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A bismuth-doped silicon substrate was analyzed by using a magnetometer based on a superconducting flux qubit. The temperature dependence of the magnetization indicates that the silicon substrate contains at least two signal sources, intentionally doped bismuth spins and a spin 1/2 system with a ratio of 0.873 to 0.127. In combination with a conventional electron spin resonance spectrometer, a candidate origin of the spin 1/2 system was identified as a dangling bond on the silicon surface. In addition, the spin sensitivity of the magnetometer was also estimated to be 12 spins/$\sqrt{\mathrm{Hz}}$ by using optimized dispersive readout.

We report experimental and theoretical results on the extremely large Lamb shift in a multimode circuit quantum electrodynamics (QED) system in the deep-strong coupling (DSC) regime, where the qubit-resonator coupling strength is comparable to or larger than the qubit and resonator frequencies. The system comprises a superconducting flux qubit (FQ) and a quarter-wavelength coplanar waveguide resonator ($\lambda/4$ CPWR) that are coupled inductively through a shared edge that contains a Josephson junction to achieve the DSC regime. Spectroscopy is performed around the frequency of the fundamental mode of the CPWR, and the spectrum is fitted by the single-mode quantum Rabi Hamiltonian to obtain the system parameters. Since the qubit is also coupled to a large number of higher modes in the resonator, the single-mode fitting does not provide the bare qubit energy but a value that incorporates the renormalization from all the other modes. We derive theoretical formulas for the Lamb shift in the multimode resonator system. As shown in previous studies, there is a cut-off frequency $\omega_{\rm{cutoff}}$ for the coupling between the FQ and the modes in the CPWR, where the coupling grows as $\sqrt{\omega_n}$ for $\omega_n/\omega_{\rm{cutoff}}\ll 1$ and decreases as $1/\sqrt{\omega_n}$ for $\omega_n/\omega_{\rm{cutoff}}\gg 1$. Here $\omega_n$ is the frequency of the $n$th mode. The cut-off effect occurs because the qubit acts as an obstacle for the current in the resonator, which suppresses the current of the modes above $\omega_{\rm{cutoff}}$ at the location of the qubit and results in a reduced coupling strength. Using our observed spectrum and theoretical formulas, we estimate that the Lamb shift from the fundamental mode is 82.3\% and the total Lamb shift from all the modes is 96.5\%., Comment: 16 pages, 4 figures

We demonstrate magnetometry of cultured neurons on a polymeric film using a superconducting flux qubit that works as a sensitive magnetometer in a microscale area. The neurons are cultured in Fe$^{3+}$ rich medium to increase magnetization signal generated by the electron spins originating from the ions. The magnetometry is performed by insulating the qubit device from the laden neurons with the polymeric film while keeping the distance between them around several micrometers. By changing temperature (12.5 - 200 mK) and a magnetic field (2.5 - 12.5 mT), we observe a clear magnetization signal from the neurons that is well above the control magnetometry of the polymeric film itself. From electron spin resonance (ESR) spectrum measured at 10 K, the magnetization signal is identified to originate from electron spins of iron ions in neurons. This technique to detect a bio-spin system can be extended to achieve ESR spectroscopy at the single-cell level, which will give the spectroscopic fingerprint of cells.

Parasitic two-level-system (TLS) defects are one of the major factors limiting the coherence times of superconducting qubits. Although there has been significant progress in characterizing basic parameters of TLS defects, exact mechanisms of interactions between a qubit and various types of TLS defects remained largely unexplored due to the lack of experimental techniques able to probe the form of qubit-defect couplings. Here we present an experimental method of TLS defect spectroscopy using a strong qubit drive that allowed us to distinguish between various types of qubit-defect interactions. By applying this method to a capacitively shunted flux qubit, we detected a rare type of TLS defect with a nonlinear qubit-defect coupling due to critical-current fluctuations, as well as conventional TLS defects with a linear coupling to the qubit caused by charge fluctuations. The presented approach could become the routine method for high-frequency defect inspection and quality control in superconducting qubit fabrication, providing essential feedback for fabrication process optimization. The reported method is a powerful tool to uniquely identify the type of noise fluctuations caused by TLS defects, enabling the development of realistic noise models relevant to noisy intermediate-scale quantum (NISQ) computing and fault-tolerant quantum control., Comment: revised version

