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In addition to describing our universe, gravitational theories profoundly inspire the study of emergent properties of exotic phases of matter. While the Anti-de Sitter/conformal field theory (AdS/CFT) correspondence is one of the most celebrated examples, the field of fractonic matter -- driven in part by gapless phases resembling linearized gravity -- has also seen rapid developments. Despite the deep implications of both areas, connections between them remain sparse, primarily due to the difficulty in constructing explicit models that encapsulate both fields' essential features. Here we demonstrate the efficacy of the recently proposed Hyperbolic Fracton Model as a concrete model for AdS/CFT duality. Using explicit numerical and analytical calculations on the discrete hyperbolic lattice, we show that the boundary state exhibits conformal field theory properties. Our main result is that bulk defects induce an emergent temperature for the boundary state, proportional to the defect perimeter, in quantitative agreement with the expected behaviour of a black hole in AdS spacetime. The Hyperbolic Fracton Model thus emerges as a unique lattice model of holographic principle equipped with a well-defined bulk Hamiltonian, and offers a promising gateway for studying a wide range of holographic phenomena., Comment: 6 pages, 7 figures

We investigate a simple variant of spin ice whose degenerate ground states are densely packed monopole configurations. An applied field drives this model through a Z2 confinement transition, in absence of any local order parameter. Instead, this hidden order turns out to be diagnosed by a string order invisible to any local probe. We describe the transition in terms of a bosonic field theory with a pairing term, as well as a Kramers-Wannier duality into a 3D Ising model, which establishes its Z2 nature. This topological transition can be thought of as a variant of the celebrated U(1) Kasteleyn transition; but instead of the traditional '3/2'-order kink, the system shows critical scaling expected near a 3D Ising transition. Remarkably, however, the magnetic response scales with the critical exponent not of the susceptibility, but of the specific heat.

The chromium spinels MgCr2O4 and ZnCr2O4 are prime examples of the highly frustrated pyrochlore lattice antiferromagnet. Experiment has carefully established that both materials, upon cooling, distort to lower symmetry and order magnetically. We study the nature of this process by a combination of density-functional-theory based energy mapping and classical Monte Carlo simulations. We first computationally establish precise Heisenberg Hamiltonian parameters for the high temperature cubic and the low temperature tetragonal and orthorhombic structures of both spinels. We then investigate the respective ordering temperatures of high symmetry and low symmetry structures. We carefully compare our results with experimental facts and find that our simulations are remarkably consistent with a type of spin-Peierls mechanism, adapted to three dimensions, where the structural distortion is mediated by a magnetic energy gain due to a lower degree of frustration.

Machine learning algorithms thrive on large data sets of good quality. Here we show that they can also excel in a typical research setting with little data of limited quality, through an interplay of insights coming from machine, and human researchers. The question we address is the unsolved problem of ordering out of a spin-liquid phase described by an emergent rank-2 $U(1)$ gauge theory, as described by [H. Yan it et al., Phys. Rev. Lett. 124, 127203 (2020)]. Published Monte Carlo simulations for this problem are consistent with a strong first-order phase transition, out of the R2-U1 spin liquid, but were too noisy for the form of low-temperature order to be identified. Using a highly-interpretable machine learning approach based on a support vector machine with a tensorial kernel (TKSVM), we re-analyze this Monte Carlo data, gaining new information about the form of order that could in turn be interpreted by traditionally-trained physicists. We find that the low-temperature ordered phase is a form of hybrid nematic order with emergent $Z_2$ symmetry, which allows for a sub-extensive set of domain walls at zero energy. This complex form of order arises due to a subtle thermal order-by-disorder mechanism, that can be understood from the fluctuations of the tensor electric field of the parent rank-2 gauge theory. These results were obtained by a back-and-forth process which closely resembles a collaboration between human researchers and machines. We argue that this "collaborative" approach may provide a blueprint for solving other problems that have not yielded to human insights alone.

