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Silicon-based quantum emitters are candidates for large-scale qubit integration due to their single-photon emission properties and potential for spin-photon interfaces with long spin coherence times. Here, we demonstrate local writing and erasing of selected light-emitting defects using femtosecond laser pulses in combination with hydrogen-based defect activation and passivation at a single center level. By choosing forming gas (N2/H2) during thermal annealing of carbon-implanted silicon, we can select the formation of a series of hydrogen and carbon-related quantum emitters, including T and Ci centers while passivating the more common G-centers. The Ci center is a telecom S-band emitter with promising optical and spin properties that consists of a single interstitial carbon atom in the silicon lattice. Density functional theory calculations show that the Ci center brightness is enhanced by several orders of magnitude in the presence of hydrogen. Fs-laser pulses locally affect the passivation or activation of quantum emitters with hydrogen for programmable formation of selected quantum emitters.

Silicon is the most scalable optoelectronic material but has suffered from its inability to generate directly and efficiently classical or quantum light on-chip. Scaling and integration are the most fundamental challenges facing quantum science and technology. We report an all-silicon quantum light source based on a single atomic emissive center embedded in a silicon-based nanophotonic cavity. We observe a more than 30-fold enhancement of luminescence, a near-unity atom-cavity coupling efficiency, and an 8-fold acceleration of the emission from the all-silicon quantum emissive center. Our work opens immediate avenues for large-scale integrated cavity quantum electrodynamics and quantum light-matter interfaces with applications in quantum communication and networking, sensing, imaging, and computing.

When engineered on scales much smaller than the operating wavelength, metal-semiconductor nanostructures exhibit properties unobtainable in nature. Namely, a uniaxial optical metamaterial described by a hyperbolic dispersion relation can simultaneously behave as a reflective metal and an absorptive or emissive semiconductor for electromagnetic waves with orthogonal linear polarization states. Using an unconventional multilayer architecture, we demonstrate luminescent hyperbolic metasurfaces, wherein distributed semiconducting quantum wells display extreme absorption and emission polarization anisotropy. Through normally incident micro-photoluminescence measurements, we observe absorption anisotropies greater than a factor of 10 and degree-of-linear polarization of emission >0.9. We observe the modification of emission spectra and, by incorporating wavelength-scale gratings, show a controlled reduction of polarization anisotropy. We verify hyperbolic dispersion with numerical simulations that model the metasurface as a composite nanoscale structure and according to the effective medium approximation. Finally, we experimentally demonstrate >350% emission intensity enhancement relative to the bare semiconducting quantum wells.

Exceptional points (EPs) can achieve intriguing asymmetric control in non-Hermitian systems due to the degeneracy of eigenstates. Here, we present a general method that extends this specific asymmetric response of EP photonic systems to address any arbitrary fully-polarized light. By rotating the meta-structures at EP, Pancharatnam-Berry (PB) phase can be exclusively encoded on one of the circular polarization-conversion channels. To address any arbitrary wavefront, we superpose the optical signals originating from two orthogonally polarized -yet degenerate- EP eigenmodes. The construction of such orthogonal EP eigenstates pairs is achieved by applying mirror-symmetry to the nanostructure geometry flipping thereby the EP eigenmode handedness from left to right circular polarization. Non-Hermitian reflective PB metasurfaces designed using such EP superposition enable arbitrary, yet unidirectional, vectorial wavefront shaping devices. Our results open new avenues for topological wave control and illustrate the capabilities of topological photonics to distinctively operate on arbitrary polarization-state with enhanced performances., (© 2024. The Author(s).)

Complex networks play a fundamental role in understanding phenomena from the collective behavior of spins, neural networks, and power grids to the spread of diseases. Topological phenomena in such networks have recently been exploited to preserve the response of systems in the presence of disorder. We propose and demonstrate topological structurally disordered systems with a modal structure that enhances nonlinear phenomena in the topological channels by inhibiting the ultrafast leakage of energy from edge modes to bulk modes. We present the construction of the graph and show that its dynamics enhances the topologically protected photon pair generation rate by an order of magnitude. Disordered nonlinear topological graphs will enable advanced quantum interconnects, efficient nonlinear sources, and light-based information processing for artificial intelligence.

