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Photo-induced reaction cross section data are of importance for a variety of current or emerging applications, such as radiation shielding design and radiation transport analyses, calculations of absorbed dose in the human body during radiotherapy, physics and technology of fission reactors (influence of photo-reactions on neutron balance) and fusion reactors (plasma diagnostics and shielding), activation analyses, safeguards and inspection technologies, nuclear waste transmutation, medical isotope production and astrophysical applications. To address these data needs the IAEA Photonuclear Data library was produced in 1999, containing evaluated photo-induced cross sections and neutron spectra for 164 nuclides which were deemed relevant for the applications. Since the release of the IAEA Photonuclear Data Library however, new experimental data as well as new methods to assess the reliability of experimental cross sections have become available. Theoretical models and input parameters used to evaluate photo-induced reactions have improved significantly over the years. In addition, new measurements of partial photoneutron cross sections using mono-energetic photon beams and advanced neutron detection systems have been performed allowing for the validation of the evaluations and assessments of the experimental data. Furthermore, technological advances have led to the construction of new and more powerful gamma-beam facilities, therefore new data needs are emerging. We report our coordinated efforts to address these data needs and present the results of the new up-to-date evaluations included in the new updated IAEA Photonuclear Data Library consisting of 219 nuclides. The new library includes 188 new evaluations produced by the CRP evaluators, and one evaluation taken from the JENDL/PD-2016 library, while 20 evaluations were retained from the previous 1999 IAEA Photonuclear Data Library. In most of the cases, the photon energy goes up to 200 MeV. A total of 55 nuclides are new in this library reflecting the progress in measurements but also the developing data needs. In this paper we discuss the new assessment method and make recommendations to the user community in cases where the experimental data are discrepant and the assessments disagree. In addition, in the absence of experimental data, we present model predictions for photo-induced reaction cross section on nuclides of potential interest to medical radioisotope production.

The validity of the Brink-Axel hypothesis, which is especially important for numerous astrophysical calculations, is addressed for 116,120,124Sn below the neutron separation energy by means of three independent experimental methods. The $\gamma$-ray strength functions (GSFs) extracted from primary $\gamma$-decay spectra following charged-particle reactions with the Oslo method and with the Shape method demonstrate excellent agreement with those deduced from forward-angle inelastic proton scattering at relativistic beam energies. In addition, the GSFs are shown to be independent of excitation energies and spins of the initial and final states. The results provide a critical test of the generalized Brink-Axel hypothesis in heavy nuclei, demonstrating its applicability in the energy region of the pygmy dipole resonance., Comment: 6 pages, 4 figures, Phys. Rev. Lett. (in press)

6 pags., 4 figs., 1 tab.-- Open Access funded by Creative Commons Atribution Licence 4.0, Inclusive one- and multi-nucleon removal cross sections have been measured for several Sn, Sb and Te isotopes just beyond the N=82 neutron shell closure. The beams were produced in the projectile fission of a U beam at the Radioactive Isotope Beam Factory at RIKEN. The experimental cross sections are compared to predictions from the most recent version of the Liege intranuclear cascade model. Although the overall agreement is good, severe discrepancies are observed for the cases of one- and two-neutron removal from Sn and Sb projectiles and one-proton knockout from all measured N=84 isotones. These discrepancies, as well as the relevance of quasi-elastic reaction channels to the one-neutron removal cross sections, are discussed. In addition, the measured inclusive one-proton knockout cross section for the semi-magic Sn projectile is compared to eikonal direct reaction theory calculations to assess if the suppression factors to these calculated cross sections, deduced from data on reactions of lighter projectile nuclei, are also applicable to heavy nuclei., We thank the staff of the RIKEN Nishina Center accelerator complex for providing high-intensity beams to the experiment. This work was supported by the Spanish Ministerio de Economía y Competitividad under contracts FPA2014-57196-C5-4-P and FPA2017-84756-C4-2-P. J.A.T. acknowledges the support of the Science and Technology Facilities Council (UK) grant ST/L005314/1 and R.O. that of JSPS KAKENHI Grant No. 26887048. G.M.T. grate-fully acknowledges funding of this research from the Research Council of Norway, Project Grant No. 222287.

Recent measurements of the nuclear level densities and γ-ray strength functions below the neutron thresholds in 180,181,182Ta are used as input in the nuclear reaction code TALYS. These experimental average quantities are utilized in the calculations of the 179,180,181Ta radiative neutron capture cross sections. From the latter, astrophysical Maxwellian-averaged (n,γ) cross sections (MACS) and reaction rates are extracted, which in turn are used in large astrophysical network calculations to probe the production mechanism of 180 Ta. These calculations are performed for two scenarios, the s-process production of 180,181Ta in Asymptotic Giant Branch (AGB) stars and the p-process nucleosynthesis of 180Tam in Type-II supernovae. Based on the results from this work, the s-process in stellar evolution is considered negligible in the production of 180Tam whereas 181Ta is partially produced by AGB stars. The new measurements strongly constrain the production and destruction rates of 180Tam at p-process temperatures and confirm significant production of nature’s rarest stable isotope 180Tam by the p-process., SCOPUS: ar.j, info:eu-repo/semantics/published

Prompt fission $\ensuremath{\gamma}$ rays (PFGs) resulting from the $^{240}\mathrm{Pu}(d,p\mathrm{f})$ reaction have been measured as a function of fissioning nucleus excitation energy ${E}_{\text{x}}$ at the Oslo Cyclotron Laboratory. We study the average total PFG multiplicity per fission, the average total PFG energy released per fission, and the average PFG energy. No significant changes in these characteristics are observed over the range $5.75l{E}_{\text{x}}l8.25$ MeV. The physical implications of this result are discussed. The experimental results are compared to simulations conducted using the computational fission model FREYA. We find that FREYA reproduces the experimental PFG characteristics within $8%$ deviation across the ${E}_{\text{x}}$ range studied. Previous excitation energy-dependent PFG measurements conducted below the second-chance fission threshold have large uncertainties, but are generally in agreement with our results within a $2\ensuremath{\sigma}$ confidence interval. However, both a published parametrization of the PFG energy dependence and the most recent PFG evaluation included in ENDF/B-VIII.0 were found to poorly describe the PFG excitation-energy dependence observed in this and previous experiments.

