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We report here the results of a measurement of the scattered versus unscattered neutron fluence on polyethylene determined via neutron activation of multiple natural indium foils from a deuterium-deuterium (D-D) neutron generator. The neutrons were produced by the High Flux Neutron Generator (HFNG) at the University of California, Berkeley, a specially designed source to maximize neutron flux on a sample while minimizing the total neutron yield. During the experiment, approximately 108 n/s were produced with the energies at the indium foils ranging from 2.2 to 2.8MeV. Both the angle-integrated and the partial angle differential results are consistent with the predictions of the Monte Carlo N-Particle Transport (MCNP) code, using ENDF/B-VII.1. This supports shielding calculations in the fast energy region with high-density polyethylene.

The $\ensuremath{\beta}$ decay of $^{125m,125}\mathrm{Ag}$ into levels in $^{125}\mathrm{Cd}$ was investigated at the Holifield Radioactive Ion Beam Facility (HRIBF). Uranium-238 targets were bombarded with 50-MeV protons with an intensity of $15\phantom{\rule{4pt}{0ex}}\ensuremath{\mu}$A, and the induced fission products were mass separated and deposited on a moving tape in the center of the VANDLE array consisting of $\ensuremath{\gamma}$ detectors and plastic scintillators. A partial decay scheme has been assigned for both $\ensuremath{\beta}$ decay of the (9/${2}^{+}$) ground state of $^{125}\mathrm{Ag}$ and its low-lying (1/${2}^{\ensuremath{-}}$) isomer, with the energy of the low-lying (11/${2}^{\ensuremath{-}}$) isomeric state in $^{125}\mathrm{Cd}$ assigned as 188.5 keV. In addition, $\ensuremath{\beta}$-delayed neutron emission probabilities were also determined to be 1.2(2)% for the (9/${2}^{+}$) $^{125}\mathrm{Ag}$ ground state and 4.6(10)% for the (1/${2}^{\ensuremath{-}}$) isomer, which are substantially lower than the previously reported value.

Excited states in ${}^{73,75}\mathrm{Ni}$ were investigated through the $\ensuremath{\beta}$ decay of ${}^{73,75}\mathrm{Co}$ in an experiment performed at the National Superconducting Cyclotron Laboratory (NSCL) at Michigan State University (MSU). The experimental results extended the level scheme of $^{73}\mathrm{Ni}$ to 3.2-MeV excitation energy and provided the experimental information on excited states in $^{75}\mathrm{Ni}$. The $\ensuremath{\beta}$-delayed neutron branching ratio for $^{73}\mathrm{Co}$ was obtained. The experimental results are discussed in comparison with shell-model calculations.

Background: Neutron-rich nuclei in the mass region around A=160 have been and will continue to be of interest for the study of nuclear structure because of the rapid onset of deformation between 88 and 90 neutrons. The observation of detailed changes in nuclear structures within this mass region has provided and will continue to provide insight into the nuclear force. Purpose: Investigations of γ rays emitted following Eu163 β-decay to Gd163 have been performed for evaluation of the nuclear structure of Gd163. Method: Data were collected at the LeRIBSS station of the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory with an array of four Clover HPGe detectors for γ-rays and two plastic scintillators for β detection. The γ rays were identified as belonging to Gd163 via mass selection and γ-γ-β, x-ray-γ, or γ-γ coincidences. Results: In total 107 new γ-ray transitions were observed in Gd163 from 53 newly identified levels. Conclusions: The structure of Gd163 has been identified for the first time. This structure has been evaluated in comparison to projected shell model, and potential energy surface calculations with good agreement.

Radioactive ^{129}Sb, which can be treated as a proton plus semimagic ^{128}Sn core within the particle-core coupling scheme, was studied by Coulomb excitation. Reduced electric quadrupole transition probabilities, B(E2), for the 2^{+}⊗πg_{7/2} multiplet members and candidate πd_{5/2} state were measured. The results indicate that the total electric quadrupole strength of ^{129}Sb is a factor of 1.39(11) larger than the ^{128}Sn core, which is in stark contrast to the expectations of the empirically successful particle-core coupling scheme. Shell-model calculations performed with two different sets of nucleon-nucleon interactions suggest that this enhanced collectivity is due to constructive quadrupole coherence in the wave functions stemming from the proton-neutron residual interactions, where adding one nucleon to a core near a double-shell closure can have a pronounced effect. The enhanced electric quadrupole strength is an early signal of the emerging nuclear collectivity that becomes dominant away from the shell closure.

