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Recent research shows that quasiparticle-induced decoherence of superconducting qubits depends on the superconducting-gap asymmetry originating from the different thicknesses of the top and bottom films in Al/AlO$_x$/Al junctions. Magnetic field is a key tuning knob to investigate this dependence as it can change the superconducting gaps in situ. We present measurements of the parity-switching time of a field-resilient 3D transmon with in-plane field up to 0.41T. At low fields, small parity splitting requires qutrit pulse sequences for parity measurements. We measure a non-monotonic evolution of the parity lifetime with in-plane magnetic field, increasing up to 0.2T, followed by a decrease at higher fields. We demonstrate that the superconducting-gap asymmetry plays a crucial role in the observed behavior. At zero field, the qubit frequency is nearly resonant with the superconducting-gap difference, favoring the energy exchange with the quasiparticles and so enhancing the parity-switching rate. With a higher magnetic field, the qubit frequency decreases and gets detuned from the gap difference, causing the initial increase of the parity lifetime, while photon-assisted qubit transitions increase, producing the subsequent decrease at higher fields. Besides giving a deeper insight into the parity-switching mechanism in conventional transmon qubits, we establish that Al-AlO$_x$-Al JJs could be used in architectures for the parity-readout and manipulation of topological qubits based on Majorana zero modes.

We investigate the effect of magnetic field on a photonic-crystal Josephson traveling-wave parametric amplifier (TWPA). We show that the observed change in photonic bandgap and plasma frequency of the TWPA can be modeled by considering the suppression of the critical current in the Josephson junctions (JJs) of the TWPA due to the Fraunhofer effect and closing of the superconducting gap. Accounting for the JJ geometry is crucial for understanding the field dependence. In one in-plane direction, the TWPA bandgap can be shifted by 2 GHz using up to 60 mT of field, without losing gain or bandwidth, showing that TWPAs without SQUIDs can be field tunable. In the other in-plane direction, the magnetic field is perpendicular to the larger side of the Josephson junctions, so the Fraunhofer effect has a smaller period. This larger side of the JJs is modulated to create the bandgap. The field interacts more strongly with the larger junctions, and as a result, the TWPA bandgap closes and reopens as the field increases, causing the TWPA to become severely compromised already at 2 mT. A slightly higher operating limit of 5 mT is found in out-of-plane field, for which the TWPA's response is hysteretic. These measurements reveal the requirements for magnetic shielding needed to use TWPAs in experiments where high fields at the sample are required; we show that with magnetic shields we can operate the TWPA while applying over 2 T to the sample.

The first JWST observations of hot Jupiters showed an unexpected detection of SO2 in their hydrogen-rich atmospheres. We investigate how much sulphur can be expected in the atmospheres of rocky exoplanets and which sulphur molecules can be expected to be most abundant and detectable by transmission spectroscopy. We run thermo-chemical equilibrium models at the crust-atmosphere interface, considering surface temperatures 500 to 5000 K, surface pressures 1 to 100 bar, and various sets of element abundances based on common rock compositions. Between 1000 K and 2000 K, we find gaseous sulphur concentrations of up to 25 percent above the rock in our models. SO2, SO, H2S and S2 are by far the most abundant sulphur molecules. SO2 shows potentially detectable features in transmission spectra at about 4 micron, between 7 and 8 micron, and beyond 15 micron. In contrast, the sometimes abundant H2S molecule is difficult to detect in these spectra, which are mostly dominated by H2O and CO2. Although the molecule PS only occurs with concentrations below 300 ppm, it can cause a strong absorption feature between 0.3 and 0.65 micron in some of our models for high surface pressures. The detection of sulphur molecules would enable a better characterisation of the planetary surface., Comment: Typos have been corrected compared to version 1

The mode-coupling theory of the glass transition (MCT) has been at the forefront of fundamental glass research for decades, yet the theory's underlying approximations remain obscure. Here we quantify and critically assess the effect of each MCT approximation separately. Using Brownian dynamics simulations, we compute the memory kernel predicted by MCT after each approximation in its derivation, and compare it with the exact one. We find that some often-criticized approximations are in fact very accurate, while the opposite is true for others, providing new guiding cues for further theory development.

