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We compare methods for signal classification applied to voltage traces from transition edge sensors (TES) which are photon-number resolving detectors fundamental for accessing quantum advantages in information processing, communication and metrology. We quantify the impact of numerical analysis on the distinction of such signals. Furthermore, we explore dimensionality reduction techniques to create interpretable and precise photon number embeddings. We demonstrate that the preservation of local data structures of some nonlinear methods is an accurate way to achieve unsupervised classification of TES traces. We do so by considering a confidence metric that quantifies the overlap of the photon number clusters inside a latent space. Furthermore, we demonstrate that for our dataset previous methods such as the signal's area and principal component analysis can resolve up to 16 photons with confidence above $90\%$ while nonlinear techniques can resolve up to 21 with the same confidence threshold. Also, we showcase implementations of neural networks to leverage information within local structures, aiming to increase confidence in assigning photon numbers. Finally, we demonstrate the advantage of some nonlinear methods to detect and remove outlier signals., Comment: Code is publicly available at https://github.com/polyquantique/Photon-Number-Classification. Data is publicly available at https://doi.org/10.5281/zenodo.14042152 and https://doi.org/10.5281/zenodo.14101974

Multiphoton interference is crucial to many photonic quantum technologies. In particular, interference forms the basis of optical quantum information processing platforms and can lead to significant computational advantages. It is therefore interesting to study the interference arising from various states of light in large interferometric networks. Here, we implement a quantum walk in a highly stable, low-loss, multiport interferometer with up to 24 ultrafast time bins. This time-bin interferometer comprises a sequence of birefringent crystals which produce pulses separated by 4.3\,ps, all along a single optical axis. Ultrafast Kerr gating in an optical fiber is employed to time-demultiplex the output from the quantum walk. We measure one-, two-, and three-photon interference arising from various input state combinations, including a heralded single-photon state, a thermal state, and an attenuated coherent state at one or more input ports. Our results demonstrate that ultrafast time bins are a promising platform to observe large-scale multiphoton interference.

In this work, we introduce a quantum-based quantitative phase microscopy technique using a phase gradient approach that is inherently background resistant and does not rely on interferometry or scanning. Here, a transparent sample is illuminated by both photons of a position-momentum entangled pair with one photon setup for position measurement in the near-field (NF) of the sample and its partner for momentum measurement in the far-field (FF). By virtue of the spatial correlation property inherent to the entanglement, both the position and momentum information of the photons can thus be obtained simultaneously. The phase profile of the sample is then deduced through a phase gradient measurement obtained by measuring the centroid shift of the photons' in the FF momentum plane for each NF position. We show that the technique, while achieving an imaging resolution of 2.76\,$\mu$m, is phase accurate to at least $\lambda/30$ and phase sensitive to $\lambda/100$ at a wavelength of 810\,nm. In addition, through the temporal correlation between the photon pairs, our technique shows resilience to strong dynamic background lights, which can prove difficult to account for in classical phase imaging techniques. We believe this work marks a significant advancement in the capabilities of quantum phase microscopy and quantum imaging in general, it showcases imaging and phase resolutions approaching those attainable with classical phase microscopes. This advancement brings quantum imaging closer to practical real-world applications, heralding new possibilities in the field.

Strongly-driven nonlinear optical processes such as spontaneous parametric down-conversion and spontaneous four-wave mixing can produce multiphoton nonclassical beams of light which have applications in quantum information processing and sensing. In contrast to the low-gain regime, new physical effects arise in a high-gain regime due to the interactions between the nonclassical light and the strong pump driving the nonlinear process. Here, we describe and experimentally observe a gain-induced group delay between the multiphoton pulses generated in a high-gain type-II spontaneous parametric down-conversion source. Since the group delay introduces distinguishability between the generated photons, it will be important to compensate for it when designing quantum interference devices in which strong optical nonlinearities are required., Comment: 18 pages, 9 figures (including supplemental material)

