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The trapped-ion system has been a leading platform for practical quantum computation and quantum simulation since the first scheme of a quantum gate was proposed by Cirac and Zoller in 1995. Quantum gates with trapped ions have shown the highest fidelity among all physical platforms. Recently, sophisticated schemes of quantum gates such as amplitude, phase, frequency modulation, or multi-frequency application, have been developed to make the gates fast, robust to many types of imperfections, and applicable to multiple qubits. Here, we review the basic principle and recent development of quantum gates with trapped ions., 19 pages, 10 figures. Review paper invited to the Journal of Korean Physical Society (JKPS) special issue commemorating the 30th anniversary of the division of atomic molecular and optical (AMO) physics

We propose and study ways speeding up of the entangling operations in the trapped ions system with high fidelity. First, we find a scheme to increase the speed of a two-qubit gate without the limitation of trap frequency, which was considered as the fundamental limit. Second, we study the fast gate scheme for entangling more than two qubits simultaneously. We apply the method of applying multiple frequency components on laser beams for the gate operations. In particular, in order to avoid infinite terms from the coupling to carrier transition, we focus on the phase-insensitive gate scheme here. We carefully study the effect of large excitation of motional mode beyond the limit of Lamb-Dicke approximation by including up to second order terms of the Lamb-Dicke parameter. We study the speed limit of multi-qubit global entangling gates without individual addressing requirements. Furthermore, our gates can be made insensitive to the fluctuation of initial motional phases which are difficult to stabilise in the phase-insensitive gate scheme., 16 pages, 8 figures

Controllable bosonic systems can provide post-classical computational power with sub-universal quantum computational capability. A network that consists of a number of bosons evolving through beam-splitters and phase-shifters between different modes, has been proposed and applied to demonstrate quantum advantages. While the network has been implemented mostly in optical systems with photons, recently alternative realizations have been explored, where major limitations in photonic systems such as photon loss, and probabilistic manipulation can be addressed. Phonons, the quantized excitations of vibrational modes, of trapped ions can be a promising candidate to realize the bosonic network. Here, we experimentally demonstrate a minimal-loss phononic network that can be programmed and in which any phononic states are deterministically prepared and detected. We realize the network with up to four collective-vibrational modes, which can be straightforwardly extended to reveal quantum advantage. We benchmark the performance of the network with an exemplary algorithm of tomography for arbitrary multi-mode states with a fixed total phonon number. We obtain reconstruction fidelities of 94.5 $\pm$ 1.95 % and 93.4 $\pm$ 3.15 % for single-phonon and two-phonon states, respectively. Our experiment demonstrates a clear and novel pathway to scale up a phononic network for various quantum information processing beyond the limitations of classical and other quantum systems.

Quantum measurements cannot be thought of as revealing preexisting results, even when they do not disturb any other measurement in the same trial. This feature is called contextuality and is crucial for the quantum advantage in computing. Here, we report the first observation of quantum contextuality simultaneously free of the detection, sharpness and compatibility loopholes. The detection and sharpness loopholes are closed by adopting a hybrid two-ion system and highly efficient fluorescence measurements offering a detection efficiency of $100\%$ and a measurement repeatability $>98\%$. The compatibility loophole is closed by targeting correlations between observables for two different ions in a Paul trap, a $^{171}\mathrm{Yb}^{+}$ ion and a $^{138}\mathrm{Ba}^{+}$ ion, chosen so measurements on each ion use different operation laser wavelengths, fluorescence wavelengths, and detectors. The experimental results show a violation of the bound for the most adversarial noncontextual models and open a new way to certify quantum systems., 8 pages, 6 figures, 1 table, 65 references

A quantum algorithm can be decomposed into a sequence consisting of single qubit and 2-qubit entangling gates. To optimize the decomposition and achieve more efficient construction of the quantum circuit, we can replace multiple 2-qubit gates with a single global entangling gate. Here, we propose and implement a scalable scheme to realize the global entangling gates on multiple $\yb$ ion qubits by coupling to multiple motional modes through external fields. Such global gates require simultaneously decoupling of multiple motional modes and balancing of the coupling strengths for all the qubit-pairs at the gate time. To satisfy the complicated requirements, we develop a trapped-ion system with fully-independent control capability on each ion, and experimentally realize the global entangling gates. As examples, we utilize them to prepare the Greenberger-Horne-Zeilinger (GHZ) states in a single entangling operation, and successfully show the genuine multi-partite entanglements up to four qubits with the state fidelities over $93.4\%$.

