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The prediction that laser plasma heating distorts the electron distribution function away from Maxwellian and towards a super-Gaussian distribution dates back four decades1. In conditions relevant to inertial confinement fusion, however, no direct evidence of this so-called ‘Langdon effect’ has previously been observed. Here we present measurements of the spatially and temporally resolved Thomson scattering spectrum that indicate the presence of super-Gaussian electron distribution functions consistent with existing theory2. In such plasmas, ion acoustic wave frequencies increase monotonically with the super-Gaussian exponent3. Our results show that the measured power transfer between crossed laser beams mediated by ion acoustic waves requires a model that accounts for the non-Maxwellian electron distribution function, whereas the standard Maxwellian calculations overpredict power transfer over a wide region of parameter space. Including this effect is expected to improve the predictive capability of crossed-beam energy transfer modelling at the National Ignition Facility in California and may restore a larger operable design space for inertial confinement fusion experiments. This is also expected to motivate further inquiry in other areas affected by non-Maxwellian electron distribution functions, such as laser absorption, heat transport and X-ray spectroscopy. In inertial confinement fusion experiments, the effect of the overlapping laser beams on the plasma is predicted to lead to a distortion of the electron distribution function, which has now been observed in experiments.

Focusing laser light onto a very small target can produce the conditions for laboratory-scale nuclear fusion of hydrogen isotopes. The lack of accurate predictive models, which are essential for the design of high-performance laser-fusion experiments, is a major obstacle to achieving thermonuclear ignition. Here we report a statistical approach that was used to design and quantitatively predict the results of implosions of solid deuterium-tritium targets carried out with the 30-kilojoule OMEGA laser system, leading to tripling of the fusion yield to its highest value so far for direct-drive laser fusion. When scaled to the laser energies of the National Ignition Facility (1.9 megajoules), these targets are predicted to produce a fusion energy output of about 500 kilojoules-several times larger than the fusion yields currently achieved at that facility. This approach could guide the exploration of the vast parameter space of thermonuclear ignition conditions and enhance our understanding of laser-fusion physics.

Electron velocity distribution functions driven by inverse bremsstrahlung heating are measured to be non-Maxwellian using a novel angularly resolved Thomson-scattering instrument and the corresponding reduction of electrons at slow velocities results in a $\ensuremath{\sim}40%$ measured reduction in inverse bremsstrahlung absorption. The distribution functions are measured to be super-Gaussian in the bulk ($v/{v}_{th}l3$) and Maxwellian in the tail ($v/{v}_{th}g3$) when the laser heating rate dominates over the electron-electron thermalization rate. Simulations with the particle code quartz show the shape of the tail is dictated by the uniformity of the laser heating.

The performance of direct-drive inertial confinement fusion implosions relies critically on the coupling of laser energy to the target plasma. Cross-beam energy transfer (CBET), the resonant exchange of energy between intersecting laser beams mediated by ponderomotively driven ion-acoustic waves (IAWs), inhibits this coupling by scattering light into unwanted directions. The variety of beam intersection angles and varying plasma conditions in an implosion results in IAWs with a range of phase velocities. Here, we show that CBET saturates through a resonance detuning that depends on the IAW phase velocity and that results from trapping-induced modifications to the ion distribution functions. For smaller phase velocities, the modifications to the distribution functions can rapidly thermalize in the presence of mid-Z ions, leading to a blueshift in the resonant frequency. For larger phase velocities, the modifications can persist, leading to a redshift in the resonant frequency. Ultimately, these results may reveal pathways toward CBET mitigation and inform reduced models for radiation hydrodynamics codes to improve their predictive capability.

Laser-plasma accelerators (LPAs) driven by picosecond-scale, kilojoule-class lasers can generate particle beams and x-ray sources that could be utilized in experiments driven by multi-kilojoule, high-energy-density science (HEDS) drivers such as the OMEGA laser at the Laboratory for Laser Energetics (LLE) or the National Ignition Facility at Lawrence Livermore National Laboratory. This paper reports on the development of the first LPA driven by a short-pulse, kilojoule-class laser (OMEGA EP) connected to a multi-kilojoule HEDS driver (OMEGA). In experiments, electron beams were produced with electron energies greater than 200 MeV, divergences as low as 32 mrad, charge greater than 700 nC, and conversion efficiencies from laser energy to electron energy up to 11%. The electron beam charge scales with both the normalized vector potential and plasma density. These electron beams show promise as a method to generate MeV-class radiography sources and improved-flux broadband x-ray sources at HEDS drivers.

