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Crystals spontaneously break the continuous translation symmetry in space, despite the invariance of the underlying energy function. This has triggered suggestions of time crystals analogously lifting translational invariance in time. Originally suggested for closed thermodynamic systems in equilibrium, no-go theorems prevent the existence of time crystals. Proposals for open systems out of equilibrium led to the observation of discrete time crystals subject to external periodic driving to which they respond with a sub-harmonic response. A continuous time crystal is an autonomous system that develops periodic auto-oscillations when exposed to a continuous, time-independent driving, as recently demonstrated for the density in an atomic Bose-Einstein condensate with a crystal lifetime of a few ms. Here we demonstrate an ultra-robust continuous time crystal in the nonlinear electron-nuclear spin system of a tailored semiconductor with a coherence time exceeding hours. Varying the experimental parameters reveals huge stability ranges of this time crystal, but allows one also to enter chaotic regimes, where aperiodic behavior appears corresponding to melting of the crystal. This novel phase of matter opens the possibility to study systems with nonlinear interactions in an unprecedented way., Comment: 12 figures, 17 pages

We discuss the implications of a small indium content (3%) in a GaAs epilayer on the electron- and nuclear-spin relaxation due to enhanced quadrupolar effects induced by the strain. Using the weakly perturbative spin-noise spectroscopy, we study the electron-spin relaxation dynamics without explicit excitation. The observed temperature dependence indicates the presence of localized states, which have an increased interaction with the surrounding nuclear spins. Time-resolved spin-noise spectroscopy is then applied to study the relaxation dynamics of the optically pumped nuclear-spin system. It shows a multi-exponential decay with time components, ranging from several seconds to hundreds of seconds. Further, we provide a measurement of the local magnetic field acting between the nuclear spins and discover a strong contribution of quadrupole effects. Finally, we apply the nuclear spin diffusion model, that allows us to estimate the concentration of the localized carrier states and to determine the nuclear spin diffusion constant characteristic for this system., Comment: 13 pages, 9 figures

The ability to extend the time scale of the coherent optical response from large ensembles of quantum emitters is highly appealing for applications in quantum information devices. In semiconductor nanostructures, spin degrees of freedom can be used as auxiliary, powerful tools to modify the coherent optical dynamics. Here, we apply this approach to negatively charged (In,Ga)As/GaAs self-assembled quantum dots which are considered as excellent quantum emitters with robust optical coherence and high bandwidth. We study 3-pulse spin-dependent photon echoes subject to moderate transverse magnetic fields up to 1 T. We demonstrate that the timescale of coherent optical response can be extended by at least an order of magnitude by the field. Without magnetic field, the photon echo decays with $T_ 2$ = 0.45 ns which is determined by the radiative lifetime of trions $T_1$ = 0.27 ns. In the presence of the transverse magnetic field, the decay of the photon echo signal is given by spin dephasing time of the ensemble of resident electrons $T_{2,e}$ ~ 4 ns. We demonstrate that the non-zero transverse g-factor of the heavy holes in the trion state plays a crucial role in the temporal evolution and magnetic field dependence of the long-lived photon echo signal., Comment: 9 pages, 4 figures, Supplementary material

The spin-noise spectroscopy (SNS) method implies high efficiency of conversion of the spin-system magnetization to the Faraday rotation angle. Generally, this efficiency cannot be estimated using the characteristics of the regular magneto-optical activity of a paramagnet. However, it may be drastically enhanced in systems with strong inhomogeneous broadening of the optical transitions. This enhancement leads to the giant spin-noise gain effect and previously allowed one to apply the SNS to rare-earth-activated crystals. We show that the nonlinear resonant Faraday effect can be used to measure the homogeneous width of the inhomogeneously broadened transition and, thus, to estimate the applicability of the SNS to this type of paramagnet. We present the theoretical description of the effect and perform measurements on intraconfigurational ($4f$-$4f$) transitions of the trivalent rare-earth ions of neodymium and ytterbium in fluorite-based crystals. The proposed experimental approach establishes new links between the effects of nonlinear optics and spin-noise characteristics of crystals with paramagnetic impurities and offers new ways of research in the physics of impurity crystals., Comment: 9 pages, 7 figures, 1 table

