Search

The tunneling of interacting charges in nanostructures is a random and noisy process, which gives rise to a variety of intriguing physical phenomena, including Coulomb blockade, the Kondo effect, and Fermi-edge singularities. Such correlation effects are visible in low-frequency measurements of the electric current or the shot noise, however, they are also expected to leave clear fingerprints in the tunneling times of individual charges. Here, we experimentally demonstrate the real-time detection and control of correlated charge tunneling in a dynamically driven quantum dot. To this end, we measure the joint distribution of waiting times between tunneling charges, and we show that subsequent waiting times are strongly correlated due to the Coulomb interactions between the tunneling charges and the external periodic drive. Our measurements are in excellent agreement with a theoretical model that allows us to develop a detailed understanding of the correlated tunneling events. We also demonstrate that the degree of correlations can be controlled by the external drive. Our experiment paves the way for systematic real-time investigations of correlated electron transport in low-dimensional nanostructures with potential applications in metrology and sensing., Comment: 7 pages, 5 figures

Spin-flips are one of the limiting factors for spin-based information processing. We demonstrate a transport approach for determining the spin-flip rates of a self-assembled InAs double quantum dot occupied by a single electron. In such devices, different Land\'e factors lead to an inhomogeneous Zeeman splitting, so that the two spin channels can never be at resonance simultaneously, leading to a spin blockade at low temperatures. This blockade is analyzed in terms of spin flips for different temperatures and magnetic fields. Our results are in good agreement with a quantum master equation that combines the dot-lead couplings with ohmic dissipation stemming from spin-flip cotunneling., Comment: 9 pages, 8 figures

Large-scale quantum networks require the implementation of long-lived quantum memories as stationary nodes interacting with qubits of light. Epitaxially grown quantum dots hold great potential for the on-demand generation of single and entangled photons with high purity and indistinguishability. Coupling these emitters to memories with long coherence times enables the development of hybrid nanophotonic devices incorporating the advantages of both systems. Here we report the first GaAs/AlGaAs quantum dots grown by droplet etching and nanohole infilling method, emitting single photons with a narrow wavelength distribution (736.2 $\pm$ 1.7 nm) close to the zero-phonon line of Silicon-vacancy centers. Polarization entangled photons are generated via the biexciton-exciton cascade with a fidelity of (0.73 $\pm$ 0.09). High single photon purity is maintained from 4 K (g$^($$^2$$^)$(0) = 0.07 $\pm$ 0.02) up to 80 K (g$^($$^2$$^)$(0) = 0.11 $\pm$ 0.01), therefore making this hybrid system technologically attractive for real-world quantum photonic applications.

The surface of semiconductor nanostructures has a major impact on their electronic and optical properties. Disorder and defects in the surface layer typically cause degradation of charge carrier transport and radiative recombination dynamics. However, surface vicinity is inevitable for many scalable nano-optical applications. Epitaxially grown quantum dots are the best candidate for high-performance single photon emission and show great potential for quantum technologies. Yet, these emitters only reveal their excellent properties if they are deeply embedded in a semiconductor host. Until today, quantum dots close to surfaces yield weak, broad, and unstable emissions. Here, we show the complete restoration of optical properties from quantum dots grown directly on a semiconductor surface. The vanishing luminescence from the as-grown sample turns into bright, ultra-stable, coherent and blinking-free single photon emission after sulphur passivation. Under quasi-resonant excitation, single photons are generated with 98.8% purity, 77% indistinguishability, linewidths down to 4 $\mu$eV and 99.69% persistency across 11 orders of magnitude in time. The emission is stable even after two years and when being subjected to nanomanufacturing processes. Some long-standing stumbling blocks for surface-dominated quantum dots are thereby removed, unveiling new possibilities for hybrid nano-devices and applications in quantum communication or sensing., Comment: New experiments show that the results have to be re-interpreted, most likely leading to a new manuscript

