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Maximal ground-state deformation should occur when both proton and neutron Fermi surfaces are located at midshell. However, subshell gaps that stabilize large deformation can exist at proton or neutron values other than midshell. One such gap may occur at Z=60 in the rare-earth region, as the energy of the first 2+ states in even-even nuclei are often lowest in an isotonic chain for neodymium (Z=60) rather than the midshell isotopes of dysprosium (Z=66). Further evidence of this deformed gap has now been observed by investigating the signature splitting systematics of the νi13/2 bands found in the odd-N, rare-earth nuclei. These were aided by the present observation of the νi13/2 band in Gd159 and the confirmation of the same structure in Sm155 via the transfer of a neutron from a Gd160 beam to a Sm154 target.

A Gd160 beam was accelerated to an energy of 1000 MeV and, separately, bombarded thick targets of Sm154 and Dy164 in order to observe neutron-rich, rare-earth nuclei via deep-inelastic collision processes. Gammasphere was utilized to observe ?-ray emissions. Many new states and transitions were observed in Gd160 as a result of so-called unsafe Coulomb excitation. The ground-state band in Gd160 has been extended to Ip=20+ and a rotational band based on the Kp=4+ state, previously associated with a hexadecapole vibration, was observed up to 18+. The quasiparticle configuration of the Kp=4+ band has been determined, and its unusual alignment behavior may result from a possible quenching of static neutron pairing. In addition, the band based on the [523]5/2 quasineutron orbital in Gd161 was extended from 11/2- to 33/2- and also displays the same unusual alignment behavior.

The rare phenomenon of nuclear wobbling motion has been investigated in the nucleus Au187. A longitudinal wobbling-bands pair has been identified and clearly distinguished from the associated signature-partner band on the basis of angular distribution measurements. Theoretical calculations in the framework of the particle rotor model are found to agree well with the experimental observations. This is the first experimental evidence for longitudinal wobbling bands where the expected signature partner band has also been identified, and establishes this exotic collective mode as a general phenomenon over the nuclear chart.

Excited states in Gd160 were populated via β decay from the low- and high-spin isomers in Eu160. The high-spin, Kπ=5- state feeds several two-quasiparticle levels, as well as a sequence associated with a γ vibration and a Kπ=4+, hexadecapole vibrational structure. The decay scheme was significantly improved with the observation of new transitions and states when compared with the two competing level schemes from over four decades ago. Configuration assignments for some of the multiquasiparticle levels have been suggested, based upon decay properties, systematics from neighboring nuclei, and comparisons with theoretical calculations. In addition, 15 new low-spin states and approximately 60 new transitions were observed resulting from the decay of the low-spin Eu160 isomer.

The second-phonon (nω=2) wobbling band has been established in the nucleus $^{135}$Pr. Conclusive evidence for its wobbling nature comes from the ΔI=1, E2 character of the transitions between the new band and the previously identified transverse wobbler band (nω=1) in this nucleus. Theoretical calculations in the framework of the quasiparticle triaxial rotor and triaxial projected shell models are found to be in good agreement with the experimental results.

Using a hybrid Gammasphere array coupled to 25 LaBr3(Ce) detectors, the lifetimes of the first three levels of the yrast band in Pd114, populated via Cf252 decay, have been measured. The measured lifetimes are τ2+=103(10)ps, τ4+=22(13)ps, and τ6+≤10ps for the 21+, 41+, and 61+ levels, respectively. Palladium-114 was predicted to be the most deformed isotope of its isotopic chain, and spectroscopic studies have suggested it might also be a candidate nucleus for low-spin stable triaxiality. From the lifetimes measured in this work, reduced transition probabilities B(E2;J→J-2) are calculated and compared with interacting boson model, projected shell model, and collective model calculations from the literature. The experimental ratio RB(E2)=B(E2;41+→21+)/B(E2;21+→01+)=0.80(42) is measured for the first time in Pd114 and compared with the known values RB(E2) in the palladium isotopic chain: the systematics suggest that, for N=68, a transition from γ-unstable to a more rigid γ-deformed nuclear shape occurs.