A number of accelerator-based isotope production facilities utilize 100- to 200-MeV proton beams due to the high production rates enabled by high-intensity beam capabilities and the greater diversity of isotope production brought on by the long range of high-energy protons. However, nuclear reaction modeling at these energies can be challenging because of the interplay between different reaction modes and a lack of existing guiding cross section data. A Tri-lab collaboration has been formed among the Lawrence Berkeley, Los Alamos, and Brookhaven National Laboratories to address these complexities by characterizing charged-particle nuclear reactions relevant to the production of established and novel radioisotopes. In the inaugural collaboration experiments, stacked-targets of niobium foils were irradiated at the Brookhaven Linac Isotope Producer (E$_p$=200 MeV) and the Los Alamos Isotope Production Facility (E$_p$=100 MeV) to measure $^{93}$Nb(p,x) cross sections between 50 and 200 MeV. The measured cross-section results were compared with literature data as well as the default calculations of the nuclear model codes TALYS, CoH, EMPIRE, and ALICE. We developed a standardized procedure that determines the reaction model parameters that best reproduce the most prominent reaction channels in a physically justifiable manner. The primary focus of the procedure was to determine the best parametrization for the pre-equilibrium two-component exciton model. This modeling study revealed a trend toward a relative decrease for internal transition rates at intermediate proton energies (E$_p$=20-60 MeV) in the current exciton model as compared to the default values. The results of this work are instrumental for the planning, execution, and analysis essential to isotope production., Comment: 37 pages, 62 figures. Revised version, published in Physical Review C

Author(s): Batchelder, JC; Chong, SA; Morrell, J; Unzueta, MA; Adams, P; Bauer, JD; Bailey, T; Becker, TA; Bernstein, LA; Fratoni, M; Hurst, AM; James, J; Lewis, AM; Matthews, EF; Negus, M; Rutte, D; Song, K; Van Bibber, K; Wallace, M; Waltz, CS | Abstract: The Cl35(n,p) and Cl35(n,α) cross sections at incident neutron energies between 2.42 and 2.74 MeV were measured using the Berkeley High Flux Neutron Generator. The cross sections for Cl35(n,p) were more than a factor of 3 to 5 less than all of the values in the neutron absorption data libraries, while the Cl35(n,α) cross sections are in reasonable agreement with the data libraries. The measured energy-differential cross section is consistent with a single resonance with a width of 293(46) keV. This result suggests that, despite the high incident neutron energy, any attempt to model (n,x) cross sections in the vicinity of the N=Z=20 shell gap requires a resolved resonance approach rather than a Hauser-Feshbach approach.

A stacked-target of natural lanthanum foils (99.9119% $^{139}$La) was irradiated using a 60 MeV proton beam at the LBNL 88-Inch Cyclotron. $^{139}$La(p,x) cross sections are reported between 35-60 MeV for nine radionuclides. The primary motivation for this measurement was the need to quantify the production of $^{134}$Ce. As a positron-emitting analogue of the promising medical radionuclide $^{225}$Ac, $^{134}$Ce is desirable for in vivo applications of bio-distribution assays for this emerging radio-pharmaceutical. The results of this measurement were compared to the nuclear model codes TALYS, EMPIRE and ALICE (using default parameters), which showed significant deviation from the measured values.

Use of deuteron-deuteron fusion neutrons may substantially improve applicability and accuracy of the 40Ar/39Ar technique., We designed and tested a compact deuteron-deuteron fusion neutron generator for application to 40Ar/39Ar geochronology. The nearly monoenergetic neutrons produced for sample irradiation are anticipated to provide several advantages compared with conventional fission spectrum neutrons: Reduction of collateral nuclear reactions increases age accuracy and precision. Irradiation parameters within the neutron generator are more controllable compared with fission reactors. Confidence in the prediction of recoil energies is improved, and their likely reduction potentially broadens applicability of the dating method to fine-grained materials without vacuum encapsulation. Resolution of variation in the 39K(n,p)39Ar neutron capture cross section at 1.3 to 3.2 MeV and discovery of a strong resonance at ~2.4 MeV illuminate future pathways to improve the technique for 40Ar/39Ar dating.

Beta + -delayed proton (or α ) emission is a typical decay mode of very neutron-deficient nuclei. Valuable information for the ground state in the precursor, such as half-life, spin, and parity, can be obtained by studying the β + -p decay properties. The high efficiency and unique experimental signature for detecting protons allow one to study states in the β + -decay daughter that are not accessible through other means. By measuring the properties of protons emitted to a known state in the daughter, information on the structure of the proton-unbound state can be obtained. The known nuclei that exhibit this decay mode are evaluated to give the recommended values for the nuclear properties of these nuclei. This includes branching ratios, and half-lives. In addition for those nuclei with known resolved proton transitions, proton energies, intensities, and the energies of the proton-emitting states are compiled. A list of experimental references for each β + -p precursor is also given. All papers published prior to June 2019 have been considered in adopting the properties given in this work.

