The current state‐of‐the‐art of satellite gravity data processing makes use of de‐aliasing products to reduce high‐frequency mass anomalies. For example, the most recent official Atmosphere and Ocean De‐aliasing products (AOD1B‐RL06) are applied for the Gravity Recovery and Climate Experiment (GRACE) and GRACE‐Follow On (GRACE‐FO) missions. The temporal resolution of AOD1B‐RL06 is 3 h, and spectrally, they are computed up to degree and order 180. In this study, we explore a refined, e.g., geometrically, physically, and numerically improved, mass integration approach that is important for computing the atmosphere part of these products. Besides, the newly available ERA5 climate data are used to produce a new set of non‐tidal atmosphere de‐aliasing product (HUST‐ERA5) that is computed hourly up to degree and order 100, covering 2002 onwards. Despite an overall agreement with AOD1B‐RL06 (correlation≥0.99), considerable discrepancies still exist between HUST‐ERA5 and AOD1B‐RL06. The possible reasons are therefore analyzed, and we find the input climate data, sampling rate and integration method may result in a product difference of ∼0.3, ∼0.15 and ∼0.05 millimeter geoid height, respectively. The total differences between HUST‐ERA5 and AOD1B‐RL06 can lead to a mean variation of ∼7.34 nm/s on the laser ranging interferometry (LRI) range‐rate residuals, for example, during January 2019, which is already close to the LRI precision. This impact is invisible for the GRACE (‐FO) gravity inversion because of the less accurate on‐board KBR (K‐band ranging) instrument, however, it will be non‐negligible and should be considered when the LRI completely replaces the KBR in the future gravity missions. Plain Language Summary: Time‐variable GRACE and GRACE‐FO satellite gravity data are unique remote sensing products that can be used for studying mass changes related to for example, water variability in aquifers, continental ice‐sheets, and oceans. The current state‐of‐the‐art of GRACE (‐FO) data processing makes use of background de‐aliasing products to reduce high‐frequency mass anomalies to focus on the dominant hydrology related signals. Thus, any errors in these products will badly affect the quality of water mass estimations. In this study, we explore a refined, that is, geometrically, physically, and numerically improved, mass integration approach to use the newly available ERA5 weather data for computing the atmosphere part of the background non‐tidal de‐aliasing products. The new set is called HUST‐ERA5 that is computed hourly up to degree and order 100, covering 2002 onwards, and freely available for download. Here we show that replacing the official de‐aliasing products with HUST‐ERA5 can lead to a mean variation of 7.34 nm/s on the Laser Ranging Interferometry (LRI) residuals, which is close to the LRI precision. This impact is invisible for the GRACE (‐FO) data because of the less accurate on‐board ranging instrument. However, it will be non‐negligible and should be considered when the LRI is functional in the future gravity missions. Key Points: Hourly ERA5 reanalysis is employed to generate the atmosphere de‐aliasing product for the first time, through a refined 3‐D vertical integration methodThe use of input fields from ERA5 and increasing the sampling rate of atmospheric products to 1 h are recommended for Gravity Recovery and Climate Experiment‐Follow On and future missionsNew sets of hourly atmospheric non‐tidal de‐aliasing and tidal components including [S1,S2,P1,K1,N2,M2,L2,T2,R2,T3,R3,S3] are produced and freely shared [ABSTRACT FROM AUTHOR]