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The discovery of van der Waals superconductors in recent years has generated a lot of excitement for their potentially novel pairing mechanisms. However, their typical atomic-scale thickness and micrometer-scale lateral dimensions impose severe challenges to investigations of pairing symmetry by conventional methods. In this report we demonstrate a new technique that employs high-quality-factor superconducting resonators to measure the kinetic inductance -- up to a part per million -- and loss of a van der Waals superconductor. We analyze the equivalent circuit model to extract the kinetic inductance, superfluid stiffness, penetration depth, and ratio of imaginary and real parts of the complex conductivity. We validate the technique by measuring aluminum and finding excellent agreement in both the zero-temperature superconducting gap as well as the complex conductivity data when compared with BCS theory. We then demonstrate the utility of the technique by measuring the kinetic inductance of multi-layered niobium diselenide and discuss the limits to the accuracy of our technique when the transition temperature of the sample, NbSe$_2$ at 7.06 K, approaches our Nb probe resonator at 8.59 K. Our method will be useful for practitioners in the growing fields of superconducting physics, materials science, and quantum sensing, as a means of characterizing superconducting circuit components and studying pairing mechanisms of the novel superconducting states which arise in layered 2D materials and heterostructures., Comment: 17 pages, 4 tables, 17 figures

The robustness of the macroscopic quantum nature of a superconductor can be characterized by the superfluid stiffness, $\rho_s$, a quantity that describes the energy required to vary the phase of the macroscopic quantum wave function. In unconventional superconductors, such as cuprates, the low-temperature behavior of $\rho_s$ drastically differs from that of conventional superconductors due to quasiparticle excitations from gapless points (nodes) in momentum space. Intensive research on the recently discovered magic-angle twisted graphene family has revealed, in addition to superconducting states, strongly correlated electronic states associated with spontaneously broken symmetries, inviting the study of $\rho_s$ to uncover the potentially unconventional nature of its superconductivity. Here we report the measurement of $\rho_s$ in magic-angle twisted trilayer graphene (TTG), revealing unconventional nodal-gap superconductivity. Utilizing radio-frequency reflectometry techniques to measure the kinetic inductive response of superconducting TTG coupled to a microwave resonator, we find a linear temperature dependence of $\rho_s$ at low temperatures and nonlinear Meissner effects in the current bias dependence, both indicating nodal structures in the superconducting order parameter. Furthermore, the doping dependence shows a linear correlation between the zero temperature $\rho_s$ and the superconducting transition temperature $T_c$, reminiscent of Uemura's relation in cuprates, suggesting phase-coherence-limited superconductivity. Our results provide strong evidence for nodal superconductivity in TTG and put strong constraints on the mechanisms of these graphene-based superconductors.

In high-sensitivity bolometers and calorimeters, the photon absorption often occurs at a finite distance from the temperature sensor to accommodate antennas or avoid the degradation of superconducting circuitry exposed to radiation. As a result, thermal propagation from the input to the temperature readout can critically affect detector performance. In this report we model the performance of a graphene bolometer, accounting for electronic thermal diffusion and dissipation via electron-phonon coupling at low temperatures in three regimes: clean, supercollision, and resonant scattering. Our results affirm the feasibility of a superconducting readout without Cooper-pair breaking by mid- and near-infrared photons, and provide a recipe for designing graphene absorbers for calorimetric single-photon detectors. We investigate the tradeoff between the input-readout distance and detector efficiency, and predict an intrinsic timing jitter of ~2.7 ps. Based on our result, we propose a spatial-mode-resolving photon detector to increase communication bandwidth.

News & Views on the graphene-based Josephson parametric amplifiers., Comment: 3 pages, 1 figure

We describe a wide-band Josephson Parametric Amplifier (JPA) that is impedance-matched using an integrated compact superconducting transmission line transformer. The impedance transformer consists of two broadside coupled transmission lines configured in a Ruthroff topology which enables a wide matching bandwidth from 2 to 18 GHz, reducing the input line impedance and the device resonance quality factor by a factor of 4. This enables gain flatness and flexibility in the choice of the amplifier's tuning range. The amplifier has up to 20dB gain, with less than 1 dB of ripple, 2-3 GHz gain-bandwidth product and -126 dBm input 1-dB compression point. Moreover, the device active area fits into a 1mm x 1mm space, thus easing integration into large quantum systems., Comment: 6 pages, 8 figures

