Search

The two-loop self-energy correction to the bound-electron $g$-factor in hydrogenlike ions is investigated, taking into account the electron-nucleus interaction exactly. This all-order calculation is required to improve the total theoretical uncertainty of the $g$-factor, which is limited by the fact that two-loop self-energy corrections have only been calculated so far in the form of an expansion in $Z\alpha$. Here, $Z$ is the nuclear charge number and $\alpha$ is the fine-structure constant. In this work, we report calculations of the last missing parts of the total two-loop self-energy correction, exactly in $Z\alpha$. We apply our theory to the recently measured $g$-factor of the hydrogenlike $^{118}$Sn$^{49+}$ ion [J. Morgner et al., Nature 622, 53 (2023)] and, with a factor of 8, improve the accuracy of its state-of-the-art theoretical value by almost one order of magnitude, enabling more detailed tests of quantum electrodynamics and new physics in strong fields., Comment: 6 pages, 4 figures

Many powerful tests of the Standard Model of particle physics and searches for new physics with precision atomic spectroscopy are plagued by our lack of knowledge of nuclear properties. Ideally, such properties may be derived from precise measurements of the most sensitive and theoretically best-understood observables, often found in hydrogen-like systems. While these measurements are abundant for the electric properties of nuclei, they are scarce for the magnetic properties, and precise experimental results are limited to the lightest of nuclei. Here, we focus on $^9$Be which offers the unique possibility to utilize comparisons between different charge states available for high-precision spectroscopy in Penning traps to test theoretical calculations typically obscured by nuclear structure. In particular, we perform the first high-precision spectroscopy of the $1s$ hyperfine and Zeeman structure in hydrogen-like $^9$Be$^{3+}$. We determine its effective Zemach radius with an uncertainty of $500$ ppm, and its bare nuclear magnetic moment with an uncertainty of $0.6$ parts-per-billion (ppb) - uncertainties unmatched beyond hydrogen. Moreover, we compare to measurements conducted on the three-electron charge state $^9$Be$^{+}$, which, for the first time, enables testing the calculation of multi-electron diamagnetic shielding effects of the nuclear magnetic moment at the ppb level. In addition, we test quantum electrodynamics (QED) methods used for the calculation of the hyperfine splitting. Our results serve as a crucial benchmark essential for transferring high-precision results of nuclear magnetic properties across different electronic configurations.

The Standard Model of particle physics describes the properties of elementary particles and their interactions remarkably well, but in particular does not account for dark matter. Isotope-shift spectroscopy is a sensitive probe of fifth forces and new particles that illuminate the dark matter sector. This method sets bounds on new bosons that couple neutrons and electrons with masses in the keV/c2 to MeV/c2 range. With increasing spectroscopic precision, such searches are limited by uncertainties of isotope masses and the understanding of nuclear structure. Here, we report on high-precision mass-ratio and isotope-shift measurements of the ytterbium isotopes $^{168,170,172,174,176}$Yb that exceed previous measurements by up to two orders of magnitude. From these measurements, we extract higher-order changes in the nuclear charge distribution along the Yb isotope chain and use these to benchmark novel ab initio calculations. Our measurements set new bounds on the existence of the proposed boson.

Ab initio QED calculations of the nuclear magnetic shielding constant in helium-like ions are presented. We combine the nonrelativistic QED approach based on an expansion in powers of the fine-structure constant $\alpha$ and the so-called ``all-order'' QED approach which includes all orders in the parameter $Z\alpha$ but uses a perturbation expansion in the parameter $1/Z$ (where $Z$ is the nuclear charge number). The combination of the two complementary methods makes our treatment applicable both to low-$Z$ and high-$Z$ ions. Our calculations confirm the presence of a rare antiscreening effect for the relativistic shielding correction and demonstrate the importance of the inclusion of the negative-energy part of the Dirac spectrum.

