Search

The probabilities for gamma-ray and particle emission as a function of the excitation energy of a decaying nucleus are valuable observables for constraining the ingredients of the models that describe the de-excitation of nuclei near the particle emission threshold. These models are essential in nuclear astrophysics and applications. In this work, we have for the first time simultaneously measured the gamma-ray and neutron emission probabilities of 208Pb. The measurement was performed in inverse kinematics at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, where a 208Pb beam interacted through the 208Pb(p,p') reaction with a hydrogen gas jet target. Instead of detecting the gamma-rays and neutrons emitted by 208Pb, we detected the heavy beam-like residues produced after gamma and neutron emission. These heavy residues were fully separated by a dipole magnet of the ESR and were detected with outstanding efficiencies. The comparison of the measured probabilities with model calculations has allowed us to test different descriptions of the gamma-ray strength function and the nuclear level density available in the literature., Comment: 23 pages, 13 figures

We report the charge-changing cross sections ($\sigma_{\text{cc}}$) of 24 $p$-shell nuclides on both hydrogen and carbon at about 900$A$ MeV, of which $^{8,9}$Li, $^{10\textendash12}$Be, $^{10,14,15}$B, $^{14,15,17\textendash22}$N and $^{16}$O on hydrogen and $^{8,9}$Li on carbon are for the first time. Benefiting from the data set,we found a new and robust relationship between the scaling factor of the Glauber model calculations and the separation energies of the nuclei of interest on both targets.This allows us to deduce proton radii ($R_p$) for the first time from the cross sections on hydrogen. Nearly identical $R_p$ values are deduced from both target data for the neutron-rich carbon isotopes, however, the $R_p$ from the hydrogen target is systematically smaller in the neutron-rich nitrogen isotopes.This calls for further experimental and theoretical investigations., Comment: 5 pages, 3 figures

Isomer spectroscopy of heavy neutron-rich nuclei beyond the N=126 closed shell has been performed for the first time at the Radioactive Isotope Beam Factory of the RIKEN Nishina Center. New millisecond isomers have been identified at low excitation energies, 985.3(19) keV in 213Tl and 874(5) keV in 215Tl. The measured half-lives of 1.34(5) ms in 213Tl and 3.0(3) ms in 215Tl suggest spins and parities 11/2- with the single proton-hole configuration h11/2 as leading component. They are populated via E1 transitions by the decay of higher-lying isomeric states with proposed spin and parity 17/2+, interpreted as arising from a single s1/2 proton hole coupled to the 8+ seniority isomer in the (A+1)Pb cores. The lowering of the 11/2- states is ascribed to an increase of the h11/2 proton effective single-particle energy as the second g9/2 orbital is filled by neutrons, owing to a significant reduction of the proton-neutron monopole interaction between the h11/2 and g9/2 orbitals. The new ms-isomers provide the first experimental observation of shell evolution in the almost unexplored N>126 nuclear region below doubly-magic 208Pb., Comment: 9 pages, 3 figures, 1 table

The cross-shell excited states of $^{34}$Si have been investigated via $\beta$-decays of the $4^-$ ground state and the $1^+$ isomeric state of $^{34}$Al. Since the valence protons and valence neutrons occupy different major shells in the ground state as well as the intruder $1^+$ isomeric state of $^{34}$Al, intruder levels of $^{34}$Si are populated via allowed $\beta$ decays. Spin assignments to such intruder levels of $^{34}$Si were established through $\gamma$-$\gamma$ angular correlation analysis for the negative parity states with dominant configurations $(\nu d_{3/2})^{-1} \otimes (\nu f_{7/2})^{1}$ as well as the positive parity states with dominant configurations $(\nu sd)^{-2} \otimes (\nu f_{7/2}p_{3/2})^2$. The configurations of such intruder states play crucial roles in our understanding of the $N=20$ shell gap evolution. A configuration interaction model derived from the FSU Hamiltonian was utilized in order to interpret the intruder states in $^{34}$Si. Shell model interaction derived from a more fundamental theory with the Valence Space In Medium Similarity Renormalization Group (VS-IMSRG) method was also employed to interpret the structure of $^{34}$Si.

Neutron-induced reaction cross sections of short-lived nuclei are imperative to understand the origin of heavy elements in stellar nucleosynthesis and for societal applications, but their measurement is extremely complicated due to the radioactivity of the targets involved. One way of overcoming this issue is to combine surrogate reactions with the unique possibilities offered by heavy-ion storage rings. In this work, we describe the first surrogate-reaction experiment in inverse kinematics, which we successfully conducted at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, using the 208Pb(p,p') reaction as a surrogate for neutron capture on 207Pb. Thanks to the outstanding detection efficiencies possible at the ESR, we were able to measure for the first time the neutron-emission probability as a function of the excitation energy of 208Pb. We have used this probability to select different descriptions of the gamma-ray strength function and nuclear level density, and provide reliable results for the neutron-induced radiative capture cross section of 207Pb at energies for which no experimental data exist., Comment: 10 pages and 5 figures

