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The ability to generate entangled states of light is a key primitive for quantum communication and distributed quantum computation. Continuously driven sources, including those based on spontaneous parametric downconversion, are usually probabilistic, whereas deterministic sources require accurate timing of the control fields. Here, we experimentally generate entangled photonic modes by continuously exciting a quantum emitter, a superconducting qubit, with a coherent drive, taking advantage of mode matching in the time and frequency domain. Using joint quantum state tomography and logarithmic negativity, we show that entanglement is generated between modes extracted from the two sidebands of the resonance fluorescence spectrum. Because the entangled photonic modes are perfectly orthogonal, they can be transferred into distinct quantum memories. Our approach can be utilized to distribute entanglement at a high rate in various physical platforms, with applications in waveguide quantum electrodynamics, distributed quantum computing, and quantum networks.

Physical devices operating out of equilibrium are inherently affected by thermal fluctuations, limiting their operational precision. This issue is pronounced at microscopic and especially quantum scales and can only be mitigated by incurring additional entropy dissipation. Understanding this constraint is crucial for both fundamental physics and technological design. For instance, clocks are inherently governed by the second law of thermodynamics and need a thermodynamic flux towards equilibrium to measure time, which results in a minimum entropy dissipation per clock tick. Classical and quantum models and experiments often show a linear relationship between precision and dissipation, but the ultimate bounds on this relationship are unknown. Our theoretical discovery presents an extensible quantum many-body system that achieves clock precision scaling exponentially with entropy dissipation. This finding demonstrates that coherent quantum dynamics can surpass the traditional thermodynamic precision limits, potentially guiding the development of future high-precision, low-dissipation quantum devices., Comment: 6 + 14 pages, 9 figures, comments welcome

Local control of superconducting circuits by high-impedance electrical gates offers potential advantages in superconducting logic, quantum processing units, and cryoelectronics. Recent experiments have reported gate-controlled supercurrent in Dayem bridges made of metallic superconductors, mediated by direct current leakage, out-of-equilibrium phonons, or possibly other mechanisms. However, a time-domain characterization of this effect has been lacking. Here, we integrate Dayem bridges made of Niobium on Silicon into coplanar-waveguide resonators, and measure the effect of the gate voltage at steady state and during pulsed operation. We consider two types of arrangements for the gate: a side-coupled gate and a remote injector. In both cases, we observe sizable changes in the real and the imaginary part of the constriction's impedance for gate voltages of the order of 1 V. However, we find striking differences in the time-domain dynamics, with the remote injector providing a faster and more controlled response. Our results contribute to our understanding of gate-controlled superconducting devices and their suitability for applications., Comment: 7 pages, 4 figures

Atom-photon bound states arise from the coupling of quantum emitters to the band edge of dispersion-engineered waveguides. Thanks to their tunable-range interactions, they are promising building blocks for quantum simulators. Here, we study the dynamics of an atom-photon bound state emerging from coupling a frequency-tunable quantum emitter - a transmon-type superconducting circuit - to the band edge of a microwave metamaterial. Employing precise temporal control over the frequency detuning of the emitter from the band edge, we examine the transition from adiabatic to non-adiabatic behavior in the formation of the bound state and its melting into the propagating modes of the metamaterial. Moreover, we experimentally observe multi-mode emission from the bound state, triggered by a fast change of the emitter's frequency. Our study offers insight into the dynamic preparation of atom-photon bound states and provides a method to characterize their photonic content, with implications in quantum optics and quantum simulation., Comment: 8 pages (4 figures) + supplementary information (5 pages)

Detecting quasiparticle tunneling events in superconducting circuits provides information about the population and dynamics of non-equilibrium quasiparticles. Such events can be detected by monitoring changes in the frequency of an offset-charge-sensitive superconducting qubit. This monitoring has so far been performed by Ramsey interferometry assisted by a readout resonator. Here, we demonstrate a quasiparticle detector based on a superconducting qubit directly coupled to a waveguide. We directly measure quasiparticle number parity on the qubit island by probing the coherent scattering of a microwave tone, offering simplicity of operation, fast detection speed, and a large signal-to-noise ratio. We observe tunneling rates between 0.8 and $7~\rm{s}^{-1}$, depending on the average occupation of the detector qubit, and achieve a temporal resolution below $10~\mu\rm{s}$ without a quantum-limited amplifier. Our simple and efficient detector lowers the barrier to perform studies of quasiparticle population and dynamics, facilitating progress in fundamental science, quantum information processing, and sensing.

