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We report on strong field ionization of S- and R-propylene oxide in circularly polarized two-color laser fields. We find that the relative helicity of the two single color laser fields affects the photoelectron circular dichroism (PECD). Further, we observe that PECD is modulated as a function of the sub-cycle release time of the electron. Our experimental observations are successfully described by a heuristic model based on electrons in chiral initial states, which are selectively liberated by the laser field and, after tunneling, interact with an achiral Coulomb potential.

We study strong field ionization of molecular hydrogen in highly intense co-rotating two-color (CoRTC) laser fields. The measured electron momentum distributions show alternating half-rings (AHR) that are characteristic for sub-cycle interference. We report on the role of the two-color field ratio for the visibility of this sub-cycle interference. The ratio of the peak electric field at 780 nm compared to the peak electric field at 390 nm $E_{780}/E_{390}$ is varied from 0.037 to 0.18. We find very good agreement with the results from our semiclassical simulation. We conclude that the AHR pattern is visible if two conditions are fulfilled. First, the amplitudes of the two pathways that lead to the sub-cycle interference have to be similar, which is the case for low two-color field ratios $E_{780}/E_{390}$. Second, the phase difference of the two pathways must be strong enough to allow for destructive interference, which is the case for high two-color field ratios $E_{780}/E_{390}$. For typical experimental conditions, we find that two-color field ratios $E_{780}/E_{390}$ in the range from 0.037 to 0.12 lead to good visibility of the AHR pattern. This guides future experiments to measure the Wigner time delay using holographic angular streaking of electrons (HASE)., Comment: 10 pages, 6 figures

We present experimental data on the strong-field ionization of the argon dimer in a co-rotating two-color (CoRTC) laser field. We observe a sub-cycle interference pattern in the photoelectron momentum distribution and infer the Wigner time delay using holographic angular streaking of electrons (HASE). We find that the Wigner time delay varies by more than 400 attoseconds as a function of the electron emission direction with respect to the molecular axis. The measured time delay is found to be independent of the parity of the dimer-cation and is in good agreement with our theoretical model based on the ionization of an aligned atomic p-orbital., Comment: 6 pages, 4 figures

We present experimental data on the strong field tunnel ionization of argon in a counter-rotating two-color (CRTC) laser field. We find that the initial momentum component along the tunneling direction changes sign comparing the rising and the falling edge of the CRTC field. If the initial momentum at the tunnel exit points in the direction of the ion at the instant of tunneling, this manifests as an enhanced Coulomb interaction of the outgoing electron with its parent ion. Our conclusions are in accordance with predictions based on strong field approximation., Comment: 6 pages, 4 figures

We report on a joint experimental and theoretical study of photoelectron circular dichroism (PECD) in methyloxirane. By detecting O 1s-photoelectrons in coincidence with fragment ions, we deduce the molecule's orientation and photoelectron emission direction in the laboratory frame. Thereby, we retrieve a fourfold differential PECD clearly beyond 50%. This strong chiral asymmetry is reproduced by ab initio electronic structure calculations. Providing such a pronounced contrast makes PECD of fixed-in-space chiral molecules an even more sensitive tool for chiral recognition in the gas phase., Comment: 5 figures

The photoelectron circular dichroism (PECD) of the O 1s-photoelectrons of trifluoromethyloxirane(TFMOx) is studied experimentally and theoretically for different photoelectron kinetic energies. The experiments were performed employing circularly polarized synchrotron radiation and coincidentelectron and fragment ion detection using Cold Target Recoil Ion Momentum Spectroscopy. The corresponding calculations were performed by means of the Single Center method within the relaxed-core Hartree-Fock approximation. We concentrate on the energy dependence of the differential PECD of uniaxially oriented TFMOx molecules, which is accessible through the employed coincident detection. We also compare results for differential PECD of TFMOx to those obtained for the equivalent fragmentation channel and similar photoelectron kinetic energy of methyloxirane (MOx), studied in our previous work. Thereby, we investigate the influence of the substitution of the methyl-group by the trifluoromethyl-group at the chiral center on the molecular chiral response. Finally, the presently obtained angular distribution parameters are compared to those available in literature., Comment: 6 figs