The nuclear level densities (NLDs) and the $\ensuremath{\gamma}$-ray strength functions ($\ensuremath{\gamma}\mathrm{SFs}$) of $^{153,155}\mathrm{Sm}$ have been extracted from ($d,p\ensuremath{\gamma}$) coincidences using the Oslo method. The experimental NLD of $^{153}\mathrm{Sm}$ is higher than the NLD of $^{155}\mathrm{Sm}$, in accordance with microscopic calculations. The $\ensuremath{\gamma}\mathrm{SFs}$ of $^{153,155}\mathrm{Sm}$ are in fair agreement with QRPA calculations based on the D1M Gogny interaction. An enhancement is observed in the $\ensuremath{\gamma}\mathrm{SF}$ for both $^{153,155}\mathrm{Sm}$ nuclei around 3 MeV in excitation energy and is attributed to the $M1$ scissors resonance (SR). Their integrated strengths were found to be in the range 1.3--2.1 and 4.4--6.4 ${\ensuremath{\mu}}_{N}^{2}$ for $^{153}\mathrm{Sm}$ and $^{155}\mathrm{Sm}$, respectively. The strength of the SR for $^{155}\mathrm{Sm}$ is comparable to those for deformed even-even Sm isotopes from nuclear resonance fluorescence measurements, while that of $^{153}\mathrm{Sm}$ is lower than expected.

Understanding the evolution of level densities in the crossover from spherical to well-deformed nuclei has been a long-standing problem in nuclear physics. We measure nuclear level densities for a chain of neodymium isotopes $^{142,144-151}$Nd which exhibit such a crossover. These results represent to date the most complete data set of nuclear level densities for an isotopic chain between neutron shell-closure and towards mid-shell. We observe a strong increase of the level densities along the chain with an overall increase by a factor of $\approx 170$ at an excitation energy of 7.5 MeV and saturation around mass 150. Level densities calculated by the shell model Monte Carlo (SMMC) are in excellent agreement with these experimental results. Based on our experimental and theoretical findings, we offer an explanation of the observed mass dependence of the level densities in terms of the intrinsic single-particle level density and the collective enhancement., 7 pages, 4 figures

We present the latest development of measuring (γ, n) cross sections and giant dipole resonance (GDR) cross sections in the IAEA photonuclear data project. Photoneutron cross sections were measured for 21 isotopes below 2n threshold to construct the γ-ray strength function (γSF) with the γSF method; (γ, n) cross sections are used as experimental constraints on the model E1 and M1 γSFs from the Hartree–Fock–Bogolyubov plus quasi-particle random phase approximation based on the Gogny D1M interaction supplemented with the M1 upbend. GDR cross sections were measured for 11 nuclei from 9Be to 209Bi by direct neutron-multiplicity sorting with a flat-efficiency neutron detector toward a goal of resolving the long-standing discrepancy between the Livermore and Saclay data. We present γSFs for the Ni isotopic chain and GDR cross sections for 159Tb as well as those updated for 209Bi.

In this paper we present the first systematic analysis of the impact of the populated vs. intrinsic spin distribution on the nuclear level density and γ-ray strength function retrieved through the Oslo Method. We illustrate the effect of the spin distribution on the recently performed 239Pu(d,pγ)240Pu experiment using a 12 MeV deuteron beam performed at the Oslo Cyclotron Lab. In the analysis we couple state-of-the-art calculations for the populated spin-distributions with the Monte-Carlo nuclear decay code RAINIER to compare Oslo Method results to the known input. We find that good knowledge of the populated spin distribution is crucial and show that the populated distribution has a significant impact on the extracted nuclear level density and γ-ray strength function for the 239Pu(d,pγ)240Pu case.

Background: Reaction rates of radiative capture reactions can play a crucial role in the nucleosynthesis of heavy nuclei in explosive stellar environments. These reaction rates depend strongly on $\ensuremath{\gamma}$-ray decay widths in the reaction products, which are, for nonresonant capture reactions at high excitation energies, derived from the $\ensuremath{\gamma}$-ray strength function and the nuclear level density. Recently, the ratio method was applied to primary $\ensuremath{\gamma}$ rays observed from ($d,p$) reactions and nuclear resonance fluorescence measurements to extract the dipole strength in atomic nuclei and to test the generalized Brink-Axel hypothesis.Purpose: The purpose of this work is to apply the ratio method to primary $\ensuremath{\gamma}$-ray intensities of the $^{63,65}\mathrm{Cu}(p,\ensuremath{\gamma})$ reactions to extract $\ensuremath{\gamma}$-ray strength information on the nuclei $^{64,66}\mathrm{Zn}$. The impact of spin distribution, total $\ensuremath{\gamma}$-ray decay widths, level densities, and width fluctuations on the application of the ratio method will be discussed. Additionally, by comparing the relative $\ensuremath{\gamma}$-ray strength at different excitation energies, conclusions on the validity of the generalized Brink-Axel hypothesis can be made.Method: The radiative proton capture reaction measurements have been performed at the HORUS $\ensuremath{\gamma}$-ray spectrometer of the University of Cologne at one excitation energy for each reaction. Primary $\ensuremath{\gamma}$-ray intensities have been determined by normalizing secondary $\ensuremath{\gamma}$-ray transitions in two-step cascades using their absolute branching ratio. The ratio method was applied to the measured primary $\ensuremath{\gamma}$-ray intensities as well as to previous measurements by Erlandsson $et$ $al.$ at different excitation energies.Results: The relative strength function curve for $^{64}\mathrm{Zn}$ from our measurement shows no significant deviation from the previous measurement at a different excitation energy. The same is true for $^{66}\mathrm{Zn}$ where both measurements were at almost the same excitation energy. Absolute $\ensuremath{\gamma}$-strength function values have been obtained by normalizing the relative curves to quasiparticle random phase approximation calculations because of the absence of experimental data in the respective energy region.Conclusion: The generalized Brink-Axel hypothesis, i.e., the independence of the strength function on the excitation energy, seems to hold in the studied energy region and nuclei. The method to obtain primary $\ensuremath{\gamma}$-ray intensities from two-step cascade spectra was shown to be a valuable and sensitive tool although its uncertainties are connected to the knowledge of the low-energy level scheme of the investigated nucleus. The scaling in the ratio method should be taken with care, because the relative strength is not a simple sum of ${f}_{E1}$ and ${f}_{M1}$ but a somewhat complex linear combination dependent on the excitation energy of the nucleus.

