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Integrated quantum light source is increasingly desirable in large-scale quantum information processing.~Despite recent remarkable advances, new material platform is constantly being explored for the fully on-chip integration of quantum light generation, active and passive manipulation, and detection. Here, for the first time, we demonstrate a gallium nitride (GaN) microring based quantum light generation in the telecom C-band, which has potential towards the monolithic integration of quantum light source.~In our demonstration, the GaN microring has a free spectral range of 330 GHz and a near-zero anomalous dispersion region of over 100 nm. The generation of energy-time entangled photon pair is demonstrated with a typical raw two-photon interference visibility of 95.5$\pm$6.5%, which is further configured to generate heralded single photon with a typical heralded second-order auto-correlation $g^{(2)}_{H}(0)$ of 0.045$\pm$0.001. Our results pave the way for developing chip-scale quantum photonic circuit.

The coexistence of quantum and classical light in the same fiber link is extremely desired in developing quantum communication. It has been implemented for different quantum information tasks, such as classical light coexisting with polarization-entangled photons at telecom O-band, and with quantum signal based quantum key distribution (QKD). In this work, we demonstrate the coexistence of energy-time entanglement based QKD and fiber optical communication at the telecom C-band. The property of noise from the classical channel is characterized with classical light at different wavelengths. With the largest noise, i.e., the worst case, the properties of energy-time entanglement are measured at different fiber optical communication rates. By measuring the two-photon interference of energy-time entanglement, our results show that a visibility of 82.01$\pm$1.10\% is achieved with a bidirectional 20 Gbps fiber optical communication over 40 km. Furthermore, by performing the BBM92 protocol for QKD, a secret key rate of 245 bits per second could be generated with a quantum bit error rate of 8.88\% with the coexisted energy-time entanglement.~Our demonstration paves the way for developing the infrastructure for quantum networks compatible with fiber optical communication., Comment: 6 pages, 3 figures

Multi-wavelength quantum light sources, especially at telecom band, are extremely desired in quantum information technology. Despite recent impressive advances, such a quantum light source with high quality remains challenging. Here we demonstrate a multi-wavelength quantum light source using a silicon nitride micro-ring with a free spectral range of 200 GHz. The generation of eight pairs of correlated photons is ensured in a wavelength range of 25.6 nm. With device optimization and noise-rejecting filters, our source enables the generation of heralded single-photons - at a rate of 62 kHz with $g^{(2)}_{h}(0)=0.014\pm0.001$, and the generation of energy-time entangled photons - with a visibility of $99.39\pm 0.45\%$ in the Franson interferometer. These results, at room temperature and telecom wavelength, in a CMOS compatible platform, represent an important step towards integrated quantum light devices for the quantum networks., Comment: 7 pages, 4 figures

To advance the full potential of quantum networks one should be able to distribute quantum resources over long distances at appreciable rates. As a consequence, all components in the networks need to have large multimode capacity to manipulate photonic quantum states. Towards this end, a multimode photonic quantum memory, especially one operating at telecom wavelength, remains a key challenge. Here we demonstrate a spectro-temporally multiplexed quantum memory at 1532 nm. Multimode quantum storage of telecom-band heralded single photons is realized by employing the atomic frequency comb protocol in a 10-m-long cryogenically cooled erbium doped silica fibre. The multiplexing encompasses five spectral channels - each 10 GHz wide - and in each of these up to 330 temporal modes, resulting in the simultaneous storage of 1650 modes of single photons. Our demonstrations open doors for high-rate quantum networks, which are essential for future quantum internet.

Quantum networks play an extremely important role in quantum information science, with application to quantum communication, computation, metrology and fundamental tests. One of the key challenges for implementing a quantum network is to distribute entangled flying qubits to spatially separated nodes, at which quantum interfaces or transducers map the entanglement onto stationary qubits. The stationary qubits at the separated nodes constitute quantum memories realized in matter while the flying qubits constitute quantum channels realized in photons. Dedicated efforts around the world for more than twenty years have resulted in both major theoretical and experimental progress towards entangling quantum nodes and ultimately building a global quantum network. Here, we review the development of quantum networks and the experimental progress over the past two decades leading to the current state of the art for generating entanglement of quantum nodes based on various physical systems such as single atoms, cold atomic ensembles, trapped ions, diamonds with Nitrogen-Vacancy centers, solid-state host doped with rare-earth ions, etc. Along the way we discuss the merits and compare the potential of each of these systems towards realizing a quantum network., Comment: 71 pages, 16 figures, 1 table, accepted by Laser & Photonics Reviews

