1. Microphysical Interactions Determine the Effectiveness of Solar Radiation Modification via Stratospheric Solid Particle Injection.
- Author
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Vattioni, S., Käslin, S. K., Dykema, J. A., Beiping, L., Sukhodolov, T., Sedlacek, J., Keutsch, F. N., Peter, T., and Chiodo, G.
- Subjects
STRATOSPHERIC aerosols ,RADIATIVE forcing ,SOLAR radiation ,MICROPHYSICS ,INJECTION wells ,OZONE layer - Abstract
Recent studies have suggested that stratospheric aerosol injection (SAI) of solid particles for climate intervention could reduce stratospheric warming compared to injection of SO2 ${\text{SO}}_{2}$. However, interactions of microphysical processes, such as settling and coagulation of solid particles, with stratospheric dynamics have not been considered. Using a global chemistry‐climate model with interactive solid particle microphysics, we show that agglomeration significantly reduces the backscatter efficiency per unit of injected material compared to mono‐disperse particles, partly due to faster settling of the agglomerates, but mainly due to increased forward‐ over backscattering with increasing agglomerate size. Despite these effects, some materials substantially reduce required injection rates as well as perturbation of stratospheric winds, age of air and stratospheric warming compared to injection of SO2 ${\text{SO}}_{2}$, with the most promising results being shown by 150 nm diamond particles. Uncertainties remain as to whether stratospheric dispersion of solid particles is feasible without formation of agglomerates. Plain Language Summary: [Stratospheric warming is an undesired side effect of climate intervention via SAI. Recent studies have shown that stratospheric warming could be reduced when injecting solid particles instead of gaseous SO2 ${\text{SO}}_{2}$. However, most of these studies looked at the stratospheric particle mass required for a given radiative forcing (RF), without accounting for gravitational settling of particles or the effect of particles sticking together after mutual collision. We show that accounting for these effects significantly reduces the amount of backward reflected radiation per unit of stratospheric particle mass decreasing the radiative efficiency of the injected material. This is due to the combined effect of faster gravitational settling and the larger fraction of forward reflected radiation over backward reflected radiation with increasing agglomerate size. However, we show that injection of diamond particles at a radius of 150 nm instead of SO2 ${\text{SO}}_{2}$ significantly reduces required stratospheric injection rates as well as perturbation of stratospheric winds, age of stratospheric air and stratospheric water vapor concentrations due to small stratospheric warming per unit of RF. However, large uncertainties remain as to whether it will be feasible to inject solid particles into the stratosphere at concentrations low enough to prohibit that the particles stick together.] Key Points: We explore stratospheric injections of six solid particles and gaseous SO2 within a climate model with comprehensive aerosol microphysicsAccounting for settling and agglomeration of solid particles can substantially reduce the radiative forcing (RF) per unit of injected materialInjection of diamond particles (r = 150 nm) instead of SO2 largely reduces stratospheric temperature, circulation and water vapor anomalies [ABSTRACT FROM AUTHOR]
- Published
- 2024
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