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The present study examines indoor and outdoor environmental particulate matter and gaseous pollutants in order to evaluate the urban air quality, the sources and pathways of pollutants, and its impact on Chennai megacity, South India. A total number of 25 air conditioner filter particulate matter samples collected from residential buildings, schools, colleges, commercial shopping malls, and buildings near urban highways were studied for indoor air quality. Similarly, outdoor air quality assessments have been done in various parts of the Chennai metropolis, including the Manali-Industrial area, the Velachery-Residential site, and the Alandur Bus Depot, as well as collected air quality data sets from the Central Pollution Control Board at continuous ambient air quality monitoring stations. The suspended atmospheric particles where the highest concentration (47%) occurred were mostly located in the roadside environments followed by commercial areas (42%), which indicates the increase in air pollution in the roadside areas. Further, environmental magnetism and ecological risk indices were studied from the collected data set. The study predicts that the air pollutants were predominantly from anthropogenic sources, such as vehicle emissions, effluents from power plants, abrasion of tires, steelworks, burning of fossil fuels and construction materials, etc. As a result, the current study suggests 68% of indoor pollutants were from the anthropogenic input, 18% from the pedogenic origin, and 14% from high heavy metal pollution at the sampling sites. This indicates that raising the ventilation rate via mechanical components significantly enhances the indoor air quality. These findings might be valuable in improving urban air quality, reducing traffic-related pollutants, and improving environmental quality.