Technologies operating on the basis of quantum mechanical laws and resources such as phase coherence and entanglement are expected to revolutionize our future. Quantum technologies are often divided into four main pillars: computing, simulation, communication, and sensing & metrology. Moreover, a great deal of interest is currently also nucleating around energy-related quantum technologies. In this Perspective, we focus on advanced superconducting materials, van der Waals materials, and moir\'e quantum matter, summarizing recent exciting developments and highlighting a wealth of potential applications, ranging from high-energy experimental and theoretical physics to quantum materials science and energy storage., Comment: 19 pages, 4 figures, 215 references, Perspective article on solid-state quantum technologies

Quantum computers can potentially achieve an exponential speedup versus classical computers on certain computational tasks, as recently demonstrated in systems of superconducting qubits. However, these qubits have large footprints due to their large capacitor electrodes needed to suppress losses by avoiding dielectric materials. This tactic hinders scaling by increasing parasitic coupling among circuit components, degrading individual qubit addressability, and limiting the spatial density of qubits. Here, we take advantage of the unique properties of the van der Waals (vdW) materials to reduce the qubit area by a factor of $>1000$ while preserving the required capacitance without increasing substantial loss. Our qubits combine conventional aluminum-based Josephson junctions with parallel-plate capacitors composed of crystalline layers of superconducting niobium diselenide (NbSe$_2$) and insulating hexagonal-boron nitride (hBN). We measure a vdW transmon $T_1$ relaxation time of 1.06 $\mu$s, which demonstrates a path to achieve high-qubit-density quantum processors with long coherence times, and illustrates the broad utility of layered heterostructures in low-loss, high-coherence quantum devices., Comment: 6 pages, 5 figures, and 1 table

Ultra low-loss microwave materials are crucial for enhancing quantum coherence and scalability of superconducting qubits. Van der Waals (vdW) heterostructure is an attractive platform for quantum devices due to the single-crystal structure of the constituent two-dimensional (2D) layered materials and the lack of dangling bonds at their atomically sharp interfaces. However, new fabrication and characterization techniques are required to determine whether these structures can achieve low loss in the microwave regime. Here we report the fabrication of superconducting microwave resonators using NbSe$_2$ that achieve a quality factor $Q > 10^5$. This value sets an upper bound that corresponds to a resistance of $\leq 192 \mu\Omega$ when considering the additional loss introduced by integrating NbSe$_2$ into a standard transmon circuit. This work demonstrates the compatibility of 2D layered materials with high-quality microwave quantum devices., Comment: 5 pages, 6 figures, 1 table

It has been suggested that certain antiferromagnetic topological insulators contain axion quasiparticles (AQs), and that such materials could be used to detect axion dark matter (DM). The AQ is a longitudinal antiferromagnetic spin fluctuation coupled to the electromagnetic Chern-Simons term, which, in the presence of an applied magnetic field, leads to mass mixing between the AQ and the electric field. The electromagnetic boundary conditions and transmission and reflection coefficients are computed. A model for including losses into this system is presented, and the resulting linewidth is computed. It is shown how transmission spectroscopy can be used to measure the resonant frequencies and damping coefficients of the material, and demonstrate conclusively the existence of the AQ. The dispersion relation and boundary conditions permit resonant conversion of axion DM into THz photons in a material volume that is independent of the resonant frequency, which is tuneable via an applied magnetic field. A parameter study for axion DM detection is performed, computing boost amplitudes and bandwidths using realistic material properties including loss. The proposal could allow for detection of axion DM in the mass range between 1 and 10 meV using current and near future technology., Comment: 78 pages + appendices, v2: reference list extended, added one more case to fig 23

Josephson junctions (JJs) are ubiquitous superconducting devices, enabling high sensitivity magnetometers and voltage amplifiers, as well as forming the basis of high performance cryogenic computer and superconducting quantum computers. While JJ performance can be degraded by quasiparticles (QPs) formed from broken Cooper pairs, this phenomenon also opens opportunities to sensitively detect electromagnetic radiation. Here we demonstrate single near-infrared photon detection by coupling photons to the localized surface plasmons of a graphene-based JJ. Using the photon-induced switching statistics of the current-biased JJ, we reveal the critical role of QPs generated by the absorbed photon in the detection mechanism. The photon-sensitive JJ will enable a high-speed, low-power optical interconnect for future JJ-based computing architectures., Comment: 12 pages, 9 figures, and 4 tables

