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719 results on '"Jong-Sung Yu"'

1. High vacancy formation energy boosts the stability of structurally ordered PtMg in hydrogen fuel cells

Author

Caleb Gyan-Barimah, Jagannath Sai Pavan Mantha, Ha-Young Lee, Yi Wei, Cheol-Hwan Shin, Muhammad Irfansyah Maulana, Junki Kim, Graeme Henkelman, and Jong-Sung Yu

Subjects
Science
Abstract

Abstract Alloys of platinum with alkaline earth metals promise to be active and highly stable for fuel cell applications, yet their synthesis in nanoparticles remains a challenge due to their high negative reduction potentials. Herein, we report a strategy that overcomes this challenge by preparing platinum-magnesium (PtMg) alloy nanoparticles in the solution phase. The PtMg nanoparticles exhibit a distinctive structure with a structurally ordered intermetallic core and a Pt-rich shell. The PtMg/C as a cathode catalyst in a hydrogen-oxygen fuel cell exhibits a mass activity of 0.50 A mgPt −1 at 0.9 V with a marginal decrease to 0.48 A mgPt −1 after 30,000 cycles, exceeding the US Department of Energy 2025 beginning-of-life and end-of-life mass activity targets, respectively. Theoretical studies show that the activity stems from a combination of ligand and strain effects between the intermetallic core and the Pt-rich shell, while the stability originates from the high vacancy formation energy of Mg in the alloy.

Published
2024
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2. Development of high-energy non-aqueous lithium-sulfur batteries via redox-active interlayer strategy

Author

Byong-June Lee, Chen Zhao, Jeong-Hoon Yu, Tong-Hyun Kang, Hyean-Yeol Park, Joonhee Kang, Yongju Jung, Xiang Liu, Tianyi Li, Wenqian Xu, Xiao-Bing Zuo, Gui-Liang Xu, Khalil Amine, and Jong-Sung Yu

Subjects
Science
Abstract

Lithium-sulfur batteries promise high energy density, but polysulfide shuttling acts as a major stumbling block toward practical development. Here, a redox-active interlayer is proposed to confine polysulfides, increase the cell capacity and improve cell cycle life.

Published
2022
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3. Direct Observation of Off‐Stoichiometry‐Induced Phase Transformation of 2D CdSe Quantum Nanosheets

Author

Hyeonjong Ma, Dongjun Kim, Soo Ik Park, Back Kyu Choi, Gisang Park, Hayeon Baek, Hyocheol Lee, Hyeongseoung Kim, Jong‐Sung Yu, Won Chul Lee, Jungwon Park, and Jiwoong Yang

Subjects
in situ transmission electron microscopy, phase transformation, quantum nanosheets, stoichiometry, two‐dimensional nanocrystals, Science
Abstract

Abstract Crystal structures determine material properties, suggesting that crystal phase transformations have the potential for application in a variety of systems and devices. Phase transitions are more likely to occur in smaller crystals; however, in quantum‐sized semiconductor nanocrystals, the microscopic mechanisms by which phase transitions occur are not well understood. Herein, the phase transformation of 2D CdSe quantum nanosheets caused by off‐stoichiometry is revealed, and the progress of the transformation is directly observed by in situ transmission electron microscopy. The initial hexagonal wurtzite‐CdSe nanosheets with atomically uniform thickness are transformed into cubic zinc blende‐CdSe nanosheets. A combined experimental and theoretical study reveals that electron‐beam irradiation can change the stoichiometry of the nanosheets, thereby triggering phase transformation. The loss of Se atoms induces the reconstruction of surface atoms, driving the transformation from wurtzite‐CdSe(112¯$ar{2}$0) to zinc blende‐CdSe(001) 2D nanocrystals. Furthermore, during the phase transformation, unconventional dynamic phenomena occur, including domain separation. This study contributes to the fundamental understanding of the phase transformations in 2D quantum‐sized semiconductor nanocrystals.

Published
2023
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4. Biocompatible Core–Shell-Structured Si-Based NiO Nanoflowers and Their Anticancer Activity

Author

Kihak Gwon, Jong-Deok Park, Seonhwa Lee, Jong-Sung Yu, and Do Nam Lee

Subjects
core–shell, Ni composite, nanoflowers, biocompatibility, anticancer activity, Pharmacy and materia medica, RS1-441
Abstract

Compared to most of nano-sized particles, core–shell-structured nanoflowers have received great attention as bioactive materials because of their high surface area with the flower-like structures. In this study, core–shell-structured Si-based NiO nanoflowers, Si@NiO, were prepared by a modified chemical bath deposition method followed by thermal reduction. The crystal morphology and basic structure of the composites were characterized by powder X-ray diffraction (PXRD), Fourier-transform infrared spectroscopy (FT-IR), scanning electron microscopy (SEM), transmission electron microscopy (TEM), specific surface area (BET) and porosity analysis (BJT), and inductively coupled plasma optical emission spectrometry (ICP-OES). The electrochemical properties of the Si@NiO nanoflowers were examined through the redox reaction of ascorbic acid with the metal ions present on the surface of the core–shell nanoflowers. This reaction favored the formation of reactive oxygen species. The Si@NiO nanoflowers showed excellent anticancer activity and low cytotoxicity toward the human breast cancer cell line (MCF-7) and mouse embryonic fibroblasts (MEFs), respectively, demonstrating that the anticancer activities of the Si@NiO nanoflowers were primarily derived from the oxidative capacity of the metal ions on the surface, rather than from the released metal ions. Thus, this proves that Si-based NiO nanoflowers can act as a promising candidate for therapeutic applications.

Published
2022
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6. Ecofriendly AgBiS2 Nanocrystal Photoanode for Highly Efficient Visible-Light-Driven Photoelectrochemical Water Splitting

Author

Jin Young Park, Gisang Park, Sung Yong Bae, Hae Jeong Kim, Duck Hoon Lee, Seonkyung Ko, Soo-Kwan Kim, Gyudong Lee, Hyung Ryul You, Hyosung Choi, Jong-Sung Yu, Younghoon Kim, and Jongmin Choi

Subjects
Materials Chemistry, Electrochemistry, Energy Engineering and Power Technology, Chemical Engineering (miscellaneous), Electrical and Electronic Engineering
Published
2023

7. Active and stable PtP2-based electrocatalysts solve the phosphate poisoning issue of high temperature fuel cells

Author

Jeong-Hoon Yu, Kiran Pal Singh, Se-Jun Kim, Tong-Hyun Kang, Kug-Seung Lee, Hyungjun Kim, Stefan Ringe, and Jong-Sung Yu

Subjects
Renewable Energy, Sustainability and the Environment, General Materials Science, General Chemistry
Abstract

Herein, we have prepared platinum phosphide (PtP2)-based cathode electrocatalysts for HT-PEMFCs. The high activity and stability of the PtP2/C-based catalysts were attributed to the high oxyphilicity of the phosphorus atoms.

Published
2023

8. Magnesium: properties and rich chemistry for new material synthesis and energy applications

Author

Cheol-Hwan Shin, Ha-Young Lee, Caleb Gyan-Barimah, Jeong-Hoon Yu, and Jong-Sung Yu

Subjects
General Chemistry
Abstract

Magnesium (Mg) has many unique properties. The present review highlights the basic properties of Mg and its application in energy processes such as photocatalysis, electrocatalysis, energy storage, solar harvesting, hydrogen storage, plasmonic, and sensing.

Published
2023

11. Strained Pt(221) Facet in a PtCo@Pt-Rich Catalyst Boosts Oxygen Reduction and Hydrogen Evolution Activity

Author

Emmanuel Batsa Tetteh, Caleb Gyan-Barimah, Ha-Young Lee, Tong-Hyun Kang, Seonghyeon Kang, Stefan Ringe, and Jong-Sung Yu

Subjects
General Materials Science
Abstract

Over the last years, the development of highly active and durable Pt-based electrocatalysts has been identified as the main target for a large-scale industrial application of fuel cells. In this work, we make a significant step ahead in this direction by preparing a high-performance electrocatalyst and suggesting new structure-activity design concepts which could shape the future of oxygen reduction reaction (ORR) catalyst design. For this, we present a new one-dimensional nanowire catalyst consisting of a L1

Published
2022

13. Progress in electrode and electrolyte materials: path to all-solid-state Li-ion batteries

Author

Sanjeev K. Sharma, Gaurav Sharma, Anurag Gaur, Anil Arya, Fateme Sadat Mirsafi, Reza Abolhassani, Horst-Günter Rubahn, Jong-Sung Yu, and Yogendra Kumar Mishra

Abstract

This review presents a brief scenario regarding the development of cathodes, anodes, and electrolytes for next-generation Li-ion batteries (LIBs) and supercapacitors for future energy technologies.

Published
2022

14. Highly bioactive and low cytotoxic Si-based NiOOH nanoflowers targeted against various bacteria, including MRSA, and their potential antibacterial mechanism

Author

Jong-Deok Park, Ihn Han, Jong-Sung Yu, Seonhwa Lee, Do Nam Lee, and Kihak Gwon

Subjects
biology, Chemistry, General Chemical Engineering, 02 engineering and technology, Nanoflower, 010402 general chemistry, 021001 nanoscience & nanotechnology, medicine.disease_cause, biology.organism_classification, Antimicrobial, Ascorbic acid, 01 natural sciences, Combinatorial chemistry, 0104 chemical sciences, Staphylococcus aureus, medicine, 0210 nano-technology, Antibacterial activity, Cytotoxicity, Bacteria, Chemical bath deposition
Abstract

With the emergence of new drug-resistant microorganisms, the development of effective antimicrobial agents is urgently required. Core-shell-structured nanomaterials have received considerable attention as antibacterial agents. We prepared a bioactive core-shell-structured silicon-based NiOOH nanoflower (Si@NiOOH) targeted against various bacteria using a modified chemical bath deposition method. Further, we investigated its potential antibacterial mechanism by evaluating electrochemical properties in a redox reaction with ascorbic acid, measuring metal ion release, and analyzing the surface area. The bactericidal rate of Si@NiOOH at 200 μg/mL towards Pseudomonas aeruginosa, Klebsiella pneumoniae, and methicillin-resistant Staphylococcus aureus was as high as 99.9%. Si@NiOOH maintained its original morphology after killing the bacteria and exhibited negligible cytotoxicity towards mouse embryonic fibroblasts. The excellent antibacterial activities of Si@NiOOH are possibly derived from its high surface area, providing a wide active site attached to the cell wall, and the high oxidative potency of the Ni(III) cations existing on its surface. The high antibacterial activity and low cytotoxicity of the nanoflower make it a promising tool for promoting wound healing and for use with medical devices and implants.

Published
2021

15. Self-Templated Formation of Fluffy Graphene-Wrapped Ni5P4 Hollow Spheres for Li-Ion Battery Anodes with High Cycling Stability

Author

Byong-June Lee, Jinliang Yuan, Gisang Park, Jong-Sung Yu, Chunfei Zhang, He Miao, and Lan Xia

Subjects
Battery (electricity), Materials science, Graphene, 02 engineering and technology, Chemical vapor deposition, Electrolyte, 010402 general chemistry, 021001 nanoscience & nanotechnology, Electrochemistry, 01 natural sciences, 0104 chemical sciences, law.invention, Anode, Chemical engineering, law, Water splitting, General Materials Science, 0210 nano-technology, Nanosheet
Abstract

Transition-metal phosphides have gained great importance in the field of energy conversion and storage such as electrochemical water splitting, fuel cells, and Li-ion batteries. In this study, a rationally designed novel fluffy graphene (FG)-wrapped monophasic Ni5P4 (Ni5P4@FG) is in-situ-synthesized using a chemical vapor deposition method as a Li-ion battery anode material. The porous and hollow structure of Ni5P4 core is greatly helpful for lithium-ion diffusion, and at the same time, the cilia-like graphene nanosheet shell provides an electron-conducting layer and stabilizes the solid electrolyte interface formed on the Ni5P4 surface. The Ni5P4@FG sample shows a high reversible capacity of 739 mAh g-1 after 300 cycles at a specific current density of 500 mA g-1. The high capacity, superior cycling stability, and improved rate capability of Ni5P4@FG are ascribed to its unique hierarchical structure. Moreover, the present efficient fabrication methodology of Ni5P4@FG has potential to be developed as a general method for the synthesis of other transition-metal phosphides.

Published
2021

17. Self-Limiting Growth of Single-Layer N-Doped Graphene Encapsulating Nickel Nanoparticles for Efficient Hydrogen Production

Author

Jinliang Yuan, Gisang Park, Chunfei Zhang, Byong-June Lee, Tong-Hyun Kang, He Miao, Jong-Sung Yu, Yunwen Wu, and Shenghong Ju

Subjects
Materials science, Graphene, Nanoparticle, chemistry.chemical_element, 02 engineering and technology, Overpotential, 021001 nanoscience & nanotechnology, law.invention, Catalysis, chemistry.chemical_compound, Nickel, Adsorption, chemistry, Chemical engineering, law, Nafion, General Materials Science, 0210 nano-technology, Hydrogen production
Abstract

Effective nonprecious metal catalysts are urgently needed for hydrogen evolution reaction (HER). The hybridization of N-doped graphene and a cost-effective metal is expected to be a promising approach for enhanced HER performance but faces bottlenecks in controllable fabrication. Herein, a silica medium-assisted method is developed for the high-efficient synthesis of single-layer N-doped graphene encapsulating nickel nanoparticles (Ni@SNG), where silica nanosheets molecule sieves tactfully assist the self-limiting growth of single-layer graphene over Ni nanoparticles by depressing the diffusion of gaseous carbon radical reactants. The Ni@SNG sample synthesized at 800 °C shows excellent activity for HER in alkaline medium with a low overpotential of 99.8 mV at 10 mA cm-2, which is close to that of the state-of-the-art Pt/C catalyst. Significantly, the Ni@SNG catalyst is also developed as a binder-free electrode in magnetic field, exhibiting much improved performance than the common Nafion binder-based electrode. Therefore, the magnetism adsorption technique will be a greatly promising approach to overcome the high electron resistance and poor adhesive stability of polymer binder-based electrodes in practical applications.

Published
2021

18. Controllable synthesis of single-layer graphene over cobalt nanoparticles and insight into active sites for efficient oxygen evolution

Author

Cheol-Hwan Shin, Gisang Park, Chunfei Zhang, CheolGi Kim, Jong-Sung Yu, Kug-Seung Lee, Byeonghwa Lim, and Joonhee Kang

Subjects
Materials science, Renewable Energy, Sustainability and the Environment, Graphene, Doping, Oxygen evolution, chemistry.chemical_element, Nanoparticle, Nanotechnology, 02 engineering and technology, General Chemistry, Chemical vapor deposition, 010402 general chemistry, 021001 nanoscience & nanotechnology, 01 natural sciences, 0104 chemical sciences, law.invention, Catalysis, Adsorption, chemistry, law, General Materials Science, 0210 nano-technology, Cobalt
Abstract

Controllable synthesis of graphene-coated metal nanoparticles (NPs) presents a major challenge when considering the practical application of these catalysts. Herein, we use silica as a radical sieve to grow graphene over cobalt NPs via chemical vapor deposition. As-prepared single-layer graphene-coated cobalt NPs with and without N doping (Co@N-SG and Co@SG) exhibit noticeable oxygen evolution reaction (OER) activity. Furthermore, a magnet-assisted binder-free Co@N-SG electrode illustrates much improved OER activity and stability over conventional binder-assisted counterparts, suggesting this as an effective way to overcome the recognized issues of high electron transfer resistance and poor adhesion of binder-based electrodes in practical applications. Interestingly, the graphene shell possesses varying defects and major OER benefitting active sites are found around said defects in the shell, while separately isolated Co@SG with a defect-free shell, despite exhibiting a slightly lower initial activity, illustrates a much-improved durable OER performance. The underlying Co affects the electron density of the graphene shell through dipole interaction and the electron density is optimized for adsorption of reaction intermediates, hence accelerating OER performance. This work will provide new clues to design efficient and durable electrocatalysts with further enhanced OER performance.