We propose a quantum information processing platform that utilizes the ultrafast time-bin encoding of photons. This approach offers a pathway to scalability by leveraging the inherent phase stability of collinear temporal interferometric networks at the femtosecond-to-picosecond timescale. The proposed architecture encodes information in ultrafast temporal bins processed using optically induced nonlinearities and birefringent materials while keeping photons in a single spatial mode. We demonstrate the potential for scalable photonic quantum information processing through two independent experiments that showcase the platform's programmability and scalability, respectively. The scheme's programmability is demonstrated in the first experiment, where we successfully program 362 different unitary transformations in up to 8 dimensions in a temporal circuit. In the second experiment, we show the scalability of ultrafast time-bin encoding by building a passive optical network, with increasing circuit depth, of up to 36 optical modes. In each experiment, fidelities exceed 97\%, while the interferometric phase remains passively stable for several days., Comment: 7 pages, 3 figures

The quantum walk (QW) has proven to be a valuable testbed for fundamental inquiries in quantum technology applications such as quantum simulation and quantum search algorithms. Many benefits have been found by exploring implementations of QWs in various physical systems, including photonic platforms. Here, we propose a novel platform to perform quantum walks using an ultrafast time-bin encoding (UTBE) scheme. This platform supports the scalability of quantum walks to a large number of steps while retaining a significant degree of programmability. More importantly, ultrafast time bins are encoded at the picosecond time scale, far away from mechanical fluctuations. This enables the scalability of our platform to many modes while preserving excellent interferometric phase stability over extremely long periods of time without requiring active phase stabilization. Our 18-step QW is shown to preserve interferometric phase stability over a period of 50 hours, with an overall walk fidelity maintained above $95\%$, Comment: 13 pages, 8 figures

In recent years, neural networks have been used to solve phase retrieval problems in imaging with superior accuracy and speed than traditional techniques, especially in the presence of noise. However, in the context of interferometric imaging, phase noise has been largely unaddressed by existing neural network architectures. Such noise arises naturally in an interferometer due to mechanical instabilities or atmospheric turbulence, limiting measurement acquisition times and posing a challenge in scenarios with limited light intensity, such as remote sensing. Here, we introduce a 3D-2D Phase Retrieval U-Net (PRUNe) that takes noisy and randomly phase-shifted interferograms as inputs, and outputs a single 2D phase image. A 3D downsampling convolutional encoder captures correlations within and between frames to produce a 2D latent space, which is upsampled by a 2D decoder into a phase image. We test our model against a state-of-the-art singular value decomposition algorithm and find PRUNe reconstructions consistently show more accurate and smooth reconstructions, with a x2.5 - 4 lower mean squared error at multiple signal-to-noise ratios for interferograms with low (< 1 photon/pixel) and high (~100 photons/pixel) signal intensity. Our model presents a faster and more accurate approach to perform phase retrieval in extremely low light intensity interferometry in presence of phase noise, and will find application in other multi-frame noisy imaging techniques.

We demonstrate the generation of photons within a fiber-cavity quantum memory, followed by later on-demand readout. Signal photons are generated by spontaneous four-wave mixing in a fiber cavity comprising a birefringent fiber with dichroic reflective end facets. The detection of the partner herald photon indicates the creation of the stored signal photon. After a delay, the signal photon is switched out of resonance with the fiber cavity by intracavity frequency translation using Bragg scattering four-wave mixing, driven by ancillary control pulses. We measure sub-Poissonian statistics in the output signal mode, with $g^{(2)}_{AC}=0.54(1)$ in the first readout bin and a readout frequency translation efficiency of $\approx$80%. The 1/e memory lifetime is $\approx$67 cavity cycles, or 1.68$\mu$s. In an alternate fiber cavity, we show a strategy for noise reduction and measure $g^{(2)}_{AC}=0.068(10)$ after one cavity cycle., Comment: 6 pages, 3 figures

