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1. Bound→free and bound→bound multichannel emission spectra from selectively excited Rydberg states in the ZnAr and CdAr van der Waals complexes

Author

J. Dudek, J.P. Zobel, Jarosław Koperski, Andrzej Kędziorski, T. Urbańczyk, K. Puczka, and M. Krośnicki

Subjects
010405 organic chemistry, Chemistry, Organic Chemistry, Van der Waals molecule, 010402 general chemistry, 01 natural sciences, Diatomic molecule, 0104 chemical sciences, Analytical Chemistry, Inorganic Chemistry, symbols.namesake, Dipole, Physics - Chemical Physics, Excited state, Physics::Atomic and Molecular Clusters, Rydberg formula, symbols, Physics::Atomic Physics, Emission spectrum, van der Waals force, Atomic physics, Electronic energy, Spectroscopy
Abstract

Multichannel dispersed emission spectra originated upon a selective excitation of Rydberg electronic energy states in the ZnAr and CdAr van der Waals (vdW) complexes are simulated and analysed as a proof-of-concept of the future experimental approach. Simulations of the emission spectra are based on ab-initio calculated interatomic potentials and transition dipole moments (TDMs), that for ZnAr were newly calculated. Experimental set-up that is under construction along with the experimental procedure are discussed.

Published
2020

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