Published
2021

19. Positive self-reconstruction in an FeNiMo phosphide electrocatalyst for enhanced overall water splitting

Author

Emmanuel Batsa Tetteh, Cheol-Hwan Shin, Caleb Gyan-Barimah, Yi Wei, Jong-Sung Yu, and Gisang Park

Subjects
Materials science, Renewable Energy, Sustainability and the Environment, Phosphide, Oxygen evolution, Energy Engineering and Power Technology, Electrolyte, Electrocatalyst, Cathode, law.invention, Anode, chemistry.chemical_compound, Fuel Technology, chemistry, Chemical engineering, law, Water splitting, Bifunctional
Abstract

Searching for low-cost and highly active bifunctional electrocatalysts toward hydrogen/oxygen evolution reactions is a grand challenge for water splitting hydrogen production. Herein, we prepare a trimetallic nickel, iron, and molybdenum phosphide (FeNiMoP) grown on nickel foam (NF) via a facile two-step process and employ it as a bifunctional electrocatalyst for full water splitting. In virtue of the superior hydrogen/oxygen evolution activity, the cell with the bifunctional FeNiMoP as both anode and cathode exhibits an initial low cell voltage of 1.50 V at a current density of 10 mA cm−2 in 1.0 M KOH electrolyte solution. Impressively, the full cell voltage decreases to 1.44 V through favorable self-reconstruction on both the anode and cathode during the electrocatalytic overall water splitting process. On the anode side, the FeNiMoP is transformed into FeNiOOH while Mo and P elements are dissolved into the electrolyte. Such transformation leads to a continuously increasing active surface area, and the dissolved Mo forms MoO42− in the electrolyte which improves the OER performance. On the cathode side, the dissolution and re-deposition of Mo oxides on the surface of the electrode greatly increase the active surface sites towards the electrolytes, and the surface absorbed Mo oxides play key roles, leading to a positive effect on HER performance. The new synthesis strategy, taking advantage of favorable structural self-reconstruction in the catalysts can be extended to other catalytic systems.

Published
2021

20. Single-Atom Iron-Based Electrocatalysts for High-Temperature Polymer Electrolyte Membrane Fuel Cell: Organometallic Precursor and Pore Texture Tailoring

Author

Kiran Pal Singh, Ha-Young Lee, Tong-Hyun Kang, Jeong-Hoon Yu, Jong-Sung Yu, Fatemeh Razmjooei, Byong-June Lee, and Hyoung-Juhn Kim

Subjects
chemistry.chemical_classification, oxygen reduction reaction, Materials science, nitrogen doping, single-atom iron, Energy Engineering and Power Technology, chemistry.chemical_element, Polymer, Electrolyte, Catalysis, Membrane, Chemical engineering, chemistry, Atom, EDTA−Fe organometallic complex, high-temperature polymer electrolyte membrane fuel cell, Materials Chemistry, Electrochemistry, Chemical Engineering (miscellaneous), Fuel cells, Texture (crystalline), Electrical and Electronic Engineering, Platinum
Abstract

The oxygen reduction reaction (ORR) activity of platinum (Pt)-based catalyst is not satisfactory in high-temperature polymer electrolyte membrane fuel cells (HT-PEMFCs) operating with a phosphoric ...

Published
2020

21. Low Temperature Synthesis of New Highly Graphitized N-Doped Carbon for Pt Fuel Cell Supports, Satisfying Doe 2025 Durability Standards for Both Catalyst and Suppor T

Author

Ha-Young Lee, Ted H. Yu, Cheol-Hwan Shin, Alessandro Fortunelli, Sang Gu Ji, Yujin Kim, Tong-Hyun Kang, Byong-June Lee, Boris V. Merinov, William A. Goddard, Chang Hyuck Choi, and Jong-Sung Yu

Subjects
History, Polymers and Plastics, Process Chemistry and Technology, Business and International Management, Catalysis, Industrial and Manufacturing Engineering, General Environmental Science
Published
2022

22. Synergistic CoN-Decorated Pt Catalyst on Two-Dimensional Porous Co–N-Doped Carbon Nanosheet for Enhanced Oxygen Reduction Activity and Durability

Author

Ha-Young Lee, Tong-Hyun Kang, Thanh-Nhan Tran, Jong-Sung Yu, Byong-June Lee, and Jong Deok Park

Subjects
Materials science, Doped carbon, Energy Engineering and Power Technology, chemistry.chemical_element, Electrocatalyst, Oxygen, Durability, Catalysis, chemistry, Chemical engineering, Materials Chemistry, Electrochemistry, Chemical Engineering (miscellaneous), Oxygen reduction reaction, Electrical and Electronic Engineering, Platinum, Nanosheet
Abstract

Herein, an oxygen reduction reaction (ORR) catalyst consisting of CoN-decorated Pt nanoparticles (NPs) on thin two-dimensional (2D) nanosheet-structured Co-N-doped porous carbon is prepared by util...

Published
2020

23. New PtMg Alloy with Durable Electrocatalytic Performance for Oxygen Reduction Reaction in Proton Exchange Membrane Fuel Cell

Author

Hyung Chul Ham, Ha-Young Lee, Sung Jong Yoo, Emmanuel Batsa Tetteh, Cheol-Hwan Shin, Jong-Sung Yu, Thanh-Nhan Tran, Seung-hoon Kim, and Jue-Hyuk Jang

Subjects
Alkaline earth metal, Materials science, Renewable Energy, Sustainability and the Environment, Alloy, Energy Engineering and Power Technology, Proton exchange membrane fuel cell, 02 engineering and technology, engineering.material, 010402 general chemistry, 021001 nanoscience & nanotechnology, 01 natural sciences, 0104 chemical sciences, Fuel Technology, Chemical engineering, Chemistry (miscellaneous), Polycrystalline alloy, Electrode, Materials Chemistry, engineering, Oxygen reduction reaction, 0210 nano-technology
Abstract

Polycrystalline alloy electrodes of Pt with alkaline earth metals (Ca, Sr, and Ba) have been shown to exhibit enhanced electrocatalytic performance for oxygen reduction reaction (ORR) relative to P...

Published
2020

24. TiO2/ZrO2 Nanoparticle Composites for Electrochemical Hydrogen Evolution

Author

Jong-Sung Yu, Kiran Pal Singh, Fatemeh Razmjooei, Ha-Young Lee, Apurba Sinhamahapatra, Choel-Hwan Shin, and Joonhee Kang

Subjects
Work (thermodynamics), Materials science, business.industry, education, technology, industry, and agriculture, Nanoparticle, equipment and supplies, Electrochemistry, Charge transfer resistance, Semiconductor, General Materials Science, Hydrogen evolution, Cubic zirconia, Composite material, Electronic conductivity, business
Abstract

Composites of different semiconductors are found to show much improved electronic conductivity and decreased charge transfer resistance. In this work, this hypothesis is tested by preparing composi...

Published
2020

25. High performance binder-free Fe–Ni hydroxides on nickel foam prepared in piranha solution for the oxygen evolution reaction

Author

Cheol-Hwan Shin, Joonhee Kang, Jong-Sung Yu, Yi Wei, and Gisang Park

Subjects
Materials science, Hydrogen, Renewable Energy, Sustainability and the Environment, Oxygen evolution, Energy Engineering and Power Technology, chemistry.chemical_element, Overpotential, Electrochemistry, chemistry.chemical_compound, Nickel, Fuel Technology, Chemical engineering, chemistry, Electrode, Hydroxide, Piranha solution
Abstract

Nickel foam (NF) can be directly utilized as an electrochemical electrode because of its conductive, rigid and porous structure. Herein, a novel robust binder-free Fe–Ni hydroxide-loaded NF electrode is prepared by simple corrosion of NF in a home-made piranha solution with an Fe3+ precursor. The roughened NF surface observed after the sample treatment indicates the formation of active species associated with amorphous Fe-hydroxide and/or FeNi-hydroxide particles. The piranha solution-corroded NF electrode generates more hydroxide groups compared to the water-corroded NF electrode, and exhibits remarkable electrochemical oxygen evolution reaction activity in alkaline medium with a low overpotential of 245 mV at 10 mA cm−2. It also maintains low working potential below 267 mV at 10 mA cm−2 over 500 h operation without any sign of degradation, indicating excellent long-term stability, which can be attributed to the robust binder-free electrode and the cooperative synergistic interaction between Fe-hydroxides and Ni-hydroxides in the FeNi hybrid composite of individually incompetent OER components, generated over the NF. The role of Fe doped in Ni(OH)2 is theoretically studied by DFT calculations, and it is found that the adsorption free energies of OH* and OOH* are significantly reduced by the addition of Fe into Ni(OH)2, accelerating the OER compared to bare Ni(OH)2. Furthermore, when the active electrode is equipped with a solar cell, a high current density of 23–24 mA cm−2 is observed for 10 h under AM 1.5G 1 sun irradiation, suggesting high possibility for the production of green hydrogen from renewable solar energy.

Published
2020

26. Sub 10 nm CoO nanoparticle-decorated graphitic carbon nitride for solar hydrogen generationviaefficient charge separation

Author

Srishti, Apurba Sinhamahapatra, Aditya Kumar, Aniruddha Mondal, Jong-Sung Yu, and Shubham Biswas

Subjects
Materials science, Aqueous solution, General Engineering, Graphitic carbon nitride, Nanoparticle, Bioengineering, Heterojunction, 02 engineering and technology, General Chemistry, Electron, 010402 general chemistry, 021001 nanoscience & nanotechnology, 01 natural sciences, Atomic and Molecular Physics, and Optics, 0104 chemical sciences, chemistry.chemical_compound, Chemical engineering, chemistry, Triethanolamine, medicine, General Materials Science, 0210 nano-technology, Absorption (electromagnetic radiation), Hydrogen production, medicine.drug
Abstract

Solar hydrogen generation is one of the most compelling concepts in modern research to address both the energy and environmental issues simultaneously for the survival of the human race. A Type II heterojunction (CoO–GCN) was fabricated by decorating sub 10 nm CoO nanoparticles (NPs) on the graphitic carbon nitride (GCN) surface. It exhibited improved absorption of UV-VIS light and efficiently separate the photogenerated electrons and holes in opposite directions. A maximum hydrogen generation rate of 9.8 mmol g−1 h−1 was recorded using CoO–GCN from 10% aqueous triethanolamine under simulated sunlight in the presence of 1 wt% Pt. The rate is 3.8 times higher than that of bare GCN. Furthermore, it showed excellent stability for up to five repeated uses. Interestingly, the study also revealed that untreated seawater could replace the deionized water. The cooperative participation of the uniform shape and size of CoO NPs firmly grafted on GCN resulted in remarkable performance for solar hydrogen generation.

Published
2020

27. Real-time monitored photocatalytic activity and electrochemical performance of an rGO/Pt nanocomposite synthesizedviaa green approach

Author

CheolGi Kim, Syafiq Ahmad, Byong-June Lee, Sri Ramulu Torati, Jong-Sung Yu, Satish Kasturi, and Yun Ji Eom

Subjects
Aqueous solution, Nanocomposite, Materials science, Graphene, Reducing agent, General Chemical Engineering, Oxide, General Chemistry, Electrochemistry, law.invention, chemistry.chemical_compound, Chemical engineering, chemistry, law, Photocatalysis, Photodegradation
Abstract

Herein, we have reported the real-time photodegradation of methylene blue (MB), an organic pollutant, in the presence of sunlight at an ambient temperature using a platinum-decorated reduced graphene oxide (rGO/Pt) nanocomposite. The photocatalyst was prepared via a simple, one-pot and green approach with the simultaneous reduction of GO and Pt using aqueous honey as a reducing agent. Moreover, the honey not only simultaneously reduced Pt ions and GO but also played a key role in the growth and dispersion of Pt nanoparticles on the surface of rGO. Various rGO/Pt nanocomposites with different percentages of Pt nanoparticles loaded on rGO were obtained by tuning the concentration of the Pt source. The high percentage of Pt nanoparticles with an average size of 2.5 nm dispersed on rGO has shown excellent electrochemical performance. The photocatalytic activity of the rGO/Pt composite was enhanced by increasing the weight percent of the Pt particles on rGO, which led to the formation of a highly efficient photocatalyst. The optimized photocatalyst exhibited remarkable photocatalytic activity and degraded 98% MB in 180 minutes; thus, it can be used for industrial and environmental applications.

Published
2020

28. Insight into the Boosted Electrocatalytic Oxygen Evolution Performance of Highly Hydrophilic Nickel–Iron Hydroxide

Author

Emmanuel Batsa Tetteh, Byong-June Lee, Yi Wei, Cheol-Hwan Shin, and Jong-Sung Yu

Subjects
Tafel equation, Materials science, Oxygen evolution, Energy Engineering and Power Technology, chemistry.chemical_element, Overpotential, Electrocatalyst, Catalysis, chemistry.chemical_compound, Nickel, chemistry, Chemical engineering, Electrode, Materials Chemistry, Electrochemistry, Chemical Engineering (miscellaneous), Hydroxide, Electrical and Electronic Engineering
Abstract

Nickel–iron based materials are well-known catalysts for the oxygen evolution reaction (OER) and have been widely investigated. However, the synergy between these two components is still controversial. Herein, we report a facile immersion method for the synthesis of binder-free nickel–iron hydroxide loaded on Ni foam (NiFe-OH/NF) with superior hydrophilic property and high OER catalytic activity. The strong hydrophilic property of the binder-free NiFe-OH/NF electrode significantly enhances an effective contact between electrocatalyst and aqueous electrolyte and favors the bubble detachment from the electrode, facilitating the electron transfer and improving the OER activity. The hydrophilic NiFe-OH/NF can achieve a geometrical current density of 100 mA cm–1 at an extremely low overpotential (219 mV), along with a Tafel slope of 56 mV dec–1 and superior long-term stability at high current density in alkaline media, strongly indicating that the hydrophilicity plays an important role in improving the OER per...

Published
2019

29. Biocompatible Core-Shell-Structured Si-Based NiO Nanoflowers and Their Anticancer Activity

Author

Kihak Gwon, Jong-Deok Park, Seonhwa Lee, Jong-Sung Yu, and Do Nam Lee

Subjects
Pharmaceutical Science, core–shell, Ni composite, nanoflowers, biocompatibility, anticancer activity
Abstract

Compared to most of nano-sized particles, core–shell-structured nanoflowers have received great attention as bioactive materials because of their high surface area with the flower-like structures. In this study, core–shell-structured Si-based NiO nanoflowers, Si@NiO, were prepared by a modified chemical bath deposition method followed by thermal reduction. The crystal morphology and basic structure of the composites were characterized by powder X-ray diffraction (PXRD), Fourier-transform infrared spectroscopy (FT-IR), scanning electron microscopy (SEM), transmission electron microscopy (TEM), specific surface area (BET) and porosity analysis (BJT), and inductively coupled plasma optical emission spectrometry (ICP-OES). The electrochemical properties of the Si@NiO nanoflowers were examined through the redox reaction of ascorbic acid with the metal ions present on the surface of the core–shell nanoflowers. This reaction favored the formation of reactive oxygen species. The Si@NiO nanoflowers showed excellent anticancer activity and low cytotoxicity toward the human breast cancer cell line (MCF-7) and mouse embryonic fibroblasts (MEFs), respectively, demonstrating that the anticancer activities of the Si@NiO nanoflowers were primarily derived from the oxidative capacity of the metal ions on the surface, rather than from the released metal ions. Thus, this proves that Si-based NiO nanoflowers can act as a promising candidate for therapeutic applications.

