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Strange metals possess transport properties that are markedly different from those of a conventional Fermi liquid. Despite strong similarities in behavior exhibited by distinct families, a consistent description of strange metallic transport and, in particular, its evolution from low to high magnetic field strength H, is still lacking. The electron nematic FeSe1−xSx is one such strange metal displaying anomalous H/T scaling in its transverse magnetoresistance as well as a separation of transport and Hall lifetimes at low H beyond its (nematic) quantum critical point at xc ∼ 0.17. Here we report a study of the Hall response of FeSe1−xSx across xc in fields up to 33 T. Upon subtraction of a normal H-linear component from the total Hall response (imposed by perfect charge compensation), we find a second component, ascribable to strange metal physics, that grows as 1/T upon approach to the quantum critical point. Through this decomposition, we reveal that lifetime separation is indeed driven primarily by the presence of the strange metal component.

Cadmium arsenide Cd$_3$As$_2$ hosts massless Dirac electrons in its ambient-conditions tetragonal phase. We report X-ray diffraction and electrical resistivity measurements of Cd$_3$As$_2$ upon cycling pressure beyond the critical pressure of the tetragonal phase and back to ambient conditions. We find that at room temperature the transition between the low- and high-pressure phases results in large microstrain and reduced crystallite size both on rising and falling pressure. This leads to non-reversible electronic properties including self-doping associated with defects and a reduction of the electron mobility by an order of magnitude due to increased scattering. Our study indicates that the structural transformation is sluggish and shows a sizable hysteresis of over 1~GPa. Therefore, we conclude that the transition is first-order reconstructive, with chemical bonds being broken and rearranged in the high-pressure phase. Using the diffraction measurements we demonstrate that annealing at ~200$^\circ$C greatly improves the crystallinity of the high-pressure phase. We show that its Bragg peaks can be indexed as a primitive orthorhombic lattice with a_HP~8.68 A b_HP~17.15 A and c_HP~18.58 A. The diffraction study indicates that during the structural transformation a new phase with another primitive orthorhombic structure may be also stabilized by deviatoric stress, providing an additional venue for tuning the unconventional electronic states in Cd3As2., 12 pages with 7 figures

Strange metals possess highly unconventional transport characteristics, such as a linear-in-temperature ($T$) resistivity, an inverse Hall angle that varies as $T^2$ and a linear-in-field ($H$) magnetoresistance. Identifying the origin of these collective anomalies has proved profoundly challenging, even in materials such as the hole-doped cuprates that possess a simple band structure. The prevailing dogma is that strange metallicity in the cuprates is tied to a quantum critical point at a doping $p*$ inside the superconducting dome. Here, we study the high-field in-plane magnetoresistance of two superconducting cuprate families at doping levels beyond $p*$. At all dopings, the magnetoresistance exhibits quadrature scaling and becomes linear at high $H/T$ ratios. Moreover, its magnitude is found to be much larger than predicted by conventional theory and insensitive to both impurity scattering and magnetic field orientation. These observations, coupled with analysis of the zero-field and Hall resistivities, suggest that despite having a single band, the cuprate strange metal phase hosts two charge sectors, one containing coherent quasiparticles, the other scale-invariant `Planckian' dissipators., Comment: 20 pages, 9 figures and 3 tables (including Supplementary Information)

There is now compelling evidence that the normal state of superconducting overdoped cuprates is a strange metal comprising two distinct charge sectors, one governed by coherent quasiparticle excitations, the other seemingly incoherent and characterized by non-quasiparticle (Planckian) dissipation. The zero-temperature superfluid density n_s(0)ns(0) of overdoped cuprates exhibits an anomalous depletion with increased hole doping pp, falling to zero at the edge of the superconducting dome. Over the same doping range, the effective zero-temperature Hall number n_{\rm H}(0) transitions from pp to 1 + pp. By taking into account the presence of these two charge sectors, we demonstrate that in the overdoped cuprates Tl_22Ba_22CuO_{6+\delta}6+δ and La_{2-x}2−xSr_xxCuO_44, the growth in n_s(0)ns(0) as pp is decreased from the overdoped side may be compensated by the loss of carriers in the coherent sector. Such a correspondence is contrary to expectations from conventional BCS theory and implies that superconductivity in overdoped cuprates emerges uniquely from the sector that exhibits incoherent transport in the normal state.

