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When multiple neutrons are emitted in a fission event they are correlated in both energy and their relative angle, which may impact the design of safeguards equipment and other instrumentation for non-proliferation applications. The most recent release of MCNP 6 . 2 contains the capability to simulate correlated fission neutrons using the event generators CGMF and FREYA . These radiation transport simulations will be post-processed by the detector response code, DRiFT , and compared directly to correlated fission measurements. DRiFT has been previously compared to single detector measurements, its capabilities have been recently expanded with correlated fission simulations in mind. This paper details updates to DRiFT specific to correlated fission measurements, including tracking source particle energy of all detector events (and non-events), expanded output formats, and digitizer waveform generation.

The SPectrometer for Ion DEtermination in fission Research (SPIDER) has been developed for measuring mass yield distributions of fission products from spontaneous and neutron-induced fission. The 2 E –2 v method of measuring the kinetic energy ( E ) and velocity ( v ) of both outgoing fission products has been utilized, with the goal of measuring the mass of the fission products with an average resolution of 1 atomic mass unit (amu). The SPIDER instrument, consisting of detector components for time-of-flight, trajectory, and energy measurements, has been assembled and tested using 229 Th and 252 Cf radioactive decay sources. For commissioning, the fully assembled system measured fission products from spontaneous fission of 252 Cf. Individual measurement resolutions were met for time-of-flight (250 ps FWHM), spacial resolution (2 mm FHWM), and energy (92 keV FWHM for 8.376 MeV). Mass yield results measured from 252 Cf spontaneous fission products are reported from an E – v measurement.

A position-sensitive, high-resolution time-of-flight detector for fission fragments has been developed. The SPectrometer for Ion DEterminiation in fission Research (SPIDER) is a $2E-2v$ spectrometer designed to measure the mass of light fission fragments to a single mass unit. The time pick-off detector pairs to be used in SPIDER have been tested with $\alpha$-particles from $^{229}$Th and its decay chain and $\alpha$-particles and spontaneous fission fragments from $^{252}$Cf. Each detector module is comprised of a thin electron conversion foil, electrostatic mirror, microchannel plates, and delay-line anodes. Particle trajectories on the order of 700 mm are determined accurately to within 0.7 mm. Flight times on the order of 70 ns were measured with 200 ps resolution FWHM. Computed particle velocities are accurate to within 0.06 mm/ns corresponding to precision of 0.5%. An ionization chamber capable of 400 keV energy resolution coupled with the velocity measurements described here will pave the way for modestly efficient measurements of light fission fragments with unit mass resolution., Comment: 15 pages 6 figures

A digital data acquisition system has been combined with a double Frisch gridded ionization chamber for use at both moderated and unmoderated neutron sources at the Los Alamos Neutron Science (LANSCE) facility. The high efficiency of the instrument combined with intense LANSCE beams and new acquisition system permits fission output measurements across 11 orders of magnitude incident neutron energy. The acquisition and analysis system is presented along with the first in-beam performance tests of the setup.

Detailed information on the fission process can be inferred from the observation, modeling and theoretical understanding of prompt fission neutron and $\gamma$-ray~observables. Beyond simple average quantities, the study of distributions and correlations in prompt data, e.g., multiplicity-dependent neutron and \gray~spectra, angular distributions of the emitted particles, $n$-$n$, $n$-$\gamma$, and $\gamma$-$\gamma$~correlations, can place stringent constraints on fission models and parameters that would otherwise be free to be tuned separately to represent individual fission observables. The FREYA~and CGMF~codes have been developed to follow the sequential emissions of prompt neutrons and $\gamma$-rays~from the initial excited fission fragments produced right after scission. Both codes implement Monte Carlo techniques to sample initial fission fragment configurations in mass, charge and kinetic energy and sample probabilities of neutron and $\gamma$~emission at each stage of the decay. This approach naturally leads to using simple but powerful statistical techniques to infer distributions and correlations among many observables and model parameters. The comparison of model calculations with experimental data provides a rich arena for testing various nuclear physics models such as those related to the nuclear structure and level densities of neutron-rich nuclei, the $\gamma$-ray~strength functions of dipole and quadrupole transitions, the mechanism for dividing the excitation energy between the two nascent fragments near scission, and the mechanisms behind the production of angular momentum in the fragments, etc. Beyond the obvious interest from a fundamental physics point of view, such studies are also important for addressing data needs in various nuclear applications. (See text for full abstract.), Comment: 39 pages, 57 figure files, published in Eur. Phys. J. A, reference added this version

The average Total Kinetic Energy (TKE ) release and fission-fragment yields in neutron-induced fission of 235 U and 238 U was measured using a Frisch-gridded ionization chamber. These observables are important nuclear data quantites that are relevant to applications and for informing the next generation of fission models. The measurements were performed a the Los Alamos Neutron Science Center and cover E n = 200 keV – 30 MeV. The double-energy (2E) method was used to determine the fission-fragment yields and two methods of correcting for prompt-neutron emission were explored. The results of this study are correlated mass and TKE data.

