landau level mixing, the WS forms at relatively higher fillings ($\nu\simeq1/3$). Here we report our measurements of the fundamental temperature vs. filling phase diagram for the 2D holes' WS-liquid \textit{thermal melting}. Moreover, via changing the 2D hole density, we also probe their Landau level mixing vs. filling WS-liquid \textit{quantum melting} phase diagram. We find our data to be in good agreement with the results of very recent calculations, although intriguing subtleties remain., Comment: Phys. Rev. Lett. (in press) (2020)

What is the fate of the ground state of a two-dimensional electron system (2DES) at very low Landau level filling factors ($\nu$) where interaction reigns supreme? An ordered array of electrons, the so-called Wigner crystal, has long been believed to be the answer. It was in fact the search for the elusive Wigner crystal that led to the discovery of an unexpected, incompressible liquid state, namely the fractional quantum Hall state at $\nu=1/3$. Understanding the competition between the liquid and solid ground states has since remained an active field of fundamental research. Here we report experimental data for a new two-dimensional system where the electrons are confined to an AlAs quantum well. The exceptionally high quality of the samples and the large electron effective mass allow us to determine the liquid-solid phase diagram for the two-dimensional electrons in a large range of filling factors near $\simeq 1/3$ and $\simeq 1/5$. The data and their comparison with an available theoretical phase diagram reveal the crucial role of Landau level mixing and finite electron layer thickness in determining the prevailing ground states.

We study two-dimensional excitons confined in a lattice potential, for high fillings of the lattice sites. We show that a quasi-condensate is possibly formed for small values of the lattice depth, but for larger ones the critical phase-space density for quasi-condensation rapidly exceeds our experimental reach, due to the increase of the excitons effective mass. On the other hand, in the regime of a deep lattice potential where excitons are strongly localised at the lattice sites, we show that an array of phase-independent quasi-condensates, different from a Mott insulating phase, is realised., 5 pages 4 figures

International audience; Emergence of algebraic quasi-long-range order is a key feature of superfluid phase transitions at two dimensions. For this reduced dimensionality interactions prevent Bose-Einstein condensation with true long range order, at any finite temperature. Here, we report the occurence of algebraic order in a strongly interacting quantum liquid formed by dipolar excitons confined in a bilayer semiconductor heterostructure. We observe a transition from exponential to algebraic decay of the excitons temporal coherence, accompanied by a universal scaling behaviour of the equation of state. Our results provide strong evidence for a Berezinskii-Kosterlitz-Thouless (BKT) transition in a multi-component boson-like system governed by strong dipolar interactions.

Quantum Hall stripe phases near half-integer filling factors $\ensuremath{\nu}\ensuremath{\ge}9/2$ were predicted by Hartree-Fock (HF) theory and confirmed by discoveries of giant resistance anisotropies in high-mobility two-dimensional electron gases. A theory of such anisotropy was proposed by MacDonald and Fisher, although they used parameters whose dependencies on the filling factor, electron density, and mobility remained unspecified. Here, we fill this void by calculating the hard-to-easy resistivity ratio as a function of these three variables. Quantitative comparison with experiment yields very good agreement, which we view as evidence for the ``plain vanilla'' smectic stripe HF phases.

We study the magnetoresistance of an ultrahigh mobility GaAs/AlGaAs two-dimensional electron system (2DES) in a weak magnetic field under low-frequency $(fl20$ GHz) microwave (MW) irradiation. We observe that, with decreasing MW frequency, microwave induced resistance oscillations (MIRO) are damped and multiphoton processes become dominant. At very low MW frequency $(fl4$ GHz), MIRO disappear gradually and an SdH-like oscillation develops. Our analysis indicates that the oscillation may originate from alternating Hall-field induced resistance oscillations (ac-HIRO), due to the transition from the elastic scattering in real space. On the other hand, from the view of photon energy, the oscillations can be understood as a multiphoton process of MIRO in the low MW frequency limit. We show that the two different nonequilibrium mechanisms of MIRO and HIRO can be unified under low-frequency MW irradiation.