© 2018 American Physical Society. An experiment was performed at Lawrence Berkeley National Laboratory's 88-in. Cyclotron to determine the mass number of a superheavy element. The measurement resulted in the observation of two α-decay chains, produced via the Am243(Ca48,xn)291-xMc reaction, that were separated by mass-to-charge ratio (A/q) and identified by the combined BGS+FIONA apparatus. One event occurred at A/q=284 and was assigned to Nh284 (Z=113), the α-decay daughter of Mc288 (Z=115), while the second occurred at A/q=288 and was assigned to Mc288. This experiment represents the first direct measurements of the mass numbers of superheavy elements, confirming previous (indirect) mass-number assignments.

Decay of $^{85}\mathrm{Ga}$ was studied by means of $\ensuremath{\beta}$-neutron-$\ensuremath{\gamma}$ spectroscopy. A pure beam of $^{85}\mathrm{Ga}$ was produced at the Holifield Radioactive Ion Beam Facility using a resonance ionization laser ion source and a high-resolution electromagnetic separator. The $\ensuremath{\beta}$-delayed neutron emission probability was measured for the first time, yielding 70(5)%. An upper limit of 0.1% for $\ensuremath{\beta}$-delayed two-neutron emission was also experimentally established for the first time. A detailed decay scheme including absolute $\ensuremath{\gamma}$-ray intensities was obtained. Results are compared with theoretical $\ensuremath{\beta}$-delayed emission models.

A next-generation, high-flux DD neutron generator has been designed, commissioned, and characterized, and is now operational in a new facility at the University of California Berkeley. The generator, originally designed for 40Ar/39Ar dating of geological materials, has since served numerous additional applications, including medical isotope production studies, with others planned for the near future. In this work, we present an overview of the High Flux Neutron Generator (HFNG) which includes a variety of simulations, analytical models, and experimental validation of results. Extensive analysis was performed in order to characterize the neutron yield, flux, and energy distribution at specific locations where samples may be loaded for irradiation. A notable design feature of the HFNG is the possibility for sample irradiation internal to the cathode, just 8 mm away from the neutron production site, thus maximizing the neutron flux (n/cm2/s). The generator's maximum neutron flux at this irradiation position is 2.58e7 n/cm2/s +/- 5% (approximately 3e8 n/s total yield) as measured via activation of small natural indium foils. However, future development is aimed at achieving an order of magnitude increase in flux. Additionally, the deuterium ion beam optics were optimized by simulations for various extraction configurations in order to achieve a uniform neutron flux distribution and an acceptable heat load. Finally, experiments were performed in order to benchmark the modeling and characterization of the HFNG., Comment: 31 pages, 20 figures

Efficient ion sources are needed for detecting ultratrace U and Th impurities in a copper matrix by mass spectrometry techniques such as accelerator mass spectrometry (AMS). Two positive ion sources, a hot-cavity surface ionization source and a resonant ionization laser ion source, are evaluated in terms of ionization efficiencies for generating ion beams of U and Th. The performances of the ion sources are characterized using uranyl nitrate and thorium nitrate sample materials with sample sizes between 20 and 40 μg of U or Th. For the surface ion source, the dominant ion beams observed are UO + or ThO + and ionization efficiencies of 2–4% have been obtained with W and Re cavities. With the laser ion source, three-step resonant photoionization of U atoms has been studied and only atomic U ions are observed. An ionization efficiency of about 9% has been demonstrated. The performances of both ion sources are expected to be further improved.

International audience; A multi-step Coulomb excitation measurement with the GRETINA and CHICO2 detector arrays was carried out with a 430-MeV beam of the neutron-rich $^{110}$Ru (t$_{1/2}$= 12 s) isotope produced at the CARIBU facility. This represents the first successful measurement following the post-acceleration of an unstable isotope of a refractory element. The reduced transition probabilities obtained for levels near the ground state provide strong evidence for a triaxial shape; a conclusion confirmed by comparisons with the results of beyond-mean-field and triaxial rotor model calculations.