It is widely known that spin-locking noise-spectroscopy is a powerful technique for the characterization of low-frequency noise mechanisms in superconducting qubits. Here we show that the relaxation rate of the driven spin-locking state of a qubit can be significantly affected by the presence of an off-resonant high-frequency two-level-system defect. Thus, both low- and high-frequency defects should be taken into account in the interpretation of spin-locking measurements and other types of driven-state noise-spectroscopy., Comment: main text (6 pages, 3 figures) + supplemental material (8 pages, 9 figures)

We control transition frequency of a superconducting flux qubit coupled to a frequency-tunable resonator comprising a direct current superconducting quantum interference device (dc-SQUID) by microwave driving. The dc-SQUID mediates the coupling between microwave photons in the resonator and a flux qubit. The polarity of the frequency shift depends on the sign of the flux bias for the qubit and can be both positive and negative. The absolute value of the frequency shift becomes larger by increasing the photon number in the resonator. These behaviors are reproduced by a model considering the magnetic interaction between the flux qubit and dc-SQUID. The tuning range of the transition frequency of the flux qubit reaches $\approx$ 1.9 GHz, which is much larger than the ac Stark/Lamb shift observed in the dispersive regime using typical circuit quantum electrodynamics devices., Comment: 5 pages, 4 figures

We report on electron spin resonance spectroscopy measurements using a superconducting flux qubit with a sensing volume of 6 fl. The qubit is read out using a frequency-tunable Josephson bifurcation amplifier, which leads to an inferred measurement sensitivity of about 20 spins in a 1 s measurement. This sensitivity represents an order of magnitude improvement when compared with flux-qubit schemes using a dc-SQUID switching readout. Furthermore, noise spectroscopy reveals that the sensitivity is limited by flicker ($1/f$) flux noise., Comment: 4 pages, 4 figures

We theoretically analyze the performance of the nuclear magnetic resonance (NMR) spectroscopy with a superconducting flux qubit (FQ). Such NMR with the FQ is attractive because of the possibility to detect the relatively small number of nuclear spins in a local region ($\sim\mu$m) with low temperatures ($\sim$ mK) and low magnetic fields ($\sim$ mT), in which other types of quantum sensing schemes cannot easily access. A sample containing nuclear spins is directly attached on the FQ, and the FQ is used as a magnetometer to detect magnetic fields from the nuclear spins. Especially, we consider two types of approaches to NMR with the FQ. One of them is to use spatially inhomogeneous excitations of the nuclear spins, which are induced by a spatially asymmetric driving with radio frequency~(RF) pulses. Such an inhomogeneity causes a change in the DC magnetic flux penetrating a loop of the FQ, which can be detected by a standard Ramsey measurement on the FQ. The other approach is to use a dynamical decoupling on the FQ to measure AC magnetic fields induced by Larmor precession of the nuclear spins. In this case, neither a spin excitation nor a spin polarization is required since the signal comes from fluctuating magnetic fields of the nuclear spins. We calculate the minimum detectable density (number) of the nuclear spins for the FQ with experimentally feasible parameters. We show that the minimum detectable density (number) of the nuclear spins with these approaches is around $10^{21}$ /cm$^3$ ($10^8$) with an accumulation time of a second., Comment: 13 pages, 11 figures

We report on experimentally measured light shifts of superconducting flux qubits deep-strongly coupled to LC oscillators, where the coupling constants are comparable to the qubit and oscillator resonance frequencies. By using two-tone spectroscopy, the energies of the six lowest levels of each circuit are determined. We find huge Lamb shifts that exceed 90% of the bare qubit frequencies and inversions of the qubits' ground and excited states when there are a finite number of photons in the oscillator. Our experimental results agree with theoretical predictions based on the quantum Rabi model., Comment: 19 pages, 7 figures, and 2 tables. Supplemental Material is included