NOON state interference (NOON-SI) is a powerful tool to improve the phase sensing precision, and plays an important role in quantum measurement. In most of the previous NOON-SI experiments, the measurements were performed in time domain where the spectral information of the involved photons was integrated and lost during the measurement. In this work, we experimentally measured the joint spectral intensities (JSIs) at different positions of the interference patterns in both time and frequency domains. It was observed that the JSIs were phase-dependent and show odd (even)-number patterns at $0$ ($\pi$) phase shift; while no interference appeared in time domain measurement, the interference pattern clearly appeared in frequency domain. To our best knowledge, the latter is the first observation of the spectrally resolved NOON state interference, which provides alternative information that cannot be extracted from the time-domain measurement. To explore its potential applications, we considered the interferometric sensing with our setup. From the Fisher information-based analysis, we show that the spectrally resolved NOON-SI has a better performance at non-zero-delay position than its non-spectrally resolved counterpart. The spectrally resolved NOON-SI scheme may be useful for quantum metrology applications such as quantum phase sensing, quantum spectroscopy, and remote synchronization.

We theoretically investigate the preparation of mid-infrared (MIR) spectrally-uncorrelated biphotons from a spontaneous parametric down-conversion process using doped LN crystals, including MgO doped LN, ZnO doped LN, and In2O3 doped ZnLN with doping ratio from 0 to 7 mol%. The tilt angle of the phase-matching function and the corresponding poling period are calculated under type-II, type-I, and type-0 phase-matching conditions. We also calculate the thermal properties of the doped LN crystals and their performance in Hong-Ou-Mandel interference. It is found that the doping ratio has a substantial impact on the group-velocity-matching (GVM) wavelengths. Especially, the GVM2 wavelength of co-doped InZnLN crystal has a tunable range of 678.7 nm, which is much broader than the tunable range of less than 100 nm achieved by the conventional method of adjusting the temperature. It can be concluded that the doping ratio can be utilized as a degree of freedom to manipulate the biphoton state. The spectrally uncorrelated biphotons can be used to prepare pure single-photon source and entangled photon source, which may have promising applications for quantum-enhanced sensing, imaging, and communications at the MIR range., Comment: 11 pages, 9 figures

We theoretically study the non-equilibrium correlations and entanglement between distant semiconductor qubits in a one-dimensional coupled-mechanical-resonator chain. Each qubit is defined by a double quantum dot (DQD) and embedded in a mechanical resonator. The two qubits can be coupled, correlated and entangled through phonon transfer along the resonator chain. We calculate the non-equilibrium correlations and steady-state entanglement at different phonon-phonon coupling rates, and find a maximal steady entanglement induced by a population inversion. The results suggest that highly tunable correlations and entanglement can be generated by phonon-qubit hybrid system, which will contribute to the development of mesoscopic physics and solid-state quantum computation.

With propagating through a dispersive medium, the temporal-spectral profile of laser pulses should be inevitably modified. Although such dispersion effect has been well studied in classical optics, its effect on a single-photon wave-packet, i.e., the matter wave of a single-photon, has not yet been entirely revealed. In this paper, we investigate the effect of dispersion on indistinguishability of single-photon wave-packets through the Hong-Ou-Mandel (HOM) interference. By dispersively manipulating two indistinguishable single-photon wave-packets before interfering with each other, we observe that the difference of the second-order dispersion between two optical paths of the HOM interferometer can be mapped to the interference curve, indicating that (1) with the same amount of dispersion effect in both paths, the HOM interference curve must be only determined by the intrinsic indistinguishability between the wave-packets, i.e., dispersion cancellation due to the indistinguishability between Feynman paths; (2) unbalanced dispersion effect in two paths cannot be cancelled and will broaden the interference curve thus providing a way to measure the second-order dispersion coefficient. Our results suggest a more comprehensive understanding of the single-photon wave-packet and pave ways to explore further applications of the HOM interference.