The investigation of the absolute scale of the effective neutrino mass remains challenging due to the exclusively weak interaction of neutrinos with all known particles in the standard model of particle physics. Currently, the most precise and least model-dependent upper limit on the electron antineutrino mass is set by the KATRIN experiment from the analysis of the tritium \b{eta}-decay. Another promising approach is the electron capture in $^{163}\mathrm{Ho}$, which is under investigation using microcalorimetry within the ECHo and HOLMES collab orations. An independently measured Q-value of this process is vital for the assessment of systematic uncertainties in the neutrino mass determination. Here, we report a direct, independent determination of this $Q$-value by measuring the free-space cyclotron frequency ratio of highly charged ions of $^{163}\mathrm{Ho}$ and $^{163}\mathrm{Dy}$ in the Penning trap experiment \textsc{Pentatrap}. Combining this ratio with atomic physics calculations of the electronic binding energies yields a $Q$-value of $2863.2(0.6)\,\mathrm{eV}/c^{2}$ - a more than 50-fold improvement over the state-of-the-art. This will enable the determination of the electron neutrino mass on a sub-eV level from the analysis of the electron capture in $^{163}\mathrm{Ho}$.

The atomic mass of uranium-238 has been determined to be $238.050\,787\,618(15)\,\text{u}$, improving the literature uncertainty by two orders of magnitude. It is obtained from a measurement of the mass ratio of $^{238}$U$^{47+}$ and $^{132}$Xe$^{26+}$ ions with an uncertainty of $3.5\times 10^{-12}$. The measurement was carried out with the Penning-trap mass spectrometer \textsc{Pentatrap} and was accompanied by a calculation of the binding energies $E_{\text{U}}$ and $E_{\text{Xe}}$ of the 47 and 26 missing electrons of the two highly charged ions, respectively. These binding energies were determined using an \textit{ab initio} multiconfiguration Dirac-Hartree-Fock (MCDHF) method to be $E_{\text{U}} = 39\,927(10)\,\text{eV}$ and $E_{\text{Xe}} = 8\,971.2(21)\,\text{eV}$. The new mass value will serve as a reference for high-precision mass measurements in the heavy mass region of the nuclear chart up to transuranium nuclides., Comment: Includes a Supplemental Material

Highly charged ions (HCIs) offer many opportunities for next-generation clock research due to the vast landscape of available electronic transitions in different charge states. The development of XUV frequency combs has enabled the search for clock transitions based on shorter wavelengths in HCIs. However, without initial knowledge of the energy of the clock states, these narrow transitions are difficult to be probed by lasers. In this Letter, we provide experimental observation and theoretical calculation of a long-lived electronic state in Nb-like Pb$^{41+}$ which could be used as a clock state. With the mass spectrometer Pentatrap, the excitation energy of this metastable state is directly determined as a mass difference at an energy of 31.2(8) eV, corresponding to one of the most precise relative mass determinations to date with a fractional uncertainty of $4\times10^{-12}$. This experimental result agrees within 1 $\sigma$ with two partially different \textit{ab initio} multi-configuration Dirac-Hartree-Fock calculations of 31.68(13) eV and 31.76(35) eV, respectively. With a calculated lifetime of 26.5(5.3) days, the transition from this metastable state to the ground state bears a quality factor of $1.1\times10^{23}$ and allows for the construction of a HCI clock with a fractional frequency instability of $<10^{-19}/\sqrt{\tau}$.

Self-energy corrections to the energy levels of bound electrons are calculated in the framework of path integrals. We arrive at the full fermion propagator, using methods of functional integrals, in the form of Schwinger-Dyson equation (SDE). From the full fermion SDE, the self-energy corrected propagator is identified and the energy shift is obtained from the poles of the spectral function. The numerical calculations are performed using complex contour integrals and the B-spline representation of basis functions. We identify ions with Lamb shifts observable via modern mass spectrometric methods.

Vacuum polarization corrections to the energy levels of bound electrons are calculated using a perturbative path integral formalism. We apply quantum electrodynamics in a framework which treats the strong binding nuclear field to all orders. The effective potential, derived from the Dyson-Schwinger equation for the photon propagator, is then considered pertubatively. Expressions for the vacuum polarization shift of binding energies is obtained from the poles of the spectral function up to second order. Numerical results are provided to select candidates for novel tests of strong-field quantum electrodynamics by means of precision mass spectrometry.

The relativistic Green's function of a free spin-1/2 fermion is derived using the Feynman path integral formalism in spherical coordinates. The Green's function is reduced to an exactly solvable path integral by an appropriate coordinate transformation. The result is given in terms of spherical Bessel functions and spherical spinors, and agrees with previous solutions of the problem.