While dephasing noise frequently presents obstacles for quantum devices, it can become an asset in the context of a Brownian-type quantum refrigerator. Here we demonstrate a novel quantum thermal machine that leverages noise-assisted quantum transport to fuel a cooling engine in steady state. The device exploits symmetry-selective couplings between a superconducting artificial molecule and two microwave waveguides. These waveguides act as thermal reservoirs of different temperatures, which we regulate by employing synthesized thermal fields. We inject dephasing noise through a third channel that is longitudinally coupled to an artificial atom of the molecule. By varying the relative temperatures of the reservoirs, and measuring heat currents with a resolution below 1 aW, we demonstrate that the device can be operated as a quantum heat engine, thermal accelerator, and refrigerator. Our findings open new avenues for investigating quantum thermodynamics using superconducting quantum machines coupled to thermal microwave waveguides.

Homo- and heterodyne detection are fundamental techniques for measuring propagating electromagnetic fields. However, applying these techniques to stationary fields confined in cavities poses a challenge. As a way to overcome this challenge, we propose to use repeated indirect measurements of a two-level system interacting with the cavity. We demonstrate numerically that the proposed measurement scheme faithfully reproduces measurement statistics of homo- or heterodyne detection at the single-shot level. The scheme can be implemented in various physical architectures, including circuit quantum electrodynamics. Our results pave the way to the implementation of quantum algorithms requiring linear detection, including quantum verification protocols, in stationary modes.

Linear bosonic modes offer a hardware-efficient alternative for quantum information processing but require access to some nonlinearity for universal control. The lack of nonlinearity in photonics has led to encoded measurement-based quantum computing, which rely on linear operations but requires access to resourceful ('nonlinear') quantum states, such as cubic phase states. In contrast, superconducting microwave circuits offer engineerable nonlinearities but suffer from static Kerr nonlinearity. Here, we demonstrate universal control of a bosonic mode composed of a superconducting nonlinear asymmetric inductive element (SNAIL) resonator, enabled by native nonlinearities in the SNAIL element. We suppress static nonlinearities by operating the SNAIL in the vicinity of its Kerr-free point and dynamically activate nonlinearities up to third order by fast flux pulses. We experimentally realize a universal set of generalized squeezing operations, as well as the cubic phase gate, and exploit them to deterministically prepare a cubic phase state in 60 ns. Our results initiate the experimental field of universal continuous-variables quantum computing., Comment: 11 pages, 6 figures and supplementary materials

Controlled quantum machines have matured significantly. A natural next step is to increasingly grant them autonomy, freeing them from time-dependent external control. For example, autonomy could pare down the classical control wires that heat and decohere quantum circuits; and an autonomous quantum refrigerator recently reset superconducting qubits to near their ground states, as is necessary before a computation. Which fundamental conditions are necessary for realizing useful autonomous quantum machines? Inspired by recent quantum thermodynamics and chemistry, we posit conditions analogous to DiVincenzo's criteria for quantum computing. Furthermore, we illustrate the criteria with multiple autonomous quantum machines (refrigerators, circuits, clocks, etc.) and multiple candidate platforms (neutral atoms, molecules, superconducting qubits, etc.). Our criteria are intended to foment and guide the development of useful autonomous quantum machines., Comment: 11 pages + appendices

The first thermal machines steered the industrial revolution, but their quantum analogs have yet to prove useful. Here, we demonstrate a useful quantum absorption refrigerator formed from superconducting circuits. We use it to reset a transmon qubit to a temperature lower than that achievable with any one available bath. The process is driven by a thermal gradient and is autonomous -- requires no external control. The refrigerator exploits an engineered three-body interaction between the target qubit and two auxiliary qudits coupled to thermal environments. The environments consist of microwave waveguides populated with synthesized thermal photons. The target qubit, if initially fully excited, reaches a steady-state excited-level population of $5\times10^{-4} \pm 5\times10^{-4}$ (an effective temperature of 23.5~mK) in about 1.6~$\mu$s. Our results epitomize how quantum thermal machines can be leveraged for quantum information-processing tasks. They also initiate a path toward experimental studies of quantum thermodynamics with superconducting circuits coupled to propagating thermal microwave fields., Comment: 7 pages (4 figures) + supplementary information (6 pages)