Holography is an established technique for measuring the wavefront of optical signals through interferometric combination with a reference wave. Conventionally the integration time of a hologram is limited by the interferometer coherence time, thus making it challenging to prepare holograms of remote objects, especially using weak illumination. Here, we circumvent this limitation by using intensity correlation interferometry. Although the exposure time of individual holograms must be shorter than the interferometer coherence time, we show that any number of randomly phase-shifted holograms can be combined into a single intensity-correlation hologram. In a proof-of-principle experiment, we use this technique to perform phase imaging and 3D reconstruction of an object at a ~3m distance using weak illumination and without active phase stabilization., Comment: 10 pages; 3 figures

Recent experimental progress in quantum optics has enabled measurement of single photons on ultrafast timescales, beyond the resolution limit of single photon detectors. The energy-time degree of freedom has emerged as a promising avenue for quantum technologies, as entanglement between the frequency and temporal properties of two photons can be fully explored and utilized. Here, we implement optical Kerr shutters in single mode fibers to map out the sub-picosecond correlations of energy-time entangled photon pairs. These measurements, in addition to joint spectral measurements of the photon pair state, are used to verify entanglement by means of the violation of a time-bandwidth inequality., Comment: 5 pages, 4 figures

Time-bin qudits have emerged as a promising encoding platform in many quantum photonic applications. However, the requirement for efficient single-shot measurement of time-bin qudits instead of reconstructive detection has restricted their widespread use in experiments. Here, we propose an efficient method to measure arbitrary superposition states of time-bin qudits and confirm it up to dimension 4. This method is based on encoding time bins at the picosecond time scale, also known as ultrafast time bins. By doing so, we enable the use of robust and phase-stable single spatial mode temporal interferometers to measure time-bin qudit in different measurement bases., Comment: 9 pages, 8 figures

Light-field microscopy (LFM) is a 3D microscopy technique whereby volumetric information of a sample is gained by simultaneously capturing both the position and momentum (angular) information of light illuminating a scene. Conventional LFM designs generally require a trade-off between position and momentum resolution, requiring one to sacrifice resolving power for increased depth of field (DOF) or vice versa. In this work, we demonstrate a LFM design that does not require this trade-off by utilizing the inherent correlations between spatial-temporal entangled photon pairs. Here, one photon from the pair is used to illuminate a sample from which the position information of the photon is captured directly by a camera. By virtue of the strong momentum anti-correlation between the two photons, the momentum information of the illumination photon can then be inferred by measuring the angle of its entangled partner on a different camera. By using a combination of ray-tracing and a Gerchberg-Saxton type algorithm for the light field reconstruction, we demonstrate that a resolving power of 5 $\mu$m can be maintained with a DOF of $\sim500$ $\mu$m, approximately 3 times of the latest LFM designs or $>100$ time that of a conventional microscope. In the extreme, at a resolving power of 100 $\mu$m, it is possible to achieve near infinite DOF., Comment: 16 pages, 9 figures

A phase-sensitive microscopy technique is proposed and demonstrated that employs the momentum correlations inherent in spontaneous parametric down-conversion. One photon from a correlated pair is focused onto a microscopic target while the other is measured in the Fourier plane. This provides knowledge of the position and angle of illumination for every photon striking the target, allowing full post-production control of the illumination angle used to form an image. The versatility of this approach is showcased with asymmetric illumination and differential phase contrast imaging, without any beam blocks or moving parts., Comment: 5 pages, 3 figures

We show a simple yet effective method that can be used to characterize the per pixel quantum efficiency and temporal resolution of a single photon event camera for quantum imaging applications. Utilizing photon pairs generated through spontaneous parametric down-conversion, the detection efficiency of each pixel, and the temporal resolution of the system, are extracted through coincidence measurements. We use this method to evaluate the TPX3CAM, with appended image intensifier, and measure an average efficiency of 7.4% and a temporal resolution of 7.3ns. Furthermore, this technique reveals important error mechanisms that can occur in post-processing. We expect that this technique, and elements therein, will be useful to characterise other quantum imaging systems., Comment: 9 pages, 5 figures