The physics of skyrmions, and in particular the issue of how to isolate and manipulate them individually, is a subject of major importance nowadays in the community of magnetism. In this article we present an in-depth extension of a study on this issue that was recently proposed by some of the authors [H. D. Rosales, et al. Phys. Rev. Lett. \textbf{130}, 106703 (2023)]. More precisely, we analyse the competition between skyrmions and a chiral spin liquid in a model on the kagome lattice. We first present an analytical overview of the low-energy states using the Luttinger-Tisza approximation. We then study the effect of thermal fluctuations thanks to large-scale Monte-Carlo simulations, and explore the entire parameter space with a magnetic field $B$, in-plane $D^{xy}$ and out-of-plane $D^z$ Dzyaloshinskii-Moriya interactions. While skyrmions and the chiral spin liquid live in different regions of the parameter space, we show how to bring them together, stabilizing a skyrmion fluid in between; a region where the density of well-defined skyrmions can be tuned before obtaining an ordered phase. We investigate in particular the melting of the skyrmion solid. Our analysis also brings to light a long-range ordered phase with Z$_3$ symmetry. At last, we initiate the study of this rich magnetic background on conduction electrons that are coupled to the local spins. We study how the different chiral magnetic textures stabilized in this model (skyrmion solid, liquid and gas and chiral spin liquid) induce a topological Quantum Hall effect. We observe in the ordered skyrmion phase the appearance of Landau levels which persist even in the skyrmion-liquid regime and gradually disappear as the skyrmion density decreases to form a gas., Comment: 19 pages, 16 figures

The Curie-Weiss law is widely used to estimate the strength of frustration in frustrated magnets. However, the Curie-Weiss law was originally derived as an estimate of magnetic correlations close to a mean-field phase transition, which -- by definition -- is absent in spin liquids. Instead, the susceptibility of spin liquids is known to undergo a Curie-law crossover between two magnetically disordered regimes. Here, we study the generic aspect of the Curie-law crossover by comparing a variety of frustrated spin models in two and three dimensions, using both classical Monte Carlo simulations and analytical Husimi tree calculations. Husimi tree calculations fit remarkably well the simulations for all temperatures and almost all lattices. We also propose a Husimi Ansatz for the reduced susceptibility $\chi T$, to be used in complement to the traditional Curie-Weiss fit in order to estimate the Curie-Weiss temperature $\theta_{\rm cw}$. Applications to materials are discussed., Comment: 26 pages, 14 figures

The centred pyrochlore lattice is a novel geometrically frustrated lattice, realized in the metal-organic framework Mn(ta)$_2$ (arXiv:2203.08780) where the basic unit of spins is a five site centred tetrahedron. Here, we present an in-depth theoretical study of the $J_1-J_2$ classical Heisenberg model on this lattice, using a combination of mean-field analytical methods and Monte Carlo simulations. We find a rich phase diagram with low temperature states exhibiting ferrimagnetic order, partial ordering, and a highly degenerate spin liquid with distinct regimes of low temperature correlations. We discuss in detail how the regime displaying broadened pinch points in its spin structure factor is consistent with an effective description in terms of a fluid of interacting charges. We also show how this picture holds in two dimensions on the analogous centred kagome lattice and elucidate the connection to the physics of thin films in ($d+1$) dimensions. Furthermore, we show that a Coulomb phase can be stabilized on the centred pyrochlore lattice by the addition of further neighbour couplings. This demonstrates the centred pyrochlore lattice is an experimentally relevant geometry which naturally hosts emergent gauge fields in the presence of charges at low energies., Comment: 29 pages, 9 figures, resubmission to SciPost with minor revisions

We study the kagome antiferromagnet for quantum spin-1/2 with first J1, second J2 and third J3 neighbour exchanges, along the J2 = J3 = J line. We use Schwinger-boson mean-field theory for the precise determination of the phase diagram, and two different rewritings of the Hamiltonian to build an intuition about the origin of the transitions. The spin liquid obtained at J = 0 remains essentially stable over a large window, up to J = 1/3, because it is only weakly frustrated by the J term. Then at J = 1/2, the intermediate Z2 spin liquid condenses into a long-range chiral order because of the change of nature of local magnetic fluctuations. As a side benefit, our Hamiltonian rewriting offers an exact solution for the ground state of our model on a Husimi cactus., Comment: Last version before publication in PRB