Photon accelerators can spectrally broaden laser pulses with high efficiency in moving electron density gradients driven in a rapidly ionizing plasma. When driven by a conventional laser pulse, the group velocity walk-off experienced by the accelerated photons and deterioration of the gradient from diffraction and plasma refraction limit the extent of spectral broadening. Here we show that a laser pulse with a shaped space-time and transverse intensity profile overcomes these limitations by creating a guiding density profile at a tunable velocity. Self-photon acceleration in this profile leads to dramatic spectral broadening and intensity steepening, forming an optical shock that further enhances the rate of spectral broadening. In this new regime, multi-octave spectra extending from 400 to 60 nm wavelengths, which support near-transform-limited $l400$ as pulses, are generated over $l100 \ensuremath{\mu}\mathrm{m}$ of interaction length.

Laser plasma instabilities are problematic for inertial confinement fusion because they can spoil illumination uniformity, reduce laser-target coupling, and create unwanted fast electrons. Recent experiments and simulations have shown that self-seeded stimulated rotational Raman scattering (SRRS) in air might achieve enough spectral broadening to mitigate these instabilities with only moderate unwanted broadening of the focal spot. The theoretical model for the simulations included chaotic broadband and spatially multimode light, but was a scalar formulation suitable for only linear polarization, where the SRRS gains and spectral broadening are limited by Stokes--anti-Stokes coupling. This paper derives a tensor formulation of SRRS theory suitable for modeling spectral broadening of arbitrarily polarized spatially and temporally incoherent light; it then describes the algorithms used to simulate the theory and provides some preliminary results that compare linear and elliptical polarizations. It begins with a paraxial wave equation for an arbitrarily polarized optical field envelope, which is phase modulated by a term proportional to a Raman driven molecular polarizability tensor. Treating the air molecules as rigid rotators, it uses a quantum treatment to derive a driven harmonic oscillator equation for that polarizability, then expresses these vector and tensor equations in terms of the field's right- and left-handed circular polarization components to derive the final coupled equations for arbitrary polarization. The formulation includes possible ac Stark shift contributions, but shows that they are negligible for intensities below $10\phantom{\rule{0.16em}{0ex}}\mathrm{GW}/{\mathrm{cm}}^{2}$. It then describes the algorithms used in the simulation code and the numerical model of the chaotic light, whose initial spectral bandwidth is broad enough to self-seed the SRRS. In this algorithm, the SRRS process accurately conserves the total energy at each axial plane along the propagation path. Finally, it compares simulations of power spectra and far-field profiles for elliptical vs linear polarization, which show that elliptically polarized light produces significantly more broadening of both profiles than linear polarization. For linear polarization, the SRRS process reduces the incident coherence time from 0.54 to 0.27 ps; for elliptical polarization, it reduces to 0.19 ps. The theory and simulation algorithms presented here provide a framework for evaluating techniques that combine beams of alternating circular polarizations with different spectra and angular divergences to improve SRRS spectral broadening without excessive focal spot broadening.

We measure cross-beam energy transfer (CBET) saturation by ion heating in a gas-jet plasma characterized using Thomson scattering. A wavelength-tunable ultraviolet (UV) probe laser beam interacts with four intense UV pump beams to drive large-amplitude ion-acoustic waves. For the highest-intensity interactions, the power transfer to the probe laser drops, demonstrating ion-acoustic wave saturation. Over this time, the ion temperature is measured to increase by a factor of 7 during the 500-ps interaction. Particle-in-cell simulations show ion trapping and a subsequent ion heating consistent with measurements. Linear kinetic CBET models are found to agree well with the observed energy transfer when the measured plasma conditions are used.

Spatiotemporal control over the intensity of a laser pulse has the potential to enable or revolutionize a wide range of laser-based applications that currently suffer from the poor flexibility offered by conventional optics. Specifically, these optics limit the region of high intensity to the Rayleigh range and provide little to no control over the trajectory of the peak intensity. Here, we introduce a nonlinear technique for spatiotemporal control, the “self-flying focus,” that produces an arbitrary trajectory intensity peak that can be sustained for distances comparable to the focal length. The technique combines temporal pulse shaping and the inherent nonlinearity of a medium to customize the time and location at which each temporal slice within the pulse comes to its focus. As an example of its utility, simulations show that the self-flying focus can form a highly uniform, meter-scale plasma suitable for advanced plasma-based accelerators.

The success of direct laser-driven inertial confinement fusion (ICF) relies critically on the efficient coupling of laser light to plasma. At ignition scale, the absolute stimulated Raman scattering (SRS) instability can severely inhibit this coupling by redirecting and strongly depleting laser light. This article describes a new dynamic saturation regime of the absolute SRS instability near one-quarter of the critical density. The saturation occurs when spatiotemporal ion-acoustic fluctuations in the plasma density detune the instability resonance. The dynamic saturation mitigates the strong depletion of laser light and enhances its transmission through the instability region, explaining the coupling of laser light to ICF targets at higher plasma densities.