Highly charged ions (HCIs) are insensitive to external perturbations and are attractive for the development of ultrastable clocks. However, only a few HCI candidates are known to provide optical clock transitions. In this Letter, we show that, as a result of strong relativistic effects, there are more than 100 suitable optical HCI clock candidates in more than 70 elements. Their transitions are embedded in the fine-structure splitting of the $nd^4$, $nd^5$ and $nd^6$ ground-state configurations with $n=3,4,5$ being the principal quantum numbers. The corresponding high multipolarity transitions in these ions have lifetimes and quality factors many orders of magnitude longer and larger, respectively, than those in state-of-the-art clocks. Their polarizabilities are also orders of magnitude smaller, rendering them more stable against external electromagnetic fields. Furthermore, within the same electronic configurations, the clock transitions in heavy ions scale up to the XUV and soft-x-ray region, thus enable the development of clocks based on shorter wavelengths. The existence of multiple clock transitions in different charge states of a single element, as well as in a whole isoelectronic sequence, would significantly enrich the detection of fine-structure constant variations, the search for new physics and the test of nuclear theories via high-precision spectroscopy., Comment: 4 pages in main text, 4 figures

The hadronic vacuum polarization correction to the $g$ factor of a bound electron is investigated theoretically. An effective hadronic Uehling potential obtained from measured cross sections of $e^- e^+$ annihilation into hadrons is employed to calculate $g$ factor corrections for low-lying hydrogenic levels. Analytical Dirac-Coulomb wave functions, as well as bound wave functions accounting for the finite nuclear radius are used. Closed formulas for the $g$ factor shift in case of a point-like nucleus are derived. In heavy ions, such effects are found to be much larger than for the free-electron $g$ factor.

The absolute atomic mass of $^{208}$Pb has been determined with a fractional uncertainty of $7\times 10^{-11}$ by measuring the cyclotron-frequency ratio $R$ of $^{208}$Pb$^{41+}$ to $^{132}$Xe$^{26+}$ with the high-precision Penning-trap mass spectrometer Pentatrap and computing the binding energies $E_{\text{Pb}}$ and $E_{\text{Xe}}$ of the missing 41 and 26 atomic electrons, respectively, with the ab initio fully relativistic multi-configuration Dirac-Hartree-Fock (MCDHF) method. $R$ has been measured with a relative precision of $9\times 10^{-12}$. $E_{\text{Pb}}$ and $E_{\text{Xe}}$ have been computed with an uncertainty of 9.1 eV and 2.1 eV, respectively, yielding $207.976\,650\,571(14)$ u (u$=9.314\,941\,024\,2(28)\times 10^{8}$ eV/c$^2$) for the $^{208}$Pb neutral atomic mass. This result agrees within $1.2\sigma$ with that from the Atomic-Mass Evaluation (AME) 2020, while improving the precision by almost two orders of magnitude. The new mass value directly improves the mass precision of 14 nuclides in the region of Z=81-84 and is the most precise mass value with A>200. Thus, the measurement establishes a new region of reference mass values which can be used e.g. for precision mass determination of transuranium nuclides, including the superheavies., Comment: 8 pages, 4 figures, to be published in EPJA

The shift of atomic energy levels due to hadronic vacuum polarization is evaluated in a semiempirical way for hydrogenlike ions and for muonic hydrogen. A parametric hadronic polarization function obtained from experimental cross sections of $e^-e^+$ annihilation into hadrons is applied to derive an effective relativistic Uehling potential. The energy corrections originating from hadronic vacuum polarization are calculated for low-lying levels using analytical Dirac-Coulomb wave functions, as well as bound wave functions accounting for the finite nuclear size. Closed formulas for the hadronic Uehling potential of an extended nucleus as well as for the relativistic energy shift in case of a point-like nucleus are derived. These results are compared to existing analytic formulas from non-relativistic theory.