Published
2021

30. Injectable hyaluronic acid hydrogel encapsulated with Si-based NiO nanoflower by visible light cross-linking: Its antibacterial applications

Author

Kihak Gwon, Jong-Deok Park, Seonhwa Lee, Won Il Choi, Youngmin Hwang, Munemasa Mori, Jong-Sung Yu, and Do Nam Lee

Subjects
Methicillin-Resistant Staphylococcus aureus, Silicon, Light, Hydrogels, General Medicine, Fibroblasts, Silicon Dioxide, Biochemistry, Anti-Bacterial Agents, Mice, Structural Biology, Nickel, Pseudomonas aeruginosa, Animals, Hyaluronic Acid, Molecular Biology
Abstract

Bacterial infections have become a severe threat to human health and antibiotics have been developed to treat them. However, extensive use of antibiotics has led to multidrug-resistant bacteria and reduction of their therapeutic effects. An efficient solution may be localized application of antibiotics using a drug delivery system. For clinical application, they need to be biodegradable and should offer a prolonged antibacterial effect. In this study, a new injectable and visible-light-crosslinked hyaluronic acid (HA) hydrogel loaded with silicon (Si)-based nickel oxide (NiO) nanoflowers (Si@NiO) as an antibacterial scaffold was developed. Si@NiO nanoflowers were synthesized using chemical bath deposition before encapsulating them in the HA hydrogel under a mild visible-light-crosslinking conditions to generate a Si@NiO-hydrogel. Si@NiO synthesis was confirmed using scanning electron microscopy, transmission electron microscopy, and powder X-ray diffraction. As-prepared Si@NiO-hydrogel exhibited enhanced mechanical properties compared to a control bare hydrogel sample. Moreover, Si@NiO-hydrogel exhibits excellent antibacterial properties against three bacterial strains (P. aeruginosa, K. pneumoniae, and methicillin-resistant Staphylococcus aureus (99.9% bactericidal rate)) and negligible cytotoxicity toward mouse embryonic fibroblasts. Therefore, Si@NiO-hydrogel has the potential for use in tissue engineering and biomedical applications owing to its injectability, visible-light crosslink ability, degradability, biosafety, and superior antibacterial property.

Published
2021

31. Cosmic Ray Background Removal With Deep Neural Networks in SBND

Author

J. Asaadi, V. Basque, M. Tripathi, G. Yarbrough, E. Raguzin, G. Scanavini, D. Kalra, Carla Bonifazi, N. McConkey, V. Meddage, A. M. Szelc, H. Ray, I. K. Furic, A. Bhanderi, I. Lepetic, W. C. Louis, M. Worcester, G. Karagiorgi, Vishvas Pandey, J. Spitz, M. Ross-Lonergan, W. Ketchum, L. Mora, T. Ham, B. Zamorano, T. Mettler, Andrew Brandt, O. Goodwin, G. Ge, C. A. Moura, V. A. Kudryavtsev, M. C. Q. Bazetto, A. Holin, Corey Adams, J. A. Nowak, D. P. Méndez, M. Roda, William Tang, M. F. Carneiro, J. I. Crespo-Anadón, L. Bagby, C. Andreopoulos, C. Cuesta, A. Navrer-Agasson, V. Di Benedetto, D. Franco, S. Tufanli, A. Scarff, B.T. Fleming, G. V. Stenico, D. Torretta, Xiaohui Qian, M. Toups, D. W. Schmitz, R. S. Fitzpatrick, H. Frandini, W. C. Griffith, S. Söldner-Rembold, B. Howard, J. Tena Vidal, E. Cristaldo, Ornella Palamara, A. P. Furmanski, S. Gollapinni, John Evans, A. A. Machado, A. Bhat, F. Psihas, R. Acciarri, Jorge Molina, N. J. C. Spooner, V. L. Pimentel, J. Zennamo, A. De Roeck, D. Barker, Roland S.G. Jones, K. Mistry, Joleen Pater, A. C. Ezeribe, Yi Chen, F. Nicolas-Arnaldos, M. Reggiani-Guzzo, M. Soderberg, T. Brooks, A. Schukraft, W. Badgett, D. Mardsen, G. A. Valdiviesso, G. Putnam, Patrick Green, A. Zglam, F. Marinho, I. L. De Icaza Astiz, R. Guenette, D. Brailsford, C. Backhouse, Laura Paulucci, M. Betancourt, A. Mastbaum, J. Mousseau, D. Garcia-Gamez, Jong-Sung Yu, M. Del Tutto, H. S. Chen, K. Mavrokoridis, S. Gao, C. Touramanis, Antonio Ereditato, J. Larkin, M. Soares Nunes, A. Mogan, I. Gil-Botella, M. Stancari, L. Kashur, E. Segreto, E. T. Worcester, M. J. Kim, G. Chisnall, W. Foreman, J. Henzerling, H. Lay, M. Babicz, P. Guzowski, G. de Sá Pereira, M. Mooney, E. Tyley, D. Rivera, C. Mariani, M. Malek, and B. R. Littlejohn

Subjects
Liquid Ar detectors, SBN program, Physics::Instrumentation and Detectors, Astrophysics::High Energy Astrophysical Phenomena, Other Fields of Physics, FOS: Physical sciences, Cosmic ray, 01 natural sciences, physics.data-an, Nuclear physics, Artificial Intelligence, neutrino physics, 0103 physical sciences, Fermilab, 010306 general physics, Projection (set theory), liquid Ar detectors, Original Research, Physics, Multidisciplinary, COSMIC cancer database, 010308 nuclear & particles physics, Detector, deep learning, UNet, Deep learning, QA75.5-76.95, Neutrino physics, Physics - Data Analysis, Statistics and Probability, Electronic computers. Computer science, SBND, Particle, High Energy Physics::Experiment, Neutrino, Event (particle physics), Data Analysis, Statistics and Probability (physics.data-an)
Abstract

The SBND Collaboration acknowledges the generous support of the following organizations: the U.S. Department of Energy, Office of Science, Office of High Energy Physics; the U.S. National Science Foundation; the Science and Technology Facilities Council (STFC), part of United Kingdom Research and Innovation, and The Royal Society of the United Kingdom; the Swiss National Science Foundation; the Spanish Ministerio de Ciencia e Innovación (PID2019-104676GB-C32) and Junta de Andalucía (SOMM17/6104/UGR, P18-FR-4314) FEDER Funds; and the São Paulo Research Foundation (FAPESP) and the National Council of Scientific and Technological Development (CNPq) of Brazil. We acknowledge Los Alamos National Laboratory for LDRD funding. This research used resources of the Argonne Leadership Computing Facility, which is a DOE Office of Science User Facility supported under Contract DEAC02- 06CH11357. SBND is an experiment at the Fermi National Accelerator Laboratory (Fermilab), a U.S. Department of Energy, Office of Science, HEP User Facility. Fermilab is managed by Fermi Research Alliance, LLC (FRA), acting under Contract No. DE-AC02-07CH11359., In liquid argon time projection chambers exposed to neutrino beams and running on or near surface levels, cosmic muons, and other cosmic particles are incident on the detectors while a single neutrino-induced event is being recorded. In practice, this means that data fromsurface liquid argon time projection chambers will be dominated by cosmic particles, both as a source of event triggers and as the majority of the particle count in true neutrino-triggered events. In this work, we demonstrate a novel application of deep learning techniques to remove these background particles by applying deep learning on full detector images from the SBND detector, the near detector in the Fermilab Short-Baseline Neutrino Program. We use this technique to identify, on a pixel-by-pixel level, whether recorded activity originated from cosmic particles or neutrino interactions., U.S. Department of Energy, Office of Science, Office of High Energy Physics, U.S. National Science Foundation, Science and Technology Facilities Council (STFC), The Royal Society of the United Kingdom, Swiss National Science Foundation, Spanish Ministerio de Ciencia e Innovación (PID2019-104676GB-C32), Junta de Andalucía (SOMM17/6104/UGR, P18-FR-4314) FEDER Funds, São Paulo Research Foundation (FAPESP), National Council of Scientific and Technological Development (CNPq) of Brazil, Los Alamos National Laboratory for LDRD, Argonne Leadership Computing Facility, Fermi National Accelerator Laboratory (Fermilab), Fermi Research Alliance, LLC (FRA) DE-AC02-07CH11359

Published
2021

32. Ru-Loaded Graphitized Porous Carbon for High Performance Electrochemical Hydrogen Evolution

Author

Choel-Hwan Shin, Ha-Young Lee, Ted Yu, William Goddard, and Jong-Sung Yu

Abstract

The performance of electrocatalysts is closely related to their supporting materials since their properties such as heteroatom doping, porosity, graphiticity, and electrical conductivity play a decisive role on catalyst performance. We report here the preparation of N-doped highly graphitized porous network-structured carbon (N-HGC) as a catalyst support for Ru nanoparticles (NPs) catalytically active for hydrogen evolution reaction (HER) using pyrolysis of g-C3N4. The as-prepared N-HGC shows high graphiticity confirmed by XRD and Raman analyses, high electrical conductivity, and large surface area along with large amount of open mesopores, containing the proper amount of N doping rich with high pyrrolic-N content for homogeneous distribution of Ru NPs. This Ru/N-HGC catalyst shows a remarkably low overpotential of 9.6 mV (vs RHE) at 10 mA/cm2, which is near ideal and far better than state-of-the-art Pt/C. It also illustrates superb stability, maintaining the HER activity for 200 h and 10k CV cycles without any significant degradation. This superb HER performance is attributed to the robust N-HGC support featuring thin carbon structure, high electrical conductivity, suitable porosity, and N pyrrolic doping. The atomistic basis for the low overpotential is explained via Grand Canonical Quantum Mechanics (GC-QM) calculations. These calculations show that the pyrrolic-N in the support strengthens the coupling to Ru NP and weakens the binding of H to Ru NP, improving the rate determining Tafel reaction.

Published
2022

33. A New TiO with in-Situ Transformed Rutile TiO2 Nanothorns As a Superb Anode Material for Lithium-Ion Battery

Author

Tong-Hyun Kang, Byong-June Lee, and Jong-Sung Yu

Abstract

Developing high-performance anodes is highly desired to meet the recent ever-increasing demands for lithium-ion battery (LIB). Herein we report a uniquely integrated hybrid structure of rutile TiO2 (r-TiO2) nanothorns in situ grown over a new porous and conductive TiO core, which is generated from pyrolysis of anatase TiO2 with Mg metal at 650℃. The new hybrid exhibits superb LIB performance as an anode with high reversible capacity and almost no capacity decay during 1000 cycles at a high current density of 20 C (4000 mA g-1). Two independent reactions of intercalation and pseudocapacitive interaction are confirmed to occur in the composite of the r-TiO2 and TiO, respectively. In particular, the excellent rate capability along with long cycle life enables the new hybrid to have ultrafast charging of the system. Furthermore, the hybrid with the job-sharing property exhibits stable charge-discharge performance over a wider potential window range of 0.01 to 3.0 V, particularly even in the low potential range of 0.01~1.0 V, which usually causes irreversible Li-intercalation and rapid capacity decay for pristine TiO2. All the properties including the wider potential window allows the hybrid to realize the highest electrochemical performance that titanium oxides have ever achieved so far.

Published
2022

34. Controllable Synthesis of N-Doped Single-Layer Graphene-Coated Cobalt Nanoparticles for Efficient Oxygen Evolution

Author

Gisang Park, Choel-Hwan Shin, Joonhee Kang, Kug-Seung Lee, Chunfei Zhang, and Jong-Sung Yu

Abstract

Controllable synthesis of graphene-coated metal nanoparticles (NPs) presents a big challenge because the shell thickness plays a key role in activity of these catalysts. Herein, we use silica as a radical sieve to grow graphene over cobalt NPs via chemical vapor deposition. As-prepared single-layer graphene-coated cobalt NPs with and without N doping (Co@N-SG and Co@SG) exhibit noticeable oxygen evolution reaction (OER) activity of 316 and 334 mV, respectively at a current density of 10 mA cm-2. Furthermore, a magnet-assisted binder-free Co@N-SG electrode illustrates much improved OER activity and stability over conventional binder-assisted counterparts, suggesting this as an effective way to overcome the recognized issues of high electron transfer resistance and poor adhesion of binder-based electrodes in practical applications. Interestingly, the graphene shell possesses varying defects and major OER active sites are found around the defects in the shell. On the other hand, separately isolated Co@SG with a defect-free shell, despite exhibiting a slightly lower initial activity, illustrates a much-improved durable OER performance. The underlying Co affects the electron density of the graphene shell through dipole interaction and the electron density is optimized for adsorption of reaction intermediates, hence accelerating OER performance. This work will provide new clues to design efficient and durable electrocatalysts with further enhanced OER performance.

Published
2022

35. Development of high-energy non-aqueous lithium-sulfur batteries via redox-active interlayer strategy

Author

Byong-June Lee, Chen Zhao, Jeong-Hoon Yu, Tong-Hyun Kang, Hyean-Yeol Park, Joonhee Kang, Yongju Jung, Xiang Liu, Tianyi Li, Wenqian Xu, Xiao-Bing Zuo, Gui-Liang Xu, Khalil Amine, and Jong-Sung Yu

Subjects
Multidisciplinary, General Physics and Astronomy, General Chemistry, General Biochemistry, Genetics and Molecular Biology
Abstract

Lithium-sulfur batteries have theoretical specific energy higher than state-of-the-art lithium-ion batteries. However, from a practical perspective, these batteries exhibit poor cycle life and low energy content owing to the polysulfides shuttling during cycling. To tackle these issues, researchers proposed the use of redox-inactive protective layers between the sulfur-containing cathode and lithium metal anode. However, these interlayers provide additional weight to the cell, thus, decreasing the practical specific energy. Here, we report the development and testing of redox-active interlayers consisting of sulfur-impregnated polar ordered mesoporous silica. Differently from redox-inactive interlayers, these redox-active interlayers enable the electrochemical reactivation of the soluble polysulfides, protect the lithium metal electrode from detrimental reactions via silica-polysulfide polar-polar interactions and increase the cell capacity. Indeed, when tested in a non-aqueous Li-S coin cell configuration, the use of the interlayer enables an initial discharge capacity of about 8.5 mAh cm−2 (for a total sulfur mass loading of 10 mg cm−2) and a discharge capacity retention of about 64 % after 700 cycles at 335 mA g−1 and 25 °C.

Published
2021

36. Self-Templated Formation of Fluffy Graphene-Wrapped Ni

Author

Chunfei, Zhang, Gisang, Park, Byong-June, Lee, Lan, Xia, He, Miao, Jinliang, Yuan, and Jong-Sung, Yu

Abstract

Transition-metal phosphides have gained great importance in the field of energy conversion and storage such as electrochemical water splitting, fuel cells, and Li-ion batteries. In this study, a rationally designed novel fluffy graphene (FG)-wrapped monophasic Ni

Published
2021

37. Tailor-Made Pt Catalysts with Improved Oxygen Reduction Reaction Stability/Durability

Author

Jong-Sung Yu, Tong-Hyun Kang, Kiran Pal Singh, Ha-Young Lee, and Emmanuel Batsa Tetteh

Subjects
chemistry.chemical_classification, Materials science, 010405 organic chemistry, business.industry, Catalyst support, Proton exchange membrane fuel cell, chemistry.chemical_element, General Chemistry, Polymer, Electrolyte, 010402 general chemistry, 01 natural sciences, Durability, Catalysis, 0104 chemical sciences, Renewable energy, chemistry, Chemical engineering, Platinum, business
Abstract

With recent technological advances, the demand for renewable energy is ever growing. Polymer electrolyte membrane fuel cells (PEMFCs) have shown great promise in subduing various environmental and ...