A planar laser pulse propagating in vacuum can exhibit an extremely large ponderomotive force. This force, however, cannot impart net energy to an electron: As the pulse overtakes the electron, the initial impulse from its rising edge is completely undone by an equal and opposite impulse from its trailing edge. Here we show that planar-like "flying focus" pulses can break this symmetry, imparting relativistic energies to electrons. The intensity peak of a flying focus-a moving focal point resulting from a chirped laser pulse focused by a chromatic lens-can travel at any subluminal velocity, forwards or backwards. As a result, an electron can gain enough momentum in the rising edge of the intensity peak to outrun and avoid the trailing edge. Accelerating the intensity peak can further boost the momentum gain. Theory and simulations demonstrate that these dynamic intensity peaks can backwards accelerate electrons to the MeV energies required for radiation and electron diffraction probes of high energy density materials.

Radiation-hydrodynamic simulations of directly driven fusion experiments at the Omega Laser Facility predict absorption accurately when targets are driven at low overlapped laser intensity. Discrepancies appear at increased intensity, however, with higher-than-expected laser absorption on target. Strong correlations with signatures of the two-plasmon decay (TPD) instability---including half-harmonic and hard-x-ray emission---indicate that TPD is responsible for this anomalous absorption. Scattered light data suggest that up to $\ensuremath{\approx}30%$ of the laser power reaching quarter-critical density can be absorbed locally when the TPD threshold is exceeded. A scaling of absorption versus TPD threshold parameter was empirically determined and validated using the laser--plasma simulation environment code.

Multibeam absolute instability thresholds for stimulated Raman scattering (SRS) and two-plasmon decay (TPD) are calculated in three dimensions for conditions relevant to direct-drive inertial confinement fusion experiments on the OMEGA laser and at the National Ignition Facility (NIF). Although multibeam effects are found to be significant for both instabilities, SRS is found to have less efficient multibeam coupling than TPD. The results are consistent with the observation of a TPD-dominated regime on the OMEGA laser and a SRS-dominated regime on the NIF despite the single-beam SRS threshold being lower than the single-beam TPD threshold on both facilities. The minimum instability threshold for NIF plasma parameters occurs for SRS near quarter-critical densities with a shared electromagnetic wave propagating along the beam axis.

Laser wakefield accelerators rely on the extremely high electric fields of nonlinear plasma waves to trap and accelerate electrons to relativistic energies over short distances. When driven strongly enough, plasma waves break, trapping a large population of the background electrons that support their motion. This limits the maximum electric field. Here we introduce a novel regime of plasma wave excitation and wakefield acceleration that removes this limit, allowing for arbitrarily high electric fields. The regime, enabled by spatiotemporal shaping of laser pulses, exploits the property that nonlinear plasma waves with superluminal phase velocities cannot trap charged particles and are therefore immune to wave breaking. A laser wakefield accelerator operating in this regime provides energy tunability independent of the plasma density and can accommodate the large laser amplitudes delivered by modern and planned high-power, short pulse laser systems.

The controlled coupling of a laser to plasma has the potential to address grand scientific challenges1–6, but many applications have limited flexibility and poor control over the laser focal volume. Here, we present an advanced focusing scheme called a ‘flying focus’, where a chromatic focusing system combined with chirped laser pulses enables a small-diameter laser focus to propagate nearly 100 times its Rayleigh length. Furthermore, the speed at which the focus moves (and hence the peak intensity) is decoupled from the group velocity of the laser. It can co- or counter-propagate along the laser axis at any velocity. Experiments validating the concept measured subluminal (−0.09c) to superluminal (39c) focal-spot velocities, generating a nearly constant peak intensity over 4.5 mm. Among possible applications, the flying focus could be applied to a photon accelerator 7 to mitigate dephasing, facilitating the production of tunable XUV sources. By combining a chromatic focusing system with chirped laser pulses, the spatiotemporal distribution of the laser pulse is controlled in the focal region. The focal spot propagates over nearly 100 times its Rayleigh length at any velocity.

Angularly resolved Thomson scattering is a novel extension of Thomson scattering, enabling the measurement of the electron velocity distribution function over many orders of magnitude. Here, details of the theoretical basis of the technique and the instrument designed for this measurement are described. Angularly resolved Thomson-scattering data from several experiments are shown with descriptions of the corresponding distribution functions. A reduced model describing the distribution function is given and used to perform a Monte Carlo analysis of the uncertainty in the measurements. The electron density and temperature were determined to a precision of 12% and 21%, respectively, on average, while all other parameters defining the distribution function were generally determined to better than 20%. It was found that these uncertainties were primarily due to limited signal to noise and instrumental effects. Measurements with this level of precision were sufficient to distinguish between Maxwellian and non-Maxwellian distribution functions.

Large diameter, flying focus driven ionization waves of arbitrary velocity (IWAV’s) were produced by a defocused laser beam in a hydrogen gas jet, and their spatial and temporal electron density characteristics were measured using a novel, spectrally resolved interferometry diagnostic. A simple analytic model predicts the effects of power spectrum non-uniformity on the IWAV trajectory and transverse profile. This model compares well with the measured data and suggests that spectral shaping can be used to customize IWAV behavior and increase controlled propagation of ionization fronts for plasma-photonics applications.