Spectrally intrinsically uncorrelated biphoton states generated from nonlinear crystals are very important but rare resources for quantum photonics and quantum information applications. Previously, such biphoton states were generated from several kinds of crystals, however, their wavelength ranges and nonlinear efficiencies were still limited for various applications. In order to explore new crystal for wider wavelength range and higher nonlinear efficiency, here we theoretically study the generation of spectrally uncorrelated biphoton states from 14 crystals in the `BBO family', including BBO, CLBO, KABO, KBBF, RBBF, CBBF, BABF, BiBO, LBO, CBO, LRB4, LCB, YCOB, and GdCOB. They satisfy three kinds of group-velocity matching condition from near-infrared to telecom wavelengths. Furthermore, heralded single photons can be generated with a purity as high as 0.98, which is achieved without any narrow filtering. The indistinguishability of photons from independent sources is examined by the Hong-Ou-Mandel interference, which results in a visibility of 98% also without any further filtering, i.e., photons from different heralded single-photon sources are highly indistinguishable. Our study may provide single-photon sources with good performance for quantum information processing at near-infrared and telecom wavelengths., Comment: 10 pages, 6 figures

Vibrational modes in mechanical resonators provide a promising candidate to interface and manipulate classical and quantum information. The observation of coherent dynamics between distant mechanical resonators can be a key step towards scalable phonon-based applications. Here we report tunable coherent phonon dynamics with an architecture comprising three graphene mechanical resonators coupled in series, where all resonators can be manipulated by electrical signals on control gates. We demonstrate coherent Rabi oscillations between spatially separated resonators indirectly coupled via an intermediate resonator serving as a phonon cavity. The Rabi frequency fits well with the microwave burst power on the control gate. We also observe Ramsey interference, where the oscillation frequency corresponds to the indirect coupling strength between these resonators. Such coherent processes indicate that information encoded in vibrational modes can be transferred and stored between spatially separated resonators, which can open the venue of on-demand phonon-based information processing.

Mechanical resonators are promising systems for storing and manipulating information. To transfer information between mechanical modes, either direct coupling or an interface between these modes is needed. In previous works, strong coupling between different modes in a single mechanical resonator and direct interaction between neighboring mechanical resonators have been demonstrated. However, coupling between distant mechanical resonators, which is a crucial request for long-distance classical and quantum information processing using mechanical devices, remains an experimental challenge. Here, we report the experimental observation of strong indirect coupling between separated mechanical resonators in a graphene-based electromechanical system. The coupling is mediated by a far-off-resonant phonon cavity through virtual excitations via a Raman-like process. By controlling the resonant frequency of the phonon cavity, the indirect coupling can be tuned in a wide range. Our results may lead to the development of gate-controlled all-mechanical devices and open up the possibility of long-distance quantum mechanical experiments.

Quantum confinement has made it possible to detect and manipulate single-electron charge and spin states. The recent focus on two-dimensional (2D) materials has attracted significant interests on possible applications to quantum devices, including detecting and manipulating either single-electron charging behavior or spin and valley degrees of freedom. However, the most popular model systems, consisting of tunable double-quantum-dot molecules, are still extremely difficult to realize in these materials. We show that an artificial molecule can be reversibly formed in atomically thin MoS2 sandwiched in hexagonal boron nitride, with each artificial atom controlled separately by electrostatic gating. The extracted values for coupling energies at different regimes indicate a single-electron transport behavior, with the coupling strength between the quantum dots tuned monotonically. Moreover, in the low-density regime, we observe a decrease of the conductance with magnetic field, suggesting the observation of Coulomb blockade weak anti-localization. Our experiments demonstrate for the first time the realization of an artificial quantum-dot molecule in a gated MoS2 van der Waals heterostructure, which could be used to investigate spin-valley physics. The compatibility with large-scale production, gate controllability, electron-hole bipolarity, and new quantum degrees of freedom in the family of 2D materials opens new possibilities for quantum electronics and its applications.