The nuclear two-photon or double-gamma ($2\gamma$) decay is a second-order electromagnetic process whereby a nucleus in an excited state emits two gamma rays simultaneously. To be able to directly measure the $2\gamma$ decay rate in the low-energy regime below the electron-positron pair-creation threshold, we combined the isochronous mode of a storage ring with Schottky resonant cavities. The newly developed technique can be applied to isomers with excitation energies down to $\sim100$\,keV and half-lives as short as $\sim10$\,ms. The half-life for the $2\gamma$ decay of the first-excited $0^+$ state in bare $^{72}\mathrm{Ge}$ ions was determined to be $23.9\left(6\right)$\,ms, which strongly deviates from expectations., Comment: Submitted to Physical Review Letters, 8 pages, 3 figures, 2 tables, 7 equations

Low-energy investigations on rare ion beams are often limited by the available intensity and purity of the ion species in focus. Here, we present the first application of a technique that combines in-flight production at relativistic energies with subsequent secondary beam storage, accumulation and finally deceleration to the energy of interest. Using the FRS and ESR facilities at GSI, this scheme was pioneered to provide a secondary beam of $^{118}$Te$^{52+}$ for the measurement of nuclear proton-capture at energies of 6 and 7 MeV/u. The technique provided stored beam intensities of about $10^6$ ions at high purity and brilliance, representing a major step towards low-energy nuclear physics studies using rare ion beams.

\noindent \textbf{Background:} Detailed spectroscopy of neutron-rich, heavy, deformed nuclei is of broad interest for nuclear astrophysics and nuclear structure. Nuclei in the r-process path and following freeze-out region impact the resulting r-process abundance distribution, and the structure of nuclei midshell in both proton and neutron number helps to understand the evolution of subshell gaps and large deformation in these nuclei. \noindent \textbf{Purpose:} To improve the understanding of the nuclear structure of $^{160}$Gd, specifically the $K^\pi$=$4^+$ bands, as well as study the $\beta$-decay of $^{160}$Eu into $^{160}$Gd. \noindent \textbf{Methods:} High-statistics decay spectroscopy of $^{160}$Gd resulting from the $\beta$-decay of $^{160}$Eu was collected using the GRIFFIN spectrometer at the TRIUMF-ISAC facility. \noindent \textbf{Results:} Two new excited states and ten new transitions were observed in $^{160}$Gd. The $\beta$-decaying half-lives of the low- and high-spin isomer in $^{160}$Eu were determined, and the low-spin state's half-life was measured to be $t_{1/2}=26.0(8)$~s, $\sim$16\% shorter than previous measurements. Lifetimes of the two $K^\pi$=$4^+$ band-heads in $^{160}$Gd were measured for the first time, as well as $\gamma$-$\gamma$ angular correlations and mixing ratios of intense transitions out of those band-heads. \noindent \textbf{Conclusions:} Lifetimes and mixing ratios suggest that the hexadecapole phonon model of the $K^\pi$=$4^+$ band-heads in $^{160}$Gd is preferred over a simple two-state strong mixing scenario, although further theoretical calculations are needed to fully understand these states. Additionally, the 1999.0 keV state in $^{160}$Gd heavily populated in $\beta$-decay is shown to have positive parity, which raises questions regarding the structure of the high-spin $\beta$-decaying state in $^{160}$Eu.

The excited states of $N=44$ $^{74}$Zn were investigated via $\gamma$-ray spectroscopy following $^{74}$Cu $\beta$ decay. By exploiting $\gamma$-$\gamma$ angular correlation analysis, the $2_2^+$, $3_1^+$, $0_2^+$ and $2_3^+$ states in $^{74}$Zn were firmly established. The $\gamma$-ray branching and $E2/M1$ mixing ratios for transitions de-exciting the $2_2^+$, $3_1^+$ and $2_3^+$ states were measured, allowing for the extraction of relative $B(E2)$ values. In particular, the $2_3^+ \to 0_2^+$ and $2_3^+ \to 4_1^+$ transitions were observed for the first time. The results show excellent agreement with new microscopic large-scale shell-model calculations, and are discussed in terms of underlying shapes, as well as the role of neutron excitations across the $N=40$ gap. Enhanced axial shape asymmetry (triaxiality) is suggested to characterize $^{74}$Zn in its ground state. Furthermore, an excited $K=0$ band with a significantly larger softness in its shape is identified. A shore of the $N=40$ ``island of inversion'' appears to manifest above $Z=26$, previously thought as its northern limit in the chart of the nuclides.

The performance of high-precision mass spectrometry of radioactive isotopes can often be hindered by large amounts of contamination, including molecular species, stemming from the production of the radioactive beam. In this paper, we report on the development of Collision-Induced Dissociation (CID) as a means of background reduction for experiments at TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). This study was conducted to characterize the quality and purity of radioactive ion beams and the reduction of molecular contaminants to allow for mass measurements of radioactive isotopes to be done further from nuclear stability. This is the first demonstration of CID at an ISOL-type radioactive ion beam facility, and it is shown that molecular contamination can be reduced up to an order of magnitude., Comment: 7 pages 7 figures