Published
2019

38. Electron transfer interpretation of the biofilm-coated anode of a microbial fuel cell and the cathode modification effects on its power

Author

Bongsu Lim, Juan-Juan Zhou, Yamin Yang, Chansoo Choi, Shao Ke, Guorong Xie, Jong-Deok Park, and Jong-Sung Yu

Subjects
Microbial fuel cell, Materials science, Bioelectric Energy Sources, Flavin Mononucleotide, Biophysics, 02 engineering and technology, Acetates, 01 natural sciences, Redox, law.invention, Electron Transport, chemistry.chemical_compound, Electron transfer, Electricity, law, Nafion, Proteobacteria, Electrochemistry, Physical and Theoretical Chemistry, Electrodes, Clostridium, 010401 analytical chemistry, Cytochromes c, General Medicine, NAD, 021001 nanoscience & nanotechnology, Carbon, Cathode, 0104 chemical sciences, Anode, Marcus theory, Chemical engineering, chemistry, Biofilms, Anaerobic bacteria, 0210 nano-technology, Oxidation-Reduction, Porosity
Abstract

Biofilm-coated electrodes and outer cell membrane-mimicked electrodes were examined to verify an extracellular electron transfer mechanism using Marcus theory for a donor-acceptor electron transfer. Redox couple-bound membrane electrodes were prepared by impregnating redox coenzymes into Nafion films on carbon cloth electrodes. The electron transfer was believed to occur sequentially from acetate to nicotinamide adenine dinucleotide (NAD), c-type cytochrome, flavin mononucleotide (FMN) (or riboflavin (RBF)) and the anode substrate. Excellent polarisation and power density characteristics were contributed by the modification of the cathode with a high-surface-area ordered mesoporous carbon or a hollow core-mesoporous shell carbon. The maximum power density of the microbial fuel cell (MFC) could be improved by a factor of two mainly due to the accelerated electron consumption by modifying the cathode surfaces within three-dimensionally interconnected mesoporous carbon particles, and the anode was coated with a mixed culture of anaerobic bacteria.

Published
2019

39. Observation of electroweak W±Z boson pair production in association with two jets in pp collisions at s=13 TeV with the ATLAS detector