Hyperspectral imaging (HSI) has a wide range of applications from environmental monitoring to biotechnology. Current snapshot HSI techniques all require a trade-off between spatial and spectral resolution and are thus unable to achieve high resolutions in both simultaneously. Additionally, the techniques are resource inefficient with most of the photons lost through spectral filtering. Here, we demonstrate a snapshot HSI technique utilizing the strong spectro-temporal correlations inherent in entangled photons using a modified quantum ghost spectroscopy system, where the target is directly imaged with one photon and the spectral information gained through ghost spectroscopy from the partner photon. As only a few rows of pixels near the edge of the camera are used for the spectrometer, almost no spatial resolution is sacrificed for spectral. Also since no spectral filtering is required, all photons contribute to the HSI process making the technique much more resource efficient.

We propose a quantum memory protocol based on trapping photons in a fiber-integrated cavity, comprised of a birefringent fiber with dichroic reflective end facets. Photons are switched into resonance with the fiber cavity by intracavity Bragg-scattering frequency translation, driven by ancillary control pulses. After the storage delay, photons are switched out of resonance with the cavity, again by intracavity frequency translation. We demonstrate storage of quantum-level THz-bandwidth coherent states for a lifetime up to 16 cavity round trips, or 200ns, and a maximum overall efficiency of 73%., Comment: 7 pages, 5 figures

To capture the 3D information of a scene, conventional techniques often require multiple 2D images of the scene to be captured from different perspectives. In this work we demonstrate the reconstruction of a scene's 3D information through ray-tracing using quantum correlated photon pairs. By capturing the two photons in different image planes using time-tagging cameras and taking advantage of the position, momentum and time correlation of the photons, the photons' propagation trajectory can be reconstructed. With this information on every photon pair, we were able to demonstrate refocusing, depth of field adjustment and parallax visualization of a 3D scene. With future camera advancements, this technique could achieve a much higher momentum resolution than conventional techniques thus giving larger depth of field and more viewing angles. The high photon correlation and low photon flux from a quantum source also makes the technique well suited for 3D imaging of light sensitive samples.

The photonic temporal degree of freedom is one of the most promising platforms for quantum communication over fiber networks and free-space channels. In particular, time-bin states of photons are robust to environmental disturbances, support high-rate communication, and can be used in high-dimensional schemes. However, the detection of photonic time-bin states remains a challenging task, particularly for the case of photons that are in a superposition of different time-bins. Here, we experimentally demonstrate the feasibility of picosecond time-bin states of light, known as ultrafast time-bins, for applications in quantum communications. With the ability to measure time-bin superpositions with excellent phase stability, we enable the use of temporal states in efficient quantum key distribution protocols such as the BB84 protocol., Comment: 8 pages, 6 figures

In this work we demonstrate spectral-temporal correlation measurements of the Hong-Ou-Mandel (HOM) interference effect with the use of a spectrometer based on a photon-counting camera. This setup allows us to take, within seconds, spectral temporal correlation measurements on entangled photon sources with sub-nanometer spectral resolution and nanosecond timing resolution. Through post processing, we can observe the HOM behaviour for any number of spectral filters of any shape and width at any wavelength over the observable spectral range. Our setup also offers great versatility in that it is capable of operating at a wide spectral range from the visible to the near infrared and does not require a pulsed pump laser for timing purposes. This work offers the ability to gain large amounts of spectral and temporal information from a HOM interferometer quickly and efficiently and will be a very useful tool for many quantum technology applications and fundamental quantum optics research.