High-resolution thermal expansion and magnetostriction measurements were performed on single crystals of $\alpha$-RuCl$_3$ in magnetic fields applied parallel to the Ru-Ru bonds. The length changes were measured in the direction perpendicular to the honeycomb planes. Our data show clear thermodynamic characteristics for the field-induced phase transition at the critical field $\mu_0H_{c1} = 7.8(2)$ T where the antiferromagnetic zigzag order is suppressed. At higher fields, a kink in the magnetostriction coefficient signals an additional phase transition around $\mu_0H_{c2} \approx 11$ T. The extracted Gr\"uneisen parameter shows typical hallmarks for quantum criticality near $H_{c1}$, but also displays anomalous behavior above $H_{c1}$. We compare our experimental data with linear spin-wave calculations employing a minimal Kitaev-Heisenberg model in the semiclassical limit. Most of the salient features are in agreement with each other, however, the peculiar features in the high-field region above $H_{c1}$ cannot be accounted for in our modelling and hence suggest a genuine quantum nature. We construct a phase diagram for $\alpha$-RuCl$_3$ showing two low-temperature transitions induced by an in-plane field along the Ru-Ru bonds., Comment: 14 pages, 10 figures

Frustrated magnets with strong spin-orbit coupling promise to host topological states of matter, with fractionalized excitations and emergent gauge fields. Kitaev's proposal for a honeycomb-lattice Majorana spin liquid has triggered an intense search for experimental realizations, with bond-dependent Ising interaction being the essential building block. A prime candidate is $\alpha$-RuCl$_3$ whose phase diagram in a magnetic field is, however, not understood to date. Here we present conclusive experimental evidence for a novel field-induced ordered phase in $\alpha$-RuCl$_3$, sandwiched between the zigzag and quantum disordered phases at low and high fields, respectively. We provide a detailed theoretical study of the relevant effective spin model which we show to display a field-induced intermediate phase as well. We fully characterize the intermediate phase within this model, including its complex spin structure, and pinpoint the parameters relevant to $\alpha$-RuCl$_3$ based on the experimentally observed critical fields. Most importantly, our study connects the physics of $\alpha$-RuCl$_3$ to that of the Kitaev-$\Gamma$ model, which displays a quantum spin liquid phase in zero field, and hence reveals the spin liquid whose signatures have been detected in a variety of dynamical probes of $\alpha$-RuCl$_3$., Comment: This article is superseded by arXiv:2012.15258, which presents neutron diffraction data obtained after this preprint was posted. This data revealed that the intermediate ordered state is characterized by a different periodicity in the direction perpendicular to the honeycomb layers requiring a 3D model

$\alpha$-RuCl$_3$ has attracted enormous attention since it has been proposed as a prime candidate to study fractionalized magnetic excitations akin to Kitaev's honeycomb-lattice spin liquid. We have performed a detailed specific-heat investigation at temperatures down to $0.4$ K in applied magnetic fields up to $9$ T for fields parallel to the $ab$ plane. We find a suppression of the zero-field antiferromagnetic order, together with an increase of the low-temperature specific heat, with increasing field up to $\mu_0H_c\approx 6.9$ T. Above $H_c$, the magnetic contribution to the low-temperature specific heat is strongly suppressed, implying the opening of a spin-excitation gap. Our data point toward a field-induced quantum critical point (QCP) at $H_c$; this is supported by universal scaling behavior near $H_c$. Remarkably, the data also reveal the existence of a small characteristic energy scale well below $1$~meV above which the excitation spectrum changes qualitatively. We relate the data to theoretical calculations based on a $J_1$--$K_1$--$\Gamma_1$--$J_3$ honeycomb model., Comment: 5 pages, 4 figures (main text), plus Supplemental Material

Interacting fermions on a lattice can develop strong quantum correlations, which lie at the heart of the classical intractability of many exotic phases of matter. Seminal efforts are underway in the control of artificial quantum systems, that can be made to emulate the underlying Fermi-Hubbard models. Electrostatically confined conduction band electrons define interacting quantum coherent spin and charge degrees of freedom that allow all-electrical pure-state initialisation and readily adhere to an engineerable Fermi-Hubbard Hamiltonian. Until now, however, the substantial electrostatic disorder inherent to solid state has made attempts at emulating Fermi-Hubbard physics on solid-state platforms few and far between. Here, we show that for gate-defined quantum dots, this disorder can be suppressed in a controlled manner. Novel insights and a newly developed semi-automated and scalable toolbox allow us to homogeneously and independently dial in the electron filling and nearest-neighbour tunnel coupling. Bringing these ideas and tools to fruition, we realize the first detailed characterization of the collective Coulomb blockade transition, which is the finite-size analogue of the interaction-driven Mott metal-to-insulator transition. As automation and device fabrication of semiconductor quantum dots continue to improve, the ideas presented here show how quantum dots can be used to investigate the physics of ever more complex many-body states.