Electron paramagnetic resonance (EPR) spectroscopy is an important technology in physics, chemistry, materials science, and biology. Sensitive detection with a small sample volume is a key objective in these areas, because it is crucial, for example, for the readout of a highly packed spin based quantum memory or the detection of unlabeled metalloproteins in a single cell. In conventional EPR spectrometers, the energy transfer from the spins to the cavity at a Purcell enhanced rate plays an essential role and requires the spins to be resonant with the cavity, however the size of the cavity (limited by the wavelength) makes it difficult to improve the spatial resolution. Here, we demonstrate a novel EPR spectrometer using a single artificial atom as a sensitive detector of spin magnetization. The artificial atom, a superconducting flux qubit, provides advantages both in terms of its quantum properties and its much stronger coupling with magnetic fields. We have achieved a sensitivity of $\sim$400 spins/$\sqrt{\mathrm{Hz}}$ with a magnetic sensing volume around $10^{-14} \lambda^3$ (50 femto-liters). This corresponds to an improvement of two-order of magnitude in the magnetic sensing volume compared with the best cavity based spectrometers while maintaining a similar sensitivity as those spectrometers . Our artificial atom is suitable for scaling down and thus paves the way for measuring single spins on the nanometer scale.

We performed magnetic field and frequency tunable electron paramagnetic resonance spectroscopy of an Er$^{3+}$ doped Y$_2$SiO$_5$ crystal by observing the change in flux induced on a direct current-superconducting quantum interference device (dc-SQUID) loop of a tunable Josephson bifurcation amplifer. The observed spectra show multiple transitions which agree well with the simulated energy levels, taking into account the hyperfine and quadrupole interactions of $^{167}$Er. The sensing volume is about 0.15 pl, and our inferred measurement sensitivity (limited by external flux noise) is approximately $1.5\times10^4$ electron spins for a 1 s measurement. The sensitivity value is two orders of magnitude better than similar schemes using dc-SQUID switching readout., Comment: Main text: 5 pages, 3 figures. Supplementary materials: 4 pages, 4 figures

An ensemble of nitrogen-vacancy (NV) centers in diamond is an attractive device to detect small magnetic fields. In particular, by exploiting the fact that the NV center can be aligned along one of four different axes due to symmetry, it is possible to extract information concerning vector magnetic fields. However, in the conventional scheme, low readout contrasts of the NV centers significantly decrease the sensitivity of the vector magnetic field sensing. Here, we propose a way to improve the sensitivity of the vector magnetic field sensing of the NV centers using multi-frequency control. Since the Zeeman energy of the NV centers depends on the direction of the axis, we can independently control the four types of NV centers using microwave pulses with different frequencies. This allows us to use every NV center for the vector field detection in parallel, which effectively increases the readout contrast. Our results pave the way to realize a practical diamond-based vector field sensor.

In the ultra-strong coupling regime of a light-matter system, the ground state exhibits non-trivial entanglement between the atom and photons. For the purposes of exploring the measurement and control of this ground state, here we analyze the dynamics of such an ultra-strongly-coupled system interacting with a driven nonlinear resonator acting as a measurement apparatus. Interestingly, although the coupling between the atom and the nonlinear resonator is much smaller than the typical energy scales of the ultra-strongly-coupled system, we show that we can generate a strong correlation between the nonlinear resonator and the light-matter system. A subsequent coarse- grained measurement on the nonlinear resonator significantly affects the light-matter system, and the phase of the light changes depending on the measurement results. Also, we investigate the conditions for when the nonlinear resonator can be entangled with the ultra-strongly coupled system, which is the mechanism that allows us to project the ground state of the ultra-strongly coupled system into a non-energy eigenstate., Comment: 10 pages, 11 figures

We report on spectra of circuit-quantum-electrodynamics (QED) systems in an intermediate regime that lies between the ultrastrong and deep-strong-coupling regimes, which have been reported previously in the literature. Our experimental results, along with numerical simulations, demonstrate that as the coupling strength increases, the spectrum of a circuit-QED system undergoes multiple qualitative transformations, such that several coupling regimes are identified, each with its own unique spectral features. The different spectral transformations can be related to crossings between energy level differences and to changes in the symmetries of the energy eigenstates. These results allow us to use qualitative spectral features to infer certain properties and parameters of the system., Comment: 7 figures

Superconducting flux qubits are a promising candidate for realizing quantum information processing and quantum simulations. Such devices behave like artificial atoms, with the advantage that one can easily tune the "atoms" internal properties. Here, by harnessing this flexibility, we propose a technique to minimize the inhomogeneous broadening of a large ensemble of flux qubits by tuning only the external flux. In addition, as an example of many-body physics in such an ensemble, we show how to observe superradiance, and its quadratic scaling with ensemble size, using a tailored microwave control pulse that takes advantage of the inhomogeneous broadening itself to excite only a sub-ensemble of the qubits. Our scheme opens up an approach to using superconducting circuits to explore the properties of quantum many-body systems.