International audience; A comprehensive systematic study is made for the collective β and γ bands in even-even isotopes with neutron numbers N=88 to 92 and proton numbers Z=62(Sm) to 70 (Yb). Data, including excitation energies, B(E0) and B(E2) values, and branching ratios from previously published experiments are collated with new data presented for the first time in this study. The experimental data are compared to calculations using a five-dimensional collective Hamiltonian (5DCH) based on the covariant density functional theory (CDFT). A realistic potential in the quadrupole shape parameters V(β,γ) is determined from potential energy surfaces (PES) calculated using the CDFT. The parameters of the 5DCH are fixed and contained within the CDFT. Overall, a satisfactory agreement is found between the data and the calculations. In line with the energy staggering S(I) of the levels in the 2γ+ bands, the potential energy surfaces of the CDFT calculations indicate γ-soft shapes in the N=88 nuclides, which become γ rigid for N=90 and N=92. The nature of the 02+ bands changes with atomic number. In the isotopes of Sm to Dy, they can be understood as β vibrations, but in the Er and Yb isotopes the 02+ bands have wave functions with large components in a triaxial superdeformed minimum. In the vicinity of Sm152, the present calculations predict a soft potential in the β direction but do not find two coexisting minima. This is reminiscent of Sm152 exhibiting an X(5) behavior. The model also predicts that the 03+ bands are of two-phonon nature, having an energy twice that of the 02+ band. This is in contradiction with the data and implies that other excitation modes must be invoked to explain their origin.

An extensive, model-independent analysis of the nature of triaxial deformation in Ge76, a candidate for neutrinoless double-beta (0νββ) decay, was carried out following multistep Coulomb excitation. Shape parameters deduced on the basis of a rotational-invariant sum-rule analysis provided considerable insight into the underlying collectivity of the ground-state and γ bands. Both sequences were determined to be characterized by the same β and γ deformation parameter values. In addition, compelling evidence for low-spin, rigid triaxial deformation in Ge76 was obtained for the first time from the analysis of the statistical fluctuations of the quadrupole asymmetry deduced from the measured E2 matrix elements. These newly determined shape parameters are important input and constraints for calculations aimed at providing, with suitable accuracy, the nuclear matrix elements relevant to 0νββ.

International audience; Triaxial Strongly Deformed (TSD) band structures have been observed in several LuHf-Ta isotopes in the A∼165 region. The occurrence of TSD bands in Lu (Z=71) and Hf (Z=72) isotopes is not consistent with predicted proton and neutron shell gaps, probably due to inadequate knowledge of energies of high-j orbitals at large triaxiality. Based on calculated shell gaps, among the Lu isotopes, 165Lu94 and 168Lu97 are good candidates for TSD structures. However, the strongest TSD band in 163Lu92 is observed to be three times more strongly populated than the corresponding one in 165Lu94, and TSD structures have not yet been observed in 168Lu97. Further, no TSD bands have been observed in 166Hf94, which is located at the centre of the predicted TSD island. The above observations appear to indicate that, at large triaxiality, TSD structures may be favored at N=92 than at N=94. Calculations by R. Bengtsson indicate that TSD band in 166W, with a positive γ value should become yrast at spin, I∼44~. The aforesaid systematic calculations of TSD and Normal Deformed (ND) structures in Hf, Yb and W isotopes further suggest that the N=92 isotones in these three elements have higher excitation energies at normal deformation in the spin range of 30-50 ~ [1]. So, the favorable position of TSD bands in the N=92 isotones may be an outcome of the fact that the band at normal deformation goes up in energy for this neutron number. There were two previous measurements to study high-spin states in 166W. In the first measurement, a 28Si beam was used by Gerl et al. [2] and four HPGe detectors were used to record data. In the second measurement by Simpson et al. [3], the p2n reaction channel was used, and the deexciting γ rays were detected using the POLYTESSA array. The positive-parity yrast band was observed up to an excitation energy of 9 MeV, and spin, I = 30~, well below where possible TSD bands are expected to be yrast. Two other negativeparity rotational bands were also reported up to spin, I = 23~.