When collecting spectroscopic data on at least four isotopes, nonlinearities in the King plot are a possible sign of Physics beyond the Standard Model. In this work, an improved approach to the search for hypothetical new interactions with isotope shift spectroscopy of few-electron ions is presented. Very careful account is taken of the small nuclear corrections to the energy levels and the gyromagnetic factors, which cause deviations from King linearity within the Standard Model and are hence a possible source of confounds. In this new approach, the experimental King nonlinearity is not compared to the vanishing prediction of the Standard Model at the leading order, but to the calculated full Standard Model contribution to King nonlinearity. This makes searching for beyond-the-Standard-Model physics with King linearity analysis possible in a very-high-precision experimental regime, avoiding confounds. The bounds which can be set on beyond-the-Standard-Model parameters remain limited by the uncertainties on the small Standard Model nuclear corrections which cause King nonlinearity. Direct comparison between theory and experiment on a single pair of isotopes is advocated as a more suitable approach for few-electron ions.

The quantum electrodynamic (QED) description of light-and-matter interaction is one of the most fundamental theories of physics and has been shown to be in excellent agreement with experimental results. Specifically, measurements of the electronic magnetic moment (or $g$ factor) of highly charged ions (HCI) in Penning traps can provide a stringent probe for QED, testing the Standard model in the strongest electromagnetic fields. When studying the difference of isotopes, even the intricate effects stemming from the nucleus can be resolved and tested as, due to the identical electron configuration, many common QED contributions do not have to be considered. Experimentally however, this becomes quickly limited, particularly by the precision of the ion masses or the achievable magnetic field stability. Here we report on a novel measurement technique that overcomes both of these limitations by co-trapping two HCIs in a Penning trap and measuring the difference of their $g$ factors directly. The resulting correlation of magnetic field fluctuations leads to drastically higher precision. We use a dual Ramsey-type measurement scheme with the ions locked on a common magnetron orbit, separated by only a few hundred micrometres, to extract the coherent spin precession frequency difference. We have measured the isotopic shift of the bound electron $g$ factor of the neon isotopes of $^{20}$Ne$^{9+}$ and $^{22}$Ne$^{9+}$ to 0.56 parts-per-trillion ($5.6 \cdot 10^{-13}$) precision relative to their $g$ factors, which is an improvement of more than two orders of magnitude compared to state-of-the-art techniques. This resolves the QED contribution to the nuclear recoil for the very first time and accurately validates the corresponding theory. Furthermore, the agreement with theory allows setting constraints for a fifth-force, resulting from Higgs-portal-type dark-matter interactions., Comment: 22 pages, 5 figures

A highly effective approach to the search for hypothetical new interactions through isotope shift spectroscopy of hydrogen-like ions is presented. A weighted difference of the g factor and ground-state energy is shown to assist in the suppression of detrimental uncertainties from nuclear structure, while preserving the hypothetical contributions from new interactions. Experimental data from only a single isotope pair is required. Account is taken of the small, subleading nuclear corrections, allowing to show that, provided feasible experimental progress is achieved in UV/X-ray spectroscopy, the presented approach can yield competitive bounds on New Physics electron coupling parameters improved by more than an order of magnitude compared to leading bounds from atomic physics.

One of the most enduring and intensively studied problems of X-ray astronomy is the disagreement of state-of-the art theory and observations for the intensity ratio of two Fe XVII transitions of crucial value for plasma diagnostics, dubbed 3C and 3D. We unravel this conundrum at the PETRA III synchrotron facility by increasing the resolving power two and a half times and the signal-to-noise ratio thousand-fold compared to our previous work. The Lorentzian wings had hitherto been indistinguishable from the background and were thus not modeled, resulting in a biased line-strength estimation. The present experimental oscillator-strength ratio $R_\mathrm{exp}=f_{\mathrm{3C}}/f_{\mathrm{3D}}=3.51(2)_{\mathrm{stat}}(7)_{\mathrm{sys}}$ agrees with our state-of-the-art calculation of $R_\mathrm{th}=3.55(2)$, as well as with some previous theoretical predictions. To further rule out any uncertainties associated with the measured ratio, we also determined the individual natural linewidths and oscillator strengths of 3C and 3D transitions, which also agree well with the theory. This finally resolves the decades-old mystery of Fe XVII oscillator strengths., Comment: Main manuscript and supplemental material at https://journals.aps.org/prl/supplemental/10.1103/PhysRevLett.129.245001/LN17392_Supplemental_Material.pdf