Graphene-based electromechanical resonators have attracted much interest recently because of the outstanding mechanical and electrical properties of graphene and their various applications. However, the coupling between mechanical motion and charge transport has not been explored in graphene. Here, we studied the mechanical properties of a suspended 50-nm-wide graphene nanoribbon, which also acts as a single-electron transistor (SET) at low temperature. Using the SET as a sensitive detector, we found that the resonance frequency could be tuned from 82 MHz to 100 MHz and the quality factor exceeded 30000. The strong charge-mechanical coupling was demonstrated by observing the SET induced ~140 kHz resonance frequency shifts and mechanical damping. We also found that the SET can enhance the nonlinearity of the resonator. Our SET-coupled graphene mechanical resonator could approach an ultra-sensitive mass resolution of ~0.55*10^(-21) g and a force sensitivity of ~1.9*10^(-19) N/(Hz)^(1/2), and can be further improved. These properties indicate that our device is a good platform both for fundamental physical studies and potential applications.

Phonon-cavity electromechanics allows the manipulation of mechanical oscillations similar to photon-cavity systems. Many advances on this subject have been achieved in various materials. In addition, the coherent phonon transfer (phonon Rabi oscillations) between the phonon cavity mode and another oscillation mode has attracted many interest in nano-science. Here we demonstrate coherent phonon transfer in a carbon nanotube phonon-cavity system with two mechanical modes exhibiting strong dynamical coupling. The gate-tunable phonon oscillation modes are manipulated and detected by extending the red-detuned pump idea of photonic cavity electromechanics. The first- and second-order coherent phonon transfers are observed with Rabi frequencies 591 kHz and 125 kHz, respectively. The frequency quality factor product fQ_m~2=10^12 Hz achieved here is larger thank k_B T_base/h, which may enable the future realization of Rabi oscillations in the quantum regime.

Recently, transition metal dichalcogenides (TMDCs) semiconductors have been utilized for investigating quantum phenomena because of their unique band structures and novel electronic properties. In a quantum dot (QD), electrons are confined in all lateral dimensions, offering the possibility for detailed investigation and controlled manipulation of individual quantum systems. Beyond the definition of graphene QDs by opening an energy gap in nanoconstrictions, with the presence of a bandgap, gate-defined QDs can be achieved on TMDCs semiconductors. In this paper, we review the confinement and transport of QDs in TMDCs nanostructures. The fabrication techniques for demonstrating two-dimensional (2D) materials nanostructures such as field-effect transistors and QDs, mainly based on e-beam lithography and transfer assembly techniques are discussed. Subsequently, we focus on transport through TMDCs nanostructures and QDs. With steady improvement in nanoscale materials characterization and using graphene as a springboard, 2D materials offer a platform that allows creation of heterostructure QDs integrated with a variety of crystals, each of which has entirely unique physical properties., Comment: Submitted to Frontiers of Physics as a review

Carbon nanotubes (CNTs) have attracted much attention for use in nanomechanical devices because of their exceptional properties, such as large resonant frequencies, low mass, and high quality factors. Here, we report the first experimental realization of parametric strong coupling between two mechanical modes on a single CNT nanomechanical resonator, by applying an extra microwave pump. This parametric pump method can be used to couple mechanical modes with arbitrary frequency differences. The properties of the mechanical resonator are detected by single-electron tunneling at low temperature, which is found to be strongly coupled to both modes. The coupling strength between the two modes can be tuned by the pump power, setting the coupling regime from weak to strong. This tunability may be useful in further phonon manipulations in carbon nanotubes.

Coupling an electromechanical resonator with carbon-nanotube quantum dots is a significant method to control both the electronic charge and the spin quantum states. By exploiting a novel micro-transfer technique, we fabricate two strongly-coupled and electrically-tunable mechanical resonators on a single carbon nanotube for the first time. The frequency of the two resonators can be individually tuned by the bottom gates, and strong coupling is observed between the electron charge and phonon modes of each resonator. Furthermore, the conductance of either resonator can be nonlocally modulated by the phonon modes in the other resonator. Strong coupling is observed between the phonon modes of the two resonators, which provides an effective long distance electron-electron interaction. The generation of phonon-mediated-spin entanglement is also theoretically analyzed for the two resonators. This strongly-coupled nanotube electromechanical resonator array provides an experimental platform for future studies of the coherent electron-phonon interaction, the phonon mediated long-distance electron interaction, and entanglement state generation.

