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Unveiling the emergence and prevalence of massive/bright galaxies during the epoch of reionization and beyond, within the first 600 million years of the Universe, stands as a pivotal pursuit in astronomy. Remarkable progress has been made by JWST in identifying an immense population of bright galaxies, which hints at exceptionally efficient galaxy assembly processes. However, the underlying physical mechanisms propelling their rapid growth remain unclear. With this in mind, millimeter and submillimeter-wave spectroscopic observations of redshifted far-infrared spectral lines, particularly the [O III] 88 micron and [C II] 158 micron lines, offers a crucial pathway to address this fundamental query. To this end, we develop a dual-polarization sideband-separating superconductor-insulator-superconductor (SIS) mixer receiver, FINER, for the Large Millimeter Telescope (LMT) situated in Mexico. Harnessing advancements from ALMA's wideband sensitivity upgrade (WSU) technology, FINER covers radio frequencies spanning 120-360 GHz, delivering an instantaneous intermediate frequency (IF) of 3-21 GHz per sideband per polarization, which is followed by a set of 10.24 GHz-wide digital spectrometers. At 40% of ALMA's light-collecting area, the LMT's similar atmospheric transmittance and FINER's 5 times wider bandwidth compared to ALMA culminate in an unparalleled spectral scanning capability in the northern hemisphere, paving the way for finer spectral-resolution detection of distant galaxies., Comment: 12 pages, 8 figures, and 3 tables. Proceedings paper presented in SPIE Astronomical Telescope and Instrumentation 2024

Nanometre- to micrometre-sized solid dust particles play a vital role in star and planet formations. Despite of their importance, however, our understanding of physical and chemical properties of dust particles is still provisional. We have conducted a condensation experiment of the vapour generated from a solid starting material having nearly cosmic proportions in elements. A laser flash heating and subsequent cooling has produced a diverse type of nanoparticles simultaneously. Here we introduce four types of nanoparticles as potential dust particles in space: amorphous silicate nanoparticles (type S); core/mantle nanoparticles with iron or hydrogenised-iron core and amorphous silicate mantle (type IS); silicon oxycarbide nanoparticles and hydrogenised silicon oxycarbide nanoparticles (type SiOC); and carbon nanoparticles (type C), all produced in a single heating-cooling event. Type IS and SiOC nanoparticles are new for potential astrophysical dust. The nanoparticles are aggregated to a wide variety of structures, from compact, fluffy, and networked. A simultaneous formation of nanoparticles, which are diverse in chemistry, shape, and structure, prompts a re-evaluation of astrophysical dust particles, Comment: 9 pages, 3 figures

We study a machine learning (ML) technique for refining images acquired during in situ observation using liquid-cell transmission electron microscopy (LC-TEM). Our model is constructed using a U-Net architecture and a ResNet encoder. For training our ML model, we prepared an original image dataset that contained pairs of images of samples acquired with and without a solution present. The former images were used as noisy images and the latter images were used as corresponding ground truth images. The number of pairs of image sets was $1,204$ and the image sets included images acquired at several different magnifications and electron doses. The trained model converted a noisy image into a clear image. The time necessary for the conversion was on the order of 10ms, and we applied the model to in situ observations using the software Gatan DigitalMicrograph (DM). Even if a nanoparticle was not visible in a view window in the DM software because of the low electron dose, it was visible in a successive refined image generated by our ML model., Comment: 33 pages, 9 figures

It has been implicitly assumed that ices on grains in molecular clouds and proto planetary disks are formed by homogeneous layers regardless of their composition or crystallinity. To verify this assumption, we observed the H2O deposition onto refractory substrates and the crystallization of amorphous ices (H2O, CO2, and CO) using an ultra-high-vacuum transmission electron microscope. In the H2O-deposition experiments, we found that three-dimensional islands of crystalline ice (Ic) were formed at temperatures above 130 K. The crystallization experiments showed that uniform thin films of amorphous CO and H2O became three-dimensional islands of polyhedral crystals; amorphous CO2, on the other hand, became a thin film of nano crystalline CO2 covering the amorphous H2O. Our observations show that crystal morphologies strongly depend not only on the ice composition, but also on the substrate. Using experimental data concerning the crystallinity of deposited ices and the crystallization timescale of amorphous ices, we illustrated the criteria for ice crystallinity in space and outlined the macroscopic morphology of icy grains in molecular clouds as follows: amorphous H2O covered the refractory grain uniformly, CO2 nano-crystals were embedded in the amorphous H2O, and a polyhedral CO crystal was attached to the amorphous H2O. Furthermore, a change in the grain morphology in a proto-planetary disk is shown. These results have important implications for the chemical evolution of molecules, non-thermal desorption, collision of icy grains, and sintering., Comment: 60 pages, 18 figures, 3 tables, published in ApJ

Low-electron-dose observation is indispensable for observing various samples using a transmission electron microscope; consequently, image processing has been used to improve transmission electron microscopy (TEM) images. To apply such image processing to in situ observations, we here apply a convolutional neural network to TEM imaging. Using a dataset that includes short-exposure images and long-exposure images, we develop a pipeline for processed short-exposure images, based on end-to-end training. The quality of images acquired with a total dose of approximately 5 e- per pixel becomes comparable to that of images acquired with a total dose of approximately 1000 e- per pixel. Because the conversion time is approximately 8 ms, in situ observation at 125 fps is possible. This imaging technique enables in situ observation of electron-beam-sensitive specimens., Comment: 8 pages, 7 figures, 3 tables