Large-scale $\textit{ab initio}$ calculations of the electric field gradient, which constitutes the electronic contribution to the electric quadrupole hyperfine constant $B$, were performed for the $5s^25p6s$ $^{1,3}\!P^{\rm o}_1$ excited states of tin, using three independent computational strategies of the variational multiconfiguration Dirac-Hartree-Fock method and a fourth approach based on the configuration interaction Dirac-Fock-Sturm theory. For the $5s^25p6s$ $^{1}\!P^{\rm o}_1$ state, the final value of $B/Q =703(50)$ MHz/b differs by $0.4\%$ from the one recently used by Yordanov ${\it et~al.}$ [Communications Physics ${\bf 3}$, 107 (2020)] to extract the nuclear quadrupole moments, $Q$, for tin isotopes in the range $^{(117-131)}$Sn from collinear laser spectroscopy measurements. Efforts were made to provide a realistic theoretical uncertainty for the final $B/Q$ value of the $5s^25p6s\,^{1}\!P^{\rm o}_1$ state based on statistical principles and on correlation with the magnetic dipole hyperfine constant $A$., Comment: 47 pages, 4 figures

A scheme to infer the temporal coherence of EUV frequency combs generated from intra-cavity high-order harmonic generation is put forward. The excitation dynamics of highly charged Mg-like ions, interacting with EUV pulse trains featuring different carrier-envelope-phase fluctuations, are simulated. While demonstrating the microscopic origin of the macroscopic equivalence between excitations induced by pulse trains and continuous-wave lasers, we show that the coherence time of the pulse train can be determined from the spectrum of the excitations. The scheme will provide a verification of the comb temporal coherence at time scales several orders of magnitude longer than current state of the art, and at the same time will enable high-precision spectroscopy of EUV transitions with a relative accuracy up to $\delta\omega/\omega\sim10^{-17}$., Comment: 6 pages, 3 figures and 1 table

State-of-the-art optical clocks achieve fractional precisions of $10^{-18}$ and below using ensembles of atoms in optical lattices or individual ions in radio-frequency traps. Promising candidates for novel clocks are highly charged ions (HCIs) and nuclear transitions, which are largely insensitive to external perturbations and reach wavelengths beyond the optical range, now becoming accessible to frequency combs. However, insufficiently accurate atomic structure calculations still hinder the identification of suitable transitions in HCIs. Here, we report on the discovery of a long-lived metastable electronic state in a HCI by measuring the mass difference of the ground and the excited state in Re, the first non-destructive, direct determination of an electronic excitation energy. This result agrees with our advanced calculations, and we confirmed them with an Os ion with the same electronic configuration. We used the high-precision Penning-trap mass spectrometer PENTATRAP, unique in its synchronous use of five individual traps for simultaneous mass measurements. The cyclotron frequency ratio $R$ of the ion in the ground state to the metastable state could be determined to a precision of $\delta R=1\cdot 10^{-11}$, unprecedented in the heavy atom regime. With a lifetime of about 130 days, the potential soft x-ray frequency reference at $\nu=4.86\cdot 10^{16}\,\text{Hz}$ has a linewidth of only $\Delta \nu\approx 5\cdot 10^{-8}\,\text{Hz}$, and one of the highest electronic quality factor ($Q=\frac{\nu}{\Delta \nu}\approx 10^{24}$) ever seen in an experiment. Our low uncertainty enables searching for more HCI soft x-ray clock transitions, needed for promising precision studies of fundamental physics in a thus far unexplored frontier.

A state-of-the-art approach for calculating the finite nuclear size correction to atomic energy levels and the bound-electron $g$ factor is introduced and demonstrated for a series of highly charged hydrogen-like ions. Firstly, self-consistent mean-field calculations based on the Skyrme-type nuclear interaction are employed in order to produce a realistic nuclear proton distribution. In the second step, the obtained nuclear charge density is used to construct the potential of an extended nucleus, and the Dirac equation is solved numerically. The ambiguity in the choice of a Skyrme parametrization is supressed by fine-tuning of only one parameter of the Skyrme force in order to accurately reproduce the experimental values of nuclear radii in each particular case. The homogeneously charged sphere approximation, the two-parameter Fermi distribution and experimental nuclear charge distributions are used for comparison with our approach, and the uncertainties of the presented calculations are estimated. In addition, suppression of the finite nuclear size effect for the specific differences of $g$ factors is demonstrated., Comment: 8 pages, 1 figure, 4 tables