The γ-ray strength function (γSF) is a nuclear quantity that governs photoabsorption in (γ, n) and photoemission in (n, γ) reactions. Within the framework of the γ-ray strength function method, we use (γ, n) cross sections as experimental constraints on the γSF from the Hartree-Fock-Bogolyubov plus quasiparticle-random phase approximation based on the Gogny D1M interaction for E1 and M1 components. The experimentally constrained γSF is further supplemented with the zero-limit M1 and E1 strengths to construct the downward γSF with which (n, γ) cross sections are calculated. We investigate (n, γ) cross sections in the context of astrophysical applications over the nickel and barium isotopic chains along the s-process path.

The new Oslo Scintillator Array (OSCAR) has been commissioned at the Oslo Cyclotron Laboratory (OCL). It consists of 30 large volume (diameter 3.5 x 8 inches) LaBr$_3$(Ce) detectors that are used for $\gamma$-ray spectroscopy. The response functions for incident $\gamma$-rays up to 20 MeV are simulated with $\texttt{Geant4}$. In addition, the resolution, and the total and full-energy peak efficiencies are extracted. The results are in very good agreement with measurements from calibration sources and experimentally obtained mono-energetic in-beam $\gamma$-ray spectra., Comment: Changes to v2 (submitted version): Accepted for NIMA with minor revisions (implemented); Changes to v1: see v2 - major changes in experimental setup and simulations [stalled version]

The cascading 3.21 and 4.44 MeV electric quadrupole transitions have been observed from the Hoyle state at 7.65 MeV excitation energy in $^{12}\mathrm{C}$, excited by the $^{12}\mathrm{C}(p,{p}^{\ensuremath{'}})$ reaction at 10.7 MeV proton energy. From the proton-$\ensuremath{\gamma}\text{\ensuremath{-}}\ensuremath{\gamma}$ triple coincidence data, a value of ${\mathrm{\ensuremath{\Gamma}}}_{\mathrm{rad}}/\mathrm{\ensuremath{\Gamma}}=6.2(6)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}4}$ was obtained for the radiative branching ratio. Using our results, together with ${\mathrm{\ensuremath{\Gamma}}}_{\ensuremath{\pi}}^{E0}/\mathrm{\ensuremath{\Gamma}}$ from Eriksen et al. [Phys. Rev. C 102, 024320 (2020)] and the currently adopted ${\mathrm{\ensuremath{\Gamma}}}_{\ensuremath{\pi}}(E0)$ values, the radiative width of the Hoyle state is determined as ${\mathrm{\ensuremath{\Gamma}}}_{\mathrm{rad}}=5.1(6)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}3}\text{ }\text{ }\mathrm{eV}$. This value is about 34% higher than the currently adopted value and will impact models of stellar evolution and nucleosynthesis.

Photoneutron cross sections were measured for $^{137}$Ba and $^{138}$Ba at energies below two-neutron threshold using quasi-monochromatic $\gamma$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. The photoneutron data are used to constrain the $\gamma$-ray strength function on the basis of the Hartree-Fock-Bogolyubov plus quasi-particle random phase approximation using the Gogny D1M interaction. Supplementing the experimentally constrained $\gamma$-ray strength function with the zero-limit E1 and M1 contributions which are unique to the deexcitation mode, we discuss radiative neutron capture cross sections relevant to the s-process nucleosynthesis of barium isotopes in the vicinity of the neutron magic number 82., Comment: arXiv admin note: substantial text overlap with arXiv:1811.00291, arXiv:1804.07654

The Oslo method has been applied to particle-$\ensuremath{\gamma}$ coincidences following the $^{239}\mathrm{Pu}(d,p)$ reaction to obtain the nuclear level density (NLD) and $\ensuremath{\gamma}$-ray strength function ($\ensuremath{\gamma}\mathrm{SF}$) of $^{240}\mathrm{Pu}$. The experiment was conducted with a 12 MeV deuteron beam at the Oslo Cyclotron Laboratory. The low spin transfer of this reaction leads to a spin-parity mismatch between populated and intrinsic levels. This is a challenge for the Oslo method as it can have a significant impact on the extracted NLD and $\ensuremath{\gamma}\mathrm{SF}$. We have developed an iterative approach to ensure consistent results even for cases with a large spin-parity mismatch, in which we couple Green's function transfer calculations of the spin-parity dependent population cross-section to the nuclear decay code rainier. The resulting $\ensuremath{\gamma}\mathrm{SF}$ shows a pronounced enhancement between 2--4 MeV that is consistent with the location of the low-energy orbital $M1$ scissors mode.

The nuclear level density and $\ensuremath{\gamma}$-decay strength of $^{192}\mathrm{Os}$ have been extracted using particle-$\ensuremath{\gamma}$ coincidence data from the $^{192}\mathrm{Os}(\ensuremath{\alpha},{\ensuremath{\alpha}}^{\ensuremath{'}}\ensuremath{\gamma})^{192}\mathrm{Os}$ reaction by means of the Oslo method. The level density is found to be a rather smooth function of excitation energy, approximately following the constant temperature model. The $\ensuremath{\gamma}$-decay strength is compared to photoneutron cross-section data above the neutron separation energy, and to $E1$ and $M1$ strengths for nuclei in this mass region derived from primary transitions following neutron capture. Our results are in good agreement with these previous data and draw a consistent picture of the $\ensuremath{\gamma}$-strength function in the range ${E}_{\ensuremath{\gamma}}\ensuremath{\approx}1.5--6\phantom{\rule{0.28em}{0ex}}\mathrm{MeV}$. Using the measured nuclear level density and $\ensuremath{\gamma}$-decay strength as input to the nuclear-reaction code talys, we provide the first experimentally constrained Maxwellian-averaged cross section (MACS) for the $^{191}\mathrm{Os}(n,\ensuremath{\gamma})^{192}\mathrm{Os}$ reaction relevant to $s$-process nucleosynthesis. The systematic uncertainties introduced by the normalization procedure of the level density and $\ensuremath{\gamma}$-strength function were investigated and propagated to the calculated Maxwellian-averaged cross section. The obtained result of the Maxwellian-averaged cross section at ${k}_{B}T=30\phantom{\rule{0.28em}{0ex}}\mathrm{keV}$, ${\ensuremath{\langle}\ensuremath{\sigma}\ensuremath{\rangle}}_{n,\ensuremath{\gamma}}=1134\ifmmode\pm\else\textpm\fi{}375\phantom{\rule{0.28em}{0ex}}\mathrm{mb}$, is in very good agreement with the theoretical estimate provided by the KADoNiS project, giving experimental support to the adopted KADoNiS value. Good agreement is also found with MACS values obtained from other libraries, such as TENDL-2017, ENDF/B-VII.0, and JEFF.

