Search

We present a search for neutrinoless double-beta ($0\nu\beta\beta$) decay of $^{136}$Xe using the full KamLAND-Zen 800 dataset with 745 kg of enriched xenon, corresponding to an exposure of $2.097$ ton yr of $^{136}$Xe. This updated search benefits from a more than twofold increase in exposure, recovery of photo-sensor gain, and reduced background from muon-induced spallation of xenon. Combining with the search in the previous KamLAND-Zen phase, we obtain a lower limit for the $0\nu\beta\beta$ decay half-life of $T_{1/2}^{0\nu} > 3.8 \times 10^{26}$ yr at 90% C.L., a factor of 1.7 improvement over the previous limit. The corresponding upper limits on the effective Majorana neutrino mass are in the range 28-122 meV using phenomenological nuclear matrix element calculations., Comment: arXiv admin note: text overlap with arXiv:2203.02139

We have established a method to measure picograms-per-gram (pg g$^{-1}$) levels of $^{238}$U and $^{232}$Th in scintillation films by combining the dry ashing method and inductively coupled plasma mass spectrometry. Trace amounts of $^{238}$U and $^{232}$Th were measured in up to 2~g of the scintillation film with almost 100% collection efficiency. This paper details the experimental procedure, including the pretreatment of the samples and labware, detection limit of the method, collection efficiencies of $^{238}$U and $^{232}$Th, and measurement of $^{238}$U and $^{232}$Th in a polyethylene naphthalate film. This method is also applicable to $^{238}$U and $^{232}$Th measurements in other low-background organic materials for rare event search experiments.

Particle dark matter could belong to a multiplet that includes an electrically charged state. WIMP dark matter ($\chi^{0}$) accompanied by a negatively charged excited state ($\chi^{-}$) with a small mass difference (e.g. $<$ 20 MeV) can form a bound-state with a nucleus such as xenon. This bound-state formation is rare and the released energy is $\mathcal{O}(1-10$) MeV depending on the nucleus, making large liquid scintillator detectors suitable for detection. We searched for bound-state formation events with xenon in two experimental phases of the KamLAND-Zen experiment, a xenon-doped liquid scintillator detector. No statistically significant events were observed. For a benchmark parameter set of WIMP mass $m_{\chi^{0}} = 1$ TeV and mass difference $\Delta m = 17$ MeV, we set the most stringent upper limits on the recombination cross section times velocity $\langle\sigma v\rangle$ and the decay-width of $\chi^{-}$ to $9.2 \times 10^{-30}$ ${\rm cm^3/s}$ and $8.7 \times 10^{-14}$ GeV, respectively at 90% confidence level.

A new ultra-low background high-purity germanium (HPGe) detector has been installed at the Kamioka underground experimental site. The background count rate in the energy range from 40 keV to 2700 keV is about 25% lower than that of the first HPGe detector installed in 2016, which has the same detector specification and similar shielding geometry. This paper describes the shielding configuration, including the cleaning of the material surface, the comparison of calibration data and simulation, the time variation of the background spectra, the sample measurement procedure, and some results of the radioactivity in the selected samples.

Cosmic-ray muons produce various radioisotopes when passing through material. These spallation products can be backgrounds for rare event searches such as in solar neutrino, double-beta decay, and dark matter search experiments. The KamLAND-Zen experiment searches for neutrinoless double-beta decay in 745kg of xenon dissolved in liquid scintillator. The experiment includes dead-time-free electronics with a high efficiency for detecting muon-induced neutrons. The production yields of different radioisotopes are measured with a combination of delayed coincidence techniques, newly developed muon reconstruction and xenon spallation identification methods. The observed xenon spallation products are consistent with results from the FLUKA and Geant4 simulation codes.

We report a measurement of the strange axial coupling constant $g_A^s$ using atmospheric neutrino data at KamLAND. This constant is a component of the axial form factor of the neutral-current quasielastic (NCQE) interaction. The value of $g_A^s$ significantly changes the ratio of proton and neutron NCQE cross sections. KamLAND is suitable for measuring NCQE interactions as it can detect nucleon recoils with low-energy thresholds and measure neutron multiplicity with high efficiency. KamLAND data, including the information on neutron multiplicity associated with the NCQE interactions, makes it possible to measure $g_A^s$ with a suppressed dependence on the axial mass $M_A$, which has not yet been determined. For a comprehensive prediction of the neutron emission associated with neutrino interactions, we establish a simulation of particle emission via nuclear deexcitation of $^{12}$C, a process not considered in existing neutrino Monte Carlo event generators. Energy spectrum fitting for each neutron multiplicity gives $g_A^s =-0.14^{+0.25}_{-0.26}$, which is the most stringent limit obtained using NCQE interactions without $M_A$ constraints. The two-body current contribution considered in this analysis relies on a theoretically effective model and electron scattering experiments and requires future verification by direct measurements and future model improvement.