Quantum light sources play a fundamental role in quantum technologies ranging from quantum networking to quantum sensing and computation. The development of these technologies requires scalable platforms, and the recent discovery of quantum light sources in silicon represents an exciting and promising prospect for scalability. The usual process for creating color centers in silicon involves carbon implantation into silicon, followed by rapid thermal annealing. However, the dependence of critical optical properties, such as the inhomogeneous broadening, the density, and the signal-to-background ratio, on centers implantation steps is poorly understood. We investigate the role of rapid thermal annealing on the dynamic of the formation of single color centers in silicon. We find that the density and the inhomogeneous broadening greatly depend on the annealing time. We attribute the observations to nanoscale thermal processes occurring around single centers and leading to local strain fluctuations. Our experimental observation is supported by theoretical modeling based on first principles calculations. The results indicate that annealing is currently the main step limiting the scalable manufacturing of color centers in silicon.

Single-aperture cavities are a key component of lasers that are instrumental for the amplification and emission of a single light mode. However, the appearance of high-order transverse modes as the size of the cavities increases has frustrated efforts to scale-up cavities while preserving single-mode operation since the invention of the laser six decades ago 1-8 . A suitable physical mechanism that allows single-mode lasing irrespective of the cavity size-a 'scale invariant' cavity or laser-has not been identified yet. Here we propose and demonstrate experimentally that open-Dirac electromagnetic cavities with linear dispersion-which in our devices are realized by a truncated photonic crystal arranged in a hexagonal pattern-exhibit unconventional scaling of losses in reciprocal space, leading to single-mode lasing that is maintained as the cavity is scaled up in size. The physical origin of this phenomenon lies in the convergence of the complex part of the free spectral range in open-Dirac cavities towards a constant governed by the loss rates of distinct Bloch bands, whereas for common cavities it converges to zero as the size grows, leading to inevitable multimode emission. An unconventional flat-envelope fundamental mode locks all unit cells in the cavity in phase, leading to single-mode lasing. We name such sources Berkeley surface-emitting lasers (BerkSELs) and demonstrate that their far-field corresponds to a topological singularity of charge two, in agreement with our theory. Open-Dirac cavities unlock avenues for light-matter interaction and cavity quantum electrodynamics., (© 2022. The Author(s), under exclusive licence to Springer Nature Limited.)

Resonant scattering, guided mode propagation phase, and/or orientation-dependent phase retardations are the three main mechanisms used to date to conceive optical metasurfaces. Here, we introduce an additional degree of freedom to address optical phase engineering by exploiting the topological features of non-Hermitian matrices operating near their singular points. Choosing metasurface building blocks to encircle a singularity following an arbitrarily closed trajectory in parameter space, we engineered a topologically protected full 2π-phase on a specific reflected polarization channel. The ease of implementation together with its compatibility with other phase-addressing mechanisms bring topological properties into the realm of industrial applications at optical frequencies and prove that metasurface technology represents a convenient test bench to study and validate topological photonic concepts.

Topology plays a fundamental role in contemporary physics and enables new information processing schemes and wave device physics with built-in robustness. However, the creation of photonic topological phases usually requires complex geometries that limit the prospect for miniaturization and integration and dispossess designers of additional degrees of freedom needed to control topological modes on-chip. By controlling the degree of asymmetry (DoA) in a photonic crystal with broken inversion symmetry, we report single-mode lasing of valley-Hall ring cavities at telecommunication wavelength. The DoA governs four photon confinement regimes at the interface of topologically distinct valley-Hall domains and evidences an interplay between the width of the topological bandgap and the quality factor of ring-like modes for single-mode operation. Our results open the door to novel optoelectronic devices and systems based on compact topological integrated circuits.

In this Letter, we present a design strategy for the realization of electrically powered bound states in the continuum (BIC) lasers. Despite growing attention of the optics community for BICs, practical uses of BICs in an active device are still unestablished. A large index contrast and out-of-plane symmetries that aid the formation of BICs are not trivial to achieve using conventional approaches for semiconductor laser design. Here, we propose a doping scheme to circumvent this issue. We also show that the introduction of material absorption due to carriers deteriorates the quality factor of BIC modes and show that a suitable compromise between electrical conductivity and optical loss can be achieved.

Planar structured interfaces, also known as metasurfaces, are continuously attracting interest owing to their ability to manipulate fundamental attributes of light, including angular momentum, phase, or polarization. However, chromatic aberration, limiting broadband operation, has remained a challenge for metasurfaces-based optical components and imagers. The limitation stems from the intrinsic dispersion of existing materials and design principles. Here we report and experimentally demonstrate polarization-independent fishnet-achromatic-metalenses with measured average efficiencies over 70% in the continuous band from the visible (640 nm) to the infrared (1200 nm). Results of the scalable platform are enabling for applications requiring broad bandwidth and high efficiency including energy harvesting, virtual reality and information processing devices, or medical imaging.