The control of a superconducting current via the application of a gate voltage has been recently demonstrated in a variety of superconducting devices. Although the mechanism underlying this gate-controlled supercurrent (GCS) effect remains under debate, the GCS effect has raised great interest for the development of the superconducting equivalent of conventional metaloxide semiconductor electronics. To date, however, the GCS effect has been mostly observed in superconducting devices made by additive patterning. Here, we show that devices made by subtractive patterning show a systematic absence of the GCS effect. Doing a microstructural analysis of these devices and comparing them to devices made by additive patterning, where we observe a GCS, we identify some material and physical parameters that are crucial for the observation of a GCS. We also show that some of the mechanisms proposed to explain the origin of the GCS effect are not universally relevant., Comment: 19 pages, 3 figures. arXiv admin note: substantial text overlap with arXiv:2302.13734

A distributed quantum computing system requires a quantum communication channel between spatially separated processing units. In superconducting circuits, such a channel can be realized by using propagating microwave photons to encode and transfer quantum information between an emitter and a receiver node. Here we experimentally demonstrate a superconducting circuit that deterministically transfers the state of a data qubit into a propagating microwave mode, with a process fidelity of 94.5%. We use a time-varying parametric drive to shape the temporal profile of the propagating mode to be time-symmetric and with constant phase, so that reabsorption by the receiving processor can be implemented as a time-reversed version of the emission. We demonstrate a self-calibrating routine to correct for time-dependent shifts of the emitted frequencies due to the modulation of the parametric drive. Our work provides a reliable method to implement high-fidelity quantum state transfer and remote entanglement operations in a distributed quantum computing network.

Encoding quantum information into superpositions of multiple Fock states of a harmonic oscillator can provide protection against errors, but it comes with the cost of requiring more complex quantum gates that need to address multiple Fock states simultaneously. Therefore, characterizing the quantum process fidelity of these gates also becomes more challenging. Here, we demonstrate the use of coherent-state quantum process tomography (csQPT) for a bosonic-mode superconducting circuit. CsQPT uses coherent states as input probes for the quantum process in order to completely characterize the quantum operation for an arbitrary input state. We show results for this method by characterizing a logical quantum gate constructed using displacement and SNAP operations on an encoded qubit. With csQPT, we are able to reconstruct the Kraus operators for the larger Hilbert space rather than being limited to the logical subspace. This allows for a more accurate determination of the different error mechanisms that lead to the gate infidelity.

In conventional metal-oxide semiconductor (CMOS) electronics, the logic state of a device is set by a gate voltage (VG). The superconducting equivalent of such effect had remained unknown until it was recently shown that a VG can tune the superconducting current (supercurrent) flowing through a nanoconstriction in a superconductor. This gate-controlled supercurrent (GCS) effect can lead to superconducting logics like CMOS logics, but with lower energy dissipation. The physical mechanism underlying the GCS effect, however, remains under debate. In this review article, we illustrate the main mechanisms proposed for the GCS effect, and the material and device parameters that mostly affect it based on the evidence reported. We will come to the conclusion that different mechanisms are at play in the different studies reported so far. We then outline studies that can help answer open questions on the effect and achieve control over it, which is key for applications. We finally give insights into the impact that the GCS effect can have towards high-performance computing with low-energy dissipation and quantum technologies., Comment: 54 pages, 16 figures, 4 tables

Bosonic quantum error correcting codes are primarily designed to protect against single-photon loss. To correct for this type of error, one can encode the logical qubit in code spaces with a definite photon parity, such as cat codes or binomial codes. Error correction requires a recovery operation that maps the error states -- which have opposite parity -- back onto the code states. Here, we realize a collection of photon-number-selective, simultaneous photon addition operations on a bosonic mode, a microwave cavity, assisted by a superconducting qubit. These operations are implemented as two-photon transitions that excite the cavity and the qubit at the same time. The additional degree of freedom of the qubit makes it possible to implement a coherent, unidirectional mapping between spaces of opposite photon parity. We present the successful experimental implementation of the drives and the phase control they enable on superpositions of Fock states. The presented technique, when supplemented with qubit reset, is suitable for autonomous quantum error correction in bosonic systems, and, more generally, opens the possibility to realize a range of non-unitary transformations on a bosonic mode.