X-ray as well as electron diffraction are powerful tools for structure determination of molecules. Studies on randomly oriented molecules in the gas-phase address cases in which molecular crystals cannot be generated or the interaction-free molecular structure is to be addressed. Such studies usually yield partial geometrical information, such as interatomic distances. Here, we present a complementary approach, which allows obtaining insight to the structure, handedness and even detailed geometrical features of molecules in the gas phase. Our approach combines Coulomb explosion imaging, the information that is encoded in the molecular frame diffraction pattern of core-shell photoelectrons and ab initio computations. Using a loop-like analysis scheme we are able to deduce specific molecular coordinates with sensitivity even to the handedness of chiral molecules and the positions of individual atoms, as, e.g., protons., Comment: 13 pages, 3 figures

We investigate the differential ionization probability of chiral molecules in the strong field regime as a function of the helicity of the incident light. To this end, we analyze the fourfold ionization of bromochlorofluoromethane (CHBrClF) with subsequent fragmentation into four charged fragments and different dissociation channels of the singly ionized methyloxirane. We observe a variation of the differential ionization probability in a range of several percent. Accordingly, we conclude that the helicity of light is a quantity that should be considered for the theoretical description of the strong field ionization rate of chiral molecules., Comment: 12 pages, 6 figures, submitted

On 3 July 2016, several instruments on board ESA's Rosetta spacecraft detected signs of an outburst event on comet 67P, at a heliocentric distance of 3.32 AU from the sun, outbound from perihelion. We here report on the inferred properties of the ejected dust and the surface change at the site of the outburst. The activity coincided with the local sunrise and continued over a time interval of 14 - 68 minutes. It left a 10m-sized icy patch on the surface. The ejected material comprised refractory grains of several hundred microns in size, and sub-micron-sized water ice grains. The high dust mass production rate is incompatible with the free sublimation of crystalline water ice under solar illumination as the only acceleration process. Additional energy stored near the surface must have increased the gas density. We suggest a pressurized sub-surface gas reservoir, or the crystallization of amorphous water ice as possible causes., Comment: 20 pages, 19 figures, 5 tables

We collect observational evidence that supports the scheme of mass transfer on the nucleus of comet 67P/Churyumov-Gerasimenko. The obliquity of the rotation axis of 67P causes strong seasonal variations. During perihelion the southern hemisphere is four times more active than the north. Northern territories are widely covered by granular material that indicates back fall originating from the active south. Decimetre sized chunks contain water ice and their trajectories are influenced by an anti-solar force instigated by sublimation. OSIRIS observations suggest that up to 20 % of the particles directly return to the nucleus surface taking several hours of travel time. The back fall covered northern areas are active if illuminated but produce mainly water vapour. The decimetre chunks from the nucleus surface are too small to contain more volatile compounds such as CO 2 or CO. This causes a north-south dichotomy of the composition measurements in the coma. Active particles are trapped in the gravitational minimum of Hapi during northern winter. They are "shock frozen" and only reactivated when the comet approaches the sun after its aphelion passage. The insolation of the big cavity is enhanced by self-heating, i. e. reflection and IR radiation from the walls. This, together with the pristinity of the active back fall, explains the early observed activity of the Hapi region. Sobek may be a role model for the consolidated bottom of Hapi. Mass transfer in the case of 67P strongly influences the evolution of the nucleus and the interpretation of coma measurements., Comment: 17 pages, 20 figures

The Southern hemisphere of the 67P/Churyumov-Gerasimenko comet has become visible from Rosetta only since March 2015. It was illuminated during the perihelion passage and therefore it contains the regions that experienced the strongest heating and erosion rate, thus exposing the subsurface most pristine material. In this work we investigate, thanks to the OSIRIS images, the geomorphology, the spectrophotometry and some transient events of two Southern hemisphere regions: Anhur and part of Bes. Bes is dominated by outcropping consolidated terrain covered with fine particle deposits, while Anhur appears strongly eroded with elongated canyon-like structures, scarp retreats, different kinds of deposits, and degraded sequences of strata indicating a pervasive layering. We discovered a new 140 m long and 10 m high scarp formed in the Anhur/Bes boundary during/after the perihelion passage, close to the area where exposed CO$_2$ and H$_2$O ices were previously detected. Several jets have been observed originating from these regions, including the strong perihelion outburst, an active pit, and a faint optically thick dust plume. We identify several areas with a relatively bluer slope (i.e. a lower spectral slope value) than their surroundings, indicating a surface composition enriched with some water ice. These spectrally bluer areas are observed especially in talus and gravitational accumulation deposits where freshly exposed material had fallen from nearby scarps and cliffs. The investigated regions become spectrally redder beyond 2 au outbound when the dust mantle became thicker, masking the underlying ice-rich layers., Comment: 16 pages, 15 figures, published online on 24 May 2017 on Mon. Not. R. Astron. Soc. stx1275, https://doi.org/10.1093/mnras/stx1275