CITATION: Brits, C. P., et al. 2019. Nuclear level densities and γ-ray strength functions of 180,181,182Ta. Physical Review C, 99(5):054330, doi:10.1103/PhysRevC.99.054330.

The Oslo method comprises a set of analysis techniques designed to extract nuclear level density and average $\gamma$-decay strength function from a set of excitation-energy tagged $\gamma$-ray spectra. Here we present a new software implementation of the entire Oslo method, called OMpy. We provide a summary of the theoretical basis and derive the essential equations used in the Oslo method. In addition to the functionality of the original analysis code, the new implementation includes novel components such as a rigorous method to propagate uncertainties throughout all steps of the Oslo method using a Monte Carlo approach. The resulting level density and $\gamma$-ray strength function have to be normalized to auxiliary data. The normalization is performed simultaneously for both quantities, thus preserving all correlations. The software is verified by the analysis of a synthetic spectrum and compared to the results of the previous implementation, the oslo-method-software., Comment: 20 pages, 6 figures. Updated v5: Eq. (C.6); v4: Major revision of App. C

The reduced transition probability B(E2;01+→21+) to the first excited 2+ state of the neutron-rich nucleus Te136, with two protons and two neutrons outside the doubly magic Sn132 core, was measured via Coulomb excitation at relativistic energies at the RIKEN Radioactive Isotope Beam Factory. A value of B(E2)=0.191(26) e2b2 was extracted from the measured inelastic scattering cross section on an Au target taking into account the contributions from both Coulomb and nuclear excitations. In addition, an upper limit for the transition strength to a 2+ state of mixed-symmetry character in the excitation energy range of 1.5-2.2 MeV was determined and compared to the predictions of various theoretical calculations. Because of the high statistics gathered in the present experiment the error of the deduced B(E2) value is dominated by the systematic uncertainties involved in the analysis of Coulomb excitation experiments at beam energies around 150 MeV/u. Therefore, the latter are for the first time assessed in detail in the present work.

Photoneutron cross sections were measured for $^{203}\mathrm{Tl}$ and $^{205}\mathrm{Tl}$ at energies between the one- and two-neutron thresholds using quasimonochromatic $\ensuremath{\gamma}$-ray beams produced in laser Compton scattering at the NewSUBARU synchrotron radiation facility. Our measurement results in cross sections significantly different from the previously reported bremsstrahlung experiment, leading to rather different giant dipole resonance (GDR) parameters, in particular to lower GDR peak energies and higher peak cross sections. The photoneutron data are used to constrain the $\ensuremath{\gamma}$-ray strength function on the basis of the Hartree-Fock-Bogolyubov plus quasiparticle random-phase approximation using the Gogny D1M interaction. Supplementing the experimentally constrained $\ensuremath{\gamma}$-ray strength function with the zero-limit $E1$ and $M1$ contributions for the de-excitation mode, we estimate the Maxwellian-averaged cross section for the s-process branching-point nucleus $^{204}\mathrm{Tl}$ in the context of the $^{205}\mathrm{Pb}\ensuremath{-}^{205}\mathrm{Tl}$ chronometry.

The neutron-deficient mercury isotopes serve as a classical example of shape coexistence, whereby at low energy near-degenerate nuclear states characterized by different shapes appear. The electromagnetic structure of even-mass 182-188 Hg isotopes was studied using safe-energy Coulomb excitation of neutron-deficient mercury beams delivered by the REX-ISOLDE facility at CERN. The population of $ 0^{+}_{1,2}$01,2+, $ 2^{+}_{1,2}$21,2+and $ 4^{+}_{1}$41+states was observed in all nuclei under study. Reduced E2 matrix elements coupling populated yrast and non-yrast states were extracted, including their relative signs. These are a sensitive probe of shape coexistence and may be used to validate nuclear models. The experimental results are discussed in terms of mixing of two different configurations and are compared with three different model calculations: the Beyond Mean Field model, the Interacting Boson Model with configuration mixing and the General Bohr Hamiltonian. Partial agreement with experiment was observed, hinting to missing ingredients in the theoretical descriptions. The neutron-deficient mercury isotopes serve as a classical example of shape coexistence, whereby at low energy near-degenerate nuclear states characterized by different shapes appear. The electromagnetic structure of even-mass 182-188 Hg isotopes was studied using safe-energy Coulomb excitation of neutron-deficient mercury beams delivered by the REX-ISOLDE facility at CERN. The population of $ 0^{+}_{1,2}$01,2+, $ 2^{+}_{1,2}$21,2+and $ 4^{+}_{1}$41+states was observed in all nuclei under study. Reduced E2 matrix elements coupling populated yrast and non-yrast states were extracted, including their relative signs. These are a sensitive probe of shape coexistence and may be used to validate nuclear models. The experimental results are discussed in terms of mixing of two different configurations and are compared with three different model calculations: the Beyond Mean Field model, the Interacting Boson Model with configuration mixing and the General Bohr Hamiltonian. Partial agreement with experiment was observed, hinting to missing ingredients in the theoretical descriptions. ispartof: The European Physical Journal A - Hadrons and Nuclei vol:55 issue:8 pages:130-130 status: published

Numerous scientific fields including astrophysics, nuclear power, and nuclear forensics require a knowledge of basic nuclear properties for large numbers of short-lived, radioactive isotopes far removed from stable nuclei. Neutron-capture cross sections are one such piece of nuclear data where direct measurements are not possible and theoretical predictions can vary by orders of magnitude. A recently developed indirect technique for inferring neutron capture rates, the β -Oslo method, has been introduced but not compared against a known, directly measured neutron capture cross section. To provide this benchmark, two indirect methods based on β decay and charged-particle reactions were used to extract the nuclear level density and γ -ray strength function of 51 Ti . The nuclear level density and γ -ray strength function from the two data sets were found to be equivalent and were used to extract the neutron capture cross section of 50 Ti which agrees with previous direct measurements at high neutron energies. The results demonstrate the validity of the β -Oslo method for extracting neutron capture cross sections of short-lived nuclei and provide a sufficiently small uncertainty to be used in various applications.