The atomic nucleus and its electrons are often thought of as independent systems that are held together in the atom by their mutual attraction. Their interaction, however, leads to other important effects, such as providing an additional decay mode for excited nuclear states, whereby the nucleus releases energy by ejecting an atomic electron instead of by emitting a 3-ray. This 'internal conversion' has been known for about a hundred years and can be used to study nuclei and their interaction with their electrons. In the inverse process - nuclear excitation by electron capture (NEEC) - a free electron is captured into an atomic vacancy and can excite the nucleus to a higher-energy state, provided that the kinetic energy of the free electron plus the magnitude of its binding energy once captured matches the nuclear energy difference between the two states. NEEC was predicted in 1976 and has not hitherto been observed. Here we report evidence of NEEC in molybdenum-93 and determine the probability and cross-section for the process in a beam-based experimental scenario. Our results provide a standard for the assessment of theoretical models relevant to NEEC, which predict cross-sections that span many orders of magnitude. The greatest practical effect of the NEEC process may be on the survival of nuclei in stellar environments, in which it could excite isomers (that is, long-lived nuclear states) to shorter-lived states. Such excitations may reduce the abundance of the isotope after its production. This is an example of 'isomer depletion', which has been investigated previously through other reactions, but is used here to obtain evidence for NEEC.

The structure of deformed neutron-rich nuclei in the rare-earth region is of significant interest for both the astrophysics and nuclear structure fields. At present, a complete explanation for the observed peak in the elemental abundances at A∼160 eludes astrophysicists, and models depend on accurate quantities, such as masses, lifetimes, and branching ratios of deformed neutron-rich nuclei in this region. Unusual nuclear structure effects are also observed, such as the unexpectedly low energies of the first 2+ levels in some even-even nuclei at N=98. In order to address these issues, mass and β-decay spectroscopy measurements of the Eu97160 and Eu99162 nuclei were performed at the Californium Rare Isotope Breeder Upgrade radioactive beam facility at Argonne National Laboratory. Evidence for a gap in the single-particle neutron energies at N=98 and for large deformation (β2∼0.3) is discussed in relation to the unusual phenomena observed at this neutron number.

Fast-rotating N=151 isotones 245Pu, 247Cm and 249Cf have been studied through inelastic excitation and transfer reactions with radioactive targets. While all have a ground-state band built on a νj15/2[734]9/2− Nilsson configuration, new excited bands have also been observed in each isotone. These odd-N excited bands allow a comparison of the alignment behavior for two different configurations, where the νj15/2 alignment is either blocked or allowed. The effect of higher order deformations is explored through cranking calculations, which help clarify the elusive nature of νj15/2 alignments. Keywords: Superheavy, Neutron-rich, Inelastic and transfer reactions, Rotational alignments, Higher-order deformations

An experiment populating low/medium-spin states in Dy156 was performed to investigate the possibility of tetrahedral symmetry in this nucleus. In particular, focus was placed on the low-spin, negative-parity states since recent theoretical studies suggest that these may be good candidates for this high-rank symmetry. The states were produced in the Nd148(C12,4n) reaction and the Gammasphere array was utilized to detect the emitted γ rays. B(E2)/B(E1) ratios of transition probabilities from the low-spin, negative-parity bands were determined and used to interpret whether these structures are best associated with tetrahedral symmetry or, as previously assigned, to octupole vibrations. In addition, several other negative-parity structures were observed to higher spin and two new sequences were established.