We present a statistical analysis of the distribution of large scale topographic features on comet 67P/Churyumov-Gerasimenko. We observe that the cumulative cliff height distribution across the surface follows a power law with a slope equal to -1.69 +- 0.02. When this distribution is studied independently for each region, we find a good correlation between the slope of the power law and the orbital erosion rate of the surface. For instance, the northern hemisphere topography is dominated by structures on the 100~m scale while the southern hemisphere topography, illuminated at perihelion, is dominated by 10~m scale terrain features. Our study suggest that the current size of a cliff is controlled not only by material cohesion but by the dominant erosional process in each region. This observation can be generalized to other comets, where we argue that primitive nuclei are characterized by the presence of large cliffs with a cumulative height power index equal to or above -1.5, while older, eroded cometary surfaces have a power index equal to or below -2.3. In effect, our model shows that a measure of the topography provides a quantitative assessment of a comet's erosional history, i.e. its evolutionary age.

Images of the nucleus and the coma (gas and dust) of comet 67P/Churyumov- Gerasimenko have been acquired by the OSIRIS (Optical, Spectroscopic, and Infrared Remote Imaging System) cameras since March 2014 using both the Wide Angle Camera (WAC) and the Narrow Angle Camera (NAC). We use images from the NAC camera to study a bright outburst observed in the southern hemisphere on July 29, 2015. The high spatial resolution of the NAC is needed to localize the source point of the outburst on the surface of the nucleus. The heliocentric distance is 1.25 au and the spacecraft-comet distance is 186 km. Aiming to better understand the physics that led to the outgassing, we used the Direct Simulation Monte Carlo (DSMC) method to study the gas flow close to the nucleus and the dust trajectories. The goal is to understand the mechanisms producing the outburst. We reproduce the opening angle of the outburst in the model and constrain the outgassing ratio between the outburst source and the local region. The outburst is in fact a combination of both gas and dust, in which the active surface is approximately 10 times more active than the average rate found in the surrounding areas. We need a number of dust particles 7.83 $\times$ 10$^{11}$ - 6.90 $\times$ 10$^{15}$ (radius 1.97 - 185 {\mu}m), which corresponds to a mass of dust 220 - 21 $\times$ 10$^{3}$kg., Comment: 8 pages, 9 figures

The ESA Rosetta spacecraft has been tracking its target, the Jupiter-family comet 67P/Churyumov-Gerasimenko, in close vicinity for over two years. It hosts the OSIRIS instruments: the Optical, Spectroscopic, and Infrared Remote Imaging System composed of two cameras, see e.g. Keller et al. (2007). In some imaging sequences dedicated to observe dust particles in the comet's coma, the two cameras took images at the same time. The aim of this work is to use these simultaneous double camera observations to calculate the dust particles' distance to the spacecraft. As the two cameras are mounted on the spacecraft with an offset of 70 cm, the distance of particles observed by both cameras can be determined by a shift of the particles' apparent trails on the images. This paper presents first results of the ongoing work, introducing the distance determination method for the OSIRIS instrument and the analysis of an example particle. We note that this method works for particles in the range of about 500 m - 6000 m from the spacecraft.

We present the results of the photometric and spectrophotometric properties of the 67P/Churyumov-Gerasimenko nucleus derived with the OSIRIS instrument during the closest fly-by over the comet, which took place on 14 th February 2015 at a distance of {\~} 6 km from the surface. Several images covering the 0{\deg}-33{\deg} phase angle range were acquired, and the spatial resolution achieved was 11 cm/pxl. The flown-by region is located on the big lobe of the comet, near the borders of the Ash, Apis and Imhotep regions. Our analysis shows that this region features local heterogeneities at the decimetre scale. We observed difference of reflectance up to 40{\%} between bright spots and sombre regions, and spectral slope variations up to 50{\%}. The spectral reddening effect observed globally on the comet surface by Fornasier et al. (2015) is also observed locally on this region, but with a less steep behaviour. We note that numerous metre-sized boulders, which exhibit a smaller opposition effect, also appear spectrally redder than their surroundings. In this region, we found no evidence linking observed bright spots to exposed water-ice-rich material. We fitted our dataset using the Hapke 2008 photometric model. The region overflown is globally as dark as the whole nucleus (geometric albedo of 6.8{\%}) and it has a high porosity value in the uppermost-layers (86{\%}). These results of the photometric analysis at a decimetre scale indicate that the photometric properties of the flown-by region are similar to those previously found for the whole nucleus., Comment: 19 pages, 16 figures, 5 tables, (also presented at DPS48/ESPC11: http://cdsads.u-strasbg.fr/abs/2016DPS....4830004F)