The root mean square radii of the proton density distribution in $^{16-24}$O derived from measurements of charge changing cross sections with a carbon target at $\sim$900$A$ MeV together with the matter radii portray thick neutron skin for $^{22 - 24}$O despite $^{22,24}$O being doubly magic. Imprints of the shell closures at $N$ = 14 and 16 are reflected in local minima of their proton radii that provide evidence for the tensor interaction causing them. The radii agree with it ab initio calculations employing the chiral NNLO$_{\mathrm{sat}}$ interaction, though skin thickness predictions are challenged. Shell model predictions agree well with the data., Comment: 6 pages, 3 figures, accepted for publication in Physical Review Letters

Nuclear Astrophysics is a field at the intersection of nuclear physics and astrophysics, which seeks to understand the nuclear engines of astronomical objects and the origin of the chemical elements. This white paper summarizes progress and status of the field, the new open questions that have emerged, and the tremendous scientific opportunities that have opened up with major advances in capabilities across an ever growing number of disciplines and subfields that need to be integrated. We take a holistic view of the field discussing the unique challenges and opportunities in nuclear astrophysics in regards to science, diversity, education, and the interdisciplinarity and breadth of the field. Clearly nuclear astrophysics is a dynamic field with a bright future that is entering a new era of discovery opportunities., Comment: 96 pages. Submitted to Journal of Physics G

We report results on the long-term variation of the neutron counting rate at the Canfranc Underground Laboratory, of importance for several low-background experiments installed there, including rare-event searches. The measurement campaign was performed employing the High Efficiency Neutron Spectrometry Array (HENSA) mounted in Hall A and lasted 412 live days. The present study is the first long-term measurement of the neutron rate with sensitivity over a wide range of neutron energies (from thermal up to 0.1 GeV and beyond) performed in any underground laboratory so far. Data on the environmental variables inside the experimental hall (radon concentration, air temperature, air pressure and humidity) were also acquired during all the measurement campaign. We have investigated for the first time the evolution of the neutron rate for different energies of the neutrons and its correlation with the ambient variables., Comment: 12 pages, 5 figures, 2 tables

We report precision mass measurements of neutron-deficient gallium isotopes approaching the proton drip line. The measurements of $^{60-63}$Ga performed with the TITAN multiple-reflection time-of-flight mass spectrometer provide a more than threefold improvement over the current literature mass uncertainty of $^{61}$Ga and mark the first direct mass measurement of $^{60}$Ga. The improved precision of the $^{61}$Ga mass has important implications for the astrophysical rp process, as it constrains essential reaction Q-values near the $^{60}$Zn waiting point. Based on calculations with a one-zone model, we demonstrate the impact of the improved mass data on prediction uncertainties of X-ray burst models. The first-time measurement of the $^{60}$Ga ground-state mass establishes the proton-bound nature of this nuclide; thus, constraining the location of the proton drip line along this isotopic chain. Including the measured mass of $^{60}$Ga further enables us to extend the evaluated $T=1$ isobaric multiplet mass equation up to $A=60$., Comment: 16 pages, 6 figures

The HENSA/ANAIS collaboration aims for the precise determination of the neutron flux that could affect ANAIS-112, an experiment looking for the dark matter annual modulation using NaI(Tl) scintillators. In this work, the first measurements of the neutron flux and Monte Carlo simulations of the neutron spectrum are reported.

We have performed a long-term measurement of the neutron flux with the High Efficiency Neutron Spectrometry Array HENSA in the Hall A of the Canfranc Underground Laboratory. The Hall A measurement campaign lasted from October 2019 to March 2021, demonstrating an excellent stability of the HENSA setup. Preliminary results on the neutron flux from this campaign are presented for the first time. In Phase 1 (113 live days) a total neutron flux of 1.66(2) $\times$10$^{-5}$ cm$^{-2}$ s$^{-1}$ is obtained. Our results are in good agreement with those from our previous shorter measurement where a reduced experimental setup was employed., Comment: Proceedings of the 17th International Conference on Topics in Astroparticle and Underground Physics (TAUP 2021)

The occurrence of octupole shapes in even-mass neutron-rich Ba isotopes has been well established. However, the situation with the odd-mass Ba and odd or odd-odd La nuclei around them is far from settled. In order to shed light on these less-studied isotopes, a fast-timing experiment was performed using GRIFFIN at TRIUMF-ISAC. A wealth of excited-state lifetimes in the 100~ps to few ns range have been measured in $^{144, 145, 146}$Ba and $^{145,146}$La populated in the $\beta^-$ and $\beta^--n$ decay of $^{145,146}$Cs. The results do not allow to draw firm conclusions on the possible octupole deformation of these nuclei but suggest different spin and parity assignments than previous works. This work highlights the need for more detailed study of the odd and odd-odd isotopes in this region to properly understand their structure., Comment: 16 pages, 7 figures

Beta-delayed neutron emission is important for nuclear structure and astrophysics as well as for reactor applications. Significant advances in nuclear experimental techniques in the past two decades have led to a wealth of new measurements that remain to be incorporated in the databases. We report on a coordinated effort to compile and evaluate all the available beta-delayed neutron emission data. The different measurement techniques have been assessed and the data have been compared with semi-microscopic and microscopic-macroscopic models. The new microscopic database has been tested against aggregate total delayed neutron yields, time-dependent group parameters in 6-and 8-group re-presentation, and aggregate delayed neutron spectra. New recommendations of macroscopic delayed-neutron data for fissile materials of interest to applications are also presented. The new Reference Database for Beta-Delayed Neutron Emission Data is available online at: http://www-nds.iaea.org/beta-delayed-neutron/database.html., Comment: 96 pages, IAEA CRP report, preliminary version