We study variability of active galactic nuclei (AGNs) by using the deep optical multiband photometry data obtained from the Hyper Suprime-Cam Subaru Strategic Program (HSC SSP) survey in the COSMOS field. The images analyzed here were taken with 8, 10, 13, and 15 epochs over three years in the $g$, $r$, $i$, and $z$ bands, respectively. We identified 491 robust variable AGN candidates, down to $i=25$ mag and with redshift up to $4.26$. Ninety percent of the variability-selected AGNs are individually identified with the X-ray sources detected in the Chandra COSMOS Legacy survey. We investigate their properties in variability by using structure function analysis and find that the structure function for low-luminosity AGNs ($L_{\mathrm{bol}}\lesssim10^{45}$ erg s$^{-1}$) shows a positive correlation with luminosity, which is the opposite trend for the luminous quasars. This trend is likely to be caused by larger contribution of the host galaxy light for lower-luminosity AGNs. Using the model templates of galaxy spectra, we evaluate the amount of host galaxy contribution to the structure function analysis and find that dominance of the young stellar population is needed to explain the observed luminosity dependence. This suggests that low-luminosity AGNs at $0.8\lesssim z\lesssim1.8$ are predominantly hosted in star-forming galaxies. The X-ray stacking analysis reveals the significant emission from the individually X-ray undetected AGNs in our variability-selected sample. The stacked samples show very large hardness ratios in their stacked X-ray spectrum, which suggests that these optically variable sources have large soft X-ray absorption by dust-free gas., Comment: 27 pages, 22 figures. Accepted for publication in ApJ

The interactions of atomic and molecular hydrogen with bare interstellar dust grain surfaces are important for understanding H2 formation at relatively high temperatures (>20 K). We investigate the diffusion of physisorbed H atoms and the desorption energetics of H2 molecules on an amorphous diamond-like carbon (DLC) surface. From temperature-programmed desorption experiments with a resonance-enhanced multiphoton ionization (REMPI) method for H2 detection, the H2 coverage-dependent activation energies for H2 desorption are determined. The activation energies decrease with increasing H2 coverage and are centered at 30 meV with a narrow distribution. Using a combination of photostimulated desorption and REMPI methods, the time variations of the surface number density of H2 following atomic and molecular hydrogen depositions are studied. From these measurements, we show that H2 formation on a DLC surface is quite efficient, even at 20 K. A significant kinetic isotope effect for H2 and D2 recombination reactions suggests that H-atom diffusion on a DLC surface is mediated by quantum mechanical tunneling. In astrophysically relevant conditions, H2 recombination due to physisorbed H-atoms is unlikely to occur at 20 K, suggesting that chemisorbed H atoms might play a role in H2 formation at relatively high temperatures., Comment: 33 pages, 8 figures, Accepted for publication in ApJ

Refractory organic compounds formed in molecular clouds are among the building blocks of the solar system objects and could be the precursors of organic matter found in primitive meteorites and cometary materials. However, little is known about the evolutionary pathways of molecular cloud organics from dense molecular clouds to planetary systems. In this study, we focus on the evolution of the morphological and viscoelastic properties of molecular cloud refractory organic matter. We found that the organic residue, experimentally synthesized at about 10 K from UV-irradiated H2O-CH3OH-NH3 ice, changed significantly in terms of its nanometer- to micrometer-scale morphology and viscoelastic properties after UV irradiation at room temperature. The dose of this irradiation was equivalent to that experienced after short residence in diffuse clouds (equal or less than 10,000 years) or irradiation in outer protoplanetary disks. The irradiated organic residues became highly porous and more rigid and formed amorphous nanospherules. These nanospherules are morphologically similar to organic nanoglobules observed in the least-altered chondrites, chondritic porous interplanetary dust particles, and cometary samples, suggesting that irradiation of refractory organics could be a possible formation pathway for such nanoglobules. The storage modulus (elasticity) of photo-irradiated organic residues is about 100 MPa irrespective of vibrational frequency, a value that is lower than the storage moduli of minerals and ice. Dust grains coated with such irradiated organics would therefore stick together efficiently, but growth to larger grains might be suppressed due to an increase in aggregate brittleness caused by the strong connections between grains., Comment: 11 pages, 8 figures

The abundant forms in which the major elements in the universe exist have been determined from numerous astronomical observations and meteoritic analyses. Iron (Fe) is an exception, in that only depletion of gaseous Fe has been detected in the interstellar medium, suggesting that Fe is condensed into a solid, possibly the astronomically invisible metal. To determine the primary form of Fe, we replicated the formation of Fe grains in gaseous ejecta of evolved stars by means of microgravity experiments. We found that the sticking probability for formation of Fe grains is extremely small; only several atoms will stick per hundred thousand collisions, so that homogeneous nucleation of metallic Fe grains is highly ineffective, even in the Fe-rich ejecta of Type Ia supernovae. This implies that most Fe is locked up as grains of Fe compounds or as impurities accreted onto other grains in the interstellar medium.

We present infrared multi-epoch observations of the dust forming nova V1280 Sco over $\sim$2000 days from the outburst. The temporal evolution of the infrared spectral energy distributions at 1272, 1616 and 1947 days can be explained by the emissions produced by amorphous carbon dust of mass (6.6--8.7)$\times$10$^{-8}$M$_{\odot}$ with a representative grain size of 0.01$~\mu$m and astronomical silicate dust of mass (3.4--4.3)$\times$10$^{-7}$M$_{\odot}$ with a representative grain size of 0.3--0.5$~\mu$m. Both of these dust species travel farther away from the white dwarf without an apparent mass evolution throughout those later epochs. The dust formation scenario around V1280 Sco suggested from our analyses is that the amorphous carbon dust is formed in the nova ejecta followed by the formation of silicate dust in the expanding nova ejecta or as a result of the interaction between the nova wind and the circumstellar medium., Comment: 47 pages, 19 figures. Accepted for publication in the Astrophysical Journal on December 2, 2015