During its two years mission around comet 67P/Churyumov-Gerasimenko, ESA's Rosetta spacecraft had the unique opportunity to follow closely a comet in the most active part of its orbit. Many studies have presented the typical features associated to the activity of the nucleus, such as localized dust and gas jets. Here we report on series of more energetic transient events observed during the three months surrounding the comet's perihelion passage in August 2015. We detected and characterized 34 outbursts with the Rosetta cameras, one every 2.4 nucleus rotation. We identified 3 main dust plume morphologies associated to these events: a narrow jet, a broad fan, and more complex plumes featuring both previous types together. These plumes are comparable in scale and temporal variation to what has been observed on other comets. We present a map of the outbursts source locations, and discuss the associated topography. We find that the spatial distribution sources on the nucleus correlates well with morphological region boundaries, especially in areas marked by steep scarps or cliffs. Outbursts occur either in the early morning or shortly after the local noon, indicating two potential processes: Morning outbursts may be triggered by thermal stresses linked to the rapid change of temperature, afternoon events are most likely related to the diurnal or seasonal heat wave reaching volatiles buried under the first surface layer. In addition, we propose that some events can be the result of a completely different mechanism, in which most of the dust is released upon the collapse of a cliff., Comment: MNRAS (2016)

Beginning in March 2014, the OSIRIS (Optical, Spectroscopic, and Infrared Remote Imaging System) cameras began capturing images of the nucleus and coma (gas and dust) of comet 67P/Churyumov-Gerasimenko using both the wide angle camera (WAC) and the narrow angle camera (NAC). The many observations taken since July of 2014 have been used to study the morphology, location, and temporal variation of the comet's dust jets. We analyzed the dust monitoring observations shortly after the southern vernal equinox on May 30 and 31, 2015 with the WAC at the heliocentric distance Rh = 1.53 AU, where it is possible to observe that the jet rotates with the nucleus. We found that the decline of brightness as a function of the distance of the jet is much steeper than the background coma, which is a first indication of sublimation. We adapted a model of sublimation of icy aggregates and studied the effect as a function of the physical properties of the aggregates (composition and size). The major finding of this article was that through the sublimation of the aggregates of dirty grains (radius a between 5 microm and 50 microm) we were able to completely reproduce the radial brightness profile of a jet beyond 4 km from the nucleus. To reproduce the data we needed to inject a number of aggregates between 8.5 x $10^{13}$ and 8.5 x $10^{10}$ for a = 5 microm and 50 microm respectively, or an initial mass of $H_2O$ ice around 22kg., Comment: 11 pages, 7 figures, 3 tables, special issue "The ESLAB 50 Symposium - spacecraft at comets from 1P/Halley to 67P/Churyumov-Gerasimenko" in the Monthly Notices of the Royal Astronomical Society

We present OSIRIS/NAC observations of decimetre-sized, likely ice-containing aggregates ejected from a confined region on the surface of comet 67P/Churyumov-Gerasimenko. The images were obtained in January 2016 when the comet was at 2 AU from the Sun out-bound from perihelion. We measure the acceleration of individual aggregates through a two-hour image series. Approximately 50% of the aggregates are accelerated away from the nucleus, and 50% towards it, and likewise towards either horizontal direction. The accelerations are up to one order of magnitude stronger than local gravity, and are most simply explained by the combined effect of gas drag accelerating all aggregates upwards, and the recoil force from asymmetric outgassing, either from rotating aggregates with randomly oriented spin axes and sufficient thermal inertia to shift the temperature maximum away from an aggregate's subsolar region, or from aggregates with variable ice content. At least 10% of the aggregates will escape the gravity field of the nucleus and feed the comet's debris trail, while others may fall back to the surface and contribute to the deposits covering parts of the northern hemisphere. The rocket force plays a crucial role in pushing these aggregates back towards the surface. Our observations show the future back fall material in the process of ejection, and provide the first direct measurement of the acceleration of aggregates in the innermost coma (<2km) of a comet, where gas drag is still significant., Comment: 11 pages, 14 figures, accepted for publication in MNRAS