The average total kinetic energy $(\overline{TKE})$ in $^{239}\mathrm{Pu}(n,f)$ has been measured for incident neutron energies between 0.5 and 50 MeV. The experiment was performed at the Los Alamos Neutron Science Center (LANSCE) using the neutron time-of-flight technique, and the kinetic energy of fission fragments post-neutron emission was measured in a double Frisch-gridded ionization chamber. This represents the first experimental study of the energy dependence of $\overline{TKE}$ in $^{239}\mathrm{Pu}$ above neutron energies of 6 MeV.

The SPectrometer for Ion DEtermination in fission Research (SPIDER) measures both position and time-of-flight (TOF) of charged particles using a system of thin carbon foils, electrostatic mirrors, microchannel plates, delay-line anodes, and a fast TDC. Tests have been conducted using 229Th and the alpha emitters in its decay chain. To date, timing resolution of 200 ps (FWHM) has been achieved corresponding to roughly 0.5% uncertainty in velocity measurements of fission fragments over a flight path of 52.1 cm. This velocity resolution, in combination with demonstrated fragment energy resolution is sufficient for 1 amu resolution of light mass fragments.

The ionization chamber component of the SPIDER detector has been designed to measure energy loss and kinetic energy of fragments produced through neutron-induced fission with energy resolutions of

Background: Neutron-rich, even-mass chromium and iron isotopes approaching neutron number $N=40$ have been important benchmarks in the development of shell-model effective interactions incorporating the effects of shell evolution in the exotic regime. Odd-mass manganese nuclei have received less attention, but provide important and complementary sensitivity to these interactions.Purpose: We report the observation of two new $\ensuremath{\gamma}$-ray transitions in $^{63}\mathrm{Mn}$, which establish the $(9/{2}^{\ensuremath{-}})$ and $(11/{2}^{\ensuremath{-}})$ levels on top of the previously known $(7/{2}^{\ensuremath{-}})$ first-excited state. The lifetime for the $(7/{2}^{\ensuremath{-}})$ and $(9/{2}^{\ensuremath{-}})$ excited states were determined for the first time, while an upper limit could be established for the $(11/{2}^{\ensuremath{-}})$ level.Method: Excited states in $^{63}\mathrm{Mn}$ have been populated in inelastic scattering from a $^{9}\mathrm{Be}$ target and in the fragmentation of $^{65}\mathrm{Fe}$. $\ensuremath{\gamma}\ensuremath{\gamma}$ coincidence relationships were used to establish the decay level scheme. A Doppler line-shape analysis for the Doppler-broadened $(7/{2}^{\ensuremath{-}})\ensuremath{\rightarrow}5/{2}^{\ensuremath{-}}$, $(9/{2}^{\ensuremath{-}})\ensuremath{\rightarrow}(7/{2}^{\ensuremath{-}}),$ and $(11/{2}^{\ensuremath{-}})\ensuremath{\rightarrow}(9/{2}^{\ensuremath{-}})$ transitions was used to determine (limits for) the corresponding excited-state lifetimes.Results: The low-lying level scheme and the excited-state lifetimes were compared with large-scale shell-model calculations using different model spaces and effective interactions in order to isolate important aspects of shell evolution in this region of structural change.Conclusions: While the theoretical $(7/{2}^{\ensuremath{-}})$ and $(9/{2}^{\ensuremath{-}})$ excitation energies show little dependence on the model space, the calculated lifetime of the $(7/{2}^{\ensuremath{-}})$ level and calculated energy of the $(11/{2}^{\ensuremath{-}})$ level reveal the importance of including the neutron ${g}_{9/2}$ and ${d}_{5/2}$ orbitals in the model space. The LNPS effective shell-model interaction provides the best overall agreement with the new data.

A scintillator based hodoscope array was recently constructed at the National Superconducting Cyclotron Laboratory (NSCL) at Michigan State University. The hodoscope will be used to measure the total kinetic energy of fragments in the focal plane of the large S800 magnetic spectrometer at the NSCL to provide atomic charge-state identification. The array consists of 32 closely packed 7.6 cm ×7.6 cm ×5.1 cm CsI(Na) crystals each coupled to a photomultiplier. All of the crystals were characterized with a γ -ray source prior to installation in the focal plane of the spectrometer. The hodoscope was then tested with a mono-energetic 76Ge primary beam as well as heavy ions from fragmentation reactions. The array is currently in place and has already been used in several recent experiments. The results of characterization of the properties of the crystals are presented here.