Geometric frustration inhibits magnetic systems from ordering, opening a window to unconventional phases of matter. The paradigmatic frustrated lattice in three dimensions to host a spin liquid is the pyrochlore, although there remain few experimental compounds thought to realize such a state. Here we go beyond the pyrochlore via molecular design in the metal-azolate framework [Mn(II)(ta)$_2$], which realizes a closely related centred pyrochlore lattice of Mn-spins with $S=5/2$. Despite a Curie-Weiss temperature of $-21$ K indicating the energy scale of magnetic interactions, [Mn(II)(ta)$_2$] orders at only 430 mK, putting it firmly in the category of highly frustrated magnets. Comparing magnetization and specific heat measurements to numerical results for a minimal Heisenberg model, we predict that this material displays distinct features of a classical spin liquid with a structure factor reflecting Coulomb physics in the presence of charges., Comment: Main: 6 pages, 3 figures. Supplementary: 15 pages, 12 figures. Updated Version

$\rm Yb_2Ti_2O_7$ is a celebrated example of a pyrochlore magnet with highly-frustrated, anisotropic exchange interactions. To date, attention has largely focused on its unusual, static properties, many of which can be understood as coming from the competition between different types of magnetic order. Here we use inelastic neutron scattering with exceptionally high energy resolution to explore the dynamical properties of $\rm Yb_2Ti_2O_7$. We find that spin correlations exhibit dynamical scaling, analogous to behavior found near to a quantum critical point. We show that the observed scaling collapse can be explained within a phenomenological theory of multiple--phase competition, and confirm that a scaling collapse is also seen in semi--classical simulations of a microscopic model of $\rm Yb_2Ti_2O_7$. These results suggest a general picture for dynamics in systems with competing ground states., Comment: 5 pages, 4 figures, 8 pages supplememtnal materials

Skyrmions are of interest both from a fundamental and technological point of view, due to their potential to act as information carriers. But one challenge concerns their manipulation, especially at high temperature where thermal fluctuations eventually disintegrate them. Here we study the competition between skyrmions and a chiral spin liquid, using the latter as an entropic buffer to impose a quasi-vacuum of skyrmions. As a result, the temperature becomes a knob to tune the skyrmion density from a dense liquid to a diluted gas, protecting the integrity of each skyrmion from paramagnetic disintegration. With this additional knob in hand, we find at high field a topological spin glass made of zero- and one-dimensional topological defects (resp. skyrmions and bimerons)., Comment: 6 pages, 4 figures. Accepted in Physical Review Letters

While there is compelling evidence for the existence of magnetic monopoles in spin ice, the direct observation of a point-like source of magnetic field in these systems remains an open challenge. One promising approach is electron holography, which combines atomic-scale resolution with extreme sensitivity to magnetic vector potentials, through the Aharonov-Bohm effect. Here we explore what holography can teach us about magnetic monopoles in spin ice, through experiments on artificial spin ice, and numerical simulations of pyrochlore spin ice. In the case of artificial spin ice, we show that holograms can be used to measure local magnetic charge. For pyrochlore spin ice, we demonstrate that holographic experiments are capable of resolving both magnetic monopoles and their dynamics, including the emergence of electric fields associated with fluctuations of closed loops of spins. These results establish that the observation of both magnetic monopoles and emergent electric fields in pyrochlore spin ice is a realistic possibility in an electron microscope with sufficiently--high phase resolution., Comment: 9 pages, 5 figures in main paper. 11 pages, 11 figures in supplemental V2: Updated citations and further details in supplemental

Machine-learning techniques have proved successful in identifying ordered phases of matter. However, it remains an open question how far they can contribute to the understanding of phases without broken symmetry, such as spin liquids. Here we demonstrate how a machine learning approach can automatically learn the intricate phase diagram of a classical frustrated spin model. The method we employ is a support vector machine equipped with a tensorial kernel and a spectral graph analysis which admits its applicability in an effectively unsupervised context. Thanks to the interpretability of the machine we are able to infer, in closed form, both order parameter tensors of phases with broken symmetry, and the local constraints which signal an emergent gauge structure, and so characterize classical spin liquids. The method is applied to the classical XXZ model on the pyrochlore lattice where it distinguishes---among others---between a hidden biaxial spin nematic phase and several different classical spin liquids. The results are in full agreement with a previous analysis by Taillefumier \emph{et al.} [Phys. Rev. X 7, 041057 (2017)], but go further by providing a systematic hierarchy between disordered regimes, and establishing the physical relevance of the susceptibilities associated with the local constraints. Our work paves the way for the search of new orders and spin liquids in generic frustrated magnets., Comment: v3: expanded discussions of interpretability; as published; 22 pages, 15 figures, 3 tables