At the fundamental level, quantum communication is ultimately limited by noise. For instance, quantum signals cannot be amplified without the introduction of noise in the amplified states. Furthermore, photon loss reduces the signal-to-noise ratio, accentuating the effect of noise. Thus, most of the efforts in quantum communications have been directed towards overcoming noise to achieve longer communication distances, larger secret key rates, or to operate in noisier environmental conditions. Here, we propose and experimentally demonstrate a platform for quantum communication based on ultrafast optical techniques. In particular, our scheme enables the experimental realization of high-rates and quantum signal filtering approaching a single spectro-temporal mode, resulting in a dramatic reduction in channel noise. By experimentally realizing a 1-ps optically induced temporal gate, we show that ultrafast time filtering can result in an improvement in noise tolerance by a factor of up to 1200 compared to a 2-ns electronic filter enabling daytime quantum key distribution or quantum communication in bright fibers., Comment: 11 pages, 9 figures

It has been recently suggested that optical interferometers may not require a phase-stable optical link between the stations if instead sources of quantum-mechanically entangled pairs could be provided to them, enabling extra-long baselines and benefiting numerous topics in astrophysics and cosmology. We developed a new variation of this idea, proposing that photons from two different sources could be interfered at two decoupled stations, requiring only a slow classical connection between them. We show that this approach could allow high-precision measurements of the relative astrometry of the two sources, with a simple estimate giving angular resolution of $10 \ \mu$as in a few hours' observation of two bright stars. We also give requirements on the instrument for these observations, in particular on its temporal and spectral resolution. Finally, we discuss possible technologies for the instrument implementation and first proof-of-principle experiments., Comment: intended for SPIE Astronomical Telescopes + Instrumentation 2020 conference

We describe a simple multivariate technique of likelihood ratios for improved discrimination of signal and background in multi-dimensional quantum target detection. The technique combines two independent variables, time difference and summed energy, of a photon pair from the spontaneous parametric down-conversion source into an optimal discriminant. The discriminant performance was studied in experimental data and in Monte-Carlo modelling with clear improvement shown compared to previous techniques. As novel detectors become available, we expect this type of multivariate analysis to become increasingly important in multi-dimensional quantum optics., Comment: The following article has been published by Applied Physics Letters. It can be found at https://aip.scitation.org/doi/10.1063/5.0012429

In order to enhance LIDAR performance metrics such as target detection sensitivity, noise resilience and ranging accuracy, we exploit the strong temporal correlation within the photon pairs generated in continuous-wave pumped semiconductor waveguides. The enhancement attained through the use of such non-classical sources is measured and compared to a corresponding target detection scheme based on simple photon-counting detection. The performances of both schemes are quantified by the estimation uncertainty and Fisher information of the probe photon transmission, which is a widely adopted sensing figure of merit. The target detection experiments are conducted with high probe channel loss (\(\simeq 1-5\times10^{-5}\)) and formidable environment noise up to 36 dB stronger than the detected probe power of \(1.64\times 10^{-5}\) pW. The experimental result shows significant advantages offered by the enhanced scheme with up to 26.3 dB higher performance in terms of estimation uncertainty, which is equivalent to a reduction of target detection time by a factor of 430 or 146 (21.6 dB) times more resilience to noise. We also experimentally demonstrated ranging with these non-classical photon pairs generated with continuous-wave pump in the presence of strong noise and loss, achieving \(\approx\)5 cm distance resolution that is limited by the temporal resolution of the detectors.

Underwater quantum communication has recently been explored using polarization and orbital angular momentum. Here, we show that spatially structured modes, e.g., a coherent superposition of beams carrying both polarization and orbital angular momentum, can also be used for underwater quantum cryptography. We also use the polarization degree of freedom for quantum communication in an underwater channel having various lengths, up to $30$ meters. The underwater channel proves to be a difficult environment for establishing quantum communication as underwater optical turbulence results in significant beam wandering and distortions. However, the errors associated to the turbulence do not result in error rates above the threshold for establishing a positive key in a quantum communication link with both the polarization and spatially structured photons. The impact of the underwater channel on the spatially structured modes is also investigated at different distances using polarization tomography., Comment: 7 pages, 3 figures, 3 tables