The absolute differential cross sections for small-angle proton elastic scattering off the nuclei $^{12,14-17}$C have been measured in inverse kinematics at energies near 700 MeV/u at GSI Darmstadt. The hydrogen-filled ionization chamber IKAR served simultaneously as a gas target and a detector for the recoil protons. The projectile scattering angles were measured with multi-wire tracking detectors. The radial nuclear matter density distributions and the root-mean-square nuclear matter radii were deduced from the measured cross sections using the Glauber multiple-scattering theory. A possible neutron halo structure in $^{15}$C, $^{16}$C and $^{17}$C is discussed. The obtained data show evidence for a halo structure in the $^{15}$C nucleus.

A high-precision branching ratio measurement for the superallowed Fermi $\beta^{+}$ emitter $^{62}$Ga was performed with the Gamma-Ray Infrastructure for Fundamental Investigations of Nuclei (GRIFFIN) spectrometer at the Isotope Separator and Accelerator (ISAC) radioactive ion beam facility at TRIUMF. The high efficiency of the GRIFFIN spectrometer allowed 63 $\gamma$-ray transitions, with intensities down to $\approx$1 part per million (ppm) per $^{62}$Ga $\beta^{+}$ decay, to be placed in the level scheme of the daughter nucleus $^{62}$Zn, establishing the superallowed $\beta$ branching ratio for $^{62}$Ga decay to be 99.8577$^{+0.0023}_{-0.0029}\%$, a factor of 4 more precise than the previous world average. For several cascades, $\gamma-\gamma$ angular correlation measurements were performed to assign spins and/or determine the mixing ratios of transitions. In particular, the spin of the 2.342 MeV excited state in the daughter nucleus $^{62}$Zn was definitively assigned as $J = 0$. This assignment resolves a discrepancy between previous measurements and has important implications for the isospin symmetry breaking correction, $\delta_{C1}$, in $^{62}$Ga superallowed Fermi $\beta$ decay., Comment: A text label in Figure 12 has been corrected compared to the original submission

The $^{80}$Ge structure was investigated in a high-statistics $\beta$-decay experiment of $^{80}$Ga using the GRIFFIN spectrometer at TRIUMF-ISAC through $\gamma$, $\beta$-$e$, $e$-$\gamma$ and $\gamma$-$\gamma$ spectroscopy. No evidence was found for the recently reported 0$_2^{+}$ 639-keV level suggested as evidence for low-energy shape coexistence in $^{80}$Ge. Large-scale shell model calculations performed in $^{78,80,82}$Ge place the $0^{+}_{2}$ level in $^{80}$Ge at 2\,MeV. The new experimental evidence combined with shell model predictions indicate that low-energy shape coexistence is not present in $^{80}$Ge.

The evolution of the traditional nuclear magic numbers away from the valley of stability is an active field of research. Experimental efforts focus on providing key spectroscopic information that will shed light into the structure of exotic nuclei and understanding the driving mechanism behind the shell evolution. In this work, we investigate the Z = 6 spin-orbit shell gap towards the neutron dripline. To do so, we employed $^{A}$N(p,2p)$^{A-1}$C quasi-free scattering reactions to measure the proton component of the 2$^+_1$ state of $^{16,18,20}$C. The experimental findings support the notion of a moderate reduction of the proton 1p$_{1/2}$-1p$_{3/2}$ spin-orbit splitting, at variance to recent claims for a prevalent Z = 6 magic number towards the neutron dripline., Comment: 27 pages, 5 figures, 2 tables. Submitted to Physics Letter B

Excited states of $^{129}$In populated following the $\beta$-decay of $^{129}$Cd were experimentally studied with the GRIFFIN spectrometer at the ISAC facility of TRIUMF, Canada. A 480-MeV proton beam was impinged on a uranium carbide target and $^{129}$Cd was extracted using the Ion Guide Laser Ion Source (IG-LIS). $\beta$- and $\gamma$-rays following the decay of $^{129}$Cd were detected with the GRIFFIN spectrometer comprising the plastic scintillator SCEPTAR and 16 high-purity germanium (HPGe) clover-type detectors. %, along with the $\beta$-particles were detected with SCEPTAR. From the $\beta$-$\gamma$-$\gamma$ coincidence analysis, 32 new transitions and 7 new excited states were established, expanding the previously known level scheme of $^{129}$In. The $\log ft$ values deduced from the $\beta$-feeding intensities suggest that some of the high-lying states were populated by the $\nu 0 g_{7/2} \rightarrow \pi 0 g_{9/2}$ allowed Gamow-Teller (GT) transition, which indicates that the allowed GT transition is more dominant in the $^{129}$Cd decay than previously reported. Observation of fragmented Gamow-Teller strengths is consistent with theoretical calculations., Comment: 13 pages, 9 figures, to be published in Physical Review C