Higher-rank generalisations of electrodynamics have recently attracted considerable attention because of their ability to host "fracton" excitations, with connections to both quantum stabilizer codes and holography. However, the search for higher-rank gauge theories in experiment has been greatly hindered by the lack of materially-relevant microscopic models. Here we show how a spin liquid described by rank-2 $U(1)$ gauge theory can arise in a magnet on the breathing pyrochlore lattice. We identify Yb-based breathing pyrochlores as candidate systems, and make explicit predictions for how the rank-2 $U(1)$ spin liquid would manifest itself in experiment., Comment: 5 pages, 4 figures, with supplemental material. To appear on Phys. Rev. Lett

We study the formation of magnetic clusters in frustrated magnets in their cooperative paramagnetic regime. For this purpose, we consider the $J_1$-$J_2$-$J_3$ classical Heisenberg model on kagome and pyrochlore lattices with $J_2 = J_3=J$. In the absence of farther-neighbor couplings, $J=0$, the system is in the Coulomb phase with magnetic correlations well characterized by pinch-point singularities. Farther-neighbor couplings lead to the formation of magnetic clusters, which can be interpreted as a counterpart of topological-charge clusters in Ising frustrated magnets [T. Mizoguchi, L. D. C. Jaubert and M. Udagawa, Phys. Rev. Lett. {\bf 119}, 077207 (2017)]. The concomitant static and dynamical magnetic structure factors, respectively $\mathcal{S}({\bm{q}})$ and $\mathcal{S}({\bm{q}},\omega)$, develop half-moon patterns. As $J$ increases, the continuous nature of the Heisenberg spins enables the half-moons to coalesce into connected `star' structures spreading across multiple Brillouin zones. These characteristic patterns are a dispersive complement of the pinch point singularities, and signal the proximity to a Coulomb phase. Shadows of the pinch points remain visible at finite energy, $\omega$. This opens the way to observe these clusters through (in)elastic neutron scattering experiments. The origin of these features are clarified by complementary methods: large-$N$ calculations, semi-classical dynamics of the Landau-Lifshitz equation, and Monte Carlo simulations. As promising candidates to observe the clustering states, we revisit the origin of "spin molecules" observed in a family of spinel oxides $AB_2$O$_4$ ($A=$ Zn, Hg, Mg, $B=$ Cr, Fe)., Comment: 23 pages, 27 figures

Fractionalization is a ubiquitous phenomenon in topological states of matter. In this work, we study the collective behavior of fractionalized topological charges and their instabilities, through the $J_1$-$J_2$-$J_3$ Ising model on a kagome lattice, which can be mapped to a model of interacting topological charges under the constraint of Gauss' law. We find that the recombination of topological charges gives rise to a yet unexplored classical spin liquid. This spin liquid is characterized by an extensive residual entropy, as well as the formation of hexamers of same-sign topological charges. The emergence of hexamers is reflected to a half-moon signal in the magnetic structure factor, which provides us a signature of this new spin liquid in neutron-scattering experiments. To study this phase, a worm algorithm has been developed which does not require the usual divergence-free condition., Comment: 5 pages, 3 figures for the main text, and 6 pages, 8 figures for Supplemental Material

The family of magnetic rare-earth pyrochlore oxides R2M2O7 plays host to a diverse array of exotic phenomena, driven by the interplay between geometrical frustration and spin-orbit interaction, which leads to anisotropy in both magnetic moments and their interactions. In this article we establish a general, symmetry--based theory of pyrochlore magnets with anisotropic exchange interactions. Starting from a very general model of nearest-neighbour exchange between Kramers ions, we find four distinct classical ordered states, all with q=0, competing with a variety of spin-liquids and unconventional forms of magnetic order. The finite-temperature phase diagram of this model is determined by Monte Carlo simulation, supported by classical spin-wave calculations. We pay particular attention to the region of parameter space relevant to the widely studied materials Er2Ti2O7, Yb2Ti2O7, and Er2Sn2O7. We find that many of the most interesting properties of these materials can be traced back to the "accidental" degeneracies where phases with different symmetries meet. These include the ordered ground state selection by fluctuations in Er2Ti2O7, the dimensional-reduction observed in Yb2Ti2O7, and the lack of reported magnetic order in Er2Sn2O7. We also discuss the application of this theory to other pyrochlore oxides., Comment: Long-paper version of "Living on the Edge", arXiv:1311.3501. 41 pages, 27 figures. Accepted for publication in Physical Review B