The decay of the primordial isotopes $^{238}\mathrm{U}$, $^{235}\mathrm{U}$, $^{232}\mathrm{Th}$, and $^{40}\mathrm{K}$ have contributed to the terrestrial heat budget throughout the Earth's history. Hence the individual abundance of those isotopes are key parameters in reconstructing contemporary Earth model. The geoneutrinos produced by the radioactive decays of uranium and thorium have been observed with the Kamioka Liquid-Scintillator Antineutrino Detector (KamLAND). Those measurements have been improved with more than 18-year observation time, and improvements in detector background levels mainly by an 8-year almost rector-free period now permit spectroscopy with geoneutrinos. Our results yield the first constraint on both uranium and thorium heat contributions. Herein the KamLAND result is consistent with geochemical estimations based on elemental abundances of chondritic meteorites and mantle peridotites. The High-Q model is disfavored at 99.76% C.L. and a fully radiogenic model is excluded at 5.2$\sigma$ assuming a homogeneous heat producing element distribution in the mantle., Comment: 13 pages, 2 figures, accepted for publication in Geophysical Research Letters on Aug 4th, 2022

We present the results of a search for core-collapse supernova neutrinos, using long-term KamLAND data from 2002 March 9 to 2020 April 25. We focus on the electron antineutrinos emitted from supernovae in the energy range of 1.8--111 MeV. Supernovae will make a neutrino event cluster with the duration of $\sim$10 s in the KamLAND data. We find no neutrino clusters and give the upper limit on the supernova rate as to be 0.15 yr$^{-1}$ with a 90% confidence level. The detectable range, which corresponds to a >95% detection probability, is 40--59 kpc and 65--81 kpc for core-collapse supernovae and failed core-collapse supernovae, respectively. This paper proposes to convert the supernova rate obtained by the neutrino observation to the Galactic star formation rate. Assuming a modified Salpeter-type initial mass function, the upper limit on the Galactic star formation rate is <(17.5--22.7) $M_{\odot} \mathrm{yr}^{-1}$ with a 90% confidence level., Comment: 10 pages, 4 figures, accepted for publication in Astrophysical Journal

The KamLAND-Zen experiment has provided stringent constraints on the neutrinoless double-beta ($0\nu\beta\beta$) decay half-life in $^{136}$Xe using a xenon-loaded liquid scintillator. We report an improved search using an upgraded detector with almost double the amount of xenon and an ultralow radioactivity container, corresponding to an exposure of 970 kg yr of $^{136}$Xe. These new data provide valuable insight into backgrounds, especially from cosmic muon spallation of xenon, and have required the use of novel background rejection techniques. We obtain a lower limit for the $0\nu\beta\beta$ decay half-life of $T_{1/2}^{0\nu} > 2.3 \times 10^{26}$ yr at 90% C.L., corresponding to upper limits on the effective Majorana neutrino mass of 36-156 meV using commonly adopted nuclear matrix element calculations., Comment: 7 pages, 3 figures

We report the results of a search for MeV-scale astrophysical neutrinos in KamLAND presented as an excess in the number of coincident neutrino interactions associated with the publicly available high-energy neutrino datasets from the IceCube Neutrino Observatory. We find no statistically significant excess in the number of observed low-energy electron antineutrinos in KamLAND, given a coincidence time window of $\pm$500s, $\pm$1,000s, $\pm$3,600s, and $\pm$10,000s around each of the IceCube neutrinos. We use this observation to present limits from 1.8 MeV to 100 MeV on the electron antineutrino fluence, assuming a mono-energetic flux. We then compare the results to several astrophysical measurements performed by IceCube and place a limit at the 90% confidence level on the electron antineutrino isotropic thermal luminosity from the TXS 0506+056 blazar., Comment: 12 pages, 5 figures

We present the results of a time-coincident event search for low-energy electron antineutrinos in the KamLAND detector with gamma-ray bursts from the Gamma-ray Coordinates Network and Fermi Gamma-ray Burst Monitor. Using a variable coincidence time window of $\pm$500s plus the duration of each gamma-ray burst, no statistically significant excess above background is observed. We place the world's most stringent 90% confidence level upper limit on the electron antineutrino fluence below 17.5 MeV. Assuming a Fermi-Dirac neutrino energy spectrum from the gamma-ray burst source, we use the available redshift data to constrain the electron antineutrino luminosity and effective temperature., Comment: 9 pages, 3 figures