We report on detailed experimental studies of a high-quality heterojunction insulated-gate field-effect transistor (HIGFET) to probe the particle-hole symmetry of the fractional quantum Hall effect (FQHE) states about half-filling in the lowest Landau level. The HIGFET is specially designed to vary the density of a two-dimensional electronic system under constant magnetic fields. We find in our constant magnetic field, variable density measurements that the sequence of FQHE states at filling factors ν=1/3,2/5,3/7… and its particle-hole conjugate states at filling factors 1-ν=2/3,3/5,4/7… have a very similar energy gap. Moreover, a reflection symmetry can be established in the magnetoconductivities between the ν and 1-ν states about half-filling. Our results demonstrate that the FQHE states in the lowest Landau level are manifestly particle-hole symmetric.

The single-particle spectral function measures the density of electronic states (DOS) in a material as a function of both momentum and energy, providing central insights into phenomena such as superconductivity and Mott insulators. While scanning tunneling microscopy (STM) and other tunneling methods have provided partial spectral information, until now only angle-resolved photoemission spectroscopy (ARPES) has permitted a comprehensive determination of the spectral function of materials in both momentum and energy. However, ARPES operates only on electronic systems at the material surface and cannot work in the presence of applied magnetic fields. Here, we demonstrate a new method for determining the full momentum and energy resolved electronic spectral function of a two-dimensional (2D) electronic system embedded in a semiconductor. In contrast with ARPES, the technique remains operational in the presence of large externally applied magnetic fields and functions for electronic systems with zero electrical conductivity or with zero electron density. It provides a direct high-resolution and high-fidelity probe of the dispersion and dynamics of the interacting 2D electron system. By ensuring the system of interest remains under equilibrium conditions, we uncover delicate signatures of many-body effects involving electron-phonon interactions, plasmons, polarons, and a novel phonon analog of the vacuum Rabi splitting in atomic systems.

I will introduce a new platform based on spin transitions in the fractional quantum Hall effect regime where parafermions - higher order non-abelian excitations - can be realized. Local (gate) control of spin transition allows formation of isolated domain walls, which consist of counter-propagating edge states of opposite polarization with fractional charge excitations. When superconductivity is induced into such a domain wall from superconducting contacts via proximity effect, parafermions are expected to be formed at the domain wall boundaries. In a multi-gate device a re-configurable network of domain walls can be formed allowing creation, braiding, manipulation and fusion of parafermions. In respect to the quantum computing application parafermons are more computationally intense than Majoranas and are a building block for Fibonacci fermions, even high order non-Abelian particles that can perform universal gate operations within the topologically protected subspace.

Two-dimensional interacting electrons exposed to strong perpendicular magnetic fields generate emergent, exotic quasiparticles phenomenologically distinct from electrons. Specifically, electrons bind with an even number of flux quanta, and transform into composite fermions (CFs). Besides providing an intuitive explanation for the fractional quantum Hall states, CFs also possess Fermi-liquid-like properties, including a well-defined Fermi sea, at and near even-denominator Landau level filling factors such as $��=1/2$ or $1/4$. Here, we directly probe the Fermi sea of the rarely studied four-flux CFs near $��=1/4$ via geometric resonance experiments. The data reveal some unique characteristics. Unlike in the case of two-flux CFs, the magnetic field positions of the geometric resonance resistance minima for $��1/4$ are symmetric with respect to the position of $��=1/4$. However, when an in-plane magnetic field is applied, the minima positions become asymmetric, implying a mysterious asymmetry in the CF Fermi sea anisotropy for $��1/4$. This asymmetry, which is in stark contrast to the two-flux CFs, suggests that the four-flux CFs on the two sides of $��=1/4$ have very different effective masses, possibly because of the proximity of the Wigner crystal formation at small $��$., 7 pages, 4 figures, supplemental materials

Recent progress in condensed matter physics, such as for graphene, topological insulators, and Weyl semimetals, often originate from the specific topological symmetries of their lattice structures. Quantum states with different degrees of freedom, e.g., spin, valley, layer, etc., arise from these symmetries, and the coherent superposition of these states form multiple energy subbands. The pseudospin, a concept analogous to the Dirac spinor matrices, is a successful description of such multisubband systems. When the electron-electron interaction dominates, many-body quantum phases arise. They usually have discrete pseudospin polarizations and exhibit sharp phase transitions at certain universal critical pseudospin energy splittings. In this Letter, we present our discovery of hydrostatic-pressure-induced degeneracy between the two lowest Landau levels. This degeneracy is evidenced by the pseudospin polarization transitions of the fragile correlated quantum liquid phases near the Landau level filling factor $\ensuremath{\nu}=3/2$. Benefitting from the constant hole concentration and the sensitive nature of these transitions, we study the fine-tuning effect of the hydrostatic pressure at the order of $10\text{ }\text{ }\ensuremath{\mu}\mathrm{eV}$, well beyond the meV-level state-of-the-art resolution of other techniques.

