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Here, we report a novel and conceptually straightforward technique to detect the spin-polarization directly, with laser spot spatial resolution, at buried ferromagnet/insulator interfaces in ambient settings. This has been accomplished by monitoring the voltage-induced change of the longitudinal MOKE signal as a function of the applied magnetic field and applying an AC voltage across the interface. For the case where the spin polarization enters the VMOKE signal, a simple quantitative model is proposed. A distinct positive majority spin polarization has been found for Fe and Co, whereas Ni exhibits a negative minority spin polarization.

A key element to tailor the properties of magnetic multilayers is the coupling between the individual magnetic layers. In case of skyrmion hosting multilayers, coupling of skyrmions across the magnetic layers is highly desirable. Here the magnetic interlayer coupling was studied in epitaxial all-oxide heterostructures of ferromagnetic perovskite SrRuO$_3$ layers separated by spacers of the strong spin-orbit coupling oxide SrIrO$_3$. This combination of oxide layers is being discussed as a potential candidate system to host N\'{e}el skyrmions. First order reversal curve (FORC) measurements were performed in order to distinguish between magnetic switching processes of the individual layers and to disentangle the signal of soft magnetic impurities from the samples$'$ signal. Additionally, FORC investigations enabled to determine whether the coupling between the magnetic layers is ferromagnetic or antiferromagnetic. The observed interlayer coupling strength was weak for all the heterostructures, with SrIrO$_3$ spacers between 2 monolayers and 12 monolayers thick., Comment: 22 pages

Magnetic droplets are non-topological magnetodynamical solitons displaying a wide range of complex dynamic phenomena with potential for microwave signal generation. Bubbles, on the other hand, are internally static cylindrical magnetic domains, stabilized by external fields and magnetostatic interactions. In its original theory, the droplet was described as an imminently collapsing bubble stabilized by spin transfer torque and, in its zero-frequency limit, as equivalent to a bubble. Without nanoscale lateral confinement, pinning, or an external applied field, such a nanobubble is unstable, and should collapse. Here, we show that we can freeze dynamic droplets into static nanobubbles by decreasing the magnetic field. While the bubble has virtually the same resistance as the droplet, all signs of low-frequency microwave noise disappear. The transition is fully reversible and the bubble can be thawed back into a droplet if the magnetic field is increased under current. Whereas the droplet collapses without a sustaining current, the bubble is highly stable and remains intact for days without external drive. Electrical measurements are complemented by direct observation using scanning transmission x-ray microscopy, which corroborates the analysis and confirms that the bubble is stabilized by pinning., Comment: 23 pages, 5 figures

Rare earth ions typically exhibit larger magnetic moments than transition metal ions and thus promise the opening of a wider exchange gap in the Dirac surface states of topological insulators. Yet, in a recent photoemission study of Eu-doped Bi$_2$Te$_3$ films, the spectra remained gapless down to $T = 20\;\text{K}$. Here, we scrutinize whether the conditions for a substantial gap formation in this system are present by combining spectroscopic and bulk characterization methods with theoretical calculations. For all studied Eu doping concentrations, our atomic multiplet analysis of the $M_{4,5}$ x-ray absorption and magnetic circular dichroism spectra reveals a Eu$^{2+}$ valence and confirms a large magnetic moment, consistent with a $4f^7 \; {^8}S_{7/2}$ ground state. At temperatures below $10\;\text{K}$, bulk magnetometry indicates the onset of antiferromagnetic (AFM) ordering. This is in good agreement with density functional theory, which predicts AFM interactions between the Eu impurities. Our results support the notion that antiferromagnetism can coexist with topological surface states in rare-earth doped Bi$_2$Te$_3$ and call for spectroscopic studies in the kelvin range to look for novel quantum phenomena such as the quantum anomalous Hall effect., Comment: 15 pages, 9 figures

Since 2000, the intensive effort in materials research to develop a diluted magnetic semiconductor exhibiting high-temperature (HT) ferromagnetism above room temperature was not successful. Here, the possible first bulk diluted HT-ferromagnetic non-metallic materials, based on the perovskite-type oxynitrides LaTa1-xCox(O,N)3-d (x = 0.01, 0.03, 0.05) are realized. The Curie temperature of the synthesized powders exceeds 600 K and the sample magnetizations are large enough to be directly attracted by permanent magnets. Cobalt clusters as a possible source for the observed HT-ferromagnetism can be excluded, since all applied characterization methods verify phase purity. Applied conventional and element-specific magnetometry imply ferromagnetic intermediate spin (IS) Co3+ which is included in a ferromagnetic host matrix. This indicates a complex magnetic interplay between the existing crystal structure, the observed anionic vacancies, and the introduced cobalt ions. These results lay the foundation for the experimental investigation and design of further diluted HT-ferromagnetic semiconductors., Comment: submitted to journal