Interaction between Rydberg atoms can significantly modify Rydberg excitation dynamics. Under a resonant driving field the Rydberg-Rydberg interaction in high-lying states can induce shifts in the atomic resonance such that a secondary Rydberg excitation becomes unlikely leading to the Rydberg blockade effect. In a related effect, off-resonant coupling of light to Rydberg states of atoms contributes to the Rydberg anti-blockade effect where the Rydberg interaction creates a resonant condition that promotes a secondary excitation in a Rydberg atomic gas. Here, we study the light-matter interaction and dynamics of off-resonant two-photon excitations and include two- and three-atom Rydberg interactions and their effect on excited state dynamics in an ensemble of cold atoms. In an experimentally-motivated regime, we find the optimal physical parameters such as Rabi frequencies, two-photon detuning, and pump duration to achieve significant enhancement in the probability of generating doubly-excited collective atomic states. This results in large auto-correlation values due to the Rydberg anti-blockade effect and makes this system a potential candidate for a high-purity two-photon Fock state source., Comment: 7 pages, 8 figures

In this work we investigate quantum-enhanced target detection in the presence of large background noise using multidimensional quantum correlations between photon pairs generated through spontaneous parametric down-conversion. Until now similar experiments have only utilized one of the photon pairs' many degrees of freedom such as temporal correlations and photon number correlations. Here, we utilized both temporal and spectral correlations of the photon pairs and achieved over an order of magnitude reduction to the background noise and in turn significant reduction to data acquisition time when compared to utilizing only temporal modes. We believe this work represents an important step in realizing a practical, real-time quantum-enhanced target detection system. The demonstrated technique will also be of importance in many other quantum sensing applications and quantum communications., Comment: 9 pages, 7 figures

We examine the propagation of optical beams possessing different polarization states and spatial modes through the Ottawa River in Canada. A Shack-Hartmann wavefront sensor is used to record the distorted beam's wavefront. The turbulence in the underwater channel is analysed, and associated Zernike coefficients are obtained in real-time. Finally, we explore the feasibility of transmitting polarization states as well as spatial modes through the underwater channel for applications in quantum cryptography., Comment: 5 pages, 4 figures. Comments welcome

We investigate the use of correlated photon pair sources for the improved quantum-level detection of a target in the presence of a noise background. Photon pairs are generated by spontaneous four-wave mixing, one photon from each pair (the herald) is measured locally while the other (the signal) is sent to illuminate the target. Following diffuse reflection from the target, the signal photons are detected by a receiver and non-classical timing correlations between the signal and herald are measured in the presence of a configurable background noise source. Quantum correlations from the photon pair source can be used to provide an enhanced signal-to-noise ratio when compared to a classical light source of the same intensity., Comment: 8 pages, 9 figures

Optically induced ultrafast switching of single photons is demonstrated by rotating the photon polarization via the Kerr effect in a commercially available single mode fiber. A switching efficiency of 97\% is achieved with a $\sim1.7$\,ps switching time, and signal-to-noise ratio of $\sim800$. Preservation of the quantum state is confirmed by measuring no significant increase in the second-order autocorrelation function $g^{(2)}(0)$. These values are attained with only nanojoule level pump energies that are produced by a laser oscillator with 80\,MHz repetition rate. The results highlight a simple switching device capable of both high-bandwidth operations and preservation of single-photon properties for applications in photonic quantum processing and ultrafast time-gating or switching.

Quantum key distribution is on the verge of real world applications, where perfectly secure information can be distributed among multiple parties. Several quantum cryptographic protocols have been theoretically proposed and independently realized in different experimental conditions. Here, we develop an experimental platform based on high-dimensional orbital angular momentum states of single photons that enables implementation of multiple quantum key distribution protocols with a single experimental apparatus. Our versatile approach allows us to experimentally survey different classes of quantum key distribution techniques, such as the 1984 Bennett \& Brassard (BB84), tomographic protocols including the six-state and the Singapore protocol, and to investigate, for the first time, a recently introduced differential phase shift (Chau15) protocol using twisted photons. This enables us to experimentally compare the performance of these techniques and discuss their benefits and deficiencies in terms of noise tolerance in different dimensions., Comment: 13 pages, 4 figures, 1 table

The encoding of quantum information in photonic time-bin qubits is apt for long distance quantum communication schemes. In practice, due to technical constraints such as detector response time, or the speed with which co-polarized time-bins can be switched, other encodings, e.g. polarization, are often preferred for operations like state detection. Here, we present the conversion of qubits between polarization and time-bin encodings using a method that is based on an ultrafast optical Kerr shutter and attain efficiencies of 97% and an average fidelity of 0.827+/-0.003 with shutter speeds near 1 ps. Our demonstration delineates an essential requirement for the development of hybrid and high-rate optical quantum networks.