Quantum systems as used for quantum computation or quantum sensing are nowadays often realized in solid state devices as e.g. complex Josephson circuits or coupled quantum-dot systems. Condensed matter as an environment influences heavily the quantum coherence of such systems. Here, we investigate electron transport through asymmetrically coupled InAs double quantum dots and observe an extremely strong temperature dependence of the coherent current peaks of single-electron tunneling. We analyze experimentally and theoretically the broadening of such coherent current peaks up to temperatures of 20 K and we are able to model it with quantum dissipation being due to two different bosonic baths. These bosonic baths mainly originate from substrate phonons. Application of a magnetic field helps us to identify the different quantum dot states through their temperature dependence., Comment: 10 pages, 6 figures

We investigate theoretically and experimentally stochastic resonance in a quantum dot coupled to electron source and drain via time-dependent tunnel barriers. A central finding is a transition visible in the current noise spectrum as a bifurcation of a dip originally at zero frequency. The transition occurs close to the stochastic resonance working point and relates to quantized pumping. For the evaluation of power spectra from measured waiting times, we generalize a result from renewal theory to the ac driven case. Moreover, we develop a master equation method to obtain phase-averaged current noise spectra for driven quantum transport., Comment: 10 pages, 6 figures

Quantum technologies involving qubit measurements based on electronic interferometers rely critically on accurate single-particle emission. However, achieving precisely timed operations requires exquisite control of the single-particle sources in the time domain. Here, we demonstrate accurate control of the emission time statistics of a dynamic single-electron transistor by measuring the waiting times between emitted electrons. By ramping up the modulation frequency, we controllably drive the system through a crossover from adiabatic to nonadiabatic dynamics, which we visualize by measuring the temporal fluctuations at the single-electron level and explain using detailed theory. Our work paves the way for future technologies based on the ability to control, transmit, and detect single quanta of charge or heat in the form of electrons, photons, or phonons., Comment: 5+2 pages, 3 figures, published in Science Advances

The complex nature of filling factor $\nu$=0 of monolayer graphene is studied in magnetotransport experiments. As function of perpendicular magnetic field a metal-insulator transition is observed, which is attributed to disorder-induced Landau level broadening in the canted antiferromagnetic phase. In the metallic regime a separation of the zeroth Landau level appears and signs of the quantum spin Hall effect are seen near $\nu$=0. In addition to local transport, nonlocal transport experiments show results being consistent with helical edge transport., Comment: 5 pages, 4 figures

Thin adhesive films can be removed from substrates, torn, and folded in distinct geometries under external driving forces. In two-dimensional materials, however, these processes can be self-driven as shown in previous studies on folded twisted bilayer graphene nanoribbons produced by spontaneous tearing and peeling from a substrate. Here, we use atomic force microscopy techniques to generate and characterize the geometrical structure of naturally self-grown folded nanoribbon structures. Measurements of nanoribbon width and interlayer separation reveal similar twist-angle dependences possibly caused by the anisotropy in the bilayer potential. In addition, analysis of the data shows an unexpected correlation between the height of the folded arc edge -parameterized by a radius R-, and the ribbon width, suggestive of a self-growth process driven by a variable cross-sectional shape. These observations are well described by an energy minimization model that includes the bilayer adhesion energy density as represented by a distance dependent Morse potential. We obtain an analytical expression for the radius R versus the ribbon width that predicts a renormalized bending rigidity and stands in good agreement with experimental observations. The newly found relation between these geometrical parameters suggests a mechanism for tailored growth of folded twisted bilayer graphene -- a platform for many intriguing physics phenomena.

We investigate the 1/f noise properties of epitaxial graphene devices at low temperatures as a function of temperature, current and magnetic flux density. At low currents, an exponential decay of the 1/f noise power spectral density with increasing temperature is observed that indicates mesoscopic conductance fluctuations as the origin of 1/f noise at temperatures below 50 K. At higher currents, deviations from the typical quadratic current dependence and the exponential temperature dependence occur as a result of nonequilibrium conditions due to current heating. By applying the theory of Kubakaddi [S. S. Kubakaddi, Phys. Rev. B 79, 075417 (2009)], a model describing the 1/f noise power spectral density of nonequilibrium mesoscopic conductance fluctuations in epitaxial graphene is developed and used to determine the energy loss rate per carrier. In the regime of Shubnikov-de Haas oscillations a strong increase of 1/f noise is observed, which we attribute to an additional conductance fluctuation mechanism due to localized states in quantizing magnetic fields. When the device enters the regime of quantized Hall resistance, the 1/f noise vanishes. It reappears if the current is increased and the quantum Hall breakdown sets in.