Author

Benjamin Jacque Gutelman, H. Zhang, William Mickael Barbe, Xiang Li, Polina Nechaeva, Mats Joakim Robert Olsson, A. Borisov, Mark Stockton, Yoichi Ikegami, G. Di Gregorio, Daniel Andreas Britzger, Marco Battaglia, Tomas Sykora, L. La Rotonda, Mauro Citterio, Valery Schegelsky, Sabrina Groh, Jorge Andres Lopez Lopez, Massimo Lazzaroni, Simen Hellesund, Bogdan Malaescu, Oldrich Kepka, Alessandra Baas, Armin Michael Nairz, Marzieh Bahmani, Kyungeon Choi, Sebastian Heer, Ondrej Hladik, Tatsumi Koi, Tomas Jakoubek, Krisztian Peters, Laurent Vacavant, Giancarlo Spigo, Kathleen Whalen, Valentinos Christodoulou, T. R. V. Billoud, F. Zhang, Vladimir Zhulanov, Athina Kourkoumeli-Charalampidi, C-Q. Li, Michel Lefebvre, Elliot Reynolds, Edson Carquin, Gabriele Chiodini, Pavel Murin, S. Willocq, Matthew Glenn Kurth, Marco Fraternali, Thibault Guillemin, P. S. Wells, Alexander Melzer, Alan James Taylor, Philip Phillips, Samuel Silverstein, E. Celebi, Chav Chhiv Chau, Philipp Thomas Koenig, Hajime Nanjo, H. H. Williams, Giada Mancini, M. A. Pleier, Qiang Li, Guillermo Nicolas Hamity, Alessandro Calandri, Vincent Croft, Emmerich Kneringer, Donatella Cavalli, U. Mallik, Tamar Zakareishvili, Wendy Taylor, C. A. Lee, Emmanuel Sauvan, Lixin Ma, P. Gadow, Sergey Karpov, Ralf Hertenberger, G. Lehmann Miotto, C. M. Vergel Infante, Nedaa Asbah, Kerim Suruliz, Monika Wielers, Adam Edward Barton, Li Zhou, Eric Lancon, Mohamed Ouchrif, Christopher Willis, Irakli Minashvili, Gabriella Gaudio, Cecilia Tosciri, R. Zou, S. De Castro, Thomas Meideck, Yiming Abulaiti, Joseph Haley, F. Wang, Y. Amaral Coutinho, Y. W. Liu, Vadim Gratchev, Tatiana Lyubushkina, Xuai Zhuang, Samira Hassani, C. Da Via, J. Llorente Merino, Umar Gul, Ian Brock, R. Kowalewski, Lukasz Zwalinski, Andreas Reiss, Masahiro Morinaga, Terry Richard Wyatt, A. T. Watson, Nurcan Ozturk, Stephen Albert Weber, Magdalena Slawinska, Huajie Cheng, Shaojun Sun, D. Golubkov, Jared David Little, Oleg Bulekov, M. Cano Bret, Thomas Trefzger, Daniel Scheirich, Runyu Bi, Daniel Bullock, Ole Røhne, Sheena Schier, D. Camarero Munoz, Peter Kodys, Corentin Allaire, Michal Simon, Steinar Stapnes, Ludovico Pontecorvo, Harish Potti, Yee Chinn Yap, Garabed Halladjian, Klaus Hamacher, Haiping Peng, Bartosz Sebastian Dziedzic, Lorenzo Massa, Christoph Amelung, F. G. Oakham, Josh Moss, Enrique Kajomovitz, M. V. Silva Oliveira, Evgenii Baldin, Louis Helary, Anna Mastroberardino, Bruno Lenzi, David Kirchmeier, Silvia Franchino, A. De Santo, Carsten Dulsen, Stephen Hillier, M.A. Haleem, Luis Hervas, Bjarne Stugu, Venugopal Ellajosyula, D. Boscherini, Miaoran Lu, Knut Oddvar Hoie Vadla, Andrea Sansoni, Frank Siegert, Judith Katzy, Silvia Biondi, Alessia Murrone, Peter Buchholz, Martine Bosman, Sergio Gonzalez-Sevilla, Tatiana Klioutchnikova, Michael Pitt, Jovan Mitrevski, K. F. Di Petrillo, J. L. La Rosa Navarro, Fabrice Balli, Zdenek Dolezal, Mark Sutton, José Salt, Danuta Kisielewska, M. Vicente Barreto Pinto, Carlo Schiavi, Anna Macchiolo, Philipp Mogg, Julia Isabell Djuvsland, Matteo Bedognetti, Matthew Peter Heath, G. A. Chelkov, Abdeslam Hoummada, Laura Jeanty, Yaquan Fang, Patrick Rieck, Benjamin Bordy Tannenwald, Paolo Iengo, Rachel Rosten, E. L. Barberio, Katharina Bianca Jakobi, Max Fredrik Isacson, Judita Mamuzic, Eitan Gozani, Fabrizio Petrucci, P. H. Sales De Bruin, Matthew Berg Epland, Giulia Gonella, Jelena Jovicevic, Janet Dietrich, Lesya Anna Horyn, Tom McCarthy, James Shank, Christian Weiser, Seyed Ruhollah Shojaii, Barbara Liberti, Daniele Madaffari, Uladzimir Kruchonak, Cristian Stanescu, Ovsat Abdinov, Kirill Prokofiev, N. De Groot, Kristian Gregersen, Tobias Bisanz, Tadej Novak, Remco Castelijn, D. P. C. Sankey, Bojan Hiti, Maximilian Hils, Alexey Buzykaev, D. Rousseau, Bo Li, Miha Zgubic, Thomas Philippe Calvet, Yicheng Guo, O. Le Dortz, Liang Li, Francois Vazeille, Ilias Panagoulias, Daniel Marley, Christophe Raymond Goudet, Tord Ekelof, Monica Verducci, L. Zhang, R. Cherkaoui El Moursli, Ruo-yu Shang, Shunichi Akatsuka, Attila Krasznahorkay, Ismet Siral, Dimitrios Iliadis, Cherifa Sabrina Amrouche, Fabio Cardillo, Antonio Ereditato, Colleen Jennifer Treado, F. A. Jimenez Morales, Harinder Singh Bawa, Nathan Allen Grieser, Tina Sfiligoj, Saverio D'Auria, Oliver Stelzer-Chilton, Oliver James Winston, Petter Nilsson, Rachel Maria Avramidou, Yongsun Kim, Andrew D. Hamilton, Arthur James Horton, T. Cuhadar Donszelmann, R. S. Orr, Thomas Alfons Beermann, Daniel Turgeman, Marija Marjanovic, Nikolai Rusakovich, Theodor Christian Herwig, Hongfang Liu, Margherita Primavera, Gabija Zemaityte, Gonzalo Enrique Orellana, Pawel Klimek, Nikola Makovec, Daniel Lawrence Briglin, Dave Charlton, Rachel Hyneman, Pedro Urrejola, Hulin Wang, Igor Gavrilenko, Matteo Bauce, Adam Jinaru, S. V. Zeißner, H. S. Chen, Antonio Limosani, S. H. Robertson, Harshna Jivan, W. Buttinger, C. J. S. Young, Zihao Jiang, Fabrizio Miano, Y. Zhao, Duc Ta, Raymond Brock, Ahmet Bingul, Elzbieta Richter-Was, Meghan Frate, Ryan White, Michal Marcisovsky, Yoav Afik, Adam James Bozson, Martin Aleksa, Giovanni Crosetti, Stefania Antonia Stucci, Andrew Stuart Bell, Patrick Bryant, Giovanna Bruni, Klaus Mönig, Flera Rizatdinova, Sabine Crépé-Renaudin, Stefania Spagnolo, Marzio Nessi, Filomena Sopkova, William Joseph Johnson, Lewis Joseph Wilkins, L. Cerda Alberich, J. G. Panduro Vazquez, Ph. Schune, W-M. Yao, Valerie Susanne Lang, Nikola Lazar Whallon, Masato Aoki, P. A. Delsart, Nicoletta Garelli, Francesco Rubbo, Michael R. Wessels, D. Chakraborty, German D Carrillo-Montoya, Oliver Kortner, Rachael Ann Creager, Paul Jackson, Ozan Arslan, John Derek Chapman, Xanthe Hoad, W. Kozanecki, S. R. Paredes Saenz, Andreas Sogaard, Marcella Capua, Oliver Ricken, Katharina Becker, Marta Lidia Rimoldi, Regina Moles-Valls, L. Manhaes de Andrade Filho, E. Sideras Haddad, Wade Cameron Fisher, David Reikher, Katharina Bierwagen, Jeremy Love, Yuta Sano, Hans Krüger, K. P. Mistry, Nicolas Maximilian Köhler, Kendall Reeves, Daniel Muenstermann, Michael Schernau, Claus Gössling, Benedetto Gorini, Olivier Arnaez, Antonia Strubig, Kevin Varvell, Djamel Eddine Boumediene, Simon Berlendis, Elliot Lipeles, Saleh Sultansoy, Antonio Salvucci, R. Tanaka, Brigitte Vachon, Arthur Eugen Bolz, Noam Hod, Jiancong Zeng, Alexander Held, Thomas Maier, Pavel Tsiareshka, Olga Igonkina, Sarah Jones, Victor Maleev, Karl Jakobs, Jan-Ulf Mjörnmark, James Boyd, G. Mc Goldrick, Frederic Deliot, Tancredi Carli, Roberto Cardarelli, Alessandra Betti, Andrew Geoffrey Foster, Mateusz Dyndal, Serena Palazzo, G. Polesello, Rebecca Hayley Pickles, Archil Durglishvili, N. Kimura, Ralf P. Richter, Y. F. Ryabov, M. Silva, M. H. Klein, Stephen Burke, Stéphane Viel, C. Dallapiccola, Johannes Erdmann, Emily McDonald, Ph. Schwemling, Giuliano Gustavino, Ruchika Nayyar, Ulrike Blumenschein, Sergey Senkin, A. Onofre, Oleh Kivernyk, Jemal Khubua, Stephen Watts, Franz E. Bauer, I. Luise, Ehud Duchovni, James Walder, Robert Leone, Petar Bokan, Silvia Resconi, Mazuza Ghneimat, Tim Adye, Verena Maria Walbrecht, R. D. Kass, Zdenek Hubacek, Giorgio Chiarelli, Ana Cueto, L. Barranco Navarro, Y. Huang, Katsuo Tokushuku, Sylvain Blunier, Tadashi Maeno, R. M. D. Carney, Jens Janssen, Pavel Staroba, Minyu Feng, Marta Maria Perego, Matthew James Sullivan, Mario Sannino, Jaroslav Guenther, Bruno Galhardo, Antonio Giannini, Carlo Enrico Pandini, Joseph Reichert, Markus Schumacher, Mahmoud Alstaty, Nicola Abraham, J. Machado Miguens, Philipp Horn, Eric Drechsler, Leigh Schaefer, Mariel Nelson Pettee, Giorgi Arabidze, D. Shoaleh Saadi, Anjishnu Bandyopadhyay, Thilo Pauly, Sarah Demers, A. Seiden, Matthias Saimpert, James Catmore, Artur Trofymov, Hideki Okawa, Soumya Mohapatra, Gerhard Brandt, Stylianos Angelidakis, Janusz Chwastowski, Sharka Todorova-Nova, Fumiya Yamane, T. Nguyen Manh, Stéphane Jézéquel, S. E. von Buddenbrock, Christian Grefe, Francesco Cirotto, Nicola Semprini-Cesari, Robert Johannes Langenberg, Sven Menke, Mogens Dam, Zuzana Barnovska-Blenessy, Thomas Daubney, L. Di Ciaccio, Mohammad Jawad Kareem, Jan Schaeffer, Evgeniya Cheremushkina, Stewart Patrick Swift, S. Chen, Remi Lafaye, Laurent Serin, Antonio Zoccoli, Jahred Adelman, Alain Bellerive, Takashi Mitani, Anna Lipniacka, Christian Ohm, Alice Polyxeni Morris, Kalliopi Iordanidou, Xiaoguang Yue, H. Hakobyan, Gregor Kramberger, Ewelina Lobodzinska, H. B. Liu, Shaun Roe, X. Y. Zhang, Olga Rezanova, Samuel Calvet, Tairan Xu, Simonetta Gentile, Igor Aleksandrov, J. B. Liu, Gregor Gessner, Alexey Dudarev, Philippe Grenier, Brad Abbott, Erich Varnes, David Lynn, Korbinian Ralf Schmidt-Sommerfeld, Maarten Boonekamp, Ingo Burmeister, Alessandra Forti, Vincent Pascuzzi, Pierre Petroff, Xiangyang Ju, M. Bomben, R. J. Sobie, Evgeniy Khramov, M. Rescigno, Tasneem Rashid, Peter Tornambe, S. P. Y. Yuen, Hiroshi Sakamoto, T. S. Lau, Brian Edward Lindquist, Azzah Aziz Alshehri, Priscilla Pani, Stephen Maxfield, Gianluca Introzzi, Jonathan Bortfeldt, Hantao Ji, Yosuke Takubo, J. A. Aguilar-Saavedra, Michael Ryan Clark, Angela Maria Burger, M. Ghasemi Bostanabad, Fabienne Ledroit-Guillon, Vadim Kantserov, Teng Jian Khoo, Rostislav Konoplich, Kehinde Gbenga Tomiwa, J. E. García Navarro, Yu. A. Tikhonov, Giacinto Piacquadio, R. J. Wang, Rafal Staszewski, Jakub Andrzej Kremer, M. Della Pietra, Konrad Kleinknecht, M. De Beurs, Huacheng Cai, Helio Takai, Romain Kukla, Benjamin Kaplan, Ina Carli, Peter Schacht, Andrew Chegwidden, Kyle Cranmer, F. Costanza, Claudio Ferretti, Soren Stamm, Dimitris Varouchas, Tobias Kupfer, Georgios Zacharis, Alexander Gavrilyuk, Antonio Boveia, Gabriel Palacino, A. T. Doyle, Johannes Balz, Francesco Maria Follega, Wouter Verkerke, Lingshan Xu, Alexey Anisenkov, Nikita Belyaev, Ann Miao Wang, G. Duckeck, Vaclav Vacek, V. Andrei, Federica Legger, Stanislav Pospisil, Shogo Kido, Andrey Kamenshchikov, Michael David Werner, Frank Fiedler, Giovanni Maccarrone, Vaclav Vrba, Radim Slovak, B. R. Mellado Garcia, Sara Ghasemi, Alessandro Mirto, Philippe Mermod, Alexander Sakharov, Aaron Liblong, Nadezda Proklova, Yun Sang Chow, Atanu Pathak, Efstathios Karentzos, S. Farrell, Yang Li, Hasko Stenzel, Teresa Barillari, A. G. Clark, Serhat Istin, Michaela Queitsch-Maitland, Samuel Meehan, Gabriele Sabato, Francesco Giuli, Antonios Leisos, Joost Vossebeld, Wladyslaw Dabrowski, Yuta Okazaki, Yann Coadou, Faig Ahmadov, J. E. Black, Karishma Sekhon, Monica Dobre, Koji Nakamura, Reiner Hauser, Bruce Gallop, Diallo Boye, Manuel Neumann, Aaron Angerami, Alejandro Alonso, Rhys Edward Owen, Alberto Cervelli, Torre Wenaus, Clara Troncon, Haonan Lu, Masaharu Nomachi, Markus Zinser, Robert Keyes, Gaetano Barone, Emery Nibigira, Francesco Gonnella, Mark Neubauer, Frued Erik Braren, P. U. E. Onyisi, Sarah Louise Barnes, D. Paredes Hernandez, Juan Pedro Ochoa-Ricoux, M. Mikuž, Andrea Sciandra, Loan Truong, Marcel Vreeswijk, Frederic Derue, T. Moa, Zeno Dixon Greenwood, Jason Tyler Colt Barkeloo, Sebastian Wahrmund, Lidija Živković, Despoina Sampsonidou, Peter Steinberg, Wei Guo, Andrew Buckley, Anatoli Romaniouk, Horst Severini, Wen-Xu Wang, Susumu Terada, Fred Wickens, Vladimir Smakhtin, Andreas Kugel, J. Del Peso, Luis March, Jeannine Wagner-kuhr, P. F. Giraud, Philipp Jonathan Lösel, Viviana Cavaliere, Marine Kuna, Felix Fidelio Klitzner, Barbara Wosiek, Z. W. 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Gomes, Martin Hoeferkamp, Giuseppe Lerner, Ayda Beddall, Andrea Gaudiello, Andrej Gorišek, Yoshihiro Shimogama, Michael Ughetto, Milos Lokajicek, Craig Blocker, Elisabeth Schopf, Sarah Kate Boutle, T. Dias Do Vale, A. M. Rodríguez Vera, Yahya Tayalati, Theodoros Alexopoulos, Martin Tripiana, Steffen Schmitt, Patrick Czodrowski, Joleen Pater, N. Viaux Maira, Haleh Khani Hadavand, Holger Herr, Daniel Pluth, Thomas James Stevenson, Dimitrii Krasnopevtsev, Andrey Kiryunin, Peter Nemethy, Lorne Levinson, Vladimir Tikhomirov, Ioulian Budagov, Makoto Tomoto, Jiangyong Jia, Kevin Kroeninger, Helen Hayward, Takashi Yamanaka, P. M. Watkins, Elemer Nagy, Shunsuke Honda, David Robinson, J. Tanaka, Kunlin Han, Trevor Vickey, Kenta Uno, Stefan Kluth, A. L. Lionti, Phillip Gutierrez, Y. Hernández Jiménez, Apostolos Tsirigotis, Gregor Herten, Miriam Lucio Martinez, Shlomit Tarem, Nishu Nishu, V. I. Martinez Outschoorn, D. Levin, Snezana Nektarijevic, M. Wu, James Pinfold, Stefania Xella, Helena Santos, Mariusz Przybycien, Fr Pastore, Gavin Grant Hesketh, Timon Heim, D. Rodriguez Rodriguez, Michael Andrew Parker, Tyler James Burch, Frank Filthaut, Jeanette Lorenz, David Milstead, Jia Jian Teoh, Ahmed Bassalat, Kevin Einsweiler, Tiesheng Dai, Dylan Cooper Frizzell, Anne-Isabelle Etienvre, Andrea Messina, Aidan Robson, Benjamin William Allen, Pavel Reznicek, Karsten Köneke, E. von Toerne, Christian Luedtke, Julien Caudron, Ambrosius Thomas Vermeulen, Gustaaf Brooijmans, Per Werner, E. Torró Pastor, Bertrand Laforge, Michael James Fenton, Rachid Mazini, Joyful Elma Mdhluli, Kurt Brendlinger, Valeria Nikolaenko, Serban Constantinescu, Adele Rimoldi, A. P. Colijn, Terutaro Nakamura, G. A. Cowan, Yousuke Kataoka, E. B. F. G. Knoops, L. 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Korn, Chrysostomos Valderanis, Yohei Yamaguchi, Saskia Falke, Oliver Majersky, Michael William Phipps, Dirk Zerwas, Sune Jakobsen, Giacomo Artoni, Jessica Metcalfe, Mihail Chizhov, Bruno Mansoulie, Paul Newman, D. Xu, Miguel Fiolhais, Alexei Klimentov, A. Soloshenko, Thomas Dennis Powell, Reinhard Schwienhorst, Denys Denysiuk, Michael A. Strauss, Steffen Maeland, J. Hrivnac, Anton Wolf, D. Berge, P. Puzo, Iain Alexander Bertram, Alexander David Sherman, Tobias Klingl, Michael Rijssenbeek, Juan Terron, Maximiliano Sioli, Marco Delmastro, Fridolin Dittus, Marco Aurelio Lisboa Leite, Fang-ying Tsai, Fabian Thiele, Miao Liu, G. H. A. Viehhauser, Tomas Davidek, Simone Monzani, Sandrine Laplace, Z. Wang, Chiara Debenedetti, S. González de la Hoz, Bernard Brickwedde, Jean-Francois Grivaz, M. Beretta, Thomas Naumann, Saminder Dhaliwal, Riccardo-Maria Bianchi, Joseph Izen, Ruslan Mashinistov, Quentin Buat, Alessandra Ciocio, K. Sliwa, Kurt Keys Hill, M. Vranjes Milosavljevic, Robert Reed, Michael Düren, Tobias Golling, Stephanie Zimmermann, Adam Bailey, Callum Robert Kilby, Eleni Myrto Asimakopoulou, Peter Sherwood, Pavel Starovoitov, Bernhard Meirose, Cristiano David Sebastiani, M. A. B. do Vale, A. A. Affolder, K. Gellerstedt, Hannah Arnold, Christian Heinz, Antonio Sidoti, Ian Hinchliffe, Carlo Alberto Gottardo, Shikma Bressler, Alexey Myagkov, Mohamad Kassem Ayoub, Arely Cortes-Gonzalez, Alexander Milov, W. K. Brooks, C. J. E. Suster, Steven Goldfarb, R. Bartoldus, Chen Zhou, George Redlinger, Frank Ellinghaus, Christian Johann Riegel, Eirik Gramstad, Nils Krumnack, Claire Gwenlan, Marina Rotaru, Thu Pham, Kouta Onogi, Ishan Pokharel, H. van der Graaf, Athanasios Manousos, Ajit S. Puri, Xin Wu, T. P. A. Åkesson, Jared Gregory Vasquez, Anthony Keith Morley, Peter Wagner, Wasikul Islam, Jozsef Toth, Elena Korolkova, G. N. Taylor, Konstantinos Papageorgiou, Benjamin Brau, Carla Sbarra, Paris Moschovakos, Markus Wobisch, Masahiro Ikeno, Nazim Huseynov, Francisco Anuar Arduh, Stefano Zambito, Jaroslava Schovancova, Wenge Wang, Andrea Dell'Acqua, E. Thomson, Ofir Gabizon, Tim Jones, Giuseppe Mornacchi, Joao Saraiva, Otilia Anamaria Ducu, S. L. Lloyd, Elham E Khoda, Matteo Negrini, S. Rodriguez Bosca, Jeroen Schouwenberg, Seppe Kuehn, Fumiaki Ito, Philip Sommer, Kirill Grevtsov, O. Bessidskaia Bylund, Danijela Bogavac, Tadeusz Kowalski, Bo Liu, Alberto Mengarelli, P. D. Thompson, Jonathan Long, Efe Yigitbasi, S. A. Olivares Pino, Josh Mcfayden, Andrew Pilkington, Vitaliano Chiarella, Bobby Samir Acharya, H. A. Neal, Andrey Ryzhov, Guillaume Unal, A. Artamonov, Daniela Bortoletto, Nello Bruscino, Robert Adam Vallance, Evgeny Starchenko, C. Padilla Aranda, J. Van Nieuwkoop, Mathieu Benoit, Jason Dhia Mansour, Wainer Vandelli, Yuji Yamazaki, Lewis James Armitage, A. M. Deiana, Roman Lysak, Veronika Magerl, Christoph Eckardt, Kun Liu, Alexander Undrus, Calum Michael Macdonald, Steven Patrick Alkire, Simon Henry Connell, Tatsuya Masubuchi, Oliver Keith Baker, Jiri Kvita, Francesco Crescioli, Juan Fuster, Rosanna Ignazzi, Vojtech Pleskot, Nicholas Adam Styles, Federico Meloni, Victoria Jane Martin, Cecile Deterre, John Alison, V. Izzo, Sara Valentinetti, A. Rodriguez Perez, Frank Winklmeier, L. R. Flores Castillo, Emily Charlotte Graham, Luc Poggioli, Christine Kourkoumelis, Pedro Jorge, Mauro Iodice, Lingxin Meng, Ruggero Turra, G. Carlino, Peter Berta, Joe Taenzer, Yong’an Liu, Paolo Massarotti, Andrea Catinaccio, Tsz Yu Ng, S. Li, Junya Usui, Till Eifert, Maia Mosidze, K. H. Hiller, Abner Soffer, Steffen Stärz, Lily Asquith, Jason Lea Oliver, R. C. W. Henderson, Arno Straessner, Monica D'Onofrio, Trygve Buanes, R. Gupta, A. Bruni, M. J. Shochet, Aimilianos Koulouris, Alexandre Rozanov, T. Kobayashi, Daniel Stefaniak Nielsen, Claudio Santoni, Stephen Jiggins, F. S. Merritt, Marco Milesi, Robert Kehoe, Tony Kwan, Baptiste Abeloos, Giordon Stark, Pavel Shatalov, Jochen Dingfelder, Alex Kastanas, Alaettin Serhan Mete, D. V. Dedovich, Amy Selvi Tee, Renat Sadykov, David Martin Bjergaard, Mutsuto Hagihara, Marco Vanadia, I. Nomidis, Chaowaroj Wanotayaroj, Samuel Webb, Robert Les, Jens Weingarten, Robert Wolff, Tony Liss, Oleg Brandt, Knut Zoch, Carl Gwilliam, Debarati Roy, Koichi Nagai, M. Garcia-Sciveres, Yu Nakahama, Nima Sherafati, Y. L. Liu, Paolo Calafiura, Alexander Solodkov, A. E. Dumitriu, Yun-Ju Lu, Lauren Tompkins, L. F. Flores, Jack Henry Lindon, Frederik Rühr, Nabila Wahab Shaikh, Kerstin Lantzsch, S. Shimizu, Milene Calvetti, Kevin Daniel Finelli, Marcin Pawel Guzik, Dominique Pallin, Christos Bakalis, Irena Nikolic-Audit, G. Otero y Garzon, A. S. White, Konstantin Vorobev, Ewa Stanecka, Gregory David Hallewell, Jiri Dolejsi, P. T. E. Taylor, Alastair Dewhurst, Heinz Pernegger, Peter Loch, Alexander Oh, S. Argyropoulos, David South, J. B. De Vivie De Regie, Arunika Sahu, Jan Kretzschmar, Marco Schioppa, John Kenneth Anders, Nicola Orlando, Enrico Tassi, Andrea Bocci, Evangelos Kourlitis, Claire David, H. T. Yang, Ioannis Maznas, B. L. Liu, K. A. Johns, Pingchuan Zhao, David Michael Handl, X. R. Chen, Yi Chen, Tae Min Hong, Teresa Lenz, A. R. Weidberg, P. A. Bruckman de Renstrom, Miriam Diamond, Miguel Arratia, Eleni Mountricha, Didier Lacour, Ondrej Penc, Dustin Biedermann, Benjamin Freund, Isabel Nitsche, Brian Le, Ryszard Stroynowski, Clara Nellist, Jens Dopke, Gokhan Unel, Hisaya Kurashige, R. El Kosseifi, H. L. Zhu, Catrin Bernius, Bakar Chargeishvili, Richard Brenner, Marisa Sandhoff, R. Araujo Pereira, Mariya Shiyakova, Danilo Giugni, Cesare Bini, Otmar Biebel, Zhen Yan, Michael Kagan, Rodney Walker, David Robert Wardrope, Ahmed Hasib, Andreas Honle, Valentina Maria Cairo, Thomas Malte Spieker, Jan Thomas Kuechler, Jesse Heilman, David William Casper, Yang Heng, W. Y. Song, Moritz Kiehn, Forrest Hays Phillips, Peilong Wang, Takuya Nobe, Michael Adersberger, M. Faucci Giannelli, Jonathan Crane, Karol Krizka, Stefan Gadatsch, E. Benhar Noccioli, Ariel Schwartzman, Mathis Kolb, Eftychia Tzovara, Petr Andreevich Gorbounov, Chung-Yau Lo, Paul Miyagawa, A. C. König, Wing Sheung Chan, Jeffrey David Shahinian, Gerjan Bobbink, M. Kuze, Marisilvia Donadelli, Laura Fabbri, Sascha Caron, Vladimir Sulin, J. E. Brau, Christopher Bee, Petr Vokac, Dingane Reward Hlaluku, Stephen Sekula, Xifeng Ruan, Nansi Andari, Lianyou Shan, Richard Nisius, Hideyuki Oide, Dugan O'Neil, Lydia Iconomidou-Fayard, Jacob Martin Pasner, Robert Astalos, Emmanuel Monnier, Alexandru Hostiuc, Madalyn Ann McKay, J-P. Meyer, Konstantin Zhukov, Natascha Savic, Christopher Hayes, Jörgen Sjölin, Andre Sopczak, Melissa Ridel, Deshan Kavishka Abhayasinghe, Sebastien Rettie, Amal Vaidya, Mark Owen, Konstantin Belotskiy, Nuno Filipe Castro, Luigi Marchese, K. J. C. Leney, Dario Barberis, Mykhailo Lisovyi, A. M. Cooper-Sarkar, Stefano Camarda, Brian Thomas Amadio, Antonio Miucci, Tova Ray Holmes, Gunnar Jakel, Liaoshan Shi, Serhat Oerdek, Francesco Lanni, Nikolai Fomin, Filipp Dubinin, Arnaud Ferrari, Marcia Begalli, R. Di Nardo, Jennifer Kathryn Roloff, Rinat Fakhrutdinov, Frederick Dallaire, Nicolo Vladi Biesuz, Elena Rocco, S. Campana, Annabelle Julia Chuinard, Paul Mircea Gravila, M. J. Da Cunha Sargedas De Sousa, Namgyun Jeong, Bijan Haney, Ilya Korolkov, Andrea Knue, Nicolas Morange, H. F.W. Sadrozinski, Laura Rehnisch, Steffen Henkelmann, Tigran Mkrtchyan, Isabelle Wingerter-Seez, Veronica Fabiani, Alessandro Tricoli, Stefan Guindon, Saime Gurbuz, Simone Michele Mazza, Silvia Fressard-Batraneanu, Ljiljana Morvaj, Norbert Wermes, Christophe Clement, Marjorie Shapiro, Cristiano Alpigiani, Soshi Tsuno, T. Kawamoto, Sara Strandberg, Tracey Berry, Marco Aurelio Diaz, Grzegorz Gach, Noemi Calace, Dean T. Yamaguchi, P. Farthouat, Maurice Becker, Bruce Barnett, E. Rizvi, Jonathan Michael Hays, Christopher Lester, Remi Zaidan, Rosy Nicolaidou, Andrew White, Yumeng Cao, Giulio Cornelio Grossi, Matthew John Baca, Tim Martin, Bernhard Matthias Flierl, Vincenzo Canale, Qiaoshi Zeng, C. C. Young, Eduard Simioni, P. H. Hansen, Osamu Jinnouchi, Tai-Hua Lin, Stanislav Nemecek, A. La Rosa, Peter Vankov, Yasuyuki Horii, Ariella Cattai, Tristan Beau, Abigail Alexandra O'Rourke, Nikolina Ilic, P. Sinervo, Mario Campanelli, Borut Paul Kerševan, Stefan Rave, Stephen Gibson, Phillip Urquijo, X. T. Meng, Johanna Gramling, Howard Gordon, Marcel Weirich, P. Francavilla, Maddalena Giulini, Andre Schoening, P. J. Hsu, E. Valdes Santurio, Sigve Haug, Mattias Birman, Joern Grosse-Knetter, Sergio Grancagnolo, Miriam Watson, Anastasia Kurova, A. T. H. Arce, Liron Barak, Geert-Jan Besjes, John Hobbs, Elisabetta Vilucchi, J. A. García Pascual, Emily Claire Hanson, Andrea Coccaro, Leonid Kurchaninov, Peng Zhang, M. J. Oreglia, Geoffrey Gilles, Stefano Rosati, Suvrajeet Sen, Othmane Rifki, Vincenzo Cavasinni, B. Pearson, Aleksandra Dimitrievska, Shigeru Odaka, Elisabeth Petit, Shensheng Han, Rosa Simoniello, Sergey Chekulaev, F. A. Di Bello, I-huan Chiu, Uli Schäfer, Michael Solar, Andre Zibell, E. Bergeaas Kuutmann, Nikita Smirnov, J. Albert, Ankita Mehta, Leszek Adamczyk, Steven Schramm, Michela Biglietti, Emanuele Cavallaro, Julia Lynne Gonski, Miroslav Havranek, Andrew Brandt, Fabrizio Trovato, Pere Rados, S. Díez Cornell, Fernando Marroquim, M. Wittgen, C. A. Johnson, Petr Jacka, Manfredi Ronzani, Zineb Idrissi, Tingting Cao, Francesco Guescini, Fabien Jeanneau, Luca Fiorini, Merve Sahinsoy, J. K. K. Liu, Jan Godlewski, J. Barreiro Guimarães da Costa, Michela Paganini, Michael Bender, Sergey Burdin, Dmitry Emeliyanov, Yasuhiro Makida, Steve McMahon, Robert Gardner, Joaquin Hoya, S. P. Denisov, Martina Laura Ojeda, Zachary Michael Schillaci, Martin Spousta, Kentaro Kawade, Morad Aaboud, Christoph Falk Anders, Maike Christina Hansen, E. K. U. Gross, Göran Jarlskog, Emily Marie Duffield, Valerio Ippolito, Marco Valente, I. P. J. Shipsey, Marc Escalier, Alyssa Montalbano, Jonathan Butterworth, H. Duran Yildiz, Kohei Yorita, Cristinel Diaconu, O. Cakir, Chris Sander, Anna Shcherbakova, Evelin Meoni, Lorenzo Rossini, Ivan Angelozzi, Stefan Stonjek, Mark Hodgkinson, D. M. Portillo Quintero, Alan Peyaud, Magda Anna Chelstowska, Simone Sottocornola, Enrico Junior Schioppa, Henso Abreu, R. E. Long, Q. Ouyang, Evangelos Leonidas Gkougkousis, Pierre Marc Luzi, Sascha Mehlhase, Sergii Raspopov, Yanyan Du, Cyril Becot, Aviv Ruben Cukierman, Cunfeng Feng, Yasushi Nagasaka, R. J. Hawkings, Dave Lewis, Ph Gris, Matt Zhang, I. I. Tsukerman, P. Johansson, William Trischuk, Helge Christoph Beck, Oxana Smirnova, Konstantinos Bachas, R. D. Schamberger, Pascal Pralavorio, Lamberto Luminari, Maciej Trzebinski, Ji Zhu, Stuart Derek Walker, Gabriella Sciolla, Victor Solovyev, Benoit Lefebvre, Thorwald Klapdor-kleingrothaus, Savanna Marie Shaw, J. A. Wilson, M. De Santis, C. A. Solans Sanchez, Tomas Slavicek, J. C. Rivera Vergara, W. Wang, Per Olov Joakim Gradin, J. Jimenez Pena, Jean-Francois Laporte, Andrew Blue, Lidia Dell'Asta, Fabrice Hubaut, Aziz Chafaq, Dmitriy Maximov, I. Turk Cakir, Miroslav Hrabovsky, G. Bernardi, Kazunori Hanagaki, Benjamin Philip Nachman, Rotem Barnea, Iurii Naryshkin, Adelina D'onofrio, Toshiaki Kaji, B. M. Waugh, Claire Antel, Charles Leggett, Fabian Huegging, Rute Pedro, M. Miñano Moya, Lorenz Hauswald, Roger Jones, Atsuhiko Ochi, E. Fullana Torregrosa, James Howarth, M. E. Pozo Astigarraga, Stephen Haywood, Sotirios Vlachos, Walter Lampl, F. Parodi, David Miller, Vladimir Vinogradov, Ece Akilli, Nikiforos Nikiforou, Francesca Ungaro, Christopher Potter, Gabriel Stoicea, A. Tavares Delgado, Davide Costanzo, Claudia Bertella, Lucio Cerrito, Peng Huo, Lara Hannan Mason, and L. Duflot