We experimentally demonstrate the lasing action of a new nanolaser design with a tunnel junction. By using a heavily doped tunnel junction for hole injection, we can replace the p-type contact material of a conventional nanolaser diode with a low-resistance n-type contact layer. This leads to a significant reduction of the device resistance and lowers the threshold voltage from 5 V to around 0.95 V at 77 K. The lasing behavior is verified by the light output versus the injection current (L-I) characterization and second-order coherence function measurements. Because of less Joule heating during current injection, the nanolaser can be operated at temperatures as high as 180 K under CW pumping. The incorporation of heavily doped tunnel junctions may pave the way for other nanoscale cavity design for improved heat management.

In the past few years, carpet cloaking has attracted interest because of its feasibility at optical frequencies and potential in stealth technologies. Metasurfaces have been proposed as a method to engineer ultra-thin carpet cloaking surfaces due to their abilities to manipulate wavefronts, polarization, and phase at subwavelength scale. However, achieving broadband carpet cloaking with a significant bandwidth is one of the key remaining challenges for metasurface designs. To date, broadband carpet cloaking based on metasurfaces has not been achieved, and operation has been limited to discrete wavelengths. Here, we propose and numerically demonstrate a novel metasurface design for broadband carpet cloaking with linear polarization at visible wavelengths from 650 nm to 800 nm. Our proposed method is a promising approach for broadband structured interfaces.

Random media introduce large degrees of freedom in device design and can thus address challenges in manipulating optical waves. Wave shaping with metasurfaces has mainly utilized periodic or quasi-periodic grids, and the potential of random arrangement of particles for devices has only come under investigation recently. The main difficulty in pursuing random metasurfaces is the identification of the degrees of freedom that optimize their efficiencies and functions. They can also encode information using the statistics of particle distribution. We propose a phase-map that accounts for the statistical nature of random media. The method takes into account effects of random near-field couplings that introduce phase errors by affecting the phase shift of elements. The proposed approach increases the efficiency of our random metasurface devices by up to ∼20%. This work paves the way toward the efficient design of random metasurfaces with potential applications in highly secure optical cryptography and information encoding.

Metasurfaces are generally designed by placing scatterers in periodic or pseudo-periodic grids. We propose and discuss design rules for functional metasurfaces with randomly placed anisotropic elements that randomly sample a well-defined phase function. By analyzing the focusing performance of random metasurface lenses as a function of their density and the density of the phase-maps used to design them, we find that the performance of 1D metasurfaces is mostly governed by their density while 2D metasurfaces strongly depend on both the density and the near-field coupling configuration of the surface. The proposed approach is used to design all-polarization random metalenses at near infrared frequencies. Challenges, as well as opportunities of random metasurfaces compared to periodic ones are discussed. Our results pave the way to new approaches in the design of nanophotonic structures and devices from lenses to solar energy concentrators.

Resonant cavities are essential building blocks governing many wave-based phenomena, but their geometry and reciprocity fundamentally limit the integration of optical devices. We report, at telecommunication wavelengths, geometry-independent and integrated nonreciprocal topological cavities that couple stimulated emission from one-way photonic edge states to a selected waveguide output with an isolation ratio in excess of 10 decibels. Nonreciprocity originates from unidirectional edge states at the boundary between photonic structures with distinct topological invariants. Our experimental demonstration of lasing from topological cavities provides the opportunity to develop complex topological circuitry of arbitrary geometries for the integrated and robust generation and transport of photons in classical and quantum regimes., (Copyright © 2017 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works.)

Metasurfaces have attracted significant attention due to their novel designs for flat optics. However, the approach usually used to engineer metasurface devices assumes that neighboring elements are identical, by extracting the phase information from simulations with periodic boundaries, or that near-field coupling between particles is negligible, by extracting the phase from single particle simulations. This is not the case most of the time and the approach thus prevents the optimization of devices that operate away from their optimum. Here, we propose a versatile numerical method to obtain the phase of each element within the metasurface (meta-atoms) while accounting for near-field coupling. Quantifying the phase error of each element of the metasurfaces with the proposed local phase method paves the way to the design of highly efficient metasurface devices including, but not limited to, deflectors, high numerical aperture metasurface concentrators, lenses, cloaks, and modulators.

