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We investigate the evolution of the second-order temporal coherence during the emission of a superradiant burst by an elongated cloud of cold Rb atoms in free space. To do so, we measure the two-times intensity correlation function $g_N^{(2)}(t_1, t_2)$ following the pulsed excitation of the cloud. By monitoring $g_N^{(2)}(t, t)$ during the burst, we observe the establishment of second-order coherence, and contrast it with the situation where the cloud is initially prepared in a steady state. We compare our findings to the predictions of the Dicke model, using an effective atom number to account for finite size effects, finding that the model reproduces the observed trend at early time. For longer times, we observe a subradiant decay, a feature that goes beyond Dicke's model. Finally, we measure the $g_N^{(2)}(t_1, t_2)$ at different times and observe the appearance of anti-correlations during the burst, that are not present when starting from a steady state.

We report experimental measurements of the dynamical polarizability of dysprosium, at a wavelength of 532 nm. We measure all three components (scalar, vector, tensor) of the anisotropic polarizability for the ground and the excited manifolds of the intercombination transition of Dy at 626 nm. The apparatus on which the measurements are performed is first presented. We obtain with this setup imaging of single Dy atoms with fidelity above 99 % and losses below 2.5 % induced by imaging. We then describe the methods used to extract the polarizability. In particular, we combine a measurement of trap frequency and trap depth on single atoms in optical tweezers, allowing us to obtain a measurement of the ground state polarizability free of errors in trap waist calibration. The obtained values give a magic condition between two Zeeman states in the ground and excited manifolds, which was used to image single atoms in optical tweezer arrays. The scalar polarizability of the ground state is in disagreement with theoretical expectations, calling for future investigations to resolve the discrepancy.

The driven Dicke model, wherein an ensemble of atoms is driven by an external field and undergoes collective spontaneous emission due to coupling to a leaky cavity mode, is a paradigmatic example of a system exhibiting a driven-dissipative phase transition as a function of driving strength. Recently, a similar phenomenon was experimentally observed, not in a cavity setting, but rather in a free-space atomic ensemble. The reason why similar behavior should emerge in free space is not obvious, as the system interacts with a continuum of optical modes, which encodes light propagation effects. Here, we present and solve a simple model to explain the behavior of the free-space system, based on the one-dimensional Maxwell-Bloch equations. On one hand, we show that a free-space ensemble at a low optical depth can exhibit similar behavior as the cavity system, as spatial propagation effects are negligible. On the other hand, in the thermodynamic limit of large atom number, we show that certain observables such as the transmittance or the atomic excited population exhibit non-analytic behavior as a function of the driving intensity, reminiscent of a phase transition. However, a closer analysis reveals that the atomic properties are highly inhomogeneous in space, and based on this we argue that the free-space system does not undergo a phase transition but rather a ``phase separation", roughly speaking, between saturated and unsaturated regions., Comment: 16 pages and 9 figures in the main text + 2 pages and 2 figures in the Appendix

We report experimental measurements of the second-order coherence function $g^{(2)}(\tau)$ of the light emitted by a laser-driven dense ensemble of $^{87}$Rb atoms. We observe a clear departure from the Siegert relation valid for Gaussian chaotic light. Measuring intensity and first-order coherence, we conclude that the violation is not due to the emergence of a coherent field. This indicates that the light obeys non-Gaussian statistics, stemming from non-Gaussian correlations in the atomic medium. More specifically, the steady-state of this driven-dissipative many-body system sustains high-order correlations in the absence of first-order coherence. These findings call for new theoretical and experimental explorations to uncover their origin and they open new perspectives for the realization of non-Gaussian states of light.

We report the preparation and observation of single atoms of dysprosium in arrays of optical tweezers with a wavelength of 532 nm imaged on the intercombination line at 626 nm. We use the anisotropic light shift specific to lanthanides and in particular a large difference in tensor and vector polarizabilities between the ground and excited states to tune the differential light shift and produce tweezers in near-magic or magic polarization. This allows us to find a regime where single atoms can be produced and imaged. Using the tweezer array toolbox to manipulate lanthanides will open new research directions for quantum physics studies by taking advantage of their rich spectrum, large spin and magnetic dipole moment.