Cross sections for the $^{47}$Ti(n,p)$^{47}$Sc and $^{64}$Zn(n,p)$^{64}$Cu reactions have been measured for quasi-monoenergetic DD neutrons produced by the UC Berkeley High Flux Neutron Generator (HFNG). The HFNG is a compact neutron generator designed as a "flux-trap" that maximizes the probability that a neutron will interact with a sample loaded into a specific, central location. The study was motivated by interest in the production of $^{47}$Sc and $^{64}$Cu as emerging medical isotopes. The cross sections were measured in ratio to the $^{113}$In(n,n')$^{113m}$In and $^{115}$In(n,n')$^{115m}$In inelastic scattering reactions on co-irradiated indium samples. Post-irradiation counting using an HPGe and LEPS detectors allowed for cross section determination to within 5% uncertainty. The $^{64}$Zn(n,p)$^{64}$Cu cross section for 2.76$^{+0.01}_{-0.02}$ MeV neutrons is reported as 49.3 $\pm$ 2.6 mb (relative to $^{113}$In) or 46.4 $\pm$ 1.7 mb (relative to $^{115}$In), and the $^{47}$Ti(n,p)$^{47}$Sc cross section is reported as 26.26 $\pm$ 0.82 mb. The measured cross sections are found to be in good agreement with existing measured values but with lower uncertainty (< 5%), and also in agreement with theoretical values. This work highlights the utility of compact, flux-trap DD-based neutron sources for nuclear data measurements and potentially the production of radionuclides for medical applications., 12 pages, submitted to NIM-B

We report total absorption spectroscopy measurements of $^{92}\mathrm{Rb}$, $^{96\mathrm{gs}}\mathrm{Y}$, and $^{142}\mathrm{Cs}$ $\ensuremath{\beta}$ decays, which are the most important contributors to the high energy ${\overline{\ensuremath{\nu}}}_{e}$ spectral shape in nuclear reactors. These three $\ensuremath{\beta}$ decays contribute 43% of the ${\overline{\ensuremath{\nu}}}_{e}$ flux near 5.5 MeV emitted by nuclear reactors. This ${\overline{\ensuremath{\nu}}}_{e}$ energy is particularly interesting due to spectral features recently observed in several experiments including the Daya Bay, Double Chooz, and RENO Collaborations. Measurements were conducted at Oak Ridge National Laboratory by means of proton-induced fission of $^{238}\mathrm{U}$ with on-line mass separation of fission fragments and the Modular Total Absorption Spectrometer. We observe a $\ensuremath{\beta}$-decay pattern that is similar to recent measurements of $^{92}\mathrm{Rb}$, with a ground-state to ground-state $\ensuremath{\beta}$ feeding of 91(3)%. We verify the $^{96\mathrm{gs}}\mathrm{Y}$ ground-state to ground-state $\ensuremath{\beta}$ feeding of 95.5(20)%. Our measurements substantially modify the $\ensuremath{\beta}$-decay feedings of $^{142}\mathrm{Cs}$, reducing the $\ensuremath{\beta}$ feeding to $^{142}\mathrm{Ba}$ states below 2 MeV by 32% when compared with the latest evaluations. Our results increase the discrepancy between the observed and the expected reactor ${\overline{\ensuremath{\nu}}}_{e}$ flux between 5 and 7 MeV, the maximum excess increases from $\ensuremath{\sim}10%$ to $\ensuremath{\sim}12%$.

$\ensuremath{\beta}$ decay of neutron-rich nuclide $^{94}\mathrm{Kr}$ was reinvestigated by means of a high resolution on-line mass separator and $\ensuremath{\beta}\ensuremath{-}\ensuremath{\gamma}$ spectroscopy. In total 22 $\ensuremath{\gamma}$-ray transitions were assigned to the decay of $^{94}\mathrm{Kr}$, and a new isomeric state was identified. The new information allows us to build detailed levels systematics in a chain of odd-odd rubidium isotopes and draw conclusions on nuclear structure for some of the observed states. The discussed level structure affects the evolution of $\ensuremath{\beta}$-decay half-lives for neutron-rich selenium, krypton, and strontium isotopes.