Ambient neutrons may cause significant background for underground experiments. Therefore, it is necessary to investigate their flux and energy spectrum in order to devise a proper shielding. Here, two sets of altogether ten moderated $^3$He neutron counters are used for a detailed study of the ambient neutron background in tunnel IV of the Felsenkeller facility, underground below 45 meters of rock in Dresden/Germany. One of the moderators is lined with lead and thus sensitive to neutrons of energies higher than 10 MeV. For each $^3$He counter-moderator assembly, the energy dependent neutron sensitivity was calculated with the FLUKA code. The count rates of the ten detectors were then fitted with the MAXED and GRAVEL packages. As a result, both the neutron energy spectrum from 10$^{-9}$ MeV to 300 MeV and the flux integrated over the same energy range were determined experimentally. The data show that at a given depth, both the flux and the spectrum vary significantly depending on local conditions. Energy integrated fluxes of $(0.61 \pm 0.05)$, $(1.96 \pm 0.15)$, and $(4.6 \pm 0.4) \times 10^{-4}$ cm$^{-2}$ s$^{-1}$, respectively, are measured for three sites within Felsenkeller tunnel IV which have similar muon flux but different shielding wall configurations. The integrated neutron flux data and the obtained spectra for the three sites are matched reasonably well by FLUKA Monte Carlo calculations that are based on the known muon flux and composition of the measurement room walls., Comment: 10 figures, 4 tables; to be published in Phys. Rev. D

Lifetimes of $2^+_1$ and $4^+_1$ states, as well as some negative-parity and non-yrast states, in $^{188-200}$Hg were measured using $\gamma-\gamma$ electronic fast timing techniques with the LaBr$_3$(Ce) detector array of the GRIFFIN spectrometer. The excited states were populated in the $\epsilon/\beta^+$-decay of $J^\pi =7^+/2^-$ $^{188-200}$Tl produced at the TRIUMF-ISAC facility. The deduced B(E2) values are compared to different interacting boson model predictions. The precision achieved in this work over previous ones allows for a meaningful comparison with the different theoretical models of these transitional Hg isotopes, which confirms the onset of state mixing in $^{190}$Hg.

An experiment addressing electron capture (EC) decay of hydrogen-like $^{142}$Pm$^{60+}$ ions has been conducted at the experimental storage ring (ESR) at GSI. The decay appears to be purely exponential and no modulations were observed. Decay times for about 9000 individual EC decays have been measured by applying the single-ion decay spectroscopy method. Both visually and automatically analysed data can be described by a single exponential decay with decay constants of 0.0126(7) s$^{-1}$ for automatic analysis and 0.0141(7) s$^{-1}$ for manual analysis. If a modulation superimposed on the exponential decay curve is assumed, the best fit gives a modulation amplitude of merely 0.019(15), which is compatible with zero and by 4.9 standard deviations smaller than in the original observation which had an amplitude of 0.23(4).

Absolute differential cross sections for elastic $p^7$Be and $p^8$B small-angle scattering were measured in inverse kinematics at an energy of 0.7 GeV/u at GSI Darmstadt. The hydrogen-filled ionization chamber IKAR was used as an active target to detect the recoil protons. The projectile tracking and isotope identification were performed with multi-wire proportional chambers and scintillation detectors. The measured cross sections were analysed using the Glauber multiple-scattering theory. The root-mean-square (rms) nuclear matter radii $R_{\rm m} = 2.42 (4)$ fm for $^7$Be and $R_{\rm m} = 2.58 (6)$ fm for $^8$B were obtained. The radial density distribution deduced for $^8$B exhibits a proton halo structure with the rms halo radius $R_{\rm h} = 4.24 (25)$ fm. A comparison of the deduced experimental radii is displayed with existing experimental and theoretical data., Comment: 18 pages, 6 figures. arXiv admin note: text overlap with arXiv:1803.02044

The half-lives of three $\beta$ decaying states of $^{131}_{~49}$In$_{82}$ have been measured with the GRIFFIN $\gamma$-ray spectrometer at the TRIUMF-ISAC facility to be $T_{1/2}(1/2^-)=328(15)$~ms, $T_{1/2}(9/2^+)=265(8)$~ms, and $T_{1/2}(21/2^+)=323(55)$~ms, respectively. The first observation of $\gamma$-rays following the $\beta n$ decay of $^{131}$In into $^{130}$Sn is reported. The $\beta$-delayed neutron emission probability is determined to be $P_{1n} = 12(7)\%$ for the $21/2^+$ state and $2.3(3)\%$ from the combined $1/2^-$ and $9/2^+$ states of $^{131}_{~49}$In$_{82}$ observed in this experiment. A significant expansion of the decay scheme of $^{131}$In, including 17 new excited states and 34 new $\gamma$-ray transitions in $^{131}_{~50}$Sn$_{81}$ is also reported. This leads to large changes in the deduced $\beta$ branching ratios to some of the low-lying states of $^{131}$Sn compared to previous work with implications for the strength of the first-forbidden $\beta$ transitions in the vicinity of doubly-magic $^{132}_{~50}$Sn$_{82}$., Comment: 14 pages, 15 figures, 5 tables