Heat capacity is an invaluable quantity in condensed matter physics, yet it has been so far experimentally inaccessible in two-dimensional (2D) van der Waals (vdW) materials, owing to their ultra-fast thermal relaxation times and the lack of suitable nano-scale thermometers. Here, we demonstrate a novel thermal relaxation calorimetry scheme that allows the first measurements of the electronic heat capacity of graphene Ce. It is enabled by the grouping of a radio-frequency Johnson noise thermometer, which can measure the electronic temperature Te with a measurement sensitivity of {\delta}Te ~ 20 mK, and an ultra-fast photo-mixed optical heater, which can simultaneously modulate Te with a frequency of up to {\Omega}=0.2 THz. This combination allows record sensitive and record fast measurements of the electronic heat capacity Ce < 10^(-19) J/K, with an electronic thermal relaxation time {\tau}e < 10^(-13), representing orders of magnitude improvements as compared to previous state-of-the-art calorimeters. These features embody a breakthrough in heat capacity metrology of nano-scale and low-dimensional systems, and provide a new avenue for the investigation of their thermodynamic quantities.

We propose a new dark-matter detection strategy that will enable the search of super-light dark matter $m_\chi \simeq 0.1$ keV, representing an improvement of the minimum detectable mass by more than three order of magnitude over the ongoing experiments. This is possible by integrating intimately the target material, $\pi$-bond electrons in graphene, into a Josephson junction to achieve a high sensitivity detector that can resolve a small energy exchange from dark matter as low as $\sim 0.1$ meV. We investigate detection prospects with pg-, ng-, and $\mu$g-scale detectors by calculating the scattering rate between dark matter and free electrons confined in two-dimensional graphene with Pauli-blocking factors included. We find not only that the proposed detector can serve as a complementary probe of super-light dark matter but also achieve higher experimental sensitivities than other proposed experiments, thanks to the extremely low energy threshold of our Josephson junction sensor., Comment: 8 pages, 4 figures, Funding agency information for the actual experiment added, Appendix expanded, More figures added

Sensitive microwave detectors are critical instruments in radioastronomy, dark matter axion searches, and superconducting quantum information science. The conventional strategy towards higher-sensitivity bolometry is to nanofabricate an ever-smaller device to augment the thermal response. However, this direction is increasingly more difficult to obtain efficient photon coupling and maintain the material properties in a device with a large surface-to-volume ratio. Here we advance this concept to an ultimately thin bolometric sensor based on monolayer graphene. To utilize its minute electronic specific heat and thermal conductivity, we develop a superconductor-graphene-superconductor (SGS) Josephson junction bolometer embedded in a microwave resonator of resonant frequency 7.9 GHz with over 99\% coupling efficiency. From the dependence of the Josephson switching current on the operating temperature, charge density, input power, and frequency, we demonstrate a noise equivalent power (NEP) of 7 $\times 10^{-19}$ W/Hz$^{1/2}$, corresponding to an energy resolution of one single photon at 32 GHz and reaching the fundamental limit imposed by intrinsic thermal fluctuation at 0.19 K., Comment: 8 pages, 4 figures

The noncentrosymmetric Td-WTe$_2$, previously known as a type-II Weyl semimetal, is expected to have higher order topological phases with topologically protected, helical one-dimensional (1D) hinge states when their scarcely separated Weyl points get annihilated. However, the detection of these hinge states is difficult in the presence of the semimetallic behaviour of the bulk. Here, we spatially resolved the hinge states by analysing the magnetic field interference of supercurrent in Nb-WTe$_2$-Nb proximity Josephson junctions. The Josephson current along the a-axis of the WTe$_2$ crystal, but not along the b-axis, showed sharp enhancements at the edges of the junction; the amount of enhanced Josephson current was comparable to the upper limits of a single 1D conduction channel. Our experimental observations provide evidence of the higher order topological phase in WTe$_2$ and its corresponding anisotropic topological hinge states, in good agreement with theoretical calculations. Our work paves the way for hinge transport studies on topological semimetals in superconducting heterostructures, including their topological superconductivity., Comment: 29 pages, 11 figures