Subjects
Physics, Nuclear and High Energy Physics, Particle physics, Muon, Luminosity (scattering theory), Large Hadron Collider, 010308 nuclear & particles physics, High Energy Physics::Phenomenology, Electroweak interaction, 7. Clean energy, 01 natural sciences, Pair production, medicine.anatomical_structure, Atlas (anatomy), 0103 physical sciences, medicine, High Energy Physics::Experiment, 010306 general physics, Lepton, Boson
Abstract

An observation of electroweak W±Z production in association with two jets in proton–proton collisions is presented. The data collected by the ATLAS detector at the Large Hadron Collider in 2015 and 2016 at a centre-of-mass energy of s=13 TeV are used, corresponding to an integrated luminosity of 36.1fb−1 . Events containing three identified leptons, either electrons or muons, and two jets are selected. The electroweak production of W±Z bosons in association with two jets is measured with an observed significance of 5.3 standard deviations. A fiducial cross-section for electroweak production including interference effects and for a single leptonic decay mode is measured to be σWZjj−EW=0.57−0.13+0.14(stat.)−0.06+0.07(syst.)fb . Total and differential fiducial cross-sections of the sum of W±Zjj electroweak and strong productions for several kinematic observables are also measured.

Published
2019

40. A facile in-situ activation of protonated histidine-derived porous carbon for electrochemical capacitive energy storage

Author

Jitendra Samdani, Hwa Jung Kim, Bon-Cheol Ku, Jun Yeon Hwang, Jae Kwan Lee, Jong-Sung Yu, and Thanh-Nhan Tran

Subjects
Materials science, General Chemical Engineering, Doping, chemistry.chemical_element, Protonation, 02 engineering and technology, 010402 general chemistry, 021001 nanoscience & nanotechnology, Electrochemistry, 01 natural sciences, 0104 chemical sciences, Chemical engineering, chemistry, Specific surface area, 0210 nano-technology, Pyrolysis, Carbon, Histidine, Power density
Abstract

A unique and effective synthesis approach to tune the structural and electrochemical properties of carbon materials (CMs) is demonstrated by template-free one-step pyrolysis of protonated histidine (His) containing each of different inorganic acids (HAs) such as HI, HBr, HCl, HNO3, H2SO4, and H3PO4. In particular, the (H3PO4)His-CM possesses high specific surface area, high capacitance, superior energy density and power density along with excellent cycle life. Such excellent electrochemical performance of (H3PO4)His-CM is attributed to the tunable structural properties of the precursor, where H3PO4 plays dual roles of in-situ activation and additional P doping in the carbon skeleton.

Published
2019

41. Efficient electrode material for electrochemical energy storage from organic waste

Author

Jong-Sung Yu and Kiran N. Chaudhari

Subjects
Supercapacitor, Battery (electricity), Materials science, Heteroatom, chemistry.chemical_element, Biomass, 02 engineering and technology, 010402 general chemistry, 021001 nanoscience & nanotechnology, Condensed Matter Physics, Electrochemistry, 01 natural sciences, Energy storage, 0104 chemical sciences, Chemical engineering, chemistry, General Materials Science, Electrical and Electronic Engineering, 0210 nano-technology, Carbon, Pyrolysis
Abstract

Heteroatom functionalities in activated carbons have a positive effect on their electrochemical properties. High surface area, reasonable heteroatom content, and high conductivity are highly appealing for energy storage applications, and imparting all three attributes in a single material is still a formidable task. In this work, this task is addressed by using a routinely discarded protein-rich biomass human hair. It offers a unique prospect as a single precursor for heteroatoms and carbon. Highly functional N and S-co-doped carbons generated by pyrolysis at 800, 900, and 1000 °C yield variable degree of heteroatoms, surface areas, and conductivities. When applied as an electrode material for Li-ion battery and supercapacitor, interestingly, the carbon generated at 900 °C shows better electrochemical performance over its counterparts. A correlative analysis of the structural features and performance is presented.

Published
2019

42. Search for light resonances decaying to boosted quark pairs and produced in association with a photon or a jet in proton–proton collisions at s=13TeV with the ATLAS detector