The first rotational sequences have been assigned to the odd-odd nucleus Re168. Coincidence relationships of these structures with rhenium x rays confirm the isotopic assignment, while arguments based on the γ-ray multiplicity (K-fold) distributions observed with the new bands lead to the mass assignment. Configurations for the two bands were determined through analysis of the rotational alignments of the structures and a comparison of the experimental B(M1)/B(E2) ratios with theory. Tentative spin assignments are proposed for the πh11/2νi13/2 band, based on energy level systematics for other known sequences in neighboring odd-odd rhenium nuclei, as well as on systematics seen for the signature inversion feature that is well known in this region. The spin assignment for the πh11/2ν(h9/2/f7/2) structure provides additional validation of the proposed spins and configurations for isomers in the Au176 → Ir172→Re168 α-decay chain.

International audience; The exact nature of the lowest Kπ=2+ rotational bands in all deformed nuclei remains obscure. Traditionally they are assumed to be collective vibrations of the nuclear shape in the γ degree of freedom perpendicular to the nuclear symmetry axis. Very few such γ bands have been traced past the usual backbending rotational alignments of high-j nucleons. We have investigated the structure of positive-parity bands in the N=90 nucleus Dy156, using the Nd148(C12,4n)Dy156 reaction at 65 MeV, observing the resulting γ-ray transitions with the Gammasphere array. The even- and odd-spin members of the Kπ=2+γ band are observed up to 32+ and 31+, respectively. This rotational band faithfully tracks the ground-state configuration to the highest spins. The members of a possible γ vibration built on the aligned yrast S band are observed up to spins 28+ and 27+. An even-spin positive-parity band, observed up to spin 24+, is a candidate for an aligned S band built on the seniority-zero configuration of the 0+2 state at 676 keV. The crossing of this band with the 0+2 band is at ℏωc=0.28(1)MeV and is consistent with the configuration of the 0+2 band not producing any blocking of the monopole pairing.

Excited states in the N=88 nucleus Tb153 were observed up to spin ∼40 in an experiment utilizing the Gammasphere array. The Tb153 states were populated in a weak α4n evaporation channel of the Cl37 + Sn124 reaction. Two previously known sequences were extended to higher spins, and a new decoupled structure was identified. The πh11/2 band was observed in the spin region where other N=88 isotopes exhibit effects of prolate to oblate shape changes leading to band termination along the yrast line, whereas Tb153 displays a persistent collective behavior. However, minor perturbations of the very highest state in both signatures of this h11/2 band are observed, which perhaps signal the start of the transition towards band termination.

The exact nature of the lowest Kπ=2+ rotational bands in all deformed nuclei remains obscure. Traditionally they are assumed to be collective vibrations of the nuclear shape in the γ degree of freedom perpendicular to the nuclear symmetry axis. Very few such γ bands have been traced past the usual backbending rotational alignments of high-j nucleons. We have investigated the structure of positive-parity bands in the N=90 nucleus Dy156, using the Nd148(C12,4n)Dy156 reaction at 65 MeV, observing the resulting γ-ray transitions with the Gammasphere array. The even- and odd-spin members of the Kπ=2+γ band are observed up to 32+ and 31+, respectively. This rotational band faithfully tracks the ground-state configuration to the highest spins. The members of a possible γ vibration built on the aligned yrast S band are observed up to spins 28+ and 27+. An even-spin positive-parity band, observed up to spin 24+, is a candidate for an aligned S band built on the seniority-zero configuration of the 02+ state at 676 keV. The crossing of this band with the 02+ band is at ?ωc=0.28(1)MeV and is consistent with the configuration of the 02+ band not producing any blocking of the monopole pairing.