Magnonic quasicrystals exceed the possibilities of spin wave (SW) manipulation offered by regular magnonic crystals, because of their more complex SW spectra with fractal characteristics. Here, we report the direct x-ray microscopic observation of propagating SWs in a magnonic quasicrystal, consisting of dipolarly coupled permalloy nanowires arranged in a one-dimensional Fibonacci sequence. SWs from the first and second band as well as evanescent waves from the band gap between them are imaged. Moreover, additional mini-band gaps in the spectrum are demonstrated, directly indicating an influence of the quasiperiodicity of the system. The experimental results are interpreted using numerical calculations and we deduce a simple model to estimate the frequency position of the magnonic gaps in quasiperiodic structures. The demonstrated features of SW spectra in one-dimensional magnonic quasicrystals allows utilizing this class of metamaterials for magnonics and makes them an ideal basis for future applications., Comment: 10 pages, 6 figures

Magnonics, i.e. the artificial manipulation of spin waves, is a flourishing field of research with many potential uses in data processing within reach. Apart from the technological applications the possibility to directly influence and observe these types of waves is of great interest for fundamental research. Guidance and steering of spin waves has been previously shown and lateral spin wave confinement has been achieved. However, true spin wave focusing with both lateral confinement and increase in amplitude has not been shown before. Here, we show for the first time spin wave focusing by realizing a Fresnel zone plate type lens. Using x-ray microscopy we are able to directly image the propagation of spin waves into the nanometer sized focal spot. Furthermore, we observe that the focal spot can be freely moved in a large area by small variations of the bias field. Thus, this type of lens provides a steerable intense nanometer sized spin wave source. Potentially, this could be used to selectively illuminate magnonic devices like nano oscillators with a steerable spin wave beam.

Magnetic droplets are non-topological dynamical solitons that can be nucleated and sustained in nano-contact based spin torque nano-oscillators (NC-STNOs) with perpendicular anisotropy free layers. While originally predicted in all-perpendicular NC-STNOs, all experimental demonstrations have so far relied on orthogonal devices with an in-plane polarizing layer that requires a strong magnetic field for droplet nucleation. Here, we instead show the nucleation and sustained operation of magnetic droplets in all-perpendicular NC-STNOs in modest perpendicular fields and over a wide range of nano-contact size. The droplet is observed electrically as an intermediate resistance state accompanied by broadband low-frequency microwave noise. Using canted fields, which introduce a non-zero relative angle between the free and fixed layer, the actual droplet precession frequency can also be determined. Finally, the droplet size, its perimeter width, and its fully reversed core are directly observed underneath a 80 nm diameter nano-contact using scanning transmission x-ray microscopy on both the Ni and Co edges. The droplet diameter is 150 nm, i.e. almost twice the nominal size of the nano-contact, and the droplet has a perimeter width of about 70 nm.

Fresnel Zone Plates (FZP) are to date very successful focusing optics for X-rays. Established methods of fabrication are rather complex and based on electron beam lithography (EBL). Here, we show that ion beam lithography (IBL) may advantageously simplify their preparation. A FZP operable from the extreme UV to the limit of the hard X-ray was prepared and tested from 450 eV to 1500 eV. The trapezoidal profile of the FZP favorably activates its 2nd order focus. The FZP with an outermost zone width of 100 nm allows the visualization of features down to 61, 31 and 21 nm in the 1st, 2nd and 3rd order focus respectively. Measured efficiencies in the 1st and 2nd order of diffraction reach the theoretical predictions.

Modern magnetic thin film devices owe their success in large part to effects emerging from interlayer coupling and exchange interaction at interfaces. A prominent example is exchange bias (EB), a magnetic coupling phenomenon found in ferromagnet (F)/antiferromagnet (AF) systems. Uncompensated pinned moments in the AF couple to the F via the interface causing an additional unidirectional anisotropy. As a result, the hysteresis of the F is shifted. The existence of such pinned moments is nowadays accepted although their physical nature and origin is still unknown. Here we present a thorough spectroscopic investigation based on X-ray magnetic circular dichroism which does for the first time provide direct information about the physics of pinned magnetic moments. Our data clearly shows that the orbital magnetic moment, which is usually widely quenched in transition metal systems, is the driving force behind exchange bias in Co/FeMn.