The 9Be(28Mg,27Na) one-proton removal reaction with a large proton separation energy of Sp(28Mg)=16.79 MeV is studied at intermediate beam energy. Coincidences of the bound 27Na residues with protons and other light charged particles are measured. These data are analyzed to determine the percentage contributions to the proton removal cross section from the elastic and inelastic nucleon removal mechanisms. These deduced contributions are compared with the eikonal reaction model predictions and with the previously measured data for reactions involving the re- moval of more weakly-bound protons from lighter nuclei. The role of transitions of the proton between different bound single-particle configurations upon the elastic breakup cross section is also quantified in this well-bound case. The measured and calculated elastic breakup fractions are found to be in good agreement., Comment: Phys. Rev. C 2014 (accepted)

The study of fission fragment yields and how they behave as a function of excitation energy provides insight into the process in which they are formed. Fission yields are also important for nuclear applications, as they can be used as a diagnostic tool. A new instrument, SPIDER (Spectrometer for Ion DEtermination in fission Research), is being developed for measuring fission yields as a function of incident neutron energy at the Los Alamos Neutron Science Center. The instrument employs a time-of-flight mass spectrometry method in which the velocity and kinetic energy of the fragments are measured in order to determine their mass. Additionally, by using Bragg peak spectroscopy, the charge of the fragments can be identified. A prototype instrument has been developed and preliminary results indicate that ∼ 1 mass unit resolution is feasible using this approach. A larger detector array is currently being designed, and will be used at study fission yields from thermal neutron energies up to at least 20 MeV.

We present a novel technique for studying the quenching of shell gaps in exotic isotopes. The method is based on extracting Gamow-Teller ($\ensuremath{\Delta}L=0$, $\ensuremath{\Delta}S=1$) transition strengths [$B(\mathrm{GT})$] to low-lying states from charge-exchange reactions at intermediate beam energies. These Gamow-Teller strengths are very sensitive to configuration mixing between cross-shell orbitals, and this technique thus provides an important complement to other tools currently used to study cross-shell mixing. This work focuses on the $N=8$ shell gap. We populated the ground and 2.24 MeV ${0}^{+}$ states in $^{12}\mathrm{Be}$ using the $^{12}\mathrm{B}({1}^{+})$ ($^{7}\mathrm{Li}$, $^{7}\mathrm{Be}$) reaction at $80\text{ }\text{ }\mathrm{MeV}/u$ in inverse kinematics. Using the ground-state $B(\mathrm{GT})$ value from $\ensuremath{\beta}$-decay measurements ($0.184\ifmmode\pm\else\textpm\fi{}0.007$) as a calibration, the $B(\mathrm{GT})$ for the transition to the second ${0}^{+}$ state was determined to be $0.214\ifmmode\pm\else\textpm\fi{}0.051$. Comparing the extracted Gamow-Teller strengths with shell-model calculations, it was determined that the wave functions of the first and second ${0}^{+}$ states in $^{12}\mathrm{Be}$ are composed of $25\ifmmode\pm\else\textpm\fi{}5%$ and $60\ifmmode\pm\else\textpm\fi{}5%$ $(0s{)}^{4}(0p{)}^{8}$ configurations, respectively.

Background: Momentum distributions of fragmentation products as a function of fragment mass have been used to study the fragmentation mechanism. The parallel component of the momentum distribution has been well studied previously and modeled. The perpendicular component, however, is much less measured or understood.Purpose: Measure both components of the linear momentum of a wide range of fragmentation products and compare the widths of the momentum distributions to previous results and descriptions.Method: The parallel and perpendicular components of the momentum vector have been measured for projectile-like fragments produced in the reactions of ${}^{76}$Ge with ${}^{9}$Be and ${}^{197}\phantom{\rule{-0.16em}{0ex}}$Au at 130 MeV/nucleon in a magnetic spectrometer.Results: The measured parallel momentum distributions of all fragments follow established systematics. The perpendicular momentum distributions of fragments produced by fragmentation by the ${}^{197}\phantom{\rule{-0.16em}{0ex}}$Au target with masses near that of the projectile exhibit a clear peak near the momentum corresponding to the grazing angle that diminishes with decreasing fragment mass.Conclusions: The interplay between Coulomb and nuclear scattering can be used to describe results for the most peripheral collisions.