A thick neutron skin emerges from the first determination of root mean square radii of the proton distributions for $^{17-22}$N from charge changing cross section measurements around 900$A$ MeV at GSI. Neutron halo effects are signaled for $^{22}$N from an increase in the proton and matter radii. The radii suggest an unconventional shell gap at $N$ = 14 arising from the attractive proton-neutron tensor interaction, in good agreement with shell model calculations. $Ab$ $initio$, in-medium similarity re-normalization group, calculations with a state-of-the-art chiral nucleon-nucleon and three-nucleon interaction reproduce well the data approaching the neutron drip-line isotopes but are challenged in explaining the complete isotopic trend of the radii., Comment: 18 pages, 3 figures

We report mass measurements of neutron-rich Ga isotopes $^{80-85}$Ga with TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). The measurements determine the masses of $^{80-83}$Ga in good agreement with previous measurements. The masses of $^{84}$Ga and $^{85}$Ga were measured for the first time. Uncertainties between $25-48$ keV were reached. The new mass values reduce the nuclear uncertainties associated with the production of A $\approx$ 84 isotopes by the \emph{r}-process for astrophysical conditions that might be consistent with a binary neutron star (BNS) merger producing a blue kilonova. Our nucleosynthesis simulations confirm that BNS merger may contribute to the first abundance peak under moderate neutron-rich conditions with electron fractions $Y_e=0.35-0.38$.

The half-lives of isotopes around the $N=82$ shell closure are an important ingredient in astrophysical simulations and strongly influence the magnitude of the second $r$-process abundance peak in the $A\sim130$ region. The most neutron-rich $N=82$ nuclei are not accessible to the current generation of radioactive beam facilities and $r$-process simulations must therefore rely on calculations of the half-lives of the isotopes involved. Half-life measurements of the experimentally accessible nuclei in this region are important in order to benchmark these calculations. The half-life of $^{130}$Cd is particularly important as it is used to tune the Gamow-Teller quenching in shell-model calculations for the $\beta$ decay of other nuclei in this region. In this work, the GRIFFIN $\gamma$-ray spectrometer at the TRIUMF-ISAC facility was used to measure the half-life of $^{130}_{~48}$Cd$_{82}$ to be $T_{1/2}= 126(4)$ ms. In addition, the half-lives of the three $\beta$ decaying states of $^{131}_{~49}$In$_{82}$ were measured to be $T_{1/2}(1/2^-)=328(15)$ ms, $T_{1/2}(9/2^+)=265(8)$ ms, and $T_{1/2}(21/2^+)=323(50)$ ms, respectively, providing an important benchmark for half-life calculations in this region., Comment: Talk presented CIPANP2018. 9 pages, LaTeX, 5 pdf figures, 1 png figure

Gamma-Ray Infrastructure For Fundamental Investigations of Nuclei, GRIFFIN, is a new high-efficiency $\gamma$-ray spectrometer designed for use in decay spectroscopy experiments with low-energy radioactive ion beams provided by TRIUMF's Isotope Separator and Accelerator (ISAC-I) facility. GRIFFIN is composed of sixteen Compton-suppressed large-volume clover-type high-purity germanium (HPGe) $\gamma$-ray detectors combined with a suite of ancillary detection systems and coupled to a custom digital data acquisition system. The infrastructure and detectors of the spectrometer as well as the performance characteristics and the analysis techniques applied to the experimental data are described.

A new detection system has been installed at the RIKEN Nishina Center (Japan) to investigate decay properties of very neutron-rich nuclei. The setup consists of three main parts: a moderated neutron counter, a detection system sensitive to the implantation and decay of radioactive ions, and gamma-ray detectors. We describe here the setup, the commissioning experiment and some selected results demonstrating its performance for the measurement of half-lives and beta-delayed neutron emission probabilities. The methodology followed in the analysis of the data is described in detail. Particular emphasis is placed on the correction of the accidental neutron background.

This is an exciting time for the study of r-process nucleosynthesis. Recently, a neutron star merger GW170817 was observed in extraordinary detail with gravitational waves and electromagnetic radiation from radio to gamma rays. The very red color of the associated kilonova suggests that neutron star mergers are an important r-process site. Astrophysical simulations of neutron star mergers and core collapse supernovae are making rapid progress. Detection of both, electron neutrinos and antineutrinos from the next galactic supernova will constrain the composition of neutrino-driven winds and provide unique nucleosynthesis information. Finally FRIB and other rare-isotope beam facilities will soon have dramatic new capabilities to synthesize many neutron-rich nuclei that are involved in the r-process. The new capabilities can significantly improve our understanding of the r-process and likely resolve one of the main outstanding problems in classical nuclear astrophysics. However, to make best use of the new experimental capabilities and to fully interpret the results, a great deal of infrastructure is needed in many related areas of astrophysics, astronomy, and nuclear theory. We will place these experiments in context by discussing astrophysical simulations and observations of r-process sites, observations of stellar abundances, galactic chemical evolution, and nuclear theory for the structure and reactions of very neutron-rich nuclei. This review paper was initiated at a three-week International Collaborations in Nuclear Theory program in June 2016 where we explored promising r-process experiments and discussed their likely impact, and their astrophysical, astronomical, and nuclear theory context., Comment: 132 pages, 18 figures, submitted to Journal of Physics G