Driven by the need to develop efficient atom-photon interfaces, recent efforts have proposed replacing cavities by large arrays of cold atoms that can support subradiant or superradiant collective states. In practice, subradiant states are decoupled from radiation, which constitutes a hurdle to most applications. In this work, we study theoretically a protocol that bypasses this limit using a one dimensional (1D) chain composed of N three-level atoms in a V-shaped configuration. Throughout the protocol, the chain behaves as a time-varying metamaterial: enabling absorption, storage and on-demand emission in a spectrally and spatially controlled mode. Taking into account the quantum nature of atoms, we establish the boundary between the linear regime and the nonlinear regime. In the nonlinear regime, we demonstrate that doubly-excited states can be coherently transferred from superradiant to subradiant states, opening the way to the optical characterization of their entanglement., Comment: 13 pages, 10 figures

A class of systems exists in which dissipation, external drive and interactions compete and give rise to non equilibrium phases that would not exist without the drive. There, phase transitions could occur without the breaking of any symmetry, yet with a local order parameter, in contrast with the Landau theory of phase transitions at equilibrium. One of the simplest driven dissipative quantum systems consists of two-level atoms enclosed in a volume smaller than the wavelength of the atomic transition cubed, driven by a light field. The competition between collective coupling of the atoms to the driving field and their cooperative decay should lead to a transition between a phase where all the atomic dipoles are phaselocked and a phase governed by superradiant spontaneous emission. Here, we realize this model using a pencil-shaped cloud of laser cooled atoms in free space, optically excited along its main axis, and observe the predicted phases. Our demonstration is promising in view of obtaining free-space superradiant lasers or to observe new types of time crystals., Comment: 9 pages, 8 figures

Since the achievement of quantum degeneracy in gases of chromium atoms in 2004, the experimental investigation of ultracold gases made of highly magnetic atoms has blossomed. The field has yielded the observation of many unprecedented phenomena, in particular those in which long-range and anisotropic dipole-dipole interactions play a crucial role. In this review, we aim to present the aspects of the magnetic quantum-gas platform that make it unique for exploring ultracold and quantum physics as well as to give a thorough overview of experimental achievements.

We report a time-resolved study of collective emission in dense ensembles of two-level atoms. We compare, on the same sample, the build-up of superradiance and subradiance from the ensemble when driven by a strong laser. This allows us to measure the dynamics of the population of superradiant and subradiant states as a function of time. In particular we demonstrate the build up in time of subradiant states through the superradiant dynamics. This illustrates the dynamics of the many-body density matrix of superradiant ensembles of two-level atoms when departing from the ideal conditions of Dicke superradiance in which symmetry forbids the population of subradiant states.

We report the efficient and fast ($\sim 2\mathrm{Hz}$) preparation of randomly loaded 1D chains of individual $^{87}$Rb atoms and of dense atomic clouds trapped in optical tweezers using a new experimental platform. This platform is designed for the study of both structured and disordered atomic systems in free space. It is composed of two high-resolution optical systems perpendicular to each other, enhancing observation and manipulation capabilities. The setup includes a dynamically controllable telescope, which we use to vary the tweezer beam waist. A D1 $\Lambda$-enhanced gray molasses enhances the loading of the traps from a magneto-optical trap. Using these tools, we prepare chains of up to $\sim 100$ atoms separated by $\sim 1 \mathrm{\mu m}$ by retro-reflecting the tweezer light, hence producing a 1D optical lattice with strong transverse confinement. Dense atomic clouds with peak densities up to $n_0 = 10^{15}\:\mathrm{at}/\mathrm{cm}^3$ are obtained by compression of an initial cloud. This high density results into interatomic distances smaller than $\lambda/(2\pi)$ for the D2 optical transitions, making it ideal to study light-induced interactions in dense samples.

We report the observation of subradiance in dense ensembles of cold $^{87}$Rb atoms operating near Dicke's regime of a large number of atoms in a volume with dimensions smaller than the transition wavelength. We validate that the atom number is the only cooperativity parameter governing subradiance. We probe the dynamics in the many-body regime and support the picture that multiply-excited subradiant states are built as a superposition of singly-excited states that decay independently. Moreover, we implement an experimental procedure to release the excitation stored in the long-lived modes in a pulse of light. This technique is a first step towards the realization of tailored light storing based on subradiance.

Fully inverted atoms placed at exactly the same location synchronize as they deexcite, and light is emitted in a burst (known as "Dicke's superradiance"). We investigate the role of finite interatomic separation on correlated decay in mesoscopic chains, and provide an understanding in terms of collective jump operators. We show that the superradiant burst survives at small distances, despite Hamiltonian dipole-dipole interactions. However, for larger separations, competition between different jump operators leads to dephasing, suppressing superradiance. Collective effects are still significant for arrays with lattice constants of the order of a wavelength, and lead to a photon emission rate that decays nonexponentially in time. We calculate the two-photon correlation function and demonstrate that emission is correlated and directional, as well as sensitive to small changes in the interatomic distance. These features can be measured in current experimental setups, and are robust to realistic imperfections., Comment: 17 pages, 13 figures

We experimentally study resonant light scattering by a one-dimensional randomly filled chain of cold two-level atoms. By a local measurement of the light scattered along the chain, we observe constructive interferences in light-induced dipole-dipole interactions between the atoms. They lead to a shift of the collective resonance despite the average interatomic distance being larger than the wavelength of the light. This result demonstrates that strong collective effects can be enhanced by structuring the geometrical arrangement of the ensemble. We also explore the high intensity regime where atoms cannot be described classically. We compare our measurement to a mean-field, nonlinear coupled-dipole model accounting for the saturation of the response of a single atom.