Laser wakefield accelerators (LWFAs) produce extremely high gradients enabling compact accelerators and radiation sources but face design limitations, such as dephasing, occurring when trapped electrons outrun the accelerating phase of the wakefield. Here we combine spherical aberration with a novel cylindrically symmetric echelon optic to spatiotemporally structure an ultrashort, high-intensity laser pulse that can overcome dephasing by propagating at any velocity over any distance. The ponderomotive force of the spatiotemporally shaped pulse can drive a wakefield with a phase velocity equal to the speed of light in vacuum, preventing trapped electrons from outrunning the wake. Simulations in the linear regime and scaling laws in the bubble regime illustrate that this dephasingless LWFA can accelerate electrons to high energies in much shorter distances than a traditional LWFA-a single 4.5 m stage can accelerate electrons to TeV energies without the need for guiding structures.

A high-intensity laser pulse propagating through a medium triggers an ionization front that can accelerate and frequency-upshift the photons of a second pulse. The maximum upshift is ultimately limited by the accelerated photons outpacing the ionization front or the ionizing pulse refracting from the plasma. Here we apply the flying focus--a moving focal point resulting from a chirped laser pulse focused by a chromatic lens--to overcome these limitations. Theory and simulations demonstrate that the ionization front produced by a flying focus can frequency-upshift an ultrashort optical pulse to the extreme ultraviolet over a centimeter of propagation. An analytic model of the upshift predicts that this scheme could be scaled to a novel table-top source of spatially coherent x-rays., Comment: 7 pages, 4 figures, 1 table

The picosecond evolution of non-Maxwellian electron distribution functions was measured in a laser-produced plasma using collective electron plasma wave Thomson scattering. During the laser heating, the distribution was measured to be approximately super-Gaussian due to inverse bremsstrahlung heating. After the heating laser turned off, collisional ionization caused further modification to the distribution function while increasing electron density and decreasing temperature. Electron distribution functions were determined using Vlasov-Fokker-Planck simulations including atomic kinetics.

As an alternative inertial confinement fusion scheme with predicted high energy gain and more robust designs, shock ignition requires a strong converging shock driven by a shaped pulse with a high-intensity spike at the end to ignite a pre-compressed fusion capsule. Understanding nonlinear laser-plasma instabilities in shock ignition conditions is crucial to assess and improve the laser-shock energy coupling. Recent experiments conducted on the OMEGA-EP laser facility have for the first time demonstrated that such instabilities can $\sim$100\% deplete the first 0.5 ns of the high-intensity laser pump. Analysis of the observed laser-generated blast wave suggests that this pump-depletion starts at 0.01--0.02 critical density and progresses to 0.1--0.2 critical density. This pump-depletion is also confirmed by the time-resolved stimulated Raman backscattering spectra. The dynamics of the pump-depletion can be explained by the breaking of ion-acoustic waves in stimulated Brillouin scattering. Such strong pump-depletion would inhibit the collisional laser energy absorption but may benefit the generation of hot electrons with moderate temperatures for electron shock ignition [Shang et al. Phys. Rev. Lett. 119 195001 (2017)].

International audience; Integrated hydrodynamics simulations of inertial confinement fusion rely on reduced physics models. To reproduce experimental trends, these models often feature tuning parameters, but this comes with a risk: over-tuning of one model can hide physics inadequacies in another. Ray-based models of cross-beam-energy transfer (CBET) represents one of these risks. Here we present an accurate and efficient model of CBET suitable for inline implementation in 3D hydrodynamics simulations. Inverse Ray Tracing (IRT) is used to compute the ray field in a 3D permittivity profile described on an unstructured tetrahedral mesh using the IFRIIT framework (Inline Field Reconstruction and Interaction using Inverse Tracing). CBET is accounted for through perturbations to the permittivity associated with ion acoustic waves driven by the overlapped fields. Large gradients in the permittivity are resolved by coupling the IRT to a recursive Adaptive Mesh Refinement (AMR) algorithm. The use of AMR also allows for the resolution of caustics, with accurate field reconstruction performed using the Etalon integral method. Comparisons of the model with wave-based solutions from the Laser Plasma Simulation Environment (LPSE) demonstrate its ability to control energy conservation and gain convergence through AMR depth only, without the use of ad hoc physical models or artificial tuning parameters.