Bulk diamond phonons have been shown to be a versatile platform for the generation, storage, and manipulation of high-bandwidth quantum states of light. Here we demonstrate a diamond quantum memory that stores, and releases on demand, an arbitrarily polarized $\sim$250 fs duration photonic qubit. The single-mode nature of the memory is overcome by mapping the two degrees of polarization of the qubit, via Raman transitions, onto two spatially distinct optical phonon modes located in the same diamond crystal. The two modes are coherently recombined upon retrieval and quantum process tomography confirms that the memory faithfully reproduces the input state with average fidelity $0.784\pm0.004$ with a total memory efficiency of $(0.76\pm0.03)\%$. In an additional demonstration, one photon of a polarization-entangled pair is stored in the memory. We report that entanglement persists in the retrieved state for up to 1.3 ps of storage time. These results demonstrate that the diamond phonon platform can be used in concert with polarization qubits, a key requirement for polarization-encoded photonic processing.

Quantum light-matter interfaces are at the heart of photonic quantum technologies. Quantum memories for photons, where non-classical states of photons are mapped onto stationary matter states and preserved for subsequent retrieval, are technical realizations enabled by exquisite control over interactions between light and matter. The ability of quantum memories to synchronize probabilistic events makes them a key component in quantum repeaters and quantum computation based on linear optics. This critical feature has motivated many groups to dedicate theoretical and experimental research to develop quantum memory devices. In recent years, exciting new applications, and more advanced developments of quantum memories, have proliferated. In this review, we outline some of the emerging applications of quantum memories in optical signal processing, quantum computation, and nonlinear optics. We review recent experimental and theoretical developments, and their impacts on more advanced photonic quantum technologies based on quantum memories., Comment: Review paper. Comments are welcome!

Controlling the properties of single photons is essential for a wide array of emerging optical quantum technologies spanning quantum sensing, quantum computing, and quantum communications. Essential components for these technologies include single photon sources, quantum memories, waveguides, and detectors. The ideal spectral operating parameters (wavelength and bandwidth) of these components are rarely similar; thus, frequency conversion and spectral control are key enabling steps for component hybridization. Here we perform signal processing of single photons by coherently manipulating their spectra via a modified quantum memory. We store 723.5 nm photons, with 4.1 nm bandwidth, in a room-temperature diamond crystal; upon retrieval we demonstrate centre frequency tunability over 4.2 times the input bandwidth, and bandwidth modulation between 0.5 to 1.9 times the input bandwidth. Our results demonstrate the potential for diamond, and Raman memories in general, to be an integrated platform for photon storage and spectral conversion., Comment: 6 pages, 4 figures

We propose and experimentally demonstrate a scheme to generate optically-controlled delays based on off-resonant Raman absorption. Dispersion in a transparency window between two neighboring, optically-activated Raman absorption lines is used to reduce the group velocity of broadband 765 nm pulses. We implement this approach in a potassium titanyl phosphate (KTP) waveguide at room temperature, and demonstrate Raman-induced delays of up to 140 fs for a 650-fs duration, 1.8-THz bandwidth, signal pulse; the available delay-bandwidth product is $\approx1$. Our approach is applicable to single photon signals, offers wavelength tunability, and is a step toward processing ultrafast photons., Comment: 5+4 pages, 4+2 figures