We describe a kinetic inductance traveling-wave (KIT) amplifier suitable for superconducting quantum information measurements and characterize its wideband scattering and noise properties. We use mechanical microwave switches to calibrate the four amplifier scattering parameters up to the device input and output connectors at the dilution refrigerator base temperature and a tunable temperature load to characterize the amplifier noise. Finally, we demonstrate the high fidelity simultaneous dispersive readout of two superconducting transmon qubits. The KIT amplifier provides low-noise amplification of both readout tones with readout fidelities of 83% and 89% and negligible effect on qubit lifetime and coherence., Comment: 5 pages, 5 figures

Antiferromagnetically doped topological insulators (A-TI) are among the candidates to host dynamical axion fields and axion-polaritons; weakly interacting quasiparticles that are analogous to the dark axion, a long sought after candidate dark matter particle. Here we demonstrate that using the axion quasiparticle antiferromagnetic resonance in A-TI's in conjunction with low-noise methods of detecting THz photons presents a viable route to detect axion dark matter with mass 0.7 to 3.5 meV, a range currently inaccessible to other dark matter detection experiments and proposals. The benefits of this method at high frequency are the tunability of the resonance with applied magnetic field, and the use of A-TI samples with volumes much larger than 1 mm$^3$., Comment: 6 pages, 4 figures. v2 accepted for publication in Physical Review Letters. Many points clarified, some parameter estimates revised

We analyze the effect of contact resistance on the Lorenz number measurement based on direct electronic thermal conductivity experiments. The contact resistance can significantly limit the experimental measured value when the Lorenz number is enhanced, but not as much so when it is suppressed, should the Wiedemann-Franz law be violated. The result provides the conditions of the potential false negative error and highlights the importance of improving the contact resistance in studying non-Fermi liquid behavior in thermal transport experiments., Comment: 6 pages, 3 figures

Generic interacting many-body quantum systems are believed to behave as classical fluids on long time and length scales. Due to rapid progress in growing exceptionally pure crystals, we are now able to experimentally observe this collective motion of electrons in solid-state systems, including graphene. We present a review of recent progress in understanding the hydrodynamic limit of electronic motion in graphene, written for physicists from diverse communities. We begin by discussing the "phase diagram" of graphene, and the inevitable presence of impurities and phonons in experimental systems. We derive hydrodynamics, both from a phenomenological perspective and using kinetic theory. We then describe how hydrodynamic electron flow is visible in electronic transport measurements. Although we focus on graphene in this review, the broader framework naturally generalizes to other materials. We assume only basic knowledge of condensed matter physics, and no prior knowledge of hydrodynamics., Comment: Review article. 79 pages, 21 figures. v2: published version

We propose to use graphene-based Josephson junctions (gJjs) to detect single photons in a wide electromagnetic spectrum from visible to radio frequencies. Our approach takes advantage of the exceptionally low electronic heat capacity of monolayer graphene and its constricted thermal conductance to its phonon degrees of freedom. Such a system could provide high sensitivity photon detection required for research areas including quantum information processing and radio-astronomy. As an example, we present our device concepts for gJj single photon detectors in both the microwave and infrared regimes. The dark count rate and intrinsic quantum efficiency are computed based on parameters from a measured gJj, demonstrating feasibility within existing technologies., Comment: 11 pages, 6 figures, and 1 table in the main text

Coulomb interaction between two closely spaced parallel layers of electron system can generate the frictional drag effect by interlayer Coulomb scattering. Employing graphene double layers separated by few layer hexagonal boron nitride (hBN), we investigate density tunable magneto- and Hall-drag under strong magnetic fields. The observed large magneto-drag and Hall-drag signals can be related with Laudau level (LL) filling status of the drive and drag layers. We find that the sign and magnitude of the magneto- and Hall-drag resistivity tensor can be quantitatively correlated to the variation of magneto-resistivity tensors in the drive and drag layers, confirming a theoretical formula for magneto-drag in the quantum Hall regime. The observed weak temperature dependence and $\sim B^2$ dependence of the magneto-drag are qualitatively explained by Coulomb scattering phase-space argument., Comment: 5 pages, 3 figures