Author

Kerstin Jon-And, Yanjun Tu, J. Silva, Kiyotomo Kawagoe, Daniel Guest, Yulia Rodina, Martin Hoeferkamp, Tairan Xu, Giuseppe Lerner, Carl Jeske, Michael Ughetto, Milos Lokajicek, F. Marroquim, Chris Sander, Anna Shcherbakova, Grigori Rybkin, Miroslav Myska, Michael Andrew Parker, Tyler James Burch, Edmund Dawe, Marco Sessa, Bellisario Esposito, Frank Merritt, Liang Guan, Tobias Bisanz, Remco Castelijn, Bojan Hiti, Wendy Taylor, Ralf Hertenberger, Peter Onyisi, Nimrod Taiblum, Till Eifert, K. K. Gan, R. Nagai, Blake Burghgrave, Evelin Meoni, Ivan Angelozzi, Stefan Stonjek, K. H. Yau Wong, A. Di Girolamo, Calin Alexa, P. Dita, Pedro Urrejola, Vakhtang Tsulaia, Michal Suk, Alexander Zaitsev, Petr Andreevich Gorbounov, Irakli Minashvili, Danuta Kisielewska, T. Vazquez Schroeder, James Boyd, Didier Ferrere, Takahiro Fusayasu, Odette Benary, Marcus Morgenstern, S. Donati, Abner Soffer, Marco Costa, Trisha Farooque, Steffen Stärz, Marco Bruschi, Lily Asquith, Mikhail Levchenko, M. Franklin, Paul Newman, T. Ženiš, Manuel Neumann, Philippe Calfayan, P. van Gemmeren, Henrik Oppen, Jing Wang, Juraj Bracinik, Jochen Meyer, I. Santoyo Castillo, Gabriel John Facini, Michel Janus, Valerio Bortolotto, Emily Nurse, Elizabeth Gallas, G. Costa, Yury Ryabov, Ioannis Gkialas, Dirk Duschinger, Nico Giangiacomi, Laurent Serin, Sau Lan Wu, Edgar Kellermann, Andrew Chisholm, Kaushik De, Damir Duvnjak, Dmitri Dedovich, Peter Davison, Georgios Iakovidis, Daniela Boerner, Mariya Shiyakova, Mikhail Demichev, Oleg Kuprash, Marcelo Vogel, A. Ezhilov, Rodger Mantifel, Ping-Kun Teng, Jan Stark, D. A. Soh, L. A. M. Wiik-Fuchs, Henry Lubatti, Marta Maria Perego, E. Yu. Soldatov, Raquel Pezoa, Louis D'eramo, K. O. H. Vadla, Carlo Schiavi, Allan G Clark, Roger Moore, Anna Macchiolo, Pavel Podberezko, Siegfried Bethke, Caterina Doglioni, Stanislav Tokár, Jean-Francois Grivaz, J. Ocariz, Philipp Mogg, Julia Isabell Djuvsland, Matteo Bedognetti, Kotaro Wakamiya, Simone Michele Mazza, Trine Poulsen, P. de Jong, Christopher Samuel Pollard, C. Malone, Mark Hodgkinson, Alena Loesle, Jiri Chudoba, D. M. Portillo Quintero, Tomoya Iizawa, Alan Peyaud, Magda Anna Chelstowska, Jorg Wotschack, Simone Sottocornola, Henso Abreu, Henrik Ohman, Y. Zhang, V. Boisvert, Stephanie Majewski, Tingting Wang, Matteo Mantoani, Stefania Spagnolo, Daniel Muenstermann, Marco Milesi, C. J. S. Young, G. Lehmann Miotto, Pietro Albicocco, Robert J. Bielski, Jun Su, Ren-You Zhang, Jelena Krstic, Joseph Haley, Nikola Lazar Whallon, Ruggero Turra, Mohamed Ouchrif, Cristiano Alpigiani, Hans Krüger, K. P. Mistry, Nicolas Maximilian Köhler, Alessandro Polini, Michael Ziolkowski, Alfred Goshaw, Roman Lysak, Michaela Mlynarikova, Christoph Eckardt, D. Amidei, Kun Liu, Kunihiro Nagano, Speranza Falciano, Olivier Arnaez, Carolyn Bertsche, A. Rodriguez Perez, Elliot Lipeles, Saleh Sultansoy, F. Wang, Y. Amaral Coutinho, Adrian Buzatu, Otmar Biebel, Amelia Jean Brennan, Ulrich Parzefall, Scott Snyder, Michael Homann, Carlos Lacasta, Masaya Ishino, R. Goncalves Gama, Michael Adersberger, Orjan Dale, Antonio Salvucci, Luiz Caloba, Laurent Schoeffel, Y. W. Liu, Alessandra Betti, Mateusz Dyndal, Ewelina Lobodzinska, H. B. Liu, William Brooks, Kerim Suruliz, Nikolaos Karastathis, Monika Wielers, Li Zhou, Eric Lancon, Wing Sheung Chan, Gerjan Bobbink, Alexey Boldyrev, Yuji Minegishi, J. W. Smith, Wladyslaw Dabrowski, Ehud Duchovni, Mario Antonelli, Kyungeon Choi, Elisa Guido, P. Teixeira-Dias, Antonia Strubig, Gian Luigi Alberghi, Jonathan Bortfeldt, David Berge, Evangelos Leonidas Gkougkousis, Pierre Marc Luzi, Sascha Mehlhase, Sergii Raspopov, Cyril Becot, Aviv Ruben Cukierman, Cunfeng Feng, Yasushi Nagasaka, R. J. Hawkings, Dave Lewis, Abbas Kenan Ciftci, Dave Robinson, Remi Lafaye, Radim Slovak, B. R. Mellado Garcia, Johannes Erdmann, Michael Ryan Clark, Christopher Willis, Manuela Campanelli, Matthew Edgar Leblanc, Elizabeth Brost, Alexandre Glazov, Tobias Flick, Gabriele D'amen, Laurent Vacavant, A. C. Taylor, Fumiaki Ito, Philip Sommer, Joe Taenzer, Andrea Catinaccio, Jens Weingarten, Robert Wolff, Andrej Filipcic, Marisilvia Donadelli, Yingchun Zhu, John Rutherfoord, F. Meloni, Val O'Shea, Darren Temple, Carl Gwilliam, Huacheng Cai, Reiner Hauser, Bruce Gallop, Xiaohu Sun, Sara Ghasemi, Alessandro Mirto, Philippe Mermod, Michael Stoebe, Michel Vetterli, Heidi Sandaker, Steve Muanza, R. Cherkaoui El Moursli, Dimitrios Sampsonidis, Imma Riu, Rebecca Anne Linck, J. Manjarres Ramos, Denys Denysiuk, F. De Lorenzi, Margherita Primavera, Manfredi Ronzani, Nicola Abraham, J. Machado Miguens, Hideyuki Oide, Dugan O'Neil, Enrico Pasqualucci, J. S. Webster, Daniel M. Levin, Stefan Simion, Andrea Sansoni, B. 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Da Cunha Sargedas De Sousa, Alexander Melzer, David Dodsworth, Helge Christoph Beck, Sergio Gonzalez-Sevilla, Oxana Smirnova, Athina Kourkoumeli-Charalampidi, Fabrizio Scuri, Sergey Peleganchuk, Ikuo Ueda, Christopher Lester, Remi Zaidan, Djamel Eddine Boumediene, Matthias Saimpert, James Catmore, Artur Trofymov, Ina Carli, Felix Rauscher, Peter Schacht, Richard Mount, Paolo Morettini, Marcin Pawel Guzik, Peter Loch, Fabienne Ledroit-Guillon, Konstantinos Bachas, Vadim Kantserov, Alan James Taylor, Philip Phillips, Samuel Silverstein, Chav Chhiv Chau, Teng Jian Khoo, Rostislav Konoplich, Alexandru Hostiuc, Kathy Pommès, Vojtech Pleskot, Mark Owen, Nikola Makovec, Joe Kroll, S. Argyropoulos, Andreas Redelbach, Alexander Paramonov, Priscilla Pani, Stephen Maxfield, Stephen Hillier, J. B. 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Capeans Garrido, Yu Nakahama, Philip James Clark, Christophe Clement, Michal Svatos, Iacopo Vivarelli, John Baines, Michael David Werner, Ioannis Nomidis, Alexey Myagkov, Luc Poggioli, Antonio Sbrizzi, Sergei Chekanov, Nabila Wahab Shaikh, Rute Pedro, Kerstin Lantzsch, Lorenz Hauswald, Roger Jones, Giuseppe Iacobucci, Gorm Aske Gram Krohn Galster, Diego Casadei, Archil Durglishvili, Werner Wiedenmann, Peter Vankov, Yasuyuki Horii, Soeren Prell, Simon Molander, Halina Abramowicz, Yuriy Ilchenko, Bradley Axen, Tristan Beau, X. T. Meng, Johanna Gramling, Howard Gordon, Marcel Weirich, E. Plotnikova, Julian Glatzer, Ksenia Gasnikova, J. A. García Pascual, Federico Scutti, Stewart Martin-Haugh, H. Bahrasemani, Daniel Whiteson, Rachael Ann Creager, Paul Jackson, Ozan Arslan, Uli Schäfer, Michael Solar, U. Gul, Andre Zibell, Andreas Warburton, Qun Ouyang, Faten Hariri, Reda Tafirout, Klaus Kurt Desch, Richard Nickerson, Julia Hrdinka, Sanmay Ganguly, E. Bergeaas Kuutmann, G. 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Pacheco Pages, Nguyen Phuong Dang, Hidetoshi Otono, L. Manhaes de Andrade Filho, Hrachya Hakobyan, Alevtina Shmeleva, Milena Bajic, Takashi Kubota, Michael Ernst, Raphael Vuillermet, Martina Javurkova, Claudia Glasman, Savannah Jennifer Thais, Rosy Nicolaidou, Kurt Brendlinger, Yoshiji Yasu, Yoram Rozen, Nora Emilia Pettersson, Margaret Susan Lutz, Oliver Majersky, Liqing Zhang, F. Luehring, O. Estrada Pastor, Brinick Simmons, Louise Heelan, Daniel Froidevaux, Fabio Tresoldi, C. S. Rogan, Davide Melini, B. Di Girolamo, Y. Sakurai, James Mueller, Junichi Tanaka, A. Bethani, A. Valero, Sune Jakobsen, Giacomo Artoni, Jessica Metcalfe, D. I. Narrias Villar, M. J. Shochet, Aimilianos Koulouris, Alexandre Rozanov, Claudio Santoni, A. Soloshenko, Reinhard Schwienhorst, T. M. H. Wolf, Katharina Maria Ecker, Giordon Stark, Pavel Shatalov, Jochen Dingfelder, Mauro Dell'Orso, Matthias Schott, Maximilian Swiatlowski, C. Haber, Hai Jiang, Alex Kastanas, Alaettin Serhan Mete, Francesco Conventi, Junichi Kanzaki, Sabrina Perrella, Joao Seixas, Chaowaroj Wanotayaroj, G. J. Besjes, Nima Sherafati, Pierfrancesco Butti, Takuya Honda, Y. L. Liu, Salvatore Bruno, Cheng-Chieh Peng, S. M. Weber, Tomáš Javůrek, David Calvet, David Sosa, Horst Oberlack, Jakub Andrzej Kremer, Gregory David Hallewell, Elvedin Tahirovic, Jiri Dolejsi, P. T. E. Taylor, Alastair Dewhurst, Heinz Pernegger, Alexander Oh, M. Della Pietra, Barbara Liberti, Ben Waugh, Yang Li, Teresa Barillari, Andrew Lankford, Els Koffeman, Sai-Juan Chen, R. Debbe, Hisaya Kurashige, R. El Kosseifi, Philipp Jonathan Lösel, Marine Kuna, Ryo Tanioka, Zhen Yan, Michael Kagan, Rodney Walker, Victor Kukhtin, Marcela Mikestikova, Stefan Richter, Chris Malena Delitzsch, Qing Wang, Sergey Senkin, Bo Liu, Veysi Erkcan Ozcan, A. De Maria, J. Lacey, J. Boudreau, Krzysztof Woźniak, M. N. K. Smith, Ian Michael Snyder, Giovanni Siragusa, Henri Bachacou, Daniel Fournier, P. D. Thompson, Dj. Sijacki, Joshuha Thomas-Wilsker, Sooraj Krishnan Radhakrishnan, Jonathan Long, Tomoaki Nakamura, Efe Yigitbasi, S. A. Olivares Pino, Josh Mcfayden, Andrew Pilkington, Vitaliano Chiarella, Bobby Samir Acharya, Sophie Henrot-Versille, H. A. Neal, Felix Mueller, R. E. Ticse Torres, Jessica Levêque, A. J. Beddall, P. Mättig, Andrey Ryzhov, Stefano Manzoni, F. La Ruffa, Guillaume Unal, A. Artamonov, Shoji Asai, Daniela Bortoletto, Sabina Czekierda, Seog Oh, Nello Bruscino, Daiki Yamaguchi, Thomas Lohse, Z. Xi, Evgeny Starchenko, C. Padilla Aranda, Karl Heinz Hiller, Mathieu Benoit, Jason Dhia Mansour, Yuji Yamazaki, Lewis James Armitage, Veronika Magerl, Metin Arik, Alexander Undrus, Calum Michael Macdonald, Simon Henry Connell, Paolo Calafiura, Xin Chen, Alexander Solodkov, Yun-Ju Lu, Lauren Tompkins, Alessandra Doria, Elvira Rossi, Kevin Daniel Finelli, Irena Nikolic-Audit, G. Otero y Garzon, Tatsuya Masubuchi, Oliver Keith Baker, Francesco Crescioli, A. S. White, Konstantin Vorobev, Marlon Barbero, David South, Evangelos Kourlitis, Ioannis Maznas, David Michael Handl, Nuno Anjos, Yi Chen, Tae Min Hong, Teresa Lenz, P. A. Bruckman de Renstrom, Cecile Deterre, John Alison, Sara Valentinetti, Frank Winklmeier, L. R. Flores Castillo, Emily Charlotte Graham, Christine Kourkoumelis, Alberto Mengarelli, Pedro Jorge, Jeanette Lorenz, R. Bartoldus, Chen Zhou, Dimitrios Fassouliotis, George Redlinger, Christian Johann Riegel, Anatoly Borisov, Eirik Gramstad, Farkhad Khalil-zada, Addolorata Farilla, Gvantsa Mchedlidze, H. J. Cheng, Sarah Heim, Lingxin Meng, Kouta Onogi, Yanyan Du, T. P. A. Åkesson, Jared Gregory Vasquez, Anthony Keith Morley, Peter Wagner, Jozsef Toth, Elena Korolkova, Claudio Luci, Paris Moschovakos, Markus Wobisch, Masahiro Ikeno, Paolo Francavilla, Stefano Zambito, Maia Mosidze, Robert Clarke, Andrea Dell'Acqua, Vakhtang Kartvelishvili, Tim Jones, Giuseppe Mornacchi, Joao Saraiva, Otilia Anamaria Ducu, O. Bessidskaia Bylund, Ricardo Piegaia, Danijela Bogavac, Tadeusz Kowalski, Wainer Vandelli, Tomas Blazek, Mauro Iodice, Sabine Elles, Junya Usui, Manuel Patrice Geisler, Jiri Hejbal, Vadim Bednyakov, Fabian-Phillipp Tepel, Laurelle Maria Veloce, Ryuichi Takashima, D. Schaefer, Simon Schmitz, Marcello Bindi, Matteo Scornajenghi, Ryan Reece, Andreas Christian Dudder, Petr Tas, Laura Gonella, Stefano Veneziano, Daniel Mauricio Rauch, Ricardo Abreu, Chilufya Mwewa, Daniel Mori, F. M. Giorgi, S. P. Mc Kee, Lorenzo Paolozzi, Reisaburo Tanaka, Livio Mapelli, Guido Volpi, Luc Goossens, Bianca Osculati, Itsuo Nakano, Timothy Michael Bristow, Harald Fox, Lashkar Kashif, Rose Elisabeth Ardell, Sophio Pataraia, Stylianos Angelidakis, Ladislav Chytka, Vassili Kazanin, Michael Holzbock, Peter Watkins, Fred Loebinger, Samina Jabbar, Edisher Tskhadadze, Mirkoantonio Casolino, Theodor Christian Herwig, Leonardo Paolo Rossi, Marzio Nessi, Jeremy Love, Kendall Reeves, R. M. D. Carney, Jens Janssen, Pavel Staroba, Minyu Feng, Sarah Demers, Wayne Allen Cribbs, Gaetano Barone, Vincenzo Izzo, Francesco Gonnella, Mark Neubauer, Frued Erik Braren, Sarah Louise Barnes, Valentina Cairo, Huaqiao Zhang, Rolf Seuster, Benjamin Weinert, G. Eigen, Mirta Dumancic, F. Safai Tehrani, Gavin Grant Hesketh, John Kenneth Anders, Yorihito Sugaya, B. Di Micco, Simon George, N. Lorenzo Martinez, Alexander Bogdanchikov, J. Urban, Sami Kama, Serena Palazzo, Ben William Whitmore, R. F. Naranjo Garcia, Shan Jin, M. zur Nedden, Sandra Leone, Marek Palka, Mohammed Ezzi, Ivor Fleck, E. Yatsenko, Florian Bauer, Patrick Czodrowski, Joleen Pater, Edoardo Gorini, N. Viaux Maira, Vladimir Tikhomirov, Ioulian Budagov, Makoto Tomoto, Takuya Tashiro, D. della Volpe, Juan Pedro Araque, Eduard Kladiva, L. Aperio Bella, Simone Monzani, Guido Gagliardi, Richa Gupta, Davide Gerbaudo, Peter Bussey, Alex Martyniuk, Shohei Shirabe, Marie-Hélène Genest, Ivan Pogrebnyak, Ruth Magdalena Jacobs, Alessandro Lapertosa, Elias Ruttinger, Shu Li, Luigi Longo, Vincent Garonne, Sandro Palestini, L. Feremenga, A. Sanchez Pineda, Alexey Antonov, Pamela Ferrari, Sw. Banerjee, Simona Serena Bocchetta, Zvi Hirsh Citron, P. Hanke, Vasiliki A Mitsou, Leonid Gladilin, Deepak Kar, Davide Boscherini, Stefania Xella, Fr Pastore, Ahmed Bassalat, Kevin Einsweiler, Ambrosius Thomas Vermeulen, Eitan Gozani, Fabrizio Miano, J. G. Panduro Vazquez, Xuan Zhang, Yuta Sano, Jiancong Zeng, Antonio Zoccoli, John Hill, Jahred Adelman, Alain Bellerive, Takashi Mitani, Anna Lipniacka, Christian Ohm, Michael David Beattie, Imran Yusuff, Gregor Kramberger, Despoina Sampsonidou, Peter Steinberg, Wei Guo, Anatoli Romaniouk, Horst Severini, Wen-Xu Wang, Stephen Jacob Sekula, Susumu Terada, Vladimir Smakhtin, Andreas Kugel, Luis March, Jeannine Wagner-kuhr, J. Chen, Junjie Zhu, Gabriel Alexandru Popeneciu, Marcel Vos, Andrew Washbrook, A. Schoening, Hubert Kroha, Hong Ma, Lara Katharina Schildgen, Cheng Guang Zhu, Calliope Louisa Sotiropoulou, Lidia Smirnova, Laurent Chevalier, Tetiana Hryn'ova, and Y. L. Chan

Subjects
Quark, Physics, Nuclear and High Energy Physics, Large Hadron Collider, Photon, 010308 nuclear & particles physics, Astrophysics::High Energy Astrophysical Phenomena, Dark matter, Resonance, 01 natural sciences, Nuclear physics, 0103 physical sciences, Mass spectrum, Substructure, High Energy Physics::Experiment, 010306 general physics, Boson
Abstract

This Letter presents a search for new light resonances decaying to pairs of quarks and produced in association with a high- pT photon or jet. The dataset consists of proton–proton collisions with an integrated luminosity of 36.1 fb −1 at a centre-of-mass energy of s=13 TeV recorded by the ATLAS detector at the Large Hadron Collider. Resonance candidates are identified as massive large-radius jets with substructure consistent with a particle decaying into a quark pair. The mass spectrum of the candidates is examined for local excesses above background. No evidence of a new resonance is observed in the data, which are used to exclude the production of a lepto-phobic axial-vector Z′ boson.

Published
2019

43. Mesopore Channel Length Control in Ordered Mesoporous Carbon Hosts for High Performance Lithium-Sulfur Batteries

Author

Dae-Soo Yang, Tong-Hyun Kang, Byong-June Lee, Jong-Sung Yu, Hyean-Yeol Park, and Seongpil Hwang

Subjects
Materials science, Renewable Energy, Sustainability and the Environment, 02 engineering and technology, 010402 general chemistry, 021001 nanoscience & nanotechnology, Condensed Matter Physics, 01 natural sciences, 0104 chemical sciences, Surfaces, Coatings and Films, Electronic, Optical and Magnetic Materials, Chemical engineering, Mesoporous carbon, Materials Chemistry, Electrochemistry, Lithium sulfur, 0210 nano-technology, Mesoporous material, Communication channel
Published
2018

44. H-doped TiO2-x prepared with MgH2 for highly efficient solar-driven hydrogen production

Author

Ha-Young Lee, Samuel S. Mao, Jong-Sung Yu, Shaohua Shen, and Apurba Sinhamahapatra

Subjects
Materials science, Hydrogen, Process Chemistry and Technology, Doping, chemistry.chemical_element, Nanoparticle, 02 engineering and technology, 010402 general chemistry, 021001 nanoscience & nanotechnology, Photochemistry, 01 natural sciences, Decomposition, Oxygen, Catalysis, 0104 chemical sciences, chemistry, 0210 nano-technology, Absorption (electromagnetic radiation), General Environmental Science, Visible spectrum, Hydrogen production
Abstract

Efficient utilization of visible light with high stability remains a critical challenge for solar-driven photochemical generation of hydrogen (H2) using particulate photocatalysts. Black TiO2 was introduced with remarkable enhancement of visible light absorption, but its efficiency in the visible light has not reached the desired level for real-world applications. Here we report a gold-colored H-doped TiO2-x (H:TiO2-x) nanoparticles prepared by controlled reduction via simultaneous presence of [Mg] and [H], which are obtained from the decomposition of MgH2. The H-doped TiO2-x exhibits a significant activity (16.1 mmolg−1h−1) and remarkable stability after Pt deposition for solar-driven H2 generation from methanol-water. The excellent photoactivity of H-doped TiO2 can be attributed to oxygen vacancies and H doping at the reduced TiO2-x surface generated by [Mg] and [H]. The H-doped TiO2 is also producing H2 from methanol-seawater with a rate of 6.1 mmolg−1h−1 under simulated sunlight.