We report the storage and retrieval of single photons, via a quantum memory, in the optical phonons of room-temperature bulk diamond. The THz-bandwidth heralded photons are generated by spontaneous parametric downconversion and mapped to phonons via a Raman transition, stored for a variable delay, and released on demand. The second-order correlation of the memory output is $g^{(2)}(0) = 0.65 \pm 0.07$, demonstrating preservation of non-classical photon statistics throughout storage and retrieval. The memory is low-noise, high-speed and broadly tunable; it therefore promises to be a versatile light-matter interface for local quantum processing applications., Comment: 6 pages, 4 figures

The unusual features of quantum mechanics are enabling the development of technologies not possible with classical physics. These devices utilize nonclassical phenomena in the states of atoms, ions, and solid-state media as the basis for many prototypes. Here we investigate molecular states as a distinct alternative. We demonstrate a memory for light based on storing photons in the vibrations of hydrogen molecules. The THz-bandwidth molecular memory is used to store 100-fs pulses for durations up to 1ns, enabling 10,000 operational time bins. The results demonstrate the promise of molecules for constructing compact ultrafast quantum photonic technologies., Comment: 5 pages, 3 figures, 1 table

The generation of large multiphoton quantum states - for applications in computing, metrology, and simulation - requires a network of high-efficiency quantum memories capable of storing broadband pulses. Integrating these memories into a fibre offers a number of advantages towards realising this goal: strong light-matter coupling at low powers, simplified alignment, and compatibility with existing photonic architectures. Here, we introduce a large-core kagome-structured hollow-core fibre as a suitable platform for an integrated fibre-based quantum memory with a warm atomic vapour. We demonstrate, for the first time, efficient optical pumping in a hollow-core photonic-crystal fibre with a warm atomic vapour, where (90 $\pm$ 1)% of atoms are prepared in the ground state. We measure high optical depths (3$\times 10^{4}$) and, also, narrow homogeneous linewidths that do not exhibit significant transit-time broadening. Our results establish that kagome fibres are suitable for implementing a broadband, room-temperature quantum memory., Comment: 10 pages, 4 figures

The complexity of ultrafast molecular photoionization presents an obstacle to the modelling of pump-probe experiments. Here, a simple optimized model of atomic rubidium is combined with a molecular dynamics model to predict quantitatively the results of a pump-probe experiment in which long range rubidium dimers are first excited, then ionized after a variable delay. The method is illustrated by the outline of two proposed feasible experiments and the calculation of their outcomes. Both of these proposals use Feshbach 87Rb2 molecules. We show that long-range molecular pump-probe experiments should observe spin-orbit precession given a suitable pump-pulse, and that the associated high-frequency beat signal in the ionization probability decays after a few tens of picoseconds. If the molecule was to be excited to only a single fine structure state state, then a low-frequency oscillation in the internuclear separation would be detectable through the timedependent ionization cross section, giving a mechanism that would enable observation of coherent vibrational motion in this molecule., Comment: 9 pages, 10 figures, PRA submission

Calculations relating to two experiments that demonstrate coherent control of preformed rubidium-85 molecules in a magneto-optical trap using ultrafast laser pulses are presented. In the first experiment, it is shown that pre-associated molecules in an incoherent mixture of states can be made to oscillate coherently using a single ultrafast pulse. A mechanism that can transfer molecular population to more deeply bound vibrational levels is used in the second. Optimal parameters of the control pulse are presented for the application of the mechanism to molecules in a magneto-optical trap. The calculations make use of an experimental determination of the initial state of molecules photoassociated by the trapping lasers in the magneto-optical trap and use shaped pulses consistent with a standard ultrafast laser system., Comment: 8 pages, 9 figures, PRA, 80, 033403 (2009)

An experimental pump-probe study of the photoassociative creation of translationally ultracold rubidium molecules is presented together with numerical simulations of the process. The formation of loosely bound excited-state dimers is observed as a first step towards a fully coherent pump-dump approach to the stabilization of Rb$_2$ into its lowest ground vibrational states. The population that contributes to the pump-probe process is characterized and found to be distinct from a background population of pre-associated molecules., Comment: Accepted for publication in Phys. Rev. A (10 pages, 9 figures)