For more than 40 years, most astrophysical observations and laboratory studies of two key soft x-ray diagnostic $2p-3d$ transitions, $3C$ and $3D$, in Fe XVII ions found oscillator strength ratios $f(3C)/f(3D)$ disagreeing with theory, but uncertainties had precluded definitive statements on this much studied conundrum. Here, we resonantly excite these lines using synchrotron radiation at PETRA III, and reach, at a millionfold lower photon intensities, a 10 times higher spectral resolution, and 3 times smaller uncertainty than earlier work. Our final result of $f(3C)/f(3D) = 3.09(8)(6)$ supports many of the earlier clean astrophysical and laboratory observations, while departing by five sigmas from our own newest large-scale ab initio calculations, and excluding all proposed explanations, including those invoking nonlinear effects and population transfers., Comment: Main text (6 pages, 3 figures), Supplmentary Material (8 pages, 4 figure), Published in Physical Review Letters

Theoretical and experimental resonance strengths for KLL dielectronic recombination (DR) into He-, Li-, Be-, and B-like mercury ions are presented, based on state-resolved DR x-ray spectra recorded at the Heidelberg electron beam ion trap. The DR resonance strengths were experimentally extracted by normalizing them to simultaneously recorded radiative recombination signals. The results are compared to state-of-the-art atomic calculations that include relativistic electron-electron correlation and configuration mixing effects. Combining the present data with other existing ones, we derive an improved semi-empirical $Z$-scaling law for DR resonance strength as a function of the atomic number, taking into account higher-order relativistic corrections, which are especially relevant for heavy highly charged ions., Comment: 11 pages, 4 figures, accepted to Phys. Rev. A

Since the advent of x-ray free-electron lasers (XFELs), considerable efforts have been devoted to achieve x-ray pulses with better temporal coherence. Here, we put forward a scheme to generate fully coherent x-ray lasers (XRLs) based on population inversion in highly charged ions (HCIs), created by fast inner-shell photoionization using XFEL pulses in a laser-produced plasma. Numerical simulations show that one can obtain high-intensity, femtosecond x-ray pulses of relative bandwidths $\Delta\omega/\omega=10^{-5}$ - $10^{-7}$ by orders of magnitude narrower than in XFEL pulses for wavelengths down to the sub-\aa{}ngstr\"om regime. Such XRLs may be applicable in the study of x-ray quantum optics and metrology, investigating nonlinear interactions between x-rays and matter, or in high-precision spectroscopy studies in laboratory astrophysics., Comment: 5 pages, 3 figures, 1 table

Numerous few-electron atomic systems are considered which can be used effectively for observing a potential variation of the fine-structure constant $\alpha$ and the electron-proton mass ratio $m_e/m_p$. We examine optical magnetic dipole transitions between hyperfine-structure components in heavy highly charged H-like and Li-like ions with observably high sensitivity to a variation of $\alpha$ and $m_e/m_p$. The experimental spectra of the proposed systems consist of a strong single line, which simplifies significantly the data analysis and shortens the necessary measurement time. Furthermore, we propose systems for an experimental test of the variation of quark masses and discuss the expected level of accuracy in assessing its limitations. Finally, we establish which constraints on the variation of these fundamental constants could be provided by measurements with a hyperfine-structure highly-charged-ion clock and some reference clock, showing that a significant improvement of the current limitations can be reached.