International audience; A Coulomb excitation campaign on $^{106,108,110}$Sn at 4.4–4.5 MeV/u was launched at the HIE-ISOLDE facility at CERN. Larger excitation cross sections and γ-ray statistics were achieved compared to previous experiments at ∼2.8 MeV/u. More precise $(B(E2;0_{1}^{ + } \to 2_{1}^{ + }))$ values, lifetimes of states via the Doppler shift attenuation method, and new $(B(E2;0_{1}^{ + } \to 2_{x}^{ + })), (B(E2;2_{1}^{ + } \to 4_{1}^{ + }))$ and $(Q(2_{1}^{ + }))$ values from the new Miniball data will be obtained and applied to test modern nuclear structure theories.

ISOLDE at CERN is a leading radioactive ion beam facility. With its upgrade, the HIE-ISOLDE project, an increase in primary beam intensity and energy is envisaged and the aim is a significant increase in intensity of the exotic beams. The high resolution separator (HRS) after the upgrade is required to suppress contaminations almost completely when the masses differ to the beam of interest by Δ m / m > 1 / 20 , 000 . Here a 120° magnet with a bending radius of 1.25 m has been chosen. The magnetic rigidity is 0.625 Tm (B-field of 0.5 T) to allow for separation of molecules of up to a mass of 300 u. The magnet comprises a yoke in wedged H-type configuration for stability and precision and pole face conductors for focusing and compensation of aberrations. The concept was derived analytically, refined with the OPERA 2D software and tested with the ray-tracing module of OPERA 3D.

Photoneutron cross sections were measured for Ni58,Ni60,Ni61, and Ni64 at energies between the one-neutron and two-neutron thresholds using quasimonochromatic γ-ray beams produced in laser Compton scattering at the NewSUBARU synchrotron radiation facility. These photoneutron data are used to extract the γ-ray strength function above the neutron threshold, complementing the information obtained by the Oslo method below the threshold. We discuss radiative neutron-capture cross sections and the Maxwellian-averaged cross sections for Ni isotopes including Ni63, a branching point nucleus along the weak s-process path. The cross sections are calculated with the experimentally constrained γ-ray strength functions from the Hartree-Fock-Bogolyubov plus quasiparticle–random-phase approximation based on the Gogny D1M interaction for both E1 and M1 components and supplemented with the M1 upbend.

We are also grateful for the financial support received from the Research Council of Norway (NFR). S.S. and G.M.T. acknowledge funding under NFR project Grants No. 210007 and No. 262952/F20. A.C.L. acknowledges financial support from the ERC-STG2014 under Grant No. 637686.

The photoneutron cross sections of Dy162,163 have been measured for the first time in an energy region from the neutron threshold (Sn) up to ≈13MeV. The (γ,n) reaction was induced with quasimonochromatic laser Compton-scattered γ rays, produced at the NewSUBARU laboratory. The corresponding γ-ray strength functions (γSF) have been calculated from the photoneutron cross sections. The data are compared to reanalyzed γSFs of Dy160-164, which are measured below Sn. The excellent agreement with the photoneutron data at Sn confirms the principle of detailed balance. Thus, a complete γSF is established covering in total the energy region of 1≤Eγ≤13 MeV. These mid-shell well-deformed dysprosium isotopes all show scissors resonances with very similar structures. We find that our data predict the same integrated scissors strength as (γ,γ′) data when integrated over the same energy range, which shows that the scissors mode very likely is consistent with the generalized Brink hypothesis. Finally, using the γSFs as input in the reaction code talys, we have deduced radiative neutron-capture cross sections and compared them to direct measurements. We find a very good agreement within the uncertainties, which gives further support to the experimentally determined γSFs., SCOPUS: ar.j, info:eu-repo/semantics/published

Single- and multi-photon spectra of pulsed γ -ray beams produced at 17, 34, and 40 MeV in the laser Compton scattering were measured with an 8” × 12” NaI(Tl) detector. By using the experimental single-photon spectra as the probability function of generating random numbers, response functions of the NaI(Tl) detector to j -fold photons ( j = 2, 3, 4 ...) were constructed. The least-square fits to the experimental multi-photon spectra by the Poisson distribution consisting of the response functions were made. The multi-photon spectra measured at 17 and 34 MeV follow the Poisson distribution. A quenching phenomenon of multi-photon spectra was observed for 40 MeV γ -rays as a result of the saturation at the photomultiplier tube of the NaI(Tl) detector. The original Poisson distributions were restored from the quenched spectra using a saturation curve in the form of y = a ⋅ x η with η =e − b x . We discuss the accuracy of photon-flux determination.