We report total absorption spectroscopy measurements of ^{92}Rb, ^{96gs}Y, and ^{142}Cs β decays, which are the most important contributors to the high energy ν[over ¯]_{e} spectral shape in nuclear reactors. These three β decays contribute 43% of the ν[over ¯]_{e} flux near 5.5 MeV emitted by nuclear reactors. This ν[over ¯]_{e} energy is particularly interesting due to spectral features recently observed in several experiments including the Daya Bay, Double Chooz, and RENO Collaborations. Measurements were conducted at Oak Ridge National Laboratory by means of proton-induced fission of ^{238}U with on-line mass separation of fission fragments and the Modular Total Absorption Spectrometer. We observe a β-decay pattern that is similar to recent measurements of ^{92}Rb, with a ground-state to ground-state β feeding of 91(3)%. We verify the ^{96gs}Y ground-state to ground-state β feeding of 95.5(20)%. Our measurements substantially modify the β-decay feedings of ^{142}Cs, reducing the β feeding to ^{142}Ba states below 2 MeV by 32% when compared with the latest evaluations. Our results increase the discrepancy between the observed and the expected reactor ν[over ¯]_{e} flux between 5 and 7 MeV, the maximum excess increases from ∼10% to ∼12%.

Decays of neutron-rich nuclei $^{82,83}\mathrm{Zn}$ and $^{82,83}\mathrm{Ga}$ produced in proton-induced fission of $^{238}\mathrm{U}$ were studied at the Holifield Radioactive Ion Beam Facility using on-line mass separation and $\ensuremath{\beta}\text{\ensuremath{-}}\ensuremath{\gamma}$ spectroscopy techniques. New $\ensuremath{\gamma}$-ray transitions were identified and level schemes, which include states at high excitation energies in the range between 3--7 MeV were constructed. These high-energy levels were identified to be populated through allowed Gamow-Teller $\ensuremath{\beta}$ transitions, and their structure was interpreted with new shell-model calculations. A $\ensuremath{\beta}$-delayed neutron branching ratio of $69\ifmmode\pm\else\textpm\fi{}7%$ was deduced for $^{82}\mathrm{Zn}$ and revised $\ensuremath{\beta}$-decay half-life values of $^{82}\mathrm{Zn}$ [155(17)(20) ms] and $^{83}\mathrm{Zn}$ [122(28) ms] were determined.

The β-delayed neutron emission of ^{83,84}Ga isotopes was studied using the neutron time-of-flight technique. The measured neutron energy spectra showed emission from states at excitation energies high above the neutron separation energy and previously not observed in the β decay of midmass nuclei. The large decay strength deduced from the observed intense neutron emission is a signature of Gamow-Teller transformation. This observation was interpreted as evidence for allowed β decay to ^{78}Ni core-excited states in ^{83,84}Ge favored by shell effects. We developed shell model calculations in the proton fpg_{9/2} and neutron extended fpg_{9/2}+d_{5/2} valence space using realistic interactions that were used to understand measured β-decay lifetimes. We conclude that enhanced, concentrated β-decay strength for neutron-unbound states may be common for very neutron-rich nuclei. This leads to intense β-delayed high-energy neutron and strong multineutron emission probabilities that in turn affect astrophysical nucleosynthesis models.

A compact isobar spectrometer and separator, based on the multi-pass-time-of-flight (MTOF) principle, is being developed by the University radioactive ion beam (UNIRIB) Consortium. It consists of two coaxial, grid-free electrostatic mirrors with auxiliary injection, focusing and extraction elements. Ions of different mass are reflected multiple times between the mirrors and separated longitudinally. Using an electron beam impact ion source and N2 as a sample gas, a mass resolving power of 110,000 (FWHM) has been achieved. In the near future, MTOF will be coupled to the on-line isotope separator UNISOR (University Isotope Separator – Oak Ridge) at Holifield radioactive ion beam facility using electrostatic beam deceleration, a radiofrequency beam cooler and a fast buncher. It will serve as a high resolution mass separator with a Bradbury–Nielsen gate, providing isotopically pure samples of exotic species in the 100Sn region and later, of neutron rich nuclei, for use in decay studies.

The α-decay chain 109Xe → 105Te → 101Sn was identified at the Holifield Radioactive Ion Beam Facility. Advances in digital electronics have made possible the identification of both alpha emitters in the same experiment despite the disparate half-lives of 13 ±2 ms and 620 ±70 ns for 109Xe and 105Te, respectively. Two α-decay transitions were observed from 109Xe with Qα values of 4067 ±10 and 4217 ±8 keV. One transition between the ground states of 105Te and 101Sn was observed with a Qα value of 4889 ±6 keV. Using the measured half-lives, branching ratios, and Qα values the reduced α-decay widths, δ2, were determined. Comparison of the δ2 value for 105Te with 213Po indicates a “superallowed" character in the α emission of 105Te.