Plasmonic/metamaterial sensors are being investigated for their high sensitivity, fast response time, and high accuracy. We propose, characterize and experimentally realize subwavelength bilayer metamaterial sensors operating in the near-infrared domain. We measure the figure-of-merit (FOM) and the bulk sensitivity (S) of the two fundamental hybridized modes and demonstrate both numerically and experimentally that the magnetic dipolar mode, degenerate with the electric quadrupolar mode, has higher sensitivity to a variation of the refractive index compared to the electric dipolar mode. In addition, the hybridized system exhibits a four fold increase in the FOM compared to a standard dipolar plasmonic system.

Metasurfaces are promising tools toward novel designs for flat optics applications. As such, their quality and tolerance to fabrication imperfections need to be evaluated with specific tools. However, most such tools rely on the geometrical optics approximation and are not straightforwardly applicable to metasurfaces. In this Letter, we introduce and evaluate for metasurfaces parameters such as intercept factor and slope error usually defined for solar concentrators in the realm of ray-optics. After proposing definitions valid in physical optics, we put forward an approach to calculate them. As examples, we design three different concentrators based on three specific unit cells and assess them numerically. The concept allows for comparison of the efficiency of the metasurfaces and their sensitivities to fabrication imperfections and will be critical for practical systems implementation.

In 1929, only three years after the advent of quantum mechanics, von Neumann and Wigner showed that Schrödinger's equation can have bound states above the continuum threshold. These peculiar states, called bound states in the continuum (BICs), manifest themselves as resonances that do not decay. For several decades afterwards the idea lay dormant, regarded primarily as a mathematical curiosity. In 1977, Herrick and Stillinger revived interest in BICs when they suggested that BICs could be observed in semiconductor superlattices. BICs arise naturally from Feshbach's quantum mechanical theory of resonances, as explained by Friedrich and Wintgen, and are thus more physical than initially realized. Recently, it was realized that BICs are intrinsically a wave phenomenon and are thus not restricted to the realm of quantum mechanics. They have since been shown to occur in many different fields of wave physics including acoustics, microwaves and nanophotonics. However, experimental observations of BICs have been limited to passive systems and the realization of BIC lasers has remained elusive. Here we report, at room temperature, lasing action from an optically pumped BIC cavity. Our results show that the lasing wavelength of the fabricated BIC cavities, each made of an array of cylindrical nanoresonators suspended in air, scales with the radii of the nanoresonators according to the theoretical prediction for the BIC mode. Moreover, lasing action from the designed BIC cavity persists even after scaling down the array to as few as 8-by-8 nanoresonators. BIC lasers open up new avenues in the study of light-matter interaction because they are intrinsically connected to topological charges and represent natural vector beam sources (that is, there are several possible beam shapes), which are highly sought after in the fields of optical trapping, biological sensing and quantum information.

Using numerical simulations, we demonstrate that the dipolar plasmonic resonance of a single metallic nanoparticle inserted in the core of a dielectric waveguide can be excited with higher order photonic modes of the waveguide only if their symmetry is compatible with the charge distribution of the plasmonic mode. For the case of a symmetric waveguide, we demonstrate that this condition is only achieved if the particle is shifted from the center of the core. The simple and comprehensive analysis presented in this contribution will serve as basis for applications in integrated nanophotonic/metamaterials devices, such as optical filters, modulators and mode converters.

Accurate and robust characterization of metasurfaces and metamaterials in terms of effective parameters is critical to the design of novel metadevices. We compute the Cramér-Rao lower bounds on the variance of any estimator for both the electric and magnetic surface susceptibilities of metasurfaces. We show that retrieval of such effective properties is inherently difficult around resonances, most notably for low-loss metasurfaces. We also put forth a least-squares estimator to mitigate this difficulty for the normal components of susceptibility tensors, which are observed to be the most ill-behaved. The present work is relevant to the development of loss-compensated metasurfaces for which noise has to be closely considered for accurate and robust device characterization.

We present a method for studying amplification of electromagnetic modes in active, circularly symmetric waveguides with hyperbolic dispersion. Using this method, we obtain a closed-form expression for the modal threshold condition. We find that modal amplification is possible in a region of the radius-wavelength phase-space with small enough radius so that propagation of the mode is permitted while modal energy and phase counter-propagate. At telecommunication frequencies, such a situation is achievable only when the absolute value of the real metal permittivity exceeds that of the active dielectric. We validate our theoretical conclusions with numerical simulations that explain the threshold condition in terms of an energy balance between the longitudinal and radial components of the electric field.