We develop a general hydrodynamic framework for computing direct current thermal and electric transport in a strongly interacting finite temperature quantum system near a Lorentz-invariant quantum critical point. Our framework is non-perturbative in the strength of long wavelength fluctuations in the background charge density of the electronic fluid, and requires the rate of electron-electron scattering to be faster than the rate of electron-impurity scattering. We use this formalism to compute transport coefficients in the Dirac fluid in clean samples of graphene near the charge neutrality point, and find results insensitive to long range Coulomb interactions. Numerical results are compared to recent experimental data on thermal and electrical conductivity in the Dirac fluid in graphene and substantially improved quantitative agreement over existing hydrodynamic theories is found. We comment on the interplay between the Dirac fluid and acoustic and optical phonons, and qualitatively explain experimentally observed effects. Our work paves the way for quantitative contact between experimentally realized condensed matter systems and the wide body of high energy inspired theories on transport in interacting many-body quantum systems., Comment: 19 + 12 pages; 8 + 3 figures; v2: very minor changes, published version

Interactions between particles in quantum many-body systems can lead to collective behavior described by hydrodynamics. One such system is the electron-hole plasma in graphene near the charge neutrality point which can form a strongly coupled Dirac fluid. This charge neutral plasma of quasi-relativistic fermions is expected to exhibit a substantial enhancement of the thermal conductivity, due to decoupling of charge and heat currents within hydrodynamics. Employing high sensitivity Johnson noise thermometry, we report the breakdown of the Wiedemann-Franz law in graphene, with a thermal conductivity an order of magnitude larger than the value predicted by Fermi liquid theory. This result is a signature of the Dirac fluid, and constitutes direct evidence of collective motion in a quantum electronic fluid., Comment: 5+5 pages, 3+7 figures

We develop a high frequency, wide bandwidth radiometer operating at room temperature, which augments the traditional technique of Johnson noise thermometry for nanoscale thermal transport studies. Employing low noise amplifiers and an analog multiplier operating at 2~GHz, auto- and cross-correlated Johnson noise measurements are performed in the temperature range of 3 to 300~K, achieving a sensitivity of 5.5~mK (110 ppm) in 1 second of integration time. This setup allows us to measure the thermal conductance of a boron nitride encapsulated monolayer graphene device over a wide temperature range. Our data shows a high power law (T$^{\sim4}$) deviation from the Wiedemann-Franz law above T$\sim$100~K., Comment: 4 pages, 4 figures

Graphene is a material with remarkable electronic properties and exceptional thermal transport properties near room temperature, which have been well examined and understood. However at very low temperatures the thermodynamic and thermal transport properties are much less well explored and somewhat surprisingly, is expected to exhibit extreme thermal isolation. Here we demonstrate an ultra-sensitive, wide-bandwidth measurement scheme to probe the thermal transport and thermodynamic properties of the electron gas of graphene. We employ Johnson noise thermometry at microwave frequency to sensitively measure the temperature of the electron gas with resolution of $4 mK/\sqrt{Hz}$ and a bandwidth of 80 MHz. We have measured the electron-phonon coupling from 2-30 K at a charge density of $2\cdot 10^{11} cm^{-2}$. Utilizing bolometric mixing, we have sensed temperature oscillations with period of 430 ps and have determined the heat capacity of the electron gas to be $2\cdot 10^{-21} J/(K\cdot \mu m^2)$ at 5 K which is consistent with that of a two dimensional, Dirac electron gas. These measurements suggest that graphene-based devices together with wide bandwidth noise thermometry can generate substantial advances in the areas of ultra-sensitive bolometry, calorimetry, microwave and terahertz photo-detection, and bolometric mixing for applications in areas such as observational astronomy and quantum information and measurement., Comment: 8 pages, 4 figures

Magnetic Resonance Force Microscopy can enable nanoscale imaging of spin lifetime. We report temperature dependent measurements of the spin correlation time $\tau_m$ of the statistical fluctuations of the spin polarization---the spin noise---of ensembles containing $\sim 100$ electron spins by this technique. Magneto-mechanical relaxation due to spin-cantilever coupling was controlled and spurious mechanisms that can affect the spin correlation time of the microscopic signal were characterized. These measurements have ramifications for optimizing spin sensitivity, understanding local spin dynamics and for nanoscale imaging., Comment: 5 pages, 5 figures, accepted in Phys. Rev. B (Rapid Comm.)