A complete set of electromagnetic moments, B(E2;0+1 2+1), Q(2+1), and g(2+1), have been measured from Coulomb excitation of semi-magic 112,114,116,118,120,122,124Sn (Z = 50) on natural carbon and titanium targets. The magnitude of the B(E2) values, measured to a precision of ~4%, disagree with a recent lifetime study [Phys. Lett. B 695, 110 (2011)] that employed the Doppler- shift attenuation method. The B(E2) values show an overall enhancement compared with recent theoretical calculations and a clear asymmetry about midshell, contrary to naive expectations. A new static electric quadrupole moment, Q(2+1), has been measured for 114Sn. The static quadrupole moments are generally consistent with zero but reveal an enhancement near midshell; this had not been previously observed. The magnetic dipole moments are consistent with previous measurements and show a near monotonic decrease in value with neutron number. The current theory calculations fail to reproduce the electromagnetic moments of the tin isotopes. The role of 2p-2h and 4p-4h intruders, which are lowest in energy at mid shell and outside of current model spaces, needs to be investigated in the future.

A new experiment devoted to the fission of 252Cf is described. It continued a series of our experiments based on correlation measurements of γ rays emitted by fission fragment pairs. The measurements of γ-γ and γ-γ-γ coincidences were done at Gammasphere with closed 252Cf sources. The open source was used for the first time in the last experiment. Fission fragment detectors were arranged in the center hole of Gammasphere. Correlations between fission fragment masses, total kinetic energy, and γ rays were observed. The first, preliminary results of data analysis are discussed.

Properties of nuclei beyond the proton drip line are studied via measurement of the spontaneous emission of protons from these exotic nuclei. Different components of the wave function of the proton emitter can be accessed by observation of fine structure in the proton spectrum. Fine structure has been observed in the proton radioactivity of 145Tm, 146Tm and 141Ho in measurements at the Holifield Radioactive Ion Beam Facility. These nuclei range over an interesting transition region going from nearly spherical to rather deformed. Detailed analysis of the rich fine structure spectrum of 146Tm is presented in terms of the particle-core vibration coupling model. Other models are discussed briefly.

Neutron-rich radioactive ion beams available from the HRIBF allow a variety of measurements around the 132Sn region, including Coulomb excitation and single-nucleon transfer. The B(E2;0+ → 2+) values for first 2+ excited states of even-even neutron-rich 132-136Te and 126-130Sn have been measured by Coulomb excitation in inverse kinematics. Neutron transfer onto a 134Te beam from 9Be and 13C targets, to populate single-particle states in 135Te, has also been studied. Gamma rays from the 13C(134Te, 12C) reaction were used to identify the νi13/2 state in 135Te, at an energy of 2109 keV. These and other results, and plans for future experiments with these neutron-rich beams, are presented.

The structure of magic neutron-rich nickel isotopes produced in the fragmentation of a 140 A MeV 86 Kr beam was investigated. For the first time four gamma transitions were assigned to the decay of the I π = 8 + , T 1 / 2 = 590 −110 +180 ns isomer, thus establishing the 0 + – 2 + – 4 + – 6 + – 8 + ground-state band in 76 Ni. The previously unknown 2 + and 4 + levels belonging to the ground-state band in 74 Ni were identified in the β decay of 74 Co ( T 1 / 2 = 30 ( 3 ) ms ) . The decay properties of 72 Co → 72 Ni were verified and confirmed on the basis of γ – γ coincidence data. The relevance of the measured level properties for the magicity of 78 Ni is analyzed with the help of advanced shell-model predictions.

The degree to which the (p, γ) and (p,α) reactions destroy 18F at temperatures ∼ 1 − 4 × 10 8 K is important for understanding the synthesis of nuclei in nova explosions and for using the long-lived radionuclide 18F, a target of gamma ray astronomy, as a diagnostic of nova mechanisms. The reactions are dominated by low-lying proton resonances near the 18F+p threshold ( E x = 6.411 MeV in 19Ne). To gain further information about these resonances, we have used the d(18F,p)19F neutron transfer reaction to selectively populate corresponding mirror states in 19F. The results would suggest 18F(p,γ)19Ne and 18F(p,α)15O reaction rates that are 2-3 times lower than reported previously.

Neutron-rich radioactive ion beams available from the HRIBF allow a variety of measurements around the 132Sn region, including Coulomb excitation, fusion-evaporation, and neutron transfer. The B ( E 2 ; 0 + → 2 + ) value for first 2+ excited states of even-even neutron-rich 132–136Te and 126–134Sn have been measured by Coulomb excitation in inverse kinematics. The results are discussed in terms of the shell model and the quasiparticle random phase approximation. Neutron transfer onto a 134Te beam, from 9Be and 13C targets to populate single-particle states in 135Te, has also been studied. Gamma rays from the 13C(134Te, 12C) reaction were used to identify the ν i 13 / 2 state in 135Te, at an energy of 2109 keV. These and other results, and plans for future experiments with these neutron-rich beams, are presented.