We experimentally demonstrate the ability of a nonlinear self-channeling beam to resist turbulence-induced spreading and scintillation. Spatio-temporal data is presented for an 850-meter long, controlled turbulence range that can generate weak to strong turbulence on demand. At this range, the effects of atmospheric losses and dispersion are significant. Simulation results are also presented and show good agreement with experiment., 8 pages, 6 figures

A 3-D ray based model for computing laser fields in dissipative and amplifying media is presented. The eikonal equation is solved using inverse ray-tracing on a dedicated nonstructured 3-D mesh. Inverse ray-tracing opens the possibility of using Complex Geometrical Optics (CGO), for which we propose a propagation formalism in a finite element mesh. Divergent fields at caustics are corrected using an etalon integral method for fold-type caustics. This method is successfully applied in dissipative media by modifying the ray-ordering and root selection rules, thereby allowing one to reconstruct the field in the entire caustic region. In addition, we demonstrate how caustics in the CGO framework can disappear entirely for sufficiently dissipative media, making the complex ray approach valid in the entire medium. CGO is shown to offer a more precise modeling of laser refraction and absorption in a dissipative medium when compared to Geometrical Optics (GO). In the framework of Inertial Confinement Fusion (ICF), this occurs mostly at intermediate temperatures or at high temperatures close to the critical density. Additionally, GO is invalid at low temperatures if an approximated expression of the permittivity is used. The inverse ray-tracing algorithm for GO and CGO is implemented in the IFRIIT code, in the framework of a dielectric permittivity described in 3-D using a piecewise linear approximation in tetrahedrons. Fields computed using GO and CGO are compared to results from the electromagnetic wave solver Laser Plasma Simulation Environment. Excellent agreement is obtained in 1-D linear and nonlinear permittivity profiles. Good agreement is also obtained for ICF-like Gaussian density profiles in 2-D. Finally, we demonstrate how the model reproduces Gaussian beam diffraction using CGO. The IFRIIT code will be interfaced inline to 3-D radiative hydrodynamic codes to describe the nonlinear laser plasma interaction in ICF and high-energy-density plasmas.

The rapid evolutions of the electron density and temperature in a laser-produced plasma were measured using collective Thomson scattering. Unprecedented picosecond time resolution, enabled by a pulse-front-tilt compensated spectrometer, revealed a transition in the plasma-wave dynamics from an initially cold, collisional state to a quasistationary, collisionless state. The Thomson-scattering spectra were compared with theoretical calculations of the fluctuation spectrum using either a conventional Bhatnagar-Gross-Krook (BGK) collision operator or the rigorous Landau collision terms: the BGK model overestimates the electron temperature by 50% in the most-collisional conditions.

A parameter regime is identified for Raman amplification at high temperatures, where deleterious laser–plasma instabilities that limit current amplification experiments are avoided, yet sufficient gain for an effective power amplifier is attained. Calculations and kinetic simulations show that even at high temperatures, an amplifier is able to satisfy the criteria set forth to present a proof-of-principle system scalable to high powers, where energy transfer efficiencies are ≥30%, intensity gains are ≥10, and output intensities are ≥100× the pump intensity.

The stimulated Raman scattering (SRS) instability can inhibit the performance of laser-driven inertial confinement fusion (ICF) implosions by scattering light into unwanted directions or by generating hot electrons that preheat the target fuel. In principle, ICF target designs can avoid parameter regimes conducive to large, linear SRS gains. In practice, kinetic inflation—the nonlinear enhancement of SRS due to electron trapping in the excited plasma wave—makes this difficult. Here, we show that laser bandwidth in the form of frequency modulation can either decrease or increase the inflationary SRS (iSRS) threshold in inhomogeneous plasmas depending on the maximum chirp of the laser pulse. The threshold, mapped out by a series of particle-in-cell simulations, exhibits a minimum when the frequency change within the pulse cancels the spatial detuning due to density inhomogeneities along the trajectory of the scattered light. By tuning the pump laser parameters away from this minimum, the iSRS threshold can be larger than at zero bandwidth, providing a path to mitigating kinetic inflation in ignition relevant plasmas.

Thresholds for the absolute stimulated Raman scattering (SRS) and two-plasma decay (TPD) instabilities driven by multiple broadband laser beams are evaluated using 3D simulations at conditions relevant to inertial confinement fusion experiments. Multibeam TPD and SRS backscatter are found to be easier to mitigate with bandwidth than the corresponding single-beam instabilities. A relative bandwidth of 1% increases the threshold for absolute SRS backscatter by a factor of 4 at conditions relevant to ongoing National Ignition Facility experiments and should be sufficient to keep all of the absolute instabilities below threshold in experiments with similar conditions.