The Sn124(Cl37,6nγ) fusion-evaporation reaction at a bombarding energy of 180 MeV has been used to significantly extend the excitation level scheme of 67155Ho88. The collective rotational behavior of this nucleus breaks down above spin I∼30 and a fully aligned noncollective (band terminating) state has been identified at Iπ=79/2-. Comparison with cranked Nilsson-Strutinsky calculations also provides evidence for core-excited noncollective states at Iπ=87/2- and (89/2+) involving particle-hole excitations across the Z=64 shell gap. A similar core-excited state in 68156Er88 at Iπ=(46+) is also presented.

A pair of transverse wobbling bands is observed in the nucleus Pr135. The wobbling is characterized by ΔI=1, E2 transitions between the bands, and a decrease in the wobbling energy confirms its transverse nature. Additionally, a transition from transverse wobbling to a three-quasiparticle band comprised of strong magnetic dipole transitions is observed. These observations conform well to results from calculations with the tilted axis cranking model and the quasiparticle rotor model.

A significant extension of the level scheme for the odd-odd nucleus Re172 was accomplished through the use of the Gammasphere spectrometer. States up to a tentative spin assignment of 39 were observed and two new structures were identified. Configuration assignments are proposed based on alignment properties and observed band crossings.

Fast-rotating N=151 isotones 245Pu, 247Cm and 249Cf have been studied through inelastic excitation and transfer reactions with radioactive targets. While all have a ground-state band built on a νj15/2[734]9/2- Nilsson configuration, new excited bands have also been observed in each isotone. These odd-N excited bands allow a comparison of the alignment behavior for two different configurations, where the νj15/2 alignment is either blocked or allowed. The effect of higher order deformations is explored through cranking calculations, which help clarify the elusive nature of νj15/2 alignments.

Excited states of Hf163 were populated using the Zr94(Ge74,5n) reaction and the decay γ rays were measured with the Gammasphere spectrometer. Two previously known bands were extended to higher spins, and nine new bands were identified. In addition to bands associated with three- and five-quasiparticle configurations, two γ-vibrational bands coupled to the i13/2 excitation were also observed. The lowest level of a newly identified, negative-parity band is proposed to be the ground state of the nucleus. A systematic delay of the high-spin proton crossing frequency with increasing quadrupole deformation from Hf162 to Hf172 was established. Extensive band searches failed to reveal a triaxial, strongly deformed structure in Hf163 similar to the one observed in several nuclei around A∼165.

A detailed level scheme for Th221 has been established in an experiment using the O18+207Pb reaction at 96 MeV. The evaporation residues from this fissile system were selected with the HERCULES detector array and residue-gated γ rays were measured with Gammasphere. Three band structures of interlinked, alternating-parity levels are observed, two of which are non-yrast. In addition, several high-lying excitations are found. The yrast band is seen up to spin-parity 37/2- and 39/2+, beyond which a high-spin feeding transition is observed. The non-yrast sequences are interpreted as parity-doublet structures, based on a configuration similar to that of the yrast band in Th223 (K=5/2). The key properties of even-odd nuclei in this mass region [B(E1)/B(E2) and B(M1)/B(E2) ratios, spin alignments, parity splittings] are reviewed.

High-spin states of 187Ir have been populated in the 176Yb(15N, 4n) reaction and measured with the YRAST Ball spectrometer. The ?h9/2 rotational band has been extended beyond the first alignment crossing, which was found at rotational frequency ??c ? 0.39 MeV. Two different scenarios for describing this crossing are considered: The alignment of an h9/2 proton or i13/2 neutron pair and it is concluded that a proton band crossing is more likely. A systematic study of the rotational alignment crossings in the ?h9/2 bands in the N=104, 106, 108 isotopes of 73Ta, 75Re, 77Ir, and 79Au is presented.

High-spin states of [Formula presented] have been populated in the [Formula presented] reaction and measured with the YRAST Ball spectrometer. The [Formula Presented] rotational band has been extended beyond the first alignment crossing, which was found at rotational frequency [Formula Presented]. Two different scenarios for describing this crossing are considered: the alignment of an [Formula Presented] proton or [Formula Presented] neutron pair and it is concluded that a proton band crossing is more likely. A systematic study of the rotational alignment crossings in the [Formula Presented] bands in the [Formula Presented] isotopes of [Formula presented] and [Formula presented] is presented. © 2003 The American Physical Society.