We report on a search for electron antineutrinos ($\bar{\nu}_e$) from astrophysical sources in the neutrino energy range 8.3 to 30.8 MeV with the KamLAND detector. In an exposure of 6.72 kton-year of the liquid scintillator, we observe 18 candidate events via the inverse beta decay reaction. Although there is a large background uncertainty from neutral current atmospheric neutrino interactions, we find no significant excess over background model predictions. Assuming several supernova relic neutrino spectra, we give upper flux limits of 60--110 cm$^{-2}$ s$^{-1}$ (90% CL) in the analysis range and present a model-independent flux. We also set limits on the annihilation rates for light dark matter pairs to neutrino pairs. These data improves on the upper probability limit of $^{8}$B solar neutrinos converting into $\bar{\nu}_e$'s, $P_{\nu_e \rightarrow \bar{\nu}_e} < 3.5\times10^{-5}$ (90% CL) assuming an undistorted $\bar{\nu}_e$ shape. This corresponds to a solar $\bar{\nu}_e$ flux of 60 cm$^{-2}$ s$^{-1}$ (90% CL) in the analysis energy range., Comment: 21 pages, 9 figures, 4 tables, accepted for publication in Astrophysical Journal

We report the result of a search for neutrinos in coincidence with solar flares from the GOES flare database. The search was performed on a 10.8 kton-year exposure of KamLAND collected from 2002 to 2019. This large exposure allows us to explore previously unconstrained parameter space for solar flare neutrinos. We found no statistical excess of neutrinos and established 90% confidence level upper limits of $8.4 \times 10^7$ cm$^{-2}$ ($3.0 \times 10^{9}$ cm$^{-2}$) on electron anti-neutrino (electron neutrino) fluence at 20 MeV normalized to the X12 flare, assuming that the neutrino fluence is proportional to the X-ray intensity., Comment: 13 pages, 9 figures, accepted October 27, 2021

The KamLAND-Zen 800 experiment is searching for the neutrinoless double-beta decay of $^{136}$Xe by using $^{136}$Xe-loaded liquid scintillator. The liquid scintillator is enclosed inside a balloon made of thin, transparent, low-radioactivity film that we call Inner Balloon (IB). The IB, apart from guaranteeing the liquid containment, also allows to minimize the background from cosmogenic muon-spallation products and $^{8}$B solar neutrinos. Indeed these events could contribute to the total counts in the region of interest around the Q-value of the double-beta decay of $^{136}$Xe. In this paper, we present an overview of the IB and describe the various steps of its commissioning minimizing the radioactive contaminations, from the material selection, to the fabrication of the balloon and its installation inside the KamLAND detector. Finally, we show the impact of the IB on the KamLAND background as measured by the KamLAND detector itself., Comment: 23 pages, 16 figures, to be submitted to JINST

There are many theories where a dark matter particle is part of a multiplet with an electrically charged state. If WIMP dark matter ($\chi^{0}$) is accompanied by a charged excited state ($\chi^{-}$) separated by a small mass difference, it can form a stable bound state with a nucleus. In supersymmetric models, the $\chi^{0}$ and the $\chi^{-}$ could be the neutralino and a charged slepton, such as the neutralino-stau degenerate model. The formation binding process is expected to result in an energy deposition of {\it O}(1--10 MeV), making it suitable for detection in large liquid scintillator detectors. We describe new constraints on the bound state formation with a xenon nucleus using the KamLAND-Zen 400 Phase-II dataset. In order to enlarge the searchable parameter space, all xenon isotopes in the detector were used. For a benchmark parameter set of $m_{\chi^{0}} = 100$ GeV and $\Delta m = 10$ MeV, this study sets the most stringent upper limits on the recombination cross section $\langle\sigma v\rangle$ and the decay-width of $\chi^{-}$ of $2.0 \times 10^{-31}$ ${\rm cm^3/s}$ and $1.1 \times 10^{-18}$ GeV, respectively (90\% confidence level).

We present the results of a search for MeV-scale electron antineutrino events in KamLAND in coincident with the 60 gravitational wave events/candidates reported by the LIGO/Virgo collaboration during their second and third observing runs. We find no significant coincident signals within a $\pm$ 500 s timing window from each gravitational wave and present 90% C.L. upper limits on the electron antineutrino fluence between $10^{8}$-$10^{13}\,{\mathrm cm^2}$ for neutrino energies in the energy range of 1.8-111 MeV., Comment: 11 pages, 2 figures, 2 tables, Accepted for publication in ApJ