Strong-field quantum-state control is investigated, taking advantage of the full---amplitude and phase---characterization of the interaction between matter and intense ultrashort pulses via transient-absorption spectroscopy. A sequence of intense delayed pulses is used, whose parameters are tailored to steer the system into a desired quantum state. We show how to experimentally enable this optimization by retrieving all quantum features of the light-matter interaction from observable spectra. This provides a full characterization of the action of strong fields on the atomic system, including the dependence upon possibly unknown pulse properties and atomic structures. Precision and robustness of the scheme are tested, in the presence of surrounding atomic levels influencing the system's dynamics., Comment: 6 pages, 4 figures

The influence of nonlinear dynamical effects is analyzed on the observed spectra of controversial 3C and 3D astrophysically relevant x-ray lines in neonlike Fe${}^{16+}$ and the A, B, C lines in natriumlike Fe${}^{15+}$ ions. First, a large-scale configuration-interaction calculation of oscillator strengths is performed with the inclusion of higher-order electron-correlation effects. Also, quantum-electrodynamic corrections to the transition energies are calculated. Further considered dynamical effects provide a possible resolution of the discrepancy between theory and experiment found by recent x-ray free-electron-laser measurements of these controversial lines. We find that, for strong x-ray sources, the modeling of the spectral lines by a peak with an area proportional to the oscillator strength is not sufficient and nonlinear dynamical effects have to be taken into account. Thus, we advocate the use of light-matter-interaction models also valid for strong light fields in the analysis and interpretation of the associated astrophysical and laboratory spectra. We investigate line-strength ratios distinguishing between the coherent and incoherent parts of the emission spectrum. In addition, the spectrum of Fe${}^{15+}$, an autoionizing ion which was also present in the recent laboratory experiment, is also analized., Comment: 16 pages, 10 figures

Direct laser acceleration of ions by short frequency-chirped laser pulses is investigated theoretically. We demonstrate that intense beams of ions with a kinetic energy broadening of about 1 % can be generated. The chirping of the laser pulse allows the particles to gain kinetic energies of hundreds of MeVs, which is required for hadron cancer therapy, from pulses of energies of the order of 100 J. It is shown that few-cycle chirped pulses can accelerate ions more efficiently than long ones, i.e. higher ion kinetic energies are reached with the same amount of total electromagnetic pulse energy.

Heavy ions channeling through crystals with multi-GeV kinetic energies can create electron-positron pairs. In the framework of the ion, the energy of virtual photons arising from the periodic crystal potential may exceed the threshold $2mc^2$. The repeated periodic collisions with the crystal ions yield high pair production rates. When the virtual photon frequency matches a nuclear transition in the ion, the production rate can be resonantly increased. In this two-step excitation-pair conversion scheme, the excitation rates are coherently enhanced, and they scale approximately quadratically with the number of crystal sites along the channel.

The phenomenon of the parity violation due to weak interaction may be studied with superconducting systems. Previous research considered the case of conventional superconductors. We here theoretically investigate the parity violation effect in an unconventional $p$-wave ferromagnetic superconductor, and find that its magnitude can be increased by three orders of magnitude, as compared to results of earlier studies. For potential experimental observations, the superconductor UGe$_2$ is suggested, together with the description of a possible experimental scheme allowing one to effectively measure and control the phenomenon. Furthermore, we put forward a setup for a further significant enhancement of the signature of parity violation in the system considered.

Line intensities and oscillator strengths for the controversial 3C and 3D astrophysically relevant lines in neonlike Fe${}^{16+}$ ions are calculated. We show that, for strong x-ray sources, the modeling of the spectral lines by a peak with an area proportional to the oscillator strength is not sufficient and non-linear dynamical effects have to be taken into account. Furthermore, a large-scale configuration-interaction calculation of oscillator strengths is performed with the inclusion of higher-order electron-correlation effects. The dynamical effects give a possible resolution of discrepancies of theory and experiment found by recent measurements, which motivates the use of light-matter interaction models also valid for strong light fields in the analysis and interpretation of astrophysical and laboratory spectra., Comment: 5 pages, 3 figures

The quest for the value of the electron's atomic mass has been subject of continuing efforts over the last decades. Among the seemingly fundamental constants which parameterize the Standard Model (SM) of physics and which are thus responsible for its predictive power, the electron mass me plays a prominent role, as it is responsible for the structure and properties of atoms and molecules. This manifests in the close link with other fundamental constants, such as the Rydberg constant and the fine-structure constant {\alpha}. However, the low mass of the electron considerably complicates its precise determination. In this work we present a substantial improvement by combining a very accurate measurement of the magnetic moment of a single electron bound to a carbon nucleus with a state-of-the-art calculation in the framework of bound-state Quantum Electrodynamics. The achieved precision of the atomic mass of the electron surpasses the current CODATA value by a factor of 13. Accordingly, the result presented in this letter lays the foundation for future fundamental physics experiments and precision tests of the SM.