Published
2018

45. Heterostructured Titanium Oxynitride-Manganese Cobalt Oxide Nanorods as High-Performance Electrode Materials for Supercapacitor Devices

Author

Jitendra Samdani, Sangaraju Shanmugam, Jong-Sung Yu, Tong-Hyun Kang, Yun Hee Jang, and Byong-June Lee

Subjects
Supercapacitor, Materials science, chemistry.chemical_element, 02 engineering and technology, Electrolyte, 010402 general chemistry, 021001 nanoscience & nanotechnology, 01 natural sciences, 0104 chemical sciences, chemistry.chemical_compound, chemistry, Chemical engineering, Electrode, Propylene carbonate, General Materials Science, Nanorod, 0210 nano-technology, Cobalt oxide, Current density, Titanium
Abstract

Metal oxynitrides have been considered recently as emerging electrode materials for supercapacitors. Herein, we converted titanate nanotubes into a series of titanium oxynitride (TiON) nanorods at nitridation temperatures of 800, 900, and 1000 °C in ammonia gas and tested them as supercapacitor electrodes. TiON-800, TiON-900, and TiON-1000 showed capacities of 60, 140, and 71 F g-1, respectively, at a current density of 1 A g-1. However, because of TiON's low capacity, a heterostructure (TiON-900/MnCo2O4) was designed based on the optimized TiON with MnCo2O4 (MCO). The heterostructure TiON-900-MCO and MCO electrode materials showed specific capacities of 515 and 381 F g-1, respectively, at a current density of 1 A g-1. The cycling stability retention of TiON-900 and MCO were 75 and 68%, respectively; moreover, the heterostructure of TiON-900-MCO reached 78% at a current density of 5 A g-1 over 5000 cycles. The increased capacity and sustained cycling stability retention are attributable to the synergistic effect of TiON-900 and MCO. A coin cell (CC)-type symmetric supercapacitor prototype of TiON-900-MCO was fabricated and tested in the voltage range of 0.0-2.0 V in 1 M LiClO4 in propylene carbonate/dimethyl carbonate electrolyte, and a 79% cycling retention capacity of TiON-900-MCO-CC was achieved over 10 000 cycles at a current density of 250 mA g-1. We demonstrated a prototypical single cell of TiON-900-MCO-CC as a sustained energy output by powering a red-light emitting diode that indicated TiON-900-MCo electrode materials' potential application in commercial supercapacitor devices.

Published
2020

46. Study of scintillation light collection, production and propagation in a 4 tonne dual-phase LArTPC

Author

P. Lutz, K. Sakashita, F. Dulucq, L. Periale, F. Noto, Kai Loo, N. Lira, Wladyslaw Henryk Trzaska, J. Marteau, Y. Karyotakis, D. Mladenov, G. Martin-Chassard, G. Lehmann-Miotto, Marzio Nessi, D. Lorca, J. Bremer, Enrique Calvo, M. Kurokawa, C. Regenfus, Antonio Ereditato, N. Geffroy, F. Duval, K. Fusshoeller, Ionel Lazanu, G. Brunetti, K. Negishi, C. Drancourt, A. Scarpelli, V. Toboaru, A. Tonazzo, F. Pietropaolo, T. Hasegawa, A. Gendotti, F. Vannucci, L. Zambelli, K. Nakayoshi, A. Gallego-Ros, F. Doizon, V. Aushev, T. Patzak, C. Cantini, J. Asaadi, E. Pennacchio, André Rubbia, J. Soto-Oton, I. Gil-Botella, L. Balleyguier, Masatoshi Maki, Denis Stanca, S. Bordoni, T. Viant, S. Horikawa, A. Chiriacescuf, A. Falcone, K. Sendai, S. Murphy, B. Aimard, A. Delbart, D. Caiulo, N. Bourgeois, S. Vilalte, B.M. Cautisanu, G. Maire, D. Stefan, L. Brunetti, I. Kreslo, S. Wu, Marc Weber, K. Cankocak, Mihai Niculescu-Oglinzanu, D. Redondo, J. Sinclair, Filippo Resnati, F. Sergiampietri, M. Parvu, D. Kryn, I. De Bonis, Animesh Chatterjee, B. Radics, B. Bourguille, Paolo Crivelli, C. de la Taille, M. Leyton, S. Bolognesi, P. Gorodetzky, Mario Campanelli, M. Calin, M. Chalifour, L. Aizawa, D. Pugnere, Alexandru Gherghel-Lascu, C. Alt, D. Duchesneau, Masahiro Ikeno, S. Shahsavarani, H. Konari, P. Cotte, J.V. Dawson, Federico Sanchez, Diana Navas-Nicolas, S. Jiménez, Y. Penichot, M. Zito, C. Girerd, L. Urda, A. Remoto, B. Carlus, C. M. Schloesser, Tomohisa Uchida, G. Brown, W. Tromeur, R. Sulej, E. Bechetoille, G. Misitano, Romul Margineanu, Masashi Tanaka, S. Conforti, C. Santos, Sampsa Vihonen, A. Verdugo, A. Saftoiu, H. Pessard, H. Mathez, P. Chiu, T.S. Mosu, R. Hanni, A.M. Blebea-Apostu, V. Galymov, Y. Onishchuk, E. Mazzucato, G. Vasseur, S. Narita, Y. Kuromori, Jukka Maalampi, Martin Auger, S. Di Luise, L. Molina Bueno, D. Autiero, A. Holin, S. Kasai, Nikolaos Charitonidis, M. Karolak, M. Shoji, A. Noury, Alexandru Jipa, G. Balik, P. Kunze, W. Mu, D. Belver, Jong-Sung Yu, C. Palomares, A. Chappuis, Katsuyu Kasami, C. Lastoria, M.C. Gomoiu, Thorsten Lux, Laura Manenti, E. Hamada, S. Emery, Alexandru Balaceanu, C. Cuesta, Oana Ristea, T. Kishishita, Laboratoire d'Annecy de Physique des Particules (LAPP), Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS), Institut de Physique des 2 Infinis de Lyon (IP2I Lyon), Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Claude Bernard Lyon 1 (UCBL), Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS), Département de Physique Nucléaire (ex SPhN) (DPHN), Institut de Recherches sur les lois Fondamentales de l'Univers (IRFU), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay, Organisation de Micro-Électronique Générale Avancée (OMEGA), École polytechnique (X)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3), AstroParticule et Cosmologie (APC (UMR_7164)), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Centre National de la Recherche Scientifique (CNRS)-Université de Paris (UP), Université Claude Bernard Lyon 1 (UCBL), Université de Lyon-Université de Lyon-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Centre National de la Recherche Scientifique (CNRS), Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-École polytechnique (X)-Centre National de la Recherche Scientifique (CNRS), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Centre National de la Recherche Scientifique (CNRS)-Université Paris Cité (UPCité), Aimard, B, Aizawa, L, Alt, C, Asaadi, J, Auger, M, Aushev, V, Autiero, D, Balaceanu, A, Balik, G, Balleyguier, L, Bechetoille, E, Belver, D, Blebea-Apostu, A, Bolognesi, S, Bordoni, S, Bourgeois, N, Bourguille, B, Bremer, J, Brown, G, Brunetti, L, Brunetti, G, Caiulo, D, Calin, M, Calvo, E, Campanelli, M, Cankocak, K, Cantini, C, Carlus, B, Cautisanu, B, Chalifour, M, Chappuis, A, Charitonidis, N, Chatterjee, A, Chiriacescuf, A, Chiu, P, Conforti, S, Cotte, P, Crivelli, P, Cuesta, C, Dawson, J, De Bonis, I, De La Taille, C, Delbart, A, Di Luise, S, Doizon, F, Drancourt, C, Duchesneau, D, Dulucq, F, Duval, F, Emery, S, Ereditato, A, Falcone, A, Fusshoeller, K, Gallego-Ros, A, Galymov, V, Geffroy, N, Gendotti, A, Gherghel-Lascu, A, Gil-Botella, I, Girerd, C, Gomoiu, M, Gorodetzky, P, Hamada, E, Hanni, R, Hasegawa, T, Holin, A, Horikawa, S, Ikeno, M, Jiménez, S, Jipa, A, Karolak, M, Karyotakis, Y, Kasai, S, Kasami, K, Kishishita, T, Konari, H, Kreslo, I, Kryn, D, Kunzé, P, Kurokawa, M, Kuromori, Y, Lastoria, C, Lazanu, I, Lehmann-Miotto, G, Leyton, M, Lira, N, Loo, K, Lorca, D, Lutz, P, Lux, T, Maalampi, J, Maire, G, Maki, M, Manenti, L, Margineanu, R, Marteau, J, Martin-Chassard, G, Mathez, H, Mazzucato, E, Misitano, G, Mladenov, D, Molina Bueno, L, Mosu, T, Mu, W, Murphy, S, Nakayoshi, K, Narita, S, Navas-Nicolás, D, Negishi, K, Nessi, M, Niculescu-Oglinzanu, M, Noto, F, Noury, A, Onishchuk, Y, Palomares, C, Parvu, M, Patzak, T, Penichot, Y, Pennacchio, E, Periale, L, Pessard, H, Pietropaolo, F, Pugnere, D, Radics, B, Redondo, D, Regenfus, C, Remoto, A, Resnati, F, Ristea, O, Rubbia, A, Saftoiu, A, Sakashita, K, Sanchez, F, Santos, C, Scarpelli, A, Schloesser, C, Sendai, K, Sergiampietri, F, Shahsavarani, S, Shoji, M, Sinclair, J, Soto-Oton, J, Stanca, D, Stefan, D, Sulej, R, Tanaka, M, Toboaru, V, Tonazzo, A, Tromeur, W, Trzaska, W, Uchida, T, Urda, L, Vannucci, F, Vasseur, G, Verdugo, A, Viant, T, Vihonen, S, Vilalte, S, Weber, M, Wu, S, Yu, J, Zambelli, L, and Zito, M

Subjects
photon: propagation, Photomultiplier, CERN Lab, Physics - Instrumentation and Detectors, Physics::Instrumentation and Detectors, tutkimuslaitteet, Performance of High Energy Physics Detector, Phase (waves), FOS: Physical sciences, Cosmic ray, Noble liquid detectors (scintillation, ionization, double-phase), Scintillator, 01 natural sciences, 7. Clean energy, High Energy Physics - Experiment, High Energy Physics - Experiment (hep-ex), Optics, 0103 physical sciences, [PHYS.HEXP]Physics [physics]/High Energy Physics - Experiment [hep-ex], [PHYS.PHYS.PHYS-INS-DET]Physics [physics]/Physics [physics]/Instrumentation and Detectors [physics.ins-det], Detectors and Experimental Techniques, 010306 general physics, Instrumentation, physics.ins-det, Mathematical Physics, scintillation counter, Physics, Scintillation, Time projection chamber, photomultiplier, 010308 nuclear & particles physics, business.industry, hep-ex, Detector, Scintillators, scintillation and light emission processes (solid, gas and liquid scintillators), Instrumentation and Detectors (physics.ins-det), time projection chamber: liquid argon, Performance of High Energy Physics Detectors, Photon detectors for UV, visible and IR photons (vacuum) (photomulti-pliers, HPDs, others), Scintillators, scintillation and light emission processes (solid, gas and liquidscintillators), Photon detectors for UV, visible and IR photons (vacuum) (photomultipliers, HPDs, others), FIS/01 - FISICA SPERIMENTALE, ilmaisimet, Scintillation counter, business, kosminen säteily, performance, Particle Physics - Experiment
Abstract

The $3 \times 1 \times 1$ m$^3$ demonstrator is a dual phase liquid argon time projection chamber that has recorded cosmic rays events in 2017 at CERN. The light signal in these detectors is crucial to provide precise timing capabilities. The performances of the photon detection system, composed of five PMTs, are discussed. The collected scintillation and electroluminescence light created by passing particles has been studied in various detector conditions. In particular, the scintillation light production and propagation processes have been analyzed and compared to simulations, improving the understanding of some liquid argon properties., Comment: 30 pages, 26 figures

Published
2020

47. Sub 10 nm CoO nanoparticle-decorated graphitic carbon nitride for solar hydrogen generation

Author

Aniruddha, Mondal, Shubham, Biswas, Srishti, Aditya, Kumar, Jong-Sung, Yu, and Apurba, Sinhamahapatra

Abstract

Solar hydrogen generation is one of the most compelling concepts in modern research to address both the energy and environmental issues simultaneously for the survival of the human race. A Type II heterojunction (CoO-GCN) was fabricated by decorating sub 10 nm CoO nanoparticles (NPs) on the graphitic carbon nitride (GCN) surface. It exhibited improved absorption of UV-VIS light and efficiently separate the photogenerated electrons and holes in opposite directions. A maximum hydrogen generation rate of 9.8 mmol g

Published
2020

48. Real-time monitored photocatalytic activity and electrochemical performance of an rGO/Pt nanocomposite synthesized

Author

Satish, Kasturi, Sri Ramulu, Torati, Yun Ji, Eom, Syafiq, Ahmad, Byong-June, Lee, Jong-Sung, Yu, and CheolGi, Kim

Abstract

Herein, we have reported the real-time photodegradation of methylene blue (MB), an organic pollutant, in the presence of sunlight at an ambient temperature using a platinum-decorated reduced graphene oxide (rGO/Pt) nanocomposite. The photocatalyst was prepared

Published
2020

50. Comparative studies of electrochemical performance and characterization of TiO2/graphene nanocomposites as anode materials for Li-secondary batteries

Author

Hochun Lee, Hasan Jamal, Jong-Sung Yu, Chang-Seop Lee, and Byung-Sun Kang

Subjects
Anatase, Materials science, Graphene, Scanning electron microscope, General Chemical Engineering, Composite number, 02 engineering and technology, 010402 general chemistry, 021001 nanoscience & nanotechnology, 01 natural sciences, 0104 chemical sciences, law.invention, chemistry.chemical_compound, X-ray photoelectron spectroscopy, chemistry, Chemical engineering, law, Titanium dioxide, Nanorod, Calcination, 0210 nano-technology
Abstract

Using graphene oxide (GO) and titanium dioxide (TiO2), various types of composites comprised of graphene-bonded and grafted anatase TiO2 were synthesized without employing a cross-linking reagent in this study. Graphene sheets were uniformly dispersed among the TiO2 particles, to enhance the cyclability and electronic conductivity of the TiO2 anode for lithium ion batteries. A composite of GO prepared with three types of TiO2 (nanoparticles, nanorods, nanofibers) were synthesized by hydrothermal followed by calcination treatment. The reduction of GO increased simultaneously after calcination under argon atmosphere at 400 °C for 4 h. To achieve overall better electrochemical performance we used the anatase type of TiO2. The physicochemical properties were characterized by scanning electron microscopy (SEM), transmission electron microscopy (TEM), X-Ray powder diffraction (XRD), X-ray photoelectron spectroscopy (XPS) and Raman spectroscopy. Surface properties were measured by the Brunauer–Emmett–Teller (BET) & Barrett–Joyner–Halenda (BJH) method. The electrochemical properties were also investigated by Galvanostatic charge-discharge and Electrochemical Impedance Spectra (EIS). TiO2 nanoparticles composite with graphene delivered rate capability of 155 mAh g−1 at 0.5 C and restored the rate capacity of 109 mAh g−1 after 20 C, with a capacity loss of 30%. TiO2 nanorods composite with graphene benefited from its unique morphology exhibited rate capability of 124 mAh g−1 at 0.5 C and regain the rate capability of 97 mAh g−1, with a capacity loss of 22%. In addition, TiO2 nanofibers graphene composite with low surface area 19 m2 g−1 and pore volume of 0.086 cm3 g−1 transported rate capability of 68 mAh g−1 at 0.5 C and recover the rate capacity of 64 mAh g−1 after 20 C owing to its higher value of lithium-ion diffusion coefficient.

Published
2018

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