We describe a digital microwave platform called Presto, designed for measurement and control of multiple quantum bits (qubits) and based on the third-generation radio-frequency system on a chip. Presto uses direct digital synthesis to create signals up to 9 GHz on 16 synchronous output ports, while synchronously analyzing response on 16 input ports. Presto has 16 DC-bias outputs, 4 inputs and 4 outputs for digital triggers or markers, and two continuous-wave outputs for synthesizing frequencies up to 15 GHz. Scaling to a large number of qubits is enabled through deterministic synchronization of multiple Presto units. A Python application programming interface configures a firmware for synthesis and analysis of pulses, coordinated by an event sequencer. The analysis integrates template matching (matched filtering) and low-latency (184 - 254 ns) feedback to enable a wide range of multi-qubit experiments. We demonstrate Presto's capabilities with experiments on a sample consisting of two superconducting qubits connected via a flux-tunable coupler. We show single-shot readout and active reset of a single qubit; randomized benchmarking of single-qubit gates showing 99.972% fidelity, limited by the coherence time of the qubit; and calibration of a two-qubit iSWAP gate., Comment: v3: peer reviewed, accepted manuscript; v2: correct theoretical gate fidelity in Sec. III C

A new type of low-pass filter based on a leaky coaxial waveguide is presented. The filter has minimal insertion loss in the pass band, while at the same time high attenuation in the stop band is achieved. Thanks to its arrangement, the filter does not present parasitic leakage paths, so that, unlike conventional resonant filters, the stop band extends to very high frequencies. It is shown that a particular stop-band attenuation can be obtained by adding or removing leaking sections. Coupling between the center coaxial structure and the leaking holes is investigated. A prototype is manufactured and scattering parameters are measured up to 145 GHz. The prototype shows an insertion loss of less than 0.15 dB up to 10 GHz and an attenuation in excess of 60 dB above 70 GHz. The proposed filter is suitable for superconducting quantum computing applications where qubits are sensitive to radiation with energy high enough to break Cooper-pairs, thereby destroying superconductivity.

Tailoring the decay rate of structured quantum emitters into their environment opens new avenues for nonlinear quantum optics, collective phenomena, and quantum communications. Here we demonstrate a novel coupling scheme between an artificial molecule comprising two identical, strongly coupled transmon qubits, and two microwave waveguides. In our scheme, the coupling is engineered so that transitions between states of the same (opposite) symmetry, with respect to the permutation operator, are predominantly coupled to one (the other) waveguide. The symmetry-based coupling selectivity, as quantified by the ratio of the coupling strengths, exceeds a factor of 30 for both the waveguides in our device. In addition, we implement a two-photon Raman process activated by simultaneously driving both waveguides, and show that it can be used to coherently couple states of different symmetry in the single-excitation manifold of the molecule. Using that process, we implement frequency conversion across the waveguides, mediated by the molecule, with efficiency of about 95%. Finally, we show that this coupling arrangement makes it possible to straightforwardly generate spatially-separated Bell states propagating across the waveguides. We envisage further applications to quantum thermodynamics, microwave photodetection, and photon-photon gates.

Hosting non-classical states of light in three-dimensional microwave cavities has emerged as a promising paradigm for continuous-variable quantum information processing. Here we experimentally demonstrate high-fidelity generation of a range of Wigner-negative states useful for quantum computation, such as Schr\"{o}dinger-cat states, binomial states, Gottesman-Kitaev-Preskill (GKP) states, as well as cubic phase states. The latter states have been long sought after in quantum optics and were never achieved experimentally before. To do so, we use a sequence of interleaved selective number-dependent arbitrary phase (SNAP) gates and displacements. We optimize the state preparation in two steps. First we use a gradient-descent algorithm to optimize the parameters of the SNAP and displacement gates. Then we optimize the envelope of the pulses implementing the SNAP gates. Our results show that this way of creating highly non-classical states in a harmonic oscillator is robust to fluctuations of the system parameters such as the qubit frequency and the dispersive shift.