We study the interplay of topological bottlenecks and energetic barriers to equilibration in a Coulomb spin liquid where a short-range energetic coupling between defects charged under an emergent gauge field supplements their entropic long-range Coulomb interaction. This work is motivated by the prevalence of memory effects observed across a wide range of geometrically frustrated magnetic materials, possibly including the spontaneous Hall effect observed in Pr2Ir2O7. Our model is canonical spin-ice model on the pyrochlore lattice, where farther-neighbour spin couplings give rise to a nearest-neighbor interaction between topological defects which can easily be chosen to be unnatural or not, i.e. attractive or repulsive between defects of equal gauge charge. Among the novel features of this model are the following. After applying a field quench, a rich dynamical approach to equilibrium emerges, dominated by multi-scale energy barriers responsible for long-lived magnetization plateaux. These even allow for the metastability of a "fragmented" spin liquid, an elusive regime where partial order co-exists with a spin liquid. Perhaps most strikingly, the attraction produces clusters of defects whose stability is due to a combination of energetic barriers for their break-up and proximity of opposite charges along with an entropic barrier generated by the topological requirement of annihilating a defect only together with an oppositely charged counterpart. These clusters may take the form of a "jellyfish" spin texture, comprising an arrangement of same-sign gauge-charges, centered on a hexagonal ring with branches of arbitrary length. The ring carries a clockwise or counterclockwise circular flow of magnetisation. This emergent toroidal degrees of freedom provides a possibility for time reversal symmetry breaking with possible relevance to the spontaneous Hall effect observed in Pr2Ir2O7., Comment: 27 pages, 31 figures

If spin liquids have been famously defined by what they are not, i.e. ordered, the past years have seen the frontier between order and spin liquid starting to fade, with a growing number of materials whose low-temperature physics cannot be explained without co-existence of (partial) magnetic order and spin fluctuations. Here we study an example of such co-existence in the presence of magnetic dipolar interactions, related to spin ice, where the order is long range and the fluctuations support a Coulomb gauge field. Topological defects are effectively coupled via energetic and entropic Coulomb interactions, the latter one being stronger than for the spin-ice ground state. Depending on whether these defects break the divergence-free condition of the Coulomb gauge field or the long-range order, they are respectively categorized as monopoles - as in spin ice - or monopole holes, in analogy with electron holes in semiconductors. The long-range order plays the role of a fully-occupied valence band, while the Coulomb spin liquid can be seen as an empty conducting band. These results are discussed in the context of other lattices and models which support a similar co-existence of Coulomb gauge field and long-range order. We conclude this work by explaining how dipolar interactions lift the spin liquid degeneracy at very low energy scale by maximizing the number of flippable plaquettes, in light of the equivalent quantum dimer model., Comment: invited paper for the special issue on "Quantum Spin Ice and Liquid in Geometrically Frustrated Magnets" edited by Y.-J. Kao, S. Onoda and S. Nakatsuji

The mathematics of gauge theories lies behind many of the most profound advances in physics in the last 200 years, from Maxwell's theory of electromagnetism to Einstein's theory of general relativity. More recently it has become clear that gauge theories also emerge in condensed matter, a prime example being the spin ice materials which host an emergent electromagnetic gauge field. In spin ice, the underlying gauge structure is revealed by the presence of pinch-point singularities in neutron-scattering measurements. Here we report the discovery of a spin liquid where the low-temperature physics is naturally described by the fluctuations of a tensor field with a continuous gauge freedom. This gauge structure underpins an unusual form of spin correlations, giving rise to pinch-line singularities--- line-like analogues of the pinch-points observed in spin ice. Remarkably, these features may already have been observed in the pyrochlore material Tb$_2$Ti$_2$O$_7$., Comment: 4 pages of main text, 3 figures