We show that in cubic crystals with anisotropic impurity centers the sum of squares of the magnetic resonance (EPR) frequencies is invariant with respect to the magnetic field direction. The connection between such an invariant and the g-tensor components of the impurity is derived for different types of centers. The established regularity is confirmed experimentally for the spin-noise spectra of a CaF2-Nd3+ crystal. We show how this property of the EPR spectra can be efficiently used for the assignment of paramagnetic centers in cubic crystals., Comment: 5 pages, 2 figures

To broaden the scope of van der Waals 2D magnets, we report the synthesis and magnetism of covalent 2D magnetic Cr$_2$Te$_3$ with a thickness down to one-unit-cell. The 2D Cr$_2$Te$_3$ crystals exhibit robust ferromagnetism with a Curie temperature of 180 K, a large perpendicular anisotropy of 7*105 J m-3, and a high coercivity of ~ 4.6 kG at 20 K. First-principles calculations further show a transition from canted to collinear ferromagnetism, a transition from perpendicular to in-plane anisotropy, and emergent half-metallic behavior in atomically-thin Cr$_2$Te$_3$, suggesting its potential application for injecting carriers with high spin polarization into spintronic devices.

Spin noise spectroscopy is a method of magnetic resonance widely used, nowadays, in atomic and semiconductor research. Classical objects of the EPR spectroscopy - dielectrics with paramagnetic impurities - seemed to be unsuitable for this technique because of large widths of allowed optical transitions and, therefore, low specific Faraday rotation (FR). We show, however, that the FR noise detected at the wavelength of a weak optical transition (with low regular FR) may increase by many orders of magnitude as its homogeneous width decreases. This spin-noise gain effect, numerically described by the ratio of the inhomogeneous linewidth to homogeneous, relates primarily to forbidden intraconfigurational transitions of impurity ions with unfilled inner electronic shells. Specifically, for the f-f transitions of rare-earth ions in crystals, this factor may reach 10$^8$. In this paper, we report on the first successful application of spin noise spectroscopy for detecting magnetic resonance of rare-earth ions in crystals., Comment: 5 pages, 3 figures

Fundamental properties of the spin-noise signal formation in a quantum-dot microcavity are studied by measuring the angular characteristics of the scattered light intensity. A distributed Bragg reflector microcavity was used to enhance the light-matter interaction with an ensemble of n-doped (In,Ga)As/GaAs quantum dots, which allowed us to study subtle effects of the noise signal formation. Detecting the scattered light outside of the aperture of the transmitted light, we measured the basic electron spin properties, like g-factor and spin dephasing time. Further, we investigated the influence of the microcavity on the scattering distribution and possibilities of signal amplification by additional resonant excitation., Comment: 5 pages, 4 figures

In the spin noise spectroscopy, the magnetic susceptibility spectrum is known to be provided by the spin-system untouched by any external perturbation, or, better to say, disturbed only by its thermal bath. We propose a new version of the spin noise spectroscopy, with the detected magnetization (Faraday-rotation) noise being stimulated by an external fluctuating magnetic field with a quasi-white spectrum. Experimental study of the stimulated spin noise performed on a $\text{BaF}_2 : \text{U}^{3+}$ crystal in a longitudinal magnetic field has revealed specific features of this approach and allowed us to identify the Van-Vleck and population-related contributions to the AC susceptibility of the system and to discover unusual magnetic-field dependence of the longitudinal spin relaxation rate in low magnetic fields. It is shown that spectra of the stimulated and spontaneous spin noise, being both closely related to the spin-system magnetic susceptibility, are still essentially different. Distinctions between the two types of the spin-noise spectra and two approaches to the spin noise spectroscopy are discussed., Comment: 6 pages, 6 figures

We implement the homodyne detection scheme for an increase of the polarimetric sensitivity in spin noise spectroscopy. Controlling the laser intensity of the local oscillator, which is guided around the sample and does not perturb the measured spin system, we are able to improve the signal-to-noise ratio. The opportunity of additional amplification of the measured signal strength allows us to reduce the probe laser intensity incident onto the sample and therefore to approach the non-perturbative regime. The efficiency of this scheme with signal enhancement by more than a factor of 3 at low probe powers is demonstrated on bulk $n$-doped GaAs where the reduced electron-spin relaxation rate is shown experimentally. Additionally, the control of the optical phase provides us with the possibility to switch between the measurement of Faraday rotation and ellipticity without changes in the optical setup., Comment: 9 pages, 4 figures, Minor revisions, New References