We observe the continuous emission of photons into a waveguide from a superconducting qubit without the application of an external drive. To explain this observation, we build a two-bath model where the qubit couples simultaneously to a cold bath (the waveguide) and a hot bath (a secondary environment). Our results show that the thermal-photon occupation of the hot bath is up to 0.14 photons, 35 times larger than the cold waveguide, leading to nonequilibrium heat transport with a power of up to 132 zW, as estimated from the qubit emission spectrum. By adding more isolation between the sample output and the first cold amplifier in the output line, the heat transport is strongly suppressed. Our interpretation is that the hot bath may arise from active two-level systems being excited by noise from the output line. We also apply a coherent drive, and use the waveguide to measure thermodynamic work and heat, suggesting waveguide spectroscopy is a useful means to study quantum heat engines and refrigerators. Finally, based on the theoretical model, we propose how a similar setup can be used as a noise spectrometer which provides a new solution for calibrating the background noise of hybrid quantum systems.

Engineering the electromagnetic environment of a quantum emitter gives rise to a plethora of exotic light-matter interactions. In particular, photonic lattices can seed long-lived atom-photon bound states inside photonic band gaps. Here we report on the concept and implementation of a novel microwave architecture consisting of an array of compact, high-impedance superconducting resonators forming a 1 GHz-wide pass band, in which we have embedded two frequency-tuneable artificial atoms. We study the atom-field interaction and access previously unexplored coupling regimes, in both the single- and double-excitation subspace. In addition, we demonstrate coherent interactions between two atom-photon bound states, in both resonant and dispersive regimes, that are suitable for the implementation of SWAP and CZ two-qubit gates. The presented architecture holds promise for quantum simulation with tuneable-range interactions and photon transport experiments in nonlinear regime.

We experimentally demonstrate the steady-state generation of propagating Wigner-negative states from a continuously driven superconducting qubit. We reconstruct the Wigner function of the radiation emitted into propagating modes defined by their temporal envelopes, using digital filtering. For an optimized temporal filter, we observe a large Wigner logarithmic negativity, in excess of 0.08, in agreement with theory. The fidelity between the theoretical predictions and the states generated experimentally is up to 99%, reaching state-of-the-art realizations in the microwave frequency domain. Our results provide a new way to generate and control nonclassical states, and may enable promising applications such as quantum networks and quantum computation based on waveguide quantum electrodynamics., Comment: 15

The ability to control and measure the temperature of propagating microwave modes down to very low temperatures is indispensable for quantum information processing, and may open opportunities for studies of heat transport at the nanoscale, also in the quantum regime. Here we propose and experimentally demonstrate primary thermometry of propagating microwaves using a transmon-type superconducting circuit. Our device operates continuously, with a sensitivity down to $4\times 10^{-4}$ photons/$\sqrt{\mbox{Hz}}$ and a bandwidth of 40 MHz. We measure the thermal occupation of the modes of a highly attenuated coaxial cable in a range of 0.001 to 0.4 thermal photons, corresponding to a temperature range from 35 mK to 210 mK at a frequency around 5 GHz. To increase the radiation temperature in a controlled fashion, we either inject calibrated, wideband digital noise, or heat the device and its environment. This thermometry scheme can find applications in benchmarking and characterization of cryogenic microwave setups, temperature measurements in hybrid quantum systems, and quantum thermodynamics.

We provide an explicit construction of a universal gate set for continuous-variable quantum computation with microwave circuits. Such a universal set has been first proposed in quantum-optical setups, but its experimental implementation has remained elusive in that domain due to the difficulties in engineering strong nonlinearities. Here, we show that a realistic three-wave mixing microwave architecture based on the SNAIL [Frattini et al., Appl. Phys. Lett. 110, 222603 (2017)] allows us to overcome this difficulty. As an application, we show that this architecture allows for the generation of a cubic phase state with an experimentally feasible procedure. This work highlights a practical advantage of microwave circuits with respect to optical systems for the purpose of engineering non-Gaussian states, and opens the quest for continuous-variable algorithms based on few repetitions of elementary gates from the continuous-variable universal set., Comment: accepted version

The parity of the number of elementary excitations present in a quantum system provides important insights into its physical properties. Parity measurements are used, for example, to tomographically reconstruct quantum states or to determine if a decay of an excitation has occurred, information which can be used for quantum error correction in computation or communication protocols. Here we demonstrate a versatile parity detector for propagating microwaves, which distinguishes between radiation fields containing an even or odd number n of photons, both in a single-shot measurement and without perturbing the parity of the detected field. We showcase applications of the detector for direct Wigner tomography of propagating microwaves and heralded generation of Schr\"odinger cat states. This parity detection scheme is applicable over a broad frequency range and may prove useful, for example, for heralded or fault-tolerant quantum communication protocols.