Laser-direct drive (LDD), along with laser indirect (X-ray) drive (LID) and magnetic drive with pulsed power, is one of the three viable inertial confinement fusion approaches to achieving fusion ignition and gain in the laboratory. The LDD programme is primarily being executed at both the Omega Laser Facility at the Laboratory for Laser Energetics and at the National Ignition Facility (NIF) at Lawrence Livermore National Laboratory. LDD research at Omega includes cryogenic implosions, fundamental physics including material properties, hydrodynamics and laser–plasma interaction physics. LDD research on the NIF is focused on energy coupling and laser–plasma interactions physics at ignition-scale plasmas. Limited implosions on the NIF in the ‘polar-drive’ configuration, where the irradiation geometry is configured for LID, are also a feature of LDD research. The ability to conduct research over a large range of energy, power and scale size using both Omega and the NIF is a major positive aspect of LDD research that reduces the risk in scaling from OMEGA to megajoule-class lasers. The paper will summarize the present status of LDD research and plans for the future with the goal of ultimately achieving a burning plasma in the laboratory.This article is part of a discussion meeting issue ‘Prospects for high gain inertial fusion energy (part 2)’.

Higher levels of hot electrons from the two-plasmon–decay instability are observed when smoothing by spectral dispersion (SSD) is turned off in directly driven inertial confinement fusion experiments at the Omega Laser Facility. This finding is explained using a hot-spot model based on speckle statistics and simulation results from the laser–plasma simulation environment. The model accurately reproduces the relative increase in hot-electron activity at two different drive intensities although it slightly overestimates the absolute number of hot electrons in all cases. Extrapolating from the current ≈ 360-GHz system while adhering to the logic of the hot-spot model suggests that a larger SSD bandwidth should significantly mitigate hot-electron generation, and legacy 1-THz OMEGA experiments appear to support this conclusion. These results demonstrate that it is essential to account for laser speckles and spatiotemporal smoothing to obtain quantitative agreement with experiments. A compilation of hot-electron data from the past two decades reveals several other important points: (1) many prior experiments are more easily understood using recent results from multibeam absolute instability theory and (2) experiments with ignition-scale conditions produce less hot electrons compared to OMEGA spherical experiments for a given vacuum overlapped intensity, which is a promising result for validating performance predictions based on hydrodynamic scaling relations.

Meter-scale nonlinear propagation of a picosecond ultraviolet laser beam in water, sufficiently intense to cause stimulated Raman scattering (SRS), nonlinear focusing, pump-Stokes nonlinear coupling, and photoexcitation, was characterized in experiments and simulations. Pump and SRS Stokes pulse energies were measured, and pump beam profiles were imaged at propagation distances up to 100 cm for a range of laser power below and above self-focusing critical power. Simulations with conduction band excitation energy U C B = 9.5 e V , effective electron mass m e f f = 0.2 m e , Kerr nonlinear refractive index n 2 = 5 × 10 − 16 c m 2 / W , and index contribution due to SRS susceptibility n 2 r = 1.7 × 10 − 16 c m 2 / W produced the best agreement with experimental data.

Laser–plasma interaction instabilities can be detrimental for direct-drive inertial confinement fusion by generating high-energy electrons that preheat the target. An experimental platform has been developed and fielded on the National Ignition Facility to investigate hot-electron production from laser–plasma instabilities at direct-drive ignition-relevant conditions. The radiation-hydrodynamic code DRACO has been used to design planar-target experiments that generate plasma and interaction conditions comparable to direct-drive ignition designs: IL ∼ 1015 W/cm2, Te > 3 keV, and density-gradient scale lengths of Ln ∼ 600 μm in the quarter-critical density region. The hot-electron properties were inferred by comparing the experimentally observed hard x-ray spectra to Monte Carlo simulations of hard x-ray emission from hot electrons depositing energy in the target. Hot-electron temperatures of ∼40 keV to 60 keV and the fraction of laser energy converted to hot electrons of ∼0.5% to 5% were inferred in plastic targets for laser intensities at the quarter-critical density surface of (∼4 to 14) × 1014 W/cm2. The use of silicon ablators was found to mitigate the hot-electron preheat by increasing the threshold laser intensity for hot-electron generation from ∼3.5 × 1014 W/cm2 in plastic to ∼6 × 1014 W/cm2 in silicon. The overall hot-electron production is also reduced in silicon ablators when the intensity threshold is exceeded.

Stimulated Raman scattering (SRS) has been explored comprehensively in planar-geometry experiments at the National Ignition Facility in conditions relevant to the corona of inertial confinement fusion ignition-scale direct-drive targets. These experiments at measured electron temperatures of 4 to 5 keV simulated density scale lengths L n of 400 to 700 μm, and laser intensities at the quarter-critical density of up to 1.5 × 1015 W/cm2 have determined SRS thresholds and the scaling behavior of SRS for various beam geometries. Several SRS mechanisms, including saturated absolute SRS near the quarter-critical density and additional SRS, including near-backscatter or sidescatter at lower densities, have been identified. Correlation of time-dependent SRS at densities ∼0.15 to 0.21 of the critical density with hot-electron signatures as well as the magnitudes of these signatures across different experiments, is observed. Further modeling work is needed to definitively identify the density region in which hot electrons are generated and will guide SRS and hot-electron preheat mitigation strategies for direct-drive-ignition designs.