The hybridization of distinct quantum systems is now seen as an effective way to engineer the properties of an entire system leading to applications in quantum metamaterials, quantum simulation, and quantum metrology. One well known example is superconducting circuits coupled to ensembles of microscopic natural atoms. In such cases, the properties of the individual atom are intrinsic, and so are unchangeable. However, current technology allows us to fabricate large ensembles of macroscopic artificial atoms such as superconducting flux qubits, where we can really tailor and control the properties of individual qubits. Here, we demonstrate coherent coupling between a microwave resonator and several thousand superconducting flux qubits, where we observe a large dispersive frequency shift in the spectrum of 250 MHz induced by collective behavior. These results represent the largest number of coupled superconducting qubits realized so far. Our approach shows that it is now possible to engineer the properties of the ensemble, opening up the way for the controlled exploration of the quantum many-body system.

The interaction between an atom and the electromagnetic field inside a cavity has played a crucial role in the historical development of our understanding of light-matter interaction and is a central part of various quantum technologies, such as lasers and many quantum computing architectures. The emergence of superconducting qubits has allowed the realization of strong and ultrastrong coupling between artificial atoms and cavities. If the coupling strength $g$ becomes as large as the atomic and cavity frequencies ($\Delta$ and $\omega_{\rm o}$ respectively), the energy eigenstates including the ground state are predicted to be highly entangled. This qualitatively new regime can be called the deep strong-coupling regime, and there has been an ongoing debate over whether it is fundamentally possible to realize this regime in realistic physical systems. By inductively coupling a flux qubit and an LC oscillator via Josephson junctions, we have realized circuits with $g/\omega_{\rm o}$ ranging from 0.72 to 1.34 and $g/\Delta\gg 1$. Using spectroscopy measurements, we have observed unconventional transition spectra, with patterns resembling masquerade masks, that are characteristic of this new regime. Our results provide a basis for ground-state-based entangled-pair generation and open a new direction of research on strongly correlated light-matter states in circuit-quantum electrodynamics., Comment: 3 figures, Methods, and Supplementary Information

Macroscopic realism is the name for a class of modifications to quantum theory that allow macroscopic objects to be described in a measurement-independent manner, while largely preserving a fully quantum mechanical description of the microscopic world. Objective collapse theories are examples which aim to solve the quantum measurement problem through modified dynamical laws. Whether such theories describe nature, however, is not known. Here we describe and implement an experimental protocol capable of constraining theories of this class, that is more noise tolerant and conceptually transparent than the original Leggett-Garg test. We implement the protocol in a superconducting flux qubit, and rule out (by ~84 s.d.) those theories which would deny coherent superpositions of 170 nA currents over a ~10 ns timescale. Further, we address the 'clumsiness loophole' by determining classical disturbance with control experiments. Our results constitute strong evidence for the superposition of states of nontrivial macroscopic distinctness., Comment: Published version; 5 + 12 pages

We demonstrate electron spin polarization detection and electron paramagnetic resonance (EPR) spectroscopy using a direct current superconducting quantum interference device (dc-SQUID) magnetometer. Our target electron spin ensemble is directly glued on the dc-SQUID magnetometer that detects electron spin polarization induced by a external magnetic field or EPR in micrometer-sized area. The minimum distinguishable number of polarized spins and sensing volume of the electron spin polarization detection and the EPR spectroscopy are estimated to be $\sim$$10^6$ and $\sim$$10^{-10}$ $\mathrm{cm}^{3}$ ($\sim$0.1 pl), respectively., Comment: 9 pages, 3 figures

Optically detected magnetic resonance (ODMR) is a way to characterize the NV centers. Recently, a remarkably sharp dip was observed in the ODMR with a high-density ensemble of NV centers, and this was reproduced by a theoretical model in [Zhu et al., Nature Communications 5, 3424 (2014)], showing that the dip is a consequence of the spin-1 properties of the NV centers. Here, we present much more details of analysis to show how this model can be applied to investigate the properties of the NV centers. By using our model, we have reproduced the ODMR with and without applied magnetic fields. Also, we theoretically investigate how the ODMR is affected by the typical parameters of the ensemble NV centers such as strain distributions, inhomogeneous magnetic fields, and homogeneous broadening width. Our model could provide a way to estimate these parameters from the ODMR, which would be crucial to realize diamond-based quantum information processing.