We have developed a scanning photoluminescence technique that can directly map out the local two-dimensional electron density with a relative accuracy of $\sim2.2\times10^8$ cm$^{-2}$. The validity of this approach is confirmed by the observation of the expected density gradient in a high-quality GaAs quantum well sample that was not rotated during the molecular beam epitaxy of its spacer layer. In addition to this global variation in electron density, we observe local density fluctuations across the sample. These random density fluctuations are also seen in samples that were continuously rotated during growth, and we attribute them to residual space charges at the substrate-epitaxy interface. This is corroborated by the fact that the average magnitude of density fluctuations is increased to $\sim9\times10^{9}$ cm$^{-2}$ from $\sim1.2\times10^9$ cm$^{-2}$ when the buffer layer between the substrate and the quantum well is decreased by a factor of seven. Our data provide direct evidence for local density inhomogeneities even in very high-quality two-dimensional carrier systems., 6 pages, 3 figures

One of the most fundamental and yet elusive collective phases of an interacting electron system is the quantum Wigner crystal (WC), an ordered array of electrons expected to form when the electrons' Coulomb repulsion energy eclipses their kinetic (Fermi) energy. In low-disorder, two-dimensional (2D) electron systems, the quantum WC is known to be favored at very low temperatures ($T$) and small Landau level filling factors ($\nu$), near the termination of the fractional quantum Hall states. This WC phase exhibits an insulating behavior, reflecting its pinning by the small but finite disorder potential. An experimental determination of a $T$ vs $\nu$ phase diagram for the melting of the WC, however, has proved to be challenging. Here we use capacitance measurements to probe the 2D WC through its effective screening as a function of $T$ and $\nu$. We find that, as expected, the screening efficiency of the pinned WC is very poor at very low $T$ and improves at higher $T$ once the WC melts. Surprisingly, however, rather than monotonically changing with increasing $T$, the screening efficiency shows a well-defined maximum at a $T$ which is close to the previously-reported melting temperature of the WC. Our experimental results suggest a new method to map out a $T$ vs $\nu$ phase diagram of the magnetic-field-induced WC precisely., Comment: The formal version is published on Phys. Rev. Lett. 122, 116601 (2019)

Using acoustic method we study dependences of transverse AC conductance, $\sigma (\omega)$, on magnetic field, temperature and the amplitude of AC electric field in a wide (75 nm) quantum well (QW) structure focusing on the vicinity of the filling factor $\nu =1/2$. Measurements are performed in the frequency domain 30-307 MHz and in the temperature domain 20-500 mK. Usually, in wide QW structures closely to $\nu =1/2$ the fractional quantum Hall effect (FQHE) regime is realized at some parameters of the sample. However, in our structure, at $\nu =1/2$ it is a compressible state corresponding to gas of composite fermions which is observed. This is confirmed by apparent frequency independence and weakly decreasing temperature dependence of $\mathrm{Re}\, \sigma(\omega)$. Comparing the dependences of this quantity on temperature and power of the acoustic wave we conclude that the observed nonlinear behavior of the conductance is compatible with heating of the composite fermions by the acoustic wave. For comparison, we also study the vicinity of $\nu = 3/2$ where the FQHE regime is clearly observed., Comment: 6 pages, 6 figures

We report on quantum Hall stripes (QHSs) formed in higher Landau levels of GaAs/AlGaAs quantum wells with high carrier density ($n_e > 4 \times 10^{11}$ cm$^{-2}$) which is expected to favor QHS orientation along unconventional $\left < 1\bar{1}0 \right >$ crystal axis and along the in-plane magnetic field $B_{||}$. Surprisingly, we find that at $B_{||} = 0$ QHSs in our samples are aligned along $\left < 110 \right >$ direction and can be reoriented only perpendicular to $B_{||}$. These findings suggest that high density alone is not a decisive factor for either abnormal native QHS orientation or alignment with respect to $B_{||}$, while quantum confinement of the 2DEG likely plays an important role., 4 pages