The kagome lattice sits at the crossroad of present research efforts in quantum spin liquids, chiral phases, emergent skyrmion excitations and anomalous Hall effects to name but a few. In light of this diversity, our goal in this paper is to build a unifying picture of the underlying magnetic degrees-of-freedom on kagome. Motivated by a growing mosaic of materials, we especially consider a broad range of nearest-neighbour interactions consisting of Dzyaloshinskii-Moriya as well as anisotropic ferro$-$ and antiferromagnetic coupling. We present a three-fold mapping on the kagome lattice which transforms the celebrated Heisenberg antiferromagnet and XXZ model onto two lines of time-reversal invariant Hamiltonians. The mapping is exact for classical and quantum spins alike, i.e. it preserves the energy spectrum of the original Heisenberg and XXZ models. As a consequence, at the classical level, all phases have an extensive ground-state degeneracy. These ground states support a variety of phenomena such as ferromagnetically induced pinch points in the structure factor and the possibility for spontaneous scalar chirality. For quantum spin$-1/2$, the XXZ model has been recently shown to be a quantum spin liquid. Applying our three-fold mapping to the XXZ model gives rise to a connected network of quantum spin liquids, centered around a paragon of quantum disorder, namely the Ising antiferromagnet. We show that this quantum disorder spreads over an extended region of the phase diagram at linear order in spin wave theory, which overlaps with the parameter region of Herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$. We conclude this work by discussing the connection of our results to the chiral spin liquids found on kagome with further nearest-neighbour interactions, and to the recently synthesized ternary intermetallic materials., Comment: 8 pages, 4 figures

We combine two aspects of magnetic frustration, multiferroicity and emergent quasi-particles in spin liquids, by studying magneto-electric monopoles. Spin ice offers to couple these emergent topological defects to external fields, and to each other, in unusual ways, making possible to lift the degeneracy underpinning the spin liquid and to potentially stabilize novel forms of charge crystals, opening the path to a "magnetic crystallography". In developing the general phase diagram including nearest-neighbour coupling, Zeeman energy, electric and magnetic dipolar interactions, we uncover the emergence of a bi-layered crystal of singly-charged monopoles, whose stability, remarkably, is strengthened by an external [110] magnetic field. Our theory is able to account for the ordering process of Tb2Ti2O7 in large field for reasonably small electric energy scales., Comment: 10 pages, 10 figures

The search for new quantum phases, especially in frustrated magnets, is central to modern condensed matter physics. One of the most promising places to look is in rare-earth pyrochlore magnets with highly-anisotropic exchange interactions, materials closely related to the spin ices Ho2Ti2O7 and Dy2Ti2O7. Here we establish a general theory of magnetic order in these materials. We find that many of their most interesting properties can be traced back to the accidental degeneracies where phases with different symmetry meet. These include the ordered ground state selection by fluctuations in Er2Ti2O7, the dimensional-reduction observed in Yb2Ti2O7, and the absence of magnetic order in Er2Sn2O7., Comment: A long-paper version of this preprint, "Living on the Edge", appears as arXiv:1603.09466 [accepted for publication in Physical Review B]. The text of v2 is otherwise unchanged from v1 (Submitted on 14 Nov 2013)

The Coulomb phase, with its dipolar correlations and pinch-point-scattering patterns, is central to discussions of geometrically frustrated systems, from water ice to binary and mixed-valence alloys, as well as numerous examples of frustrated magnets. The emergent Coulomb phase of lattice-based systems has been associated with divergence-free fields and the absence of long-range order. Here, we go beyond this paradigm, demonstrating that a Coulomb phase can emerge naturally as a persistent fluctuating background in an otherwise ordered system. To explain this behavior, we introduce the concept of the fragmentation of the field of magnetic moments into two parts, one giving rise to a magnetic monopole crystal, the other a magnetic fluid with all the characteristics of an emergent Coulomb phase. Our theory is backed up by numerical simulations, and we discuss its importance with regard to the interpretation of a number of experimental results.

At low temperatures, a spin ice enters a Coulomb phase - a state with algebraic correlations and topologically constrained spin configurations. In Ho2Ti2O7, we have observed experimentally that this process is accompanied by a non-standard temperature evolution of the wave vector dependent magnetic susceptibility, as measured by neutron scattering. Analytical and numerical approaches reveal signatures of a crossover between two Curie laws, one characterizing the high temperature paramagnetic regime, and the other the low temperature topologically constrained regime, which we call the spin liquid Curie law. The theory is shown to be in excellent agreement with neutron scattering experiments. On a more general footing, i) the existence of two Curie laws appears to be a general property of the emergent gauge field for a classical spin liquid, and ii) sheds light on the experimental difficulty of measuring a precise Curie-Weiss temperature in frustrated materials; iii) the mapping between gauge and spin degrees of freedom means that the susceptibility at finite wave vector can be used as a local probe of fluctuations among topological sectors., Comment: 10 pages, 5 figures