Mesoscopic systems constitute appealing platforms to study many-body physics with light and matter degrees of freedom. The Kondo effect refers to the screening of a spin-1/2 impurity by a cloud of conduction electrons, then forming a many-body Fermi liquid ground state. The Kondo resonance produces a phase shift in the transmitted electronic wave packet which depends on the symmetry and nature of the many-body ground state. Theoretical calculations suggest that the Kondo resonance can interact with the irradiation photon field and should give rise to a {\pi}-phase shift of the photon signal in the case where the ground state is a Fermi liquid. This {\pi}-phase shift of microwave photon is driven from the Korringa-Shiba relation of quantum impurity Fermi-liquid ground states. We report the first observation of such a {\pi}-phase shift in a graphene double quantum dot within a circuit quantum electrodynamics architecture where the microwave photons couple to the pseudo-spin or charge degrees of freedom. The observed Kondo temperature TK ~ 550 mK is in agreement with DC conductance measurements. All our results support the formation of a Kondo resonance located above the Fermi level of the electronic reservoirs and the occurrence of an SU(4) Fermi-liquid ground state. We finally study how the Kondo-photon interactions can be tuned by inter-dot electron tunnel coupling strengths. Our experimental achievements may contribute to a better understanding of many-body physics in hybrid circuit systems, and open up new applications in atomic thin materials from the light-matter interaction.

We report a technique that can noninvasively add multiple DC wires into a 3D superconducting microwave cavity for electronic devices that require DC electrical terminals. We studied the influence of our DC lines on the cavity performance systematically. We found that the quality factor of the cavity is reduced if any of the components of the electrical wires cross the cavity equipotential planes. Using this technique, we were able to incorporate a quantum dot (QD) device into a 3D cavity. We then controlled and measured the QD transport signal using the DC lines. We have also studied the heating effects of the QD by the microwave photons in the cavity.

With recent advances in the circuit quantum electrodynamics (cQED) architecture, hybrid systems that couple nano-devices to microwave resonators have been developing rapidly. Here we report an experimental demonstration of two graphene double quantum dots (DQDs) coupled over a distance of up to 60 {\mu}m, through a microwave resonator. We jointly measure the two DQDs' coupling to the resonator, which causes a nonlinear response in the resonator reflection amplitude in the vicinity of the degeneracy points of the two DQDs. This phenomenon is explained by the Tavis-Cummings (T-C) mode. We further characterize this nonlocal coupling by measuring the correlation between the DC currents in the two DQDs. This correlation is observed to be strongly dependent on the average photon number in the resonator. Our results explore T-C physics in electronic transport, and also contribute to the study of nonlocal transport and future implementations of remote electronic entanglement.

We use an on-chip superconducting resonator as a sensitive meter to probe the properties of graphene double quantum dots at microwave frequencies. Specifically, we investigate the charge dephasing rates in a circuit quantum electrodynamics architecture. The dephasing rates strongly depend on the number of charges in the dots, and the variation has a period of four charges, over an extended range of charge numbers. Although the exact mechanism of this fourfold periodicity in dephasing rates is an open problem, our observations hint at the fourfold degeneracy expected in graphene from its spin and valley degrees of freedom.

We have designed and fabricated a half-wavelength reflection line resonator (RLR) that consists of a pair of two coupled microstrip lines on a GaAs/AlGaAs heterostructure. By changing the top gate voltage on a square of two dimensional electron gas under the resonator, a large range of the quality factors can be obtained. Energy loss in the two-dimensional electron gas can be minimized, thus realizing a versatile resonator suitable for integration with semiconductor quantum circuits., Comment: 9 pages, 3 figures

The novel concept of non-compensated n-p codoping has made it possible to create tunable intermediate bands in the intrinsic band gap of TiO2, making the codoped TiO2 a promising material for developing intermediate band solar cells (IBSCs). Here we investigate the quantum efficiency of such IBSCs within two scenarios - with and without current extracted from the extended intermediate band. Using the ideal equivalent circuit model, we find that the maximum efficiency of 57% in the first scenario and 53% in the second are both much higher than the Shockley-Queisser limit from single gap solar cells. We also obtain various key quantities of the circuits, a useful step in realistic development of TiO2 based solar cells invoking device integration. These equivalent circuit results are also compared with the efficiencies obtained directly from consideration of electron transition between the energy bands, and both approaches reveal the intriguing existence of double peaks in the maximum quantum efficiency as a function of the relative location of IBs., Comment: This paper has been withdrawn by the author due to a crucial sign error in the last description