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Detecting nuclear spins using single Nitrogen-Vacancy (NV) centers is of particular importance in nano-scale science and engineering, but often suffers from the heating effect of microwave fields for spin manipulation, especially under high magnetic fields. Here, we realize an energy-efficient nano-scale nuclear-spin detection using a phase-modulation electron-nuclear double resonance scheme. The microwave field can be reduced to 1/250 of previous requirements and the corresponding power is over four orders lower. Meanwhile, the microwave-induced broadening to the line-width of the spectroscopy is significantly canceled and we achieve a nuclear-spin spectrum with a resolution down to 2.1 kHz under a magnetic field at 1840 Gs. The spectral resolution can be further improved by upgrading the experimental control precision. This scheme can also be used in sensing microwave fields and extended to a wide range of applications in the future.

Quantum state readout plays a pivotal role in quantum technologies, spanning applications in sensing, computation, and secure communication. In this work, we introduce a new approach for efficiently reading populations of hybrid-spin states in the nitrogen-vacancy center of diamond using a single laser pulse, which utilizes the excited state level anti-crossing mechanism at around 500 Gs. Reading spin state populations through this approach achieves the same outcome as traditional quantum state diagonal tomography but significantly reduces the experimental time by an order of magnitude while maintaining fidelity. Moreover, this approach may be extended to encompass full-state tomography, thereby obviating the requirement for a sequence of spin manipulations and mitigating errors induced by decoherence throughout the procedure.

Low-dimensional quantum materials that remain strongly ferromagnetic down to mono layer thickness are highly desired for spintronic applications. Although oxide materials are important candidates for next generation of spintronic, ferromagnetism decays severely when the thickness is scaled to the nano meter regime, leading to deterioration of device performance. Here we report a methodology for maintaining strong ferromagnetism in insulating LaCoO3 (LCO) layers down to the thickness of a single unit cell. We find that the magnetic and electronic states of LCO are linked intimately to the structural parameters of adjacent "breathing lattice" SrCuO2 (SCO). As the dimensionality of SCO is reduced, the lattice constant elongates over 10% along the growth direction, leading to a significant distortion of the CoO6 octahedra, and promoting a higher spin state and long-range spin ordering. For atomically thin LCO layers, we observe surprisingly large magnetic moment (0.5 uB/Co) and Curie temperature (75 K), values larger than previously reported for any mono layer oxide. Our results demonstrate a strategy for creating ultra thin ferromagnetic oxides by exploiting atomic hetero interface engineering,confinement-driven structural transformation, and spin-lattice entanglement in strongly correlated materials., Comment: 24 pages, 5 figures, 1 supporting information with 13 figures

The nitrogen-vacancy (N-V) center in diamond is a widely-used platform for quantum information processing and metrology. The electron-spin state of N-V center could be initialized and readout optically, and manipulated by resonate microwave fields. In this work, we analyze the dependence of electron-spin initialization on widths of laser pulses. We build a numerical model to simulate this process and verify the simulation results in experiment. Both simulations and experiments reveal a fact that shorter laser pulses are helpful to the electron-spin polarization. We therefore propose to use extremely-short laser pulses for electron-spin initialization. In this new scheme, the spin-state contrast could be improved about 10% in experiment by using laser pulses as short as 4 ns in width. Furthermore, we provide a mechanism to explain this effect which is due to the occupation time in the meta-stable spin-singlet states of N-V center. Our new scheme is applicable in a broad range of NV-based applications in the future., Comment: 7 pages, 4 figures