Statistical $\gamma$-decay from highly excited states is determined by the nuclear level density (NLD) and the $\gamma$-ray strength function ($\gamma$SF). These average quantities have been measured for several nuclei using the Oslo method. For the first time, we exploit the NLD and $\gamma$SF to evaluate the $\gamma$-width in the energy region below the neutron binding energy, often called the quasi-continuum region. The lifetimes of states in the quasi-continuum are important benchmarks for a theoretical description of nuclear structure and dynamics at high temperature. The lifetimes may also have impact on reaction rates for the rapid neutron-capture process, now demonstrated to take place in neutron star mergers., Comment: CGS16, Shanghai 2017, Proceedings, 5 pages, 3 figures

© The Authors, published by EDP Sciences, 2018. Precise spectroscopic information on the fast neutron induced fission of the 238U(n,f) reaction was recently gained using a new technique which involved coupling of the Miniball high resolution y-ray spectrometer and the LICORNE directional neutron source. The experiment allowed measurement of the isotopic fission yields for around 40 even-even nuclei at an incident neutron energy of around 2 MeV where yield data are very sparse. In addition spectroscopic information on very neutron-rich fission products was obtained. Results were compared to models, both the JEFF-3.1.1 data base and the GEF code, and large discrepancies for the S1 fission mode in the Sn/Mo isotope pair were discovered. This suggests that current models are overestimating the role played by spherical shell effects in fast neutron induced fission. In late 2017 and 2018 the nu-ball hybrid spectrometer will be constructed at the IPN Orsay to perform further experimental investigations with directional neutrons coupled to a powerful hybrid Ge/LaBr3 detector array. This will open up new possibilities for measurements of fission yields for fast-neutron-induced fission using the spectroscopic technique and will be complimentary to other methods being developed. ispartof: SCIENTIFIC WORKSHOP ON NUCLEAR FISSION DYNAMICS AND THE EMISSION OF PROMPT NEUTRONS AND GAMMA RAYS (THEORY-4) vol:169 ispartof: 4th Scientific Workshop on Nuclear Fission Dynamics and the Emission of Prompt Neutrons and Gamma Rays (Theory) location:BULGARIA, Varna date:20 Jun - 22 Jun 2017 status: published

The $\ensuremath{\gamma}$ decay of $^{65}\mathrm{Ni}$ has been studied from particle-$\ensuremath{\gamma}$ coincidence data on the $^{64}\mathrm{Ni}(d,p\ensuremath{\gamma})^{65}\mathrm{Ni}$ reaction. $\ensuremath{\gamma}$-ray spectra at excitation energies below ${E}_{x}\ensuremath{\approx}2\phantom{\rule{4pt}{0ex}}\mathrm{MeV}$ have been studied and compared with previous measurements. Coincidences corresponding to ${E}_{x}\ensuremath{\approx}4.4--6.1\phantom{\rule{4pt}{0ex}}\mathrm{MeV}$ have been used to constrain the shape of the nuclear level density and $\ensuremath{\gamma}$-strength function of $^{65}\mathrm{Ni}$ by means of the Oslo method. The experimental $\ensuremath{\gamma}$-strength function presents an enhancement at $\ensuremath{\gamma}$ energies below ${E}_{\ensuremath{\gamma}}\ensuremath{\approx}3\phantom{\rule{4pt}{0ex}}\mathrm{MeV}$. In addition, a resonance-like structure centered at ${E}_{\ensuremath{\gamma}}\ensuremath{\approx}4.6\phantom{\rule{4pt}{0ex}}\mathrm{MeV}$ is seen together with accumulated strength at ${E}_{\ensuremath{\gamma}}\ensuremath{\approx}2.6--3.6\phantom{\rule{4pt}{0ex}}\mathrm{MeV}$. The obtained results contribute to the systematic study of $\ensuremath{\gamma}$ decay in the Ni isotopes, which is of great interest for the understanding of both single-particle and collective nuclear structure phenomena.

Author(s): Rose, SJ; Zeiser, F; Wilson, JN; Oberstedt, A; Oberstedt, S; Siem, S; Tveten, GM; Bernstein, LA; Bleuel, DL; Brown, JA; Crespo Campo, L; Giacoppo, F; Gorgen, A; Guttormsen, M; Hadynska, K; Hafreager, A; Hagen, TW; Klintefjord, M; Laplace, TA; Larsen, AC; Renstrom, T; Sahin, E; Schmitt, C; Tornyi, TG; Wiedeking, M | Abstract: Prompt-fission γ rays are responsible for approximately 5% of the total energy released in fission, and therefore important to understand when modeling nuclear reactors. In this work we present prompt γ-ray emission characteristics in fission as a function of the nuclear excitation energy of the fissioning system. Emitted γ-ray spectra were measured, and γ-ray multiplicities and average and total γ energies per fission were determined for the U(d,pf)233 reaction for excitation energies between 4.8 and 10 MeV, and for the Pu(d,pf)239 reaction between 4.5 and 9 MeV. The spectral characteristics show no significant change as a function of excitation energy above the fission barrier, despite the fact that an extra ∼5 MeV of energy is potentially available in the excited fragments for γ decay. The measured results are compared with model calculations made for prompt γ-ray emission with the fission model code gef. Further comparison with previously obtained results from thermal neutron induced fission is made to characterize possible differences arising from using the surrogate (d,p) reaction.

Fast-neutron-induced fission of 238U at an energy just above the fission threshold is studied with a novel technique which involves the coupling of a high-efficiency γ-ray spectrometer (MINIBALL) to an inverse-kinematics neutron source (LICORNE) to extract charge yields of fission fragments via γ−γ coincidence spectroscopy. Experimental data and fission models are compared and found to be in reasonable agreement for many nuclei; however, significant discrepancies of up to 600% are observed, particularly for isotopes of Sn and Mo. This indicates that these models significantly overestimate the standard 1 fission mode and suggests that spherical shell effects in the nascent fission fragments are less important for low-energy fast-neutron-induced fission than for thermal neutron-induced fission. This has consequences for understanding and modeling the fission process, for experimental nuclear structure studies of the most neutron-rich nuclei, for future energy applications (e.g., Generation IV reactors which use fast-neutron spectra), and for the reactor antineutrino anomaly.

Excited states in the nucleus 133Sn, with one neutron outside the doubly-magic 132Sn core, were populated following one-neutron knockout from a 134Sn beam on a carbon target at relativistic energies at the Radioactive Isotope Beam Factory at RIKEN. Besides the rays emitted in the decay of the known neutron single-particle states in 133Sn additional strength in the energy range 3.5-5.5 MeV was observed for the fi rst time. Since the neutron-separation energy of 133Sn is low, Sn=2.402(4) MeV, this observation provides direct evidence for the radiative decay of neutron- unbound states in this nucleus. The ability of electromagnetic decay to compete successfully with neutron emission at energies as high as 3 MeV above threshold is attributed to a mismatch between the wave functions of the initial and final states in the latter case. These fi ndings suggest that in the region south-east of 132Sn nuclear structure effects may play a signifi cant role in the neutron vs. competition in the decay of unbound states. As a consequence, the common neglect of such effects in the evaluation of the neutron-emission probabilities in calculations of global b -decay properties for astrophysical simulations may have to be reconsidered.

