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Flexible transparent electrodes, encompassing the combination of optical transparency and electrical conductivity, empower numerous optoelectronic applications. While the main efforts nowadays concentrate on developing wire meshes and conductive oxides, those technologies are still in a quest to find a balance between price, performance, and versatility. Here we propose a new platform, encompassing the advantages of nanophotonic design and roll-to-roll large-scale lithography fabrication tools, granting an ultimate balance between optical, electrical, and mechanical properties. The design is based on an array of silica microspheres deposited on a patterned thin aluminum film attached to a flexible polymer matrix. Microspheres are designed to squeeze 80% light through nanoscale apertures with the aid of the photonic nanojet effect given the light impinges the structure from the top. The photonic structure blocks the transmission for the backpropagation direction thus granting the device with the high 5-fold level of asymmetry. The patterned layer demonstrates a remarkable 2.8 {\Omega}/sq sheet resistance comparable to that of a continuous metal layer. The high conductivity is shown to be maintained after a repeatable application of strain on the flexible electrode. The technical specifications of the demonstrated transparent electrode establish it as a viable option for integrating into advanced optoelectronic devices such as solar cells, touchscreens, and organic light-emitting diodes to name a few. Its notable capacity to optimize light transmittance while ensuring consistent electrical performance, alongside its mechanical flexibility, makes the demonstrated device an essential component for applications, where such attributes are critically required., Comment: 16 pages, 5 pages, 1 table

Structured environment controls dynamics of light-matter interaction processes via modified local density of electromagnetic states. In typical scenarios, where nanosecond-scale fluorescent processes are involved, mechanical conformational changes of the environment during the interaction processes can be safely neglected. However, slow decaying phosphorescent complexes (e.g. lanthanides) can efficiently sense micro- and millisecond scale motion via near-field interactions. As the result, lifetime statistics can inherit information about nano-scale mechanical motion. Here we study light-matter interaction dynamics of phosphorescent dyes, diffusing in a proximity of a plasmonic nanoantenna. The interplay between the time-varying Purcell enhancement and stochastic motion of molecules is considered via a modified diffusion equation, and collective decay phenomena is analysed. Fluid properties, such as local temperature and diffusion coefficient are mapped on phosphorescent lifetime distribution extracted with the help of inverse Laplace transform. We present rather simple photonic platform enabling contactless all-optical thermometry and diffusion measurement and paving a way for a plethora of possible applications. Among them, the proposed analysis can be used for detailed studies of nanofluidic processes in lab-on-a-chip devices, which are extremely hard or even impossible to analyse with other optical methods., Comment: 12 pages, 4 figures

Light-matter interaction dynamics is governed by the strength of local coupling constants, tailored by surrounding electromagnetic structures. Characteristic decay times in dipole-allowed fluorescent transitions are much faster than mechanical conformational changes within an environment and, as the result, the latter can be assumed static during the emission process. However, slow-decaying compounds can break this commonly accepted approximation and introduce new interaction regimes. Here, slow decaying phosphorescent compounds are proposed to perform quantum sensing of nearby structure's motion via observation of collective velocity-dependent lifetime distributions. In particular, characteristic decay of an excited dye molecule, being comparable with its passage time next to a resonant particle, is modified via time-dependent Purcell enhancement, which leaves distinct signatures on properties of emitted light. Velocity mapping of uniformly moving particles within a fluid solution of phosphorescent dyes was demonstrated via analysis of modified lifetime distributions. The proposed interaction regime enables performing studies of a wide range of phenomena, where time-dependent light-matter interaction constants can be utilized for extraction of additional information about a process, Comment: 15 pages, 4 figures

Light-matter interaction processes are significantly affected by surrounding electromagnetic environment. Dielectric materials are usually introduced into an interaction picture via their classical properties, e.g. permittivity, appearing in constitutive relations. While this approach was proven to be applicable in many occasions, it might face limitations when an emitter is situated very close to a material boundary. In this case nonlocal extend of a quantum wave function of an emitter becomes comparable with a distance to a boundary and a lattice constant of a material. Here a semi-classical model, taking into account material's granularity, is developed. In particular, spontaneous emission process in the vicinity of flat boundaries is considered. The material boundary is divided into a pair areas - far zone is modeled as a continuous phase, while the near zone next to a nonlocal emitter is represented with a discrete array of polarizable particles. This array resembles optical properties of the continuous phase under the standard homogenization procedure. Local field effects were shown to lead orders of magnitude corrections to spontaneous emission rates in the case of sub-nanometer emitter-surface separation distances. The developed mesoscopic model enables addressing few aspects of local field corrections in quite complex scenarios, where quantum ab initio techniques yet face challenges owing to involved computational complexity. The developed method could be utilized for designs of quantum sources and networks, enhanced with structured electromagnetic environment., Comment: 15 pages, 5 figures

Quality of spatial separation between electric and magnetic fields in an electromagnetic wave is fundamentally constrained by nonlocal nature of Maxwell equations. While electric and magnetic energy densities in a wave, propagating in vacuum, are equal at each point in space, carefully designed photonic structures can enable surpassing this limit. Here, a set of high index dielectric tubes was for the first time proposed and theoretically and experimentally demonstrated to deliver a record high spatial separation, overcoming the free space scenario by more than three orders of magnitude with simultaneous enhancement of the magnetic field. Separation effect in the proposed structure is enabled by the near-field interference on anapole-like states, designed by tuning geometrical parameters of coupled dielectric tubes. The void layout of the structure enables the direct observation of the effect with near-field probes and could be further employed for relevant applications. Novel devices, providing tunable high quality separation between electric and magnetic fields, are extremely important for metrology, spectroscopy, spintronics, and opto-electronic applications., Comment: 19 pages, 5 figures