Dipolar quantum droplets are exotic quantum objects that are self-bound due to the subtle balance of attraction, repulsion and quantum correlations. Here we present a systematic study of the critical atom number of these self-bound droplets, comparing the experimental results with extended mean-field Gross-Pitaevskii equation (eGPE) and quantum Monte-Carlo simulations of the dilute system. The respective theoretical predictions differ, questioning the validity of the current theoretical state-of-the-art description of quantum droplets within the eGPE framework and indicating that correlations in the system are significant. Furthermore, we show that our system can serve as a sensitive testing ground for many-body theories in the near future.

In this article we develop the framework to describe Bose-Fermi mixtures of magnetic atoms, focusing on the interaction of bosonic self-bound dipolar quantum droplets with a small number of fermions. We find an attractive interaction potential due to the dipolar interaction with several bound states, which can be occupied by one fermion each, resulting in a very weak back-action on the bosons. We conclude, that these impurities might act as unique probes giving access to inherent properties of dipolar quantum droplets., Comment: To appear in the "Focus issue: Quantum Optics and Beyond - in honour of Wolfgang Schleich" of Physica Scripta

We present transport measurements on a dipolar superfluid using a Bose-Einstein condensate of Dy-162 with strong magnetic dipole-dipole interactions. By moving an attractive laser beam through the condensate we observe an anisotropy in superfluid flow. This observation is compatible with an anisotropic critical velocity for the breakdown of dissipationless flow, which, in the spirit of the Landau criterion, can directly be connected to the anisotropy of the underlying dipolar excitation spectrum. In addition, the heating rate above this critical velocity reflects the same anisotropy. Our observations are in excellent agreement with simulations based on the Gross-Pitaevskii equation and highlight the effect of dipolar interactions on macroscopic transport properties, rendering dissipation anisotropic.

We report on the observation of the scissors mode of a single dipolar quantum droplet. The existence of this mode is due to the breaking of the rotational symmetry by the dipole-dipole interaction, which is fixed along an external homogeneous magnetic field. By modulating the orientation of this magnetic field, we introduce a new spectroscopic technique for studying dipolar quantum droplets. This provides a precise probe for interactions in the system allowing to extract a background scattering length for \textsuperscript{164}Dy of $69(4)\,a_0$. Our results establish an analogy between quantum droplets and atomic nuclei, where the existence of the scissors mode is also only due to internal interactions. They further open the possibility to explore physics beyond the available theoretical models for strongly-dipolar quantum gases.

We explore the phase diagram of a finite-sized dysprosium dipolar Bose-Einstein condensate in a cylindrical harmonic trap. We monitor the final state after the scattering length is lowered from the repulsive BEC regime to the quantum droplet regime. Either an adiabatic transformation between a BEC and a quantum droplet is obtained or, above a critical trap aspect ratio $\lambda_{\rm c}=1.87(14)$, a modulational instability results in the formation of multiple droplets. This is in full agreement with the predicted structure of the phase diagram with a crossover region below $\lambda_{\rm c}$ and a multistable region above. Our results provide the missing piece connecting the previously explored regimes resulting in a single or multiple dipolar quantum droplets.

We study theoretically and experimentally the behaviour of a strongly confined dipolar Bose-Einstein condensate, in the regime of quantum-mechanical stabilization by beyond-mean-field effects. Theoretically, we demonstrate that self-organized striped ground states are predicted in the framework of the extended Gross-Pitaevskii theory. Experimentally, by tilting the magnetic dipoles we show that self-organized striped states can be generated, likely in their metastable state. Matter-wave interference experiments with multiple stripes show that there is no long-range off-diagonal order (global phase coherence). We outline a parameter range where global phase coherence could be established, thus paving the way towards the observation of supersolid states in this system., Comment: 9 pages, 7 figures