Vibrational degrees of freedom in trapped-ion systems have recently been gaining attention as a quantum resource, beyond the role as a mediator for entangling quantum operations on internal degrees of freedom, because of the large available Hilbert space. The vibrational modes can be represented as quantum harmonic oscillators and thus offer a Hilbert space with infinite dimension. Here we review recent theoretical and experimental progress in the coherent manipulation of the vibrational modes, including bosonic encoding schemes in quantum information, reliable and efficient measurement techniques, and quantum operations that allow various quantum simulations and quantum computation algorithms. We describe experiments using the vibrational modes, including the preparation of non-classical states, molecular vibronic sampling, and applications in quantum thermodynamics. We finally discuss the potential prospects and challenges of trapped-ion vibrational-mode quantum information processing., 19 pages, 12 figures, review paper

Realizing a long coherence time quantum memory is a major challenge of current quantum technology. Until now, the longest coherence-time of a single qubit was reported as 660 s in a single 171Yb+ ion-qubit through the technical developments of sympathetic cooling and dynamical decoupling pulses, which addressed heating-induced detection inefficiency and magnetic field fluctuations. However, it was not clear what prohibited further enhancement. Here, we identify and suppress the limiting factors, which are the remaining magnetic-field fluctuations, frequency instability and leakage of the microwave reference-oscillator. Then, we observe the coherence time of around 5500 s for the 171Yb+ ion-qubit, which is the time constant of the exponential decay fit from the measurements up to 960 s. We also systematically study the decoherence process of the quantum memory by using quantum process tomography and analyze the results by applying recently developed resource theories of quantum memory and coherence. Our experimental demonstration will accelerate practical applications of quantum memories for various quantum information processing, especially in the noisy-intermediate-scale quantum regime., Extending qubit coherence times represent one of the key challenges for quantum technologies. Here, after properly suppressing magnetic-field fluctuations, frequency instability and leakage of the microwave reference-oscillator, the authors infer coherence times of 5500 s for an Yb ion qubit.

Various quantum applications can be reduced to estimating expectation values, which are inevitably deviated by operational and environmental errors. Although errors can be tackled by quantum error correction, the overheads are far from being affordable for near-term technologies. To alleviate the detrimental effects of errors on the estimation of expectation values, quantum error mitigation techniques have been proposed, which require no additional qubit resources. Here we benchmark the performance of a quantum error mitigation technique based on probabilistic error cancellation in a trapped-ion system. Our results clearly show that effective gate fidelities exceed physical fidelities, i.e., we surpass the break-even point of eliminating gate errors, by programming quantum circuits. The error rates are effectively reduced from (1.10 ± 0.12) × 10−3 to (1.44 ± 5.28) × 10−5 and from (0.99 ± 0.06) × 10−2 to (0.96 ± 0.10) × 10−3 for single- and two-qubit gates, respectively. Our demonstration opens up the possibility of implementing high-fidelity computations on a near-term noisy quantum device., Quantum error mitigation promises to improve expectation values’ estimation without the resource overhead of quantum error correction. Here, the authors test probabilistic error cancellation using trapped ions, decreasing single- and two-qubit gates’ error rates by two and one order of magnitude respectively.

A long-time quantum memory capable of storing and measuring quantum information at the single-qubit level is an essential ingredient for practical quantum computation and com-munication. Recently, there have been remarkable progresses of increasing coherence time for ensemble-based quantum memories of trapped ions, nuclear spins of ionized donors or nuclear spins in a solid. Until now, however, the record of coherence time of a single qubit is on the order of a few tens of seconds demonstrated in trapped ion systems. The qubit coherence time in a trapped ion is mainly limited by the increasing magnetic field fluctuation and the decreasing state-detection efficiency associated with the motional heating of the ion without laser cooling. Here we report the coherence time of a single qubit over $10$ minutes in the hyperfine states of a \Yb ion sympathetically cooled by a \Ba ion in the same Paul trap, which eliminates the heating of the qubit ion even at room temperature. To reach such coherence time, we apply a few thousands of dynamical decoupling pulses to suppress the field fluctuation noise. A long-time quantum memory demonstrated in this experiment makes an important step for construction of the memory zone in scalable quantum computer architectures or for ion-trap-based quantum networks. With further improvement of the coherence time by techniques such as magnetic field shielding and increase of the number of qubits in the quantum memory, our demonstration also makes a basis for other applications including quantum money.