The folding of monolayer graphene leads to new layered systems, termed twisted bilayer graphene (TBG), generally displaying a certain interlayer rotation away from crystallographic alignment. We here present an atomic force microscopy study on folded graphene, revealing unexpectedly large twist angle dependent modulations of ~3 angstrom in interlayer distance. At the TBG surface, we find enhanced friction attributable to superlubricity in between incommensurate layers. At the bended edge, the radius of curvature scales with the folded length, congruent to earlier studies on carbon nanotubes., Comment: 5 pages, 4 figures

The electronic dispersion of a graphene bilayer is highly dependent on rotational mismatch between layers and can be further manipulated by electrical gating. This allows for an unprecedented control over electronic properties and opens up the possibility of flexible band structure engineering. Here we present novel magnetotransport data in a twisted bilayer, crossing the energetic border between decoupled monolayers and coupled bilayer. In addition a transition in Berry phase between pi and 2pi is observed at intermediate magnetic fields. Analysis of Fermi velocities and gate induced charge carrier densities suggests an important role of strong layer asymmetry for the observed phenomena., Comment: 20 pages main paper + 10 pages supporting information

The electronic properties of bilayer graphene strongly depend on relative orientation of the two atomic lattices. Whereas Bernal-stacked graphene is most commonly studied, a rotational mismatch between layers opens up a whole new field of rich physics, especially at small interlayer twist. Here we report on magnetotransport measurements on twisted graphene bilayers, prepared by folding of single layers. These reveal a strong dependence on the twist angle, which can be estimated by means of sample geometry. At small rotation, superlattices with a wavelength in the order of 10 nm arise and are observed by friction atomic force microscopy. Magnetotransport measurements in this small-angle regime show the formation of satellite Landau fans. These are attributed to additional Dirac singularities in the band structure and discussed with respect to the wide range of interlayer coupling models.

The influence of high magnetic fields on coherent transport is investigated. A monolayer graphene quantum ring is fabricated and the Aharonov-Bohm effect is observed. For increased magnitude of the magnetic field higher harmonics appear. This phenomenon is attributed to an increase of the phase coherence length due to reduction of spin flip scattering.

We demonstrate the high fidelity splitting of electron pairs emitted on demand from a dynamic quantum dot by an electronic beam splitter. The fidelity of pair splitting is inferred from the coincidence of arrival in two detector paths probed by a measurement of the partitioning noise. The emission characteristic of the on-demand electron source is tunable from electrons being partitioned equally and independently to electron pairs being split with a fidelity of 90%. For low beam splitter transmittance we further find evidence of pair bunching violating statistical expectations for independent fermions.

The spin-dependent dynamical blockade was investigated in a lateral quantum dot in a magnetic field. Spin-polarized edge channels in the two-dimensional leads and the spatial distribution of Landau orbitals in the dot modulate the tunnel coupling of the quantum dot level spectrum. In a measurement of the electron shot noise we observe a pattern of super-Poissonian noise which is correlated to the spin-dependent competition between different transport channels.

Electron transport in nano-scale structures is strongly influenced by the Coulomb interaction which gives rise to correlations in the stream of charges and leaves clear fingerprints in the fluctuations of the electrical current. A complete understanding of the underlying physical processes requires measurements of the electrical fluctuations on all time and frequency scales, but experiments have so far been restricted to fixed frequency ranges as broadband detection of current fluctuations is an inherently difficult experimental procedure. Here we demonstrate that the electrical fluctuations in a single electron transistor (SET) can be accurately measured on all relevant frequencies using a nearby quantum point contact for on-chip real-time detection of the current pulses in the SET. We have directly measured the frequency-dependent current statistics and hereby fully characterized the fundamental tunneling processes in the SET. Our experiment paves the way for future investigations of interaction and coherence induced correlation effects in quantum transport., Comment: 7 pages, 3 figures, published in Nature Communications (open access)

