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Abstract: Roof rainwater harvesting (RWH) has the potential to augment water supplies for urban and suburban uses throughout the United States (U.S.). Studies of the performance of RWH at the building and city scales in the U.S. are available, but a countrywide overview of the potential performance of RWH at the county scale has not been done before. Three approaches were taken: (1) assess the viability of RWH in terms of the rainfall that could be captured in relation to the water demand in each county (excluding agriculture), (2) evaluate the performance of a “typical” domestic RWH system across all counties with metrics related to its ability to supply the potable and nonpotable demand, and (3) evaluate the effect of adding a 50% rainwater reuse component to the analysis. We find RWH could be a viable supplemental water source in the U.S., particularly in counties of the Pacific Northwest, Central, and Eastern regions (percent demand covered >50%). Low population density counties have the potential to meet their annual water needs with RWH, while high‐density counties could only source a small portion (~20%) of their annual demand with RWH. Typical RWH systems in counties in the Central and Eastern U.S. performed better than in Western counties. Adding a reuse component can be a key factor in making RWH attractive in many areas of the country. This work can inform future water infrastructure investment and planning in the U.S. [ABSTRACT FROM AUTHOR]