Low-temperature illumination of a two-dimensional electron gas in GaAs quantum wells is known to greatly improve the quality of high-field magnetotransport. The improvement is known to occur even when the carrier density and mobility remain unchanged, but what exactly causes it remains unclear. Here, we investigate the effect of illumination on microwave photoresistance in low magnetic fields. We find that the amplitude of microwave-induced resistance oscillations grows dramatically after illumination. Dingle analysis reveals that this growth reflects a substantial increase in the single-particle (quantum) lifetime, which likely originates from the light-induced redistribution of charge enhancing the screening capability of the doping layers.

Microwave spectroscopy within the Landau filling ($\ensuremath{\nu}$) range of the integer quantum Hall effect (IQHE) has revealed pinning mode resonances signifying Wigner solids (WSs) composed of quasiparticles or -holes. We study pinning modes of WSs in wide quantum wells (WQWs) for $0.8\ensuremath{\le}\ensuremath{\nu}\ensuremath{\le}1.2$, varying the density, $n$, and tilting the sample by angle $\ensuremath{\theta}$ in the magnetic field. Three distinct WS phases are accessed. One phase, S1, is phenomenologically the same as the WS observed in the IQHEs of narrow QWs. The second phase, S2, exists at $\ensuremath{\nu}$ further from $\ensuremath{\nu}=1$ than S1, and requires a sufficiently large $n$ or $\ensuremath{\theta}$, implying S2 is stabilized by the Zeeman energy. The melting temperatures of S1 and S2, estimated from the disappearance of the pinning mode, show different behavior versus $\ensuremath{\nu}$. At the largest $n$ or $\ensuremath{\theta}$, S2 disappears and the third phase, S1A, replaces S1, also exhibiting a pinning mode. This occurs as the WQW $\ensuremath{\nu}=1$ IQHE becomes a two-component, Halperin-Laughlin ${\mathrm{\ensuremath{\Psi}}}_{111}$ state. We interpret S1A as a WS of the excitations of ${\mathrm{\ensuremath{\Psi}}}_{111}$, which has not been previously observed.

Pinning modes of a Wigner solid show remarkably small screening by a fractional quantum Hall liquid in close proximity., We studied a bilayer system hosting two-dimensional electron systems (2DESs) in close proximity but isolated from one another by a thin barrier. One 2DES has low electron density and forms a Wigner solid (WS) at high magnetic fields. The other has much higher density and, in the same field, exhibits fractional quantum Hall states (FQHSs). The WS spectrum has resonances which are understood as pinning modes, oscillations of the WS within the residual disorder. We found the pinning mode frequencies of the WS are strongly affected by the FQHSs in the nearby layer. Analysis of the spectra indicates that the majority layer screens like a dielectric medium even when its Landau filling is ~1/2, at which the layer is essentially a composite fermion (CF) metal. Although the majority layer is only ~ one WS lattice constant away, a WS site only induces an image charge of ~0.1e in the CF metal.

The fractional quantum Hall state (FQHS) observed at a half-filled Landau level in an interacting two-dimensional electron system (2DES) is among the most exotic states of matter as its quasiparticles are expected to be Majoranas with non-Abelian statistics. We demonstrate here the unexpected presence of such a state in a novel 2DES with a strong band-mass anisotropy. The FQHS we observe has unusual characteristics. While its Hall resistance is well-quantized at low temperatures, it exhibits highly-anisotropic in-plane transport resembling compressible stripe/nematic charge-density-wave phases. More striking, the anisotropy sets in suddenly below a critical temperature, suggesting a finite-temperature phase transition. Our observations highlight how anisotropy modifies the many-body phases of a 2DES, and should further fuel the discussion surrounding the enigmatic even-denominator FQHS., Comment: Accepted for publication in Phys. Rev. Lett