We report final-state-exclusive measurements of the light charged fragments in coincidence with 26Ne residual nuclei following the direct two-proton removal from a neutron-rich 28Mg secondary beam. A Dalitz-plot analysis and comparisons with simulations show that a majority of the triple- coincidence events with two protons display phase-space correlations consistent with the (two-body) kinematics of a spatially-correlated pair-removal mechanism. The fraction of such correlated events, 56(12) %, is consistent with the fraction of the calculated cross section, 64 %, arising from spin S = 0 two-proton configurations in the entrance-channel (shell-model) 28Mg ground state wave function. This result promises access to an additional and more specific probe of the spin and spatial correlations of valence nucleon pairs in exotic nuclei produced as fast secondary beams., Comment: accepted for publication in Physical Review Letters

We present a novel technique for studying the quenching of shell gaps in exotic isotopes. The method is based on extracting Gamow-Teller (ΔL=0, ΔS=1) transition strengths [B(GT)] to low-lying states from charge-exchange reactions at intermediate beam energies. These Gamow-Teller strengths are very sensitive to configuration mixing between cross-shell orbitals, and this technique thus provides an important complement to other tools currently used to study cross-shell mixing. This work focuses on the N=8 shell gap. We populated the ground and 2.24 MeV 0+ states in 12Be using the 12B(1+) (7Li, 7Be) reaction at 80 MeV/u in inverse kinematics. Using the ground-state B(GT) value from β-decay measurements (0.184±0.007) as a calibration, the B(GT) for the transition to the second 0+ state was determined to be 0.214±0.051. Comparing the extracted Gamow-Teller strengths with shell-model calculations, it was determined that the wave functions of the first and second 0+ states in 12Be are composed of 25±5% and 60±5% (0s)4(0p)8 configurations, respectively.

New measurements and reaction model calculations are reported for single neutron pickup reactions onto a fast \nuc{22}{Mg} secondary beam at 84 MeV per nucleon. Measurements were made on both carbon and beryllium targets, having very different structures, allowing a first investigation of the likely nature of the pickup reaction mechanism. The measurements involve thick reaction targets and $\gamma$-ray spectroscopy of the projectile-like reaction residue for final-state resolution, that permit experiments with low incident beam rates compared to traditional low-energy transfer reactions. From measured longitudinal momentum distributions we show that the $\nuc{12}{C} (\nuc{22}{Mg},\nuc{23}{Mg}+\gamma)X$ reaction largely proceeds as a direct two-body reaction, the neutron transfer producing bound \nuc{11}{C} target residues. The corresponding reaction on the \nuc{9}{Be} target seems to largely leave the \nuc{8}{Be} residual nucleus unbound at excitation energies high in the continuum. We discuss the possible use of such fast-beam one-neutron pickup reactions to track single-particle strength in exotic nuclei, and also their expected sensitivity to neutron high-$\ell$ (intruder) states which are often direct indicators of shell evolution and the disappearance of magic numbers in the exotic regime., Comment: 8 pages, 5 figures

$^{9}\mathrm{Be}$-induced inelastic scattering of $^{62,64,66}\mathrm{Fe}$ and $^{60,62,64}\mathrm{Cr}$ was performed at intermediate beam energies. Excited states in $^{64}\mathrm{Cr}$ were measured for the first time. Energies and population patterns of excited states in these neutron-rich Fe and Cr nuclei are compared and interpreted in the framework of large-scale shell-model calculations in different model spaces. Evidence for increased collectivity and for distinct structural changes between the neighboring Fe and Cr isotopic chains near $N=40$ is presented.

Two new experiments were carried out at the NSCL to explore the details of the linear moment and excitation energy distributions of projectile fragmentation production. In the first experiment the full linear momentum distributions of fragments from the reaction of a 76 Ge beam with beryllium and gold targets were measured in the S800 spectrometer. The results indicate a strong contribution of "far side" or attractive scattering to the near-projectile products with the gold target. In the second experiment the excitation energy of primary projectile fragments from peripheral nuclear reactions at intermediate energies was carried out at the NSCL. Sodium, neon and fluorine isotopes produced by the fragmentation of a neutron-rich 32Mg beam by a beryllium target were observed in a magnetic spectrometer in coincidence with fast neutrons detected using the Modular Neutron Array (MoNA). A new technique based on an analysis of the observed neutron multiplicity distributions was used to estimate the excitation energy and mass of the precursor intermediate products for the first time. A strong correlation between the neutron multiplicity and the total mass loss was observed indicating that large excitation energies were created in the prefragments by the initial collision. These findings are generally consistent with the internuclear cascade model of the collision dynamics but not with macroscopic abrasion-ablation models.