The simultaneous presence of two competing inter-particle interactions can lead to the emergence of new phenomena in a many-body system. Among others, such effects are expected in dipolar Bose-Einstein condensates, subject to dipole-dipole interaction and short-range repulsion. Magnetic quantum gases and in particular Dysprosium gases, offering a comparable short-range contact and a long-range dipolar interaction energy, remarkably exhibit such emergent phenomena. In addition an effective cancellation of mean-field effects of the two interactions results in a pronounced importance of quantum-mechanical beyond mean-field effects. For a weakly-dominant dipolar interaction the striking consequence is the existence of a new state of matter equilibrated by the balance between weak mean-field attraction and beyond mean-field repulsion. Though exemplified here in the case of dipolar Bose gases, this state of matter should appear also with other microscopic interactions types, provided a competition results in an effective cancellation of the total mean-field. The macroscopic state takes the form of so-called quantum droplets. We present the effects of a long-range dipolar interaction between these droplets., Comment: Revised manuscript for publication in a special issue of JPhysB

Self-bound many-body systems are formed through a balance of attractive and repulsive forces and occur in many physical scenarios. Liquid droplets are an example of a self-bound system, formed by a balance of the mutual attractive and repulsive forces that derive from different components of the inter-particle potential. It has been suggested that self-bound ensembles of ultracold atoms should exist for atom number densities that are 10^8 times lower than in a helium droplet, which is formed from a dense quantum liquid. However, such ensembles have been elusive up to now because they require forces other than the usual zero-range contact interaction, which is either attractive or repulsive but never both. On the basis of the recent finding that an unstable bosonic dipolar gas can be stabilized by a repulsive many-body term, it was predicted that three-dimensional self-bound quantum droplets of magnetic atoms should exist. Here we report the observation of such droplets in a trap-free levitation field. We find that this dilute magnetic quantum liquid requires a minimum, critical number of atoms, below which the liquid evaporates into an expanding gas as a result of the quantum pressure of the individual constituents. Consequently, around this critical atom number we observe an interaction-driven phase transition between a gas and a self-bound liquid in the quantum degenerate regime with ultracold atoms. These droplets are the dilute counterpart of strongly correlated self-bound systems such as atomic nuclei and helium droplets.

Quantum fluctuations are the origin of genuine quantum many-body effects, and can be neglected in classical mean-field phenomena. Here we report on the observation of stable quantum droplets containing $\sim$ 800 atoms which are expected to collapse at the mean-field level due to the essentially attractive interaction. By systematic measurements on individual droplets we demonstrate quantitatively that quantum fluctuations stabilize them against the mean-field collapse. We observe in addition interference of several droplets indicating that this stable many-body state is phase coherent.

We study the dynamics of counterflowing bosonic and fermionic lithium atoms. First, by tuning the interaction strength we measure the critical velocity vc of the system in the BEC-BCS crossover in the low temperature regime and we compare it to the recent prediction of Castin et al., Comptes Rendus Physique, 16, 241 (2015). Second, raising the temperature of the mixture slightly above the superfluid transitions reveals an unexpected phase-locking of the oscillations of the clouds. We interpret this observation as resulting from a Zeno-like effect induced by dissipation.

Ferrofluids show unusual hydrodynamic effects due to the magnetic nature of their constituents. For increasing magnetization a classical ferrofluid undergoes a Rosensweig instability and creates self-organized ordered surface structures or droplet crystals. A Bose-Einstein condensate with strong dipolar interactions is a quantum ferrofluid that also shows superfluidity. The field of dipolar quantum gases is motivated by the search for new phases that break continuous symmetries. The simultaneous breaking of continuous symmetries like the phase invariance for the superfluid state and the translational symmetry for a crystal provides the basis of novel states of matter. However, interaction-induced crystallization in a superfluid has not been observed. Here we use in situ imaging to directly observe the spontaneous transition from an unstructured superfluid to an ordered arrangement of droplets in an atomic dysprosium Bose-Einstein condensate. By utilizing a Feshbach resonance to control the interparticle interactions, we induce a finite-wavelength instability and observe discrete droplets in a triangular structure, growing with increasing atom number. We find that these states are surprisingly long-lived and measure a hysteretic behaviour, which is typical for a crystallization process and in close analogy to the Rosensweig instability. Our system can show both superfluidity and, as shown here, spontaneous translational symmetry breaking. The presented observations do not probe superfluidity in the structured states, but if the droplets establish a common phase via weak links, this system is a very good candidate for a supersolid ground state.