We experimentally investigate a superconducting qubit coupled to the end of an open transmission line, in a regime where the qubit decay rates to the transmission line and to its own environment are comparable. We perform measurements of coherent and incoherent scattering, on- and off-resonant fluorescence, and time-resolved dynamics to determine the decay and decoherence rates of the qubit. In particular, these measurements let us discriminate between non-radiative decay and pure dephasing. We combine and contrast results across all methods and find consistent values for the extracted rates. The results show that the pure dephasing rate is one order of magnitude smaller than the non-radiative decay rate for our qubit. Our results indicate a pathway to benchmark decoherence rates of superconducting qubits in a resonator-free setting., Comment: 13 pages, 6 figures

Multi-photon emitters are a sought-after resource in quantum photonics. Nonlinear interactions between a multi-level atomic system and a coherent drive can lead to resonant two-photon emission, but harvesting light from this process has remained a challenge due to the small oscillator strengths involved. Here we present a study of two-photon resonance fluorescence at microwave frequencies, using a superconducting, ladder-type artificial atom, a transmon, strongly coupled to a waveguide. We drive the two-photon transition between the ground and second-excited state at increasingly high powers and observe a resonance fluorescence peak whose intensity becomes comparable to single-photon emission until it splits into a Mollow-like triplet. We measure photon correlations of frequency-filtered spectral lines and find that while emission at the fundamental frequency stays antibunched, the resonance fluorescence peak at the two-photon transition is superbunched. Our results provide a route towards the realization of multi-photon sources in the microwave domain.

Heralding techniques are useful in quantum communication to circumvent losses without resorting to error correction schemes or quantum repeaters. Such techniques are realized, for example, by monitoring for photon loss at the receiving end of the quantum link while not disturbing the transmitted quantum state. We describe and experimentally benchmark a scheme that incorporates error detection in a quantum channel connecting two transmon qubits using traveling microwave photons. This is achieved by encoding the quantum information as a time-bin superposition of a single photon, which simultaneously realizes high communication rates and high fidelities. The presented scheme is straightforward to implement in circuit QED and is fully microwave-controlled, making it an interesting candidate for future modular quantum computing architectures.

Networks of nonlinear resonators offer intriguing perspectives as quantum simulators for non-equilibrium many-body phases of driven-dissipative systems. Here, we employ photon correlation measurements to study the radiation fields emitted from a system of two superconducting resonators, coupled nonlinearly by a superconducting quantum interference device (SQUID). We apply a parametrically modulated magnetic flux to control the linear photon hopping rate between the two resonators and its ratio with the cross-Kerr rate. When increasing the hopping rate, we observe a crossover from an ordered to a delocalized state of photons. The presented coupling scheme is intrinsically robust to frequency disorder and may therefore prove useful for realizing larger-scale resonator arrays.

The duration and fidelity of qubit readout is a critical factor for applications in quantum information processing as it limits the fidelity of algorithms which reuse qubits after measurement or apply feedback based on the measurement result. Here we present fast multiplexed readout of five qubits in a single 1.2 GHz wide readout channel. Using a readout pulse length of 80 ns and populating readout resonators for less than 250 ns we find an average correct assignment probability for the five measured qubits to be $97\%$. The differences between the individual readout errors and those found when measuring the qubits simultaneously are within $1\%$. We employ individual Purcell filters for each readout resonator to suppress off-resonant driving, which we characterize by the dephasing imposed on unintentionally measured qubits. We expect the here presented readout scheme to become particularly useful for the selective readout of individual qubits in multi-qubit quantum processors., Comment: 13 pages, 10 figures

Active qubit reset is a key operation in many quantum algorithms, and particularly in error correction codes. Here, we experimentally demonstrate a reset scheme of a three level transmon artificial atom coupled to a large bandwidth resonator. The reset protocol uses a microwave-induced interaction between the $|f,0\rangle$ and $|g,1\rangle$ states of the coupled transmon-resonator system, with $|g\rangle$ and $|f\rangle$ denoting the ground and second excited states of the transmon, and $|0\rangle$ and $|1\rangle$ the photon Fock states of the resonator. We characterize the reset process and demonstrate reinitialization of the transmon-resonator system to its ground state with $0.2\%$ residual excitation in less than $500 \, \rm{ns}$. Our protocol is of practical interest as it has no requirements on the architecture, beyond those for fast and efficient single-shot readout of the transmon, and does not require feedback.