Plasma-based accelerators have made impressive progress in recent years. However, the beam energy spread obtained in these accelerators is still at the $\ensuremath{\sim}1%$ level, nearly one order of magnitude larger than what is needed for challenging applications like coherent light sources or colliders. In plasma accelerators, the beam energy spread is mainly dominated by its energy chirp (longitudinally correlated energy spread). Here we demonstrate that when an initially chirped electron beam from a linac with a proper current profile is sent through a low-density plasma structure, the self-wake of the beam can significantly reduce its energy chirp and the overall energy spread. The resolution-limited energy spectrum measurements show at least a threefold reduction of the beam energy spread from 1.28% to 0.41% FWHM with a dechirping strength of $\ensuremath{\sim}1\text{ }\text{ }(\mathrm{MV}/\mathrm{m})/(\mathrm{mm}\text{ }\mathrm{pC})$. Refined time-resolved phase space measurements, combined with high-fidelity three-dimensional particle-in-cell simulations, further indicate the real energy spread after the dechirper is only about 0.13% (FWHM), a factor of 10 reduction of the initial energy spread.

We study the joint probability distribution function of the work and the change of photon number of the nonequilibrium process of driving the electromagnetic (EM) field in a three-dimensional cavity with an oscillating boundary. The system is initially prepared in a grand canonical equilibrium state and we obtain the analytical expressions of the characteristic functions of work distributions in the single-resonance and multiple-resonance conditions. Our study demonstrates the validity of the fluctuation theorems of the grand canonical ensemble in nonequilibrium processes with particle creation and annihilation. In addition, our work illustrates that in the high temperature limit, the work done on the quantized EM field approaches its classical counterpart; while in the low temperature limit, similar to Casimir effect, it differs significantly from its classical counterpart., Comment: 14 pages, 3 figures

We develop a deterministic method to generate and verify arbitrarily high NOON states of quantized vibrations (phonons), through the coupling to the internal state. We experimentally create the entangled states up to $N=9$ phonons in two vibrational modes of a single trapped ${^{171}\mathrm{Yb}}^{+}$ ion. We observe an increasing phase sensitivity of the generated NOON state as the number of phonons $N$ increases and obtain the fidelity from the contrast of the phase interference and the population of the phonon states through the two-mode projective measurement, which are significantly above the classical bound. We also measure the quantum Fisher information of the generated state and observe Heisenberg scaling in the lower bounds of phase sensitivity as $N$ increases. Our scheme is generic and applicable to other photonic or phononic systems such as circuit QED systems or nanomechanical oscillators, which have Jaynes-Cummings-type of interactions.

We extend the well-known static duality [M. Girardeau, J. Math. Phys. 1, 516 (1960)JMAPAQ0022-248810.1063/1.1703687; T. Cheon and T. Shigehara, Phys. Rev. Lett. 82, 2536 (1999)PRLTAO0031-900710.1103/PhysRevLett.82.2536] between one-dimensional (1D) bosons and 1D fermions to the dynamical version. By utilizing this dynamical duality, we find the duality of nonequilibrium work distributions between interacting 1D bosonic (Lieb-Liniger model) and 1D fermionic (Cheon-Shigehara model) systems with dual contact interactions. As a special case, the work distribution of the Tonks-Girardeau gas is identical to that of 1D noninteracting fermionic system even though their momentum distributions are significantly different. In the classical limit, the work distributions of Lieb-Liniger models (Cheon-Shigehara models) with arbitrary coupling strength converge to that of the 1D noninteracting distinguishable particles, although their elementary excitations (quasiparticles) obey different statistics, e.g., the Bose-Einstein, the Fermi-Dirac, and the fractional statistics. We also present numerical results of the work distributions of Lieb-Liniger model with various coupling strengths, which demonstrate the convergence of work distributions in the classical limit.

The quantum Rabi model, involving a two-level system and a bosonic field mode, is arguably the simplest and most fundamental model describing quantum light-matter interactions. Historically, due to the restricted parameter regimes of natural light-matter processes, the richness of this model has been elusive in the lab. Here, we experimentally realize a quantum simulation of the quantum Rabi model in a single trapped ion, where the coupling strength between the simulated light mode and atom can be tuned at will. The versatility of the demonstrated quantum simulator enables us to experimentally explore the quantum Rabi model in detail, including a wide range of otherwise unaccessible phenomena, as those happening in the ultrastrong and deep strong coupling regimes. In this sense, we are able to adiabatically generate the ground state of the quantum Rabi model in the deep strong coupling regime, where we are able to detect the nontrivial entanglement between the bosonic field mode and the two-level system. Moreover, we observe the breakdown of the rotating-wave approximation when the coupling strength is increased, and the generation of phonon wave packets that bounce back and forth when the coupling reaches the deep strong coupling regime. Finally, we also measure the energy spectrum of the quantum Rabi model in the ultrastrong coupling regime., Comment: 8 pages, 4 figures