We study a mesoscopic circuit of two quantized current sources, realized by non-adiabatic single- electron pumps connected in series with a small micron-sized island in between. We find that quantum transport through the second pump can be locked onto the quantized current of the first one by a feedback due to charging of the mesoscopic island. This is confirmed by a measurement of the charge variation on the island using a nearby charge detector. Finally, the charge feedback signal clearly evidences loading into excited states of the dynamic quantum dot during single-electron pump operation.

We study the tuning mechanisms of the Ruderman-Kittel-Kasuya-Yosida (RKKY) exchange interaction between two lateral quantum dots in the Kondo regime. At zero magnetic field we observe the expected splitting of the Kondo resonance and measure the RKKY interaction strength J as a function of the asymmetry between the two Kondo temperatures. At finite magnetic fields a chiral coupling between the quantum dots is observed in the Kondo chessboard and we probe the presence of the exchange interaction by analyzing the Kondo temperature with magnetic field., Comment: 4 pages, 4 figures

Magnetotunneling spectroscopy was employed to probe the confinement in vertical Si/Ge double-barrier resonant tunneling diodes with regularly distributed Ge quantum dots. Their current-voltage characteristics reveal a step-like behavior in the vicinity of zero bias, indicating resonant tunneling of heavy-holes via three-dimensionally confined unoccupied hole states in Ge quantum dots. Assuming parabolic confinement we extract the strength of the confinement potential of quantum dots., Comment: 4 pages, 3 figures

Measurements of single electron tunneling through a quantum dot using a quantum point contact as charge detector have been performed for very long time traces with very large event counts. This large statistical basis is used for a detailed examination of the counting statistics for varying symmetry of the quantum dot system. From the measured statistics we extract high order cumulants describing the distribution. Oscillations of the high order cumulants are observed when varying the symmetry. We compare this behavior to the observed oscillation in time dependence and show that the variation of both system variables lead to the same kind of oscillating response., Comment: 3 pages

We report on measurements of single electron tunneling through a quantum dot using a quantum point contact as non-invasive charge detector with fast time response. We elaborate on the unambiguous identification of individual tunneling events and determine the distribution of transferred charges, the so-called full counting statistics. We discuss our data analysis, including the error estimates of the measurement, and show that the quality of our experimental results is sufficiently high to extract cumulants of the distribution up to the 20th order for short times., Comment: 4 pages, 3 figures, Contribution to EP2DS18-MSS14, Kobe, Japan, July 2009

Noise is a result of stochastic processes that originate from quantum or classical sources. Higher-order cumulants of the probability distribution underlying the stochastic events are believed to contain details that characterize the correlations within a given noise source and its interaction with the environment, but they are often difficult to measure. Here we report measurements of the transient cumulants <> of the number n of passed charges to very high orders (up to m=15) for electron transport through a quantum dot. For large m, the cumulants display striking oscillations as functions of measurement time with magnitudes that grow factorially with m. Using mathematical properties of high-order derivatives in the complex plane we show that the oscillations of the cumulants in fact constitute a universal phenomenon, appearing as functions of almost any parameter, including time in the transient regime. These ubiquitous oscillations and the factorial growth are system-independent and our theory provides a unified interpretation of previous theoretical studies of high-order cumulants as well as our new experimental data., Comment: 19 pages, 4 figures, final version as published in PNAS

We study the Fermi-edge singularity appearing in the current-voltage characteristics for resonant tunneling through a localized level at finite temperature. An explicit expression for the current at low temperature and near the threshold for the tunneling process is presented which allows to coalesce data taken at different temperatures to a single curve. Based on this scaling function for the current we analyze experimental data from a GaAs-AlAs-GaAs tunneling device with embedded InAs quantum dots obtained at low temperatures in high magnetic fields., Comment: 12 pages, 5 figures