An array for decay studies of neutron-rich nuclei has been commissioned for use at the UNISOR separator at Holifield Radioactive Ion Beam Facility. This array consists of three segmented clover Ge detectors, plastic scintillators, and a high-resolution (∼1 keV) Si conversion electron spectrometer. These detectors are mounted on a support that surrounds a moving tape collector. This system has been named clover array for radioactive decay studies. The detectors have been outfitted with digital flash ADCs (XIA DGFs) that fit the preamp signals, with built-in pileup rejection.

Particle radioactivity studies using the XIA DGF-4C digital signal processing units at the Recoil Mass Separator of Oak Ridge National Laboratory are presented. Proton emission signals were observed starting from 500 ns after recoil implantation. An energy threshold below 100 keV for particle detection was achieved. For the 145 Tm and 146 Tm decay, evidence for the fine structure in proton emission was obtained. An experiment to search for a new proton emitter 149 Lu is described as an example where the combination of a 56 Ni radioactive beam and digital signal processing is a major advantage.

The level structures of \(^{108,110,112}\)Ru (\(Z=44\)) and \(^{112,114,115,116,117,118}\)Pd (\(Z=46\)) have been significantly expanded through studies of prompt \(\gamma \)-\(\gamma \)-\(\gamma \) and \(\gamma \)-\(\gamma \)-\(\gamma \)-\(\gamma \) coincidences observed with Gammasphere following the spontaneous fission of \(^{252}\)Cf. Chiral doublet bands were observed in \(^{110,112}\)Ru. Softness to triaxiality perturbs the bands of \(^{108}\)Ru and even-\(N\) Pd isotopes. In \(^{112}\)Ru, evidence for wobbling motion is found in the behavior of the \(\gamma \) vibrational band. Similar evidence for wobbling motion is found in \(^{114}\)Pd, the \(N = 68\) isotone of \(^{112}\)Ru. A transition from triaxial prolate to triaxial oblate was found in \(^{112-116}\)Pd with shape coexistent bands in \(^{115}\)Pd. New levels were observed in \(^{162,163}\)Gd.

The excited states of odd-odd $^{82}\mathrm{As}$ are studied in the $\ensuremath{\beta}$ decay of $^{82}\mathrm{Ge}$. An isotopically pure beam of $^{83}\mathrm{Ga}$ was produced at the Holifield Radioactive Ion Beam Facility using a resonance ionization laser ion source and high-resolution electromagnetic separation. The atoms of $^{82}\mathrm{Ge}$ are created after $\ensuremath{\beta}$-delayed neutron emission in the decay of $^{83}\mathrm{Ga}$. The number of $^{82}\mathrm{Ge}$ atoms is found by normalization to the 1348-keV $\ensuremath{\gamma}$ ray. Detailed analysis of the decay scheme is compared with shell-model calculations with several commonly used $fpg$ shell interactions.

High-precision reduced electric-quadrupole transition probabilities $B(E2;{0}_{1}^{+}\ensuremath{\rightarrow}{2}_{1}^{+})$ have been measured from single-step Coulomb excitation of semi-magic $^{58,60,62,64}\mathrm{Ni}$ ($Z=28$) beams at 1.8 MeV per nucleon on a natural carbon target. The energy loss of the nickel beams through the carbon target were directly measured with a zero-degree Bragg detector and the absolute $B(E2)$ values were normalized by Rutherford scattering. The $B(E2)$ values disagree with recent lifetime studies that employed the Doppler-shift attenuation method. The present high-precision $B(E2)$ values reveal an asymmetry about $^{62}\mathrm{Ni}$, midshell between $N=28$ and 40, with larger values towards $^{56}\mathrm{Ni}$ ($Z=N=28$). The experimental $B(E2)$ values are compared with shell-model calculations in the full $pf$ model space and the results indicate a soft $^{56}\mathrm{Ni}$ core.