Sharing information coherently between nodes of a quantum network is at the foundation of distributed quantum information processing. In this scheme, the computation is divided into subroutines and performed on several smaller quantum registers connected by classical and quantum channels. A direct quantum channel, which connects nodes deterministically, rather than probabilistically, is advantageous for fault-tolerant quantum computation because it reduces the threshold requirements and can achieve larger entanglement rates. Here, we implement deterministic state transfer and entanglement protocols between two superconducting qubits fabricated on separate chips. Superconducting circuits constitute a universal quantum node capable of sending, receiving, storing, and processing quantum information. Our implementation is based on an all-microwave cavity-assisted Raman process which entangles or transfers the qubit state of a transmon-type artificial atom to a time-symmetric itinerant single photon. We transfer qubit states at a rate of $50 \, \rm{kHz}$ using the emitted photons which are absorbed at the receiving node with a probability of $98.1 \pm 0.1 \%$ achieving a transfer process fidelity of $80.02 \pm 0.07 \%$. We also prepare on demand remote entanglement with a fidelity as high as $78.9 \pm 0.1 \%$. Our results are in excellent agreement with numerical simulations based on a master equation description of the system. This deterministic quantum protocol has the potential to be used as a backbone of surface code quantum error correction across different nodes of a cryogenic network to realize large-scale fault-tolerant quantum computation in the circuit quantum electrodynamic architecture., Comment: 11 pages 8 Figures

Single-photon detection is an essential component in many experiments in quantum optics, but remains challenging in the microwave domain. We realize a quantum non-demolition detector for propagating microwave photons and characterize its performance using a single-photon source. To this aim we implement a cavity-assisted conditional phase gate between the incoming photon and a superconducting artificial atom. By reading out the state of this atom in single shot, we reach an internal photon detection fidelity of 71%, limited by the coherence properties of the qubit. By characterizing the coherence and average number of photons in the field reflected off the detector, we demonstrate its quantum non-demolition nature. We envisage applications in generating heralded remote entanglement between qubits and for realizing logic gates between propagating microwave photons.

The process of photosynthesis, the main source of energy in the animate world, converts sunlight into chemical energy. The surprisingly high efficiency of this process is believed to be enabled by an intricate interplay between the quantum nature of molecular structures in photosynthetic complexes and their interaction with the environment. Investigating these effects in biological samples is challenging due to their complex and disordered structure. Here we experimentally demonstrate a new approach for studying photosynthetic models based on superconducting quantum circuits. In particular, we demonstrate the unprecedented versatility and control of our method in an engineered three-site model of a pigment protein complex with realistic parameters scaled down in energy by a factor of $10^5$. With this system we show that the excitation transport between quantum coherent sites disordered in energy can be enabled through the interaction with environmental noise. We also show that the efficiency of the process is maximized for structured noise resembling intramolecular phononic environments found in photosynthetic complexes., Comment: 8+12 pages, 4+12 figures

An excited emitter decays by radiating a photon into a quantized mode of the electromagnetic field, a process known as spontaneous emission. If the emitter is driven to a higher excited state, it radiates multiple photons in a cascade decay. Atomic and biexciton cascades have been exploited as sources of polarization-entangled photon pairs. Because the photons are emitted sequentially, their intensities are strongly correlated in time, as measured in a double-beam coincidence experiment. Perhaps less intuitively, their phases can also be correlated, provided a single emitter is deterministically prepared into a superposition state, and the emitted radiation is detected in a phase-sensitive manner and with high efficiency. Here we have met these requirements by using a superconducting artificial atom, coherently driven to its second-excited state and decaying into a well-defined microwave mode. Our results highlight the coherent nature of cascade decay and demonstrate a novel protocol to generate entanglement between itinerant field modes.