Background: $\beta$-delayed multiple neutron emission has been observed for some nuclei with A$\leq$100, with $^{100}$Rb being the heaviest $\beta$2n emitter measured to date. So far, only 25 P$_{2n}$ values have been determined for the $\sim$300 nuclei that may decay in this way. Accordingly, it is of interest to measure P$_{2n}$ values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such measurement for nuclei with A$>$100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition, the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the $r$-process, and safety inputs for nuclear reactors. Purpose: To determine for the first time the two neutron branching ratio, P$_{2n}$ value, for $^{136}$Sb through a direct neutron measurement, and to provide precise P$_{1n}$ values for $^{136}$Sb and $^{136}$Te. Method: Pure beams were provided by the JYFLTRAP at the IGISOL facility of the University of Jyv\"askyl\"a, Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point, and the BELEN detector, based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the $\beta$- and neutron- growth-and-decay curves and the $\beta$-one-neutron and $\beta$-two-neutron time correlations. Results: The P$_{2n}$ value of $^{136}$Sb was found to be 0.14(3)\% and the measured P$_{1n}$ values for $^{136}$Sb and $^{136}$Te were found to be 32.2(15)\% and 1.47(6)\%, respectively. The measured P$_{2n}$ value is a factor 44 smaller than predicted by the FRDM+QRPA model used for $r$-process calculations., Comment: 11 pages, 10 figures

The emission of neutron pairs from the neutron-rich $N\!=\!12$ isotones $^{18}$C and $^{20}$O has been studied by high-energy nucleon knockout from $^{19}$N and $^{21}$O secondary beams, populating unbound states of the two isotones up to 15~MeV above their two-neutron emission thresholds. The analysis of triple fragment-$n$-$n$ correlations shows that the decay $^{19}$N$(-1p)^{18}$C$^*\!\rightarrow^{16}$C+$n$+$n$ is clearly dominated by direct pair emission. The two-neutron correlation strength, the largest ever observed, suggests the predominance of a $^{14}$C core surrounded by four valence neutrons arranged in strongly correlated pairs. On the other hand, a significant competition of a sequential branch is found in the decay $^{21}$O$(-1n)^{20}$O$^*\!\rightarrow^{18}$O+$n$+$n$, attributed to its formation through the knockout of a deeply-bound neutron that breaks the $^{16}$O core and reduces the number of pairs., Comment: 6 pages, 4 figures, accepted for publication in Phys. Rev. Lett

The absolute differential cross section for small-angle proton elastic scattering on the proton-rich $^8$B nucleus has been measured in inverse kinematics for the first time. The experiment was performed using a secondary radioactive beam with an energy of 0.7 GeV/u at GSI, Darmstadt. The active target, namely hydrogen-filled time projection ionization chamber IKAR, was used to measure the energy, angle and vertex point of the recoil protons. The scattering angle of the projectiles was simultaneously determined by the tracking detectors. The measured differential cross section is analyzed on the basis of the Glauber multiple scattering theory using phenomenological nuclear-density distributions with two free parameters. The radial density distribution deduced for $^8$B exhibits a halo structure with the root-mean-square (rms) matter radius $R_{\rm m} = 2.58 (6)$ fm and the rms halo radius $R_{\rm h} = 4.24 (25)$ fm. The results on $^8$B are compared to those on the mirror nucleus $^8$Li investigated earlier by the same method. A comparison is also made with previous experimental results and theoretical predictions for both nuclei.

A precision mass investigation of the neutron-rich titanium isotopes $^{51-55}$Ti was performed at TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). The range of the measurements covers the $N=32$ shell closure and the overall uncertainties of the $^{52-55}$Ti mass values were significantly reduced. Our results confirm the existence of a weak shell effect at $N=32$, establishing the abrupt onset of this shell closure. Our data were compared with state-of-the-art \textit{ab-initio} shell model calculations which, despite very successfully describing where the $N=32$ shell gap is strong, overpredict its strength and extent in titanium and heavier isotones. These measurements also represent the first scientific results of TITAN using the newly commissioned Multiple-Reflection Time-of-Flight Mass Spectrometer (MR-TOF-MS), substantiated by independent measurements from TITAN's Penning trap mass spectrometer.

Background: Odd-odd nuclei, around doubly closed shells, have been extensively used to study proton-neutron interactions. However, the evolution of these interactions as a function of the binding energy, ultimately when nuclei become unbound, is poorly known. The $^{26}$F nucleus, composed of a deeply bound $\pi0d\_{5/2}$ proton and an unbound $\nu0d\_{3/2}$ neutron on top of an $^{24}$O core, is particularly adapted for this purpose. The coupling of this proton and neutron results in a $J^{\pi} = 1^{+}\_1 - 4^{+}\_1$ multiplet, whose energies must be determined to study the influence of the proximity of the continuum on the corresponding proton-neutron interaction. The $J^{\pi} = 1^{+}\_1, 2^{+}\_1,4^{+}\_1$ bound states have been determined, and only a clear identification of the $J^{\pi} =3^{+}\_1$ is missing.Purpose: We wish to complete the study of the $J^{\pi} = 1^{+}\_1 - 4^{+}\_1$ multiplet in $^{26}$F, by studying the energy and width of the $J^{\pi} =3^{+}\_1$ unbound state. The method was firstly validated by the study of unbound states in $^{25}$F, for which resonances were already observed in a previous experiment.Method: Radioactive beams of $^{26}$Ne and $^{27}$Ne, produced at about $440A$\,MeV by the FRagment Separator at the GSI facility, were used to populate unbound states in $^{25}$F and $^{26}$F via one-proton knockout reactions on a CH$\_2$ target, located at the object focal point of the R$^3$B/LAND setup. The detection of emitted $\gamma$-rays and neutrons, added to the reconstruction of the momentum vector of the $A-1$ nuclei, allowed the determination of the energy of three unbound states in $^{25}$F and two in $^{26}$F. Results: Based on its width and decay properties, the first unbound state in $^{25}$F is proposed to be a $J^{\pi} = 1/2^-$ arising from a $p\_{1/2}$ proton-hole state. In $^{26}$F, the first resonance at 323(33)~keV is proposed to be the $J^{\pi} =3^{+}\_1$ member of the $J^{\pi} = 1^{+}\_1 - 4^{+}\_1$ multiplet. Energies of observed states in $^{25,26}$F have been compared to calculations using the independent-particle shell model, a phenomenological shell-model, and the ab initio valence-space in-medium similarity renormalization group method.Conclusions: The deduced effective proton-neutron interaction is weakened by about 30-40\% in comparison to the models, pointing to the need of implementing the role of the continuum in theoretical descriptions, or to a wrong determination of the atomic mass of $^{26}$F., Comment: 14 pages, 7 figures, 3 tables, submitted to PRC