Unambiguous and complete determination of the Fermi surface is a primary step in understanding the electronic properties of topical metals and semi-metals, but only in a relatively few cases has this goal been realized. In this work, we present a systematic high-field quantum oscillation study up to 35 T on ZrSiS, a textbook example of a nodal-line semimetal with only linearly dispersive bands crossing the Fermi energy. The topology of the Fermi surface is determined with unprecedented precision and all pockets are identified by comparing the measured angle dependence of the quantum oscillations to density functional theory calculations. Comparison of the Shubnikov-de Haas and de Haas-van Alphen oscillations at low temperatures and analysis of the respective Dingle plots reveal the presence of significantly enhanced scattering on the electron pocket. Above a threshold field that is aligned along the c-axis of the crystal, the specific cage-like Fermi surface of ZrSiS allows for electron-hole tunneling to occur across finite gaps in momentum space leading to quantum oscillations with a complex frequency spectrum. Additional high-frequency quantum oscillations signify magnetic breakdown orbits that encircle the entire Dirac nodal loop. We suggest that the persistence of quantum oscillations in the resistivity to high temperatures is caused by Stark interference between orbits of nearly equal masses., Comment: 14 pages, 13 figures

The recent discovery of a non-magnetic nematic quantum critical point (QCP) in the iron chalcogenide family FeSe$_{1-x}$S$_{x}$ has raised the prospect of investigating, in isolation, the role of nematicity on the electronic properties of correlated metals. Here we report a detailed study of the normal state transverse magnetoresistance (MR) in FeSe$_{1-x}$S$_{x}$ for a series of S concentrations spanning the nematic QCP. For all temperatures and \textit{x}-values studied, the MR can be decomposed into two distinct components: one that varies quadratically in magnetic field strength $\mu_{0}\textit{H}$ and one that follows precisely the quadrature scaling form recently reported in metals at or close to a QCP and characterized by a \textit{H}-linear MR over an extended field range. The two components evolve systematically with both temperature and S-substitution in a manner that is determined by their proximity to the nematic QCP. This study thus reveals unambiguously the coexistence of two independent charge sectors in a quantum critical system. Moreover, the quantum critical component of the MR is found to be less sensitive to disorder than the quadratic (orbital) MR, suggesting that detection of the latter in previous MR studies of metals near a QCP may have been obscured., Comment: 19 pages (including Supplemental Material), 12 figures

Correlated electron systems are highly susceptible to various forms of electronic order. By tuning the transition temperature towards absolute zero, striking deviations from conventional metallic (Fermi-liquid) behaviour can be realized. Evidence for electronic nematicity, a correlated electronic state with broken rotational symmetry, has been reported in a host of metallic systems1–5 that exhibit this so-called quantum critical behaviour. In all cases, however, the nematicity is found to be intertwined with other forms of order, such as antiferromagnetism5–7 or charge-density-wave order8, that might themselves be responsible for the observed behaviour. The iron chalcogenide FeSe1−xSx is unique in this respect because its nematic order appears to exist in isolation9–11, although until now, the impact of nematicity on the electronic ground state has been obscured by superconductivity. Here we use high magnetic fields to destroy the superconducting state in FeSe1−xSx and follow the evolution of the electrical resistivity across the nematic quantum critical point. Classic signatures of quantum criticality are revealed: an enhancement in the coefficient of the T2 resistivity (due to electron–electron scattering) on approaching the critical point and, at the critical point itself, a strictly T-linear resistivity that extends over a decade in temperature T. In addition to revealing the phenomenon of nematic quantum criticality, the observation of T-linear resistivity at a nematic critical point also raises the question of whether strong nematic fluctuations play a part in the transport properties of other ‘strange metals’, in which T-linear resistivity is observed over an extended regime in their respective phase diagrams. The pattern of electrical resistivity in an unconventional superconductor at high magnetic fields and low temperatures across the nematic quantum critical point reveals two classic signatures of quantum criticality.

In underdoped cuprates, an incommensurate charge density wave (CDW) order is known to coexist with superconductivity. A dip in T_{c} at the hole doping level where the CDW is strongest (n_{p}≃0.12) suggests that CDW order may suppress superconductivity. We investigate the interplay of charge order with superconductivity in underdoped YBa_{2}Cu_{3}O_{7-δ} by measuring the temperature dependence of the Hall coefficient R_{H}(T) at high magnetic field and at high hydrostatic pressure. We find that, although pressure increases T_{c} by up to 10 K at 2.6 GPa, it has very little effect on R_{H}(T). This suggests that pressure, at these levels, only weakly affects the CDW and that the increase in T_{c} with pressure cannot be attributed to a suppression of the CDW. We argue, therefore, that the dip in T_{c} at n_{p}≃0.12 at ambient pressure is probably not caused by the CDW formation.

In underdoped cuprates, an incommensurate charge density wave (CDW) order is known to coexist with superconductivity. A dip in T_{c} at the hole doping level where the CDW is strongest (n_{p}≃0.12) suggests that CDW order may suppress superconductivity. We investigate the interplay of charge order with superconductivity in underdoped YBa_{2}Cu_{3}O_{7-δ} by measuring the temperature dependence of the Hall coefficient R_{H}(T) at high magnetic field and at high hydrostatic pressure. We find that, although pressure increases T_{c} by up to 10 K at 2.6 GPa, it has very little effect on R_{H}(T). This suggests that pressure, at these levels, only weakly affects the CDW and that the increase in T_{c} with pressure cannot be attributed to a suppression of the CDW. We argue, therefore, that the dip in T_{c} at n_{p}≃0.12 at ambient pressure is probably not caused by the CDW formation.