One of the most fascinating ground states of an interacting electron system is the so-called Wigner crystal where the electrons, in order to minimize their repulsive Coulomb energy, form an ordered array. Here we report measurements of the critical filling factor ($\nu_{C}$) below which a magnetic-field-induced, quantum Wigner crystal forms in a dilute, two-dimensional electron layer when a second, high-density electron layer is present in close proximity. The data reveal that the Wigner crystal forms at a significantly smaller $\nu_{C}$ compared to the $\nu_{C}$ ($\simeq 0.20$) in single-layer two-dimensional electron systems. The measured $\nu_{C}$ exhibits a strong dependence on the interlayer distance, reflecting the interaction and screening from the adjacent, high-density layer., Comment: The formal version is published on Phys. Rev. B (2018)

In a number of widely studied materials, such as Si, AlAs, Bi, graphene, MoS_{2}, and many transition metal dichalcogenide monolayers, electrons acquire an additional, spinlike degree of freedom at the degenerate conduction band minima, also known as "valleys." External symmetry-breaking fields such as mechanical strain, or electric or magnetic fields, can tune the valley polarization of these materials, making them suitable candidates for "valleytronics." Here we study a quantum well of AlAs, where the two-dimensional electrons reside in two energetically degenerate valleys. By fabricating a strain-inducing grating on the sample surface, we engineer a spatial modulation of the electron population in different valleys, i.e., a "valley superlattice" in the quantum well plane. Our results establish a novel manipulation technique of the valley degree of freedom, paving the way to realizing a valley-selective layered structure in multivalley materials, with potential application in valleytronics.

The enigmatic even-denominator fractional quantum Hall state at Landau level filling factor ν=5/2 is arguably the most promising candidate for harboring Majorana quasiparticles with non-Abelian statistics and, thus, of potential use for topological quantum computing. The theoretical description of the ν=5/2 state is generally believed to involve a topological p-wave pairing of fully-spin-polarized composite fermions through their condensation into a non-Abelian Moore-Read Pfaffian state. There is, however, no direct and conclusive experimental evidence for the existence of composite fermions near ν=5/2 or for an underlying fully-spin-polarized Fermi sea. Here, we report the observation of composite fermions very near ν=5/2 through geometric resonance measurements and find that the measured Fermi wave vector provides direct demonstration of a Fermi sea with full spin polarization. This lends crucial credence to the model of 5/2 fractional quantum Hall effect as a topological p-wave paired state of composite fermions.

We propose an experimentally-feasible system based on spin transitions in the fractional quantum Hall effect regime where parafermions, high-order non-abelian excitations, can be potentially realized. We provide a proof-of-concept experiments showing that in specially designed heterostructures spin transitions at a filling factor 2/3 can be induced electrostatically, allowing local control of polarization and on-demand formation of helical domain walls with fractionalized charge excitations, a pre-requisite ingredient for parafermions formation. We also present exact diagonalization numerical studies of domain walls formed between domains with different spin polarization in the fractional quantum Hall effect regime and show that they indeed possess electronic and magnetic structure needed for parafermion formation when coupled to an s-wave superconductor.

Low-defect two-dimensional electron systems (2DESs) are essential for studies of fragile many-body interactions that only emerge in nearly-ideal systems. As a result, numerous efforts have been made to improve the quality of modulation-doped ${\mathrm{Al}}_{x}{\mathrm{Ga}}_{1\ensuremath{-}x}\mathrm{As}$/GaAs quantum wells (QWs), with an emphasis on purifying the source material of the QW itself or achieving better vacuum in the deposition chamber. However, this approach overlooks another crucial component that comprises such QWs, the ${\mathrm{Al}}_{x}{\mathrm{Ga}}_{1\ensuremath{-}x}\mathrm{As}$ barrier. Here we show that having a clean Al source and hence a clean barrier is instrumental to obtain a high-quality GaAs 2DES in a QW. We observe that the mobility of the 2DES in GaAs QWs declines as the thickness or Al content of the ${\mathrm{Al}}_{x}{\mathrm{Ga}}_{1\ensuremath{-}x}\mathrm{As}$ barrier beneath the QW is increased, which we attribute to the surface segregation of oxygen atoms that originate from the Al source. This conjecture is supported by the improved mobility in the GaAs QWs as the Al cell is cleaned out by baking.