Although the observation of wobbling was once thought to be possibly confined to lutetium isotopes in N≈94 nuclei, the identification of this exotic collective mode in 167Ta has raised the question of the role of the proton Fermi surface with regard to this phenomenon. To investigate this issue, an experiment was performed to populate high-spin states in the N=94 nucleus 169Re. The heavy-ion reaction 55Mn+118Sn was used in conjunction with Gammasphere to detect the emitted γ rays. More than 130 new transitions were added to the 169Re level scheme, including the first identification of the πi13/2 rotational sequence in this nucleus. This configuration is the structure on which all known wobbling sequences are based, but no wobbling band was observed, likely owing to the fact that the πi13/2 sequence is located at a relatively high energy in comparison with the other structures found in 169Re. Nine decay sequences are now established in this nucleus and are described within the context of the cranked shell model. In addition, significant extension of the level scheme of the odd-odd 170Re nucleus was possible and a discussion of the residual interactions for the πh 9/2νi13/2 and πi13/2νi13/2 configurations in this region is given as well.

Two new rotational bands of distinct character have been identified in 164Hf. They are suggested to correspond to the long-anticipated triaxial strongly deformed (TSD) bands predicted by theoretical studies. The bands have been linked to known states, and the level spins and energies could be determined. The bands are also substantially stronger in intensity and are located at lower spins than the previously observed TSD bands in 168Hf, hereby making 164Hf the best even-even system so far for the study of TSD structures in the A∼160 mass region. Cranking calculations based on the modified-oscillator model suggest that the bands are associated with four-quasiparticle configurations that involve high-j intruder (i13/2)2 proton orbitals.

The phenomenon of wobbling can only occur for a nuclear shape with stable triaxial deformation. To date, only a few examples of this exotic collective mode have been observed in lutetium and tantalum isotopes. A search for a wobbling sequence was performed in 171Re to determine if this feature can be observed in Z>73 nuclei. No evidence was found for wobbling; however, an interaction between the πi13/2 sequence and another positive-parity band may give an indication on why wobbling may not occur in this nucleus. The level scheme for 171Re was significantly extended and interpretations for the decay sequences are proposed within the context of the cranked shell model.

High-spin properties of the nucleus 171Hf were studied through the 128Te(48Ca,5n) reaction. Previously known bands have been extended to significantly higher spins and four new bands have been extracted from these data. The results are discussed within the framework of the cranked shell model aided by a comparison with level structures in the neighboring nuclei. The band crossings at rotational frequencies ∼500 keV are interpreted as caused by the alignments of h11/2 and h9/2 proton orbitals. Band ED2 exhibits an alignment pattern similar to that of band ED1 which was reported in a recent paper and proposed to be built on a second potential energy minimum involving the deformation-driving proton i13/2 - h9/2 configuration. It is likely that band ED2 is also associated with a deformation enhanced with respect to that of the normal deformed structures. Further experimental investigation is needed to ascertain the nature of this band.

A new collective band with high dynamic moment of inertia in 158Er at spins beyond band termination has been found in addition to the two previously reported ones. The measured transition quadrupole moments (Qt) of these three bands are very similar. These three bands have been suggested to possess a triaxial strongly deformed shape, based on comparisons with calculations using the cranked Nilsson-Strutinsky model and with tilted axis cranking calculations using the Skyrme-Hartree-Fock model. In addition, three collective bands with similar high dynamic moments of inertia, tentatively assigned to 157Ho, have been observed. Thus, it is suggested that all these structures share a common underlying character and that they are most likely associated with triaxial strongly deformed minima which are predicted to be close to the yrast line at spin 50 - 70h.