During the commissioning of the first of the two detectors of the Double Chooz experiment, an unexpected and dominant background caused by the emission of light inside the optical volume has been observed. A specific study of the ensemble of phenomena called "Light Noise" has been carried out in-situ, and in an external laboratory, in order to characterize the signals and to identify the possible processes underlying the effect. Some mechanisms of instrumental noise originating from the PMTs were identified and it has been found that the leading one arises from the light emission localized on the photomultiplier base and produced by the combined effect of heat and high voltage across the transparent epoxy resin covering the electric components. The correlation of the rate and the amplitude of the signal with the temperature has been observed. For the first detector in operation the induced background has been mitigated using online and offline analysis selections based on timing and light pattern of the signals, while a modification of the photomultiplier assembly has been implemented for the second detector in order to blacken the PMT bases., Comment: 24 pages, 24 figures. Minor revision to be published in the Journal of Instrumentation (JINST), Corresponding author: R. Santorelli

Using the Double Chooz detector, designed to measure the neutrino mixing angle $\theta_{13}$, the products of $\mu^-$ capture on $^{12}$C, $^{13}$C, $^{14}$N and $^{16}$O have been measured. Over a period of 489.5 days, $2.3\times10^6$ stopping cosmic $\mu^-$ have been collected, of which $1.8\times10^5$ captured on carbon, nitrogen, or oxygen nuclei in the inner detector scintillator or acrylic vessels. The resulting isotopes were tagged using prompt neutron emission (when applicable), the subsequent beta decays, and, in some cases, $\beta$-delayed neutrons. The most precise measurement of the rate of $^{12}\mathrm C(\mu^-,\nu)^{12}\mathrm B$ to date is reported: $6.57^{+0.11}_{-0.21}\times10^{3}\,\mathrm s^{-1}$, or $(17.35^{+0.35}_{-0.59})\%$ of nuclear captures. By tagging excited states emitting gammas, the ground state transition rate to $^{12}$B has been determined to be $5.68^{+0.14}_{-0.23}\times10^3\,\mathrm s^{-1}$. The heretofore unobserved reactions $^{12}\mathrm C(\mu^-,\nu\alpha)^{8}\mathrm{Li}$, $^{13}\mathrm C(\mu^-,\nu\mathrm n\alpha)^{8}\mathrm{Li}$, and $^{13}\mathrm C(\mu^-,\nu\mathrm n)^{12}\mathrm B$ are measured. Further, a population of $\beta$n decays following stopping muons is identified with $5.5\sigma$ significance. Statistics limit our ability to identify these decays definitively. Assuming negligible production of $^{8}$He, the reaction $^{13}\mathrm C(\mu^-,\nu\alpha)^{9}\mathrm{Li}$ is found to be present at the $2.7\sigma$ level. Limits are set on a variety of other processes., Comment: 21 pages, 14 figures. Minor revisions. Corresponding author: M. Strait

Dust jets, i.e. fuzzy collimated streams of cometary material arising from the nucleus, have been observed in-situ on all comets since the Giotto mission flew by comet 1P/Halley in 1986. Yet their formation mechanism remains unknown. Several solutions have been proposed, from localized physical mechanisms on the surface/sub-surface (see review in Belton (2010)) to purely dynamical processes involving the focusing of gas flows by the local topography (Crifo et al. 2002). While the latter seems to be responsible for the larger features, high resolution imagery has shown that broad streams are composed of many smaller features (a few meters wide) that connect directly to the nucleus surface. We monitored these jets at high resolution and over several months to understand what are the physical processes driving their formation, and how this affects the surface. Using many images of the same areas with different viewing angles, we performed a 3-dimensional reconstruction of collimated jets, and linked them precisely to their sources on the nucleus. Results.We show here observational evidence that the Northern hemisphere jets of comet 67P arise from areas with sharp topographic changes and describe the physical processes involved. We propose a model in which active cliffs are the main source of jet-like features, and therefore the regions eroding the fastest on comets. We suggest that this is a common mechanism taking place on all comets., Comment: Accepted by Astronomy & Astrophysics on 4 December 2015

The attenuation of vacuum ultraviolet light in liquid argon in the context of its application in large liquid noble gas detectors has been studied. Compared to a previous publication several technical issues concerning transmission measurements in general are addressed and several systematic effects were quantitatively measured. Wavelength-resolved transmission measurements have been performed from the vacuum ultraviolet to the near-infrared region. On the current level of sensitivity with a length of the optical path of 11.6 cm, no xenon-related absorption effects could be observed, and pure liquid argon is fully transparent down to the short wavelength cut-off of the experimental setup at 118 nm. A lower limit for the attenuation length of pure liquid argon for its own scintillation light has been estimated to be 1.10 m based on a very conservative approach., Comment: 14 pages, 22 figures