A liquid scintillator base experiment KamLAND-Zen has set a lower limit on neutrinoless double beta decay half-life, and upgrade project KamLAND-Zen 800 has started in 2019. Unfortunately, this project expects some backgrounds, and one of the main backgrounds is beta/gamma-ray from 214Bi in container of xenon loaded liquid scintillator (mini-balloon). In order to reject the background, we suggest using scintillation film for the future mini-balloon. If we can tag alpha-ray from 214Po by scintillation detection, we can eliminate 214Bi events by delayed coincidence analysis. Recently, it was reported that polyethylene naphthalate (PEN) can be used as a scintillator with blue photon emission. PEN has chemical compatibility for strong solvent, thus it has a possibility to use in liquid scintillator. In this presentation, we will mention the results for feasibility studies about transparency and emission spectra, light yield, radioactivity, strength of film etc.. We also show the test-sized scintillation balloon with an 800-mm diameter and discussions about how to use the scintillation balloon in KamLAND., Comment: 3 pages, 4 figures, Proceedings of the 16th International Conference on Topics in Astroparticle and Underground Physics (TAUP 2019), September 9-13, 2019, Toyama, Japan

Environmental radioactivity is a dominant background for rare decay search experiments, and it is difficult to completely remove such an impurity from detector vessels. We propose a scintillation balloon as the active vessel of a liquid scintillator in order to identify this undesirable radioactivity. According to our feasibility studies, the scintillation balloon enables the bismuth--polonium sequential decay to be tagged with a 99.7\% efficiency, assuming a KamLAND (Kamioka Liquid scintillator AntiNeutrino Detector)-type liquid scintillator detector. This tagging of sequential decay using alpha-ray from the polonium improves the sensitivity to neutrinoless double-beta decay with rejecting beta-ray background from the bismuth., Comment: 11 pages, 9 figures

We present a search for low energy antineutrino events coincident with the gravitational wave events GW150914 and GW151226, and the candidate event LVT151012 using KamLAND, a kiloton-scale antineutrino detector. We find no inverse beta-decay neutrino events within $\pm 500$ seconds of either gravitational wave signal. This non-detection is used to constrain the electron antineutrino fluence and the luminosity of the astrophysical sources., Comment: 11 pages, 4 figures, as published in ApJL. Updated to replace power law spectrum with Fermi Dirac spectrum

A search for double-beta decays of 136Xe to excited states of 136Ba has been performed with the first phase data set of the KamLAND-Zen experiment. The 0+1, 2+1 and 2+2 transitions of 0{\nu}\{beta}\{beta} decay were evaluated in an exposure of 89.5kg-yr of 136Xe, while the same transitions of 2{\nu}\{beta}\{beta} decay were evaluated in an exposure of 61.8kg-yr. No excess over background was found for all decay modes. The lower half-life limits of the 2+1 state transitions of 0{\nu}\{beta}\{beta} and 2{\nu}\{beta}\{beta} decay were improved to T(0{\nu}, 0+ \rightarrow 2+) > 2.6\times10^25 yr and T(2{\nu}, 0+ \rightarrow 2+) > 4.6\times10^23 yr (90% C.L.), respectively. We report on the first experimental lower half-life limits for the transitions to the 0+1 state of 136Xe for 0{\nu}\{beta}\{beta} and 2{\nu}\{beta}\{beta} decay. They are T (0{\nu}, 0+ \rightarrow 0+) > 2.4\times10^25 yr and T(2{\nu}, 0+ \rightarrow 0+) > 8.3\times10^23 yr (90% C.L.). The transitions to the 2+2 states are also evaluated for the first time to be T(0{\nu}, 0+ \rightarrow 2+) > 2.6\times10^25 yr and T(2{\nu}, 0+ \rightarrow 2+) > 9.0\times10^23 yr (90% C.L.). These results are compared to recent theoretical predictions., Comment: 16 pages, 4 figures. Published in Nuclear Physics A

In the late stages of nuclear burning for massive stars ($M>8~M_{\sun}$), the production of neutrino-antineutrino pairs through various processes becomes the dominant stellar cooling mechanism. As the star evolves, the energy of these neutrinos increases and in the days preceding the supernova a significant fraction of emitted electron anti-neutrinos exceeds the energy threshold for inverse beta decay on free hydrogen. This is the golden channel for liquid scintillator detectors because the coincidence signature allows for significant reductions in background signals. We find that the kiloton-scale liquid scintillator detector KamLAND can detect these pre-supernova neutrinos from a star with a mass of $25~M_{\sun}$ at a distance less than 690~pc with 3$\sigma$ significance before the supernova. This limit is dependent on the neutrino mass ordering and background levels. KamLAND takes data continuously and can provide a supernova alert to the community., Comment: 19 pages, 6 figures, 1 table

We search for electron anti-neutrinos ($\overline{\nu}_e$) from long and short-duration gamma-ray bursts~(GRBs) using data taken by the KamLAND detector from August 2002 to June 2013. No statistically significant excess over the background level is found. We place the tightest upper limits on $\overline{\nu}_e$ fluence from GRBs below 7 MeV and place first constraints on the relation between $\overline{\nu}_e$ luminosity and effective temperature., Comment: 16 pages and 5 figures