$\ensuremath{\gamma}$-ray transitions in ${}^{134}\text{Te}$, ${}^{135}\text{Te}$, and ${}^{136}\text{Te}$ were measured from ${}^{9}\text{Be}$-induced reactions with a radioactive ${}^{132}\text{Sn}$ beam at a sub-Coulomb barrier energy of 3 MeV per nucleon using particle-$\ensuremath{\gamma}$ coincidence spectroscopy. The transitions were selected by gating on alpha-like particles in a CsI detector following a combination of $({}^{9}\text{Be},\ensuremath{\alpha}1n)$, $({}^{9}\text{Be},\ensuremath{\alpha}2n)$, and $({}^{9}\text{Be},\ensuremath{\alpha}3n)$ incomplete fusion-evaporation reactions. Distorted-wave Born approximation calculations suggest little to no contribution from the $({}^{9}\text{Be},{}^{7}\text{He})$, $({}^{9}\text{Be},{}^{6}\text{He})$, and $({}^{9}\text{Be},{}^{5}\text{He})$ direct reactions.$\ensuremath{\gamma}$-ray transitions from previously known ${2}^{+}\ensuremath{\bigotimes}\ensuremath{\nu}\phantom{\rule{0.16em}{0ex}}2{f}_{7/2}$ and ${4}^{+}\ensuremath{\bigotimes}\ensuremath{\nu}\phantom{\rule{0.16em}{0ex}}2{f}_{7/2}$ multiplet members in ${}^{135}\text{Te}$ are observed. A new $\ensuremath{\gamma}$ ray is observed, assigned to the third-excited state in ${}^{135}\text{Te}$, and new ${2}^{+}\ensuremath{\bigotimes}\ensuremath{\nu}\phantom{\rule{0.16em}{0ex}}2{f}_{7/2}$ multiplet members are suggested. In addition, spin assignments are made by using recent one-neutron transfer data. The updated experimental data for ${}^{135}\text{Te}$ are compared to shell-model calculations for a relatively complete set of states up to the yrast ${15/2}^{\ensuremath{-}},{4}^{+}\ensuremath{\bigotimes}\ensuremath{\nu}\phantom{\rule{0.16em}{0ex}}2{f}_{7/2}$ multiplet member at 1505 keV.

Single-neutron states in $^{133}\mathrm{Sn}$ and $^{209}\mathrm{Pb}$, which are analogous to single-electron states outside of closed atomic shells in alkali metals, were populated by the ($^{9}\mathrm{Be}$, $^{8}\mathrm{Be}$) one-neutron transfer reaction in inverse kinematics using particle-$\ensuremath{\gamma}$ coincidence spectroscopy. In addition, the ${s}_{1/2}$ single-neutron hole-state candidate in $^{131}\mathrm{Sn}$ was populated by ($^{9}\mathrm{Be}$, $^{10}\mathrm{Be}$). Doubly closed-shell $^{132}\mathrm{Sn}$ (radioactive) and $^{208}\mathrm{Pb}$ (stable) beams were used at sub-Coulomb barrier energies of 3 MeV per nucleon. Level energies, $\ensuremath{\gamma}$-ray transitions, absolute cross sections, spectroscopic factors, asymptotic normalization coefficients, and excited-state lifetimes are reported and compared with shell-model expectations. The results include a new transition and precise level energy for the $3{p}_{1/2}$ candidate in $^{133}\mathrm{Sn}$, new absolute cross sections for the $1{h}_{9/2}$ candidate in $^{133}\mathrm{Sn}$ and $3{s}_{1/2}$ candidate in $^{131}\mathrm{Sn}$, and new lifetimes for excited states in $^{133}\mathrm{Sn}$ and $^{209}\mathrm{Pb}$. This is the first report on excited-state lifetimes of $^{133}\mathrm{Sn}$, which allow for a unique test of the nuclear shell model and $^{132}\mathrm{Sn}$ double-shell closure.

Single-neutron states in (133)Sn and (209)Pb, which are analogous to single-electron states outside of closed atomic shells in alkali metals, were populated by the ((9)Be, (8)Be) one-neutron transfer reaction in inverse kinematics using particle-γ coincidence spectroscopy. In addition, the s(1/2) single-neutron hole-state candidate in (131)Sn was populated by ((9)Be, (10)Be). Doubly closed-shell (132)Sn (radioactive) and (208)Pb (stable) beams were used at sub-Coulomb barrier energies of 3 MeV per nucleon. Level energies, γ-ray transitions, absolute cross sections, spectroscopic factors, asymptotic normalization coefficients, and excited-state lifetimes are reported and compared with shell-model expectations. The results include a new transition and precise level energy for the 3p(1/2) candidate in (133)Sn, new absolute cross sections for the 1h(9/2) candidate in (133)Sn and 3s(1/2) candidate in (131)Sn, and new lifetimes for excited states in (133)Sn and (209)Pb. This is the first report on excited-state lifetimes of (133)Sn, which allow for a unique test of the nuclear shell model and (132)Sn double-shell closure.