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Fragmentation of liquid metal droplets irradiated by linearly and circularly polarized femtosecond laser pulses is observed in our experiment. The obtained shadowgraph snapshots demonstrate that a circularly polarized pulse may produce several randomly-oriented jets effused from the expanding droplets, while a linearly polarized laser pulse generates strictly the cruciform jets. The latter orientation is tied with polarization plane, rotation of which causes rotation of the cruciform jets by the same angle. To shed light on the experimental data we performed molecular dynamics simulation of droplet expansion induced by angle-dependent heating. Our simulation shows that the jet directions are determined by an oriented angle-dependent energy distribution within a frontal hemisphere layer of droplet after absorption of linearly polarized light. As a result, the produced flow velocity field guided by surface tension forms two high-speed opposite jets oriented across the electric field vector as in our experiment. A shock-wave pulse generated in the frontal layer has angle-dependent amplitude inherited from the oriented energy deposition. The release part of shock pulse produces a cavitation zone nearby the droplet center, and thus an expanding spherical shell is formed from the droplet. The flow velocities within a rearside hemisphere of the shell, produced after reflection of the shock wave from the rear side of droplet, generate two low-speed opposite jets oriented along the electric field vector. Thus we found that the cruciform jets are originated independently from the frontal and rear sides of droplet, and a pair of frontal jets is faster than a pair of rearside jets., Comment: 11 pages, 10 figures

The fragmentation of a liquid metal droplet induced by a nanosecond laser pulse has been studied well. However, the fragmentation mechanism may be different, when a subpicosecond laser pulse is applied. To discover the details of the fragmentation process, we perform a hydrodynamic simulation of a liquid tin droplet irradiated by a femtosecond laser pulse. We have found that the pressure pulse induced by an instantaneous temperature growth in the skin layer propagates from the one side of the surface of a spherical droplet and focuses in its center; at the release a big cavity is formed at the center of a droplet; the pressure wave release at the backside surface may cause the spallation., Comment: Accepted to Journal of Physics: Conference Series

We report an experimental and numerical investigation of the fragmentation mechanisms of micrometer-sized metal droplet irradiated by ultrashort laser pulses. The results of the experiment show that the fast one-side heating of such a droplet may lead to either symmetric or asymmetric expansion followed by different fragmentation scenarios. To unveil the underlying processes leading to fragmentation we perform simulation of liquid-tin droplet expansion produced by the initial conditions similar to those in experiment using the smoothed particle hydrodynamics (SPH) method. Simulation demonstrates that a thin heated surface layer generates a ultrashort shock wave propagating from the frontal side to rear side of the droplet. Convergence of such shock wave followed by a rarefaction tale to the droplet center results in the cavitation of material inside the central region by the strong tensile stress. Reflection of the shock wave from the rear side of droplet produces another region of highly stretched material where the spallation may occur producing a thin spallation layer moving with a velocity higher than expansion of the central shell after cavitation. It is shown both experimentally and numerically that the threshold laser intensity necessary for the spallation is higher than the threshold required to induce cavitation in the central region of droplet. Thus, the regime of asymmetrical expansion is realized if the laser intensity exceeds the spallation threshold. The transverse and longitudinal expansion velocities obtained in SPH simulations of different regimes of expansion are agreed well with our experimental data.