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The heavy-ion inelastic scattering of the neutron-rich nucleus $^{29}$Ne to its excited states was studied using a 100.1 MeV/u $^{29}$Ne rare isotope beam on $^{181}$Ta and $^{9}$Be targets. The combined setup consisting of the GRETINA array, the TRIPLEX device and the S800 Spectrograph facilitates the simultaneous measurements of the two inelastic reactions, providing the first measurement of the transition strengths for this isotope. A sizable E2 strength B(E2↑) which amounts to 163(30) e$^{2}$fm$^{4}$ was determined in the excitation to the 931-keV state, demonstrating a large degree of collectivity. The present results of B(E2↑) are compared to various shell-model calculations, confirming the role of intruder configurations in $^{29}$Ne at the boundary of the island of inversion.

Discovering unexplored high-spin states in neutron-rich nuclei can open up a new direction to study band structure and the associated shell structure in isospin-asymmetric many-body systems. However, experimental reach has so far been limited to neutron-deficient or stable nuclei which are preferentially produced in fusion reactions used in such studies. Here, we report the first γ-ray spectroscopy with fusion reactions using a reaccelerated rare-isotope beam of 45K performed at the ReA3 facility of the National Superconducting Cyclotron Laboratory. Using particle and γ-ray coincidence techniques, three new higher-lying states around 6 MeV and five new γ-ray transitions were identified for 46Ca, suggesting three independent band structures formed from different particle-hole configurations. The rotational-like band built on the 0+2 state is established up to the tentatively assigned 6+2 state. New results are compared to large-scale shell model calculations, confirming the validity of the effective interaction describing particle-hole excitations across the Z=20 and N=28 shell gaps in the vicinity of doubly magic 48Ca.

The shape and collectivity of 106Cd was investigated via a sub-barrier-energy Coulomb excitation experiment performed at the National Superconducting Cyclotron Laboratory Re-accelerator facility using the JANUS setup. Transition matrix elements between low-lying states were found to agree with adopted values, and information on the shape and collectivity of higher-lying states was extracted for the first time. Locally optimized large-scale shell-model calculations were found to describe well the B(E2) transition strengths but failed to reproduce the spectroscopic quadrupole moments Qs. An analysis of the E2 rotational invariants and the normalized quadrupole moment qs indicates that this may be due to a significant degree of triaxiality in 106Cd which is not captured by the present shell-model calculations. Analogous calculations for the Fe isotopes (two protons below the Z=28 magic number) reveal the critical role of high-j neutron configurations for the description of quadrupole moments in the heavy Fe and Cd isotopes (two protons below magic Z=50), but this effect is insufficient to explain the shape of 106Cd, posing a puzzle for the understanding of nuclear structure towards N=50.

The shape and collectivity of 106Cd was investigated via a sub-barrier-energy Coulomb excitation experiment performed at the National Superconducting Cyclotron Laboratory Re-accelerator facility using the JANUS setup. Transition matrix elements between low-lying states were found to agree with adopted values, and information on the shape and collectivity of higher-lying states was extracted for the first time. Locally optimized large-scale shell-model calculations were found to describe well the B(E2) transition strengths but failed to reproduce the spectroscopic quadrupole moments Qs. An analysis of the E2 rotational invariants and the normalized quadrupole moment qs indicates that this may be due to a significant degree of triaxiality in 106Cd which is not captured by the present shell-model calculations. Analogous calculations for the Fe isotopes (two protons below the Z=28 magic number) reveal the critical role of high-j neutron configurations for the description of quadrupole moments in the heavy Fe and Cd isotopes (two protons below magic Z=50), but this effect is insufficient to explain the shape of 106Cd, posing a puzzle for the understanding of nuclear structure towards N=50.

Energy differences between isobaric analogue states have been extracted for the A=79, $^{79}$Zr/$^{79}$Y mirror pair following their population via nucleon-knockout reactions from intermediate-energy rare-isotope beams. These are the heaviest nuclei where such measurements have been made to date. The deduced mirror energy differences (MED) are compared with predictions from a new density-functional based approach, incorporating isospin-breaking effects of both Coulomb and nuclear charge-symmetry breaking and configuration mixing.