Cross-beam energy transfer (CBET) is a laser-plasma instability that significantly impacts laser energy deposition in laser-driven inertial confinement fusion (ICF) experiments. Radiation-hydrodynamics simulations, which are used to design and tune ICF implosions, use ray-based CBET models, but existing models require artificial multipliers to conserve energy and to obtain quantitative agreement with experiments. The discretization of the ray trajectories in traditional ray-based CBET models does not account for the rapid variation in CBET gain as rays pass through caustics. We introduce a model that allows one to treat caustics much more accurately and greatly improves energy conservation. The ray-based CBET calculations show excellent agreement with laser absorption from two-dimensional wave-based calculations (0.3% difference) and a three-dimensional 60-beam OMEGA implosion (2.4% difference) without artificial multipliers.

Nonlocal heat flux was measured in laser-produced coronal plasmas using a novel Thomson scattering technique. The measured heat flux was smaller than the classical values inferred from the measured plasma conditions in regions with large temperature gradients and agreed with classical values for weak gradients. Vlasov-Fokker-Planck simulations self-consistently calculated the electron distribution functions used to reproduce the measured Thomson scattering spectra and to determine the heat flux. Multigroup nonlocal simulations overestimated the measured heat flux.

Flying focus is a technique that uses a chirped laser beam focused by a highly chromatic lens to produce an extended focal region within which the peak laser intensity can propagate at any velocity. When that intensity is high enough to ionize a background gas, an ionization wave will track the intensity isosurface corresponding to the ionization threshold. We report on the demonstration of such ionization waves of arbitrary velocity. Subluminal and superluminal ionization fronts were produced that propagated both forward and backward relative to the ionizing laser. All backward and all superluminal cases mitigated the issue of ionization-induced refraction that typically inhibits the formation of long, contiguous plasma channels.

Three-dimensional laser-plasma interaction simulations show that laser frequency detuning by an amount achievable with current laser technology can be used to suppress the two-plasmon decay (TPD) instability and the corresponding hot-electron generation. For the plasma conditions and laser configuration in a direct-drive inertial confinement fusion implosion on the OMEGA laser, the simulations show that $\ensuremath{\sim}0.7%$ laser frequency detuning is sufficient to eliminate TPD-driven hot-electron generation in current experiments. This allows for higher ablation pressures in future implosion designs by using higher laser intensities.

We present an unusual example of truly long-range propagation of high-power laser pulses through strong atmospheric turbulence. A form of nonlinear self-channeling is achieved when the laser power is close to the self-focusing power of air and the transverse dimensions of the pulse are smaller than the coherence diameter of turbulence. In this mode, nonlinear self-focusing counteracts diffraction, and turbulence-induced spreading is greatly reduced. Furthermore, the laser intensity is below the ionization threshold so that multiphoton absorption and plasma defocusing are avoided. Simulations show that the pulse can propagate many Rayleigh lengths (several kilometers) while maintaining a high intensity. In the presence of aerosols, or other extinction mechanisms that deplete laser energy, the pulse can be chirped to maintain the channeling.

Ultra-short pulse lasers are dominated by solid-state technology, which typically operates in the near-infrared. Efforts to extend this technology to longer wavelengths are meeting with some success, but the trend remains that longer wavelengths correlate with greatly reduced power. The carbon dioxide (CO 2 ) laser is capable of delivering high energy, 10μm wavelength pulses, but the gain structure makes operating in the ultra-short pulse regime difficult. The U.S. Naval Research Laboratory is currently building a novel CO 2 laser which uses solid state injection seeding, with pressure and power broadening, to generate high power, picosecond pulses. As a way of relaxing the requirements on the seed pulse and gain medium, we propose to use ionization blue-shifting during pre-amplification to broaden the laser bandwidth. The time changing index of refraction associated with laser-plasma generation will spectrally blue-shift the pulse. This can be dispersively compressed outside of the amplifier. This mechanism was proposed [1] to explain the observation of 600fs pulses generated by a high pressure CO 2 laser. We carried out simulations using a modified version of the co2amp code [2] which models CO 2 pumping with the Boltzmann equation, laser amplification with the Maxwell- Bloch equations, and beam propagation with Huygens-Fresnel integration, and now photoionization and collisional ionization.

An intense, short laser pulse incident on a dielectric can excite electrons from valence to the conduction band. As these electrons undergo scattering, from both ion centers and acoustic phonons, they emit Bremsstrahlung radiation. Here we present 1D model that describes the laser pulse dielectric interaction and the resulting Bremsstrahlung emission. Characteristics of the radiation (power, energy and spectra) are computed for arbitrary ratios of electron collision frequency to radiation frequency [1]. The conversion efficiency of laser pulse energy into bremsstrahlung radiation depends strongly on both the fluence and duration of the pulse, saturating at values of about $10 ^{-5}$. Depending on whether the fluence is above or below the damage threshold of the material, the emission can originate either from the surface or the bulk of the dielectric. The radiation may provide a broadband light source for diagnostics.