In this contribution we discuss new experimental approaches to indirectly provide information on neutron-capture rates relevant to the $r$-process. In particular, we focus on applications of the Oslo method to extract fundamental nuclear properties for reaction-rate calculations: the nuclear level density and the $\gamma$ strength function. Two methods are discussed in detail, the Oslo method in inverse kinematics and the beta-Oslo method. These methods present a first step towards constraining neutron-capture rates of importance to the $r$-process.

A particularly challenging part of the question of how elements heavier than iron are created in extreme, astrophysical environments is the creation of the so-called p-nuclei, which are believed to be mainly produced in the O-Ne layer of type II supernovae or type Ia supernovae. The lack of needed nuclear data presents an obstacle in nailing down the precise site and astrophysical conditions for the production of these isotopes. Astrophysical model calculations are able to reproduce abundance patterns of most p-isotopes reasonably well, with some pivotal exceptions. In particular, p-isotopes of mass 92 ≤ A ≤ 98 are underproduced in calculations compared to the actual abundance of these isotopes. The p-isotope 92Mo represents one of the most severe cases of underproduction. State-of-the-art p-process calculations systematically underestimate the observed solar abundance of this isotope. The main destruction mechanism of this isotope in the standard description of the p-process is through the 92Mo(γ, p)91Nb reaction. Measurements on the nuclear level density and average gamma strength function of 92Mo have been carried out at the Oslo Cyclotron Laboratory. TALYS cross section and reaction rate calculations where the experimental results are used as input will be presented. The data provide stringent constraints on the 91Nb(p, γ)92Mo (and consequently the inverse) reaction rate. The reaction rate extracted in this work was used in reaction network calculations for the scenario of a p-process taking place in a type II supernova explosion as the shock front passes through the O-Ne layer of a 25 solar mass star.

Experimental results of the $^{237}$Np($d, p \gamma)^{238}$Np reaction are presented, which verifies the generalized Brink-Axel (gBA) hypothesis for $\gamma$ transitions between states in the quasi-continuum. The gBA hypothesis holds not only for specific collective resonances, but for the full dipole strength below the neutron separation energy. We discuss the validity of the gBA hypothesis also for lighter systems like $^{92}$Zr where the concept of a unique $\gamma$-ray strength function ($\gamma$SF) is problematic due to large Porter-Thomas fluctuations. Methods for studying the $\gamma$SF and the fluctuations as function of excitation energy are presented., Comment: 8 pages, 4 figures, PoS proceedings for The 26th International Physics Conference 11-16 September, 2016, Adelaide, Australia

Nuclear level densities and $\gamma$-ray strength functions of $^{56,57}$Fe have been extracted from proton-$\gamma$ coincidences. A low-energy enhancement in the $\gamma$-ray strength functions up to a factor of 30 over common theoretical E1 models is confirmed. Angular distributions of the low-energy enhancement in $^{57}$Fe indicate its dipole nature, in agreement with findings for $^{56}$Fe. The high statistics and the excellent energy resolution of the large-volume LaBr$_{3}$(Ce) detectors allowed for a thorough analysis of $\gamma$ strength as function of excitation energy. Taking into account the presence of strong Porter-Thomas fluctuations, there is no indication of any significant excitation-energy dependence in the $\gamma$-ray strength function, in support of the generalized Brink-Axel hypothesis., Comment: 24 pages, 17 figures, accepted for publication in J. Phys. G: Nucl. Phys; Special Issue

The structure of neutron-rich 96,98Sr nuclei was investigated by low-energy safe Coulomb excitation of radioactive beams at the REX-ISOLDE facility, CERN, with the MINIBALL spectrometer. A rich set of transitional and diagonal E2 matrix elements, including those for non-yrast structures, has been extracted from the differential Coulomb-excitation cross sections. The results support the scenario of a shape transition at N = 60, giving rise to the coexistence of a highly deformed prolate and a spherical configuration in 98Sr, and are compared to predictions from several theoretical calculations. The experimental data suggest a significant contribution of the triaxal degree of freedom in the ground state of both isotopes. In addition, experimental information on low-lying states in 98Rb has been obtained.

Particle-$\ensuremath{\gamma}$ coincidence data have been analyzed to obtain the nuclear level density and the $\ensuremath{\gamma}$-strength function of $^{64}\mathrm{Ni}$ by means of the Oslo method. The level density found in this work is in very good agreement with known energy levels at low excitation energies as well as with data deduced from particle-evaporation measurements at excitation energies above ${E}_{x}\ensuremath{\approx}5.5$ MeV. The experimental $\ensuremath{\gamma}$-strength function presents an enhancement at $\ensuremath{\gamma}$ energies below ${E}_{\ensuremath{\gamma}}\ensuremath{\approx}3$ MeV and possibly a resonancelike structure centered at ${E}_{\ensuremath{\gamma}}\ensuremath{\approx}9.2$ MeV. The obtained nuclear level density and $\ensuremath{\gamma}$-strength function have been used to estimate the $(n,\ensuremath{\gamma})$ cross section for the $s$-process branch-point nucleus $^{63}\mathrm{Ni}$, of particular interest for astrophysical calculations of elemental abundances.