One of the promising systems to realize quantum computation is a hybrid system where a superconducting flux qubit plays a role of a quantum processor and the NV center ensemble is used as a quantum memory. We have theoretically and experimentally studied the effect of magnetic fields on this hybrid system, and found that the lifetime of the vacuum Rabi oscillation is improved by applying a few mT magnetic field to the NV center ensemble. Here, we construct a theoretical model to reproduce the vacuum Rabi oscillations with/without magnetic fields applied to the NV centers, and we determine the reason why magnetic fields can affect the coherent properties of the NV center ensemble. From our theoretical analysis, we quantitatively show that the magnetic fields actually suppress the inhomogeneous broadening from the strain in the NV centers.

Here, we propose a scheme to generate a controllable Ising interaction between superconducting flux qubits. Existing schemes rely on inducting couplings to realize Ising interactions between flux qubits, and the interaction strength is controlled by an applied magnetic field On the other hand, we have found a way to generate an interaction between the flux qubits via capacitive couplings. This has an advantage in individual addressability, because we can control the interaction strength by changing an applied voltage that can be easily localized. This is a crucial step toward the realizing superconducting flux qubit quantum computation., Comment: 10 pages, 15 figures

Here, we propose a way to control the interaction between qubits with always-on Ising interaction. Unlike the standard method to change the interaction strength with unitary operations, we fully make use of non-unitary properties of projective measurements so that we can effectively turn the interaction on or off via feedforward. Our scheme is useful to generate two- or three-dimensional cluster states that are universal resources for fault-tolerant quantum computation with this scheme, and it provides an alternative way to realize a scalable quantum pro, Comment: 7 pages, 2 figures

Here, we propose a counter-intuitive use of a hybrid system where the coherence time of a quantum system is actually improved via a coupling with an unstable system. If we couple a two-level system with a single NV center, then a dark state of the NV center naturally forms after the hybridization. We show that this dark state becomes robust against environmental fluctuations due to the coupling even when the coherence time of the two-level system is much shorter than that of the NV center. Our proposal opens a new way to use a quantum hybrid system for the realization of robust quantum information processing

We have built a hybrid system composed of a superconducting flux qubit (the processor) and an ensemble of nitrogen-vacancy centers in diamond (the memory) that can be directly coupled to one another and demonstrated how information can be transferred from the flux qubit to the memory, stored and subsequently retrieved. We have established the coherence properties of the memory, and succeeded in creating an entangled state between the processor and memory, demonstrating how the entangled state's coherence is preserved. Our results are a significant step towards using an electron spin ensemble as a quantum memory for superconducting qubits., Comment: 5 pages, 3 figures

Electron-spin nitrogen-vacancy color centers in diamond are a natural candidate to act as a quantum memory for superconducting qubits because of their large collective coupling and long coherence times. We report here the first demonstration of strong coupling and coherent exchange of a single quantum of energy between a flux-qubit and an ensemble of nitrogen-vacancy color centers., Comment: 5 pages, 4 figures, already published in the 13th October 2011 issue of Nature journal

Detailed schemes are investigated for experimental verification of Quantum Zeno effect with a superconducting qubit. A superconducting qubit is affected by a dephasing noise whose spectrum is 1/f, and so the decay process of a superconducting qubit shows a naturally non-exponential behavior due to an infinite correlation time of 1/f noise. Since projective measurements can easily influence the decay dynamics having such non-exponential feature, a superconducting qubit is a promising system to observe Quantum Zeno effect. We have studied how a sequence of projective measurements can change the dephasing process and also we have suggested experimental ways to observe Quantum Zeno effect with a superconducting qubit. It would be possible to demonstrate our prediction in the current technology.