Quantum field theories describe a variety of fundamental phenomena in physics. However, their study often involves cumbersome numerical simulations. Quantum simulators, on the other hand, may outperform classical computational capacities due to their potential scalability. Here we report an experimental realization of a quantum simulation of fermion–antifermion scattering mediated by bosonic modes, using a multilevel trapped ion, which is a simplified model of fermion scattering in both perturbative and non-perturbative quantum electrodynamics. The simulated model exhibits prototypical features in quantum field theory including particle pair creation and annihilation, as well as self-energy interactions. These are experimentally observed by manipulating four internal levels of a 171Yb+ trapped ion, where we encode the fermionic modes, and two motional degrees of freedom that simulate the bosonic modes. Our experiment establishes an avenue towards the efficient implementation of field modes, which may prove useful in studies of quantum field theories including non-perturbative regimes., Simulation of quantum field theory using quantum systems would in principle allow avoidance of the exponential overhead required for classical simulations. Here, the authors use a multilevel trapped ion to simulate the processes of self-interaction and particle-antiparticle creation/annihilation.

In this chapter, we illustrate how a trapped ion system can be used for the experimental study of quantum thermodynamics, in particular, quantum fluctuation of work. As technology of nano/micro scale develops, it becomes critical to understand thermodynamics at the quantum mechanical level. The trapped ion system is a representative physical platform to experimentally demonstrate quantum phenomena with excellent control and precision. We provide a basic introduction of the trapped ion system and present the theoretical framework for the experimental study of quantum thermodynamics. Then we bring out two concrete examples of the experimental demonstrations. Finally, we discuss the results and the future of the experimental study of quantum thermodynamics with trapped ion systems.

Quantum simulation of complex quantum systems and their properties often requires the ability to prepare initial states in an eigenstate of the Hamiltonian to be simulated. In addition, to compute the eigenvalues of a Hamiltonian is in general a non-trivial problem. Here, we propose a hybrid quantum-classical probabilistic method to compute eigenvalues and prepare eigenstates of Hamiltonians which are simulatable with a trapped-ion quantum processor., Comment: 9 pages, 6 figures

We show that a high-energy electron bunch can be used to capture the instantaneous longitudinal and transverse field structures of the highly transient, microscopic, laser-excited relativistic wake with femtosecond resolution. The spatiotemporal evolution of wakefields in a plasma density up ramp is measured and the reversal of the plasma wake, where the wake wavelength at a particular point in space increases until the wake disappears completely only to reappear at a later time but propagating in the opposite direction, is observed for the first time by using this new technique.

Although nonequilibrium work and fluctuation relations have been studied in detail within classical statistical physics, extending these results to open quantum systems has proven to be conceptually difficult. For systems that undergo decoherence but not dissipation, we argue that it is natural to define quantum work exactly as for isolated quantum systems, using the two-point measurement protocol. Complementing previous theoretical analysis using quantum channels, we show that the nonequilibrium work relation remains valid in this situation, and we test this assertion experimentally using a system engineered from an optically trapped ion. Our experimental results reveal the work relation's validity over a variety of driving speeds, decoherence rates, and effective temperatures and represent the first confirmation of the work relation for non-unitary dynamics., 21 pages, 7 figures

A quantum state is fully characterized by its density matrix or equivalently by its quasiprobabilities in phase space. A scheme to identify the quasiprobabilities of a quantum state is an important tool in the recent development of quantum technologies. One of the most fundamental interaction models in quantum optics is the so-called Jaynes-Cummings model (JCM), which has been massively studied theoretically and experimentally. However, the expected essential dynamics of the field states under the resonant JCM has not been observed experimentally due to the lack of a proper reconstruction scheme. In this paper, we further develop a highly efficient vacuum measurement scheme and study the JCM dynamics in a trapped ion system with the capability of the vacuum measurement to reconstruct its quasiprobability $Q$ function, which is a preferred choice to study the core of the dynamics of a quantum state in phase space. During the JCM dynamics, the Gaussian peak of the initial coherent state bifurcates and rotates around the origin of phase space. They merge at the so-called revival time at the other side of phase space. The measured $Q$ function agrees with the theoretical prediction. Moreover, we reconstruct the Wigner function by deconvoluting the $Q$ function and observe the quantum interference in the Wigner function at half of the revival time, where the vibrational state becomes nearly disentangled from the internal energy states and forms a superposition of two composite states. The scheme can be applied to other physical setups including cavity or circuit-QED and optomechanical systems.