We present the results of precision mass measurements of neutron-rich cadmium isotopes. These nuclei approach the $N=82$ closed neutron shell and are important to nuclear structure as they lie near doubly-magic $^{132}$Sn on the chart of nuclides. Of particular note is the clear identification of the ground state mass in $^{127}$Cd along with the isomeric state. We show that the ground state identified in a previous mass measurement which dominates the mass value in the Atomic Mass Evaluation is an isomeric state. In addition to $^{127/m}$Cd, we present other cadmium masses measured ($^{125/m}$Cd and $^{126}$Cd) in a recent TITAN experiment at TRIUMF. Finally, we compare our measurements to new \emph{ab initio} shell-model calculations and comment on the state of the field in the $N=82$ region., Comment: 8 Pages with citations, 3 Figures, 2 Tables

$Background:$ Previous measurements of $\beta$-delayed neutron emitters comprise around 230 nuclei, spanning from the $^{8}$He up to $^{150}$La. Apart from $^{210}$Tl, with a minuscule branching ratio of 0.007\%, no other neutron emitter is measured yet beyond $A=150$. Therefore new data are needed, particularly in the heavy mass region around N=126, in order to guide theoretical models and to understand the formation of the third r-process peak at $A\sim195$. $Purpose:$ To measure both, $\beta$-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb and Bi isotopes beyond $N=126$. $Method:$ Ions of interest are produced by fragmentation of a $^{238}$U beam, selected and identified via the GSI-FRS fragment separator. A stack of segmented silicon detectors (SIMBA) is used to measure ion-implants and $\beta$-decays. An array of 30 $^3$He tubes embedded in a polyethylene matrix (BELEN) is used to detect neutrons with high efficiency and selectivity. A self-triggered digital system is employed to acquire data and to enable time-correlations. The latter are analyzed with an analytical model and results for the half-lives and neutron-branching ratios are derived using the binned Maximum-Likelihood method. $Results:$ Twenty new $\beta$-decay half-lives are reported for $^{204-206}$Au, $^{208-211}$Hg,$^{211-216}$Tl,$^{215-218}$Pb and $^{218-220}$Bi, nine of them for the first time. Neutron emission probabilities are reported for $^{210,211}$Hg and $^{211-216}$Tl. $Conclusions:$ The new $\beta$-decay half-lives are in good agreement with previous measurements in this region. The measured neutron emission probabilities are comparable or smaller than values predicted by global models like RHB+RQRPA., Comment: 17 pages, 21 figures, will be submitted at PRC

Several modes of electroweak radioactive decay require an interaction between the nucleus and bound electrons within the constituent atom. Thus, the probabilities of the respective decays are not only influenced by the structure of the initial and final states in the nucleus, but can also depend strongly on the atomic charge. Conditions suitable for the partial or complete ionization of these rare isotopes occur naturally in hot, dense astrophysical environments, but can also be artificially generated in the laboratory to selectively block certain radioactive decay modes. Direct experimental studies on such scenarios are extremely difficult due to the laboratory conditions required to generate and store radioactive ions at high charge states. A new electron-beam ion trap (EBIT) decay setup with the TITAN experiment at TRIUMF has successfully demonstrated such techniques for performing spectroscopy on the radioactive decay of highly charged ions., Comment: Invited article for "Atoms" special issue on "Perspectives of Atomic Physics Using Highly Charged Ions"

Proton radii of $^{12-19}$C densities derived from first accurate charge changing cross section measurements at 900$A$ MeV with a carbon target are reported. A thick neutron surface evolves from $\sim$ 0.5 fm in $^{15}$C to $\sim$ 1 fm in $^{19}$C. The halo radius in $^{19}$C is found to be 6.4$\pm$0.7 fm as large as $^{11}$Li. Ab initio calculations based on chiral nucleon-nucleon and three-nucleon forces reproduce well the radii., Comment: 5 pages, 4 figures, accepted for publication in Phys. Rev. Lett