Optical frequency combs have had a remarkable impact on precision spectroscopy. Enabling this technology in the x-ray domain is expected to result in wide-ranging applications, such as stringent tests of astrophysical models and quantum electrodynamics, a more sensitive search for the variability of fundamental constants, and precision studies of nuclear structure. Ultraprecise x-ray atomic clocks may also be envisaged. In this work, an x-ray pulse-shaping method is put forward to generate a comb in the absorption spectrum of an ultrashort high-frequency pulse. The method employs an optical-frequency-comb laser, manipulating the system's dipole response to imprint a comb on an excited transition with a high photon energy. The described scheme provides higher comb frequencies and requires lower optical-comb peak intensities than currently explored methods, preserves the overall width of the optical comb, and may be implemented by presently available x-ray technology.

A general mechanism for the generation of frequency combs referenced to atomic resonances is put forward. The mechanism is based on the periodic phase control of a quantum system's dipole response. We develop an analytic description of the comb spectral structure, depending on both the atomic and the phase-control properties. We further suggest an experimental implementation of our scheme: Generating a frequency comb in the soft-x-ray spectral region, which can be realized with currently available techniques and radiation sources. The universality of this mechanism allows the generalization of frequency-comb technology to arbitrary frequencies, including the hard-x-ray regime by using reference transitions in highly charged ions.

Autoresonance laser acceleration of electrons is theoretically investigated using circularly polarized focused Gaussian pulses. Many-particle simulations demonstrate feasibility of creating over 10-GeV electron bunches of ultra-high quality (relative energy spread of order 10^-4), suitable for fundamental high-energy particle physics research. The laser peak intensities and axial magnetic field strengths required are up to about 10^18 W/cm^2 (peak power ~10 PW) and 60 T, respectively. Gains exceeding 100 GeV are shown to be possible when weakly focused pulses from a 200-PW laser facility are used.

An x-ray pulse-shaping scheme is put forward for imprinting an optical frequency comb onto the radiation emitted on a driven x-ray transition, thus producing an x-ray frequency comb. A four-level system is used to describe the level structure of N ions driven by narrow-bandwidth x rays, an optical auxiliary laser, and an optical frequency comb. By including many-particle enhancement of the emitted resonance fluorescence, a spectrum is predicted consisting of equally spaced narrow lines which are centered on an x-ray transition energy and separated by the same tooth spacing as the driving optical frequency comb. Given a known x-ray reference frequency, our comb could be employed to determine an unknown x-ray frequency. While relying on the quality of the light fields used to drive the ensemble of ions, the model has validity at energies from the 100 eV to the keV range., Comment: 11 pages, 2 figures

Interaction of a frequency-chirped laser pulse with single protons and a hydrogen plasma cell is studied analytically and by means of particle-in-cell simulations, respectively. Feasibility of generating ultra-intense (10^7 particles per bunch) and phase-space collimated beams of protons (energy spread of about 1 %) is demonstrated. Phase synchronization of the protons and the laser field, guaranteed by the appropriate chirping of the laser pulse, allows the particles to gain sufficient kinetic energy (around 250 MeV) required for such applications as hadron cancer therapy, from state-of-the-art laser systems of intensities of the order of 10^21 W/cm^2., Comment: 5 pages, 4 figures

During the past decade, the interaction of high-intensity lasers with solid targets has attracted much interest, regarding its potential in accelerating charged particles. In spite of tremendous progress in laser-plasma based acceleration, it is still not clear which particle beam quality will be accessible within the upcoming multi petawatt (1 PW = 10$^{15}$ W) laser generation. Here, we show with simulations based on the coupled relativistic equations of motion that protons stemming from laser-plasma processes can be efficiently post-accelerated using crossed laser beams focused to spot radii of a few laser wavelengths. We demonstrate that the crossed beams produce monoenergetic accelerated protons with kinetic energies $> 200$ MeV, small energy spreads ($\approx$ 1$%$) and high densities as required for hadron cancer therapy. To our knowledge, this is the first scheme allowing for this important application based on an all-optical set-up., Comment: 14 pages, 3 figures, 1 table