We have recently successfully demonstrated a new technique for production and study of many of the most exotic neutron-rich nuclei at moderate spins. LICORNE, a newly developed directional inverse-kinematic fast neutron source at the IPN Orsay, was coupled to the MINIBALL high resolution γ-ray spectrometer to study nuclei the furthest from stability using the 238U(n,f) reaction. This reaction and 232Th(n,f) are the most neutron-rich fission production mechanisms achievable and can be used to simultaneously populate hundreds of neutron-rich nuclei up to spins of ≈ 16ℏ. High selectivity in the experiment was achieved via triple γ-ray coincidences and the use of a 400 ns period pulsed neutron beam, a technique which is unavailable to other population mechanisms such as 235U(nth,f) and 252Cf(SF). The pulsing allows time correlations to be exploited to separate delayed γ rays from isomeric states in the hundreds of nuclei produced, which are then used to cleanly select a particular nucleus and its exotic binary partners. In the recent experiment, several physics cases are simultaneously addressed such as shape coexistence, the evolution of shell closures far from stability, and the spectroscopy of nuclei in the r-process path near N = 82. Preliminary physics results on anomalies in the 238U(n,f) fission yields and the structure of the 138Te and 100Sr nuclei will soon be published. A future project, ν-ball, to couple LICORNE with a hybrid escape-suppressed spectrometer to refine further the technique and achieve a large increase in the observational limit is discussed. ispartof: pages:395-401 ispartof: Acta Physica Polonica B vol:48 issue:3 pages:395-401 ispartof: location:Zakopane: POLAND status: published

One of the greatest questions for modern physics to address is how elements heavier than iron are created in extreme, astrophysical environments. A particularly challenging part of that question is the creation of the so-called p-nuclei, which are believed to be mainly produced in some types of supernovae. The lack of needed nuclear data presents an obstacle in nailing down the precise site and astrophysical conditions. In this work, we present for the first time measurements on the nuclear level density and average strength function of $^{92}$Mo. State-of-the-art p-process calculations systematically underestimate the observed solar abundance of this isotope. Our data provide stringent constraints on the $^{91}$Nb$(p,{\gamma})^{92}$Mo reaction rate, which is the last unmeasured reaction in the nucleosynthesis puzzle of $^{92}$Mo. Based on our results, we conclude that the $^{92}$Mo abundance anomaly is not due to the nuclear physics input to astrophysical model calculations., Comment: Submitted to PRC

We investigated the U238(d,p) reaction as a surrogate for the n+U238 reaction. For this purpose we measured for the first time the γ-decay and fission probabilities of U∗239 simultaneously and compared them to the corresponding neutron-induced data. We present the details of the procedure to infer the decay probabilities, as well as a thorough uncertainty analysis, including parameter correlations. Calculations based on the continuum-discretized coupled-channels method and the distorted-wave Born approximation (DWBA) were used to correct our data from detected protons originating from elastic and inelastic deuteron breakup. In the region where fission and γ emission compete, the corrected fission probability is in agreement with neutron-induced data, whereas the γ-decay probability is much higher than the neutron-induced data. We have performed calculations of the decay probabilities with the statistical model and of the average angular momentum populated in the U238(d,p) reaction with the DWBA to interpret these results.

The $\ensuremath{\gamma}$-ray strength functions and level densities of $^{73,74}\mathrm{Ge}$ have been extracted up to the neutron-separation energy ${S}_{n}$ from particle-$\ensuremath{\gamma}$ coincidence data using the Oslo method. Moreover, the $\ensuremath{\gamma}$-ray strength function of $^{74}\mathrm{Ge}$ above ${S}_{n}$ has been determined from photoneutron measurements; hence these two experiments cover the range of ${\mathrm{E}}_{\ensuremath{\gamma}}\ensuremath{\approx}1$--13 MeV for $^{74}\mathrm{Ge}$. The obtained data show that both $^{73,74}\mathrm{Ge}$ display an increase in strength at low $\ensuremath{\gamma}$ energies. The experimental $\ensuremath{\gamma}$-ray strength functions are compared with $M1$ strength functions deduced from average $B(M1)$ values calculated within the shell model for a large number of transitions. The observed low-energy enhancements in $^{73,74}\mathrm{Ge}$ are adopted in the calculations of the $^{72,73}\mathrm{Ge}(n,\ensuremath{\gamma})$ cross sections, where there are no direct experimental data. Calculated reaction rates for more neutron-rich germanium isotopes are shown to be strongly dependent on the presence of the low-energy enhancement.

The electromagnetic structure of 140Sm was studied in a low-energy Coulomb excitation experiment with a radioactive ion beam from the REX-ISOLDE facility at CERN. The 2+ and 4+ states of the ground-state band and a second 2+ state were populated by multistep excitation. The analysis of the differential Coulomb excitation cross sections yielded reduced transition probabilities between all observed states and the spectroscopic quadrupole moment for the 2+ 1 state. The experimental results are compared to large-scale shell model calculations and beyond-mean-field calculations based on the Gogny D1S interaction with a five-dimensional collective Hamiltonian formalism. Simpler geometric and algebraic models are also employed to interpret the experimental data. The results indicate that 140Sm shows considerable γ softness, but in contrast to earlier speculation no signs of shape coexistence at low excitation energy. This work sheds more light on the onset of deformation and collectivity in this mass region. 15 pages, 12 figures ispartof: Physical Review C vol:93 issue:5 status: published

The nuclear level density and the γ -ray strength function have been extracted for 89 Y by using the Oslo method on 89Y(p,p′γ)89Y coincidence data. The γ-ray strength function displays a low-energy enhancement consistent with previous observations in this mass region (93–98Mo). Shell-model calculations support the conclusion that the observed enhancement is due to strong, low-energy M1 transitions at high excitation energies. The data were further used as input for calculations of the 88 Sr(p,γ )89 Y and 88 Y(n,γ )89 Y cross sections with the TALYS reaction code. Comparison with cross-section data, where available, as well as with values from the BRUSLIB library, shows a satisfying agreement.

The level density and gamma-ray strength function (gammaSF) of 243Pu have been measured in the quasi-continuum using the Oslo method. Excited states in 243Pu were populated using the 242Pu(d,p) reaction. The level density closely follows the constant-temperature level density formula for excitation energies above the pairing gap. The gammaSF displays a double-humped resonance at low energy as also seen in previous investigations of actinide isotopes. The structure is interpreted as the scissors resonance and has a centroid of omega_{SR}=2.42(5)MeV and a total strength of B_{SR}=10.1(15)mu_N^2, which is in excellent agreement with sum-rule estimates. The measured level density and gammaSF were used to calculate the 242Pu(n,gamma) cross section in a neutron energy range for which there were previously no measured data.