We report on the observation of weakly-bound dimers of bosonic Dysprosium with a strong universal s-wave halo character, associated with broad magnetic Feshbach resonances. These states surprisingly decouple from the chaotic backgound of narrow resonances, persisting across many such narrow resonances. In addition they show the highest reported magnetic moment $\mu\simeq20\,\mu_{\rm B}$ of any ultracold molecule. We analyze our findings using a coupled-channel theory taking into account the short range van der Waals interaction and a correction due to the strong dipole moment of Dysprosium. We are able to extract the scattering length as a function of magnetic field associated with these resonances and obtain a background scattering length $a_{\rm bg}=91(16)\,a_0$. These results offer prospects of a tunability of the interactions in Dysprosium, which we illustrate by observing the saturation of three-body losses.

The low temperature unitary Bose gas is a fundamental paradigm in few-body and many-body physics, attracting wide theoretical and experimental interest. Here we first present a theoretical model that describes the dynamic competition between two-body evaporation and three-body re-combination in a harmonically trapped unitary atomic gas above the condensation temperature. We identify a universal magic trap depth where, within some parameter range, evaporative cooling is balanced by recombination heating and the gas temperature stays constant. Our model is developed for the usual three-dimensional evaporation regime as well as the 2D evaporation case. Experiments performed with unitary 133 Cs and 7 Li atoms fully support our predictions and enable quantitative measurements of the 3-body recombination rate in the low temperature domain. In particular, we measure for the first time the Efimov inelasticity parameter $\eta$ * = 0.098(7) for the 47.8-G d-wave Feshbach resonance in 133 Cs. Combined 133 Cs and 7 Li experimental data allow investigations of loss dynamics over two orders of magnitude in temperature and four orders of magnitude in three-body loss. We confirm the 1/T 2 temperature universality law up to the constant $\eta$ *.

We determine {\`a} la Landau the critical velocity $v\_c^{L}$ of a moving impurity in a Fermi superfluid, that is by restricting to the minimal excitation processes of the superfluid. $v\_c^{L}$ is then the minimal velocity at which these processes are energetically allowed. The Fermi superfluid actually exhibits two excitation branches~: one is the fermionic pair-breaking excitation, as predicted by BCS theory; the other one is bosonic and sets pairs into motion, as predicted by Anderson's RPA. $v\_c^{L}$ is the smallest of the two corresponding critical velocities $v\_{c,f}^{L}$ and $v\_{c,b}^{L}$. In the parameter space (superfluid interaction strength, fermion-to-impurity mass ratio), we identify two transition lines, corresponding to a discontinuity of the first-order and second-order derivatives of $v\_c^{L}$. These two lines meet in a triple point and split the plane in three domains. We briefly extend this analysis to the very recently realized case at ENS, where the moving object in the Fermi superfluid is a weakly interacting Bose superfluid of impurities, rather than a single impurity. For a Bose chemical potential much smaller than the Fermi energy, the topology of the transition lines is unaffected; a key result is that the domain $v\_c^{L}=c$, where $c$ is the sound velocity in the Fermi superfluid, is turned into a domain $v\_c^{L}=c+c\_B$, where $c\_B$ is the sound velocity in the Bose superfluid, with slightly shifted boundaries., Comment: final version, both in english and in french

Superconductivity and superfluidity of fermionic and bosonic systems are remarkable many-body quantum phenomena. In liquid helium and dilute gases, Bose and Fermi superfluidity has been observed separately, but producing a mixture in which both the fermionic and the bosonic components are superfluid is challenging. Here we report on the observation of such a mixture with dilute gases of two Lithium isotopes, 6Li and 7Li. We probe the collective dynamics of this system by exciting center-of-mass oscillations that exhibit extremely low damping below a certain critical velocity. Using high precision spectroscopy of these modes we observe coherent energy exchange and measure the coupling between the two superfluids. Our observations can be captured theoretically using a sum-rule approach that we interpret in terms of two coupled oscillators.

Following the bichromatic sub-Doppler cooling scheme on the D1 line of 40K recently demonstrated in (Fernandes et al. 2012), we introduce a similar technique for 7Li atoms and obtain temperatures of 60 uK while capturing all of the 5x10^8 atoms present from the previous stage. We investigate the influence of the detuning between the the two cooling frequencies and observe a threefold decrease of the temperature when the Raman condition is fulfilled. We interpret this effect as arising from extra cooling due to long-lived coherences between hyperfine states. Solving the optical Bloch equations for a simplified, \Lambda-type three-level system we identify the presence of an efficient cooling force near the Raman condition. After transfer into a quadrupole magnetic trap, we measure a phase space density of ~10^-5. This laser cooling offers a promising route for fast evaporation of lithium atoms to quantum degeneracy in optical or magnetic traps., Comment: 8 pages, 8 figures; submitted to Phys. Rev. A; V2 contains edits in response to referee's comments