The strong coupling limit of cavity quantum electrodynamics (QED) implies the capability of a matter-like quantum system to coherently transform an individual excitation into a single photon within a resonant structure. This not only enables essential processes required for quantum information processing but also allows for fundamental studies of matter-light interaction. In this work we demonstrate strong coupling between the charge degree of freedom in a gate-detuned GaAs double quantum dot (DQD) and a frequency-tunable high impedance resonator realized using an array of superconducting quantum interference devices (SQUIDs). In the resonant regime, we resolve the vacuum Rabi mode splitting of size $2g/2\pi = 238$ MHz at a resonator linewidth $\kappa/2\pi = 12$ MHz and a DQD charge qubit dephasing rate of $\gamma_2/2\pi = 80$ MHz extracted independently from microwave spectroscopy in the dispersive regime. Our measurements indicate a viable path towards using circuit based cavity QED for quantum information processing in semiconductor nano-structures.

Thermal Markovian dynamics is typically obtained by coupling a system to a sufficiently hot bath with a large heat capacity. Here we present a scheme for inducing Markovian dynamics using an arbitrarily small and cold heat bath. The scheme is based on injecting phase noise to the small bath. Several unique signatures of small bath are studied. We discuss realizations in ion traps and superconducting qubits and show that it is possible to create an ideal setting where the system dynamics is indifferent to the internal bath dynamics., Comment: V2 contains new contributions by the new authors SG and RO about experimental realization in superconducting circuits and ion traps. In addition, the discussion on system-bath correlation in V2 was extended. The study of generalized Gibbs states was omitted in V2, but can still be found in V1. More generally, V2 is a clearer and more concise version

What is the role of coherence in determining the distribution of work done on a quantum system? We approach this question from an operational perspective and consider a setup in which the internal energy of a closed system is recorded by a quantum detector before and after the system is acted upon by an external drive. We find that the resulting work distribution depends on the initial state of the detector as well as on the choice of the final measurement. We consider two complementary measurement schemes, both of which show clear signatures of quantum interference. We specifically discuss how to implement these schemes in the circuit QED architecture, using an artificial atom as the system and a quantized mode of the electromagnetic field as the detector. Different measurement schemes can be realized by preparing the field either in a superposition of Fock states or in a coherent state and exploiting state-of-the art techniques for the characterization of microwave radiation at the quantum level. More generally, the single bosonic mode we utilize is arguably the minimal quantum detector capable of capturing the complementary aspects of the work distribution discussed here., Comment: 12 pages, 3 figures

Berry's geometric phase naturally appears when a quantum system is driven by an external field whose parameters are slowly and cyclically changed. A variation in the coupling between the system and the external field can also give rise to a geometric phase, even when the field is in the vacuum state or any other Fock state. Here we demonstrate the appearance of a vacuum-induced Berry phase in an artificial atom, a superconducting transmon, interacting with a single mode of a microwave cavity. As we vary the phase of the interaction, the artificial atom acquires a geometric phase determined by the path traced out in the combined Hilbert space of the atom and the quantum field. Our ability to control this phase opens new possibilities for the geometric manipulation of atom-cavity systems also in the context of quantum information processing., Comment: 5 + 6 pages

We discuss work performed on a quantum two-level system coupled to multiple thermal baths. To evaluate the work, a measurement of photon exchange between the system and the baths is envisioned. In a realistic scenario, some photons remain unrecorded as they are exchanged with baths that are not accessible to the measurement, and thus only partial information on work and heat is available. The incompleteness of the measurement leads to substantial deviations from standard fluctuation relations. We propose a recovery of these relations, based on including the mutual information given by the counting efficiency of the partial measurement. We further present the experimental status of a possible implementation of the proposed scheme, i.e. a calorimetric measurement of work, currently with nearly single-photon sensitivity.

It is shown that strong driving of a quantum system substantially enhances the Lamb shift induced by broadband reservoirs which are typical for solid-state devices. By varying drive parameters the impact of environmental vacuum fluctuations with continuous spectral distribution onto system observables can be tuned in a distinctive way. This provides experimentally feasible measurement schemes for the Lamb shift in superconducting circuits based on Cooper pair boxes, where it can be detected either in shifted dressed transition frequencies or in pumped charge currents., Comment: 5 pages, 4 figures + 4 pages supplemental material

We demonstrate local detection of the electron temperature in a two-dimensionalmicrodomain using a quantum dot. Our method relies on the observation that a temperature bias across the dot changes the functional form of Coulomb-blockade peaks. We apply our results to the investigation of electron-energy relaxation at subkelvin temperatures, find that the energy flux from electrons into phonons is proportional to the fifth power of temperature, and give a measurement of the coupling constant., Comment: 5 pages, 4 figures