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Quantum spins of mesoscopic size are a well-studied playground for engineering non-classical states. If the spin represents the collective state of an ensemble of qubits, its non-classical behavior is linked to entanglement between the qubits. In this work, we report on an experimental study of entanglement in dysprosium's electronic spin. Its ground state, of angular momentum $J=8$, can formally be viewed as a set of $2J$ qubits symmetric upon exchange. To access entanglement properties, we partition the spin by optically coupling it to an excited state $J'=J-1$, which removes a pair of qubits in a state defined by the light polarization. Starting with the well-known W and squeezed states, we extract the concurrence of qubit pairs, which quantifies their non-classical character. We also directly demonstrate entanglement between the 14- and 2-qubit subsystems via an increase in entropy upon partition. In a complementary set of experiments, we probe decoherence of a state prepared in the excited level $J'=J+1$ and interpret spontaneous emission as a loss of a qubit pair in a random state. This allows us to contrast the robustness of pairwise entanglement of the W state with the fragility of the coherence involved in a Schr\"odinger cat state. Our findings open up the possibility to engineer novel types of entangled atomic ensembles, in which entanglement occurs within each atom's electronic spin as well as between different atoms., Comment: 14 pages, 10 figures

Quantum Hall systems are characterized by the quantization of the Hall conductance -- a bulk property rooted in the topological structure of the underlying quantum states. In condensed matter devices, material imperfections hinder a direct connection to simple topological models. Artificial systems, such as photonic platforms or cold atomic gases, open novel possibilities by enabling specific probes of topology or flexible manipulation e.g. using synthetic dimensions. However, the relevance of topological properties requires the notion of a bulk, which was missing in previous works using synthetic dimensions of limited sizes. Here, we realize a quantum Hall system using ultracold dysprosium atoms, in a two-dimensional geometry formed by one spatial dimension and one synthetic dimension encoded in the atomic spin $J=8$. We demonstrate that the large number of magnetic sublevels leads to distinct bulk and edge behaviors. Furthermore, we measure the Hall drift and reconstruct the local Chern marker, an observable that has remained, so far, experimentally inaccessible. In the center of the synthetic dimension -- a bulk of 11 states out of 17 -- the Chern marker reaches 98(5)\% of the quantized value expected for a topological system. Our findings pave the way towards the realization of topological many-body phases., Comment: 18 pages, 16 figures

We report on an experimental study of the Lipkin-Meshkov-Glick model of quantum spins interacting at infinite range in a transverse magnetic field, which exhibits a ferromagnetic phase transition in the thermodynamic limit. We use Dysprosium atoms of electronic spin $J=8$, subjected to a quadratic Zeeman light shift, to simulate $2J=16$ interacting spins $1/2$. We probe the system microscopically using single magnetic sublevel resolution, giving access to the spin projection parity, which is the collective observable characterizing the underlying $\mathbb{Z}_2$ symmetry. We measure the thermodynamic properties and dynamical response of the system, and study the quantum critical behavior around the transition point. In the ferromagnetic phase, we achieve coherent tunneling between symmetry-broken states, and test the link between symmetry breaking and the appearance of a finite order parameter., Comment: 13 pages, 13 figures

The precision of a quantum sensor can overcome its classical counterpart when its constituents are entangled. In gaussian squeezed states, quantum correlations lead to a reduction of the quantum projection noise below the shot noise limit. However, the most sensitive states involve complex non-gaussian quantum fluctuations, making the required measurement protocol challenging. Here we measure the sensitivity of non-classical states of the electronic spin $J = 8$ of dysprosium atoms, created using light-induced non-linear spin coupling. Magnetic sublevel resolution enables us to reach the optimal sensitivity of non-gaussian (oversqueezed) states, well above the capability of squeezed states and about half the Heisenberg limit., Comment: 10 pages, 9 figures

Coherent superposition states of a mesoscopic quantum object play a major role in our understanding of the quantum to classical boundary, as well as in quantum-enhanced metrology and computing. However, their practical realization and manipulation remains challenging, requiring a high degree of control of the system and its coupling to the environment. Here, we use dysprosium atoms - the most magnetic element in its ground state - to realize coherent superpositions between electronic spin states of opposite orientation, with a mesoscopic spin size J=8. We drive coherent spin states to quantum superpositions using non-linear light-spin interactions, observing a series of collapses and revivals of quantum coherence. These states feature highly non-classical behavior, with a sensitivity to magnetic fields enhanced by a factor 13.9(1.1) compared to coherent spin states - close to the Heisenberg limit 2J=16 - and an intrinsic fragility to environmental noise., Comment: 11 pages, 6 figures

We characterize the anisotropic differential ac-Stark shift for the Dy $626$ nm intercombination transition, induced in a far-detuned $1070$ nm optical dipole trap, and observe the existence of a "magic polarization" for which the polarizabilities of the ground and excited states are equal. From our measurements we extract both the scalar and tensorial components of the dynamic dipole polarizability for the excited state, $\alpha_E^\text{s} = 188 (12)\,\alpha_\text{0}$ and $\alpha_E^\text{t} = 34 (12)\,\alpha_\text{0}$, respectively, where $\alpha_\text{0}$ is the atomic unit for the electric polarizability. We also provide a theoretical model allowing us to predict the excited state polarizability and find qualitative agreement with our observations. Furthermore, we utilize our findings to optimize the efficiency of Doppler cooling of a trapped gas, by controlling the sign and magnitude of the inhomogeneous broadening of the optical transition. The resulting initial gain of the collisional rate allows us, after forced evaporation cooling, to produce a quasi-pure Bose-Einstein condensate of $^{162}$Dy with $3\times 10^4$ atoms., Comment: 6 pages, 4 figures