Counterdiabatic driving (CD) exploits auxiliary control fields to tailor the nonequilibrium dynamics of a quantum system, making possible the suppression of dissipated work in finite-time thermodynamics and the engineering of optimal thermal machines with no friction. We show that while the mean work done by the auxiliary controls vanishes, CD leads to a broadening of the work distribution. We derive a fundamental inequality that relates nonequilibrium work fluctuations to the operation time and quantifies the thermodynamic cost of CD in both critical and noncritical systems., 5+3 pages, 3 figures

The past two decades witnessed important developments in the field of non-equilibrium statistical mechanics. Among these developments, the Jarzynski equality, being a milestone following the landmark work of Clausius and Kelvin, stands out. The Jarzynski equality relates the free energy difference between two equilibrium states and the work done on the system through far from equilibrium processes. While experimental tests of the equality have been performed in classical regime, the verification of the quantum Jarzynski equality has not yet been fully demonstrated due to experimental challenges. Here, we report an experimental test of the quantum Jarzynski equality with a single \Yb ion trapped in a harmonic potential. We perform projective measurements to obtain phonon distributions of the initial thermal state. Following that we apply the laser induced force on the projected energy eigenstate, and find transition probabilities to final energy eigenstates after the work is done. By varying the speed of applying the force from equilibrium to far-from equilibrium regime, we verified the quantum Jarzynski equality in an isolated system., 18 pages, 4 figures, 1 table

In the version of this Letter originally published, in Fig. 2c legend, the entry ‘LO phase noise’ should not have been included. This has now been corrected in the online versions.

A dynamic photo-thermal model of carbon dioxide (CO(2)) laser tissue ablation was developed, based on McKenzie's three-zone model, with the following improvements: (1) the laser-irradiated tissue from the surface to the inside was divided into a carbonized zone, a dried zone, a dehydrating zone, a thermally damaged wet (TDW) zone and an uncoagulated zone; (2) the carbonized and dried tissues were analyzed as porous media, with convection heat transfer between the vapor from the dehydrating tissue and the porous dried/carbonized tissue taken into account; (3) the interactions of temperature distribution, deposited laser energy distribution and dynamic changes in optical and thermal properties as well as blood perfusion rate were included. The finite difference method was used to solve numerically for the temperature and deposited laser energy fields, and the boundary positions of the zones.

A quantum simulator is an important device that may soon outperform current classical computations. A basic arithmetic operation, the complex conjugate, however, is considered to be impossible to be implemented in such a quantum system due to the linear character of quantum mechanics. Here, we present the experimental quantum simulation of such an unphysical operation beyond the regime of unitary and dissipative evolutions through the embedding of a quantum dynamics in the electronic multilevels of a 171Yb+ ion. We perform time reversal and charge conjugation, which are paradigmatic examples of antiunitary symmetry operators, in the evolution of a Majorana equation without the tomographic knowledge of the evolving state. Thus, these operations can be applied regardless of the system size. Our approach offers the possibility to add unphysical operations to the toolbox of quantum simulation, and provides a route to efficiently compute otherwise intractable quantities, such as entanglement monotones., Quantum simulation has the potential to enable experimentally studying problems which are not directly tractable in a laboratory or computationally. Here, the authors simulate the Majorana equation with a ytterbium ion, which requires them to simulate antiunitary and therefore unphysical operations.

In classical computational chemistry, the coupled-cluster ansatz is one of the most commonly used $ab~initio$ methods, which is critically limited by its non-unitary nature. The unitary modification as an ideal solution to the problem is, however, extremely inefficient in classical conventional computation. Here, we provide the first experimental evidence that indeed the unitary version of the coupled cluster ansatz can be reliably performed in physical quantum system, a trapped ion system. We perform a simulation on the electronic structure of a molecular ion (HeH$^+$), where the ground-state energy surface curve is probed, energies of excited-states are studied and the bond-dissociation is simulated non-perturbatively. Our simulation takes advantages from quantum computation to overcome the intrinsic limitations in classical computation and our experimental results indicate that the method is promising for preparing molecular ground-states for quantum simulation., Comment: 6 pages, 4 figures

We report the first experimental realization of the geometric Landau-Zener-St\"{u}ckelberg (LZS) interferometry proposed by [Phys. Rev. Lett. 107, 207002 (2011)] in a single trapped ion system. Different from a conventional LZS interferometer, the interference fringes of our geometric interferometer originate solely from geometric phase. We also observe the robustness of the interference contrast against noise or fluctuation in the experimental parameters. Our scheme can be applied to other complex systems subject to relatively large errors in system control., Comment: 5 pages, 4 figures