One of the most remarkable examples of emergent quasi-particles, is that of the "fractionalization" of magnetic dipoles in the low energy configurations of materials known as "spin ice", into free and unconfined magnetic monopoles interacting via Coulomb's 1/r law [Castelnovo et. al., Nature, 451, 42-45 (2008)]. Recent experiments have shown that a Coulomb gas of magnetic charges really does exist at low temperature in these materials and this discovery provides a new perspective on otherwise largely inaccessible phenomenology. In this paper, after a review of the different spin ice models, we present detailed results describing the diffusive dynamics of monopole particles starting both from the dipolar spin ice model and directly from a Coulomb gas within the grand canonical ensemble. The diffusive quasi-particle dynamics of real spin ice materials within "quantum tunneling" regime is modeled with Metropolis dynamics, with the particles constrained to move along an underlying network of oriented paths, which are classical analogues of the Dirac strings connecting pairs of Dirac monopoles., Comment: 26 pages, 12 figures

We study the low-temperature behaviour of spin ice when uniaxial pressure induces a tetragonal distortion. There is a phase transition between a Coulomb liquid and a fully magnetised phase. Unusually, it combines features of discontinuous and continuous transitions: the order parameter exhibits a jump, but this is accompanied by a divergent susceptibility and vanishing domain wall tension. All these aspects can be understood as a consequence of an emergent SU(2) symmetry at the critical point. We map out a possible experimental realisation.

We discuss the nearest neighbour spin ice model in the presence of a magnetic field placed along the cubic [100] direction. As recently shown in Phys. Rev. Lett. 100, 067207, 2008, the symmetry sustaining ordering transition observed at low temperature is a three dimensional Kasteleyn transition. We confirm this with numerical data using a non-local algorithm that conserves the topological constraints at low temperature and from analytic calculations from a Bethe lattice of corner sharing tetrahedra . We present a thermodynamic description of the Kasteleyn transition and discuss the relevance of our results to recent neutron scattering experiments on spin ice materials.

Magnetic monopoles have eluded experimental detection since their prediction nearly a century ago by Dirac. Recently it has been shown that classical analogues of these enigmatic particles occur as excitations out of the topological ground state of a model magnetic system, dipolar spin ice. These quasi-particle excitations do not require a modification of Maxwell's equations, but they do interact via Coulombs law and are of magnetic origin. In this paper we present an experimentally measurable signature of monopole dynamics and show that magnetic relaxation measurements in the spin ice material $Dy_{2}Ti_{2}O_{7}$ can be interpreted entirely in terms of the diffusive motion of monopoles in the grand canonical ensemble, constrained by a network of "Dirac strings" filling the quasi-particle vacuum. In a magnetic field the topology of the network prevents charge flow in the steady state, but there is a monopole density gradient near the surface of an open system.

We examine the statistical mechanics of spin-ice materials with a [100] magnetic field. We show that the approach to saturated magnetisation is, in the low-temperature limit, an example of a 3D Kasteleyn transition, which is topological in the sense that magnetisation is changed only by excitations that span the entire system. We study the transition analytically and using a Monte Carlo cluster algorithm, and compare our results with recent data from experiments on Dy2Ti2O7., Comment: 4 pages, 5 figures

We study numerically spatio-temporal fluctuations during the out-of-equilibrium relaxation of the three-dimensional Edwards-Anderson model. We focus on two issues. (1) The evolution of a growing dynamical length scale in the glassy phase of the model, and the consequent collapse of the distribution of local coarse-grained correlations measured at different pairs of times on a single function using {\it two} scaling parameters, the value of the global correlation at the measuring times and the ratio of the coarse graining length to the dynamical length scale (in the thermodynamic limit). (2) The `triangular' relation between coarse-grained local correlations at three pairs of times taken from the ordered instants $t_3 \leq t_2 \leq t_1$. Property (1) is consistent with the conjecture that the development of time-reparametrization invariance asymptotically is responsible for the main dynamic fluctuations in aging glassy systems as well as with other mechanisms proposed in the literature. Property (2), we stress, is a much stronger test of the relevance of the time-reparametrization invariance scenario., Comment: 24 pages, 12 figs