Ongoing NRL experiments have revealed long-lived $( \sim 20$ microseconds), efficient microwave reflection from a laser generated plasma region in air. This phenomenon is distinct from the short-lived response $( \sim 10$ ns) typical for laser produced air plasma filaments and represents a thousand-fold increase in the duration of the influence of the plasma region. We believe that the cause of the long-lived reflection is a hightemperature, low-density cavitation region created from dynamic expansion of the laser plasma region. The reduced recombination times in this region allow a sufficiently high plasma density $( > 10 \wedge 13$ cm-3) to persist for much longer timescales. Low power microwave scattering experiments with a Ka-band source will be presented. Results simulating this interaction using an in-house hydrodynamic code (SPARC) that are then fed into an electromagnetic scattering simulations will be discussed. Lastly, we will present preliminary results from recent high power experiments using a 5 MW, X-band Magnicon source.

Photoelectron spectra and ionization rates encompassing relativistic intensities and hydrogenlike ions with relativistic binding energies are obtained using a quasiclassical S-matrix approach. These results, along with those based on the imaginary time method, are compared with three-dimensional, ½-period ab initio simulations for a wide range of ionization potentials and electric field amplitudes. Significant differences between the three results are demonstrated. Time-dependent simulations indicate that the peak ionization current can occur before the peak of the electric field.

An intense, short laser pulse incident on a transparent dielectric can excite electrons from the valence to the conduction band. As these electrons undergo scattering, both from phonons and ions, they emit bremsstrahlung. Here we present a theory of bremsstrahlung emission appropriate for the interaction of laser pulses with dielectrics. Simulations of the interaction, incorporating this theory, illustrate characteristics of the radiation (power, energy, and spectra) for arbitrary ratios of electron collision frequency to radiation frequency. The conversion efficiency of laser pulse energy into bremsstrahlung depends strongly on both the intensity and duration of the pulse, saturating at values of about 10^{-5}. Depending on whether the intensity is above or below the damage threshold of the material, the emission can originate either from the surface or the bulk of the dielectric, respectively. The bremsstrahlung emission may provide a broadband light source for diagnostics.

Ultrarelativistic photoelectron spectra exhibit unexpected characteristics in a paraxial laser focus. The photoelectron energy scales superponderomotively, and the usual parabolic momentum distribution is distorted into a variety of intricate patterns, depending on the location of the ion. These patterns include discrete contours, which in some cases can be easily identified with a particular subcycle burst of ionization current. An analytical formula for the maximum photoelectron energy in a paraxial radiation field is given, and high-resolution momentum distributions with narrowly peaked features are presented. These narrowly peaked features suggest application to electron injection into plasma-based accelerators.

Underwater UV laser pulse propagation experiments were performed at intensities spanning the linear and nonlinear regimes. Measurements and simulations show strong coupling to molecular Raman modes and suggest strong ionization-induced refraction near the beam focus.

The excitation of THz radiation by the interaction of an ultra short laser pulse with the modes of a miniature corrugated plasma waveguide is considered. The axially corrugated waveguide supports the electromagnetic (EM) modes with appropriate polarization and subluminal phase velocities that can be phase matched to the ponderomotive potential associated with laser pulse, making significant THz generation possible. This process is studied via full format Particle-in-Cell (PIC) simulations that, for the first time, model the nonlinear dynamics of the plasma and the self-consistent evolution of the laser pulse in the case where the laser pulse energy is entirely depleted. It is found that the generated THz is characterized by lateral emission from the channel, with a spectrum that may be narrow or broad depending on the laser intensity. A range of realistic laser pulse and plasma parameters is considered with the goal of maximizing the conversion efficiency of optical energy to THz radiation. As an example, a fixed drive pulse (0.55 J) with a spot size of 15 $\mu m$ and duration of 15 $fs$ produces 37.8 mJ of THz radiation in a 1.5 cm corrugated plasma waveguide with an on axis average density of $1.4\times10^{18} cm^{-3}$.

A chirped laser pulse focused by a chromatic lens exhibits a dynamic, or flying, focus in which the trajectory of the peak intensity decouples from the group velocity. In a medium, the flying focus can trigger an ionization front that follows this trajectory. By adjusting the chirp, the ionization front can be made to travel at an arbitrary velocity along the optical axis. We present analytical calculations and simulations describing the propagation of the flying focus pulse, the self-similar form of its intensity profile, and ionization wave formation. The ability to control the speed of the ionization wave and, in conjunction, mitigate plasma refraction has the potential to advance several laser-based applications, including Raman amplification, photon acceleration, high-order-harmonic generation, and THz generation.