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Stretchable electrodes are critical to the development of advanced technologies such as human–machine interaction, flexible sensing, and wearable power supply, making them of significant research value. However, the current preparation methods for high‐performance stretchable electrodes are complex and inefficient, posing challenges for their large‐scale application in the realm of flexible wearables. To address this need, a straightforward and efficient embedding strategy is reported for fabricating stretchable silver nanowire/thermoplastic elastomer composite electrodes (referred to as Strem‐AT) utilizing the viscoelasticity and outstanding mechanical properties of polymer elastomers to achieve outstanding extensibility, conductivity, and a smooth surface. These electrodes exhibit excellent tensile behavior, low surface roughness, and stable electrical properties, enabling their successful integration into stretchable sensors and intrinsically stretchable organic photovoltaic cells (IS‐OPV). When applied to human skin joints for motion detection, the sensor demonstrates remarkable stretchability and stable signal output. Importantly, the all‐polymer IS‐OPV exhibits a top‐notch power conversion efficiency (PCE) of >12.5% and a PCE80% strain exceeding 50%. Furthermore, even after subjecting high‐strain stretching at 50% for 1000 cycles, the IS‐OPV can retain 76% of the initial PCE. This study presents a multifunctional stretchable electrode with high repeatability and easy‐to‐scale fabrication in wearable sensors and photovoltaics. [ABSTRACT FROM AUTHOR]

Intrinsically stretchable organic photovoltaic cells (OPVs) have garnered significant attention as crucial devices for powering next‐generation wearable electronics. Despite the rapid power conversion efficiency gains in champion OPVs, their brittle stretchability has failed to meet the demands of the Internet of Things era, severely hindering further development and practical applications. In this regard, a new dual‐donor polymer blending strategy is demonstrated for constructing intrinsically stretchable OPVs by designing a novel high‐molecular–weight conjugated polymer PM6‐HD. This PM6 derivative featuring long alkyl chains can reach a sufficiently high molecular weight and thus exhibits a high fracture strain exceeding 90%, which is ≈12 times higher than the benchmark PM6. Synergistic optimization of mechanical properties and photovoltaic performance in polymer:small molecule and all‐polymer systems constructed from the physical blends of PM6 and PM6‐HD is achieved. Crucially, the resulting intrinsically stretchable OPV demonstrates excellent stretchability and stability, with a record PCE80% strain of 50.3% and the efficiency retention of above 80% even after 1000 cycles of cyclic stretching at high strains. This work contributes to the advancement of intrinsically stretchable OPV technology and opens up new possibilities for its integration into wearable electronic devices. [ABSTRACT FROM AUTHOR]

Composite materials with multi-layer structure were prepared by combining polyurethane film and waste polyphenylene sulfide filters by hot melting, which could be used as sound-absorbing materials to contribute to the noise control and reutilization of industrial waste. The structure, mechanical property, pore size distribution and stability of waste polyphenylene sulfide filters were investigated and could directly affect the quality of recycled products. The effects of layer numbers, layering sequence and polyurethane film thickness on sound absorption and insulation properties were also analyzed using an impedance tube absorption test system. The results showed that multi-layer materials had a better sound absorption effect than single-layer polyphenylene sulfide filters at low frequency. The sound absorption coefficients of the single-layer sample was only 0.081 at 1000 Hz, while the sound absorption coefficients of the five-layer sample could reach 0.26. The sound absorption properties of multi-layer materials were slightly affected by layering sequence, but polyurethane film thickness had a significant effect on sound absorption properties. The α of the SUS1 and USU1 samples were 0.151 and 0.170, while the α of the SUS3 and USU3 samples were only 0.076 and 0.056, respectively. Meanwhile, the sound insulation properties of multi-layer materials could be significantly influenced by the polyurethane film position. The sound transmission loss of the SUSUSU3 sample was just 32.83 dB, whereas that of the USUSU3 sample could reach 47.94 dB. Moreover, when polyurethane film was located on the sound facing side of multi-layer materials, the increase in polyurethane film thickness could cause the average sound reduction index of the USUSU sample to increase from 28.76 dB to 47.94 dB. [ABSTRACT FROM AUTHOR]