The structure of exotic nuclei provides valuable tests for state-of-the-art nuclear theory. In particular electromagnetic transition rates are more sensitive to aspects of nuclear forces and many-body physics than excitation energies alone. We report the first lifetime measurement of excited states in $^{21}$O, finding τ1/2+=420−32+35(stat)−12+34(sys) ps. This result together with the deduced level scheme and branching ratio of several γ-ray decays are compared to both phenomenological shell-model and ab initio calculations based on two- and three-nucleon forces derived from chiral effective field theory. We find that the electric quadrupole reduced transition probability of B(E2;1/2+→5/2g.s.+)=0.71−0.06−0.06+0.07+0.02 e$^{2}$fm$^{4}$, derived from the lifetime of the 1/2+ state, is smaller than the phenomenological result where standard effective charges are employed, suggesting the need for modifications of the latter in neutron-rich oxygen isotopes. We compare this result to both large-space and valence-space ab initio calculations, and by using multiple input interactions we explore the sensitivity of this observable to underlying details of nuclear forces.

The development of advanced γ-ray tracking arrays allows for a sensitive new technique to investigate elusive states of exotic nuclei with fast rare-isotope beams. By taking advantage of the excellent energy and position resolution of the Gamma-Ray Energy Tracking In-beam Nuclear Array, we developed a novel technique to identify in-flight isomeric decays of the 0⁺₂ state in 32Mg populated in a two-proton removal reaction. We confirm the 0⁺₂→2+1γ-ray transition of ³²Mg and constrain the 0⁺₂ decay lifetime, suggesting a large collectivity. The small partial cross section populating the 0⁺₂ state in this reaction provides experimental evidence for the reduced occupancy of the normal configuration of the 0⁺₂ state, indicating the intruder dominance of this state.

An enhanced low-energy electric dipole (E1) strength is identified for the weakly bound excited states of the neutron-rich isotope ^{27}Ne. The Doppler-shift lifetime measurements employing a combination of the γ-ray tracking array GRETINA, the plunger device, and the S800 spectrograph determine the lower limit of 0.030 e^{2} fm^{2} or 0.052 W.u. for the 1/2^{+}→3/2^{-} E1 transition in ^{27}Ne, representing one of the strongest E1 strengths observed among the bound discrete states in this mass region. This value is at least 30 times larger than that measured for the 3/2^{-} decay to the 3/2_{gs}^{+} ground state. A comparison of the present results to large-scale shell-model calculations points to an important role of core excitations and deformation in the observed E1 enhancement, suggesting a novel example of the electric dipole modes manifested in weakly bound deformed systems.

Current understanding of the behaviour of plasma discharges within packed bed reactors (PBRs) is very poor, and the effects of many of the parameters that can be varied are still unknown. This article investigates the effects of particle size (180μm–2000μm) of two different commonly used packing materials (Al2O3 and BaTiO3) on the conversion of CO2 in PBRs. The reactor behaviour is observed through determination of product gas composition and plasma power consumption in order to determine CO2 conversion and reactor efficiency. Electrical characterisation techniques are used to determine reactor burning voltage, and capacitances. These capacitances are subsequently used to quantify the occurrence of reactor partial discharging over a range of different operating conditions.The results indicate that smaller particles (down to 180μm) can significantly increase CO2 conversion by up to 70%, provided that the voltage applied is sufficiently high to generate a discharge in the void spaces of the packing material. However, with decreasing particle size, the reactor burning voltage is found to increase rapidly, as well as the tendency of the reactor towards partial discharging.

Lifetime measurements of excited states in the neutron-rich nucleus S-43 were performed by applying the recoil-distance method on fast rare-isotope beams in conjunction with the Gamma-Ray Energy Tracking In-beam Nuclear Array. The new data based on gamma gamma coincidences and lifetime measurements resolve a doublet of (3/2(-)) and (5/2(-)) states at low excitation energies. Results were compared to the posdthorn pi(sd) - nu(pf) shell model and antisymmetrized molecular dynamics calculations. The consistency with the theoretical calculations identifies a possible appearance of three coexisting bands near the ground state of S-43: the K-pi =1/2(-) band built on a prolate-deformed ground state, a band built on an isomer with a 1f(7/2)(-1) character, and a suggested excited band built on a newly discovered doublet state. The latter further confirms the collapse of the N = 28 shell closure in the neutron-rich region.